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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS2000

Limits on Line Bisector Variability for Stars with Extrasolar Planets

We present an analysis of high-resolution synoptic spectra of ten F- and G-type stars, seven of which exhibit periodic radial velocity variations due to the presence of one or more substellar companions. We searched for subtle periodic variations in photospheric line asymmetry, as characterized by line bisectors. In principle, periodic variations in line asymmetry observed at lower spectral resolution could mimic the radial velocity signature of a companion, but we find no significant evidence of such behavior in our data. Observations were obtained from 1998 March to 1999 February using the National Solar Observatory (NSO) 1.52-m McMath-Pierce Solar Telescope Facility on Kitt Peak in conjunction with the solar-stellar spectrograph, achieving a resolving power of 1.2x10(exp5). To characterize line asymmetry, we first measured line bisectors for the unblended Fe I photospheric line at 625.26 nm. To improve sensitivity to small fluctuations, we then combined points in each bisector to form a velocity displacement with respect to the line core. We searched for periodic variations in this displacement, finding no substantial difference between stars with substellar companions and those without reported companions. We find no correlation between bisector velocity displacement and the known orbital phase of substellar companions around our target stars. Simulations of a periodic signal with noise levels that mimic our measurement errors suggest that we can exclude bisector variations with amplitudes greater than about 20 m/s. These results support the conclusion that extrasolar planets best explain the observed periodic variations in radial velocity.

Povich, M. S.↗
NASA NTRS2000

Validation of MODIS Aerosol Retrievals during PRIDE

The Puerto Rico Dust Experiment (PRIDE) was held in Roosevelt Roads, Puerto Rico from June 26 to July 24, 2000. It was intended to study the radiative and microphysical properties of Saharan dust transported into Puerto Rico. PRIDE had the unique distinction of being the first major field experiment to allow direct comparison of aerosol retrievals from MODIS (MODerate Imaging Spectro-radiometer - aboard the Terra satellite) with data from a variety of ground, shipboard and air-based instruments. Over the ocean the MODIS algorithm retrieves optical depth as well as information about the aerosol's size. During PRIDE, MODIS passed over Roosevelt Roads approximately once per day during daylight hours. Due to sunglint and clouds over Puerto Rico, aerosol retrievals can be made from only about half the MODIS scenes. In this study we try to "validate" our aerosol retrievals by comparing to measurements taken by sun-photometers from multiple platforms, including: Cimel (AERONET) from the ground, Microtops (handheld) from ground and ship, and the NASA-Ames sunphotometer from the air.

Levy, R.↗
NASA NTRS2000

Comparison of Aerosol Single Scattering Albedos Derived By Diverse Techniques in Two North Atlantic Experiments

Aerosol single scattering albedo w (the ratio of scattering to extinction) is important in determining aerosol climatic effects, in explaining relationships between calculated and measured radiative fluxes, and in retrieving aerosol optical depths from satellite radiances. Recently, two experiments in the North Atlantic region, TARFOX and ACE-2, determined aerosol w by a variety of techniques. The techniques included fitting of calculated to measured fluxes; retrievals of w from skylight radiances; best fits of complex refractive index to profiles of backscatter, extinction, and size distribution; and in situ measurements of scattering and absorption at the surface and aloft. Both TARFOX and ACE-2 found a fairly wide range of values for w at midvisible wavelengths, with 0.85 less than wmidvis less than 0.99 for the marine aerosol impacted by continental pollution. Frequency distributions of w could usually be approximated by lognormals in wmax-w, with some occurrence of bimodality, suggesting the influence of different aerosol sources or processing. In both TARFOX and ACE-2, closure tests between measured and calculated radiative fluxes yielded best-fit values of wmidvis of 0.90+/-0.04 for the polluted boundary layer. Although these results have the virtue of describing the column aerosol unperturbed by sampling, they are subject to questions about representativeness and possible artifacts (e.g., unknown gas absorption). The other techniques gave larger values for wmidvis for the polluted boundary layer, with a typical result of wmidvis = 0.95+/-0.04, Current uncertainties in vv are large in terms of climate effects. More tests are needed of the consistency among different methods and of humidification effects on w.

