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At least 307 records · Page 17

Precision ultranarrow-linewidth resonance excitation (PURE) preparation of a molecular beam of nitric oxide molecules for inelastic scattering with argon

We recently reported a novel technique that utilizes narrow-linewidth lasers to selectively excite molecules into a pure quantum state with a well-resolved, tunable distribution of velocities [O. A. Krohn and D. W. Chandler, J. Phys. Chem. Lett. 15(50), 12455–12463 (2024)]. We refer to the preparation of molecules by this technique as precision ultranarrow-linewidth resonant excitation (PURE) preparation. Here, in this study, we pair this PURE preparation methodology with active frequency stabilization of the quantum cascade laser that drives the excitation. In doing so, highly velocity-resolved packets of molecules are possible, with the limitations of this velocity resolution set by the stability of the laser locking and the spectral linewidth of the transition. We show that side-of-fringe locking to a Doppler-broadened absorption spectrum of our target molecule is sufficiently stable for PURE preparation of molecules for long timescales (several hours) with highly resolved velocity spreads (σ < 3 m/s). To demonstrate the scientific utility of this new capability, we present differential cross sections from scattering between a neat molecular beam of argon and a velocity-selected beam of nitric oxide (NO) in a pure quantum state. We observe well-resolved quantum diffraction oscillations in the forward-scattered collisions as well as general trends consistent with prior characterized collisions of NO + Ar.

Krohn, Olivia A. [Sandia National Laboratories (SN↗

Gamma rays and gravitational waves from inelastic Higgs portal dark matter

We explore a simple and predictive dark matter scenario involving a complex scalar field, ϕ , coupled to the Higgs portal with no additional field content. In the UV, the field possesses a global U ( 1 ) symmetry which is broken by mass terms and Higgs portal interactions. In the mass basis, the complex field splits into a pair of real scalars with a small mass splitting (in analogy to pseudo-Dirac fermions), such that the Higgs portal acquires both diagonal and off-diagonal terms with respect to these eigenstates. In the parameter space where the off-diagonal interaction predominates, this scenario is safe from direct detection constraints. Moreover, this model provides a viable explanation for the longstanding Galactic Center γ -ray excess. Additionally, this model influences the Higgs potential in a way that could facilitate a strong first-order electroweak phase transition in the early Universe, potentially leading to a stochastic gravitational wave background that could fall within the reach of upcoming space-based detectors.

Hooper, Dan [Wisconsin U., Madison] (ORCID:0009000↗

Measurements of higher-order cumulants of multiplicity and net-electric charge distributions in inelastic proton-proton interactions by NA61/SHINE

This paper presents the energy dependence of multiplicity and net-electric charge fluctuations in p+p interactions at beam momenta 20, 31, 40, 80, and 158 \(\text{ Ge }\hspace{-1.00006pt}\text{ V }\!/\!c\). Results are corrected for the experimental biases and quantified with the use of cumulants and factorial cumulants. Cumulant ratios are an essential tool in the search for the critical point of strongly interacting matter in heavy ion collisions. Measurements performed in p+p interactions provide a vital baseline estimation in these studies. The measured signals are compared with the string hadronic models Epos1.99 and FTFP-BERT.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Erratum to: Measurements of higher-order cumulants of multiplicity and net-electric charge distributions in inelastic proton-proton interactions by NA61/SHINE

This Erratum replaces, due to a discovery of coding mistakes, the following quantities: κ 3 /κ 1 of the h + − h − distribution presented in Fig. 6 and Table 6, κ 4 listed in Table 4, and $\hat{C}$ 4 presented in Fig. 7 and Table 5. All mentioned figures and tables were updated.

High-Energy Particle Collision Data Analysis↗

A Multiscale Inelastic Internal State Variable Corrosion Model

We present a corrosion internal state variable (ISV) damage model based upon the integrated computational materials engineering (ICME) hierarchical multiscale paradigm. Structure–property experiments for magnesium alloys were used where the only inputs were the volume fractions of each element of the periodic table. This macroscale ISV corrosion model finds its basis in Horstemeyer’s mechanical damage model, which includes three separate ISVs for damage nucleation, growth, and coalescence, as well as Walton’s inclusion of corrosion, which introduces five new ISVs for pit nucleation, growth, and coalescence, along with general corrosion and intergranular corrosion. While Walton’s corrosion ISVs are phenomenological in nature, herein we develop a multiscale physical basis for the corrosion ISVs. The parameters for the macroscale corrosion ISVs were garnered from the mesoscale Butler–Volmer equations. Pure magnesium with differing amounts of aluminum were used in corrosion tests to exemplify the different pitting, general corrosion, and intergranular corrosion rates, and the macroscale ISV model was calibrated with said data, in which the only inputs to the model are the volume percentages of the elements magnesium and aluminum. Although magnesium alloys were used to motivate and calibrate the model, the model is abstract enough to possibly capture other material systems as well.

Chemistry↗