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NASA NTRS2012

The Rotation Temperature of Methanol in Comet 103P/Hartley 2

Considered to be relics from Solar System formation, comets may provide the vital information connecting Solar Nebula and its parent molecular cloud. Study of chemical and physical properties of comets is thus important for our better understanding of the formation of Solar System. In addition, observing organic molecules in comets may provide clues fundamental to our knowledge on the formation of prebiotically important organic molecules in interstellar space, hence, may shed light on the origin of life on the early Earth. Comet 103PIHartley 2 was fIrst discovered in 1986 and had gone through apparitions in 1991, 1997, and 2004 with an orbital period of about 6 years, before its latest return in 2010. 2010 was also a special year for Comet 103PIHartley 2 because of the NASA EPOXI comet-flyby mission.

Chuang, Yo-Ling↗
NASA NTRS2012

Development of Primary Volatile Production in COMET C/20O9 Pl (GARRADD) During its 2011-2O12 Apparition

We quantified primary volatiles in comet C/2009 Pl (Garradd) through pre- and post-perihelion observations acquired during its apparition in 2011-12 [1,2,3]. Detected volatiles include H2O, CO, CH4, C2H2, C2H6, HCN, NH3, H2CO, and CH3OH. We present production rates and chemical abundance ratios (relative to water) for all species, and I-D spatial profiles for multiple primary volatiles. We discuss these findings in the context of an emerging taxonomy based on primary volatiles in comets [4]. We used three spectrometer/telescope combinations. On UT 20ll August 7 (Rh 2.4 AU) and September 17-21 (Rh 2.0 AU), we used CRIRES at ESO's Very Large Telescope (VLT) [1]. On September 8 and 9 (Rh 2.1 AU), we used NIRSPEC at Keck-2 and CSHELL at IRTF [2]. Using NIRSPEC on October 13 and 2012 January 08 (Rh 1.83 and 1.57 AU, respectively), we detected nine primary volatiles pre-perihelion, and six post-perihelion [3]. CO was enriched in Garradd while C2H2 was strongly depleted. C2H6 and CH3OH displayed abundances close to those measured for the majority of Oort cloud comets observed to date. The high fractional abundance of CO identifies comet C12009 P1 as a CO-rich comet. Spatial profiles revealed notable differences among individual primary species. Given the relatively large heliocentric distance of C/2009 Pl, we explored the effect of water not being fully sublimated within our field of view and we identi$, the "missing" water fraction needed to reconcile the retrieved abundance ratios with the mean values found for "organics-normal" comets.

Mumma, M. J.↗
NASA NTRS2011

Navigation of the EPOXI Spacecraft to Comet Hartley 2

On November 4, 2010, the EPOXI spacecraft flew by the comet Hartley 2, marking the fourth time that a NASA spacecraft successfully captured high resolution images of a cometary nucleus. EPOXI is the extended mission of the Deep Impact mission, which delivered an impactor on comet Tempel-1 on July 4, 2005. EPOXI officially started in September 2007 and eventually took over 3 years of flight time and had 3 Earth gravity assists to achieve the proper encounter conditions. In the process, the mission was redesigned to accommodate a new comet as the target and changes in the trajectory to achieve better imaging conditions at encounter. Challenges in navigation of the spacecraft included precision targeting of several Earth flybys and the comet encounter, uncertainties in determining the ephemeris of the comet relative to the spacecraft, and the high accuracy trajectory knowledge needed to image the comet during the encounter. This paper presents an overview of the navigation process used for the mission.

