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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 307 records · Page 17
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Wind-driven emissions of coarse-mode particles in an urban environment

Abstract. Quantifying surface–atmosphere exchange rates of particles is important for understanding the role of suspended particulate matter in radiative transfer, clouds, precipitation, and climate change. Emissions of coarse-mode particles with a diameter greater than 0.5 µm provide giant cloud condensation nuclei and ice nuclei. These emissions are critical for understanding the evolution of cloud microphysical properties yet remain poorly understood. Here we introduce a new method that uses lidar retrievals of the elastic backscatter and Doppler velocity to obtain surface number emissions of particles with a diameter greater than 0.53 µm. The technique is applied to study particle number fluxes over a 2-month period from 1 June to 10 August 2022 during the TRACER campaign at an urban site near Houston, TX, USA. We found that all the observed fluxes were positive (upwards), indicating particle emission from the surface. The fluxes followed a diurnal pattern and peaked near noon local time. Flux intensity varied through the 2 months with multi-day periods of strong fluxes and multi-day periods of weak fluxes. Emission particle number fluxes peaked near ∼ 100 cm−2 s−1. The daily averaged emission fluxes correlated with friction velocity and were anticorrelated with surface relative humidity. The emission flux can be parameterized as F= 3000 u*4, where u* is the friction velocity in m s−1 and the emission flux F is in cm−2 s−1. The u* dependence is consistent with emission from wind-driven erosion. Estimated values for the mass flux are in the lower range of literature values from non-urban sites. These results demonstrate that urban environments may play an important role in supplying coarse-mode particles to the boundary layer. We anticipate that quantification of these emissions will help constrain aerosol–cloud interaction models that use prognostic aerosol schemes.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Sizing ice hydrometeor populations using the dual-wavelength radar ratio

Dual-wavelength (3.2 and 0.32 cm, i.e., X- and W-radar bands) radar ratio (DWR) measurements in ice clouds and precipitation using Canada's National Research Council Institute for Aerospace Research airborne radar are compared to closely collocated particle microphysical in situ sampling data in order to develop relations between DWR and characteristic hydrometeor size. This study uses the radar and in situ data sets collected during the In-Cloud ICing and Large-drop Experiment (ICICLE) campaign in midlatitude frontal clouds. Since atmospheric particle scattering at X band is predominantly in the Rayleigh regime and the W-band frequency is the highest frequency usually used for hydrometeor remote sensing, the X–W-band combination provides a relatively strong dual-wavelength reflectivity difference. This study considers radar and in situ measurements conducted in relatively homogeneous cloud and precipitation conditions. Measurements show that under these conditions, the difference between the X-band radar reflectivities observed with vertical and horizontal pointing of the radar beam are generally small and often negligible. However, W-band reflectivities at vertical beam pointing are, on average, larger than those for horizontal beam pointing by about 4 dB, which is a non-Rayleigh scattering effect from preferentially oriented non-spherical particles. A horizontal radar beam DWR–mean volume particle size relation, D v , provides robust estimates of this characteristic size for populations of particles with different habits. Uncertainties of D v retrievals using DWR are around 0.6 mm when D v is greater than approximately 1 mm. Size estimates using vertical radar beam DWRs have larger uncertainties due to smaller dual-wavelength signals and stronger influences of hydrometeor habits and orientations at this geometry of beam pointing. Mean relations among different characteristic sizes, which describe the entire particle size distribution (PSD), such as D v , and other sizes used in various applications (e.g., the mean, effective, and median sizes) are derived, so the results of this study can be used for estimating different PSD characteristic sizes.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Physics of beam-driven ion cyclotron emission in the large plasma device

