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NASA NTRS2024

Toward Prebiotic Chemistry on Titan: Impact Experiments on Organic Haze Particles

Impacts are critical to producing the aqueous environments necessary to stimulate prebiotic chemistry on Titan's surface. Furthermore, organic hazes resting on the surface are a likely feedstock of biomolecules. In this work, we conduct impact experiments on laboratory-produced organic haze particles and haze/sand mixtures and analyze these samples for life's building blocks. Samples of unshocked haze and sand particles are also analyzed to determine the change in biomolecule concentrations and distributions from shocking. Across all samples, we detect seven nucleobases, nine proteinogenic amino acids, and five other biomolecules (e.g., urea) using a blank subtraction procedure to eliminate signals due to contamination. We find that shock pressures of 13 GPa variably degrade nucleobases, amino acids, and a few other organics in haze particles and haze/sand mixtures; however, certain individual biomolecules become enriched or are even produced from these events. Xanthine, threonine, and aspartic acid are enriched or produced in impact experiments containing sand, suggesting these minerals may catalyze the production of these biomolecules. On the other hand, thymine and isoleucine/norleucine are enriched or produced in haze samples containing no sand, suggesting catalytic grains are not necessary for all impact shock syntheses. Uracil, glycine, proline, cysteine, and tyrosine are the most unstable to impact-related processing. These experiments suggest that impacts alter biomolecule distributions on Titan's surface, and that organic hazes co-occurring with fine-grained material on the surface may provide an initial source for further prebiotic chemistry on Titan.

impact experiments↗
NASA NTRS1974

Radio observations of Titan

Saturn and Titan have been observed at three frequencies (1420, 2695, and 8085 MHz) with the NRAO interferometer. A clear positive Titan detection has been obtained at 8085 MHz. Assuming Titan's radius is 2500 km, the radio brightness temperature (i.e. for unit emissivity) is 115 + or - 35 K.

Briggs, F. H.↗
NASA NTRS1974

The albedo of Titan

The irradiance of Titan has been measured from 0.50 to 1.08 micron in 30 A bandpasses spaced 0.01 to 0.02 micron apart. Geometric albedos have been computed at the wavelengths of measurement using a standard solar flux distribution after Labs and Neckel (1967). The maximum value of p sub lambda (0) is 0.37 at 0.68, 0.75, and 0.834 micron; the minimum value, in the centers of the strongest methane absorption bands, is 0.10 at 0.887 and 1.012 micron. The brightness of Titan at the time of the present measurements has been compared with that of previous modern photoelectric measurements. Within the apparent consistency of the different photoelectric systems, the brightness of Titan appears to undergo changes with time.

Younkin, R. L.↗
NASA NTRS1976

A Titan exploration study: Science, technology and mission planning options, volume 1

Mission concepts and technology advancements that can be used in the exploration of the outer planet satellites were examined. Titan, the seventh satellite of Saturn was selected as the target of interest. Science objectives for Titan exploration were identified, and recommended science payloads for four basic mission modes were developed (orbiter, atmospheric probe, surface penetrator and lander). Trial spacecraft and mission designs were produced for the various mission modes. Using these trial designs as a base, technology excursions were then made to find solutions to the problems resulting from these conventional approaches and to uncover new science, technology and mission planning options. Several mission modes were developed that take advantage of the unique conditions expected at Titan. They include a combined orbiter, atmosphere probe and lander vehicle, a combined probe and surface penetrator configuration and concepts for advanced remote sensing orbiters.

Tindle, E. L.↗
NASA NTRS1975

Lunar occultation of Saturn. I - The diameters of Tethys, Dione, Rhea, Titan, and Iapetus

The diameters of Tethys, Dione, Rhea, Titan and Iapetus were determined from observations of their March 30, 1974, lunar occultations, made with the Mauna Kea 224 and 61 cm telescopes. Light curves were obtained simultaneously in four colors, and the difference between the time of occultation at the two telescopes provided a direct measurement of the slope of the lunar limb, found to be small in all cases. The satellite diameters were determined by least-squares fits of model occultation light curves to the data. Titan's diameter must be at least 5800 km, much larger than the currently accepted value of 5000 km, making it the largest satellite in the solar system. This larger diameter implies a low mean density. For the other four satellites arguments are presented in favor of accepting the occultation diameters corresponding to limb darkened disks. Except for Titan, the lunar occultation diameters generally agree with previous diskmeter and radiometric determinations.

