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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 307 records · Page 17
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Structural and Improper Ferroelectric Properties of TbInO 3 Single Crystal Grown by Laser Floating Zone

The honeycomb TbInO 3 has attracted wide research attention due to its fascinating physical properties. However, TbInO 3 single crystal was difficult to grow owing to the high melting point and serious volatilization of indium during the crystal growth. In this study, the volatilization of the indium element was effectively suppressed by controlling the growth atmosphere and pressure. The excess ratio of indium oxide was determined, and pure hexagonal TbInO 3 crystal was obtained by the laser floating zone method. Systematic studies on the crystal structure and optical and ferroelectric properties were carried out. The structure distortion resulted in the improper geometric ferroelectric revealed by single crystal diffraction and Raman spectrum measurements. The topological vortex domains and P-E hysteresis loop demonstrated the presence of ferroelectricity. TbInO 3 crystal has great potential application in vortex memory.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Spectroscopic Fourth-order Coronagraph for the Characterization of Terrestrial Planets at Small Angular Separations from Host Stars

We propose a new approach for high-contrast imaging at the diffraction limit using segmented telescopes in a modest observation bandwidth. This concept, named “spectroscopic fourth-order coronagraphy,” is based on a fourth-order coronagraph with a focal-plane mask that modulates the complex amplitude of the Airy disk along one direction. While coronagraphs applying the complex amplitude mask can achieve the theoretical limit performance for any arbitrary pupils, the focal-plane mask severely limits the bandwidth. Here, focusing on the fact that the focal-plane mask modulates the complex amplitude along one direction, we noticed that the mask can be optimized for each spectral element generated by a spectrograph. We combine the fourth-order coronagraph with two spectrographs to produce a stellar spectrum on the focal plane and reconstruct a white pupil on the Lyot stop. Based on the wave-front analysis of an optical design applying an Offner-type imaging spectrograph, we found that the achievable contrast of this concept is 10{sup −10} at 1.2–1.5 times the diffraction limit over the wavelength range of 650–750 nm for the entrance pupil of the LUVOIR telescope. Thus, this coronagraph concept could bring new habitable planet candidates not only around G- and K-type stars beyond 20–30 pc but also around very nearby M-type stars. This approach potentially promotes the characterization of the atmospheres of nearby terrestrial planets with future on- and off-axis segmented large telescopes.

47 OTHER INSTRUMENTATION↗
DOE OSTI2022

Improving Cosmological Constraints from Galaxy Cluster Number Counts with CMB-cluster-lensing Data: Results from the SPT-SZ Survey and Forecasts for the Future

Abstract We show the improvement to cosmological constraints from galaxy cluster surveys with the addition of cosmic microwave background (CMB)-cluster lensing data. We explore the cosmological implications of adding mass information from the 3.1 σ detection of gravitational lensing of the CMB by galaxy clusters to the Sunyaev–Zel’dovich (SZ) selected galaxy cluster sample from the 2500 deg 2 SPT-SZ survey and targeted optical and X-ray follow-up data. In the ΛCDM model, the combination of the cluster sample with the Planck power spectrum measurements prefers σ 8 Ω m / 0.3 0.5 = 0.831 ± 0.020 . Adding the cluster data reduces the uncertainty on this quantity by a factor of 1.4, which is unchanged whether the 3.1 σ CMB-cluster lensing measurement is included or not. We then forecast the impact of CMB-cluster lensing measurements with future cluster catalogs. Adding CMB-cluster lensing measurements to the SZ cluster catalog of the ongoing SPT-3G survey is expected to improve the expected constraint on the dark energy equation of state w by a factor of 1.3 to σ ( w ) = 0.19. We find the largest improvements from CMB-cluster lensing measurements to be for σ 8 , where adding CMB-cluster lensing data to the cluster number counts reduces the expected uncertainty on σ 8 by respective factors of 2.4 and 3.6 for SPT-3G and CMB-S4.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Second harmonic generation in topological insulators under quantizing magnetic fields

