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At least 307 records · Page 17

Overmoded subterahertz surface wave oscillator with pure TM{sub 01} mode output

Overmoded O-type Cerenkov generators using annular electron beams are facing the problem of multi-modes output due to the inevitable structural discontinuities. A simple but effective method to achieve the pure TM{sub 01} mode output is applied on the 0.14 THz overmoded surface wave oscillator (SWO) in this paper. In spite of still using an overmoded slow wave structure to ensure the easy fabrication, the followed smooth circular waveguide is shrinkingly tapered to the output waveguide with appropriate radius that it cuts off other higher modes except TM{sub 01} mode. Moreover, the modified device here has the same power capacity as the previous one according to the numerical analysis. By optimized lengths of the transition waveguide and tapered waveguide, particle-in-cell simulation results indicate that the subterahertz wave with output power increased 14.2% at the same frequency is obtained from the proposed SWO under the previous input conditions, and importantly, the output power is all carried by TM{sub 01} mode as expected. Further simulation results in the pulse regime confirm the feasibility of the optimized structure in the actual experiments. This simple and viable design is also applicable to overmoded devices in the lower frequency band of subterahertz wave.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Five-cell superconducting RF module with a PBG coupler cell: design and cold testing of the copper prototype

We report the design and experimental data for a copper prototype of a superconducting radio-frequency (SRF) accelerator module. The five-cell module has an incorporated photonic band gap (PBG) cell with couplers. The purpose of the PBG cell is to achieve better higher order mode (HOM) damping, which is vital for preserving the quality of high-current electron beams. Better HOM damping raises the current threshold for beam instabilities in novel SRF accelerators. The PBG design also increases the real-estate gradient of the linac because both HOM damping and the fundamental power coupling can be done through the PBG cell instead of on the beam pipe via complicated end assemblies. First, we will discuss the design and accelerating properties of the structure. The five-cell module was optimized to provide good HOM damping while maintaining the same accelerating properties as conventional elliptical-cell modules. We will then discuss the process of tuning the structure to obtain the desired accelerating gradient profile. Finally, we will list measured quality factors for the accelerating mode and the most dangerous HOMs.

43 PARTICLE ACCELERATORS↗

Solvothermal synthesis of uranium(VI) phases with aromatic carboxylate ligands: A dinuclear complex with 4-hydroxybenzoic acid and a 3D framework with terephthalic acid

With the coordination of dimethylformamide (DMF), two new uranium(VI) complexes with either 4-hydroxybenzoic acid (H{sub 2}phb) or terephthalic acid (H{sub 2}tph) have been synthesized under solvothermal conditions and structurally characterized. [(UO{sub 2}){sub 2}(Hphb){sub 2}(phb)(DMF)(H{sub 2}O){sub 3}]·4H{sub 2}O (1) has a dinuclear structure constructed with both pentagonal and hexagonal bipyramidal uranium polyhedra linked through a µ{sub 2}-bridging ligand via both chelating carboxylate arm and alcohol oxygen bonding, first observation of such a coordination mode of 4-hydroxybenzoate for 5 f ions. [(UO{sub 2})(tph)(DMF)] (2) has a three-dimensional (3D) framework built with pentagonal bipyramidal uranium polyhedra linked with µ{sub 4}-terephthalate ligands. The 3D channeled structure is facilitated by the unique carboxylate bonding with nearly linear C–O–U angles and the coordination of DMF molecules. The presence of phb ligands in different coordination modes, uranyl ions in diverse environments and DMF in complex 1, and tph ligand, DMF and uranyl ion in complex 2 has been confirmed by Raman spectroscopy. In addition, their thermal stability and photoluminescence properties have been investigated. - Graphical abstract: With the coordination of dimethylformamide, two new uranyl complexes with either 4-hydroxybenzoate or terephthalate have been synthesized under solvothermal conditions and structurally characterized. - Highlights: • Solvent facilitates the synthesis of two new uranium(VI) complexes. • A dinuclear complex with both penta- and hexagonal bipyramidal uranium polyhedral. • A unique µ{sub 2}-bridging mode of 4-hydroxybenzoate via alcohol oxygen for 5 f ions. • A 3D framework with uranium polyhedra and µ{sub 4}-terephthalate ligands. • Vibration modes and photoluminescence properties are reported.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Investigating ICRF Core Physics with a Hybrid Method using {delta}f Particles