Abstract Ion cyclotron emission (ICE) is widely observed from spatially localised minority energetic ion populations in toroidal magnetically confined fusion (MCF) plasmas, both tokamaks and stellarators. Its spectral structure is typically regular with narrow suprathermal peaks, whose frequency separation matches a local energetic ion cyclotron frequency. Here we report the first computational (fully nonlinear self-consistent kinetic particle-in-cell code) and analytical (linear magnetoacoustic cyclotron instability (MCI)) studies of ICE observations from cylindrical plasmas contained in the Large Plasma Device (LAPD). Because LAPD is cylindrical, the plasma physics giving rise to the observed ICE spectrum necessarily excludes toroidal effects. Our approach, previously successful for toroidal plasma ICE, assumes slab geometry and hence is well adapted to LAPD. ICE from LAPD is strongly electrostatic, as distinct from electromagnetic, and is driven by 15 keV beam ions for which the ratio of perpendicular speed to the local Alfven speed, v ⊥ / v A , is 0.15, lower than in MCF plasmas from which beam-driven ICE has previously been observed. Our results are in good agreement with these observations. There is congruence between simulated ICE spectra, obtained in the saturated nonlinear regime of our computations, and observed ICE spectra; the underlying physics is essentially the same as in toroidal plasmas; and there is alignment with linear analytical theory where appropriate. The present work establishes a mapping from the cylindrical LAPD ICE observations to toroidal MCF ICE observations. The LAPD spectra are instances of beam-driven MCI-type ICE in its sub-Alfvenic, predominantly electrostatic manifestation, which has precedents in MCF stretching back to the 1990s. An interesting corollary is that, for many purposes, ICE in toroidal MCF plasmas ‘might as well’ be occurring in a cylinder.

Samant, O. (ORCID:0000000226055363)↗
DOE OSTI2020

Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea

The Arctic is rapidly transforming due to sea ice loss, increasing shipping activity, and oil and gas development. Associated marine and combustion emissions influence atmospheric aerosol composition, impacting complex aerosol–cloud–climate feedbacks. To improve understanding of the sources and processes determining Arctic aerosol composition, atmospheric particles were collected aboard the Korean icebreaker R/V Araon cruising within the Bering Strait and Chukchi Sea during August 2016. Offline analyses of individual particles by microspectroscopic techniques, including scanning electron microscopy with energy dispersive X-ray spectroscopy and atomic force microscopy with infrared spectroscopy, provided information on particle size, morphology, and chemical composition. The most commonly observed particle types were sea spray aerosol (SSA), comprising ~60–90%, by number, of supermicron particles, and organic aerosol (OA), comprising ~50–90%, by number, of submicron particles. Sulfate and nitrate were internally mixed within both SSA and OA particles, consistent with particle multiphase reactions during atmospheric transport. Within the Bering Strait, SSA and OA particles were more aged, with greater number fractions of particles containing sulfate and/or nitrate, compared to particles collected over the Chukchi Sea. This is indicative of greater pollution influence within the Bering Strait from coastal and inland sources, while the Chukchi Sea is primarily influenced by marine sources.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Some exactly solvable and tunable frustrated spin models

In this report we discuss three exactly solvable spin models of geometric frustration. First, we discuss a 1-parameter subfamily of the 16 vertex model, which can be mapped to a planar Ising model and solved via Fisher-Dubedát decorations. We then consider a 1-parameter family generalization of the Villain’s fully frustrated model, which interpolates between Onsager’s 2D Ising model and the Villain one. We then discuss spin ice models on a tree, which can be solved exactly using recursions a lá Bethe.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Impact of biomass burning aerosols on radiation, clouds, and precipitation over the Amazon: relative importance of aerosol–cloud and aerosol–radiation interactions

Biomass burning (BB) aerosols can influence regional and global climate through interactions with radiation, clouds, and precipitation. Here, we investigate the impact of BB aerosols on the energy balance and hydrological cycle over the Amazon Basin during the dry season. We performed simulations with a fully coupled meteorology–chemistry model, the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem), for a range of different BB emission scenarios to explore and characterize nonlinear effects and individual contributions from aerosol–radiation interactions (ARIs) and aerosol–cloud interactions (ACIs). The ARIs of BB aerosols tend to suppress low-level liquid clouds by local warming and increased evaporation and to facilitate the formation of high-level ice clouds by enhancing updrafts and condensation at high altitudes. In contrast, the ACIs of BB aerosol particles tend to enhance the formation and lifetime of low-level liquid clouds by providing more cloud condensation nuclei (CCN) and to suppress the formation of high-level ice clouds by reducing updrafts and condensable water vapor at high altitudes (>8 km). For scenarios representing the lower and upper limits of BB emission estimates for recent years (2002–2016), we obtained total regional BB aerosol radiative forcings of –0.2 and 1.5 W m –2 , respectively, showing that the influence of BB aerosols on the regional energy balance can range from modest cooling to strong warming. We find that ACIs dominate at low BB emission rates and low aerosol optical depth (AOD), leading to an increased cloud liquid water path (LWP) and negative radiative forcing, whereas ARIs dominate at high BB emission rates and high AOD, leading to a reduction of LWP and positive radiative forcing. In all scenarios, BB aerosols led to a decrease in the frequency of occurrence and rate of precipitation, caused primarily by ACI effects at low aerosol loading and by ARI effects at high aerosol loading. The dependence of precipitation reduction on BB aerosol loading is greater in a strong convective regime than under weakly convective conditions. Overall, our results show that ACIs tend to saturate at high aerosol loading, whereas the strength of ARIs continues to increase and plays a more important role in highly polluted episodes and regions. This should hold not only for BB aerosols over the Amazon, but also for other light-absorbing aerosols such as fossil fuel combustion aerosols in industrialized and densely populated areas. The importance of ARIs at high aerosol loading highlights the need for accurately characterizing aerosol optical properties in the investigation of aerosol effects on clouds, precipitation, and climate.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Atmospheric fungal nanoparticle bursts