We theoretically investigate the second harmonic generation (SHG) of topological insulator surface states in a perpendicular magnetic field. Our theory is based on the microscopic expression of the second-order magneto-optical conductivity developed from the density matrix formalism, taking into account hexagonal warping effects on the surface states' band structure. Using numerically exact Landau-level energies and wave functions including hexagonal warping, we calculate the spectrum of SHG conductivities under normal incidence for different values of magnetic field and chemical potential. The imaginary parts of the SHG conductivities show prominent resonant peaks corresponding to one-photon and two-photon inter-Landau-level transitions. Treating the hexagonal warping term perturbatively, these transitions are clarified analytically within a perturbation theory from which approximate selection rules for the allowable optical transitions for SHG are determined. Furthermore, our results show extremely high SHG susceptibility that is easily tunable by magnetic field and doping level for topological surface states in the far-infrared regime, exceeding that of many conventional nonlinear materials. This work highlights the key role of hexagonal warping effects in generating second-order optical responses and provides insights into the nonlinear magneto-optical properties of the topological insulators.

Landau levels↗
DOE OSTI2023

Snapshot multispectral imaging using a diffractive optical network

Abstract Multispectral imaging has been used for numerous applications in e.g., environmental monitoring, aerospace, defense, and biomedicine. Here, we present a diffractive optical network-based multispectral imaging system trained using deep learning to create a virtual spectral filter array at the output image field-of-view. This diffractive multispectral imager performs spatially-coherent imaging over a large spectrum, and at the same time, routes a pre-determined set of spectral channels onto an array of pixels at the output plane, converting a monochrome focal-plane array or image sensor into a multispectral imaging device without any spectral filters or image recovery algorithms. Furthermore, the spectral responsivity of this diffractive multispectral imager is not sensitive to input polarization states. Through numerical simulations, we present different diffractive network designs that achieve snapshot multispectral imaging with 4, 9 and 16 unique spectral bands within the visible spectrum, based on passive spatially-structured diffractive surfaces, with a compact design that axially spans ~72 λ m , where λ m is the mean wavelength of the spectral band of interest. Moreover, we experimentally demonstrate a diffractive multispectral imager based on a 3D-printed diffractive network that creates at its output image plane a spatially repeating virtual spectral filter array with 2 × 2 = 4 unique bands at terahertz spectrum. Due to their compact form factor and computation-free, power-efficient and polarization-insensitive forward operation, diffractive multispectral imagers can be transformative for various imaging and sensing applications and be used at different parts of the electromagnetic spectrum where high-density and wide-area multispectral pixel arrays are not widely available.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Optical suppression of defect-related photoluminescence in GeSn

Reports of photoluminescence from GeSn grown on Ge substrates by molecular beam epitaxy have been limited. We find that one limiting factor to observing photoluminescence is due to localized defect states marked by photoluminescence at 2400 nm and originating from the Ge substrate and buffer layer. In this study, we report on an optical study utilizing doped Ge(001) substrates to effectively suppress defect-related photoluminescence in GeSn layers by filling localized defect trap states. For this experiment, a GeSn layer with Sn content up to 10.5 ± 0.5% was grown on a doped Ge(001) substrate. Analysis of the physics of the photoluminescence spectrum collected from the GeSn thin film shows an emission at the expected wavelength of 2300 nm for 10.5 ± 0.5% Sn content and the absence of the typically observed defect-related signal at 2400 nm. This understanding is further confirmed using short-pulse optical excitation of the GeSn grown on undoped Ge substrates.

Chemical vapor deposition↗
DOE OSTI2020

Spectroscopic classification, variability, and SED of the Fermi -detected CSS 3C 286: the radio-loudest NLS1 galaxy?

