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At least 325 records · Page 18

A safeguards approach for molten salt reactors: Direct gamma-spectrometry of 233 U

Multidimensional gamma-spectrometry is a potential solution for safeguarding future thorium-fueled molten salt reactors (MSRs). A high-sensitivity system developed at Pacific Northwest National Laboratory (PNNL), the Advanced Radionuclide Gamma spectrOmeter (ARGO), has demonstrated direct 233 U assay in freshly irradiated fuel salt samples using a dual-detector configuration and the 97.1 keV gamma-emission. These measurements were made using 1.4 x 10 6 Bq of 233 U activity (at 1.4 x 10 8 fissions), at relatively high dead times (10.4%), and using short count durations of ~800 s. Other major emissions were also evaluated (42.5 keV, 54.7 keV, 146.4 keV), in additional to limited (1.96%) Compton suppression, but provided less consistent determination of the 233 U activity. Accurate 233 U measurement was also demonstrated using its four coincidence gamma-emissions (42.5 keV, 54.7 keV; 42.5 keV, 278.1 keV; 146.4 keV, 174.2 keV; 146.4 keV, 219 keV). Further improvements in coincidence measurements may be achievable with improvements in the detector configuration and nuclear data. Whilst this demonstration utilized the ARGO laboratory system, a similar dual-detector configuration could be utilized for online safeguards measurements.

Gamma-spectrometry↗

Rate-induced aging effects on Parallel-Plate Avalanche Counter (PPAC) caused by heavy ion beams

The Facility for Rare Isotope Beams (FRIB) is one of the premier scientific user facilities for nuclear science with radioactive beams, capable of producing most (approximately 80%) of the isotopes expected to exist, from oxygen to uranium, at energies up to 200 MeV/u. With the increase in beam power from the present 10 kW to the planned 400 kW, FRIB experiments are about to enter a new era. An unprecedented rate capability as well as stable performance of all the planned instrumentation intended for beam diagnostics and beam tuning is required at the expected high beam intensities (> 1 MHz). A summary of aging phenomena at high heavy-ion beam rates observed in the Advanced Rare Isotope Separator (ARIS) detectors for beam diagnostics, including Parallel Plate Avalanche Counters (PPAC) and plastic scintillation for time-of-flight measurements, is discussed. Current research and development project to mitigate rate-induced aging are presented.

Aging effects↗

Study of asymmetries of Cd(Zn)Te devices investigated using photo-induced current transient spectroscopy, Rutherford backscattering, surface photo-voltage spectroscopy, and gamma ray spectroscopies

Despite these recent advancements in preparing the surface of Cd(Zn)Te devices for detector applications, large asymmetries in the electronic properties of planar Cd(Zn)Te detectors are common. Furthermore, for the development of patterned electrode geometries, selection of each electrode surface is crucial for minimizing dark current in the device. This investigation presented here has been carried out with three objectives. Each objective is oriented towards establishing reliable methods for the selection of the anode and cathode surfaces independent of the crystallographic orientation. The objectives of this study are (i) investigate how the asymmetry in I-V characteristics of Cd(Zn)Te devices may be associated with the TeO2 interfacial layer using Rutherford backscattering to study the structure at the Au-Cd(Zn)Te interface, (ii) develop an understanding of how the concentration of the active traps in Cd(Zn)Te varies with the external bias, and (iii) propose non-destructive methods for selection of the anode and cathode which are independent of crystallographic orientation. The spectroscopic methods employed in this investigation include Rutherford backscattering spectroscopy, photo-induced current transient spectroscopy, and surface photo-voltage spectroscopy, as well as gamma ray spectroscopy to demonstrate the influence on detector properties.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Thin film charged particle detectors

Silicon tracking detectors have grown to cover larger surface areas up to hundreds of square meters, and are even taking over other sub-detectors, such as calorimeters. However, further improvements in tracking detector performance are more likely to arise from the ability to make a low mass detector comprised of a high ratio of active sensor to inactive materials, where dead materials include electrical services, cooling, mechanical supports, etc. In addition, the cost and time to build these detectors is currently large. Therefore, advancements in the fundamental technology of tracking detectors may need to look at a more transformative approach that enables extremely large area coverage with minimal dead material and is easier and faster to build. The advancement of thin film fabrication techniques has the potential to revolutionize the next-to-next generation of particle detector experiments. Some thin film deposition techniques have already been developed and widely used in the industry to make LED screens for TVs and monitors. If large area thin film detectors on the order of several square meters can be fabricated with similar performance as current silicon technologies, they could be used in future particle physics experiments. This paper aims to review the key fundamental performance criteria of existing silicon detectors and past research to use thin films and other semi-conductor materials as particle detectors in order to explore the important considerations and challenges to pursue thin film detectors.

