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Many-body Nuclear Dynamics

The principal goal of this work was to better understand the fusion of neutron-rich nuclei a topic relevant to the fields of both nuclear physics and nuclear astrophysics. The work provides insight into the structure and reactions of neutron-rich nuclei namely the extent of their neutron density distribution and its polarizability. By comparing the fusion excitation functions for a chain of isotopes with a common target nucleus changes in the attractive nuclear potential are assessed. This change in the attractive potential is related to changes in the neutron density distribution with increasing number of neutrons or changes in fusion dynamics with increasing neutron number. The impact of the pairing of valence neutrons and protons on the fusion cross-section is also examined. Measurement of an isotopic chain is a powerful tool to address this topic. The experimental program made use of several different accelerator facilities. The core of the experimental work involved experiments at the ReA3 accelerator and the Facility for Rare Isotope Beams (FRIB) situated at Michigan State University, at GANIL, the French national nuclear physics laboratory, and the University of Notre Dame. At ReA3 the degree to which α-clusters associated with fusion of 28,30,32 Si + 28 Si result from the collision dynamics or reflect an initial α-cluster structure was explored. Alpha clusters observed in fusion reactions exceed the predictions of the standard statistical model. This experiment provides a measure of how clusterization is impacted by the increasing neutron-richess of the system. In the experiment at GANIL we investigated fusion in 19 O + 12 C and 20 O + 12 C. This experiment utilized the recently developed active-target detector MuSIC@Indiana. Using this proven, highly efficient, active-target detector we measured the fusion excitation function for these neutron-rich systems. Grounded by these experimental measurements, theoretical models were used to examine the role of unpaired valence neutrons on the fusion cross-section at energies just above the fusion barrier.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutron Fluence and Kerma Responses to Bare, Steel-Reflected, and Lucite-Reflected Steady-State Operations of the ORNL Health Physics Research Reactor

The experiments evaluated in this report were conducted at the Health Physics Research Reactor (HPRR), also known as the Fast Burst Reactor. The reactor was designed and built at Oak Ridge National Laboratory (ORNL) in 1961. In this evaluation, a total of 12 experiments were evaluated (6 shield configurations and two responses). Six of them are considered acceptable as benchmark experiments and are thoroughly described: the measurands are bare, steel-shielded and Lucite-shielded neutron fluences and neutron KERMA responses to steady-state operations of the HPRR. It is important to mention that there is a general lack of information in the experimental methodology and neutron spectrum unfolding, and in some cases, unexpected and unexplained discrepancies between calculation and experiment. The HPRR’s unique characteristics were that it is a fast reactor, the use of a Lucite shield as the shielding material, and the use of the neutron fluence as the main benchmark measurand. There are no known, significant correlations between benchmarks in this evaluation and benchmarks in other evaluations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Leptogenesis in parity solutions to the strong CP problem and Standard Model parameters

We study the simplest theories with exact spacetime parity that solve the strong CP problem and successfully generate the cosmological baryon asymmetry via decays of right-handed neutrinos. Lower bounds are derived for the masses of the right-handed neutrinos and for the scale of spontaneous parity breaking, v R . For generic thermal leptogenesis, v R ≳ 10 12 GeV, unless the small observed neutrino masses arise from fine-tuning. We compute v R in terms of the top quark mass, the QCD coupling, and the Higgs boson mass and find this bound is consistent with current data at 1σ. Future precision measurements of these parameters may provide support for the theory or, if v R is determined to be below 10 12 GeV, force modifications. However, modified cosmologies do not easily allow reductions in v R — no reduction is possible if leptogenesis occurs in the collisions of domain walls formed at parity breaking, and at most a factor 10 reduction is possible with non-thermal leptogenesis. Standard Model parameters that yield low values for v R can only be accommodated by having a high degree of degeneracy among the right-handed neutrinos involved in leptogenesis. If future precision measurements determine v R to be above 10 12 GeV, it is likely that higher-dimensional operators of the theory will yield a neutron electric dipole moment accessible to ongoing experiments. This is especially true in a simple UV completion of the neutrino sector, involving gauge singlet fermions, where the bound from successful leptogenesis is strengthened to v R ≳ 10 13 GeV.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Preliminary Activation Wire Analysis for the POKER Experiment Flattop Irradiation

