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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 307 records · Page 17
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Atom-at-a-Time Radioactive Molecule Identification: Looking toward Studies of Superheavy Elements

The chemical behavior of superheavy elements (SHEs, Z > 103) remains poorly understood. Their chemical properties are expected to deviate from established trends, challenging the predictive power of the periodic table. To investigate these elements experimentally, they must first be synthesized through nuclear reactions and then quickly subjected to chemical studies before they decay. Given the low production rates of these reactions and the need for measurements on an atom-at-a-time basis, innovative techniques are needed. Here, to address these challenges, a novel gas-phase chemistry method has been developed at Lawrence Berkeley National Laboratory, utilizing the Berkeley Gas-filled Separator and FIONA. This technique enables the production, identification, and study of molecular species formed by SHEs. As a proof of concept, we present measurements on the formation and identification of 151,152 HoO + molecules, demonstrating the capability to study the production of radioactive molecules under controlled conditions and directly identify them via their mass-to-charge ratio. These measurements validate the effectiveness of this technique for low-statistics SHE studies, highlighting the potential of this approach to ignite the next generation of experimental SHE chemistry research, offering a path to re-evaluate SHE placement on the periodic table.

Chemistry↗
NASA NTRS1985

Elemental technetium as a cosmic-ray clock

Several radioactive isotopes have been proposed as clocks for the study of the mean cosmic ray confinement time, T sub e. Measurements of Be-10 and Al-26 give a value for T sub e of about 10 Myr when one uses a leaky box cosmic ray propagation model. It is important to obtain additional measurements of T sub e from other radioactive isotopes in order to check whether the confinement is the same throughout the periodic table. The possible use of Tc (Z = 43) as a cosmic clock is investigated. Since all isotopes of Tc are radioactive, one might be able to group these isotopes and use the elemental abundance as a whole. The results of the calculations are somewhat inconclusive for two reasons. First, the beta + decay half lives of two of the Tc isotopes relevant to our calculation are not known. Second, the dependence of the Tc abundance on the mean confinement time is rather weak when one considers the number of events expected in 4 trays of plastic track detectors. However, a future, finite measurement of the Beta + half lives and the possible use of the entire collecting area of the HNC to detect Tc nuclei could make the use of Tc as a cosmic ray clock more attractive.

Drach, J.↗
NASA NTRS1988

Gamma radiation background measurements from Spacelab 2

A Nuclear Radiation Monitor incorporating a NaI(Tl) scintillation detector was flown as part of the verification flight instrumentation on the Spacelab 2 mission, July 29 to August 6, 1985. Gamma-ray spectra were measured with better than 20 s resolution throughout most of the mission in the energy range 0.1 to 30 MeV. Knowledge of the decay characteristics and the geomagnetic dependence of the counting rates enable measurement of the various components of the Spacelab gamma-ray background: prompt secondary radiation, Earth albedo, and delayed induced radioactivity. The status of the data analysis and present relevant examples of typical background behavior are covered.

Paciesas, William S.↗
NASA NTRS1989

Gamma radiation background measurements from Spacelab 2

A Nuclear Radiation Monitor incorporating a NaI(Tl) scintillation detector was flown as part of the verification flight instrumentation on the Spacelab 2 mission, July 29 to August 6, 1985. Gamma-ray spectra were measured with better than 20 s resolution throughout most of the mission in the energy range 0.1 to 30 MeV. Knowledge of the decay characteristics and the geomagnetic dependence of the counting rates enable measurement of the various components of the Spacelab gamma-ray background: prompt secondary radiation, earth albedo, and delayed induced radioactivity. The status of the data analysis and present relevant examples of typical background behavior are covered.

Paciesas, William S.↗
DOE OSTI2025

Technical Assessment of Off-Gas System Technologies for Potential Use in Molten Salt Reactors