Deep Impact (DI)↗
NASA NTRS2016

Comet Dust: The Diversity of "Primitive" Particles and Implications

Comet dust is primitive and shows significant diversity. Our knowledge of the properties of primitive particles has expanded significantly through microscale investigations of cosmic dust samples ( IDP's(Interplanetary Dust Particles) and AMM's (Antarctic Micrometeorites)) and of comet dust samples (Stardust and Rosetta's COSIMA), as well as through remote sensing (spectroscopy and imaging) via Spitzer and via spacecraft encounters with 103P/Hartley 2 and 67P/Churyumov-Gerasimenko. Microscale investigations show that comet dust and cosmic dust are particles of unequilibrated materials, including aggregates of materials unequilibrated at submicron scales. We call unequilibrated materials "primitive" and we deduce they were incorporated into ice-rich (H2O-, CO2-, and CO-ice) parent bodies that remained cold, i.e., into comets, because of the lack of aqueous or thermal alteration since particle aggregation; yet some Stardust olivines suggest mild thermal metamorphism. Primitive particles exhibit a diverse range of: structure and typology; size and size distribution of constituents; concentration and form of carbonaceous and organic matter; D-, N-, and O- isotopic enhancements over solar; Mg-, Fe-contents of the silicate minerals; the compositions and concentrations of sulfides, and of less abundant mineral species such as chondrules, CAIs and carbonates. The uniformity within a group of samples points to: aerodynamic sorting of particles and/or particle constituents; the inclusion of a limited range of oxygen fugacities; the inclusion or exclusion of chondrules; a selection of organics. The properties of primitive particles imply there were disk processes that resulted in different comets having particular selections of primitive materials. The diversity of primitive particles has implications for the diversity of materials in the protoplanetary disk present at the time and in the region where the comets formed.

Wooden, Diane H.↗
NASA NTRS2015

The CO2 Abundance in Comets C2012 K1 (PanSTARRS), C2012 K5 (LINEAR), and 290P Jager as Measured with Spitzer

Carbon dioxide is one of the most abundant ices present in comets and is therefore important for understanding cometary composition and activity. We present analysis of observations of CO2 and [O I] emission in three comets to measure the CO2 abundance and evaluate the possibility of employing observations of [O I] emission in comets as a proxy for CO2. We obtained NIR imaging sensitive to CO2 of comets C/2012 K1 (PanSTARRS), C/2012 K5 (LINEAR), and 290P/Jager with the IRAC instrument on Spitzer. We acquired observations of [O I] emission in these comets with the ARCES echelle spectrometer mounted on the 3.5-m telescope at Apache Point Observatory and observations of OH with the Swift observatory (PanSTARRS) and with Keck HIRES (Jager). The CO2/H2O ratios derived from the Spitzer images are 12.6 +/- 1.3% (PanSTARRS), 28.9 +/- 3.6% (LINEAR), and 31.3 +/- 4.2% (Jager). These abundances are derived under the assumption that contamination from CO emission is negligible. The CO2 abundance for PanSTARRS is close to the average abundance measured in comets at similar heliocentric distance to date, while the abundances measured for LINEAR and Jager are significantly larger than the average abundance. From the coma morphology observed in PanSTARRS and the assumed gas expansion velocity, we derive a rotation period for the nucleus of about 9.2 h. Comparison of H2O production rates derived from ARCES and Swift data, as well as other observations, suggest the possibility of sublimation from icy grains in the inner coma. We evaluate the possibility that the [O I] emission can be employed as a proxy for CO2 by comparing CO2/H2O ratios inferred from the [O I] lines to those measured directly by Spitzer. We find that for PanSTARRS we can reproduce the observed CO2 abundance to an accuracy of approximately 20%. For LINEAR and Jager, we were only able to obtain upper limits on the CO2 abundance inferred from the [O I] lines. These upper limits are consistent with the CO2 abundances measured by Spitzer.

McKay, Adam J.↗
NASA NTRS2016

On the Absence of EUV Emission from Comet C/2012 S1 (ISON)

When the sungrazing comet C2012 S1 (ISON) made its perihelion passage within two solar radii of the Sun's surface, it was expected to be a bright emitter at extreme ultraviolet (EUV) wavelengths. However, despite solar EUV telescopes repointing to track the orbit of the comet, no emission was detected. This null result is interesting in its own right, offering the possibility of placing limits on the size and composition of the nucleus. We explain the lack of detection by considering the properties of the comet and the solar atmosphere that determine the intensity of EUV emission from sungrazing comets. By comparing these properties with those of sungrazing comet C2011 W3 (Lovejoy), which did emit in the EUV, we conclude that the primary factor resulting in non-detectable EUV emission from C2012 S1 (ISON) was an insufficiently large nucleus. We conclude that the radius of C2012 S1 (ISON) was at least a factor of four less than that of C2011 W3 (Lovejoy). This is consistent with white-light observations in the days before perihelion that suggested the comet was dramatically reducing in size on approach.

