Cascade effects in certain atomic lifetime measurements
Hanle cascade effects on atomic lifetime reliability from collisional excitation experiments
SEARCH · Search NASA
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.
Hanle cascade effects on atomic lifetime reliability from collisional excitation experiments
Deactivation and radiative lifetime of CO Cameron forbidden transition spectral bands produced by photon absorption
Quantitative discussion of the photochemistry and lifetime against photodecomposition of five interstellar molecules: H2CO, NH3, H2O, CH4, and CO. For the first four molecules, primary photochemical decomposition processes yielding atomic and molecular hydrogen are considered in addition to photoionization. The quantum yield for decomposition of these molecules is unity. For CO, only decomposition to ground-state carbon and oxygen atoms occur, but the quantum yield is not known and may be considerably less than unity. The radiation field in obscuring clouds is estimated, using an interstellar extinction curve for the Perseus region.
Discussion of the factors affecting the intensity of forbidden transitions in diatomic molecules. It is shown that using Franck-Condon factors to predict relative band intensities is less reliable for forbidden transitions than it is for allowed transitions. The intensity of the 0,0 and 1,0 bands of the a super 3 pi-super 1 sigma Cameron system of CO are calculated using perturbation theory. The intensity arises from spin-orbit mixing of the A super 1 pi state with the a super 3 pi state. From the known spin-orbit coupling constant of the a super 1 pi state and the known intensity of the fourth positive A super 1 pi-super 1 sigma transition, the oscillator strengths of the 0,0 and 1,0 bands are calculated to be 1.63 x 10 to the minus 7th power and 1.99 x 10 to the minus 7th power. Lifetimes of various rotational levels are shown to range from 2.9 to several hundred milliseconds.-
Demonstration that rapid dissociative recombination of CO2(+) in a flowing, helium afterglow is an efficient source of CO in the a super 3 pi metastable state. Ions produced by mixing CO2 with He(2 super 3 S) recombine to produce a CO metastable afterglow with a number density as great as 10 to the 9th per sq cm. Monitoring of the (a super 3 pi-X super 1 sigma) Cameron transition in CO was used to study the lifetime and quenching of CO (a super 3 pi) by CO2, N2, NO, and He. Recombination of CO2(+) also produces CO in the d super 3 delta and a' super 3 sigma states.
It is shown that the production of small nitrogen to carbon ratios is possible, in contrast to the equilibrium production in the ordinary CN cycle. Associated with such a production are high ratios of C-13/C-12 and of N-15/N-14. The final ratios depend on the conditions under which cessation of hydrogen burning occurs under astrophysical circumstances. A table showing proton capture mean lifetimes of CN nuclei is provided together with tables of the equilibrium abundances in a fast CN cycle. The ratios of final abundances of nitrogen to carbon as functions of temperature are also presented.
The removal of radiation belt electrons through pitch-angle scattering by the observed obliquely propagating plasmaspheric whistler wave band is investigated. Electron lifetimes are calculated as a function of L and energy. The effects of high latitude interactions and of oblique wave propagation with the resulting diffusion at all cyclotron harmonics are quantitatively incorporated into the calculations. The inclusion of these effects appears to extend the role of whistler-driven electron pitch-angle diffusion to provide an explanation of the positioning of the quiet time radiation belt electron slot and the electron losses within the slot region.
The ice particles are formed when liquid and/or humid gases vent to the space. These submicroscopic ice particles are potential contamination sources of the environments during Skylab operations. The critical size of ice particle and its nucleation rate based on the theory of homogeneous and heterogeneous nucleation by sublimation are analyzed. The equations which are pertinent for studying the growth and evaporation of the ice particles are formulated. The mechanisms affecting the lifetime of ice particle are discussed. The gas dynamic techniques for experimental study of ice particle formation are proposed.
A time-of-flight method for measurement of the lifetime of metastable molecules is described. The method is applicable to a molecular beam that has molecules in several different metastable excited states. As compared to methods used previously, the method has the advantages that it does not require selective excitation or quenching of the different states; moreover, it does not require a determination of the relative populations or velocity distributions of molecules in the excited states.
By directly measuring the donor fluorescence lifetime as a function of acceptor concentration in the laser dye mixture Rhodamine 6G-Cresyl violet, we found that the Stern-Volmer relation is obeyed, from which the rate of excitation transfer is determined. The experimental results indicate that the dominant mechanism responsible for the efficient excitation transfer is that of resonance transfer due to long range dipole-dipole interaction.
