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NASA NTRS2005

Overview of Aerosol Distribution

Our knowledge of atmospheric aerosols (smoke, pollution, dust or sea salt particles, small enough to be suspended in the air), their evolution, composition, variability in space and time and interaction with clouds and precipitation is still lacking despite decades of research. Understanding the global aerosol system is fundamental for progress in climate change and hydrological cycle research. While a single instrument was used to demonstrate 50 years ago that the global CO2 levels are rising, posing threat of global warming, we need an array of satellites and field measurements coupled with chemical transport models to understand the global aerosol system. This complexity of the aerosol problem results from their short lifetime (1 week) and variable chemical composition. A new generation of satellites provides exciting opportunities to measure the global distribution of aerosols, distinguishing natural from anthropogenic aerosol and measuring their interaction with clouds and climate. I shall discuss these topics and application of the data to air quality monitoring.

Kaufman, Yoram↗
NASA NTRS2002

Chemistry-Climate Interactions in the Goddard Institute for Space Studies General Circulation Model: New Insights into Modeling the Pre-Industrial Atmosphere - 2

We investigate the chemical (hydroxyl and ozone) and dynamical response to changing from present day to pre-industrial conditions in the Goddard Institute for Space Studies General Circulation Model (GISS GMC). We identify three main improvements not included by many other works. Firstly, our model includes interactive cloud calculations. Secondly we reduce sulfate aerosol which impacts NOx partitioning hence Ox distributions. Thirdly we reduce sea surface temperatures and increase ocean ice coverage which impact water vapor and ground albedo respectively. Changing the ocean data (hence water vapor and ozone) produces a potentially important feedback between the Hadley circulation and convective cloud cover. Our present day run (run 1, control run) global mean OH value was 9.8 x 10(exp 5) molecules/cc. For our best estimate of pre-industrial conditions run (run 2) which featured modified chemical emissions, sulfate aerosol and sea surface temperatures/ocean ice, this value changed to 10.2 x 10(exp 5) molecules/cc. Reducing only the chemical emissions to pre-industrial levels in run 1 (run 3) resulted in this value increasing to 10.6 x 10(exp 5) molecules/cc. Reducing the sulfate in run 3 to pre-industrial levels (run 4) resulted in a small increase in global mean OH (10.7 x 10(exp 5) molecules/cc). Changing the ocean data in run 4 to pre-industrial levels (run 5) led to a reduction in this value to 10.3 x 10(exp 5) molecules/cc. Mean tropospheric ozone burdens were 262, 181, 180, 180, and 182 Tg for runs 1-5 respectively.

Grenfell, J. Lee↗
NASA NTRS2008

Atmospheric Radiative Transfer for Satellite Remote Sensing

I will discuss the science of satellite remote sensing which involves the interpretation and inversion of radiometric measurements made from space. The goal of remote sensing is to retrieve some physical aspects of the medium which are sensitive to the radiation at specific wavelengths. This requires the use of fundamentals of atmospheric radiative transfer. I will talk about atmospheric radiation or, more specifically, about the interactions of solar radiation with aerosols and cloud particles. The focus will be more on cloudy atmospheres. I will also show how a standard one-dimensional approach, that is traced back at least 100 years, can fail to interpret the complexity of real clouds. I n these cases, three-dimensional radiative transfer should be used. Examples of satellite retrievals will illustrate the cases.

Marshak, Alexander↗
NASA NTRS2005

It's a Sooty Problem: Black Carbon and Aerosols from Space

Our knowledge of atmospheric aerosols (smoke, pollution, dust or sea salt particles, small enough to be suspended in the air), their evolution, composition, variability in space and time and interaction with solar radiation, clouds and precipitation is lacking despite decades of research. Just recently we recognized that understanding the global aerosol system is fundamental for progress in climate change and hydrological cycle research. While a single instrument was used to demonstrate 50 yrs ago that the global CO2 levels are rising, posing thread to our climate, we need an may of satellites, surface networks of radiometers, elaborated laboratory and field experiments coupled with chemical transport models to understand the global aerosol system. This complexity of the aerosol problem results from their short lifetime (1 week), variability of the chemical composition and complex chemical and physical processes in the atmosphere. The result is a heterogeneous distribution of aerosol and their properties. The new generation of satellites and surface networks of radiometers provides exciting opportunities to measure the aerosol properties and their interaction with clouds and climate. However farther development in the satellite capability, aerosol chemical models and climate models is needed to fully decipher the aerosol secrets with accuracy required to predict future climates.