Bryans, Paul↗
NASA NTRS2017

Beyond 3 Au from the Sun: the Hypervolatiles CH4, C2H6, and CO in the Distant Comet C2006 W3 (Christensen)

Comet C/2006 W3 (Christensen) remained outside a heliocentric distance (Rh) of 3.1 au throughout its apparition, but it presented an exceptional opportunity to directly sense a suite of molecules released from its nucleus. The Cryogenic Infrared Echelle Spectrograph at ESO-VLT detected infrared emissions from the three hypervolatiles (CO, CH4, and C2H6) that have the lowest sublimation temperatures among species that are commonly studied in comets by remote sensing. Even at Rh 3.25 au, the production rate of each molecule exceeded those measured for the same species in a number of other comets, although these comets were observed much closer to the Sun. Detections of CO at Rh = 3.25, 4.03, and 4.73 au constrained its post-perihelion decrease in production rate, which most likely dominated the outgassing. At 3.25 au, our measured abundances scaled as CO/CH4/C2H6 approx. = 100/4.4/2.1. The C2H6/CH4 ratio falls within the range of previously studied comets at Rh < 2 au, while CO/CH4 is comparatively high and similar to in situ measurements from Rosetta at approx.10 km from the nucleus of 67P/Churyumov-Gerasimenko conducted at a very similar Rh (3.15 au). The independent detections of H2O (Herschel Space Observatory) and CO (this work) imply a coma abundance H2O/CO approx. = 20% in C/2006 W3 near Rh = 5 au. All these measurements are of high value for constraining models of nucleus sublimation (plausibly CO-driven) beyond Rh = 3au, where molecular detections in comets are still especially sparse.

Bonev, Boncho P.↗
NASA NTRS2007

Fragmentation hierarchy of bright sungrazing comets and the birth and orbital evolution of the Kreutz System. II. the case for cascading fragmentation

We examine the process of cascading fragmentation for the Kreutz sungrazer system to continue our exploration of its birth, orbital evolution, and temporal clumping. We modify and broaden the two-superfragment model from Paper I to include clusters of ~30 bright comets spanning four centuries and 1000 SOHO sungrazers from 1996 to 2006. The spectacular parent sungrazer X/1106 C1 is assumed to have tidally split shortly after perihelion into a train of major protofragments immersed in a cloud of particulate debris, which at larger heliocentric distances were breaking up nontidally over and over again. We describe potential evolutionary paths for the Kreutz system by linking X/1106 C1 in subgroup I-type orbit with the comet of February 423 in one scenario or with the comet of February 467 in another. The latter scenario accounts for sungrazer clusters in as early as the 16th century, suggests that the progenitor object may have been observed as the comet of 214 BCE, is quite consistent with the orbital distribution of the SOHO sungrazers that sample the central filament of the Kreutz system between the clusters of major sungrazers, and predicts future clusters until ~2120. Comet X/1106 C1 and the common parent of C/1882 R1 and C/1965 S1 were two first-generation fragments of the progenitor that split nontidally on the way to its 5th century perihelion, reminiscent of the superfragments in Paper I. We provide computational tools needed for solving the problem of the Kreutz system’s orbital evolution, but no unique scenarios are presented for the individual comets. Another cluster of bright sungrazers is expected to arrive in the coming decades, its earliest member possibly just several years from now.