Aerosol nanoparticles play an important role in the climate system by affecting cloud formation and properties, as well as in human health because of their deep reach into lungs and the circulatory system. Determining nanoparticle sources and composition is a major challenge in assessing their impacts in these areas. The sudden appearance of large numbers of atmospheric nanoparticles is commonly attributed to secondary formation from gas-phase precursors, but in many cases, the evidence for this is equivocal. We report the detection of a mode of fungal fragments with a mobility diameter of roughly 30 nm released in episodic bursts in ambient air over an agricultural area in northern Oklahoma. These events reached concentrations orders of magnitude higher than other reports of biological particles and show similarities to unclarified events reported previously in the Amazon. These particles potentially represent a large source of both cloud-forming ice nuclei and respirable allergens in a variety of ecosystems.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Proposal for broad-range directional detection of light dark matter in cryogenic ice

We propose hexagonal ice (H 2 ⁡O) as a new target for light dark matter (DM) direct detection. Ice, a polar material, is suitable for single phonon detection through DM scattering for which we consider light dark photon and light scalar mediator models. We report a rate sensitivity down to a DM mass of ~keV, constituting a broader mass range than other promising candidates. We find better sensitivity for near-term experimental thresholds from the presence of high-frequency phonons. These advantages, and ice’s availability, make it highly promising for single-phonon detection.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Enhanced energy confinement after series of pellets in Wendelstein 7-X

A series of ice pellets was injected into the advanced stellarator Wendelstein 7-X (W7-X). Although the pellets were small and slow, deep and efficient particle fueling could be observed experimentally. The most striking feature appearing after the injection of the pellets, however, was a transient increase in the energy confinement time. This transient phase resembled in several aspects modes of enhanced confinement after gas-puff or pellet injection, as observed in other fusion experiments. All experimental attempts, to prolong this phase, failed. In this paper, discharges are described that show the enhanced energy confinement, and some conditions are summarized which seem to be essential in order to generate it. The focus here is on deep particle fueling by pellets, and shaping of the density profiles during and after the series of pellets. During this time, neutral gas particle re-fueling at the plasma edge is reduced, while density profile peaking and low impurity radiation losses are present.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Tethered balloon-borne profile measurements of atmospheric properties in the cloudy atmospheric boundary layer over the Arctic sea ice during MOSAiC: Overview and first results

The tethered balloon-borne measurement system BELUGA (Balloon-bornE moduLar Utility for profilinG the lower Atmosphere) was deployed over the Arctic sea ice for 4 weeks in summer 2020 as part of the Multidisciplinary drifting Observatory for the Study of Arctic Climate expedition. Using BELUGA, vertical profiles of dynamic, thermodynamic, aerosol particle, cloud, radiation, and turbulence properties were measured from the ground up to a height of 1,500 m. BELUGA was operated during an anomalously warm period with frequent liquid water clouds and variable sea ice conditions. Three case studies of liquid water phase, single-layer clouds observed on 3 days (July 13, 23, and 24, 2020) are discussed to show the potential of the collected data set to comprehensively investigate cloud properties determining cloud evolution in the inner Arctic over sea ice. Simulated back-trajectories show that the observed clouds have evolved within 3 different air masses (“aged Arctic,” “advected over sea ice,” and “advected over open ocean”), which left distinct fingerprints in the cloud properties. Strong cloud top radiative cooling rates agree with simulated results of previous studies. The weak warming at cloud base is mostly driven by the vertical temperature profile between the surface and cloud base. In-cloud turbulence induced by the cloud top cooling was similar in strength compared to former studies. From the extent of the mixing layer, it is speculated that the overall cloud cooling is stronger and thus faster in the warm oceanic air mass. Larger aerosol particle number concentrations and larger sizes were observed in the air mass advected over the sea ice and in the air mass advected over the open ocean.

