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DOE OSTI2021

Numerical modeling of a proton spin-flipping system in the spin transparency mode at an integer spin resonance in JINR's Nuclotron

In this paper we propose a lattice insertion for the Nuclotron ring called a “spin navigator” that can adjust any direction of the proton polarization in the orbital plane using weak solenoids. The polarization control is realized in the spin transparency mode at the energy of 108 MeV, which corresponds to the integer spin resonance γ G = 2. The requirements on the navigator solenoid fields are specified considering the criteria for stability of the spin motion during any manipulation of the polarization direction in an experiment. Additionally, this paper presents the results of numerical modeling of the proton spin dynamics in the Nuclotron ring operated in the spin transparency mode. The verified spin navigator is aimed at an experimental study of a spin-flipping system using the Nuclotron ring. The results are relevant to the NICA (JINR), EIC (BNL) and COSY (FZJ) facilities where the spin transparency mode can be applied for polarization control.

47 OTHER INSTRUMENTATION↗

DOE OSTI2020

Revealing Molecular Mechanisms in Hierarchical Nanoporous Carbon via Nuclear Magnetic Resonance

Hierarchical nanoporous carbons (HNC) have been proven to be an effective adsorbent for the adsorption of volatile organic compounds (VOCs) and CO 2 . However, questions remain regarding the hierarchical structure regulation, the adsorption mechanisms of adsorbate uptake, and interactions within the HNC. Here, we synthesize HNC from wood, using a microwave-induced heating method incorporating K 2 CO 3 activation. Our HNC exhibit Murray's law multiscale structures, prompting a molecular-scale study of adsorbate adsorption via nuclear magnetic resonance (NMR). NMR chemical shifts are consistent with ring-current effects from the adsorbent. Our NMR technique provides a convenient way to quantitate adsorption of adsorbate in HNC. VOC vapor adsorption results show NMR chemical-shift changes with time, suggesting initial adsorption into mesopores, followed by diffusion into micropores. Schroeder's paradox is demonstrated by differences in observed shifts for adsorbed liquid vis-à-vis vapor phase in these HNC. These HNC show high CO 2 adsorption capacity, portending applications to carbon capture.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1993

The IR properties of ringed galaxies and the IRAS database

Our study of the Infrared Astronomy Satellite (IRAS) properties of ringed galaxies has been largely successful. We have identified what we think is the probable cause of the differences in the IRAS properties among non-interacting barred galaxies as the pattern speed of the bar. The key to identifying this parameter has been our focusing the study on outer-ringed galaxies where we know precisely what is present in the central regions (from available BVI CCD images in our library of images). The theory is that outer rings, through their morphology and other characteristics, can be identified with the outer Lindblad resonance, one of the major resonances in galaxy structure. Using a library of n-body simulations for comparison, we can reliably infer both low and high pattern speed galaxies from the appearance of outer rings and the existence of other ring features. It is clear that in some barred galaxies, the bar pattern speed is high enough to avoid an inner Lindblad resonance, hence such objects do not contain nuclear or circumnuclear star formation. The IRAS observations are most sensitive to nuclear star formation in early-type barred galaxies, and will thus select those barred galaxies where the pattern speed is low enough to allow an inner Lindblad resonance to exist. High pattern speed barred galaxies therefore weaken the correlation between bars and infrared excess. This finding helps to reconcile the inconsistent results found between different studies on the correlation between bars and far-IR emission.

Buta, Ronald J.↗

NASA NTRS1976

Orbital resonances in the solar system

Orbital resonances are defined as any system of two or more satellites (including planets) orbiting the same primary and whose orbital mean motions are in a ratio of small whole numbers. Known orbital resonances in the solar system are identified, including those involving Jupiter's satellites Io, Europa, and Ganymede; Saturn's satellites Mimas and Tethys, Enceladus and Dione, and Titan and Hyperion; Saturn's ring gaps and Mimas; various asteroids and Jupiter; and the planets Neptune and Pluto. The stability of orbital resonances is examined, the origin of orbital commensurabilities is investigated, and a simple model of the simplest kind of eccentricity-type resonance is outlined. A method is described by which tides carry a noncommensurate pair of satellites into a stable libration, and current ideas concerning the formation of the gaps in Saturn's rings and the asteroid belt are discussed. Various approaches to the analysis of orbital resonances are laid out and illustrated. Three two-body commensurabilities in Saturn's satellite system are analyzed numerically.

