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DOE OSTI2020

Analysis of Nuclear Materials on Both Sides of Regulatory Control: from IAEA Safeguards to Global Counter-Nuclear Smuggling

Global nuclear security is dependent upon the sustained and verifiable control of radiological and nuclear (R/N) materials within nuclear facilities, under the administrative purview of national governments. It is the responsibility of each country to account for their R/N materials holdings and to ensure that they do not escape regulatory control and fall into the wrong hands. The Office of Nuclear Smuggling Detection and Deterrence (NSDD) is tasked with providing support to foreign partners in developing the tools and expertise to detect, disrupt, and investigate R/N materials encountered out of regulatory control, in such circumstances as at border crossings and other checkpoints, or in the course of routine policework. Thankfully, such incidents are infrequent, and NSDD continues to work bilaterally with partner countries to strengthen their capabilities to combat nuclear smuggling and trafficking incidents in their countries. For the vast majority of R/N materials that remain under regulatory control, however, it is critical that their safe storage and use be independently verified. Even a single loss incident of R/N materials, particularly of special nuclear materials (highly-enriched uranium and plutonium) has the potential to cause a catastrophe. How can the international community be assured that R/N materials currently under national regulatory control remain there?

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

DOE OSTI2022

IRAD-MPE Radiological and Nuclear Security Threats (Day 1) [Slides]

This module is designed to enhance awareness regarding radiological and nuclear security threats and the types of radioactive materials that can be used for criminal purposes or terrorist acts. The goals are to: (1) Review the Threat Assessment Process for MPEs, (2) Recognize Potential Radiological and Nuclear Security Threats, (3) Understand the basics of Radiological Dispersal Devices (RDD) and Radiological Exposure Devices (RED), (4) Learn about Medical, Commercial, and Naturally Occurring Radioactive Materials (NORM) sources, and (5) Understand the term Material Out of Regulatory Control (MORC).

61 RADIATION PROTECTION AND DOSIMETRY↗

DOE OSTI2025

Three-Channel Sunphotometer Cloud Mode Value-Added Product Report

A primary source of uncertainty in Earth system model (ESM) predictions is the representation of cloud processes and associated cloud feedback. Several fundamental cloud properties critical to the understanding of aerosol-cloud interactions are poorly constrained by observations, with key deficiencies in our observations of cloud and precipitation droplet sizes and cloud optical depth. Observations of these cloud properties are often challenging to estimate from remote-sensing platforms and costly to obtain from in situ aircraft. Nevertheless, observations of boundary-layer clouds, and improved knowledge of stratocumulus cloud (Sc) processes, are especially important to ESM advancement. This is because these clouds have extensive coverage and exert controls on boundary-layer dynamics and the global radiative energy balance.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

Excited-State and Nonadiabatic Molecular Dynamics Methods with Broad Applicability

Electronically excited states play a pivotal role in the capture, transformation, storage, and emission of radiative energy. Despite much recent progress for small model systems, excited state properties and dynamics in many larger molecular devices and materials have remained elusive for experiment and theory. Nonadiabatic transitions between electronic states turn radiative energy into heat and are particularly difficult to control. This project aims to develop new electronic structure and nonadiabatic molecular dynamics (NAMD) methods to simulate, predict, and ultimately control the flow and transformation of excitation energy in a wide-range of light-driven molecular devices such as dyes, photocatalysts, and fluorescence emitters.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2021

Deciphering Time-Dependent DNA Damage Complexity, Repair, and Oxygen Tension: A Mechanistic Model for FLASH-Dose-Rate Radiation Therapy

Irradiation with ultrahigh dose rates (FLASH) has reemerged as a promising radiation therapy approach to effectively lower potential damage burden on normal tissue without sacrificing tumor control. However, the large number of recent FLASH studies have been conducted under vastly different experimental conditions and circumstances (ie, investigated biological endpoint, radiation quality, and environmental oxygen level), with unverified biological mechanisms of action and unexplored interplay effect of the main dependencies. To facilitate radiobiological investigation of FLASH phenomena and assessment of clinical applicability, we present an extension of the mechanistic radiobiological model “UNified and VERSatile bio response Engine” (UNIVERSE).