Russell, P. B.↗
NASA NTRS1994

Global- to Micro-Scale Evolution of the Pinatubo Aerosol: Using Composite Data Sets to Build the Picture and Assess Consistency of Different Measurements

This paper brings together experimental. evidence required to build realistic models of the global evolution of physical, chemical, and optical properties of the aerosol resulting from the 1991 Pinatubo volcanic eruption. Such models are needed to compute the effects of the aerosol on atmospheric chemistry, dynamics, radiation, and temperature. Whereas there is now a large and growing body of post-Pinatubo measurements by a variety of techniques, some results are in conflict, and a self-consistent, unified picture is needed, along with an assessment of remaining uncertainties. This paper examines data from photometers, radiometers, impactors, optical counters/sizers, and lidars operated on the ground, aircraft, balloons, and spacecraft.

Russell, P. B.↗
NASA NTRS2001

Airborne Sun photometry and Closure Studies in SAFARI-2000 Dry Season Campaign

From August 13 to September 25, the Southern African Regional Science Initiative's (SAFARI 2000) dry-season airborne campaign studied the complex interactions between the region's ecosystems, air pollution, atmospheric circulation, land-atmosphere interactions, and land use change. The field campaign was timed to coincide with the annual winter fire season in Southern Africa. This challenging campaign. which coordinated ground-based measurement teams, multiple research aircraft, and satellite overpasses across nine African nations, was head quartered at the Petersburg International Airport in South Africa's Northern Province. Among many others, unique coordinated observations were made of the evolution of massive, thick haze layers produced by industrial emissions, biomass burning, marine and biogenic sources. The NASA Ames Airborne Tracking 14-channel Sunphotometer (AATS-14) was operated successfully aboard the University of Washington CV-580 during 24 data flights. The AATS-14 instrument measures the transmission of the direct solar beam at 14 discrete wavelengths (3501558 nm) from which we derive spectral aerosol optical depths (AOD), columnar water vapor (CWV) and columnar ozone. Flying at different altitudes over a fixed location allows derivation of layer AOD and CWV. Data taken during feasible vertical profiles allows derivation of aerosol extinction and water vapor density. In the talk, we show comparisons with ground-based AERONET sun/sky photometer results, with ground based MPL-Net lidar data, and with measurements from a lidar aboard the high flying ER-2 aircraft. We will use measurements from the Ames Solar Spectral Flux Radiometer to derive estimates of solar spectral forcing as a function of aerosol thickness. Validations of TOMS and Terra satellite aerosol and water-vapor retrievals will also be discussed.

Schmid, B.↗
NASA NTRS2000

Comparison of Columnar Water Vapor Measurements During The Fall 1997 ARM Intensive Observation Period: Solar Transmittance Methods

In the fall of 1997, during an Intensive Observation Period (IOP), the Atmospheric Radiation Measurement (ARM) program conducted a study of water vapor abundance measurement at its Southern Great Plains (SGP) site. Among a large number of instruments, four sun-tracking radiometers were present to measure the columnar water vapor (CWV). All four solar radiometers retrieve CWV by measuring total solar transmittance in the 0.94-gm water vapor absorption band and subtracting contributions due to Rayleigh, ozone and aerosol transmittances. The aerosol optical depth comparisons among the same four radiometers has been presented elsewhere (Geophys. Res. Lett., 26, 17, 2725-2728, 1999). We have used three different methods to retrieve CWV. In a first round of comparison no attempt was made to standardize on the same radiative transfer model and its underlying water vapor spectroscopy. In the second round of comparison we used the same line-by-line code (which includes recently corrected H2O spectroscopy) to retrieve CAN from all four suntracking radiometers. This decreased the mean CWV by 8% or 13%. The spread of 8% in the solar radiometer results found when using the same model is an indication of the other-than-model uncertainties involved in determining CWV from solar transmittance measurements with current instrumentation.