Activation foils, or in this case wires, are commonly deployed to critical experiments at the Na tional Criticality Experiments Research Center (NCERC) to provide additional neutron diagnostics and provide additional energy-dependent responses to tie back to neutronic and/or multi-physics simulations.

07 ISOTOPE AND RADIATION SOURCES↗

An entropy-based debiasing approach to quantifying experimental coverage for novel applications of interest in the nuclear community

This manuscript proposes a novel information-theoretic approach to the quantification of experimental relevance, i.e., coverage, to achieve optimal data assimilation results for nuclear engineering applications. Specifically, this work posits the need for a new metric, called coverage (q C ) of an application’s quantity of interest, i.e., eigenvalue or power peaking for an advanced reactor concept, defined herein as the theoretically maximum achievable reduction in the quantity’s uncertainty given measurements from a pool of experiments in a manner that is independent of the data assimilation procedure employed. Currently, reduction in a quantity’s uncertainty is strongly biased by the underlying assumptions of the assimilation procedure to account for the under-determined nature of such problems and the similarity criterion employed to identify relevant experiments. To address this challenge, this work has developed a coverage metric, q C , based on mutual information, which establishes a new conceptual framework for assessing coverage, one that is independent of the model parameters and responses degree of variations in both the experimental and application domains, i.e., linear vs non-linear, and their prior uncertainty distributions, i.e., Gaussian vs. non-Gaussian. The q C is an entropic measure capable of addressing coverage for general nonlinear problems with non-Gaussian uncertainties and inclusive of the measurement uncertainties from multiple experiments. Numerical experiments from manufactured analytical problems as well as a set of benchmarks from the ICSBEP handbook are employed to demonstrate its theoretical and practical performance as compared to the c k -based experiment selection methodology, commonly employed in the neutronic community. The manuscript then employs other well-known adaptations to existing data assimilation methodologies for nonlinear and non-Gaussian problems capable of achieving the coverage posited by q C .

Bayesian data assimilation↗

Hybrid Star Models in the Light of New Multimessenger Data

Abstract Recent astrophysical mass inferences of compact stars HESS J1731-347 and PSR J0952-0607, with extremely small and large masses respectively, as well as the measurement of the neutron skin of Ca in the CREX experiment challenge and constrain the models of dense matter. We examine the concept of hybrid stars—objects containing quark cores surrounded by nucleonic envelopes—as models that account for these new data along with other inferences. We employ a family of 81 nucleonic equations of state (EOSs) with variable skewness and slope of symmetry energy at saturation density and a constant speed-of-sound EOS for quark matter. For each nucleonic EOS, a family of hybrid EOSs is generated by varying the transition density, the energy jump, and the speed of sound. These models are tested against the data from GW170817 and J1731-347, which favor low-density soft EOS and J0592-0607 and J0740+6620, which require high-density stiff EOS. The addition of J0592-0607's mass measurement to the constraints has no significant impact on the parameter space of the admissible EOS, but allows us to explore the potential effect of pulsars more massive than J0740+6620, if such exists. We then examine the occurrence of twin configurations and quantify the ranges of masses and radii that they can possess. It is shown that including J1731-347 data favors EOSs that predict low-mass twins with M ≲ 1.3 M ⊙ that can be realized if the deconfinement transition density is low. If combined with large speed of sound in quark matter such models allow for maximum masses of hybrid stars in 2.0–2.6 M ⊙ .