Chodas, Paul W.↗
NASA NTRS2022

The breakup of a long-period comet is not a likely match to the Chicxulub impactor

Since the discovery of Ir in the clay layer at the K-Pg boundary, scientists have sought to constrain the origin of the extraterrestrial impactor that triggered the end-Cretaceous mass extinction of the non-avian dinosaurs and other species. While the first proposal was for an asteroid, for a while some theories invoked a cometary impactor to explain perceived periodicities in mass extinctions. Such models have long been disfavored by the mass of Ir in the layer, inferred to be 2.0−2.8×10^(11)cu.g. The size of the Chicxulub crater leads to an estimated asteroid impactor diameter, D≈10km. Comets typically impact at higher speeds, reducing the impactor mass for the same impact energy. Although it is increasingly recognized that a continuum exists between comets and asteroids, ’comets’ are considered to be more ice-rich (estimates for 67P/Churyumov-Gerasimenko are about 20%;), implying lower Ir contents per impactor mass. A carbonaceous chondrite-like asteroid of the appropriate size would likely deliver ≈2.3×10^(11)g of Ir, in the center of the estimated mass range of the global Ir layer; but a comet would only deliver ∼0.1×10^(11)g, because it would be less massive. Although these conclusions are long standing, Siraj and Loeb have recently argued anew in favor of a comet over an asteroid, based on dynamical and geochemical evidence. Here we demonstrate that their arguments are based on misinterpretations of the literature, and that an asteroid is in fact still highly favored over a comet.

Steven J. Desch↗
NASA NTRS2022

The breakup of a long-period comet is not a likely match to the Chicxulub impactor

Since the discovery of Ir in the clay layer at the K-Pg boundary [1], scientists have sought to constrain the origin of the extraterrestrial impactor that triggered the end-Cretaceous mass extinction of the non-avian dinosaurs and other species. While the first proposal was for an asteroid, for a while some theories invoked a cometary impactor to explain perceived periodicities in mass extinctions. Such models have long been disfavored by the mass of Ir in the layer, inferred to be2.0−2.8×1011g. The size of Chicxulub crater leads to an estimated asteroid impactor diameter,D≈10 km. Comets typically impact at higher speeds, reducing the impactor mass for the same impact energy. Although it is increasingly recognized that a continuum exists between comets and asteroids, ’comets’ are considered to be more ice-rich (estimates for67P/ Churyumov-Gerasimenko are about 20%;), implying lower Ir contents per impactor mass. A carbonaceous chondrite-like asteroid of the appropriate size would likely deliver≈2.3×1011gof Ir, in the center of the estimated mass range of the global Ir layer; but a comet would only deliver∼0.1×1011g, because it would be less massive. Although these conclusions are long standing, Siraj & Loeb have recently argued anew in favor of a comet over an asteroid, based on dynamical and geochemical evidence. Here we demonstrate that their arguments are based on misinterpretations of the literature, and that an asteroid is in fact still highly favored over a comet.

Steven J Desch↗
DOE OSTI2012

Comet whole-core solution to a stylized 3-dimensional pressurized water reactor benchmark problem with UO{sub 2}and MOX fuel

A stylized pressurized water reactor (PWR) benchmark problem with UO{sub 2} and MOX fuel was used to test the accuracy and efficiency of the coarse mesh radiation transport (COMET) code. The benchmark problem contains 125 fuel assemblies and 44,000 fuel pins. The COMET code was used to compute the core eigenvalue and assembly and pin power distributions for three core configurations. In these calculations, a set of tensor products of orthogonal polynomials were used to expand the neutron angular phase space distribution on the interfaces between coarse meshes. The COMET calculations were compared with the Monte Carlo code MCNP reference solutions using a recently published an 8-group material cross section library. The comparison showed both the core eigenvalues and assembly and pin power distributions predicated by COMET agree very well with the MCNP reference solution if the orders of the angular flux expansion in the two spatial variables and the polar and azimuth angles on the mesh boundaries are 4, 4, 2 and 2. The mean and maximum differences in the pin fission density distribution ranged from 0.28%-0.44% and 3.0%-5.5%, all within 3-sigma uncertainty of the MCNP solution. These comparisons indicate that COMET can achieve accuracy comparable to Monte Carlo. It was also found that COMET's computational speed is 450 times faster than MCNP. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2011