Schmid, B.↗
NASA NTRS2000

Desert Dust Layers Over Polluted Marine Boundary Layers: ACE-2 Measurements and ACE-Asia Plans

Aerosols in ACE-Asia are expected to have some commonalties with those in ACE-2, along with important differences. Among the commonalities are occurrences of desert dust layers over polluted marine boundary layers. Differences include the nature of the dust (yellowish in the East Asia desert outflow, vs. reddish-brown in the Sahara Outflow measured in ACE-2) and the composition of boundary-layer aerosols (e.g., more absorbing, soot and organic aerosol in-the Asian plume, caused by coal and biomass burning, with limited controls). In this paper we present ACE-2 measurements and analyses as a guide to our plans for ACE-2 Asia. The measurements include: (1) Vertical profiles of aerosol optical depth and extinction (380-1558 nm), and of water vapor column and concentration, from the surface through the elevated desert dust, measured by the 14-channel Ames Airborne Tracking Sunphotometer (AATS-14); (2) Comparisons of airborne and shipborne sunphotometer optical depths to satellite-retrieved values, with and without desert dust; (3) Comparisons between airborne Sunphotometer optical depth and extinction spectra and those derived from coincident airborne in situ measurements of aerosol size distribution, scattering and absorption; (4) Comparisons between size distributions measured in situ and retrieved from sunphotometer optical depth spectra; (5) Comparisons between aerosol single scattering albedo values obtained by several techniques, using various combinations of measurements of backscatter, extinction, size distribution, scattering, absorption, and radiative flux. We show how analyses of these data can be used to address questions important to ACE-Asia, such as: (1) How do dust and other absorbing aerosols affect the accuracy of satellite optical depth retrievals? How important are asphericity effects? (2) How important are supermicron dust and seasalt aerosols to overall aerosol optical depth and radiative forcing? How well are these aerosols sampled by aircraft inlets and instruments? (3) How consistent are suborbital in situ and remote measurements of aerosols, among themselves and with satellite retrievals? What are the main reasons for observed inconsistencies?

Russell, Philip B.↗
NASA NTRS2001

Shortwave Radiative Fluxes, Solar-Beam Transmissions, and Aerosol Properties: TARFOX and ACE-2 Find More Absorption from Flux Radiometry than from Other Measurements

The Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX) and the Second Aerosol Characterization Experiment (ACE-2) made simultaneous measurements of shortwave radiative fluxes, solar-beam transmissions, and the aerosols affecting those fluxes and transmissions. Besides the measured fluxes and transmissions, other obtained properties include aerosol scattering and absorption measured in situ at the surface and aloft; aerosol single scattering albedo retrieved from skylight radiances; and aerosol complex refractive index derived by combining profiles of backscatter, extinction, and size distribution. These measurements of North Atlantic boundary layer aerosols impacted by anthropogenic pollution revealed the following characteristic results: (1) Better agreement among different types of remote measurements of aerosols (e.g., optical depth, extinction, and backscattering from sunphotometers, satellites, and lidars) than between remote and in situ measurements; 2) More extinction derived from transmission measurements than from in situ measurements; (3) Larger aerosol absorption inferred from flux radiometry than from other measurements. When the measured relationships between downwelling flux and optical depth (or beam transmission) are used to derive best-fit single scattering albedos for the polluted boundary layer aerosol, both TARFOX and ACE-2 yield midvisible values of 0.90 +/- 0.04. The other techniques give larger single scattering albedos (i.e. less absorption) for the polluted boundary layer, with a typical result of 0.95 +/- 0.04. Although the flux-based results have the virtue of describing the column aerosol unperturbed by sampling, they are subject to questions about representativeness and other uncertainties (e.g., unknown gas absorption). Current uncertainties in aerosol single scattering albedo are large in terms of climate effects. They also have an important influence on aerosol optical depths retrieved from satellite radiances. More tests are needed of the consistency among different methods and of the effects of changing humidity on aerosol.

