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At least 307 records · Page 17

The Experimental Programs on Light Pseudoscalar Meson Decays

The decays of the low-lying pseudoscalar mesons (?0, ?, and ??) allow access to a plethora of physics probes, from measurements of fundamental properties of matter such as the up-down quark mass ratio, to studies of channels that access higher-order terms in Chiral Perturbation theory, to tests of fundamental symmetries and searches for signatures of physics beyond the Standard Model. Several experiments have studied pseudoscalar decays: these experiments include PrimEx in Hall B at Jefferson Lab, A2 at the MAMI electron accelerator facility, the KLOE-II experiment at the DA?NE ?-factory, WASA-at-COSY at the cooler synchrotron COSY storage ring, and BESIII at the Beijing charm factory. In Hall D at Jefferson Lab, PrimEx-eta uses the Primakoff process to measure the ? radiative width using the GlueX spectrometer. In the near future the Jefferson Lab Eta Factory (JEF) experiment will use the GlueX spectrometer with an upgraded forward calorimeter to study ?(?) decay channels with a focus on all-neutral final states. Finally, a proposal for a new experiment, ``Rare Eta Decays with a TPC for Optical Photons'' (REDTOP) utilizing a proton beam on fixed targets, is under development. Highlights from previous and ongoing experiments and plans for future experiments will be presented.

Taylor, Simon↗

Galvanic Corrosion of Carbon Steel and Stainless Steel Couples: Effects of γ-Radiation and Solution Environment - 20348

Galvanic corrosion between carbon steel (CS) and stainless steel (SS) in different aqueous environments was investigated using a combination of electrochemical measurements and surface characterizations. In a basic environment (pH 10.6), the galvanic effect is negligible due to the high corrosion resistance of both alloys. In an acidic to near neutral environment (pH 6.0), the galvanic effect is more significant. Coupling to SS, increasing temperature, and irradiation at this pH have a synergistic effect on the corrosion progression of CS, and their effects vary with time. Initially, the oxidation rate of CS increases after galvanic coupling to SS. Increasing temperature or applying γ-radiation accelerates this oxidation process. However, at a longer time when the saturation limits of metal cations are reached, they also lead to the formation and growth of oxides on CS at a much faster rate, resulting in the suppression of the subsequent Fe dissolution. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Department of Energy’s Atmospheric System Research (ASR) Program’s Workshop on the Future of Atmospheric Large Eddy Simulation (LES): Workshop Report

Large-eddy simulation (LES) is used as a tool to understand physical processes such as turbulence, aerosols, clouds, precipitation, radiation, the interactions among all these, and their interactions with the underlying surface. Over the next 10 years, LES will drive fundamental progress in open scientific questions in these areas as LES is increasingly used to gain understanding of complex interacting physical processes involving atmospheric turbulence. This growth will be driven both by scientific demand and the expansion of computational resources needed to conduct LES, and the form that the growth takes will largely be determined by how computational resources are leveraged for scientific gain. In particular, we suggest that computational resources are likely to be leveraged in two separate but not necessarily distinct ways. On one hand, growth in computational resources will allow LES to be made more routine, that is, performed more frequently, while on the other hand, the computational expense (measured in total floating point operations) afforded to individual LES will expand dramatically, allowing simulations to increase in both domain size and resolution as well as physical detail. Current U.S. Department of Energy (DOE) projects such as LES ARM Symbiotic Simulation and Observation Activity (LASSO) are leading the way in conducting routine LES, building large, public databases that are accessible for data science, sensitivity studies, and training for machine learning. LES will also become more routine as it becomes more accessible for individual researchers to address their scientific questions of interest. Scientific questions addressed by LES over the next 10 years are likely to include cloud organization and aggregation; aerosol cloud interactions and atmospheric chemistry (including geo-engineering); urban-scale LES; atmospheric extreme events, ranging from small-scale severe weather to wildfires; and ocean-wave-atmosphere interactions. Further LES-related research will likely grow significantly in areas related to societal impact studies of air quality and extreme weather events, applications to renewable energy forecasting and resource assessment, and aid in decision-making processes. The growth in the use of LES in atmospheric science research will drive the need for better physical process representations (e.g., cloud aerosol microphysics, radiation, and atmospheric chemistry) at the scales resolved by LES. To date, many of the process representations used by LES have been taken directly from coarser-resolution models. Promising methods for LES process representations include superdroplet and quadrature methods for microphysics, 3D approaches for radiation, and better representation of chemistry and aerosol processes. At LES resolution, land-atmosphere interactions for complex terrains, land cover/types, biogeochemistry, and plant canopy models are needed as an improvement beyond traditional and widely used Monin-Obuhkov similarity theory.

