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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 307 records · Page 17

X-Ray Spectroscopic Studies of X-Pinch Plasmas with 3-5 Picosecond Resolution: A Quest for Clear Experimental Evidence for Radiative Collapse in the X-ray Spectra (Final Report)

Dense Z-pinch plasmas produced from current-carrying exploding wires frequently produce very brief (less than 0.1 nanosecond), intense, bursts of soft X-rays from tiny (about 1 micrometer), very hot (10-30 million K) regions of the plasma. This project addresses the physical processes that lead to those tiny, high-energy density plasmas and develops means to measure the conditions just before and during the X-ray bursts. One possible relevant process is radiative collapse, which starts if the power radiated by a dense Z-pinch, proportional to the density-squared, exceeds the resistive heating rate from the current flow, thereby cooling the plasma and enabling the magnetic pinching force to exceed the outward plasma thermal pressure. As the resulting radius reduction further increases the radiation rate, this process produces a runaway magnetic implosion. A competing mechanism is a sausage-like instability that can develop in a Z-pinch plasma at a lower current than is needed to induce radiative collapse. This mechanism can also produce tiny hot spots in the neck regions of the sausage-shaped plasma column. It is also possible that these two mechanisms work together to produce the X-ray emitting hot spots. If radiative collapse does contribute to hot spot formation, it would be terminated when the plasma becomes so dense that the radiation cannot escape, enabling the plasma kinetic pressure to build up and stop the current-driven implosion. This project aims to study the development of the hot spots by means of high temporal and spatial resolution X-ray spectroscopy to determine if there is evidence for the presence of the radiative collapse mechanism. Progress toward this goal is presented. To summarize, during the four-year period 09/15/2017 - 9/14/2021, we have collected necessary spectroscopic data to determine the plasma conditions and continue to do so. We are also now in the process of calibrating diagnostic systems (especially the x-ray streak camera system) and analyzing data to determine plasma conditions as a function of time before, during and after the X-ray burst.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Deep learning for NLTE spectral opacities

Computer simulations of high energy density science experiments are computationally challenging, consisting of multiple physics calculations including radiation transport, hydrodynamics, atomic physics, nuclear reactions, laser–plasma interactions, and more. To simulate inertial confinement fusion (ICF) experiments at high fidelity, each of these physics calculations should be as detailed as possible. However, this quickly becomes too computationally expensive even for modern supercomputers, and thus many simplifying assumptions are made to reduce the required computational time. Much of the research has focused on acceleration techniques for the various packages in multiphysics codes. In this work, we explore a novel method for accelerating physics packages via machine learning. The non-local thermodynamic equilibrium (NLTE) package is one of the most expensive calculations in the simulations of indirect drive inertial confinement fusion, taking several tens of percent of the total wall clock time. We explore the use of machine learning to accelerate this package, by essentially replacing the physics calculation with a deep neural network that has been trained to emulate the physics code. Overall, we demonstrate the feasibility of this approach on a simple problem and perform a side-by-side comparison of the physics calculation and the neural network inline in an ICF Hohlraum simulation. We show that the neural network achieves a 10× speed up in NLTE computational time while achieving good agreement with the physics code for several quantities of interest.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Analysis of the laser welding keyhole using inline coherent imaging

Laser beam welding is a widely used fusion welding process in many industrial applications such as automotive, aerospace, energy, defense, and medical products. Industry has a fundamental need to model the laser welding process to minimize experimental testing and improve confidence in production welds. However, computational models attempting to predict weld formation are limited by an incomplete understanding of the beam-material interactions. As a consequence, these models do not accurately predict the mechanisms associated with laser weld formation. To improve the current state of prediction capabilities, it is vital to better detect/measure the physical aspects of the weld pool during high energy density welding. In this work, a novel real-time laser weld monitoring device using inline coherent imaging (ICI) was used to provide a fundamental understanding of laser weld formation via vaporization. The objective of this work was to investigate and quantify the relationship relating laser weld parameters and the vapor capillary (keyhole) through a state-of-the-art measurement technique. Bead-on-plate laser beam welds were produced with partial penetration on 304L stainless steel, 2205 duplex stainless steel, and Ti-6Al-4V. Keyhole monitoring was performed using a commercially available ICI system to collect keyhole penetration data in real time. These measurements were reconstructed to generate the vapor capillary shape at different welding parameters. Process parameters significantly influenced the keyhole shape and the keyhole root position relative to the process beam. Finally, the keyhole geometry showed distinct differences between the stainless steel alloys and Ti-6Al-4V.