We have observed a chromospheric brightening in the H alpha and Ca II K lines with a diameter of about 1 arc second. The time structure of this event, obtained with a relative resolution of 1 second, shows the rise time to be 4 seconds, the lifetime (FWHM) to be 20 seconds, and the decay time to be 5 seconds. This imposes new constraints on flare-point models. These restrictions can be accommodated easily by either an infall-impact flare model or a model invoking the precipitation of high-energy particles from the corona.
Centerline H alpha filtergrams providing nearly full-day coverage of the sun are used to study the lifetimes of enhanced network features near active regions. In the two cases studied the fraction remaining of those features present at an original epoch remains near unity for 50 hr, then drops exponentially with a 1/e decay time of 30 hr. Histories of representative enhanced network features are discussed.-
A photoexcitation technique is suggested which is direct and convenient, requiring little special equipment. No change in the dimensions of the crystal sample is necessary. Although related to the technique of interposing a filter between the light source and the sample, it differs in that the filter is part of the crystal itself. Basically, one of the electrodes is split into two electrodes, one collecting charge from carriers excited in the bulk. This phenomenon in which the carriers follow very closely the electric field lines has been used in position-sensitive semiconductor radiation detectors (Norbeck and Carlson, 1963) but has not been applied to lifetime measurements. In a sense, the split electrode creates a sample without a surface.
Measurements were taken to determine the effects that solar cell processing steps have on the minority carrier lifetime in silicon. The experimental work included measurements of diffusion lengths of the silicon at various stages of cell fabrication, of solar cell properties, and of the PN junction properties for ingots covering a wide range of doping and other ingot properties. Resistivities covered the range of 0.01 to 10 ohm-cm, and combinations of extreme concentrations (high and low) of dislocations and oxygen were included. The results showed that the major cell process steps did not usually cause any appreciable change in diffusion lengths. The solar cell currents obtained supported the diffusion length measurements. The effects of heavy doping concentrations on solar cell performance were studied. Attempts were made to relate the voltage behavior of the cells with the diode properties and the properties of the ingots.
A FORTRAN coded computer program which determines secular variations in mean orbital elements of earth satellites and the lifetime of the orbit is described. The dynamical model treats a point mass satellite subject to solar and lunar disturbing gravitational fields, second, third and fourth harmonics of the earth's oblate potential, earth's atmospheric drag, and solar radiation pressure. Each of these disturbing functions may be selectively simulated. Data preparation instructions, a sample problem, and definitions of output quantities are included.
The four Galilean satellites of Jupiter present a long-term collision hazard to an uncontrolled orbiting spacecraft that repeatedly enters the spatial region occupied by the satellites. Satellite close encounters and the likelihood of collision over a wide range of initial orbit conditions were analyzed. The effect of orbit inclination was of key interest. The scope of the analysis was restricted to orbital dynamic considerations alone, i.e. the question of biological contamination given the event of collision was not considered. A quarantine or orbiter lifetime of 50 years was assumed. This time period begins at spacecraft shutdown following completion of the mission objectives. A numerical approach was adopted wherein each initial orbit is propagated for 50 years, and satellite closest encounter distances recorded on every revolution. The computer program includes approximations of the three major perturbation effects on the long-term motion of the orbiter: (1) Jupiter oblateness, (2) solar gravity, and (3) satellite gravity.
The implications of recent determinations of the cosmic-ray lifetime are discussed. It is concluded that the observations are consistent with a 'dynamical halo' model in which cosmic rays are confined in an outward-moving galactic halo by self-generated hydromagnetic waves. Alternative models which do not incorporate a halo, but which have the cosmic rays propagate in regions of reduced density in the galactic disk, are also briefly discussed.
An experimental investigation of hollow cathodes for 30-cm Hg bombardment thrusters was carried out. Both main and neutralizer cathode configurations were tested with both rolled foil inserts coated with low work function material and impregnated porous tungsten inserts. Temperature measurements of an impregnated insert at various positions in the cathode were made. These, along with the cathode thermal profile are presented. A theory for rolled foil and impregnated insert operation and lifetime in hollow cathodes is developed. Several endurance tests, as long as 18000 hours at emission currents of up to 12 amps were attained with no degradation in performance.