Particle-in-cell simulations of ICRF core physics yield a significant amount of noise that can overwhelm the low amplitude signals associated with ICRH. To overcome this noise, we employ a hybrid approach that uses a fluid model for electrons and the delta-f particle-in-cell (DFPIC) method for ions. Noise is reduced to a level well below the amplitude of the signal and time steps are permitted to go beyond the electron time scales. With this formulation we have explored minority heating scenarios in Alcator C-Mod and high harmonic heating scenarios in NSTX. We can also employ the fluid model for both electrons and ions to investigate cold plasma scenarios. Here we examine ion test particles with particular attention paid to particle paths near resonance layers. We present our technique for investigating full particle orbits from a single toroidal mode expansion.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Vibrational spectra and nonlinear optical coefficients of rhombohedral CsGe X 3 halide compounds with X = I , Br, Cl

The zone-center phonons are calculated here for rhombohedral CsGeX 3 compounds with X=I, Br, Cl using density functional perturbation theory in a plane-wave pseudopotential method. The infrared absorption and reflection spectra are simulated and show that the absorption has a strong contribution from the LO as well asTO modes. Both the lowest and highest IR active modes have strong oscillator strengths for each symmetry (A 1 and E) and correspond to motions of either the Cs or Ge ions relative to the halogen ions. respectively. The intermediate modes have low oscillator strength because their mode pattern shows less clearly a dipole pattern.The polarization dependent Raman spectra for various back scattering configurations are simulated. Only the highest modes of each symmetry have a strong Raman intensity. The findings for the Raman spectra are found to be in good agreement with the available experimental data for polycrystalline films when averaging over directions. The Born effective charges and high and low frequency dielectric tensors as well as the second-order nonlinear optical coefficients are calculated. The ratio of the static to the high-frequency dielectric constants are extremely high and analyzed in terms of the contribution of each mode to the Lyddane-Sachs-Teller relation. The nonlinear optical coefficients decrease strongly from I to Br to Cl in reverse order of the band gaps and are foundto be consistent with available experimental results

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

High multi-photon visible upconversion emissions of Er{sup 3+} singly doped BiOCl microcrystals: A photon avalanche of Er{sup 3+} induced by 980 nm excitation

Under 980 nm excitation, high multi-photon upconversion (UC) emission from the {sup 2}H{sub 11/2}/{sup 4}S{sub 3/2} (green) and {sup 4}F{sub 9/2} (red) levels of Er{sup 3+} ions were observed from Er{sup 3+} singly doped BiOCl microcrystals. These high-energy excited states were populated by a three to ten photon UC process conditionally, which depended on the pump power density and the Er{sup 3+} ion doping concentration, characterizing as a hetero-looping enhanced energy transfer avalanche UC process. UC emission lifetime and Raman analysis suggest that the unusual UC phenomena are initiated by the new and intense phonon vibration modes of BiOCl lattices due to Er{sup 3+} ions doping.

36 MATERIALS SCIENCE↗

Density response of a trapped Fermi gas: A crossover from the pair vibration mode to the Goldstone mode

We consider the density response of a trapped two-component Fermi gas. Combining the Bogoliubov-deGennes method with the random phase approximation allows the study of both collective and single-particle excitations. Calculating the density response across a wide range of interactions, we observe a crossover from a weakly interacting pair vibration mode to a strongly interacting Goldstone mode. The crossover is associated with a depressed collective mode frequency and an increased damping rate, in agreement with density response experiments performed in strongly interacting atomic gases.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Two Leading ENSO Modes and El Niño Types in the Zebiak–Cane Model

Modern instrumental records reveal that El Niño events differ in their spatial patterns and temporal evolutions. Attempts have been made to categorize them roughly into two main types: eastern Pacific (EP; or cold tongue) and central Pacific (CP; or warm pool) El Niño events. In this study, a modified version of the Zebiak–Cane (MZC) coupled model is used to examine the dynamics of these two types of El Niño events. Linear eigenanalysis of the model is conducted to show that there are two leading El Niño–Southern Oscillation (ENSO) modes with their SST patterns resembling those of two types of El Niño. Thus, they are referred to as the EP and CP ENSO modes. These two modes are sensitive to changes in the mean states. The heat budget analyses demonstrate that the EP (CP) mode is dominated by thermocline (zonal advective) feedback. Therefore, the weak (strong) mean wind stress and deep (shallow) mean thermocline prefer the EP (CP) ENSO mode because of the relative dominance of thermocline (zonal advective) feedback under such a mean state. Consistent with the linear stability analysis, the occurrence ratio of CP/EP El Niño events in the nonlinear simulations generally increases toward the regime where the linear CP ENSO mode has relatively higher growth rate. These analyses suggest that the coexistence of two leading ENSO modes is responsible for two types of El Niño simulated in the MZC model. This model result may provide a plausible scenario for the observed ENSO diversity.

