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At least 307 records · Page 17

Evaluation of Getters for Helium Purification

• Helium-3 is a vital commodity in both medical and defense applications • Ultra-low cryogenic coolant (MRI imaging, etc.) • Neutron detectors • Being investigated as possible fusion fuel • Managed and distributed by DOE-OS • New PDRD project exploring helium isotope separation • Limited supply • Only available from tritium decay • Prohibitively difficult to separate from helium-4 • SRS Tritium Facility provides a steady source

Angelette, Lucas M.↗

Impact of Time Dependent Reactor and Sensor Physics on Core Power Synthesis

Online synthesis of the power distribution is critical in the operation and control of nuclear power reactors to ensure that the core is operating within safety margins, and to provide essential knowledge associated with the burnup of the fuel. In light water reactors (LWRs), power synthesis is achieved by using some a priori knowledge of the state of the reactor core and updating based on the signals coming from in-core sensors—namely, self-powered neutron detectors (SPNDs). This report aims to study the effects of fuel burnup and sensor degradation on the ability to accurately synthesize the power distribution in a LWR. Several modeling tools were used to simulate power synthesis based on the responses of SPNDs, with emitters made out of Rh or V. A representative pressurized water reactor low-enriched uranium (LEU) core was modeled using the Polaris/Purdue Advanced Reactor Core Simulator (PARCS) approach. The Monte Carlo N-Particle Transport 6 (MCNP6) code was used, as well, to calculate response functions between different segments of fuel to individual SPNDs; this is a crucial parameter for power synthesis. The Oak Ridge Isotope GENeration (ORIGEN) package in the Standardized Computer Analyses for Licensing Evaluation (SCALE) code was used to model the time-dependent isotopic transmutation in the SPND emitters. All these data were fed into a custom code that enacted the point-based iterative (PBI) method to simulate power synthesis. Developmental work was also performed on high-fidelity SPND models in the GEometry ANd Tracking 4 (Geant4) code, which enables higher-accuracy modeling of the current responses from SPNDs. In this work, five sets of time-dependent power synthesis test cases were conducted. In these test cases, systematic changes in the input conditions enabled an analysis of the effect of (1) slightly inaccurate a priori power distribution assumptions with respect to fuel burnup, (2) highly inaccurate a priori assumptions with respect to fuel burnup (such that burnup is not included in the a priori assumed distribution), and (3) differences between Rh and V SPNDs in terms of downstream consequences of the transmutation in the emitters. The authors discovered that one may permissibly have slightly inaccurate a priori assumptions of the fuel burnup (such that the level of burnup may be slightly under- or over-approximated by the accumulated burnup in approximately 9.3 full power days), but to not account for burnup at all in the a priori assumption leads to severe levels of error, approaching 25% at maximum. The authors also discovered that V SPNDs are extraordinarily robust in the low-enriched uranium fuel cycle considered in this modeling work, whereas Rh SPNDs undergo significant transmutation that can result in large errors in the synthesized power distribution.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Expansion of the Fuel Motion Monitoring System

The Idaho National Laboratory (INL) Transient Reactor Test Facility (TREAT) Fuel Motion Monitoring System (FMMS) is a diagnostic tool used to visualize the movement and location of fuel within the nuclear reactor during transient experiments. TREAT is designed to test the behavior of nuclear fuel under accident conditions, such as a rapid power increase. The TREAT FMMS, also referred to as the “hodoscope” because of the system’s massive steel collimator component, is located on the North beam port of the reactor. While the FMMS system is capable of incorporating a total of 360 sensors, initial refurbishment efforts resulted in a array of 96 fast neutron detectors. This initial array was configured to provide a narrow (2 channels) full-length view of experiment vessels with an extended 4-channel–wide region in the center of the array capable of providing a full view of all initially planned experiments. Planning and efforts to expand the FMMS array began immediately following the restart of TREAT. An additional 96 detectors were evaluated, characterized, and prepared for installation at TREAT during the summer of 2018. Unfortunately, funding reductions forced the project towards a 5-year hiatus. In October of 2023 funding from the Department of Energy’s Nuclear Science User Facilities enabled the expansion to recommence. This report serves to document the activities performed to expand the FMMS detector array to 192 channels in order to provide a broader view of the larger and more sophisticated test capsules currently planned for future irradiation in the TREAT reactor. This expansion also included doubling the data acquisition capability, addressing the new heat load on the system, and synchronizing the time for all digital components.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Impact of Time-Dependent Reactor and Sensor Physics on Core Power Synthesis (Rev.1)