Kaufman, Yoram J.↗
NASA NTRS2012

The Use of Satellite-Measured Aerosol Optical Depth to Constrain Biomass Burning Emissions Source Strength in a Global Model GOCART

Small particles in the atmosphere, called "atmospheric aerosol" have a direct effect on Earth climate through scattering and absorbing sunlight, and also an indirect effect by changing the properties of clouds, as they interact with solar radiation as well. Aerosol typically stays in the atmosphere for several days, and can be transported long distances, affecting air quality, visibility, and human health not only near the source, but also far downwind. Smoke from vegetation fires is one of the main sources of atmospheric aerosol; other sources include anthropogenic pollution, dust, and sea salt. Chemistry transport models (CTMs) are among the major tools for studying the atmospheric and climate effects of aerosol. Due to the considerable variation of aerosol concentrations and properties on many temporal and spatial scales, and the complexity of the processes involved, the uncertainties in aerosol effects on climate are large, as is featured in the latest report of Intergovernmental Panel on Climate Change (IPCC) in 2007. Reducing this uncertainty in the models is very important both for predicting future climate scenarios and for regional air quality forecasting and mitigation. During vegetation fires, also called biomass burning (BB) events, complex mixture of gases and particles is emitted. The amount of BB emissions is usually estimated taking into account the intensity and size of the fire and the properties of burning vegetation. These estimates are input into CTMs to simulate BB aerosol. Unfortunately, due to large variability of fire and vegetation properties, the quantity of BB emissions is very difficult to estimate and BB emission inventories provide numbers that can differ by up to the order of magnitude in some regions. Larger uncertainties in data input make uncertainties in model output larger as well. A powerful way to narrow the range of possible model estimates is to compare model output to observations. We use satellite observations of aerosol properties, specifically aerosol optical depth, which is directly proportional to the amount of aerosol in the atmosphere, and compare it to the model output. Assuming the model represents aerosol transport and particle properties correctly, the amount of BB emissions determines the simulated aerosol optical depth. In this study, we explore the regional performance of 13 commonly used emission estimates. These are each input to global Goddard Chemistry Aerosol Radiation and Transport (GOCART) model. We then evaluate how well each emission estimate reproduces the smoke aerosol optical depth measured by the MODIS instrument. We compared GOCART-simulate aerosol optical depth with that measured from the satellite for 124 fire cases around the world during 2006 and 2007. We summarize the regional performance of each emission inventory and discuss reasons for their differences by considering the assumptions made during their development. We also show that because stronger wind disperses smoke plumes more readily, in cases with stronger wind, a larger increase in emission amount is needed to increase aerosol optical depth. In quiet, low-wind-speed environments, BB emissions produce a more significant increase in aerosol optical depth, other things being equal. Using the region-specific, quantitative relationships derived in our paper, together with the wind speed obtained from another source for a given fire case, we can constrain the amount of emission required in the model to reproduce the observations. The results of this paper are useful to the developers of BB emission inventories, as they show the strengths and weaknesses of individual emission inventories in different regions of the globe, and also for modelers who use these inventories and wish to improve their model results.

Petrenko, Mariya↗
NASA NTRS2014

Current and Future Perspectives of Aerosol Research at NASA Goddard Space Flight Center

Aerosols are tiny atmospheric particles that are emitted from various natural and anthropogenic sources. They affect climate through direct and indirect interactions with solar and thermal radiation, clouds, and atmospheric circulation (Solomon et al. 2007). The launch of a variety of sophisticated satellite-based observing systems aboard the Terra, Aqua, Aura, SeaWiFS (see appendix for all acronym expansions), CALIPSO, and other satellites in the late 1990s to mid-2000s through the NASA EOS and other U.S. and non-U.S. programs ushered in a golden era in aerosol research. NASA has been a leader in providing global aerosol characterizations through observations from satellites, ground networks, and field campaigns, as well as from global and regional modeling. AeroCenter (http://aerocenter.gsfc.nasa.gov/), which was formed in 2002 to address the many facets of aerosol research in a collaborative manner, is an interdisciplinary union of researchers (~200 members) at NASA GSFC and other nearby institutions, including NOAA, several universities, and research laboratories. AeroCenter hosts a web-accessible regular seminar series and an annual meeting to present up-to-date aerosol research, including measurement techniques; remote sensing algorithms; modeling development; field campaigns; and aerosol interactions with radiation, clouds, precipitation, climate, biosphere, atmospheric chemistry, air quality, and human health. The 2013 annual meeting was held at the NASA GSFC Visitor Center on 31 May 2013, which coincided with the seventh anniversary of the passing of Yoram Kaufman, a modern pioneer in satellite-based aerosol science and the founder of AeroCenter. The central theme of this year's meeting was "current and future perspectives" of NASA's aerosol science and satellite missions.