Russell, Philip B.↗
NASA NTRS2000

Airborne Sunphotometry of African Dust and Marine Boundary Layer Aerosols in PRIDE

The Puerto Rico Dust Experiment (PRIDE) was conducted during summer 2000 to study the radiative, microphysical and transport properties of Saharan dust in the Caribbean region. During PRIDE, NASA Ames Research Center's six-channel airborne autotracking sunphotometer (AATS-6) was operated aboard a Piper Navajo airplane based at Roosevelt Roads Naval Station on the northeast coast of Puerto Rico. AATS-6 measurements were taken during 21 science flights off the coast of Puerto Rico in the western Caribbean. Data were acquired within and above the Marine Boundary Layer (MBL) and the Saharan Aerosol Layer (SAL) up to 5.5 km altitude tinder a wide range of dust loadings. Aerosol optical depth (AOD) spectra and columnar water vapor (CWV) values have been calculated from the AATS-6 measurements by using sunphotometer calibration data obtained at Mauna Loa Observatory (3A kin ASL) before (May) and after (October) PRIDE. Mid-visible AOD values measured near the surface during PRIDE ranged from 0.07 on the cleanest day to 0.55 on the most turbid day. Values measured above the MBL were as high as 0.35; values above the SAL were as low as 0.01. The fraction of total column AOD due to Saharan dust cannot be determined precisely from AATS-6 AOD data alone due to the uncertainty in the extent of vertical mixing of the dust down through the MBL. However, analyses of ground-based and airborne in-situ aerosol sampling measurements and ground-based aerosol lidar backscatter data should yield accurate characterization of the vertical mixing that will enable calculation of the Saharan dust AOD component from the sunphotometer data. Examples will be presented showing measured AATS-6 AOD spectra, calculated aerosol extinction and water vapor density vertical profiles, and aerosol size distributions retrieved by inversion of the AOD spectra. Near sea-surface AOD spectra acquired by AATS-6 during horizontal flight legs at 30 m ASL are available for validation of AOD derived from coincident satellite sensor (TOMS, MODIS, MISR) measurements. AATS-6 AOD data acquired during numerous aircraft ascents and descents through the MBL and the SAL should permit atmospheric column closure analyses with respect to aerosol optical depth, extinction, and size distribution by comparison with coincident aircraft-based in-situ particle size distribution measurements and ground-based (Cabras Island, Puerto Rico) micropulse lidar aerosol backscatter measurements. The aerosol information derived from the column closure analyses can be used subsequently to calculate radiative flux changes, which can then be compared with coincident spectral flux measurements taken from aboard the aircraft with a solar spectral flux radiometer.

Livingston, John M.↗
NASA NTRS2000

Airborne Aerosol Closure Studies During PRIDE

The Puerto Rico Dust Experiment (PRIDE) was conducted during June/July of 2000 to study the properties of Saharan dust aerosols transported across the Atlantic Ocean to the Caribbean Islands. During PRIDE, the NASA Ames Research Center six-channel (380 - 1020 nm) airborne autotracking sunphotometer (AATS-6) was operated aboard a Piper Navajo airplane alongside a suite of in situ aerosol instruments. The in situ aerosol instrumentation relevant to this paper included a Forward Scattering Spectrometer Probe (FSSP-100) and a Passive Cavity Aerosol Spectrometer Probe (PCASP), covering the radius range of approx. 0.05 to 10 microns. The simultaneous and collocated measurement of multi-spectral aerosol optical depth and in situ particle size distribution data permits a variety of closure studies. For example, vertical profiles of aerosol optical depth obtained during local aircraft ascents and descents can be differentiated with respect to altitude and compared to extinction profiles calculated using the in situ particle size distribution data (and reasonable estimates of the aerosol index of refraction). Additionally, aerosol extinction (optical depth) spectra can be inverted to retrieve estimates of the particle size distributions, which can be compared directly to the in situ size distributions. In this paper we will report on such closure studies using data from a select number of vertical profiles at Cabras Island, Puerto Rico, including measurements in distinct Saharan Dust Layers. Preliminary results show good agreement to within 30% between mid-visible aerosol extinction derived from the AATS-6 optical depth profiles and extinction profiles forward calculated using 60s-average in situ particle size distributions and standard Saharan dust aerosol refractive indices published in the literature. In agreement with tendencies observed in previous studies, our initial results show an underestimate of aerosol extinction calculated based on the in situ size distributions relative to the extinction obtained from the sunphotometer measurements. However, a more extensive analysis of all available AATS-6 and in situ size distribution data is necessary to ascertain whether the preliminary results regarding the degree of extinction closure is representative of the entire range of dust conditions encountered in PRIDE. Finally, we will compare the spectral extinction measurements obtained in PRIDE to similar data obtained in Saharan dust layers encountered above the Canary Islands during ACE-2 (Aerosol Characterization Experiment) in July 1997. Thus, the evolution of Saharan dust spectral properties during its transport across the Atlantic can be investigated, provided the dust origin and microphysical properties are found to be comparable.