54 ENVIRONMENTAL SCIENCES↗

The impact of r -process heating on the dynamics of neutron star merger accretion disc winds and their electromagnetic radiation

Neutron star merger accretion discs can launch neutron-rich winds of >10 -2 M⊙. This ejecta is a prime site for r-process nucleosynthesis, which will produce a range of radioactive heavy nuclei. The decay of these nuclei releases enough energy to accelerate portions of the wind by ~0.1c. Here, we investigate the effect of r-process heating on the dynamical evolution of disc winds. We extract the wind from a 3D general relativistic magnetohydrodynamic simulation of a disc from a post-merger system. This is used to create inner boundary conditions for 2D hydrodynamic simulations that continue the original 3D simulation. We perform two such simulations: one that includes the r-process heating, and another one that does not. We follow the hydrodynamic simulations until the winds reach homology (60 s). Using time-dependent multifrequency multidimensional Monte Carlo radiation transport simulations, we then calculate the kilonova light curves from the winds with and without dynamical r-process heating. We find that the r-process heating can substantially alter the velocity distribution of the wind, shifting the mass-weighted median velocity from 0.06c to 0.12c. The inclusion of the dynamical r-process heating makes the light curve brighter and bluer at $\sim 1\, \mathrm{d}$ post-merger. However, the high-velocity tail of the ejecta distribution and the early ($\lesssim 1\, \mathrm{d}$) light curves are largely unaffected.

79 ASTRONOMY AND ASTROPHYSICS↗

Wireless System Development for GaN-Based Transmitters for Advanced Nuclear Reactor Environments

The market for consumer electronics is dominated by Si-based electronics. Many Si-based complementary metal–oxide–semiconductor (CMOS) devices are reaching their limitations in terms of switching frequencies, voltages, currents, and temperatures. Furthermore, these devices are widely known to be susceptible to ionizing radiation and neutrons. Advanced nuclear reactors, especially microreactors and small modular reactors, require wireless electronics that can survive larger neutron and gamma doses than Si CMOS. Because of their size, electronics will need to be placed closer to the reactor cores, and cabling capabilities may be limited. However, GaN high-electron-mobility transistors (HEMTs) have been shown to switch faster with higher gains, and they can achieve current and voltage limits beyond traditional Si CMOS. However, they have less market maturity and have undergone less testing. These GaN HEMTs have been shown to survive ionizing radiation with little effects, but the effects of neutron radiation remain widely unknown. In this report, a wireless electronic system capable of supporting multiple radiation-hardened (rad-hard) sensors is presented. The proposed transmission scheme was designed to be simple to increase the likelihood of success in the immature GaN HEMT process and in high-radiation environments. The transmission system was tested using software-defined radios to emulate the transmission scheme before the transmitter circuitry in the GaN process was developed.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

AI-Assisted Conceptual Development of a Pre-Geometric Cosmological Model - An Exercise in AI-Assisted Conceptual Framework Generation, Paper III: Cosmological Structure and Predictions