Astronomy & Astrophysics↗

Neutron diffraction: a primer

Because of the neutron’s special properties, neutron diffraction may be considered one of the most powerful techniques for structure determination of crystalline and related matter. Neutrons can be released from nuclear fission, from spallation processes, and also from low-energy nuclear reactions, and they can then be used in powder, time-of-flight, texture, single crystal, and other techniques, all of which are perfectly suited to clarify crystal and magnetic structures. With high neutron flux and sufficient brilliance, neutron diffraction also excels for diffuse scattering, for in situ and operando studies as well as for high-pressure experiments of today’s materials. For these, the wave-like neutron’s infinite advantage (isotope specific, magnetic) is crucial to answering important scientific questions, for example, on the structure and dynamics of light atoms in energy conversion and storage materials, magnetic matter, or protein structures. In this primer, we summarize the current state of neutron diffraction (and how it came to be), but also look at recent advances and new ideas, e.g., the design of new instruments, and what follows from that.

36 MATERIALS SCIENCE↗

Upgrade and characterization of the fast-channels of Imaging Neutral Particle Analyzers in the DIII-D tokamak

This publication presents the characterization of the recently upgraded fast (MHz) channels of the DIII-D Imaging Neutral Particle Analyzers. The new system allows for a phase space resolution of < 10 keV and < 10 cm. The main source of noise is due to the background radiation (neutrons and gammas) present in the diagnostic lab during experiments, which can hit the photomultipliers and generate large spikes in signal. Good linear correlations (r 2 > 0.9) are found between the average rate of noise spikes in the fast channels and the average neutron rate. Additional noise is caused by the scintillation of the optical fibers used to guide the signal to the acquisition system, which is induced by neutron and gamma impacts. A correlation factor r 2 > 0.6 between the baseline noise caused by this scintillation and the signals in the neutron diagnostic was found. Possible mitigation strategies, such as the use of shielding and filters, are discussed. These allow to reduce the noise spike rate by an order of magnitude and the noise baseline by a factor 4. Despite the noise, it is shown that the upgraded fast channels provide enough signal-to-noise ratio to observe coherent fluctuations of the energetic particle population.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

The Fuel Motion Monitoring System at TREAT - Current Status and Future Plans

An important component of the United States Nuclear Fuel Safety Transient Testing Program, the Fuel Motion Monitoring System (FMMS) at Idaho National Laboratory's Transient Reactor Test Facility (TREAT) is fast-neutron hodoscope capable of imaging the location, movement, and relocation of nuclear fuel experiments under simulated transient accident conditions. The FMMS was refurbished in parallel with the TREAT restart program starting in 2014, restoring 96-channels of fast-neutron detection. Since returning to operation in 2017 the FMMS has supported many fuel safety experiments supporting accident tolerant fuel development, light-water reactor safety, space thermal nuclear propulsion fuel development, and advanced reactor research and development. In Phase 2 of the FMMS restoration. work is now under way to expand the FMMS' field-of-view by adding an additional 96 channels of fast neutron detectors to the system's hodoscope, along with an expanded data acquisition system and associated transient timing electronics. An overview of the FMSS system and its fast-neutron detectors will be presented along with examples of current FMMS imaging performance and associated information.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