ABSTRACT 3C 286 is a well-known calibrator source in radio astronomy. It is also one of very few compact steep-spectrum (CSS) sources detected in γ-rays. Here, we perform a detailed spectroscopic and variability analysis and present the first quasi-simultaneous optical to X-ray spectral energy distribution (SED) in order to reveal physical mechanisms that dominate its emission at different wavelengths, and arrive at a reliable optical source classification. The first main result of our study reveals several pitfalls when applying simple broad- or narrow-line Seyfert 1 (BLS1 or NLS1) classification criteria that only look at the [O iii]–Hβ complex. [O iii] and Hβ can be dominated by the same outflow components, in which case full width at half-maximum (Hβ) is no reliable classification criterion, and extinction by intrinsic or intervening material can make the highest velocity Hβ component undetectable. After careful combination of all information from ultraviolet (UV)–optical spectra along with multiwavelength data, we confirm that 3C 286 can be classified as NLS1 galaxy, with line properties and supermassive black hole mass (of order 108 M⊙ and accreting near the Eddington limit) close to the BLS1 regime, making it an important borderline object. The quasi-simultaneous SED taken with Swift shows a sharp rise in the optical–UV, implying the presence of a strong accretion-disc component with extreme UV excess, consistent with emission-line diagnostics. Finally, we report the discovery of X-ray variability of 3C 286, plausibly dominated by jet emission, and variable by at least a factor of ∼4. This result suggests to exercise caution when using 3C 286 as radio calibrator in high-resolution radio very long baseline interferometry observations.

Yao, Su↗
DOE OSTI2021

Visible-light Phase Curves from the Second Year of the TESS Primary Mission

We carried out a systematic study of full-orbit phase curves for known transiting systems in the northern ecliptic sky that were observed during Year 2 of the TESS primary mission. We applied the same methodology for target selection, data processing, and light-curve fitting as we did in our Year 1 study. Out of the 15 transiting systems selected for analysis, seven—HAT-P-7, KELT-1, KELT-9, KELT-16, KELT-20, Kepler-13A, and WASP-12—show statistically significant secondary eclipses and day–night atmospheric brightness modulations. Small eastward dayside hot-spot offsets were measured for KELT-9b and WASP-12b. KELT-1, Kepler-13A, and WASP-12 show additional phase-curve variability attributed to the tidal distortion of the host star; the amplitudes of these signals are consistent with theoretical predictions. We combined occultation measurements from TESS and Spitzer to compute dayside brightness temperatures, TESS-band geometric albedos, Bond albedos, and phase integrals for several systems. The new albedo values solidify the previously reported trend between dayside temperature and geometric albedo for planets with 1500 K < T {sub day} < 3000 K. For Kepler-13Ab, we carried out an atmospheric retrieval of the full secondary eclipse spectrum, which revealed a noninverted temperature–pressure profile, significant H{sub 2}O and K absorption in the near-infrared, evidence for strong optical atmospheric opacity due to sodium, and a confirmation of the high geometric albedo inferred from our simpler analysis. We explore the implications of the phase integrals (ratios of Bond to geometric albedos) for understanding exoplanet clouds. We also report updated transit ephemerides for all of the systems studied in this work.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Multiwavelength Afterglow Analysis of GRB 221009A: Unveiling the Evolution of a Cooling Break in a Wind-like Medium

Gamma-ray bursts (GRBs) are the most energetic explosions in the Universe, and their afterglow emission provides an opportunity to probe the physics of relativistic shock waves in an extreme environment. Several key pieces for completing the picture of GRB afterglow physics are still missing, including jet properties, the emission mechanism, and particle acceleration. Here, we present a study of the afterglow emission of GRB 221009A, the most energetic GRB ever observed. Using optical, X-ray, and gamma-ray data up to approximately 2 days after the trigger, we trace the evolution of the multiwavelength spectrum and the physical parameters behind the emission process. The broadband spectrum is consistent with the synchrotron emission emitted by relativistic electrons with its index of p = 2.29 ± 0.02. We identify a break energy at keV and an exponential cutoff at GeV in the observed multiwavelength spectrum. The break energy increases in time from $16.0^{+7.1}_{-4.9}$ keV at 0.65 days to $46.8^{+25.0}_{-15.5}$ keV at 1.68 days, favoring a stellar-wind-like profile of the circumburst medium with k = 2.4 ± 0.1 as in ρ(r) ∝ r -k . The high-energy attenuation at around 0.4 to 4 GeV is attributed to the maximum of the particle acceleration in the relativistic shock wave. This study confirms that the synchrotron process can explain the multiwavelength afterglow emission and its evolution.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Characterization and Evaluation of Scintillating Fiber System Components