Redemann, Jens↗
NASA NTRS2001

Airborne Sunphotometer Studies of Aerosol Properties and Effects, Including Closure Among Satellite, Suborbital Remote, and In situ Measurements

Airborne sunphotometry has been used to measure aerosols from North America, Europe, and Africa in coordination with satellite and in situ measurements in TARFOX (1996), ACE-2 (1997), PRIDE (2000), and SAFARI 2000. Similar coordinated measurements of Asian aerosols are being conducted this spring in ACE-Asia and are planned for North American aerosols this summer in CLAMS. This paper summarizes the approaches used, key results, and implications for aerosol properties and effects, such as single scattering albedo and regional radiative forcing. The approaches exploit the three-dimensional mobility of airborne sunphotometry to access satellite scenes over diverse surfaces (including open ocean with and without sunglint) and to match exactly the atmospheric layers sampled by airborne in situ measurements and other radiometers. These measurements permit tests of the consistency, or closure, among such diverse measurements as aerosol size-resolved chemical composition; number or mass concentration; light extinction, absorption, and scattering (total, hemispheric back and 180 deg.); and radiative fluxes. In this way the airborne sunphotometer measurements provide a key link between satellite and in situ measurements that helps to understand any discrepancies that are found. These comparisons have led to several characteristic results. Typically these include: (1) Better agreement among different types of remote measurements than between remote and in situ measurements. (2) More extinction derived from transmission measurements than from in situ measurements. (3) Larger aerosol absorption inferred from flux radiometry than from in situ measurements. Aerosol intensive properties derived from these closure studies have been combined with satellite-retrieved fields of optical depth to produce fields of regional radiative forcing. We show results for the North Atlantic derived from AVHRR optical depths and aerosol intensive properties from TARFOX and ACE-2. Companion papers show analogous, preliminary results for Asian-Pacific aerosols and results of SAFARI-2000 closure studies on African aerosols.

Russlee, Philip B.↗
NASA NTRS2000

Solar Spectral Radiative Forcing Due to Dust Aerosol During the Puerto Rico Dust Experiment

During the Puerto Rico Dust Experiment (PRIDE) upwelling and downwelling solar spectral irradiance was measured on board the SPAWAR Navajo and downwelling solar spectral flux was measured at a surface site using the NASA Ames Solar Spectral Flux Radiometer. These data will be used to determine the net solar radiative forcing of dust aerosol and to quantify the solar spectral radiative energy budget in the presence of elevated aerosol loading. We will assess the variability in spectral irradiance using formal principal component analysis procedures and relate the radiative variability to aerosol microphysical properties. Finally, we will characterize the sea surface reflectance to improve aerosol optical depth retrievals from the AVHRR satellite and to validate SeaWiFS ocean color products.