Molten salt reactors (MSRs) are a class of Generation IV advanced reactor technologies aimed to enhance and improve the safety, fuel utilization and cost-effectiveness of nuclear power generation. MSR concepts are based on using a molten salt mixture as a primary nuclear reactor coolant, while the fuel can be either directly dissolved in the coolant (i.e., fluid-fueled) or can be in a separate solid form (i.e., salt-cooled solid-fueled). MSRs can be operated in either thermal or fast neutron spectra, as simple fissile convertors, or breeder reactors (e.g., utilizing both fissile and fertile fuels), as well as accelerator-driven sub-critical reactors or transuranic element burners. Operation of MSRs will necessitate management and treatment of the off-gas streams released to the headspace of the reactor where, in some designs, a cover gas can be circulated to remove certain fission products and maintain an inert atmosphere. An inert MSR cover gas swept over or sparged into the salt will confine radionuclides emerging from the free surface, including radioactive noble and non-noble gases, aerosols, and volatile species. The elements and compounds of these species will have a wide range of thermochemical and physical properties, some of which will decay to different products in the off-gas stream. Therefore, system components used to manage and treat MSR off-gas streams will need to be robust under dynamic reactor and chemistry conditions to support adequate reactor performance by managing the composition and species in the salt coolant and cover gas space. Off-gas system components would perform as a radionuclide boundary to the reactor vessel and a primary means for preventing radionuclide release; therefore, they are of high safety significance for MSR operations. This report reviews various technologies and materials for potential implementation in the design of an MSR off-gas system per a general conceptual framework. The reviewed technologies operate based on scrubbing, capture, delay, or separation of species in the off-gas stream. These include molten hydroxide scrubbers, solid sorbents, delay off-gas systems, particle traps, and cryogenic distillation. Since aspects of an off-gas system will be design-specific, the approach is to provide general discussions on attributes of these technologies and materials, including target off-gas stream species, operational parameters and conditions of importance to decontamination factors, implementation maturity, system component monitoring, potential off-normal conditions and considerations for waste products. The information aims to support the U.S. Nuclear Regulatory Commission in their safety evaluations for MSR designs.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
NASA NTRS1974

Neutron and proton activation measurements from Skylab

Radioactivity induced by high-energy protons and secondary neutrons (from nuclear interactions) in various samples returned from different locations in Skylab was measured directly by gamma-ray spectroscopy measurements of decay gamma rays from the samples. Incident fluxes were derived from the activation measurements, using known nuclear cross-section. Neutron and proton flux values were found to range from 0.2 to 5 particles/sq cm-sec, depending on the energy range and location in Skylab. The thermal neutron flux was less than 0.07 neutrons/sq cm-sec. The results are useful for data analysis and planning of future high-energy astronomy experiments.

Fishman, G. J.↗
NASA NTRS2002

Potential Operating Orbits for the SAFE-400

Safety must be ensured during all phases of space fission system design, development, fabrication, launch, operation, and shutdown. One potential space fission system application is fission electric propulsion (FEP), in which fission energy is converted into electricity and used to power high efficiency (Isp is greater than 3000s) electric thrusters. For these types of systems it is important to determine which operational scenarios ensure safety while allowing maximum mission performance and flexibility. Space fission systems are essentially non-radioactive at launch, prior to extended operation at high power. Once high power operation begins, system radiological inventory steadily increases as fission products build up. For a given fission product isotope, the maximum radiological inventory is typically achieved once the system has operated for a length of time equivalent to several half-lives. After that time, the isotope decays at the same rate it is produced, and no further inventory builds in. For an FEP mission beginning in Earth orbit, altitude and orbital lifetime increase as the propulsion system operates. Two simultaneous effects of fission propulsion system operation are thus (1) increasing fission product inventory and (2) increasing orbital lifetime. Phrased differently, as fission products build up, more time is required for the fission products to naturally convert back into non-radioactive isotopes. Simultaneously, as fission products build up, orbital lifetime increases, providing more time for the fission products to naturally convert back into non-radioactive isotopes. Operational constraints required to ensure safety can thus be quantified.

Houts, Mike↗
NASA NTRS1997

AXAF Detector Backgrounds Produced By Cosmic Ray Protons

One of the science instruments on the Advanced X-ray Astrophysics Facility (AXAF), planned for launch in 1998 into a highly elliptical (10,000 km x 140,000 km) orbit, is a microchannel plate High Resolution Camera (HRC). This detector is designed to provide imaging and spectroscopic observations of x-rays emitted by stellar sources in the 0.1 to 10 keV energy range. Described here are analyses made to determine the expected time-dependent detector background from prompt and delayed (activation) radiation initiated by galactic cosmic-ray (GCR) proton interactions in the spacecraft and payload. Numerical simulations were made using the coupled set of Monte Carlo radiation transport codes, analysis software, and data bases shown. The major codes are HETC for nucleon-meson transport, EGS for simulating electromagnetic cascades, and MORSE for low-energy (less than 15 MeV) neutron transport. The simulation follows the transport history of photons in the energy range from - 100 GeV down to approx. 0.1 keV due to gamma-ray sources from neutral pion decay, high-energy (spallation) collisions, and low-energy neutron inelastic scattering and capture reactions. Also included is radioisotope production and the tracking of gamma-rays, electrons, and positrons from induced radioactivity.

Armstrong, T. W.↗
NASA NTRS1992

Radioactive 7Be materials flown on LDEF

Following the discovery of the atmospheric cosmogenic radionuclide Be-7 on the Long Duration Exposure Facility (LDEF), we began a search for other known nuclides produced by similar mechanisms. None of the others have the narrow gamma-ray line emission of Be-7 decay which enable its rapid detection and quantification. A search for Be-10 atoms on LDEF clamp plates using accelerator mass spectrometry is described. An unexpected result was obtained.