Idaho National Laboratory is studying long scintillation fibers (SF) in a project called “TRIPWIRE” which aims to verify containment in inaccessible nuclear waste repositories. This system will continuously monitor ionizing radiation, electromagnetic fields, and seismic activity in the vicinity of nuclear waste. Previous experiments have determined a better alternative to long SF is to couple shorter SF to kilometer scale optical fiber (OF) to reach electronics far outside of the repository. Minor signal attenuation from coupling these fibers has been observed using optical spectrometry. This experiment characterized two photomultiplier tubes (PMT) to reduce this loss by matching their spectral response characteristics to the SF’s emission spectrum. The experiment created a comparison between the two PMTs showing results that suggest other characteristics are playing a major role in improving signal attenuation when the SF is coupled to OF.

98 - NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL↗
DOE OSTI2022

Distributed Fiber Optic Sensing to Identify Locations of Resistive Transitions in REBCO Conductors and Magnets

High-temperature superconductors such as REBa 2 Cu 3 O 7-x (REBCO, RE = rare earth) can generate strong magnetic fields that are promising for applications in particle accelerators and compact fusion reactors. Traditionally, voltage taps are installed in superconducting magnets to measure the voltage signals due to resistive transitions. The voltage-tap-based diagnostics is important for the development of magnet technology as it can help pinpoint the locations in the magnet windings that limit the magnet performance. The architecture of the multi-tape REBCO cable such as CORC wires, however, makes it difficult to apply the voltage-tap-based diagnostics to identify the locations of resistive transitions. Distributed fiber optic sensing (DFOS) has the potential to address this issue. In this paper, we report the measurements of thermal strain along a CORC wire based on optical frequency domain reflectometry with a maximum spatial resolution of 0.65 mm and a temporal resolution of 10 Hz. The optical fiber is co-wound with the CORC wire that is epoxy impregnated. During the test, current was increased until a resistive transition occurred in the conductor. The spectrum shift of the reflected light along the fiber was recorded. The results suggested that with proper thermal isolation from the cryogen, DFOS can be used to identify the locations of resistive transitions in CORC wires and magnets. In conclusion, the results will allow a better understanding of the causes of resistive transitions in REBCO conductors and magnets, which will help improve the REBCO magnet technology.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

XRISM Forecast for the Coma Cluster: Stormy, with a Steep Power Spectrum

The XRISM Resolve microcalorimeter array measured the velocities of hot intracluster gas at two positions in the Coma galaxy cluster: ${3}^{{\prime} }\times {3}^{{\prime} }$ squares at the center and at 6$^{\prime} $ (170 kpc) to the south. We find the line-of-sight velocity dispersions in those regions to be σ z = 208 ± 12 km s −1 and 202 ± 24 km s −1 , respectively. The central value corresponds to a 3D Mach number of M = 0.24 ± 0.015 and a ratio of the kinetic pressure of small-scale motions to thermal pressure in the intracluster plasma of only 3.1% ± 0.4%, at the lower end of predictions from cosmological simulations for merging clusters like Coma, and similar to that observed in the cool core of the relaxed cluster A2029. Meanwhile, the gas in both regions exhibits high line-of-sight velocity differences from the mean velocity of the cluster galaxies, Δv z = 450 ± 15 km s −1 and 730 ± 30 km s −1 , respectively. A small contribution from an additional gas velocity component, consistent with the cluster optical mean, is detected along a sight line near the cluster center. The combination of the observed velocity dispersions and bulk velocities is not described by a Kolmogorov velocity power spectrum of steady-state turbulence; instead, the data imply a much steeper effective slope (i.e., relatively more power at larger linear scales). This may indicate either a very large dissipation scale, resulting in the suppression of small-scale motions, or a transient dynamic state of the cluster, where large-scale gas flows generated by an ongoing merger have not yet cascaded down to small scales.