Meteorology & Atmospheric Sciences↗

Towards Universal Non-Dimensional Characterization of the Oscillatory Dynamics of Wind Turbine Rotors of Multiple Sizes

One concern in the field of Horizontal Axis Wind Turbines (HAWTs) is what control strategies are needed to handle gust pulses in the wind to prevent extreme oscillations of the blades to reduce fatigue stress, prevent blade rupture, and extend the turbine’s operational life. In order to design innovative control strategies to modify the blade’s oscillatory response, it is crucial to establish the fundamental vibrational behavior of the blades when excited by gust pulses of different frequencies and amplitudes present in the fluctuating wind inflow. In a series of previous works, the authors presented a novel Reduced-Order Characterization (ROC) technique that provided an energy-based characterization of the fundamental modes of oscillation of wind turbine rotors when excited by combinations of wind gust pulses of different frequencies and amplitudes. The main focus of the present work is to extend these original notions of energy-based ROC to a universal technique expressed in terms of non-dimensional quantities that could be applied to turbines of any size, operating in any set of wind conditions, as long as they share geometrical and material similarity. The ROC technique provides a simple formula that is capable of predicting the dominant vibrational modes of a blade with sufficient precision to be useful in the determination of a control decision that can be computed in real time, an aspect of fundamental importance in dealing with rapid fluctuations in wind conditions.

Yates, North (ORCID:000900052204261X)↗

Tunable Mode Coupling in Nanocontact Spin-Torque Oscillators

Recent experiments on spin-torque oscillators have revealed interactions between multiple magneto-dynamic modes, including mode coexistence, mode hopping, and temperature-driven crossover between modes. The initial multimode theory indicates that a linear coupling between several dominant modes, arising from the interaction of the subdynamic system with a magnon bath, plays an essential role in the generation of various multimode behaviors, such as mode hopping and mode coexistence. In this work, we derive a set of rate equations to describe the dynamics of coupled magneto-dynamic modes in a nanocontact spin-torque oscillator. Here, expressions for both linear and nonlinear coupling terms are obtained, which allow us to analyze the dependence of the coupled dynamic behaviors of modes on external experimental conditions as well as intrinsic magnetic properties. For a minimal two-mode system, we further map the energy and phase difference of the two modes onto a two-dimensional phase space and demonstrate in the phase portraits how the manifolds of periodic orbits and fixed points vary with an external magnetic field as well as with the temperature.

36 MATERIALS SCIENCE↗

The electronic properties and lattice dynamics of (Na{sub 0.5}Bi{sub 0.5})TiO{sub 3}: From cubic to tetragonal and rhombohedral phases

The structural, electronic and dynamical properties of the cubic, tetragonal and rhombohedral phases of a lead-free ferroelectrics, (Na{sub 0.5}Bi{sub 0.5})TiO{sub 3} (NBT), have been studied with a density functional formalism. The direct band gap is determined to be 2∼3 eV for three phases, suggesting them to be good optical material. The equilibrium structures were given, and the importance of Bi atom in the low-symmetry ferroelectric phases were investigated with the electron localization functions analysis. The vibration modes at the Γ point were calculated to provide a basis for analyzing the Raman and IR spectra. Soft modes were found in both the cubic and the tetragonal phases, providing a clue in understanding the ferroelectric phase transition in NBT.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Point defect weakened thermal contraction in monolayer graphene

We investigate the thermal expansion behaviors of monolayer graphene and three configurations of graphene with point defects, namely the replacement of one carbon atom with a boron or nitrogen atom, or of two neighboring carbon atoms by boron-nitrogen atoms, based on calculations using first-principles density functional theory. It is found that the thermal contraction of monolayer graphene is significantly decreased by point defects. Moreover, the corresponding temperature for negative linear thermal expansion coefficient with the maximum absolute value is reduced. The cause is determined to be point defects that enhance the mechanical strength of graphene and then reduce the amplitude and phonon frequency of the out-of-plane acoustic vibration mode. Such defect weakening of graphene thermal contraction will be useful in nanotechnology to diminish the mismatching or strain between the graphene and its substrate.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Ultrafast spectroscopy of super high frequency mechanical modes of doubly clamped beams

We use ultrafast pump-probe spectroscopy to study the mechanical vibrations in the time domain of doubly clamped silicon nitride beams. Beams with two different clamping conditions are investigated. Finite element method calculations are performed to analyse the mode spectra of both structures. By calculating the strain integral on the surface of the resonators, we are able to reproduce the effect of the detection mechanism and identify all the measured modes. We show that our spectroscopy technique combined with our modelling tools allow the investigation of several different modes in the super high frequency range (3-30 GHz) and above, bringing more information about the vibration modes of nanomechanical resonators.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