INFRARED SPECTROSCOPY OF COMET 73P/SCHWASSMANN-WACHMANN 3 USING THE SPITZER SPACE TELESCOPE

We have used the Spitzer Space Telescope Infrared Spectrograph (IRS) to observe the 5-37 {mu}m thermal emission of comet 73P/Schwassmann-Wachmann 3 (SW3), components B and C. We obtained low spectral resolution (R {approx} 100) data over the entire wavelength interval, along with images at 16 and 22 {mu}m. These observations provided an unprecedented opportunity to study nearly pristine material from the surface and what was until recently the interior of an ecliptic comet-the cometary surface having experienced only two prior perihelion passages, and including material that was totally fresh. The spectra were modeled using a variety of mineral types including both amorphous and crystalline components. We find that the degree of silicate crystallinity, {approx}35%, is somewhat lower than most other comets with strong emission features, while its abundance of amorphous carbon is higher. Both suggest that SW3 is among the most chemically primitive solar system objects yet studied in detail, and that it formed earlier or farther from the Sun than the bulk of the comets studied so far. The similar dust compositions of the two fragments suggest that these are not mineralogically heterogeneous, but rather uniform throughout their volumes. The best-fit particle size distribution for SW3B has a form dn/da {approx} a{sup -3.5}, close to that expected for dust in collisional equilibrium, while that for SW3C has dn/da {approx} a{sup -4.0}, as seen mostly in active comets with strong directed jets, such as C/1995 O1 Hale-Bopp. The total mass of dust in the comae plus nearby tail, extrapolated from the field of view of the IRS peak-up image arrays, is (3-5) x 10{sup 8} kg for B and (7-9) x 10{sup 8} kg for C. Atomic abundances derived from the spectral models indicate a depletion of O compared to solar photospheric values, despite the inclusion of water ice and gas in the models. Atomic C may be solar or slightly sub-solar, but its abundance is complicated by the potential contribution of spectrally featureless mineral species to the portion of the spectra most sensitive to the derivation of the C abundance. We find a relatively high bolometric albedo, {approx}0.13 for the dust, considering the large amount of dark carbonaceous material, but consistent with the presence of abundant small particles and strong emission features.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

SEARCHING FOR COMETS ON THE WORLD WIDE WEB: THE ORBIT OF 17P/HOLMES FROM THE BEHAVIOR OF PHOTOGRAPHERS

We performed an image search for 'Comet Holmes', using the Yahoo{exclamation_point} Web search engine, on 2010 April 1. Thousands of images were returned. We astrometrically calibrated-and therefore vetted-the images using the Astrometry.net system. The calibrated image pointings form a set of data points to which we can fit a test-particle orbit in the solar system, marginalizing over image dates and detecting outliers. The approach is Bayesian and the model is, in essence, a model of how comet astrophotographers point their instruments. In this work, we do not measure the position of the comet within each image, but rather use the celestial position of the whole image to infer the orbit. We find very strong probabilistic constraints on the orbit, although slightly off the Jet Propulsion Lab ephemeris, probably due to limitations of our model. Hyperparameters of the model constrain the reliability of date meta-data and where in the image astrophotographers place the comet; we find that {approx}70% of the meta-data are correct and that the comet typically appears in the central third of the image footprint. This project demonstrates that discoveries and measurements can be made using data of extreme heterogeneity and unknown provenance. As the size and diversity of astronomical data sets continues to grow, approaches like ours will become more essential. This project also demonstrates that the Web is an enormous repository of astronomical information, and that if an object has been given a name and photographed thousands of times by observers who post their images on the Web, we can (re-)discover it and infer its dynamical properties.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

The unexpectedly bright comet C/2012 F6 (Lemmon) unveiled at near-infrared wavelengths