Godiva IV Simulated Radiation Field Characterization and Variance Reduction

Godiva IV is a system comprised of highly enriched uranium alloyed with molybdenum in the form of fuel plate rings. The reactor, along with its predecessors, was designed with the unique ability to satisfy interests in the super-prompt-critical reactor operation space. Originally, the reactor was part of the Los Alamos Critical Experiments Facility (LACEF) at Technical Area-18 (TA-18). The radiation field around Godiva at this facility was well characterized and understood. As a fast neutron system, the neutron spectrum in and around Godiva was close to a Watt Fission spectrum. The Kiva where Godiva IV was located at LACEF was made of thin, sheet metal walls which did not contribute significantly to the neutron spectrum. Following the transition of LACEF to the National Critical Experiments and Research Center (NCERC) in Nevada, Godiva-IV was moved from TA-18 to the Device Assembly Facility (DAF) at the Nevada National Security Site (NNSS). Part of this move brought renewed interest in radiation field characterization. The new facility introduced significant changes to the environment surrounding Godiva, and preliminary foil irradiation results suggested that the room contribution to the neutron spectrum was significant. Unlike at TA-18, a large thermal neutron signature was added to the fast spectrum from Godiva due to significant room return. A primary goal due to the additional complexity that the room return adds to the Godiva IV radiation emission spectrum was the development of an efficient Monte Carlo N-Particle (MCNP) calculation capable of characterizing the neutron spectrum anywhere in the room around Godiva. A campaign of activation foil irradiations and analysis were completed to support the validation of the MCNP model. The modeling of these foils in MCNP can be easily done with a standard volumetric neutron flux tally. However, given the multitude of locations and reaction rates to be modeled, further steps must be taken to increase the efficiency of these calculations in MCNP. During this study, a benchmark model currently under development for Godiva IV was used. A qualitative assessment of the thermal neutron contributors was performed using spatial neutron distribution plots. Additional detail was added to the model based on the qualitative results showing the thermal spectrum’s large sensitivity to hydrogenous material. Neutron energy spectra was evaluated at discrete locations in the room around Godiva to quantify the relative contribution of various components. It was discovered that the concrete walls are the largest contributor to the thermal signature, with minor contributions from plastic components surrounding Godiva. Following these results, two different variance reduction techniques were implemented to improve the problem efficiency in these calculations. In the first approach, an F5 point detector tally was implemented in the standard Godiva IV criticality problem. The second approach involved a weight-window generator implementation with an F5 point detector tally in a fixed source problem. The weight window implementation reduced the runtime from 42739.55 minutes to 1803.34 minutes (computer time), compared to the F5 KCODE implementation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

d -Electron Heavy Fermion Behavior in a Near-Room-Temperature Polar Metallic Ferrimagnet: A Case of Mn 5 SiC

Polycrystalline Mn 5 SiC was synthesized by using a high-temperature solid-state method. Mn 5 SiC adopts a polar space group (Cmc2 1 ) with six crystallographic Mn sites confirmed by X-ray and neutron diffraction, transmission electron microscopy, and second harmonic generation experiments. The complex crystal structure features edge-sharing trigonal prisms and icosahedra, as well as face/edge-sharing pentagonal prisms. Magnetic measurements indicate ferrimagnetic ordering with a transition temperature of 284 K. The ferrimagnetic structure (magnetic space group Cm’c’2 1 ) was further identified by powder neutron diffraction, where collinear Mn spins align along the crystallographic c-axis. The refined magnetic moment for each crystallographic Mn site at 4 K is 1.8(2), −2.42(9), −1.72(8), 0.51(6), 0.50(4), and 1.7(2) μ B . Density functional theory calculations confirm both the metallic behavior and the ferrimagnetic structure observed experimentally and further provide insight into the observed Mn moment dependence across crystallographic sites. The resistivity and specific heat measurements and density functional theory calculations reveal a substantially large Kadowaki–Woods ratio of 5 × 10 –5 μΩ·cm/(mJ/mol) 2 and a many-body renormalization factor of 5.5, indicating the unusual heavy Fermion behavior in such an itinerant magnetic metal.

Messegee, Zachary T. [George Mason University, Fai↗

Neutron-Antineutron Transition Search at DUNE

Neutron-antineutron transition is a baryon number violating process with ΔB=2, providing a unique insight into potential explanations of the baryon asymmetry in our universe, especially in the context of post-sphaleron baryogenesis. Studies have been conducted across various neutron-rich environments, including free neutron sources, neutron stars, and bound neutrons in large underground neutrino detectors, among which large neutrino experiments have historically obtained the most stringent constraints. The forthcoming Deep Underground Neutrino Experiment (DUNE) will offer especially strong prospects for this search, enabled by the high spatial resolution of its liquid argon time projection chamber. This poster presents a recent study on neutron-antineutron transition at DUNE using machine-learning based event classification.