This paper develops the cosmological consequences of the replication-driven cosmogenesis framework introduced in Paper I and the emergent geometric structure established in Paper II. After the replication epoch freezes out, the coherent sector occupies a finite spectral band and contains a population of excited states. The relaxation of these excited coherent configurations does not produce coherent radiation; instead, all released energy flows into the incoherent substrate, where the randomizer acts as a rapid phase-scrambling mechanism. This process generates an effectively thermal radiation bath, providing a natural reheating mechanism that requires neither inflaton oscillations nor scalar-field potentials, and can be contrasted with standard scenarios of nonperturbative reheating dynamics. Subsequent symmetry-breaking transitions in the coherent vacuum inject additional radiation, yielding a multi-stage thermal history with well-defined energy transfers. We derive the effective equations of state for each component—the cosmological vacuum, the coherent vacuum, and the radiation bath—and show how their interplay produces an FRW-like expansion. The discrete sequence of coherent-state relaxations imprints a distinctive multi-peaked stochastic gravitational-wave background, whose spectral structure reflects the underlying hierarchy of coherent frequencies. Potential observational signatures in the LISA and mid-band frequency ranges are highlighted, providing concrete avenues to test this replication-based cosmological framework in the context of standard cosmological gravitational-wave backgrounds and LISA-oriented forecasts.

79 ASTRONOMY AND ASTROPHYSICS↗

Radiolytic evaluation of select sulfur chlorides (S 2 Cl 2 and SOCl 2 ) for advanced low temperature chlorination of zirconium-based used nuclear fuel cladding

New sulfur chloride compounds—sulfur monochloride (S 2 Cl 2 ) and thionyl chloride (SOCl 2 )—have been proposed as alternative chlorinating agents for the chemical decladding of zirconium-based used nuclear fuel cladding materials. However, the radiation stability of these compounds has not been thoroughly evaluated, despite envisioned process conditions involving intense, multi-component radiation fields. Knowledge of the radiation chemistry of these sulfur chlorides is essential for the development and optimization of alternative chlorination technologies. To this end, we present preliminary findings on the gamma radiolysis of neat S 2 Cl 2 and SOCl 2 at ambient temperature up to ~ 34 MGy. In this study, Raman spectroscopy and density functional theory calculations were used to identify the Raman-active degradation products from S 2 Cl 2 and SOCl 2 radiolysis. Both sulfur chloride compounds exhibited significant radiation resistance, with respect to changes in the Raman signatures of the parent compounds and the ingrowth of Raman-active degradation products. For S 2 Cl 2 , molecular chlorine (Cl 2 ) was directly identified as the predominant degradation product, which was completely consumed at higher absorbed doses (> 9 MGy). Similarly, the main degradation product from SOCl 2 radiolysis was also Cl 2 , although in this system it continued to grow in with dose over the entire dose range. Further, an “S=O” containing degradation product(s) was also identified as a compliment to Cl 2 . Overall, the perceived radiation resistance of these sulfur chloride compounds makes them suitable for inclusion in a used nuclear fuel chemical decladding process, especially as radiolytically formed Cl 2 can be used to reform the parent compounds, thereby increasing the longevity of the solvents used.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Assessment of Cloud Mask Forecasts from the WRF-Solar Ensemble Prediction System: Preprint

Numerical weather prediction (NWP) models are important tools used by government agencies and the renewable energy enterprise to forecast solar radiation. Cloud prediction, a key process of NWP models, has the highest impact on the accuracy of solar forecasting. This study uses satellite observations from the National Solar Radiation Data Base (NSRDB) to evaluate the cloud mask forecast by the WRF-Solar Ensemble Prediction System (WRF-Solar EPS). Preliminary analysis of the data in 2018 demonstrates the need of further improvement in predicting thin and low-level clouds. The information obtained from this work will be used to enhance the WRF-Solar EPS in reproducing the cloud field over the contiguous U.S. and reducing solar forecasting errors.