Pilewskie, P.↗
NASA NTRS2001

Sunphotometric Measurement of Columnar H2O and Aerosol Optical Depth During the 3rd Water Vapor IOP in Fall 2000 at the SGP ARM Site

We conducted ground-based measurements with the Ames Airborne Tracking 6-channel Sunphotometer (AATS-6) during the 3rd Water Vapor IOP (WVIOP3), September 18 - October 8, 2000 at the SGP ARM site. For this deployment our primary result was columnar water vapor (CWV) obtained from continuous solar transmittance measurements in the 0.94-micron band. In addition, we simultaneously measured aerosol optical depth (AOD) at 380, 450, 525, 864 and 1020 nm. During the IOP, preliminary results of CWV and AOD were displayed in real-time. The result files were made available to other investigators by noon of the next day. During WVIOP3 those data were shown on the daily intercomparison plots on the IOP web-site. Our preliminary results for CWV fell within the spread of values obtained from other techniques. After conclusion of WVIOP3, AATS-6 was shipped directly to Mauna Loa, Hawaii for post-mission calibration. The updated calibration, a cloud screening technique for AOD, along with other mostly cosmetic changes were applied to the WVIOP3 data set and released as version 0.1. The resulting changes in CWV are small, the changes in AOD and Angstrom parameter are more noticeable. Data version 0.1 was successfully submitted to the ARM External Data Center. In the poster we will show data examples for both CWV and AOD. We will also compare our CWV results with those obtained from a GPS (Global Positioning System) slant path method.

Schmid, B↗
NASA NTRS1994

Cloud-Aerosol Interactions in Tropical Storms

During the Coupled Ocean-Atmosphere Response Experiment (COARE) of the Tropical Ocean and the Global Atmosphere (TOGA) program we measured cloud and aerosol particles aboard the NASA DC-8 over the warm pool of the western Pacific. Instruments on the aircraft included a condensation nuclei counter, optical particle counters, two-dimensional shadow probes and an ice crystal replicator. The size range covered by these instruments was from =0.01 micron to 6.4 mm diameter; particle shapes were determined for particles of sizes D greater than 1 micron.

Puesschel, R. F.↗
NASA NTRS1994

Pinatubo Aerosol Evolution: Using Composite Data Sets to Build the Global- To Micro-Scale Picture and Assess Consistency of Different Measurements

This paper brings together experimental evidence required to build realistic models of the global evolution of physical, chemical, and optical properties of the aerosol resulting from the 1991 Pinatubo volcanic eruption. Such models are needed to compute the effects of the aerosol on atmospheric chemistry, dynamics, radiation, and temperature. Whereas there is now a large and crowing body of post-Pinatubo measurements by a variety of techniques, some results are in conflict, and a self-consistent, unified picture is needed, along with an assessment of remaining uncertainties. This paper examines, data from photometers, radiometers, impactors, optical counter/sizers, and lidars operated on the ground, aircraft, balloons, and spacecraft. Example data sources include: (1) Tracking sunphotometers and lidars at Mauna Loa Observatory (MLO) and on the DC-8. (2) Particle spectrometers and wire impactors on the ER-2 and DC-8. (3) Dustsondes (particle counter/sizers on balloons). and (3) SAGE II, SAM II, AVHRR, CLAES, and ISAMS sensors on a variety of satellites. We assess the mutual consistency of these disparate data sets and recommend 'consensus' properties and uncertainties in the process of developing a composite data set. Recommended properties include the spatial and temporal evolution of particle chemical composition, shape, wavelength-and temperature-dependent refractive index, size distribution, and optical depth spectra. Supporting references are cited and representative data shown.