62 RADIOLOGY AND NUCLEAR MEDICINE↗

DOE OSTI2026

Overview of the ASDEX Upgrade results

After a 26-month vent ASDEX Upgrade (AUG) went back in operation with a newly designed upper W-divertor suitable for alternative divertor configurations (featuring in-vessel coils and cryo-pump). Parameter scans and an extensive set of measurements were obtained and their interpretation is ongoing. Prompted by the ITER wall change, dedicated experiments on non-boronized plasma startup were contrasted to that employing asymmetric and more symmetric boronizations. The asymmetric boronization proved to be as beneficial as the more symmetric one, which is in contrast to previous model calculations assuming perfect sticking of boron (measurements suggest sticking ≈ 0.3). In the startup phase also the impurity influxes at the outboard limiters were investigated contrasting the unboronized case featuring cold edges (low- Z radiation) to the boronized case, in which the lifetime of the boron layers could be estimated. Pedestal stability investigations revealed that the quasi-continuous exhaust (QCE) regime is obtained when ballooning modes are active in the vicinity of the separatrix and the global peeling-ballooning stability is high enough. Thus, at high enough shaping and high gas flux both can be achieved and QCE is a consequence. The closely related enhanced D-alpha (EDA) mode is not clearly distinguishable from QCE, e.g. the quasi-coherent mode characteristic for EDA also shows up in QCE. In QCE the impurity transport is behaving benign as could be measured for Ne with a novel analysis method making use of a comprehensive set of CXRS measurements. For high radiative fractions the regime of the X-point radiator (XPR) is accessible at AUG and the understanding of its access conditions and behaviour is further developed. Due to the localized radiative cooling at the X-point the XPR can be well diagnosed and thus controlled. For negative triangularity shapes, further experiments at increased shaping resulted in strongly heated L-mode plasmas avoiding ELMs. Two integrated modelling approaches towards ITER suggested that core W-accumulation will be no issue for ITER and that the fusion yield in ITER may be Q = 12 (i.e. ITPA20-IL scaling is too pessimistic). Further, investigations of the ITER ramp-down in AUG provide insights into maintaining position control. Various aspects of shattered pellet injection were investigated in AUG and one of the results show that with increasing Ne fraction the radiation during the current quench increases and the current decay becomes faster.

ASDEX Upgrade↗

DOE OSTI2021

Moving Beyond the Standard of Care: Accelerate Testing of Radiation-Drug Combinations

Radiation therapy is a major treatment modality used in > 60% of cancer patients as definitive local treatment for inoperable locoregionally confined tumors and as palliative therapy. Although cytotoxic chemotherapy enhances the effectiveness of treatment, the benefit over radiation therapy alone is modest. There is a need to enhance the effectiveness of local tumor control over what sequentially or concurrently administered cytotoxic chemotherapy provides. Although many biological pathways are known to enhance the effectiveness of radiation therapy, there is currently a paucity of drugs approved for use in combination. Several clinical trials have tested the effectiveness of combining targeted agents or immunotherapies with radiation therapy, but the results of these trials have been negative, likely stemming from the relative lack of preclinical evidence using appropriate experimental standardization or model systems. Accelerating the identification of agents tested in an appropriate clinical context and experimental systems or models would greatly enhance the potential to bring forward early testing of drugs that would not only be safe but also more effective. This article provides an overview of the opportunities and challenges of developing therapeutics to combine with radiation therapy, and some guidance toward preclinical and early clinical testing to improve the chance that advanced phase testing of drug-radiation combinations would be successful in the long term.

62 RADIOLOGY AND NUCLEAR MEDICINE↗

DOE OSTI2021

High Temperature Alloys Session 1

Section III Division 5 overview Code materials VHTR materials 617 and 800H Qualification of additional materials Corrosion effects Operating plant experience Additive/advanced manufacturing Control rod sleeves Pressure Vessel Steels Allowed materials Elevated temperature limits and properties Supply chain Welding Radiation damage

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2022

Processes controlling helium bubble dynamics at varying temperatures in simulated radioactive materials

Alpha-radiation damage is known to degrade materials exposed to harsh radiation environments via swelling and embrittlement by nano-scale helium bubbles. How these bubbles grow under varying temperature is essential to understanding and predicting material failure and optimization. Using in situ X-ray scattering, we probed ≈1012 bubbles before, during and after annealing at different temperatures in He-implanted aluminum to reveal a critical growth activation temperature that depends strongly on the helium implantation conditions. An analysis of the data aided by our molecular dynamics simulations identifies multiple temperature-dependent bubble growth mechanisms above and below the critical growth activation temperature. Moreover, the irreversible bubble growth that occurs after annealing for ≈4 h was evaluated using dislocation dynamics and found to negligibly affect the yield strength but may affect subsequent bubble growth at temperature. These in situ results provide valuable insight into bubble growth never observed before and reveal, for the first time, bubble shrinkage after cooling.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Chiral catalysis of nuclear fusion in molecules