aerocenter↗
NASA NTRS2010

Highlights from 40 Years of Satellite UV Measurements

This year we are celebrating the 40th anniversary of the launch of the Backscatter Ultraviolet (BUV) instrument on NASA's Nimbus-4 satellite. The purpose of this instrument was to demonstrate the capability to measure total column ozone and its vertical distribution from space. The success of this instrument led to about a dozen instruments of this type on various NASA and NOAA satellites. These instruments used a single photomultiplier tube (PMT) that restricted the measurements to 6-12 discrete wavelengths in the 250-380 nm range. With the availability of solid-state detector arrays in the past decade it has been possible to make similar measurements but with hyperspectral (contiguous in wavelength) sampling and enhanced spectral resolution. This has allowed global mapping of several weakly-absorbing trace gases including S0 2, NO2, BrO, HCHO, and CIIOCHO. Since these measurements are affected by clouds and aerosols, a great deal of effort has gone into understanding their effect on ultraviolet radiation- both upwelling and downwelling. The downwelling UV radiation is chemically and biologically active and has both negative (genetic damage, air pollution) and positive (production of vitamin D and OH radical) environmental effects. I will discuss how the interaction of Rayleigh-scattered UV radiation with clouds and aerosols produce a variety of interesting effects that are leading to new methods of remote sensing of their properties. The UV measurements can greatly enhance the information that one derives from more traditional methods that use infrared and visible part of the solar spectrum.

Bhartia, Pawan K.↗
NASA NTRS2012

Dispersion of the Volcanic Sulfate Cloud from the Mount Pinatubo Eruption

We simulate the transport of the volcanic cloud from the 1991 eruption of Mount Pinatubo with the GEOS-5 general circulation model. Our simulations are in good agreement with observational data. We tested the importance of initial condition corresponding to the specific meteorological situation at the time of the eruption by employing reanalysis from MERRA. We found no significant difference in the transport of the cloud. We show how the inclusion of the interaction between volcanic sulfate aerosol and radiation is essential for a reliable simulation of the transport of the volcanic cloud. The absorption of long wave radiation by the volcanic sulfate induces a rising of the volcanic cloud up to the middle stratosphere, combined with divergent motion from the latitude of the eruption to the tropics. Our simulations indicate that the cloud diffuses to the northern hemisphere through a lower stratospheric pathway, and to mid- and high latitudes of the southern hemisphere through a middle stratospheric pathway, centered at about 30 hPa. The direction of the middle stratospheric pathway depends on the season. We did not detect any significant change of the mixing between tropics and mid- and high latitudes in the southern hemisphere.

Aquila, Valentina↗
NASA NTRS2022

Aerosol Detection from the Cloud Aerosol Transport System on the International Space Station: Algorithm Overview and Implications for Diurnal Sampling

Concentrations of particulate aerosols and their vertical placement in the atmosphere determine their interaction with the Earth system and their impact on air quality. Space-based lidar, such as the Cloud–Aerosol Transport System (CATS) technology demonstration instrument, is well-suited for determining the vertical structure of these aerosols and their diurnal cycle. Through the implementation of aerosol-typing algorithms, vertical layers of aerosols are assigned a type, such as marine, dust, and smoke, and a corresponding extinction-to-backscatter (lidar) ratio. With updates to the previous aerosol-typing algorithms, we find that CATS, even as a technology demonstration, observed the documented seasonal cycle of aerosols, comparing favorably with the Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) space-based lidar and the NASA Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2) model reanalysis. By leveraging the unique orbit of the International Space Station, we find that CATS can additionally resolve the diurnal cycle of aerosol altitude as observed by ground-based instruments over the Maritime Continent of Southeast Asia.