Yu, Kaiwen [UC, Irvine (main)]↗

Studying MeV Scale Neutron Interactions in DUNE ND-LAr 2x2 Demonstrator

The Deep Underground Neutrino Experiment (DUNE) is a long-baseline neutrino oscillation experiment designed to make high-precision measurements of neutrino oscillation parameters and probe for new physics using a neutrino beam produced at Fermilab and measured at a near detector complex and a far detector located 1,300 km away at the Sanford Underground Research Facility. Precise neutrino energy reconstruction is essential for these measurements, with neutron production in neutrino–argon interactions representing a significant source of systematic uncertainty, as neutrons can carry away significant energy, making their detection and characterization crucial. DUNE’s near detector complex includes ND-LAr, a Liquid Argon Time Projection Chamber (LArTPC) detector designed to mirror the far detector technology and constrain neutrino–argon interaction systematics. The DUNE 2x2 Demonstrator, a pixelated LArTPC based on the ArgonCube design, serves as a prototype for ND-LAr. During 2x2 operations from October to November 2026, an Americium–Beryllium (AmBe) neutron source was deployed near the detector cryostat to obtain a high-statistics sample of neutron interactions. This poster presents progress in studying MeV-scale neutron interactions in this dataset by identifying de-excitation gammas from neutron capture on argon, providing a method for neutron identification and charge readout system calibration in future DUNE detectors.

Mao, Edgar [Syracuse U.] (ORCID:0009000600893306)↗

Ab initio calculations of overlap integrals for μ → e conversion in nuclei

The rate for μ → e conversion in nuclei is set to provide the most stringent test of lepton-flavor symmetry and a window into physics beyond the Standard Model. However, to disentangle new lepton-flavor-violating interactions, in combination with information from μ → ey and μ → 3e, it is critical that uncertainties at each step of the analysis be controlled and fully quantified. In this regard, nuclear response functions related to the coupling to neutrons are notoriously problematic, since they are not directly constrained by experiment. We address these shortcomings by combining ab initio calculations with a recently improved determination of charge distributions from electron scattering by exploiting strong correlations among charge, point-proton, and point-neutron radii and densities. We present overlap integrals for 27 Al, 48 Ca, and 48 Ti including full covariance matrices, allowing, for the first time, for a comprehensive consideration of nuclear structure uncertainties in the interpretation of μ → e experiments.

ab initio calculations↗

Diagnostics: Chapter 8 of the special issue: on the path to tokamak burning plasma operation