41 EE - Solar Energy Technologies Office (EE-4S)↗

Experimental Report: Multi-Instrument Comparison of AAF Size Distribution Instruments

Aerosols are particles suspended in the atmosphere, ranging in size from nanometers to micrometers. Their size distribution affects key atmospheric processes, including nucleation, coagulation, scavenging, activation, and radiative properties (Seinfeld and Pandis 2016). Aerosol size distribution is a critical parameter in atmospheric science, influencing processes such as cloud formation and radiative forcing. Accurate representation of aerosol size distributions is essential for understanding their impact on climate, air quality, and human health. However, aerosol size and composition vary significantly across time and space due to meteorological conditions and natural or anthropogenic sources. (Wu and Boor 2021). Various instruments are used to measure aerosol size distributions, each with distinct principles, advantages, and limitations. This report begins with an in-depth overview of aerosol size-distribution comparison studies, focusing on the passive cavity aerosol spectrometer probe (PCASP), portable optical particle spectrometer (POPS), ultra-high-sensitivity aerosol spectrometer (UHSAS), aerodynamic particle sizer (APS), and scanning mobility particle sizer (SMPS). All of these instruments are used by the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) Aerial Facility (AAF), which commissioned this comparison and report. The report evaluates the strengths and weaknesses of these instruments, highlights their applications, and discusses efforts to merge data from multiple instruments for comprehensive analysis.

54 ENVIRONMENTAL SCIENCES↗

How do supernova remnants cool? – I. Morphology, optical emission lines, and shocks

ABSTRACT Supernovae (SNe) inject ∼1051 erg in the interstellar medium, thereby shocking and heating the gas. A substantial fraction of this energy is later lost via radiative cooling. We present a post-processing module for the flash code to calculate the cooling radiation from shock-heated gas using collisional excitation data from mappings v. When applying this tool to a simulated SN remnant (SNR), we find that most energy is emitted in the EUV. However, optical emission lines ([O iii], [N ii], [S ii], H α, H β) are usually best observable. Our shock detection scheme shows that [S ii] and [N ii] emissions arise from the thin shell surrounding the SNR, while [O iii], H $\rm \alpha$, and H $\rm \beta$ originate from the volume-filling hot gas inside the SNR bubble. We find that the optical emission lines are affected by the SNR’s complex structure and its projection on to the plane of the sky because the escaping line luminosity can be reduced by 10–80 per cent due to absorption along the line of sight. Additionally, the subtraction of contaminating background radiation is required for the correct classification of an SNR on the oxygen or sulphur BPT diagrams. The electron temperature and density obtained from our synthetic observations match well with the simulation but are very sensitive to the assumed metallicity.

Astronomy & Astrophysics↗

International Radiological/Nuclear Training for Emergency Response - Major Public Events Virtual Workshop: Alarm Interdiction and Adjudication and Source Recovery (Day 4) [Slides]

The objective of this presentation is for participants to understand the process for interdicting and adjudicating radiation alarms and review operational scenarios for radiological emergency response best practices. The specific goal is for participants to: (1) Become familiar with the Primary and Secondary Inspection process for alarm interdiction, investigation, and adjudication, (2) Gain knowledge of common operational scenarios where alarm interdiction, investigation and adjudication are conducted as best practices, and (3) Review several scenarios that could be encountered as part of the Nuclear Security measures for an MPE.

61 RADIATION PROTECTION AND DOSIMETRY↗

Spatial Interpolation of Air Pollutant and Meteorological Variables in Central Amazonia

The Amazon Rainforest is highlighted by the global community both for its extensive vegetation cover that constantly suffers the effects of anthropic action and for its substantial biodiversity. This dataset presents data of meteorological variables from the Amazon Rainforest region with a spatial resolution of 0.001° in latitude and longitude, resulting from an interpolation process. The original data were obtained from the GoAmazon 2014/5 project, in the Atmospheric Radiation Measurement (ARM) repository, and then processed through mathematical and statistical methods. The dataset presented here can be used in experiments in the field of Data Science, such as training models for predicting climate variables or modeling the distribution of species.