Online synthesis of power distribution is critical in the operation and control of nuclear power reactors to ensure that the core is operating within safety margins and to provide essential knowledge associated with the burnup of the fuel. In light-water reactors, power synthesis is achieved by using some a priori knowledge of the state of the reactor core and updating based on the signals coming from in-core sensors—namely, self-powered neutron detectors (SPNDs). This report examines the effects of fuel burnup and sensor degradation on the ability to accurately synthesize the power distribution in a pressurized water reactor (PWR), considering the typical low-enriched uranium (LEU, 3%-5% enrichment) fuel cycle as well as the higher enrichment LEU+ (5%-8% enrichment) fuel cycle. Several modeling tools were used to simulate power synthesis based on the responses of SPNDs, with emitters made out of Rh or V. A representative PWR LEU core was modeled using the Polaris/Purdue Advanced Reactor Core Simulator (PARCS) approach. The Monte Carlo N-Particle Transport 6 (MCNP6) code was used as well to calculate response functions between different segments of fuel to individual SPNDs; this is a crucial parameter for power synthesis. The Oak Ridge Isotope GENeration (ORIGEN) package in the Standardized Computer Analyses for Licensing Evaluation (SCALE) code was used to model the time-dependent isotopic transmutation in the SPND emitters. All these data were fed into a custom code that enacted the point-based iterative method to simulate power synthesis. Developmental work was also performed on high-fidelity SPND models in the GEometry ANd Tracking 4 (Geant4) code, which enables higher-accuracy modeling of the current responses from SPNDs. In this work, five sets of time-dependent power synthesis test cases were conducted. In these test cases, systematic changes in the input conditions enabled an analysis of the effect of (1) slightly inaccurate a priori power distribution assumptions with respect to fuel burnup, (2) highly inaccurate a priori power distribution assumptions with respect to fuel burnup (such that burnup is not included in the a priori assumed distribution), and (3) differences between Rh and V SPNDs in terms of downstream consequences of the transmutation in the emitters and the extended nature of the LEU+ fuel cycle in comparison with LEU. The authors discovered that one may permissibly have slightly inaccurate a priori assumptions of the fuel burnup (such that the level of burnup may be slightly underapproximated or overapproximated by the accumulated burnup in approximately 9.3 full power days), but to not account for burnup at all in the a priori assumptions leads to severe levels of error, approaching 25% at maximum (for LEU). The authors also discovered that V SPNDs are extraordinarily robust in both the LEU and LEU+ fuel cycles considered in this modeling work, whereas Rh SPNDs undergo significant transmutation that can result in large errors in the synthesized power distribution.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Luminescence properties of europium doped and sodium co-doped LiCaAlF 6

This paper serves as a literature review of scintillating thermal neutron detectors, along with a study of sodium and europium doped LiCaAlF 6 (LiCAF) polycrystalline material. A set of polycrystalline LiCAF material was synthesized with 2 molar percent of europium (Eu 2+ ) and co-doped with 0, 1, and 2 molar percent of sodium (Na + ), with a stoichiometric synthesis approach in a glassy-carbon crucible. The quantum yield and photoluminescence spectrum at room temperature was analyzed. For the first time, we have demonstrated that Na-co-doping directly alters the quantum yield. The quantum yield for LiCAF:Eu 2+ , with 0, 1, and 2 molar percent of sodium (Na + ) was 0.578, 0.635, and 0.580, respectively. The photoluminescence (PL) spectrum was also analyzed for all samples. The photo-luminescence excitation (PLE) spectrum showed a maximum at 300 nm, while the emission spectrum showed a maximum at 370 nm, corresponding to the Eu 2+ 5d-4f transitions.

36 MATERIALS SCIENCE↗

HighNESS conceptual design report: Volume II. The NNBAR experiment.

A key aim of the HighNESS project for the European Spallation Source is to enable cutting-edge particle physics experiments. This volume presents a conceptual design report for the NNBAR experiment. NNBAR would exploit a new cold lower moderator to make the first search in over thirty years for free neutrons converting to anti-neutrons. The observation of such a baryon-number-violating signature would be of fundamental significance and tackle open questions in modern physics, including the origin of the matter-antimatter asymmetry. This report shows the design of the beamline, supermirror focusing system, magnetic and radiation shielding, and anti-neutron detector necessary for the experiment. A range of simulation programs are employed to quantify the performance of the experiment and show how background can be suppressed. For a search with full background suppression, a sensitivity improvement of three orders of magnitude is expected, as compared with the previous search. Civil engineering studies for the NNBAR beamline are also shown, as is a costing model for the experiment.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Detection of entrapped moisture in honeycomb sandwich structures

Thermal neutron moisture detection system detects entrapped moisture in intercellular areas of bonded honeycomb sandwich structures. A radium/beryllium fast neutron source bombards a specimen. The emitted thermal neutrons from the target nucleus are detected and counted by a boron trifluoride thermal neutron detector.