Arctic↗
DOE OSTI2023

Extensively Microtwinned Diamond with Nanolaminates of Lonsdaleite Formed by Flash Laser Heating of Glassy Carbon

Diamond’s unique properties on the nanoscale make it one of the most important materials for use in biosensors and quantum computing and for components that can withstand the harsh environments of space. We synthesize oriented, faceted diamond particles by flash laser heating of glassy carbon at 16 GPa and 2300 K. Detailed transmission electron microscopy shows them to consist of a mosaic of diamond nanocrystals frequently joined at twin boundaries forming microtwins. Striking 3-fold translational periodicity was observed in both imaging and diffraction. This periodicity was shown to originate from nanodimensional wedge-shaped overlapping regions of twinned diamond and not from a possible 9R polytype, which has also been reported in other group IVa elements and water ice. Extended bilayers of hexagonal layer stacking were observed, forming lonsdaleite nanolaminates. In conclusion, the particles exhibited optical fluorescence with a rapid quench time (<1 ns) attributed to their unique twinned microstructure.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2021

Improving GCM Representation of Convective Cloud Microphysics by Using ARM Raman Lidar and Cloud Radar Observations

The overall objective of this Department of Energy (DOE) Atmospheric System Research (ASR) funded project is to improve the representation of convective cloud microphysics in global climate models (GCMs) and check it by comparing the model simulations with observations. We have derived the cloud ice water content by synthesizing ARM Raman lidar (RL) and cloud radar observations at the Atmospheric Radiation Measurement (ARM) sites. Noting that the simulated anvil clouds in terms of their macro- and micro-physical properties are sensitive to the parameterization of convective microphysical processes, observed ice water content in anvil clouds provides a useful constraint on these parameterizations. We have improved the convective microphysics parameterization scheme by (1) considering sedimentation for cloud ice crystals that do not fall in the original scheme, (2) applying a new terminal velocity parameterization that depends on the environmental conditions for convective snow, (3) adding a new hydrometeor category, “rimed ice,” to the original four-class (cloud liquid, cloud ice, rain, and snow) scheme, and (4) allowing convective clouds to detrain snow particles into stratiform clouds. We have examined the impact of improved convective cloud microphysics parameterization on the simulated global climate from GCM simulations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Counterflow Virtual Impactor (CVI) Inlet Aboard Aircraft (INLETCVI-AIR) Instrument Handbook

The counterflow virtual impactor (CVI) inlet separates out and samples cloud elements via inertial impaction. Warm, dry, particle-free carrier gas of known composition is pumped to the tip of the inlet in the direction opposite of the flow of air. The flow lines of the incoming free stream air are split. Larger droplets and ice crystals suspended in the sample air have enough inertia to penetrate the counterflow and enter the sample flow, while smaller, unactivated particles follow the streamlines of the air flowing around the inlet’s tip (Noone et al. 1988). The instrument is capable of sampling cloud elements as a function of cut size by changing the velocity of counterflow at the probe tip. The CVI cut size is usually defined as a diameter of a smallest particle for which penetration rate is 50%. For the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facilityGulfstream-159 aircraft’s CVI inlet, that value is usually around 13 microns. The dry heated air, normally used as the carrier gas, also serves to evaporate water from the hydrometeor, leaving the residuals to be sampled by in-cabin aerosol instrumentation. The number concentration of the droplet residue in the CVI sample line is usually increased with respect to corresponding cloud element number concentration. The CVI performance as a concentrator is usually described via CVI enhancement factor, which is a conversion factor between ambient volumetric concentration (not adjusted to standard temperature and pressure) and volumetric concentration in the CVI sample line.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

AERO-MAP: a data compilation and modeling approach to understand spatial variability in fine- and coarse-mode aerosol composition