This chapter presents the activity conducted by the ITPA topical group (TG) on Diagnostics over about the last 15 years. Following a general introduction of the ITER Diagnostics led by their measurement roles, the document is organized in several subchapters detailing the design support, research and development activity conducted by each of the specialist working groups (WGs) of the TG. Please note that the magnetic diagnostics were supported at the TG without a specific WG. Their status is included in the general introduction. In the following some highlights of the subchapter’s contents are provided. Recent advances in ITER first wall (FW) diagnostics for the measurements of plasma-metallic wall interaction in support of the ITER research plan are reported. An InfraRed imaging Video Bolometer for ITER has been developed and tested on several tokamaks to measure the radiated power loss. A laser-induced breakdown spectroscopy (LIBS) technique which utilizes a pulsed laser beam to ablate locally by forming a crater, will measure local tritium inventory in the FW material. Real-time Residual Gas Analyzers will measure the neutral gas composition in a divertor port and an equatorial port during plasma operation. Due to the full metallic FW environment, the plasma-wall interaction in ITER will face several challenges such as the compromised radiated power and divertor heat flux measurements by reflection. Ray tracing and analysis codes have been developed to eliminate and correct the effects of reflection in the measurements. The characteristics of the reflecting surfaces depending on the roughness and angle of the incidence have been measured by dedicated experiments, and the results were applied to the reflection elimination. For the measurement of the metallic impurity radiation induced by eroded metallic atoms, a vacuum ultraviolet spectrometer has been developed and tested. An extensive thermonuclear diagnostic suite will be required to support the operation of ITER and the planned experimental program for future burning plasma experiments. Due to the harsh environmental conditions, the implementation of diagnostic systems in ITER is a major challenge. These conditions include high levels of neutron and gamma fluxes, neutron heating, particle bombardment. Therefore, the selection and design of diagnostic systems must take into account a number of phenomena previously unseen in diagnostic design. For this reason, the measurement of neutrons and confined or lost fast ions, with particular emphasis on alpha particles, is critical to ITER. The diagnostics associated with these measurements will be important for future plasma-burning experiments at ITER. The high neutron emission and very large plasma size in ITER make neutron diagnostics the main diagnostic method used to measure plasma parameters such as fusion power, fusion power density, ion temperature, energy of fast ions and their spatial distributions in the plasma core. Active spectroscopy techniques are methods where a neutral particle beam is injected into the plasma and information on plasma parameters is extracted from the measurement of line emission resulting from the beam-plasma interaction, either by plasma ions or by beam atoms. Spatial localization is achieved by crossing the beamline and multiple observation lines. The ITER plasma will be a high temperature, moderately dense, fully ionized collisional plasma. The plasma facing surfaces are principally metallic being fashioned from beryllium or tungsten but many other elements, arising from either structural or from operational needs, may enter this plasma. The energy range of the emitted photons range from meV (infra-red) to multi keV (x-rays) and originate from all areas of the plasma volume. The primary role of passive emission diagnostics is to identify what is in the plasma from spectral signatures. Extracting quantitative information from these measurements such as impurity content, ion temperature, rotation, degree of detachment and radiated power depends on calibrated instruments, a physics model of the atomic and molecular processes and plasma transport and an analysis workflow that takes into account environmental effects such as reflections. The particular needs for ITER have prompted a multi-machine, many-year effort to address all these aspects and this chapter reviews the work on diagnostic design, experiments and new analysis techniques. An overview of the laser diagnostics to be implemented on ITER is also provided in this paper. This includes descriptions of the Thomson scattering in the core, edge and divertor regions, polarimetry and interferometry diagnostics used for measuring plasma density and also measurements of helium density in the divertor using Laser Induced Flourescence. Techniques which can allow improvements on current measurements are also addressed in particular expanding poloidal polarimetry measurements to measure field fluctuations and proposed use of dispersion interferometery which has a number of advantages over existing methods. This paper identifies particular areas where further research and testing on existing tokamaks is useful even at this advanced stage to inform the design of diagnostics for ITER. Outstanding areas of concern for the implementation of laser diagnostics, in particular with a view to reliable operation are identified. An overview of the latest developments of microwave diagnostic systems and techniques is given. The primary focus is the contributions for ITER—the next step burning plasma experiment—which is supplemented by describing recent progress of techniques applicable for fusion experiments beyond ITER. The contributions are intentionally kept concise, and are being supplemented by a rich list of references for further studies. Radiation induced effects are receiving continuous and well-deserved attention of the ITER diagnostic community and they are in many cases one of the primary design drivers of the ITER diagnostic systems. The paper summarizes recent progress in this area focusing primarily on the ITER diagnostics but in some cases provides also outlook