We acquired near-infrared spectra of the Oort cloud comet C/2012 F6 (Lemmon) at three different heliocentric distances (R {sub h}) during the comet's 2013 perihelion passage, providing a comprehensive measure of the outgassing behavior of parent volatiles and cosmogonic indicators. Our observations were performed pre-perihelion at R {sub h} = 1.2 AU with CRIRES (on 2013 February 2 and 4), and post-perihelion at R {sub h} = 0.75 AU with CSHELL (on March 31 and April 1) and R {sub h} = 1.74 AU with NIRSPEC (on June 20). We detected 10 volatile species (H{sub 2}O, OH* prompt emission, C{sub 2}H{sub 6}, CH{sub 3}OH, H{sub 2}CO, HCN, CO, CH{sub 4}, NH{sub 3}, and NH{sub 2}), and obtained upper limits for two others (C{sub 2}H{sub 2} and HDO). One-dimensional spatial profiles displayed different distributions for some volatiles, confirming either the existence of polar and apolar ices, or of chemically distinct active vents in the nucleus. The ortho-para ratio for water was 3.31 ± 0.33 (weighted mean of CRIRES and NIRSPEC results), implying a spin temperature >37 K at the 95% confidence limit. Our (3σ) upper limit for HDO corresponds to D/H < 2.45 × 10{sup –3} (i.e., <16 Vienna Standard Mean Ocean Water, VSMOW). At R {sub h} = 1.2 AU (CRIRES), the production rate for water was Q(H{sub 2}O) = 1.9 ± 0.1 × 10{sup 29} s{sup –1} and its rotational temperature was T {sub rot} ∼ 69 K. At R {sub h} = 0.75 AU (CSHELL), we measured Q(H{sub 2}O) = 4.6 ± 0.6 × 10{sup 29} s{sup –1} and T {sub rot} = 80 K on March 31, and 6.6 ± 0.9 × 10{sup 29} s{sup –1} and T {sub rot} = 100 K on April 1. At R {sub h} = 1.74 AU (NIRSPEC), we obtained Q(H{sub 2}O) = 1.1 ± 0.1 × 10{sup 29} s{sup –1} and T {sub rot} ∼ 50 K. The measured volatile abundance ratios classify comet C/2012 F6 as rather depleted in C{sub 2}H{sub 6} and CH{sub 3}OH, while HCN, CH{sub 4}, and CO displayed abundances close to their median values found among comets. H{sub 2}CO was the only volatile showing a relative enhancement. The relative paucity of C{sub 2}H{sub 6} and CH{sub 3}OH (with respect to H{sub 2}O) suggests formation within warm regions of the nebula. However, the normal abundance of HCN and hypervolatiles CH{sub 4} and CO, and the enhancement of H{sub 2}CO, may indicate a possible heterogeneous nucleus of comet C/2012 F6 (Lemmon), possibly as a result of radial mixing within the protoplanetary disk.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

THE SPATIAL DISTRIBUTION OF OH AND CN RADICALS IN THE COMA OF COMET ENCKE

Multiple potential parent species have been proposed to explain CN abundances in comet comae, but the parent has not been definitively identified for all comets. This study examines the spatial distribution of CN radicals in the coma of comet Encke and determines the likelihood that CN is a photodissociative daughter of HCN in the coma. Comet Encke is the shortest orbital period (3.3 years) comet known and also has a low dust-to-gas ratio based on optical observations. Observations of CN were obtained from 2003 October 22 to 24, using the 2.7 m telescope at McDonald Observatory. To determine the parent of CN, the classical vectorial model was modified by using a cone shape in order to reproduce Encke's highly aspherical and asymmetric coma. To test the robustness of the modified model, the spatial distribution of OH was also modeled. This also allowed us to obtain CN/OH ratios in the coma. Overall, we find the CN/OH ratio to be 0.009 {+-} 0.004. The results are consistent with HCN being the photodissociative parent of CN, but we cannot completely rule out other possible parents such as CH{sub 3}CN and HC{sub 3}N. We also found that the fan-like feature spans {approx}90 Degree-Sign , consistent with the results of Woodney et al..