Elliot, J. L.↗
NASA NTRS1977

Axel dust on Saturn and Titan

The observed sharp drop in the geometric albedo of Titan shortward of 6000 A (also observed for Jupiter and Saturn) has been tentatively attributed to the presence of small absorbing particles referred to as Axel dust. The properties of Axel dust particles are studied, with the effect of scattering included through Mie theory, in an attempt to obtain a physically plausible set of parameters that properly characterizes the dust. Quantitative characteristics of the dust are described, scattering and absorption properties of various particle size distributions are calculated, and fits are made to observations of Titan and Saturn. It is found that: (1) a flat distribution of particle radii up to 0.1 micron and an imaginary part of the refractive index that varies as the -2.5 power of wavelength produce a good fit for Titan provided the extinction optical depth of the satellite's atmosphere is about 10 at 5000 A; (2) a clear layer of about 7 km-am hydrogen is required above the dust for a good fit to Saturn with the same dust properties; and (3) the inclusion of dust significantly increases the computed abundance of methane over the value given by reflecting-layer models.

Podolak, M.↗
NASA NTRS1978

Evolution of a nitrogen atmosphere on Titan

Photochemical calculations indicate that if NH3 outgassed from Titan it should have been converted to a dense N2 atmosphere during the lifetime of the satellite. A crucial step in the process involves a gas phase reaction of N2H4 with H. The most favorable conditions for this step would be the intermediate production of a CH4-H2 greenhouse capable of raising the gas temperature to 150 K. Subsequently about 20 bars of N2 could have evolved. The pressure-induced opacity of 20 bars of N2 should suffice to explain the recently measured 200 K surface temperature. Unlike the situation on Jupiter, NH3 is not recycled on Titan by reactions involving N2 or N2H4. This may explain the failure of recent attempts to detect NH3 in the upper atmosphere of Titan.

Atreya, S. K.↗
NASA NTRS1978

Detection of the Kuiper bands in the spectrum of Titan

New spectra of Titan centered at 7500 A, at resolutions of 4 and 1 A are presented. Weak absorptions coincident with features observed in the spectra of Uranus and Neptune are found. This observation suggests methane abundances in excess of 1 km-am, thereby, emphasizing the complexity of line formation in Titan's atmosphere. The question of the total atmospheric pressure of Titan must be reexamined.

Danehy, R. G.↗
NASA NTRS1978

Organic chemistry on Titan

Observations of nonequilibrium phenomena on the Saturn satellite Titan indicate the occurrence of organic chemical evolution. Greenhouse and thermal inversion models of Titan's atmosphere provide environmental constraints within which various pathways for organic chemical synthesis are assessed. Experimental results and theoretical modeling studies suggest that the organic chemistry of the satellite may be dominated by two atmospheric processes: energetic-particle bombardment and photochemistry. Reactions initiated in various levels of the atmosphere by cosmic ray, Saturn wind, and solar wind particle bombardment of a CH4 - N2 atmospheric mixture can account for the C2-hydrocarbons, the UV-visible-absorbing stratospheric haze, and the reddish color of the satellite. Photochemical reactions of CH4 can also account for the presence of C2-hydrocarbons. In the lower Titan atmosphere, photochemical processes will be important if surface temperatures are sufficiently high for gaseous NH3 to exist. Hot H-atom reactions initiated by photo-dissociation of NH3 can couple the chemical reactions of NH3 and CH4 and produce organic matter.

Chang, S.↗
NASA NTRS1979

Study of entry and landing probes for exploration of Titan

Saturn's largest moon, Titan, is a totally unique planetary body which is certain to yield exciting new phenomena. Current information is lacking in detail to distinguish between a thin methane rich atmosphere and a thick nitrogen rich atmosphere. Therefore, both the thin and thick atmospheric models were used for the study of various Titan probe classes described in this report. The technical requirements, conceptual design, science return, schedule, cost and mission implications of three probe classes that could be used for exploration of Titan are defined. The three probe classes were based on a wide range of exploration mission possibilities.

Source record↗
NASA NTRS1980

An entry and landing probe for Titan

Results of a recent study of entry and landing probes for the exploration of Titan are presented. The probes considered were based on a wide range of exploration mission possibilities. They included: an atmospheric science probe; an intermediate, atmospheric and limited surface science probe; and a larger atmospheric and expanded surface science probe. Because of lower gravity on Titan and its atmosphere characteristics, the entry environment is less severe than that of Mars. However, the large uncertainties in the current definition of the atmosphere and uncertainties in Titan's surface characteristics have required trade-offs of various combinations of entry and descent shapes and hard lander configurations. Results show that all probe classes are feasible without major developments.

Murphy, J. P.↗
NASA NTRS1980

Preliminary results of polarimetry and photometry of Titan at large phase angles from Pioneer 11

The imaging photopolarimeter (IPP) aboard the Pioneer 11 spacecraft measured the linear polarization of the integrated disk of Titan in red and blue light at a variety of phase angles from 15 to 97 deg. The large polarization (54%) measured in blue light at 90 deg phase constrains the size of the aerosols near the top of Titan's atmosphere to have radii smaller than about 0.09 microns if they have a refractive index of 2.0. The polarization at 90 deg phase in red light is smaller (41%) and implies that the optical thickness of the layer of small aerosols is about 0.6 above an effectively depolarizing surface. The shape of the polarization versus phase curve in blue light suggests increasing particle size with increasing depth into the atmosphere. The limb darkening of Titan was measured at 28 deg phase by using the imaging mode of the IPP. The limb darkening observed in both colors is reasonably consistent with that given by the scattering models derived from the polarization observations.