54 ENVIRONMENTAL SCIENCES↗

A new self-adaptive reconstruction method to identify defects through Wigner–Seitz approach

A new self-adaptive reconstruction method based on local atomic structure at any given molecular dynamics (MD) step has been developed in this article. The method can be used in Wigner–Seitz defect analysis approach to correctly and efficiently explore the information of both point defects and complex defect clusters (e.g. dislocation loops and voids) formed after a displacement cascade where the cascade interacts with grain boundaries and/or dislocations. The algorithm and validation are provided in detail. Results for identification of radiation defects during and after cascades interacting with a dislocation network show that the new method can well recognize all simple and complex defects and defect clusters. Thus, this new method provides a totally new way to explore the density and size of radiation defects at atomic scale after complex MD evolution processes, providing correct information to understand and predict radiation damage in materials through atomic simulations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Progress on Producing an ODS Ferritic Alloy by High Deformation Processing of Reactive Powders

Oxide dispersion-strengthened (ODS) ferritic alloys, such as 14YWT, are considered as benchmarks for fuel cladding and core structural materials in advanced nuclear energy reactor systems that require high temperature strength and creep properties as well as resistance to radiation damage. Unfortunately, the popular processing method of mechanical alloying (MA) is time-consuming, incurs high manufacturing costs, and typically produces anisotropy in the microstructure and mechanical properties of ODS ferritic alloys. These considerations hinder their acceptance in many high-performance, high-temperature materials for advanced nuclear energy reactors. This work package is pursuing an alternative solid-state processing to MA involving high deformation at high temperatures for producing an ODS ferritic alloy for fuel cladding. This report summarizes the concept for this processing method and the progress toward selecting the reactive and ferritic alloy powders, preparing 316L stainless steel cans for filling with blended powder followed by degassing, and choosing the heat treatments and forging parameters for performing the first two forging experiments. The preliminary results of optical microscopy performed on polished samples that were cut in three orthogonal directions revealed remnant porosity in both samples. The analysis of the porosity using ImageJ revealed a lesser amount of ~2.49% in the HiLoMe-1 sample that was processed with the three heat treatments and forging parameters compared to ~5.70% for the Hi-1 sample that was processed with only the first sintering heat treatment and forging parameter. These initial results will provide insights that can be leveraged to improve the densification of the powders in future forging experiments that will be continued into FY24 for determining the optimum heat treatments and forging parameters coupled with detailed microstructure characterization studies for producing the ODS ferritic alloy.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Double copy root of Hawking thermality

The Hawking radiation spectrum from a collapsing null shell can be derived via the double copy of a simpler gauge theory calculation. Analyzing the non-abelian Yang-Mills root of this process, we demonstrate that the radiation spectrum is thermal in the color charge eigenvalue 𝜆, not energy. Considering the 𝑆⁢𝑈⁡(𝑁 𝑐 ) gauge theory in the large 𝑁 𝑐 limit, we find the differential spectrum ⅆ⁢𝑁/ⅆ⁢𝜆 is a product of the gravitationally familiar Planck-like factor and the color phase space density, modeled here as the Wigner semicircle from random matrix theory. This reveals that apparent energy thermality in gravity is the direct dual of charge thermality in its underlying non-abelian gauge theory.

Carrasco, John Joseph M. [Northwestern University,↗

Monte Carlo Simulations in Support of NorthStar Irradiation Facility Commissioning Procedure

NorthStar Medical Radioisotopes LLC is constructing an irradiation facility at which electron accelerators will induce photo-transmutation (i.e., neutron knockout) of molybdenum-100 (Mo-100) to produce medically useful Mo-99. The facility will house two high-intensity electron RhodotronTM accelerators developed by IBA Industrial. The nominal power of each Rhodotron is 125kW at 40 MeV beam energy. The production target is made of metallic molybdenum enriched with Mo-100 isotope. It will be irradiated by electron beams and will itself play a role in electron conversion to intense X-rays. A full description of the NorthStar target as well as the concept of radiation shielding of the facility can be found in our previous report. The NorthStar irradiation facility is under commissioning now. The goal of the present work is to support the commissioning process by: (1) Studying residual radiation and activation to minimize personnel exposure and inform radiation waste management; (2) Using computational fluid dynamics (CFD) of the irradiated target to ensure the facility design is safe and reliable; and (3) Helping to determine radiation protection requirements during operation. Monte Carlo simulations are used for the analyses. Most of the results are presented as 3D arrays representing spatial distribution of values across simulated geometries: radiation energy depositions, ambient doses, residual isotopes accumulated, and residual doses.

07 ISOTOPE AND RADIATION SOURCES↗