At low energies, nuclear fusion is strongly affected by electron screening of the Coulomb repulsion among the fusing nuclei. It may thus be possible to catalyze nuclear fusion in molecules (i.e., to fuse specific nuclei in situ) through quantum control of electron wave functions in intense laser fields. The circularly polarized (chiral) laser field can effectively squeeze the electron wave functions, greatly enhancing the screening in the spatial region relevant for the fusion process. Here, we estimate the corresponding fusion probabilities, and find that the proposed chiral catalysis of nuclear fusion in molecules may be observable, potentially with important practical applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2025

Design of a remote-controlled mount for IOTA’s magnet undulator

The SLAC undulator is essential for studies of synchrotron radiation produced by a single electron in IOTA. Since IOTA is meant for different experiments, the undulator is not always needed, so it must be pushed and pulled back depending upon the nature of the experiment. Moving the undulator manually result in significant time loss about 30 minutes for the controlled access, and about 30 minutes to achieve beam injector in IOTA. Because the operation is done manually is not easy to ensure a good repeatability of the undulator position. That’s why IOTA’s team decided to set-up a completely remote-controlled mount.

42 ENGINEERING↗

DOE OSTI2021

(Paper) TRIPWIRE: Multi-modal Distributed Sensing For Repository Verification

Underground geological repositories for storing used nuclear fuel are being planned and developed around the world. Research is being performed to understand technical aspects of sealing entombed materials and underground repositories to ensure the radiological and nuclear materials remain contained. To support safeguards verification for these facilities research at Idaho National Laboratory (INL) is underway to develop and demonstrate a multi-modal sensor system, TRIPWIRE, for containment verification in inaccessible radiological and nuclear waste repositories. The TRIPWIRE system will continuously monitor ionizing radiation and electromagnetic fields in the vicinity of emplaced nuclear materials buried in a repository, reporting on disturbances with a real-time alarm control station. The system will use long-length scintillating fiber bundles (SFBs) to perform area radiation monitoring; these will be coupled to kilometer-scale multimodal optical communication fibers – all light sensors and electronic components used with this system will be located above ground. Electromagnetic fields, and changes in local dielectric conditions caused by intrusion and soil movement, will be monitored using commercial grade, ported "leaky" coaxial cables (PCCs), with control electronics also located above ground. Tamper-indicating self-diagnostic assessments will be done using optical and electronic time domain reflectometry in the SFBs and PCCs, respectively. The result will be a long, kilometer-scale multi-modal SFB-PCC system. Simulation and modeling are being used to inform the work and a demonstration of the system's utility is planned at a nuclear storage facility in the future.

98 - NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL↗

DOE OSTI2022

Progress of Tripwire: Multi-Modal Distributed Sensing for Repository Verification

This project is developing and demonstrating a multi-modal sensor system, TRIPWIRE, for containment verification in inaccessible radiological and nuclear waste repositories. The TRIPWIRE system will continuously monitor ionizing radiation and electromagnetic fields in the vicinity of emplaced nuclear materials buried in a repository, reporting on disturbances with a real-time alarm control station. The system will use long-length scintillating fiber bundles (SFBs) to perform area radiation monitoring; these will be coupled to kilometer-scale multimodal optical communication fibers – all light sensors and electronic components used with this system will be located above ground. Electromagnetic fields, and changes in local dielectric conditions caused by intrusion and soil movement, will be monitored using commercial grade, ported "leaky" coaxial cables (PCCs), with control electronics also located above ground. This paper documents the results of the simulations and modeling efforts that have helped identify the optimal placement of the SFBs. Additionally, the paper includes the current progress on the multi-modal SFB-PCC system, including the fabrication of long-length (>3-m) fibers and their coupling to optical fibers.