Peale, S. J.↗

NASA NTRS2006

Ultimate Whispering Gallery Mode Resonator and Nontrivial Relationship between Spectrum and Shape

Using a similarity between morphologies of an optical planar waveguide and a whispering gallery resonator, we theoretically propose and experimentally demonstrate a one dimensional ring-like macroscopic object characterized with high finesse and small mode volume.

whispering gallery mode resonator↗

NASA NTRS1974

Application of the Brown-Shook model to the Kirkwood gaps and resonant asteroids

The mathematical model developed by Brown and Shook is used to explain the absence of asteroids in the Kirkwood gaps as well as the existence of some resonant asteroids with orbital periods commensurable to that of Jupiter. In addition, this model can possibly explain the biased number distributions at the commensurable positions of both resonant gaps and clusters. However, this resonant model is probably not applicable to the Saturnian ring system due to the possible cosmogonic plasma process during its formation.

Ip, W. H.↗

NASA NTRS1990

High-T(sub c) squid application in medicine and geophysics

In the Laboratory a high-T(sub c) one-hole squid was built from Y1Ba2Cu3O(7-x) ceramics obtained by a standard procedure of solid state reaction. The ceramics with critical current density J(sub c) is greater than 100 A/sq cm was selected. In the middle of 10 x 10 x 2 mm ceramics pellet a 0.8 mm hole was drilled in which superconducting loop of the squid was located. Between the hole and the edge of the pellet a cut was mechanically filed out with a bridge inside it connecting the superconducting ring. A scheme of the magnetometer is presented. The resonant frequency shift of the tank circuit, the connection of the squid with this circuit, and the squid inductance are evaluated. One of the most interesting fields of the squid-based magnetometer application is biomagnetism, particularly, the human heart magnetocardiogram measuring. The low-temperature squids were used in this area and many interesting and important scientific results have been obtained. The observations have shown that the main noise contribution was not due to the squid but to the Earth's magnetic field variations, industrial inductions, and mainly to the vibrations caused by liquid nitrogen boiling and by vibrations of the box. Further attempts are needed to reduce the magnetic noise inductions. Nevertheless, the estimations promise the maximum signal/noise relation of the high-T(sub c) squid-magnetocardiometer to be not less than 10:1 in a bandwidth of 60 Hz. Apparently, such resolution would be enough not only for steady cardiogram reading but even for thin structure investigation at average technique application.

Polushkin, V. N.↗

NASA NTRS1991

High-T(c) squid application in medicine and geophysics

In our laboratory of high-T(sub c), a one-hole squid was built from Y1Ba2Cu3O(7-x) ceramics obtained by a standard procedure of solid state reaction. The ceramics with critical current density J(sub c) is greater than 100 A/sq cm was selected. In the middle of a 10 x 10 x 2 mm ceramics pellet, a 0.8 mm hole was drilled in which the superconducting loop of the squid was located. Between the hole and the edge of the pellet, a cut was mechanically filed out with a bridge inside it connecting the superconducting ring. A scheme of the magnetometer is presented. The resonant frequency shift of the tank circuit, the connection of the squid with this circuit, and the squid inductance are evaluated. One of the most interesting fields of the squid-based magnetometer application is biomagnetism, particularly, the human heart magnetocardiogram measuring. The low-temperature squids were used in this area and many interesting and important scientific results have been obtained. The observations have shown that the main noise contribution was not due to the squid but to the Earth's magnetic field variations, industrial inductions, and mainly to the vibrations caused by liquid nitrogen boiling and by vibrations of the box. Further attempts are needed to reduce the magnetic noise inductions. Nevertheless, the estimations promise the maximum signal/noise relation of the high-T(sub c) squid-magnetocardiometer to be not less than 10:1 in a bandwidth of 60 Hz. Apparently, such resolution would be enough not only for steady cardiogram reading but even for thin structure investigation at average technique application.

Polushkin, V. N.↗

NASA NTRS2010

Ring-laser gyroscope system using dispersive element(s)

A ring-laser gyroscope system includes a ring-laser gyroscope (RLG) and at least one dispersive element optically coupled to the RLG's ring-shaped optical path. Each dispersive element has a resonant frequency that is approximately equal to the RLG's lasing frequency. A group index of refraction defined collectively by the dispersive element(s) has (i) a real portion that is greater than zero and less than one, and (ii) an imaginary portion that is less than zero.