Russell, Philip B.↗
NASA NTRS1994

Aerosol Optical Depth Determinations for BOREAS

Automated tracking sun photometers were deployed by NASA/Ames Research Center aboard the NASA C-130 aircraft and at a ground site for all three Intensive Field Campaigns (IFCs) of the Boreal Ecosystem-Atmosphere Study (BOREAS) in central Saskatchewan, Canada during the summer of 1994. The sun photometer data were used to derive aerosol optical depths for the total atmospheric column above each instrument. The airborne tracking sun photometer obtained data in both the southern and northern study areas at the surface prior to takeoff, along low altitude runs near the ground tracking sun photometer, during ascents to 6-8 km msl, along remote sensing flightlines at altitude, during descents to the surface, and at the surface after landing. The ground sun photometer obtained data from the shore of Candle Lake in the southern area for all cloud-free times. During the first IFC in May-June ascents and descents of the airborne tracking sun photometer indicated the aerosol optical depths decreased steadily from the surface to 3.5 kni where they leveled out at approximately 0.05 (at 525 nm), well below levels caused by the eruption of Mt. Pinatubo. On a very clear day, May 31st, surface optical depths measured by either the airborne or ground sun photometers approached those levels (0.06-0.08 at 525 nm), but surface optical depths were often several times higher. On June 4th they increased from 0.12 in the morning to 0.20 in the afternoon with some evidence of brief episodes of pollen bursts. During the second IFC surface aerosol optical depths were variable in the extreme due to smoke from western forest fires. On July 20th the aerosol optical depth at 525 nm decreased from 0.5 in the morning to 0.2 in the afternoon; they decreased still further the next day to 0.05 and remained consistently low throughout the day to provide excellent conditions for several remote sensing missions flown that day. Smoke was heavy for the early morning of July 24th but cleared partially by 10:30 local time and cleared fully by 11:30. Heavy smoke characterized the rest of the IFC in both study areas.

Wrigley, R. C.↗
NASA NTRS1994

Pinatubo Aerosol Evolution: Using Composite Data Sets to Build the Global- to Micro-Scale Picture and Assess Consistency of Different Measurements

This paper brings together experimental evidence required to build realistic models of the global evolution of physical, chemical, and optical properties of the aerosol resulting from the 1991 Pinatubo volcanic eruption. Such models are needed to compute the effects of the aerosol on atmospheric chemistry, dynamics, radiation, and temperature. Whereas there is now a large and growing body of post-Pinatubo measurements by a variety of techniques, some results are in conflict, and a self-consistent, unified picture is needed, along with an assessment of remaining uncertainties. This paper examines data from photometers, radiometers, impactors, optical counters/sizers, and lidars operated on the ground, aircraft, balloons, and spacecraft. Example data sources include: - Tracking sunphotometers and lidars at Mauna Loa Observatory (MLO) and on the DC-8 - Particle spectrometers and wire impactors on the ER-2 and DC-8 - Dustsondes (particle counters/sizers on balloons) - SAGE II, SAM II, AVHRR, CLAES, and ISAMS sensors on a variety of satellites. We assess the mutual consistency of these disparate data sets and recommend 'consensus" properties and uncertainties in the process of developing a composite data set. Recommended properties include the spatial and temporal evolution of particle chemical composition, shape, wavelength and temperature-dependent refractive index, size distribution, and optical depth spectra. Supporting references are cited and representative data shown.

Russell, P. B.↗
NASA NTRS2001

Transport of Aerosols from Asia and Their Radiative Effects Over the Western Pacific: A 3-D Model Study for ACE-Asia Experiment During Spring 2001

The Aerosol Characterization Experiment-Asia (ACE-Asia) took place in Spring 2001 in the East Asia-West Pacific Ocean. During the ACE-Asia intensive field operation period, high concentrations of dust and anthropogenic aerosols were observed over the Yellow Sea and the Sea of Japan, which were transported out from the Asian continent, with the plume often extending to 6-8 km altitude. The multi-component aerosols originated from Asia are expected to exert a significant radiative forcing over the Pacific region. We present here results from the Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model of aerosol transport and radiative forcing in the context of ACE-Asia. The model calculated aerosol concentrations, extinctions, optical thickness, size distributions, and vertical profiles are compared with the aircraft and ship measurements, and the distributions of aerosols are compared with satellite data. The model will be used to understand the origins of the aerosols observed in ACE-Asia, estimate the contributions from anthropogenic and natural aerosols to the total aerosol optical thickness, investigate the effects of humidification and clouds on aerosol properties, and assess the radiative forcing of Asian aerosols over the Pacific region and in the northern hemisphere.

Chin, Mian↗