Tomasko, M. G.↗
NASA NTRS1981

Titan's hydrogen torus

A model of Titan's hydrogen torus, capable of describing its time evolution under the influence of the gravitational fields of both the satellite and the planet, is presented. Estimated lifetimes for hydrogen atoms near Titan's orbit of the order of 10 to the 7th s, based on recent Pioneer 11 measurements, suggest that the torus completely encircles Saturn and is angularly unsymmetric, having an enhanced gas density near the satellite. New model calculations confirm this and provide an explanation for the torus detected by the Copernicus satellite and the UV instrument of Pioneer 11. Agreement between calculated and observed Lyman alpha intensities suggests a hydrogen escape flux between 1 x 10 to the 9th/sq cm-s and 3 x 10 to the 9th/sq cm-s should be operative at Titan. This produces a torus containing some 10 to the 34th hydrogen atoms.

Smyth, W. H.↗
NASA NTRS1981

The 1-mm brightness temperature of Titan

Titan has been observed with the 5-m Hale telescope at an effective wavelength of 1 mm. Adopting a value of 2700 km for the radius of Titan, a brightness temperature of 86 + or - 12 K is found at 1 mm. By a comparison of the results with previous measurements at longer wavelengths, it is concluded that the satellite surface is the source of the 1-mm radiation. Since the measured brightness temperature is close to the equilibrium temperature of a blackbody at the distance of Saturn, it is believed there is no significant greenhouse effect on Titan.

Roellig, T. L.↗
NASA NTRS1981

Implications of Titan's north-south brightness asymmetry

Voyager 1 images of Titan, when normalized to remove limb darkening, reveal an axially symmetric brightness pattern with significant north-south asymmetry. This interhemispheric contrast seems to be a response to seasonal solar heating variations resulting from Titan's inclined spin axis. The contrast significantly lags the solar forcing, indicating that its production involves the atmosphere well below the unit optical depth level. The contrast has a significant effect on Titan's disk-integrated brightness as seen from earth, and probably accounts for most of the observed long term variation, with solar UV variations accounting for the remainder.

Sromovsky, L. A.↗
NASA NTRS1982

Production and condensation of organic gases in the atmosphere of Titan

The rates and altitudes for the dissociation of atmospheric constituents on Titan are calculated for solar ultraviolet radiation, the solar wind, Saturn magnetospheric particles, the Saturn co-rotating plasma, and cosmic rays. Laboratory experiments show that a variety of simple gas phase organic molecules and more complex organic solids called tholins are produced by such irradiations of simulated Titanian atmospheres. Except for ultraviolet wavelengths longward of the methane photodissociation continuum, most dissociation events occur between about 3100 and 3600 km altitude, corresponding well to the region of EUV opacity detected by Voyager. For a wide variety of simple to moderately complex organic gases in the Titanian atmosphere, condensation occurs below the top of the main cloud deck at about 2825 km. It is proposed that such condensates, beginning with CH4 at about 2615 km, comprise the principal mass of the Titan clouds. There is a distinct tendency for the atmosphere of Titan to act as a fractional distillation device, molecules of greater complexity condensing out at higher altitudes.

Sagan, C.↗
NASA NTRS1982

The induced magnetosphere of Titan

No evidence was found for an intrinsic magnetic field, nor for the development of a bow shock wave, as the corotating Saturnian magnetoplasma convected past Titan during the Voyager 1 close encounter of November 12, 1980. The observation of a well-developed, induced bipolar magnetic tail is evidence, however, of a strong electrodynamic interaction. Three thin, current-carrying regions were crossed which correspond to the inbound and outbound tail magnetopause and an imbedded tail neutral sheet. The interaction is unique among those observed to date in the solar system, in that it is intermediate with respect to sonic and Alfvenic Mach numbers by comparison with Titan in the solar wind and Io in the Jovian magnetosphere. The draping of the Saturnian magnetic field around the ionosphere of Titan is suggested by results of the analysis of magnetic field data.

Ness, N. F.↗
NASA NTRS1982

The plumes of Titan

The plasma density enhancements observed during the Voyager 1 Titan encounter are interpreted in terms of a single plume of plasma wrapped around Saturn by corotation. Consideration is given to the radial motions of the plume driven by fluctuations in solar wind pressure and the dispersal of the plasma by the centrifugal interchange instability, by heating, and by azimuthal acceleration. It is shown that Saturn cannot readily impose corotation directly on the plume and, incidentally, that the total dissipation associated with the Titan-magnetosphere interaction is insufficient to supply the power to produce the observed Titan ultraviolet airglow. A pickup velocity of 8 km/s is inferred on the basis of the observed velocity and a standing wave model. It is found that the Voyager plasma observations are consistent with the predictions of the model.

Eviatar, A.↗