98 - NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL↗

DOE OSTI2022

Progress of Tripwire: Multi-modal Distributed Sensing for Repository Verification

98 - NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL↗

DOE OSTI2023

A Novel Platform for Evaluating Dose Rate Effects on Oxidative Damage to Peptides: Toward a High-Throughput Method to Characterize the Mechanisms Underlying the FLASH Effect

High dose rate radiation has gained considerable interest recently as a possible avenue for increasing the therapeutic window in cancer radiation treatment. The sparing of healthy tissue at high dose rates relative to conventional dose rates, while maintaining tumor control, has been termed the FLASH effect. Although the effect has been validated in animal models using multiple radiation sources, it is not yet well understood. Here, in this work, we demonstrate a new experimental platform for quantifying oxidative damage to protein sidechains in solution as a function of radiation dose rate and oxygen availability using liquid chromatography mass spectrometry. Using this reductionist approach, we show that for both X-ray and electron sources, isolated peptides in solution are oxidatively modified to different extents as a function of both dose rate and oxygen availability. Our method provides an experimental platform for exploring the parameter space of the dose rate effect on oxidative changes to proteins in solution.

61 RADIATION PROTECTION AND DOSIMETRY↗

DOE OSTI2025

Control of wakefield in sub-THz dielectric-lined waveguides using multiple-bunch excitation

Beam-driven wakefield accelerators offer the potential to achieve accelerating fields approaching the sub-GV/m range, paving the way for compact and cost-effective next-generation high-energy colliders. This method typically employs a two-bunch system: a drive bunch that excites an electromagnetic wakefield in a solid-state or plasma medium, and a witness bunch that extracts energy from the wake for acceleration. Our research focuses on two key challenges in wakefield acceleration using structures. First, we investigate strategies to suppress transverse instabilities by employing non-cylindrical geometries that damp dipole modes. Second, we explore methods to precisely terminate the wakefield after the interaction region, thereby improving the efficiency of energy transfer. This paper presents detailed simulation results and the corresponding experimental design developed to validate these concepts. Furthermore, the proposed experiment will be carried out at the Argonne Wakefield Accelerator (AWA) facility, focusing on controlling wakefield duration through tailored drive and witness bunch configurations and evaluating dielectric-lined structures with non-cylindrical cross sections.

43 PARTICLE ACCELERATORS↗

DOE OSTI2023

Benchmarking magnetised three-wave coupling for laser backscattering: analytic solutions and kinetic simulations

Understanding magnetised laser–plasma interactions is important for controlling magneto-inertial fusion experiments and developing magnetically assisted radiation and particle sources. For nanosecond pulses at non-relativistic intensities, interactions are dominated by coherent three-wave interactions, whose nonlinear coupling coefficients became known only recently when waves propagate at oblique angles with the magnetic field. In this paper, backscattering coupling coefficients predicted by warm-fluid theory are benchmarked using particle-in-cell simulations in one spatial dimension, and excellent agreements are found for a wide range of plasma temperatures, magnetic field strengths and laser propagation angles, when the interactions are mediated by electron-dominant hybrid waves. Systematic comparisons between theory and simulations are made possible by a rigorous protocol. On the theory side, the initial boundary value problem of linearised three-wave equations is solved, and the transient-time solutions allow the effects of growth and damping to be distinguished. On the simulation side, parameters are carefully chosen and calibration runs are performed to ensure that comparisons are well controlled. Fitting simulation data to analytical solutions yields numerical growth rates that match theory predictions within error bars. Although warm-fluid theory is found to be valid for a wide parameter range, genuine kinetic effects have also been observed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2020

Evaluation of radiation hardness of High-Voltage silicon vertical JFETs

In the future ATLAS Inner Tracker, each silicon strip module will be equipped with a switch able to separate the high voltage supply from the sensor in case the latter becomes faulty. The switch, placed in between the HV supply and the sensor, needs to sustain a high voltage in its OFF state, to offer a low resistance path for the sensor leakage current in the ON state, and be radiation hard up to 1.2 * 10 15 neq/cm 2 along with other requirements. While GaN JFETs have been selected as suitable rad-hard switch, a silicon vertical HV-JFET was developed by Brookhaven National Laboratory as an alternative option. Pre-irradiation results showed the functionality of the device and proved that the silicon HV-JFET satisfied the pre-irradiation requirements for the switch. To assess its suitability after irradiation, a few p-type HV-JFETs have been neutron irradiated at Jozef Stefan Institute (JSI, Ljubljana, Slovenia). Overall, this paper reports the static characterization of these irradiated devices and the TCAD numerical simulations used to get an insight of the physics governing the post-irradiation behaviour.

47 OTHER INSTRUMENTATION↗