2205↗

DCTRGAN: improving the precision of generative models with reweighting

Significant advances in deep learning have led to more widely used and precise neural network-based generative models such as Generative Adversarial Networks (Gans). We introduce a post-hoc correction to deep generative models to further improve their fidelity, based on the Deep neural networks using the Classification for Tuning and Reweighting (Dctr) protocol. The correction takes the form of a reweighting function that can be applied to generated examples when making predictions from the simulation. We illustrate this approach using Gans trained on standard multimodal probability densities as well as calorimeter simulations from high energy physics. We show that the weighted Gan examples significantly improve the accuracy of the generated samples without a large loss in statistical power. This approach could be applied to any generative model and is a promising refinement method for high energy physics applications and beyond.

47 OTHER INSTRUMENTATION↗

Completion document for MRT 8824 - Upgrade NIF’s gaseous radiochemistry diagnostics (RAGS) to support weapons science

This milestone highlights the successful upgrade and deployment of the Radiochemical Analysis of Gaseous Samples (RAGS) system, which delivers high-quality measurements (<20% uncertainty) of activated gaseous species from NIF implosions. These measurements are critical for supporting Stockpile Stewardship Program (SSP) relevant platforms, including LANL’s Double Shell and LLNL’s Pushered Single Shell campaigns. The RAGS diagnostic technique enables analysis of short-range mixing in implosions using high-Z shells, which are otherwise inaccessible to conventional x-ray diagnostic methods. By facilitating the investigation of high-Z material mixing into fusion burn, this system provides essential data for quantifying and interpreting results in high-energy density (HED) experiments. This report details the physics motivation, diagnostic fundamentals, planned and enacted upgrade work, and the quantification of uncertainty for the upgraded system.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Reduced mixing in inertial confinement fusion with early-time interface acceleration

In inertial confinement fusion (ICF) implosions, the interface between the cryogenic DT fuel and the ablator is unstable to shock acceleration (the Richtmyer-Meshkov instability, RM) and constant acceleration (Rayleigh-Taylor instability, RT). Instability growth at this interface can reduce the final compression, limiting fusion burnup. If the constant acceleration is in the direction of the lighter material (negative Atwood number), the RT instability produces oscillatory motion that can stabilize against RM growth. Theory and simulations suggest this scenario occurred at early times in some ICF experiments on the National Ignition Facility, possibly explaining their favorable performance compared to one-dimensional simulations. In conclusion, this characteristic is being included in newer, lower adiabat designs, seeking to improve compression while minimizing ablator mixing into the fuel.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A Covalent Organic Framework for Fast-Charge and Durable Rechargeable Mg Storage

High safety, low cost and high volumetric capacity rechargeable magnesium batteries (RMBs) are promising alternatives to lithium ion batteries. However, lack of high power, high energy and stable cathodes for RMBs hinders their commercialization. Herein, an environmentally benign, low cost and sustainable covalent organic framework (COF) cathode for Mg storage is reported for the first time. It delivers a high power density of 2.8 kW kg -1 , a high specific energy density of 146 Wh kg -1 , and ultra-long cycle life of 3000 cycles with very slow capacity decay rate of 0.0196% per cycle, representing one of the best cathodes to date. The comprehensive electrochemical analysis proves that triazine ring sites in COF are redox centers for reversible reaction with magnesium ions, and the ultra-fast reaction kinetic is mainly attributed to pseudocapacitive behavior. The high-rate Mg storage of COF offers new opportunities for the development of ultra-stable and fast charge RMBs.

36 MATERIALS SCIENCE↗

Principles and applications of x-ray light sources driven by laser wakefield acceleration

One of the most prominent applications of modern particle accelerators is the generation of radiation. In a synchrotron or an x-ray free electron laser (XFEL), high energy electrons oscillating in periodic magnetic structures emit bright x rays. In spite of their scientific appeal that will remain evident for many decades, one limitation of synchrotrons and XFELs is their typical mile-long size and their cost, which often limits access to the broader scientific community. Here, this tutorial reviews the principles and prospects of using plasmas produced by intense lasers as particle accelerators and x-ray light sources, as well as some of the applications they enable. A plasma is an ionized medium that can sustain electrical fields many orders of magnitude higher than that in conventional radio frequency accelerator structures and can be used to accelerate electrons. When short, intense laser pulses are focused into a gas, it produces electron plasma waves in which electrons can be trapped and accelerated to GeV energies. This process, laser-wakefield acceleration (LWFA), is analogous to a surfer being propelled by an ocean wave. Many radiation sources, from THz to gamma-rays, can be produced by these relativistic electrons. This tutorial reviews several LWFA-driven sources in the keV-MeV photon energy range: betatron radiation, inverse Compton scattering, bremsstrahlung radiation, and undulator/XFEL radiation. X rays from laser plasma accelerators have many emerging applications. They can be used in innovative and flexible x-ray imaging and x-ray absorption spectroscopy configurations, for use in biology, industry, and high-energy density science.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