Gregory, John C.↗
DOE OSTI2025

Detection and quantification of trace technetium in the presence of molybdenum using laser-induced breakdown spectroscopy

Technetium (Tc) is a very important element that is encountered in many aspects, from its presence in radioactive waste and its potential environmental impact to its use as a medical radioisotope. Its detection and quantification in liquid samples is traditionally cumbersome, involving detailed sample preparation and analysis by mass spectrometry or scintillation. This article demonstrates the first comprehensive emission spectral analysis of Tc from a liquid sample by immobilization in a polymer and analysis by laser-induced breakdown spectroscopy (LIBS). A survey of LIBS spectra was completed to identify the strongest analytical lines for quantification of trace Tc in the presence of Mo. The quantification of Tc in a Mo-containing matrix was selected because Tc radioisotopes are the daughter products of Mo isotope decay. The first reported calibration curves by LIBS are provided with limits of detection and quantification down to 0.710 µg mL −1 and 1.39 µg mL −1 , respectively. Ultimately, this study demonstrated the feasibility of trace Tc quantification using LIBS and will serve as a reference for future research related to monitoring this radioactive species.

Andrews, Hunter B. [Oak Ridge National Laboratory ↗
DOE OSTI2025

Sterile-neutrino search based on 259 days of KATRIN data

Neutrinos are the most abundant fundamental matter particles in the Universe and play a crucial part in particle physics and cosmology. Neutrino oscillation, discovered about 25 years ago, shows that the three known species mix with each other. Anomalous results from reactor and radioactive-source experiments suggest a possible fourth neutrino state, the sterile neutrino, which does not interact through the weak force. The Karlsruhe Tritium Neutrino (KATRIN) experiment, primarily designed to measure the neutrino mass using tritium β-decay, also searches for sterile neutrinos suggested by these anomalies. A sterile-neutrino signal would appear as a distortion in the β-decay energy spectrum, characterized by a discontinuity in curvature (kink) related to the sterile-neutrino mass. This signature, which depends only on the shape of the spectrum rather than its absolute normalization, offers a robust, complementary approach to reactor experiments. Here we report the analysis of the energy spectrum of 36 million tritium β-decay electrons recorded in 259 measurement days within the last 40 eV below the endpoint. The results exclude a substantial part of the parameter space suggested by the gallium anomaly and challenge the Neutrino-4 claim. Together with other neutrino-disappearance experiments, KATRIN probes sterile-to-active mass splittings from a fraction of an eV 2 to several hundred eV 2 , excluding light sterile neutrinos with mixing angles above a few per cent.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1990

Noble gases in the howardites Bholghati and Kapoeta

Analyses of noble gases in whole rock samples of the howardites Bholghati and Kapoeta and grain-size separates of Kapoeta yield evidence for excesses of the Xe isotopes Xe-129 , Xe-131, Xe-132, Xe-134, and Xe-136 in a low-temperture component, similar to lunar excess fission Xe. Such a component may be able to provide chronometric information if the relative abundances of radioactive progenitors (I-129, Pu-244, and U-238) can be determined, but the isotopic spectra obtained are not sufficiently precise to do so. Eucritic clast BH-5 in Bholghati contains Xe produced in situ by the decay of Pu-244. Calculated fission Xe retention ages are 30-70 Ma after the formation of the solar system, consistent with the apparent presence of Sm-146 decay products. Both the clast and the matrix of Bholghati have K-Ar ages of about 2 Ga, suggesting a common thermal event at least that recently.

Swindle, T. D.↗
NASA NTRS1990

A limit on the production of Ni-56 in a type I supernova

The data from the Gamma-Ray Spectrometer on the Solar Maximum Mission satellite have been searched for evidence of gamma-ray line emission from the decay of Co-56 in the type Ia SN, 1986G. No significant flux at either 847 or 1238 keV, the energies of the two strongest decay lines is found. Based on the data, a 3-sigma upper limit of 0.4 solar masses (D/3 Mpc)-squared on the amount of Ni-56 produced in the explosion is set. This value is consistent with radioactive models of type I light curves. For distances less than 3 Mpc, the limit is inconsistent with most models of SN Ia as thermonuclear explosions of white dwarfs.