coma cluster↗
DOE OSTI2023

Phonon Anharmonicity and Spin–Phonon Coupling in CrI 3

We report on the far-infrared, temperature-dependent optical properties of a CrI 3 transition metal halide single crystal, a van der Waals ferromagnet (FM) with a Curie temperature of 61 K. In addition to the expected phonon modes determined by the crystalline symmetry, the optical reflectance and transmittance spectra of CrI 3 single crystals show many other excitations as a function of temperature as a consequence of the combination of a strong lattice anharmonicity and spin–phonon coupling. This complex vibrational spectrum highlights the presence of entangled interactions among the different degrees of freedom in CrI 3 .

36 MATERIALS SCIENCE↗
DOE OSTI2024

Semi-Dirac Fermions in a Topological Metal

Topological semimetals with massless Dirac and Weyl fermions represent the forefront of quantum materials research. In two dimensions, a peculiar class of fermions that are massless in one direction and massive in the perpendicular direction was predicted 16 years ago. These highly exotic quasiparticles—the semi-Dirac fermions—ignited intense theoretical and experimental interest but remain undetected. Using magneto-optical spectroscopy, we demonstrate the defining feature of semi-Dirac fermions— B 2 / 3 scaling of Landau levels—in a prototypical nodal-line metal ZrSiS. In topological metals, including ZrSiS, nodal lines extend the band degeneracies from isolated points to lines, loops, or even chains in the momentum space. With calculations and theoretical modeling, we pinpoint the observed semi-Dirac spectrum to the crossing points of nodal lines in ZrSiS. Crossing nodal lines exhibit a continuum absorption spectrum but with singularities that scale as B 2 / 3 at the crossing. Our work sheds light on the hidden quasiparticles emerging from the intricate topology of crossing nodal lines and highlights the potential to explore quantum geometry with linear optical responses. Published by the American Physical Society 2024

Shao, Yinming (ORCID:0000000228910028)↗
DOE OSTI2021

Narrow-band high-lying excitons with negative-mass electrons in monolayer WSe2

Monolayer transition-metal dichalcogenides (TMDCs) show a wealth of exciton physics. Here, we report the existence of a new excitonic species, the high-lying exciton (HX), in single-layer WSe 2 with an energy of ~3.4 eV, almost twice the band-edge A-exciton energy, with a linewidth as narrow as 5.8 meV. The HX is populated through momentum-selective optical excitation in the K-valleys and is identified in upconverted photoluminescence (UPL) in the UV spectral region. Strong electron-phonon coupling results in a cascaded phonon progression with equidistant peaks in the luminescence spectrum, resolvable to ninth order. Ab initio GW-BSE calculations with full electron-hole correlations explain HX formation and unmask the admixture of upper conduction-band states to this complex many-body excitation. These calculations suggest that the HX is comprised of electrons of negative mass. The coincidence of such high-lying excitonic species at around twice the energy of band-edge excitons rationalizes the excitonic quantum-interference phenomenon recently discovered in optical second-harmonic generation (SHG) and explains the efficient Auger-like annihilation of band-edge excitons.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Phased plan for the implementation of the time-resolving magnetic recoil spectrometer on the National Ignition Facility (NIF)