2022 LaserNetUS Users' Meeting

Organized and funded in 2018 through the US Department of Energy, Office of Fusion Energy Sciences (FES), LaserNetUS was created to provide vastly improved access to unique lasers for researchers. LaserNetUS is a network of ten high-power laser facilities, both academic and national laboratories, across the United States and Canada. These labs operate many of the premier mid- to large-scale high-intensity laser facilities in the US and Canada that are designed to be used in pioneering experimental studies in high energy density plasma and high field optical science. The network’s principal goal is to provide access to these state-of-the-art laser facilities to a broad range of researchers in the US and abroad. In its over four years of operation, LaserNetUS has awarded beamtime for over 60 user experiments to researchers from 25 different institutions. Over 400 user scientists, many of whom are students and post-docs, have participated in experiments at LaserNetUS facilities so far. The network now has over 1250 members. The LaserNetUS institutions are Colorado State University, Lawrence Berkeley National Lab, Lawrence Livermore National Lab, SLAC National Lab, The Ohio State University, University of Michigan, University of Nebraska-Lincoln, Institut National de la Recherche Scientifique, University of Rochester, and University of Texas at Austin. LaserNetUS hosted its first in-person Annual Users’ Meeting at Colorado State University in Fort Collins, CO, Aug 16-18, 2022. The meeting had 158 attendees, including 39 sponsored students and post-docs whose attendance and travel to the meeting were covered by DOE funds. Attendees included the 2018 Nobel Laureate in Physics, Donna Strickland. The program consisted of 5 plenary talks and several invited and contributed talks, a user community forum, a poster session, and built-in time for networking. The event focused on students and early career professionals. The poster session was held in combination with a reception to facilitate discussions and maximize interactions between the participants. The 39 sponsored students each presented a poster at the poster session, giving them valuable practice in sharing their research with others in the field. Many students and postdocs also gave talks during the main programming. Lunch and coffee breaks were provided for attendees for the duration of the conference on CSU’s campus. This allowed for networking among all participants. The building used to host the conference also had plenty of seating outside the auditorium, which was conducive to smaller one-on-one meetings and discussions between participants. There was also a lab tour of CSU’s Advanced Beam Laboratory. The day before and after the conference also included satellite meetings for the lab PIs and the Scientific Advisory Board. DOE support was used for rental of the auditorium and supporting rooms, student participation, 50% of the food costs, and transportation to the Advanced Beam Lab.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Machine-learned quantum molecular dynamics calculations of warm dense equation of state and ionic transport coefficients of deuterated water

White dwarf models require accurate equations of state and ionic transport coefficients in the warm dense matter regime, where kinetic theory models and tabulated equations of state are often inaccurate. In this work, spectral-partitioned density functional theory and machine-learned interatomic potentials are combined to perform large-scale, first-principles quantum molecular dynamics simulations of deuterated water (D 2 O) near the principal Hugoniot. This approach retains Kohn-Sham accuracy while achieving orders-of-magnitude speedup, yielding converged equation of state and transport properties over a broad pressure and temperature range. The results reveal the thermodynamic conditions under which ionic transport models for interdiffusivity and shear viscosity converge and identify those in closest agreement with density functional theory benchmarks at temperatures in the warm dense matter regime. The present framework extends first-principles transport calculations to higher temperatures than previously achieved, and provides an efficient, scalable, and general approach for studying transport properties in complex multicomponent mixtures.

79 ASTRONOMY AND ASTROPHYSICS↗

Observation of a magneto-Rayleigh-Taylor instability in magnetically collimated plasma jets

We present the direct experimental observation of the formation of a diamagnetic cavity and magneto-Rayleigh-Taylor (MRT) instability in a β ≈ 1 high energy density plasma. Proton radiography is used to measure the two dimensional path-integrated magnetic field in a laser-produced plasma propagating parallel to a preimposed magnetic field. Flutelike structures, associated with the MRT instability, are observed to grow at the surface of the cavity, with a measured wavelength of 1.2 mm and growth time of 4 ns. These measurements are in good agreement with predictions of three dimensional magnetohydrodynamic simulations using the GORGON code. Published by the American Physical Society 2024