Smith, David D.↗

NASA NTRS2009

A Computational and Experimental Study of Resonators in Three Dimensions

In a previous work by the present authors, a computational and experimental investigation of the acoustic properties of two-dimensional slit resonators was carried out. The present paper reports the results of a study extending the previous work to three dimensions. This investigation has two basic objectives. The first is to validate the computed results from direct numerical simulations of the flow and acoustic fields of slit resonators in three dimensions by comparing with experimental measurements in a normal incidence impedance tube. The second objective is to study the flow physics of resonant liners responsible for sound wave dissipation. Extensive comparisons are provided between computed and measured acoustic liner properties with both discrete frequency and broadband sound sources. Good agreements are found over a wide range of frequencies and sound pressure levels. Direct numerical simulation confirms the previous finding in two dimensions that vortex shedding is the dominant dissipation mechanism at high sound pressure intensity. However, it is observed that the behavior of the shed vortices in three dimensions is quite different from those of two dimensions. In three dimensions, the shed vortices tend to evolve into ring (circular in plan form) vortices, even though the slit resonator opening from which the vortices are shed has an aspect ratio of 2.5. Under the excitation of discrete frequency sound, the shed vortices align themselves into two regularly spaced vortex trains moving away from the resonator opening in opposite directions. This is different from the chaotic shedding of vortices found in two-dimensional simulations. The effect of slit aspect ratio at a fixed porosity is briefly studied. For the range of liners considered in this investigation, it is found that the absorption coefficient of a liner increases when the open area of the single slit is subdivided into multiple, smaller slits.

Tam, C. K. W.↗

NASA NTRS1982

The C ring of Saturn: A high resolution view of some of its structure

Voyager 2 photopolarimeter stellar occultation data on Saturn C ring are discussed. The overall shape is much like the W-shape of other Saturnian rings and the Uranian epsilon ring. The inner structure is quite complex and it is not possible to locate the region of the weaker 1980S27 resonance. There appear to be pseudoperiodic structures, with very pronounced variations in optical depth. Possibly two isolated resonances in close proximity can develop a gravitational interaction that leads to wave patterns imposed upon the intervening ring material. The strength of the variations noted in optical depth between 90140 and 90175 km is too large to be an artifact. It could be temporal, however.

Lane, A. L.↗

DOE OSTI2023

Suppression of Parasitic Voltage Oscillation in Power Modules by Turn-Off Current Zero Placement

This paper presents a frequency-domain analysis of the turn-off equivalent switching network of a hard-switched semiconductor switching cell. This paper also proposes a novel method to suppress parasitic voltage ringing by placing the turn-off current zero at the parasitic resonant frequency. The turn-off current was decomposed into ramp functions and a constant-valued function to facilitate obtaining the frequency components of the turn-off current using the Laplace transform of standard signals. The proposed frequency-domain modeling of the parasitic voltage ringing and the suppression were validated by detailed circuit simulation using parameters corresponding to prior literature with experimental validation.

Galigekere, Veda Prakash↗

DOE OSTI2026

Two-mirror resonator for next-generation Compton gamma-ray source

The next-generation Compton gamma-ray sources (CGSs) based on storage rings require a high-power, well-focused laser beam as a photon driver, which can be realized using a Fabry-Perot cavity (FPC). In this work, we reexamine the behavior and performance of a two-mirror, nearly concentric resonator by introducing a new figure of merit representing the cavity’s proximity to instability. This figure of merit is used to analyze various aspects of the cavity design, including misalignment, beam coupling limitations, and beam size scaling. We then examine several factors affecting the gamma-ray flux, such as the interaction area, crossing angle for collision, frequency matching between the electron and laser beams, and intrabeam scattering effects. Using an example CGS, we demonstrate how to make improved design choices for a two-mirror resonator to enhance the gamma-ray beam flux. This work shows that simple two-mirror Fabry-Perot cavities are well suited as the laser driver for the next-generation storage ring-based CGS, while offering superior advantages in gamma-ray beam polarization control compared to more complex four-mirror, nonplanar resonators.

Delooze, Will↗

DOE OSTI2026

Polarization transmission in the Hadron Storage Ring of the Electron-Ion Collider

The successful operation of the future Electron-Ion Collider is contingent on maintaining high hadron beam polarization up to 275 GeV. The Hadron Storage Ring lattice, however, features a symmetry-breaking interaction region that excites strong, nonsystematic spin resonances, posing a significant threat to polarization preservation. This paper systematically investigates two complementary strategies to ensure high polarization transmission. The first method involves optimizing the vertical betatron phase advance between Siberian snakes to orchestrate a cancellation of depolarizing kicks across the ring. We demonstrate through simulations that both dynamic and fixed-optics solutions based on this principle can successfully preserve polarization through the strongest resonances. The second, more powerful approach involves optimizing the snake rotation axes to suppress resonance driving terms at their source. We revisit established symmetric configurations, such as the Lee-Courant schemes, and introduce a novel, highly symmetric “Doubly Lee-Courant” (DLC) scheme, which enforces a local 𝜋 spin phase advance across every consecutive pair of snakes. Our analysis reveals a clear performance hierarchy, with the DLC configuration providing an exceptionally robust and energy-insensitive baseline for polarization preservation. We conclude that a hybrid strategy, using a DLC snake scheme as a symmetric foundation and betatron phase tuning for fine corrections, offers the most effective path forward for the EIC and future high-energy polarized-beam facilities.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2020

Isomer-Dependent Reaction Mechanisms of Cyclic Ether Intermediates: cis -23-Dimethyloxirane and trans -23-Dimethyloxirane.