Solid state detectors↗

Nuclear cardiograph and scintigraphy

Extensive advances in the technology of detectors, data analysis systems, and tracers used have resulted in greatly expanded applications of radioisotopes to the assessment of cardiac function and disease. The development of nuclear cardiology has proceeded along four lines: (1) radionuclide angiography, (2) myocardial perfusion imaging, (3) intracoronary microsphere imaging, and (4) regional myocardial blood flow determination using inert gases.

Mclaughlin, P.↗

NASA's present and future sensor technology developments

NASA's overall sensing, data acquisition, and instrumentation programs are reviewed. The review shows that the trends in advanced sensor technology involve increased use of solid-state sensors, multiapplication sensors, standardized instrumentation, and miniaturized detectors. Examples are given of several new technologies, showing how improvements in sensor operational capability (such as enhanced sensitivity and spectral range) derived from these advances have resulted in relaxed spacecraft stability requirements, mission time savings, and savings in weight, size, and power. The introduction of multiapplication sensors and standardized instrumentation will result in measurement cost reduction and improved compatibility with standardized spacecraft.

Rubin, B.↗

The future of large format HgCdTe arrays for astronomy

Rockwell has developed the 256 x 256 Near Infrared Camera and Multi-Object Spectrometer 3 (NICMOS3) FPA for the Hubble Space Telescope under funding from NASA through the University of Arizona. Since 1989, dozens of science grade devices have been delivered to astronomers throughout the world for ground based infrared observations. These devices have excellent sensitivity at 77 K with mean dark currents of 0.1 e(-)/s, noise of 25 e(-), and quantum efficiency of 55-70%. Pixel yields as high as 99.9% have been achieved. Our present plans are to develop a 1024 x 1024 focal plane array (FPA) with 2.5 micron cutoff and make it available to astronomers. Such large arrays are made possible by the advances in detector material size (3 in. diameter producible alternative to CdTe for epitaxy (PACE-I) wafers), multiplexer advances (ability to verify the design in detail and availability of advanced foundries), and novel hybridization and reliability approaches.

Vural, K.↗

GaN/AlGaN Avalanche Photodiode Detectors for High Performance Ultraviolet Sensing Applications

The shorter wavelengths of the ultraviolet (UV) band enable detectors to operate with increased spatial resolution, variable pixel sizes, and large format arrays, benefitting a variety of NASA, defense, and commercial applications. AlxGa1-xN semiconductor alloys, which have attracted much interest for detection in the UV spectral region, have been shown to enable high optical gains, high sensitivities with the potential for single photon detection, and low dark current performance in ultraviolet avalanche photodiodes (UV-APDs). We are developing GaN/AlGaN UV-APDs with large pixel sizes that demonstrate consistent and uniform device performance and operation. These UV-APDs are fabricated through high quality metal organic chemical vapor deposition (MOCVD) growth on lattice-matched, low dislocation density GaN substrates with optimized material growth and doping parameters. The use of these low defect density substrates is a critical element to realizing highly sensitive UV-APDs and arrays with suppressed dark current under high electric fields.Optical gains greater than 5X10 (exp 6) with enhanced quantum efficiencies over the 350-400 nm spectral range have been demonstrated, enabled by a strong avalanche multiplication process. Furthermore, we are developing 6X6 arrays of devices to test high gain UV-APD array performance at ~355 nm. These variable-area GaN/AlGaN UV-APD detectors and arrays enable advanced sensing performance over UV bands of interest with high resolution detection for NASA Earth Science applications.