Hallmark, W. B.↗

Noncontacting device to indicate deflection of turbopump internal rotating parts

Phase 2 (development) which was concluded for the ultrasonic Doppler device and the light-pipe-reflectance device is reported. An ultrasonic Doppler breadboard system was assembled which accurately measured runout in the J-2 LOX pump impeller during operation. The transducer was mounted on the outside of the pump volute using a C-clamp. Vibration was measured by conducting the ultrasonic wave through the volute housing and through the fluid in the volute to the impeller surface. The impeller vibration was also measured accurately using the light-pipe probe mounted in an elastomeric-gland fitting in the pump case. A special epoxy resin developed for cryogenic applications was forced into the end of the fiber-optic probe to retain the fibers. Subsequently, the probe suffered no damage after simultaneous exposure to 2150 psi and 77 F. Preliminary flash X-radiographs were taken of the turbine wheel and the shaft-bearing-seal assembly, using a 2-megavolt X-ray unit. Reasonable resolution and contrast was obtained. A fast-neutron detector was fabricated and sensitivity was measured. The results demonstrated that the technique is feasible for integrated-time measurements requiring, perhaps, 240 revolutions to obtain sufficient exposure at 35,000 rpm. The experimental verification plans are included.

Hamilton, D. B.↗

Correlation of irradiation data using activation fluences and irradiation temperature.

Nil-ductility transition temperature data for A302-B ferritic steel were analyzed by using multiple regression. Four independent variables were used - i.e., specimen temperature during irradiation, and time-integrated specific activations (activation fluences) of fast-, intermediate-, and thermal-neutron detectors. The results of these analyses were predictive equations having the increase in transition temperature as the dependent variable. For a reference point, a similar analysis was also performed using the flux integral above 1 MeV and the irradiation temperature as independent variables. Also, the effect of excluding irradiation temperature from these analyses was studied. The results of the analyses showed that excellent correlation was achieved by using activation fluences and irradiation temperature as the independent variables. Irradiation temperature was found to account for from 29 to 46% of the data variability depending on the model used.

Lynch, J. H.↗

Water detection at the moon, Mars and comets with a combined neutron gamma ray instrument

Measuring the fluxes of thermal and epithermal neutrons at a planetary object in conjunction with gamma-ray spectroscopic observations will provide information about the chemical composition of the surface which is less model dependent than the gamma ray measurements by themselves. Researchers devised a passive neutron detector for this purpose. An experimental model was designed and built. Three variables provided the basis for a set of experiments: thickness of the Sm and B layers, the presence or absence of the ACS, and the position of the source relative to the PND's cylindrical axis. Experimental results are given.

Metzger, Albert E.↗

Feasibility study of a long duration balloon flight with NASA/GSFC and Soviet Space Agency Gamma Ray Spectrometers

A feasibility study of conducting a joint NASA/GSFC and Soviet Space Agency long duration balloon flight at the Antarctic in Jan. 1993 is reported. The objective of the mission is the verification and calibration of gamma ray and neutron remote sensing instruments which can be used to obtain geochemical maps of the surface of planetary bodies. The gamma ray instruments in question are the GRAD and the Soviet Phobos prototype. The neutron detectors are supplied by Los Alamos National Laboratory and the Soviet Phobos prototype. These are to be carried aboard a gondola that supplies the data and supplies the power for the period of up to two weeks.

Sharp, William E.↗

High LET, passive space radiation dosimetry and spectrometry

The development of high linear energy transfer (LET), passive radiation dosimetry and spectrometry is needed for the purpose of accurate determination of equivalent doses and assessment of health risks to astronauts on long duration missions. Progress in the following research areas is summerized: intercomparisons of cosmic ray equivalent dose and LET spectra measurements between STS missions and between astronauts; increases LET spectra measurement accuracy with ATAS; space radiation measurements for intercomparisons of passive (PNTD, TLD, TRND, Emulsion) and active (TEPC, RME-111) dosimeters; interaction of cosmic ray particles with nuclei in matter; radiation measurements after long duration space exposures; ground based dosimeter calibrations; neutron detector calibrations; radiation measurements on Soviet/Russian spacecraft; space radiation measurements under thin shielding; and space radiation.

Benton, E. V.↗

Mars Odyssey Science: The First Year and Beyond

The 2001 Mars Odyssey orbital science mission officially began in late February, 2002. The spacecraft carries three science instrument packages: the Gamma Ray Spectrometer suite (GRS), the Thermal Emission Imaging System (THEMIS), and the Martian Radiation Environment Experiment (MARIE). The GRS suite of three instruments includes the Gamma Sensor Subsystem (GSS), the Neutron Spectrometer (NS) and the High Energy Neutron Detector (HEND). THEMIS consists of two cameras sharing a single set of telescopic optics: a 5-band visible imager and a 10-band thermal infrared imager. Spacecraft and instrument performance have been nominal to this point in the science mission.