for the possible solutions for even more demanding radiation environment of fusion reactors beyond ITER. Despite advancements in the area of modeling and simulation of various radiation induced effects, experimental testing in a nuclear environment as close as possible to the target one is still seen as unavoidable for proper qualification of particular diagnostic functional elements. Recent advancement within three diagnostic areas: optical diagnostics, magnetics and bolometers is covered. Encouraging results on qualification of silica glass vacuum window assemblies are presented. In the area of magnetic sensors, progress of irradiation tests performed on ITER in-vessel LTCC inductive sensors is presented with outlook for novel technological approaches to inductive sensors utilizing thick printing and photolithography technologies being highlighted. Summary of advancements in the area of steady state magnetic field sensors based on Hall effect is given. New results of neutron irradiation test of the ITER borosilicate glass inserts for vacuum electrical feedthroughs are summarized finding negligible swelling at target level of neutron fluence. Off-line irradiation tests of fiber optic current sensors for plasma current measurement demonstrated that both for gamma doses up to 5 MGy and a total neutron fluence up to 10 15 cm −2 , radiation induced changes are still compatible with required measurement accuracy on ITER. The ITER bolometers are given as an example how considering radiation effects may influence the diagnostic design. Finally, outlook for future main R&D directions is outlined. All optical and laser-based diagnostics in ITER will be using mirrors to guide plasma radiation toward detectors, cameras and sensors. In the hostile plasma, radiation and particle environment the optical characteristics of diagnostic mirrors will degrade directly affecting the entire performance of involved diagnostic systems. An assessment of factors affecting mirror performance is provided. Among the prime adverse factors are deposition of plasma impurities, sputtering of mirror surface and steam ingress in the vicinity of mirrors. Within the International Tokamak Physics Activity with active support by ITER central team and domestic agencies, the structured research and development (R&D) program on mitigation of risks for diagnostic mirrors is underway. Within this program the mirror material development, the passive mitigation of mirror degradation by using diagnostic ducts and shutters along with an active mirror recovery program comprising the in-situ mirror cleaning and calibration is underway. Recent developments in diagnostic mirror R&D are described in this Chapter along with an example of their implementation of R&D solutions in ITER Infrared Thermography diagnostic. An assessment of still open engineering and physics questions, considerations on mirror risks during an early phase of ITER operation are given along with an overview of diagnostic mirror evolution in the late ITER operation stage toward the demonstration fusion power plant. Several crucial areas of diagnostic R&D outlined in ITER Research Plan are addressed. The basic control groups in a fusion reactor can be broken-down in five categories: (1) plasma position, magnetic configuration, and plasma current control, (2) profile control and confinement optimization, (3) MHD control and suppression, (4) edge dissipation control, radiation and plasma exhaust control and (5) break-down optimization. These categories are coupled via the physics (a control action in one domain will affect the other domains) and via shared actuators (e.g. ECRH for impurity accumulation avoidance, current density distribution control and MHD suppression). Consequently, a supervisory control system should determine the priority of the various control tasks, their couplings, and the interfaces with the safety and interlock system. For the systematic development of the various controllers taking the complexity of the plasma and the control system into account, a model-based approach is required. A short historical overview is given of the developments in systems and control theory and control engineering with special emphasis on those developments that are most relevant for Nuclear Fusion research and operation. An overview is given of the state of the field of fusion plasma control for the control categories. It will be shown how synthetic diagnostics are being developed in ITER and how they are used in diagnostic design and design validation and how they can be in model-based controller synthesis using relatively simple models. In modern control methods, multiple diagnostics are used to constrain relatively simple models. The constrained models provide an estimate for the state. This opens the route to state controllers, such as model predictive control. A major challenge in nuclear fusion research is the coherent combination of data from heterogeneous diagnostics and modeling codes for machine control and safety as well as physics studies. Measured data from different diagnostics often provide information about the same subset of physical parameters. Additionally, information provided by some diagnostics might be needed for the analysis of other diagnostics. A joint analysis of complementary and redundant data allows, e.g. to improve the reliability of parameter estimation, to increase the spatial and temporal resolution of profiles, to obtain synergistic effects, to consider diagnostics interdependencies and to find and resolve data inconsistencies. Physics-based modeling and parameter relationships provide additional information improving the treatment of ill-posed inversion problems. A coherent combination of all kind of available information within a probabilistic framework allows for improved data analysis results. The concept of integrated data analysis (IDA) in the framework of Bayesian probability theory is outlined and contrasted with conventional data analysis. Components of the probabilistic approach are summarized and specific ingredients beneficial for data analysis at fusion devices are discussed.