Edward P Nowottnick↗
NASA NTRS2018

Radiative Heating Profiles over Ascension Island during the 2016 and 2017 Biomass Burning Seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between cloud morphology and the environmental conditions in which marine boundary layer clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean, where it is likely that the absorbing and heating properties of these aerosols modify the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to observe thermodynamic, cloud and aerosol properties during two consecutive biomass burning seasons from July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). These observations in conjunction with radiation transfer modeling were used to assess the impact of biomass burning carbonaceous aerosol plumes as they passed over the site.Thermodynamic profiles were generated using a combination of radiosonde data and thermodynamic profilers to provide high temporal resolution profiles of quantities that are important for cloud development, such as CAPE and CIN. Coincident Ka-band radar and lidar profiles were used to characterize the cloud and sub-cloud structure. The resulting thermodynamic and cloud profiles are used as input forcing for the Rapid Radiative Transfer Model (RRTM) to compute radiative heating profiles over the observation site. Idealized experiments using RRTM, with and without aerosols present, are used to assess the impacts of the absorbing aerosol on the heating rate profiles.

Cumulus↗
NASA NTRS2017

Integrative Analysis of Desert Dust Size and Abundance Suggests Less Dust Climate Cooling

Desert dust aerosols affect Earths global energy balance through interactions with radiation, clouds, and ecosystems. But the magnitudes of these effects are so uncertain that it remains unclear whether atmospheric dust has a net warming or cooling effect on global climate. Consequently, it is still uncertain whether large changes in atmospheric dust loading over the past century have slowed or accelerated anthropogenic climate change, and the climate impact of possible future alterations in dust loading is similarly disputed. Here we use an integrative analysis of dust aerosol sizes and abundance to constrain the climatic impact of dust through direct interactions with radiation. Using a combination of observational, experimental, and model data, we find that atmospheric dust is substantially coarser than represented in current climate models. Since coarse dust warms global climate, the dust direct radiative effect (DRE) is likely less cooling than the 0.4 W m superscript 2 estimated by models in a current ensemble. We constrain the dust DRE to -0.20 (-0.48 to +0.20) W m superscript 2, which suggests that the dust DRE produces only about half the cooling that current models estimate, and raises the possibility that dust DRE is actually net warming the planet.

Atmospheric chemistry↗
NASA NTRS2016

Multi-Sensor Cloud and Aerosol Retrieval Simulator and Remote Sensing from Model Parameters : Aerosols - Part 2

The Multi-sensor Cloud Retrieval Simulator (MCRS) produces a simulated radiance product from any high-resolution general circulation model with interactive aerosol as if a specific sensor such as the Moderate Resolution Imaging Spectroradiometer (MODIS) were viewing a combination of the atmospheric column and land ocean surface at a specific location. Previously the MCRS code only included contributions from atmosphere and clouds in its radiance calculations and did not incorporate properties of aerosols. In this paper we added a new aerosol properties module to the MCRS code that allows users to insert a mixture of up to 15 different aerosol species in any of 36 vertical layers. This new MCRS code is now known as MCARS (Multi-sensor Cloud and Aerosol Retrieval Simulator). Inclusion of an aerosol module into MCARS not only allows for extensive, tightly controlled testing of various aspects of satellite operational cloud and aerosol properties retrieval algorithms, but also provides a platform for comparing cloud and aerosol models against satellite measurements. This kind of two-way platform can improve the efficacy of model parameterizations of measured satellite radiances, allowing the assessment of model skill consistently with the retrieval algorithm. The MCARS code provides dynamic controls for appearance of cloud and aerosol layers. Thereby detailed quantitative studies of the impacts of various atmospheric components can be controlled. In this paper we illustrate the operation of MCARS by deriving simulated radiances from various data field output by the Goddard Earth Observing System version 5 (GEOS-5) model. The model aerosol fields are prepared for translation to simulated radiance using the same model sub grid variability parameterizations as are used for cloud and atmospheric properties profiles, namely the ICA technique. After MCARS computes modeled sensor radiances equivalent to their observed counterparts, these radiances are presented as input to operational remote-sensing algorithms. Specifically, the MCARS-computed radiances are input into the processing chain used to produce the MODIS Data Collection 6 aerosol product (MOYD04). TheMOYD04 product is of course normally produced from MOYD021KM MODIS Level-1B radiance product directly acquired by the MODIS instrument. MCARS matches the format and metadata of a MOYD021KM product. The resulting MCARS output can be directly provided to MODAPS (MODIS Adaptive Processing System) as input to various operational atmospheric retrieval algorithms. Thus the operational algorithms can be tested directly without needing to make any software changes to accommodate an alternative input source. We show direct application of this synthetic product in analysis of the performance of the MOD04 operational algorithm. We use biomass-burning case studies over Amazonia employed in a recent Working Group on Numerical Experimentation (WGNE)-sponsored study of aerosol impacts on numerical weather prediction (Freitas et al., 2015). We demonstrate that a known low bias in retrieved MODIS aerosol optical depth appears to be due to a disconnect between actual column relative humidity and the value assumed by the MODIS aerosol product.