North Pacific meridional mode has larger impacts on El Niño evolution than the March Madden-Julian Oscillation

The El Niño–Southern Oscillation (ENSO) is a key driver of global climate variability. Early-season westerly wind bursts (WWBs) have long been suggested to be important for ENSO evolution and diversity, with the Madden-Julian Oscillation (MJO) among the main sources of WWBs. However, MJO’s contribution to ENSO evolution has been difficult to quantify. Here, using an ensemble hindcast approach specifically designed to isolate internal atmospheric variability, we evaluate the influences of March MJO on subsequent ENSO development. Our results show that the March MJO, under favorable background conditions, by itself has limited impacts on ENSO due to weak equatorial air-sea coupling in spring. In comparison, the North Pacific Oscillation–induced meridional mode exerts a more sustained influence on ENSO evolution. A cyclonic circulation anomaly over Hawaii, associated with the Pacific-North American pattern, also plays a role. These findings suggest that March MJO activity alone may not be a reliable predictor for ENSO evolution, but underscore the importance of North Pacific atmospheric variability.

Science & Technology - Other Topics↗

Theoretical study of NMR, infrared and Raman spectra on triple-decker phthalocyanines

Electronic structures and magnetic properties of multi-decker phthalocyanines were studied by theoretical calculation. Electronic structures, excited processes at multi-states, isotropic chemical shifts of {sup 13}C, {sup 14}N and {sup 1}H-nuclear magnetic resonance (NMR), principle V-tensor in electronic field gradient (EFG) tensor and asymmetry parameters (η), vibration mode in infrared (IR) and Raman spectra of triple-decker phthalocyanines were calculated by density functional theory (DFT) and time-dependent DFT using B3LYP as basis function. Electron density distribution was delocalized on the phthalocyanine rings with electron static potential. Considerable separation of chemical shifts in {sup 13}C, {sup 14}N and {sup 1}H-NMR was originated from nuclear spin interaction between nitrogen and carbon atoms, nuclear quadrupole interaction based on EFG and η of central metal under crystal field. Calculated optical absorption at multi-excited process was derived from overlapping π-orbital on the phthalocyanine rings. The vibration modes in IR and Raman spectra were based on in-plane deformation and stretching vibrations of metal-ligand coordination bond on the deformed structure.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Surveillance and diagnostics of the beam mode vibrations of the Ringhals PWRs

Surveillance of core barrel vibrations has been performed in the Swedish Ringhals PWRs for several years. This surveillance is focused mainly on the pendular motion of the core barrel, which is known as the beam mode. The monitoring of the beam mode has suggested that its amplitude increases along the cycle and decreases after refuelling. In the last 5 years several measurements have been taken in order to understand this behaviour. Besides, a non-linear fitting procedure has been implemented in order to better distinguish the different components of vibration. By using this fitting procedure, two modes of vibration have been identified in the frequency range of the beam mode. Several results coming from the trend analysis performed during these years indicate that one of the modes is due to the core barrel motion itself and the other is due to the individual flow induced vibrations of the fuel elements. In this work, the latest results of this monitoring are presented. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Theoretical investigation of the dielectric-filled relativistic magnetron

The fundamental mode frequency of a dielectric-filled relativistic magnetron is studied theoretically by the method of the equivalent circuit, and an exact fundamental mode frequency formula is derived. To prove the validity of the theoretical formula, simulation investigation is performed. The simulation results agree well with the theoretical formula, and the relative error does not exceed 3%. The comparative results verify the creditability of the theoretical formula.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

System studies of rf current drive for MST

Two rf schemes are being studied on the MST reversed field pinch for their potential in current profile control experiments. MHD modeling has shown that a substantial externally-driven off axis parallel current can improve stability of the dominant core tearing modes. A radially localized axisymmetric population of fast electrons has been observed by SXR emission during LH injection (100kW at 800MHz), and is consistent with CQL3D modeling which predicts a small driven current. Computational work suggests that doubling the input power will statistically improve the LH-induced SXR signal to background ratio, and that about 2MW of injected power (an order of magnitude increase) will drive enough current for stabilization of tearing modes. Additionally, a 1 MW 5.5 GHz electron Bernstein wave (EBW) experiment is under construction, which utilizes a very simple and compact antenna compatible with the demands of the RFP. EBW allows access to electron cyclotron heating and current drive in the overdense plasma. Coupling of the external electromagnetic wave to the EBW has been demonstrated, and initial tests at {approx}100kW power have produced a small, localized xray flux consistent with rf heating and high diffusivity of fast electrons. Computational work is currently underway to answer the very important questions of how much power is required, and what level of electron diffusivity is tolerable, to generate a consequential amount of EBW current.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