Plaut, J. J.↗

K/TH in Achondrites and Interpretation of Grand Data for the Dawn Mission

The Dawn mission will explore 4 Vesta [1], a highly differentiated asteroid believed to be the parent body of the howardite, eucrite and diogenite (HED) meteorite suite [e.g. 2]. The Dawn spacecraft is equipped with a gamma-ray and neutron detector (GRaND), which will enable measurement and mapping of elemental abundances on Vesta s surface [3]. Drawing on HED geochemistry, Usui and McSween [4] proposed a linear mixing model for interpretation of GRaND data. However, the HED suite is not the only achondrite suite representing asteroidal basaltic crusts; others include the mesosiderites, angrites, NWA 011, and possibly Ibitira, each of which is thought to have a distinct parental asteroid [5]. Here we critically examine the variability of GRaND-analyzed elements, K and Th, in HED meteorites, and propose a method based on the K-Th systematics to distinguish between HED and the other differentiated achondrites. Maps of these elements might also recognize incompatible element enriched areas such as mapped locally on the Moon (KREEP) [6], and variations in K/Th ratios might indicate impact volatilization of K. We also propose a new mixing model using elements that will be most reliably measured by GRaND, including K.

Usui, T.↗

The Electron Calorimeter (ECAL) Long Duration Balloon Experiment

Accurate measurements of the cosmic ray electron energy spectrum in the energy region 50 GeV to greater than 1 TeV may reveal structure caused by the annihilation of exotic dark matter particles and/or individual cosmic ray sources. Here we describe a new long duration balloon (LDB) experiment, ECAL, optimized to directly measure cosmic ray electrons up to several TeV. ECAL includes a double layer silicon matrix, a scintillating optical fiber track imager, a neutron detector and a fully active calorimeter to identify more than 90% of the incident electrons with an energy resolution of about 1.7% while misidentifying only 1 in 200,000 protons and 0.8% of secondary gamma rays as electrons. Two ECAL flights in Antarctica are planned for a total exposure of 50 days with the first flight anticipate for December 2009.

Guzik, T. G.↗

Fast Ray Tracing of Lunar Digital Elevation Models

Ray-tracing (RT) of Lunar Digital Elevation Models (DEM)'s is performed to virtually derive the degree of radiation incident to terrain as a function of time, orbital and ephemeris constraints [I- 4]. This process is an integral modeling process in lunar polar research and exploration due to the present paucity of terrain information at the poles and mission planning activities for the anticipated spring 2009 launch of the Lunar Reconnaissance Orbiter (LRO). As part of the Lunar Exploration Neutron Detector (LEND) and Lunar Crater Observation and Sensing Satellite (LCROSS) preparations RI methods are used to estimate the critical conditions presented by the combined effects of high latitude, terrain and the moons low obliquity [5-7]. These factors yield low incident solar illumination and subsequently extreme thermal, and radiation conditions. The presented research uses RT methods both for radiation transport modeling in space and regolith related research as well as to derive permanently shadowed regions (PSR)'s in high latitude topographic minima, e.g craters. These regions are of scientific and human exploration interest due to the near constant low temperatures in PSRs, inferred to be < 100 K. Hydrogen is thought to have accumulated in PSR's through the combined effects of periodic cometary bombardment and/or solar wind processes, and the extreme cold which minimizes hydrogen sublimation [8-9]. RT methods are also of use in surface position optimization for future illumination dependent on surface resources e.g. power and communications equipment.

McClanahan, Timothy P.↗

Dawn: An Ion-Propelled Journey to the Beginning of the Solar System

The Dawn mission is designed to perform a scientific investigation of the two heaviest mainbelt asteroids Vesta and Ceres. These bodies are believed to preserve records of the physical and chemical conditions present during the formation of the solar system. The mission uses an ion propulsion system to enable the single Dawn spacecraft and its complement of scientific instruments to orbit both of these asteroids. Dawn's three science instruments - the gamma ray and neutron detector, the visible and infrared mapping spectrometer, and the primary framing camera - were successfully tested after launch and are functioning normally. The ion propulsion system includes three ion thrusters of the type flown previously on NASA's Deep Space 1 mission. A minimum of two ion thrusters is necessary to accomplish the Dawn mission. Checkout of two of the ion thrusters was completed as planned within 30 days after launch. This activity confirmed that the spacecraft has two healthy ion thrusters. While further checkout activities are still in progress, the activities completed as of the end of October indicate that the spacecraft is well on its way toward being ready for the start of the thrusting-cruise phase of the mission beginning December 15th.

Vesta↗