aerosol retrieval↗
NASA NTRS2018

PACE Technical Report Series, Volume 4: Cloud Retrievals in the PACE Mission: PACE Science Team Consensus Document

Earth is a complex dynamical system exhibiting continuous change in its atmosphere, ocean,and surface elements. Nearly all (99.97%) of the energy driving these systems is linked to the Sun. Measurements of reflected sunlight contain a unique signature of wavelength-specific scattering and absorption interactions occurring between incoming solar energy and atmospheric (molecules, aerosols,clouds) and surface features Clouds can affect significantly both shortwave and long wave radiation, depending on altitude/vertical structure, thermodynamic phase, and optical properties. Low, warm, and optically thick clouds predominantly have a cooling effect, while high, cold, optically thin clouds can cause warming by absorbing warmer radiation emitted from the surface and lower atmosphere.When the net difference between outgoing and incoming solar radiation is matched by the net infrared radiation emitted to space, the Earth's climate is in radiative balance. While radiative forcing components (GHGs, aerosols - direct and indirect) contribute to a net radiative imbalance, climate sensitivity is ultimately determined by the contribution of various system feed backs. The role of cloud feedback in a warming climate is currently the largest inter-model uncertainty in climate sensitivity and therefore in climate prediction [Bony and Dufresne 2005]. A comprehensive understanding of current cloud propertiesand dynamic/microphysical processes requires a global perspective from satellites.

Plankton, Aerosol, Cloud, ocean Ecosystem (PACE)↗
NASA NTRSDate not supplied

TPSAS-NF1676L-10947-DND

There are large uncertainties in quantifying dust effects on the climate because of the limitations on the measurements and observations of dust-cloud-precipitation-dynamics interactions. As a major terrestrial source of atmospheric aerosols, dusts may serve as a significant climate forcing for the changing climate due to its effect on solar and thermal radiation as well as on clouds and precipitation processes. Latest satellites measurements enable us to determine dust loadings and cloud distributions and can potentially be used to reduce the uncertainties in the estimations of aerosol effects on climate. This study uses sensors on various satellites to investigate the impact of mineral dust on cloud microphysical and precipitation processes in convective systems. A trans-Atlantic dust outbreak of Saharan origin occurring in early March 2004 is considered. For the observed convective systems under a given convective strength, small hydrometeors were found more prevalent in the dusty stratiform regions than in those regions that were dust free. Evidence of abundant cloud ice particles in the dust regions, particularly at altitudes where heterogeneous nucleation of mineral dust prevails, further supports the observed changes of clouds and precipitation. These microphysical effects of the dusts on clouds are to shift the size spectrum of precipitation-sized hydrometeors from heavy precipitation to light precipitation and ultimately to suppress precipitation and increase the lifecycle of cloud systems, especially for stratiform clouds.

B Lin↗
NASA NTRS2018

Characterizing Differences in the Aerosol Plume and Cloud Structure over Ascension Island During the 2016 and 2017 Biomass Burning Seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between marine boundary cloud morphology and the environmental conditions in which the clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean. It is likely that the absorbing and heating properties of these aerosols influence the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus in this region; however, this has yet to be quantified. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). Through the use of AMF1 observations, the Modern Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), and back trajectories from the Hybrid Single-Particle Lagrangian Integrated Trajectory model (HYSPLIT), it will be demonstrated that differences in the atmospheric circulation during the two years result in varying aerosol conditions over Ascension Island. When the aerosol plume is overhead, the aerosol loading is higher during the 2016 season as a result of a weaker subtropical high-pressure system. Furthermore, the aerosol plume originates from central Africa in 2016, but further south in 2017. Contrasts in the season-to-season and day-to-day aerosol loading are used to categorize boundary layer cloud and sub-cloud turbulence measurements above Ascension Island using the AMF1 Doppler lidar and cloud radar.