Abstract. Aerosol particles are an important part of the Earth climate system, and their concentrations are spatially and temporally heterogeneous, as well as being variable in size and composition. Particles can interact with incoming solar radiation and outgoing longwave radiation, change cloud properties, affect photochemistry, impact surface air quality, change the albedo of snow and ice, and modulate carbon dioxide uptake by the land and ocean. High particulate matter concentrations at the surface represent an important public health hazard. There are substantial data sets describing aerosol particles in the literature or in public health databases, but they have not been compiled for easy use by the climate and air quality modeling community. Here, we present a new compilation of PM2.5 and PM10 surface observations, including measurements of aerosol composition, focusing on the spatial variability across different observational stations. Climate modelers are constantly looking for multiple independent lines of evidence to verify their models, and in situ surface concentration measurements, taken at the level of human settlement, present a valuable source of information about aerosols and their human impacts complementarily to the column averages or integrals often retrieved from satellites. We demonstrate a method for comparing the data sets to outputs from global climate models that are the basis for projections of future climate and large-scale aerosol transport patterns that influence local air quality. Annual trends and seasonal cycles are discussed briefly and are included in the compilation. Overall, most of the planet or even the land fraction does not have sufficient observations of surface concentrations – and, especially, particle composition – to characterize and understand the current distribution of particles. Climate models without ammonium nitrate aerosols omit ∼ 10 % of the globally averaged surface concentration of aerosol particles in both PM2.5 and PM10 size fractions, with up to 50 % of the surface concentrations not being included in some regions. In these regions, climate model aerosol forcing projections are likely to be incorrect as they do not include important trends in short-lived climate forcers.

Mahowald, Natalie M. (ORCID:000000022873997X)↗
DOE OSTI2021

Chirping ion cyclotron emission (ICE) on NSTX-U

In this work, we report on the discovery on NSTX-U of a qualitatively new type of non-thermal emission from plasmas in the ion-cyclotron frequency range (ICE). This new type of ICE is weakly damped, γ damp /ω ICE ≈ 0.14%, low order eigenmodes, excited by a fast ion population radially located near an internal transport barrier. The ICE appears as repetitive bursts with durations of ≈1 ms, and the bursts exhibit frequency chirps upwards and/or downwards with maximum δf/f ≈ 1%. We refer to this chirping ICE as ch-ICE. The bursts are longer than the typical ICE bursts of ≈100 μs reported previously for NSTX and NSTX-U, for simplicity, NSTX(-U). The chirping resembles that seen in modeling of weakly unstable fast particle driven instabilities (cf, Berk et al 1997 Phys. Lett. A 234 213). These data also provide some preliminary indications of non-linear coupling between the ch-ICE harmonics. Despite extensive experimental and theoretical studies of ICE, theoretical understanding of ICE remains qualitative at best. The detailed experimental observations of ICE from NSTX(-U) find a wide variation in the ICE characteristics. The new observations of ch-ICE presented here, combined with the characteristics of ICE on NSTX(-U) previously reported (Fredrickson et al 2019 Phys. Plasmas 26 032111), could guide the development of more complete theoretical models of ICE.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

The color of magnetic monopole noise

We relate the anomaly in the noise color of spin ice to the emergent nature of its magnetic monopoles and their random walk. Monopoles are quasi-particles, and the spin vacuum in which they wander is not structureless. Rather, the underlying spin ensemble filters the thermal white noise, leading to non-trivial coevolution. Thus, monopoles can be considered as "dressed" random walkers, activated by a non-trivial stochastic noise that subsumes mutual interactions and the coevolution of their spin vacuum. From this, we suggest that recent experimental results are interpretable in terms of monopole subdiffusion. Furthermore, we then conjecture relations between the color of the noise and other observables, such as relaxation time, monopole density, the dynamic exponent, and the order of the annihilation reaction, which suggests to us the introduction of spin-ice-specific critical exponents in a neighborhood of the ice manifold criticality.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Graupel Precipitating From Thin Arctic Clouds With Liquid Water Paths Less Than 50 g m -2

Rimed precipitation growth can efficiently remove moisture and aerosols from the boundary layer, yet thin low-level Arctic mixed-phase clouds are generally thought to precipitate pristine and aggregated ice crystals. Here we present automated surface photographic measurements showing that only 34% of precipitation particles exhibit negligible riming and that graupel particles ≥ in diameter commonly fall from clouds with liquid water paths less than 50 g m -2 . Analyses indicate that significant riming enhancement can occur provided sustained updrafts of 0.4 m s -1 , consistent with those measured in Arctic clouds. A Lagrangian numerical simulation that tracks falling particles suggests that similar updraft speeds can account for about one half of the observed riming enhancement. Riming enhancement appears particularly likely when weak temperature inversions are observed at cloud top, but a full explanation remains to be determined.

54 ENVIRONMENTAL SCIENCES↗