Oxiranes are a class of cyclic ethers formed in abundance during low-temperature combustion of hydrocarbons and biofuels, either via chain-propagating steps that occur from unimolecular decomposition of β-hydroperoxyalkyl radicals (β-˙QOOH) or from reactions of HÒO with alkenes. The cis- and trans-isomers of 2,3-dimethyloxirane are intermediates of n-butane oxidation, and while rate coefficients for β-˙QOOH → 2,3-dimethyloxirane + OH are reported extensively, subsequent reaction mechanisms of the cyclic ethers are not. As a result, chemical kinetics mechanisms commonly adopt simplified chemistry to describe the consumption of 2,3-dimethyloxirane by convoluting several elementary reactions into a single step, which may introduce mechanism truncation error—uncertainty derived from missing or incomplete chemistry. The present research examines the isomerdependence of 2,3-dimethyloxirane reaction mechanisms in support of ongoing efforts to minimize mechanism truncation error. Reaction mechanisms are inferred via the detection of products from Cl-initiated oxidation of both cis-2,3-dimethyloxirane and trans-2,3-dimethyloxirane using multiplexed photoionization mass spectrometry (MPIMS). The experiments were conducted at 10 Torr and temperatures of 650 K and 800 K. To complement the experiments, the enthalpies of stationary points on the ˙R + O 2 surfaces were computed at the ccCA-PS3 level of theory. In total, 28 barrier heights were computed on the 2,3-dimethyloxiranylperoxy surfaces. Two notable aspects are low-lying pathways that form resonance-stabilized ketohydroperoxide-type radicals caused by ˙QOOH ring-opening when the unpaired electron is localized adjacent to the ether group, and cis-trans isomerization of ˙R and ˙QOOH radicals, via inversion, which enable reaction pathways otherwise restricted by stereochemistry. Several species were identified in the MPIMS experiments from ring opening of 2,3-dimethyloxiranyl radicals. Neither of the two conjugate alkene isomers prototypical of ˙R + O 2 reactions were detected. Products were also identified from decomposition of ketohydroperoxide-type radicals. The present work provides the first analysis of 2,3-dimethyloxirane oxidation chemistry and reveals that consumption pathways are complex and require the expansion of submechanisms in chemical kinetics mechanisms.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

In-situ dehydrogenation of lignin-based jet fuel: A novel and sustainable liquid organic hydrogen carrier

A new and sustainable liquid organic hydrogen carrier, Lignin Jet Fuel-based Liquid Organic Hydrogen Carrier (LJF-HyC), has been discovered. This innovative LOHC is created from Lignin Jet Fuel (LJF) through dehydrogenation reactions. The process was carried out in situ using platinum nanoparticles supported on zeolite, resulting in a significant increase in aromatic carbon content. This increase indicates the successful formation of aromatic rings via C–H dissociation. In-situ Nuclear Magnetic Resonance (NMR) and gas chromatographic analyses revealed the formation of unsaturated and partially unsaturated compounds, including alkylbenzenes, tetralins, naphthalenes with double bond equivalence of 4–8, from six apparent reaction pathways, four of which can be major. The original LJF, consisting primarily of mono-, di-, and tricyclohexylalkanes (96 wt%), was converted to dehydrogenated products, constituting approximately 18.5 wt% of the LJF composition. These findings pave the way for developing sustainable hydrogen carriers derived from sustainable aviation fuels.

08 HYDROGEN↗

NASA NTRS1982

The whistler nozzle phenomenon

The whistler nozzle is a simple device which can induce jet self-excitations of controllable amplitudes and frequencies and appears highly promising for many applications involving turbulent transport, combustion and aerodynamic noise. The characteristics of this curious phenomenon are documented for different values of the controlling parameters and attempts to explain the phenomenon. It is shown that the whistler excitation results from the coupling of two independent resonance mechanisms: shear-layer tone resulting from the impingement of the pipe-exit shear layer on the collar lip, and organ-pipe resonance of the pipe-nozzle. The crucial role of the shear-layer tone in driving the organ-pipe resonance is proven by reproducing the event in pipe-ring and pipe-hole configurations in the absence of the collar. It is also shown that this phenomenon is the strongest when the self-excitation frequency matches the preferred mode of the jet.

Hussain, A. K. M. F.↗

NASA NTRS1983

The 'whistler-nozzle' phenomenon

Hussain, A. K. M. F.↗