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

High-temperature ion-thermal behavior from average-atom calculations

Atom-in-jellium calculations of the Einstein frequency were used to calculate the mean displacement of an ion over a wide range of compression and temperature. Expressed as a fraction of the Wigner-Seitz radius, the displacement is a measure of the asymptotic freedom of the ion at high temperature, and thus of the change in heat capacity from six to three quadratic degrees of freedom per atom. A functional form for free energy was proposed based on the Maxwell-Boltzmann distribution as a correction to the Debye free energy, with a single free parameter representing the effective density of potential modes to be saturated. Finally, this parameter was investigated using molecular dynamics simulations, and found to be ~0.2 per atom. In this way, the ion-thermal contribution can be calculated for a wide-range equation of state (EOS) without requiring a large number of molecular dynamics simulations. Example calculations were performed for carbon, including the sensitivity of key EOS loci to ionic freedom.

74 ATOMIC AND MOLECULAR PHYSICS↗

Dataset from 3D FLASH Computation of National Ignition Facility Shot N210201-001

This data comes from a 3D FLASH [Fryxell et al. ApJS 131, 273 (2000); Tzeferacos et al. HEDP 17, 24-31(2015)] computation of a cylindrical implosion experiment performed at the National Ignition Facility (shot number N210201-001). FLASH is an open-access radiation-hydrodynamics code being used to simulate high-energy-density systems.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Laboratory for Laser Energetics Targets Inertial Confinement Fusion

The University of Rochester’s Laboratory for Laser Energetics is targeting laser-driven inertial confinement fusion, as part of National Nuclear Security Administration’s Stockpile Stewardship Program and in the quest for clean sources of energy. The Laboratory for Laser Energetics (LLE) is home to two extremely powerful lasers—OMEGA and OMEGA EP—and researchers are using them to explore laser-driven inertial confinement fusion (ICF). ICF involves compressing a small amount of fuel consisting of hydrogen isotopes, deuterium (D), and tritium (T), and heating it to temperatures greater than the center of stars. “When these conditions are reached, the fuel undergoes fusion—releasing enormous energy that can be used for research relevant to the National Nuclear Security Administration’s (NNSA) Stockpile Stewardship Program (SSP) and to drive carbon-free power plants,” explains Valeri Goncharov, distinguished scientist and director of the Theory Division at LLE. LLE was established at the University of Rochester in 1970 and is the largest U.S. Department of Energy university-based research program in the nation, supported by the National Nuclear Security Administration as part of its Stockpile Stewardship Program (SSP). “As a center for exploring the interaction of intense radiation with matter, LLE is a unique national resource for research and education in science and technology,” says Goncharov. “Our current research includes exploring fusion for the SSP program and as a future source of energy, developing new laser and materials technologies, and pursuing a better understanding of high-energy-density phenomena.”

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Key metrics of progress in the NIF ignition implosions and future challenges on the path to higher yields

Successful demonstration of an implosion that meets the physics metrics for ignition on the National Ignition Facility (NIF) in August 2021 and demonstration of target energy gain G > 1 in December 2022 represented the culmination of more than a decade of research on the NIF. An in-depth analysis of the key ignition metrics achieved on the NIF over the past decade shows sustained progress toward identifying and mitigating degradation effects. Ignition implosions on the NIF have progressed from early experiments whose compressed fuel conditions were degraded by a factor of 10–20 below the ignition threshold with yields of only 1%–2% of the laser energy, to current experiments that significantly exceed the ignition threshold and in the best experiments achieve yields greater than twice the laser energy. It is very likely that NIF can get more than 20 MJ of yield and possibly 50–70 MJ yields when fully optimized at an ultraviolet laser energy of 2.6 MJ following the completion of the NIF Extended Yield Capability Project. Achieving these higher yields will also require improvements to capsules at larger size and possibly with alternate materials, as well as an improved understanding of hohlraum and capsule physics. Now that NIF has achieved ignition, the design of a Next Generation High Energy Density Facility that could achieve the National Nuclear Security Administration long-term goal of substantially higher yields than the NIF can proceed with a more confident physics base. We evaluate these opportunities including possible applications for inertial fusion energy and likely challenges to achieving this level of performance over the next decade.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Energy storage technology with extreme high energy density capability

A capacitor includes a first electrode having a substrate and a plurality of nanostructures physically and electrically coupled to the substrate. The capacitor also includes a solid, non-conductive interlayer deposited over the nanostructures to coat the nanostructures, and extending between the nanostructures, and a second electrode deposited over the interlayer and extending between the nanostructures. The interlayer insulates the first and second electrode layers from one another.

Gao, Kaizhong↗