The time-resolving magnetic recoil spectrometer (MRSt) is a transformative diagnostic that will be used to measure the time-resolved neutron spectrum from an inertial confinement fusion implosion at the National Ignition Facility (NIF). It uses a CD foil on the outside of the hohlraum to convert fusion neutrons to recoil deuterons. An ion-optical system positioned outside the NIF target chamber energy-disperses and focuses forward-scattered deuterons. A pulse-dilation drift tube (PDDT) subsequently dilates, un-skews, and detects the signal. While the foil and ion-optical system have been designed, the PDDT requires more development before it can be implemented. Therefore, a phased plan is presented that first uses the foil and ion-optical systems with detectors that can be implemented immediately—namely CR-39 and hDISC streak cameras. These detectors will allow the MRSt to be commissioned in an intermediate stage and begin collecting data on a reduced timescale, while the PDDT is developed in parallel. A CR-39 detector will be used in phase 1 for the measurement of the time-integrated neutron spectra with excellent energy-resolution, necessary for the energy calibration of the system. Streak cameras will be used in phase 2 for measurement of the time-resolved spectrum with limited spectral coverage, which is sufficient to diagnose the time-resolved ion temperature. Simulations are presented that predict the performance of the streak camera detector, indicating that it will achieve excellent burn history measurements at current yields, and good time-resolved ion-temperature measurements at yields above 3 × 10 17 . The PDDT will be used for optimal efficiency and resolution in phase 3.

47 OTHER INSTRUMENTATION↗
DOE OSTI2022

Mid- to Far-Infrared Anisotropic Dielectric Function of HfS 2 and HfSe 2

The far-infrared (far-IR) remains a relatively underexplored region of the electromagnetic spectrum extending roughly from 20 to 100 µm in free-space wavelength. Research within this range has been restricted due to a lack of optical materials that can be optimized to reduce losses and increase sensitivity, as well as by the long free-space wavelengths associated with this spectral region. Here the exceptionally broad Reststrahlen bands of two Hf-based transition metal dichalcogenides (TMDs) that can support surface phonon polaritons (SPhPs) within the mid-infrared (mid-IR) into the terahertz (THz) are reported. In this vein, the IR transmission and reflectance spectra of hafnium disulfide (HfS 2 ) and hafnium diselenide (HfSe 2 ) flakes are measured and their corresponding dielectric functions are extracted. These exceptionally broad Reststrahlen bands (HfS 2 : 165 cm -1 ; HfSe 2 : 95 cm -1 ) dramatically exceed that of the more commonly explored molybdenum- (Mo) and tungsten- (W) based TMDs (≈5–10 cm -1 ), which results from the over sevenfold increase in the Born effective charge of the Hf-containing compounds. Further, this work therefore identifies a class of materials for nanophotonic and sensing applications in the mid- to far-IR, such as deeply sub-diffractional hyperbolic and polaritonic optical antennas, as is predicted via electromagnetic simulations using the extracted dielectric function.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Optical spectral observations of three binary millisecond pulsars

We present the results of optical spectroscopy of stellar companions to three binary millisecond pulsars, PSRs J0621+2514, J2317+1439, and J2302+4442, obtained with the Gran Telescopio Canarias. The spectrum of the J0621+2514 companion shows a blue continuum and prominent Balmer absorption lines. The latter are also resolved in the spectrum of the J2317+1439 companion, showing that both are DA-type white dwarfs. No spectral features are detected for the J2302+4442 companion; however, its broad-band magnitudes and the spectral shape of the continuum emission imply that this is also a DA-type white dwarf. Based on the spectral analyses, we conclude that the companions of J0621+2514 and J2317+1439 are relatively hot, with effective temperatures T eff = 8600 ± 200 and 9600 ± 2000 K, respectively, while the J2302+4442 companion is significantly cooler, T eff <6000 K. We also estimated the distance to J0621+2514 of 1.1 ± 0.3 kpc and argue that its companion and the companion of J2317+1439 are He-core white dwarfs providing constraints on their cooling ages of $\lesssim$2 Gyr.

79 ASTRONOMY AND ASTROPHYSICS↗