ITER↗

A flavor of SO(10) unification with a spinor Higgs

We investigate Higgs Parity unification — a realization of SO(10) grand unification based on the Higgs Parity mechanism in which the Standard Model (SM) Higgs resides in a spinor representation. The theory has an intermediate left-right symmetric stage where the SU(2)R symmetry breaking scale is fixed by the vanishing of the SM Higgs quartic coupling. The strong CP problem is solved by parity. Gauge coupling unification successfully predicts αs(MZ) to within 1%. The spinor Higgs naturally leads to a seesaw origin for SM flavor observables. We identify a novel mechanism where large mixing of third generation fermions with additional heavy vector-like fermions accounts for the anarchical nature of the PMNS matrix and the lack of hierarchy in the neutrino mass spectrum, relative to the up-quarks. A fit to quark and lepton masses and mixings, with a minimal parameter set, predicts 1) A testable relation between the top quark mass and αs(MZ) which is about (1 – 2)σ from current best fit values, 2) The order of magnitude of the baryon asymmetry of the universe, via leptogenesis from second-generation right-handed neutrino decays. 3) The proton decay and the neutron EDM are likely observable in next generation experiments, and 4) A normal ordered neutrino mass spectrum where 0νββ decay and the mass of the lightest neutrino are out of reach of next generation experiments.

Baryo-and Leptogenesis↗

Polyethylene Upcycling to Liquid Alkanes in Molten Salts under Neat and External Hydrogen Source-Free Conditions

Development of facile approaches to convert plastic waste into liquid fuels under neat conditions is highly desired but challenging, particularly without noble metal catalysts and an external hydrogen source. Herein, highly efficient and selective polyethylene-to-gasoline oil (branched C 6 –C 12 alkanes) conversion was achieved under mild conditions (<170 °C) using commercially available AlCl 3 -containing molten salts as reaction media and to provide catalytic sites (no extra solvents, additives, or hydrogen feeding). The high catalytic efficiency and selectivity was ensured by the abundant active Al sites with strong Lewis acidity (comparable to the Al type in acidic zeolite) and highly ionic nature of the molten salts to stabilize the carbenium intermediates. Dynamic genesis of the Al sites was elucidated via time-resolved Al K-edge soft X-ray and 27 Al NMR, confirming the tricoordinated Al 3+ as active sites and its coordination with the as-generated alkene/aromatic intermediates. Further, the carbenium formation and polyethylene chain variation was illustrated by inelastic neutron scattering (INS) and an isotope-labeling experiment. Theoretical simulations further demonstrated the successive hydride abstraction, β-scission, isomerization, and internal hydrogen transfer reaction pathway with AlCl 3 as active sites. This facile catalytic system can further achieve the conversion of robust, densely assembled, and high molecular weight plastic model compounds to liquid alkane products in the diesel range.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Comment on ‘Resonant inelastic x-ray scattering from U 3 O 8 and UN’

In a recent manuscript, Lawrence Bright et al (2023 J. Phys.: Condens. Matter 35 175501) reported the resonant inelastic x-ray scattering spectra of U 3 O 8 , as well as UN. Their goal was to identify electronic multiplets associated with a 5f 1 configuration with ground state 2 F 5/2 . Complete active space self-consistent field with spin–orbit coupling (CASSCF-SOC) predicted that 2 F 5/2 transitions should be observable at 190 and 328 meV. However, these energies were not accessible in their experiment. Here they suggested that the recent inelastic neutron scattering results of Miskowiec et al (2021 Phys. Rev. B 103 205101) could have been sensitive to these transitions. Here we show that transitions of this possible origin appear in that dataset near 198, 262, 362, and potentially 448 meV.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