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

NARROW DUST JETS IN A DIFFUSE GAS COMA: A NATURAL PRODUCT OF SMALL ACTIVE REGIONS ON COMETS

Comets often display narrow dust jets but more diffuse gas comae when their eccentric orbits bring them into the inner solar system and sunlight sublimates the ice on the nucleus. Comets are also understood to have one or more active areas covering only a fraction of the total surface active with sublimating volatile ices. Calculations of the gas and dust distribution from a small active area on a comet's nucleus show that as the gas moves out radially into the vacuum of space it expands tangentially, filling much of the hemisphere centered on the active region. The dust dragged by the gas remains more concentrated over the active area. This explains some puzzling appearances of comets having collimated dust jets but more diffuse gaseous atmospheres. Our test case is 67P/Churyumov-Gerasimenko, the Rosetta mission target comet, whose activity is dominated by a single area covering only 4% of its surface.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

THE DUAL ORIGIN OF THE NITROGEN DEFICIENCY IN COMETS: SELECTIVE VOLATILE TRAPPING IN THE NEBULA AND POSTACCRETION RADIOGENIC HEATING

We propose a scenario that explains the apparent nitrogen deficiency in comets in a way that is consistent with the fact that the surfaces of Pluto and Triton are dominated by nitrogen-rich ice. We use a statistical thermodynamic model to investigate the composition of the successive multiple guest clathrates that may have formed during the cooling of the primordial nebula from the most abundant volatiles present in the gas phase. These clathrates agglomerated with the other ices (pure condensates or stoichiometric hydrates) and formed the building blocks of comets. We report that molecular nitrogen is a poor clathrate former, when we consider a plausible gas-phase composition of the primordial nebula. This implies that its trapping into cometesimals requires a low disk temperature ({approx}20 K) in order to allow the formation of its pure condensate. We find that it is possible to explain the lack of molecular nitrogen in comets as a consequence of their postformation internal heating engendered by the decay of short-lived radiogenic nuclides. This scenario is found to be consistent with the presence of nitrogen-rich ice covers on Pluto and Triton. Our model predicts that comets should present xenon-to-water and krypton-to-water ratios close to solar xenon-to-oxygen and krypton-to-oxygen ratios, respectively. In contrast, the argon-to-water ratio is predicted to be depleted by a factor of {approx}300 in comets compared to solar argon-to-oxygen, as a consequence of poor trapping efficiency and radiogenic heating.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2013

GROUND-BASED INFRARED DETECTIONS OF CO IN THE CENTAUR-COMET 29P/SCHWASSMANN-WACHMANN 1 AT 6.26 AU FROM THE SUN

We observed Comet 29P/Schwassmann-Wachmann 1 (hereafter, 29P) in 2012 February and May with CRIRES/VLT and NIRSPEC/Keck-II, when the comet was at 6.26 AU from the Sun and about 5.50 AU from Earth. With CRIRES, we detected five CO emission lines on several nights in each epoch, confirming the ubiquitous content and release of carbon monoxide from the nucleus. This is the first simultaneous detection of multiple lines from any (neutral) gaseous species in comet 29P at infrared wavelengths. It is also the first extraction of a rotational temperature based on the intensities of simultaneously measured spectral lines in 29P, and the retrieved rotational temperature is the lowest obtained in our infrared survey to date. We present the retrieved production rates ({approx}3 Multiplication-Sign 10{sup 28} molecules s{sup -1}) and remarkably low ({approx}5 K) rotational temperatures for CO, and compare them with results from previous observations at radio wavelengths. Along with CO, we pursued detections of other volatiles, namely H{sub 2}O, C{sub 2}H{sub 6}, C{sub 2}H{sub 2}, CH{sub 4}, HCN, NH{sub 3}, and CH{sub 3}OH. Although they were not detected, we present sensitive upper limits. These results establish a new record for detections by infrared spectroscopy of parent volatiles in comets at large heliocentric distances. Until now considered to be a somewhat impossible task with IR ground-based facilities, these discoveries demonstrate new opportunities for targeting volatile species in distant comets.

79 ASTRONOMY AND ASTROPHYSICS↗