Collow, Allison B. Marquardt↗
NASA NTRS2019

Aerosol Radiative Effects over Ascension Island Using LASIC Observations and MERRA-2

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between marine boundary cloud morphology and the environmental conditions in which the clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean. It is likely that the absorbing and heating properties of these aerosols influence the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus in this region; however, this has yet to be quantified. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). Thermodynamic profiles will be analyzed through the unique combination of sounding data from radiosonde launches and microwave profiling radiometers, giving observations of additional quantities important for cloud development such as CAPE and CIN at a fine temporal resolution. The thermodynamic profiles will be presented in conjunction with detailed observations of the cloud structure over the site from a K-band cloud radar, micropulse lidar, and laser ceilometer. Finally, the observed thermodynamic and cloud profiles will be used as input forcing, alongside aerosols from the Modern Era Retrospective analysis for Research and Applications, version 2 (MERRA-2), for the Rapid Radiative Transfer Model (RRTM) to gain information regarding the radiative heating profiles. Idealized experiments using RRTM with and without aerosols will be used to quantify the impact of biomass burning carbonaceous aerosol plumes as they pass over the site.

Collow, Allie↗
NASA NTRS2019

Thermodynamic, Cloud, and Radiative Heating Profiles over Ascension Island During the 2016 and 2017 Biomass Burning Seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between marine boundary cloud morphology and the environmental conditions in which the clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean. It is likely that the absorbing and heating properties of these aerosols influence the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus in this region; however, this has yet to be quantified. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). Thermodynamic profiles will be analyzed through the unique combination of sounding data from radiosonde launches and microwave profiling radiometers, giving observations of additional quantities important for cloud development such as CAPE and CIN at a fine temporal resolution. The thermodynamic profiles will be presented in conjunction with detailed observations of the cloud structure over the site from a K-band cloud radar, micropulse lidar, and laser ceilometer. Finally, the observed thermodynamic and cloud profiles will be used as input forcing, alongside aerosols from the Modern Era Retrospective analysis for Research and Applications, version 2 (MERRA-2), for the Rapid Radiative Transfer Model (RRTM) to gain information regarding the radiative heating profiles. Idealized experiments using RRTM with and without aerosols will be used to quantify the impact of biomass burning carbonaceous aerosol plumes as they pass over the site.

Collow, Allison B.↗
NASA NTRS2020

Radiative Heating from Biomass Burning Aerosol and its Impact on Cloud Structure in the Southeast Atlantic

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between marine boundary cloud morphology and the environmental conditions in which the clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean. It is likely that the absorbing and heating properties of these aerosols influence the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus in this region; however, this has yet to be quantified. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to collect observations of cloud and aerosol properties during two consecutive biomass burning seasons during July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). Thermodynamic profiles will be analyzed through the unique combination of sounding data from radiosonde launches and microwave profiling radiometers, giving observations of additional quantities important for cloud development such as CAPE and CIN at a fine temporal resolution. The thermodynamic profiles will be presented in conjunction with detailed observations of the cloud structure over the site from a K-band cloud radar, micropulse lidar, and laser ceilometer. The observed thermodynamic and cloud profiles will be used as input forcing, alongside aerosols from the Modern Era Retrospective analysis for Research and Applications, version 2 (MERRA-2), for the Rapid Radiative Transfer Model (RRTM) to gain information regarding the radiative heating profiles. Idealized experiments using RRTM with and without aerosols will be used to quantify the impact of biomass burning carbonaceous aerosol plumes as they pass over the site. Due to documented discrepancies in the single scatter albedo (SSA) between models and observations, further sensitivity experiments will demonstrate the importance of the optical properties of biomass burning aerosol in accurately representing heating within the column. Finally, the heating rates will be put into context of the cloud structure over the site from the perspective of the mass flux closure from the University of Washington shallow convective scheme.

Collow, Allison↗