Matz, Steven M.↗
DOE OSTI2025

First on-line commissioning experiments at the St. Benedict facility

Nuclear beta decays provide an excellent probe of fundamental symmetries due to their mediation by the weak interaction. In particular, precise measurements of these decays provide constraints on the unitarity of the Cabbibo-Kobayashi-Maskawa (CKM) quark-mixing matrix. While superallowed pure Fermi decays currently set the most precise limits, the alternative suite of superallowed mixed mirror decays has been ill-studied. These nuclei can provide an important consistency check of calculation and measurement methods employed for the pure Fermi decays, more critically needed now in the wake of a 2.4σ deviation from unitarity of the CKM matrix. In order to remedy the gap in data for mirror decays, the Superallowed Transition Beta-Neutrino Decay Ion Coincidence Trap (St. Benedict) facility is being commissioned at the University of Notre Dame’s Nuclear Science Laboratory (NSL). In this paper, we present first results of the commissioning of the St. Benedict facility on-line at the TwinSol radioactive beam facility. The results of initial commissioning experiments involving the St. Benedict gas catcher, RF carpet, RFQ ion guide and RFQ cooler-buncher will be presented.

beta decay↗
NASA NTRS2000

Natural transfer of viable microbes in space

The possibility and probability of natural transfer of viable microbes from Mars to Earth and Earth to Mars traveling in meteoroids during the first 0.5 Ga and the following 4 Ga are investigated, including: --radiation protection against the galactic cosmic ray nuclei and the solar rays, dose rates as a function of the meteorite's radial column mass (radius x density), combined with dose rates generated by natural radioactivity within the meteorite; and survival curves for some bacterial species using NASA's HZETRN transport code --other factors affecting microbe survival: vacuum; central meteorite temperatures at launch, orbiting, and arrival; pressure and acceleration at launch; spontaneous DNA decay; metal ion migration --mean sizes and numbers of unshocked meteorites ejected and percentage falling on Earth, using current semiempirical results --viable flight times for the microbe species Bacillus subtilis and Deinococcus radiodurans R1 --the approximate fraction of microbes (with properties like the two species studied) viably arriving on Earth out of those ejected from Mars during the period 4 Ga BP to the present time, and during the 700 Ma from 4.5 to 3.8 Ga. Similarly, from Earth to Mars. The conclusion is that if microbes existed or exist on Mars, viable transfer to Earth is not only possible but also highly probable, due to microbes' impressive resistance to the dangers of space transfer and to the dense traffic of billions of martian meteorites which have fallen on Earth since the dawn of our planetary system. Earth-to-Mars transfer is also possible but at a much lower frequency.

Non-NASA Center↗
NASA NTRS1975

On emission lines in the cosmic gamma-ray background

The composite spectrum of gamma-rays is calculated which results from the decay of Ni-56 to Co-56 to Fe-56 throughout the history of the universe. The results for several cosmological models are presented and compared with the Apollo 15 measurements at low resolution of the cosmic background. The radioactivity background is a significant fraction of the total, and several of its features may be detectable.-

Clayton, D. D.↗
DOE OSTI2024

On-line installation of the Superallowed Transition Beta-Neutrino Decay Ion Coincidence Trap

The Cabibbo-Kobayashi-Maskawa quark mixing matrix currently does not satisfy unitarity at the 2σ-level. This could be the result of an inaccurate value of one or both of its largest matrix elements V us and V ud . In the case of V ud , the most precise measurement is obtained from the f t -value measurements of superallowed beta-transitions between 0 + states. The accuracy of this determination can, in turn, be tested by extracting V ud in other transitions including superallowed transitions between mirror nuclei. The Superallowed Transition Beta-Neutrino Decay Ion Coincidence Trap (St. Benedict) is currently under construction at the Nuclear Science Laboratory of the University of Notre Dame to perform such a determination, with the goal of shedding more light on this tension with unitarity. St. Benedict will take a radioactive ion beam produced by TwinSol , thermalize it in a large volume gas catcher, then transport it in two separate differentially-pumped volumes using a radio-frequency (RF) carpet and a radio-frequency quadrupole (RFQ) ion guide before injecting it in an RFQ trap to create cool ion bunches for injection in the measurement Paul trap. In this paper, we detail the installation of the beam preparation components of St. Benedict, and present the results of the first RIBs successfully stopped and extracted from its gas catcher.

Brodeur, M.↗
NASA NTRS1977

Release of radiogenic gases from the moon

The rate of escape of Ar-40 from the moon is calculated from mass-spectrometer data obtained at the Apollo-17 landing site. It is shown that the rate of loss of Ar from the moon varies significantly over periods the order of one lunation and that the average loss rate is about 3 t/a, corresponding to about 6% of the present rate of Ar production by K decay within the moon. These features of the Ar loss-rate data are interpreted as evidence that this gas originates in the partially molten asthenosphere, which in turn requires that early differentiation only affected the outer 600 to 1,000 km of the moon, trapping significant amounts of radioactive materials in the present asthenosphere. The relationship between the venting of Ar and other radiogenic gases in the lunar atmosphere is discussed.

Hodges, R. R., Jr.↗