Sood, Ashok K.↗

Design of the DUNE APATF cryogenic system

Fermi National Accelerator Laboratory (FNAL) is developing the international Long- Baseline Neutrino Facility (LBNF) and Deep Underground Neutrino Experiment (DUNE) to advance neutrino science. The flagship of the DUNE project consists of a large particle detector constructed one-mile (1.6 km) beneath the surface at the Sanford Underground Research Facility (SURF) in Lead, SD. The SURF detector is the largest of its type ever built and is comprised of four cryostats totaling 70,000 tons of liquid argon (LAr) to record neutrino interactions with unprecedented precision. Each cryostat houses a detector, the first includes 150 Anode Panel Assemblies (APA) submersed within 17,500 tons of LAr. Before installing 150 APA within the SURF detector they will be cryogenically cooled to nominally 90 K at the APA Test Facility (APATF) utilizing nitrogen flows. The APATF cryogenic system is entirely located one-mile underground at the SURF facility and includes nominally 13 kW of refrigeration at 80 K, cryogenic transfer lines, APA test cryostats, a cryogenic control system, and various control and pressure safety elements to ensure performance and safety requirements are achieved. The APATF preliminary design is in progress and major considerations include an efficient, costeffective mechanism to deliver the required refrigeration to the APATF underground, support of rigid testing intervals to support the DUNE operating schedule, temperature stability of the APA and electronics within cryostats, efficient cryogenic system operation to minimize heat leak and/or liquid nitrogen consumption, thermo-mechanical stability and flexibility of components, and pressure safety of the APATF cryogenic system. Installation and integration of the APATF cryogenic system within the footprint and to adjacent sub-systems is also discussed.

43 PARTICLE ACCELERATORS↗

Advanced Detector and Waveform Digitizer for Water Vapor DIAL Systems

Measurement of atmospheric water vapor has become a major requirement for understanding moist-air processes. Differential absorption lidar (DIAL) is a technique best suited for the measurement of atmospheric water vapor. NASA Langley Research Center is continually developing improved DIAL systems. One aspect of current development is focused on the enhancement of a DIAL receiver by applying state-of-the-art technology in building a new compact detection system that will be placed directly on the DIAL receiver telescope. The newly developed detection system has the capability of being digitally interfaced with a simple personal computer, using a discrete input/output interface. This has the potential of transmitting digital data over relatively long distances instead of analog signals, which greatly reduces measurement noise. In this paper, we discuss some results from the new compact water vapor DIAL detection system which includes a silicon based avalanche photodiode (APD) detector, a 14-bit, 10-MHz waveform digitizer, a microcontroller and other auxiliary electronics. All of which are contained on a small printed-circuit-board. This will significantly reduce the weight and volume over the current CAMAC system and eventually will be used in a water vapor DIAL system on an unpiloted atmospheric vehicle (UAV) aircraft, or alternatively on an orbiting spacecraft.

Refaat, Tamer F.↗

Low power implementation of high frequency SiPM readout for Cherenkov and scintillation detectors in TOF-PET

State-of-the-art (SoA) electronic readout for silicon photomultiplier (SiPM)-based scintillation detectors that demonstrate experimental limits in achievable coincidence time resolution (CTR) leverage low noise, high frequency signal processing to facilitate a single photon time response that is near the limit of the SiPMs architecture. This readout strategy can optimally exploit fast luminescence and prompt photon populations, and promising measurements show detector concepts employing this readout can greatly advance PET detector CTR, relative to SoA in clinical systems. However, the technique employs power hungry components which make the electronics chain impractical for channel-dense time-of-flight (TOF)-PET detectors. We have developed and tested a low noise and high frequency readout circuit which is performant at low power and consists of discrete elements with small footprints, making it feasible for integration into TOF-PET detector prototypes. A 3 × 3 mm 2 Broadcom SiPM with this readout chain exhibited sub-100 ps single photon time resolution at 10 mW of power consumption, with a relatively minor performance degradation to 120 ± 2 ps FWHM at 5 mW. CTR measurements with 3 × 3 × 20 mm 3 LYSO and fast LGSO scintillators demonstrated 127 ± 3 ps and 113 ± 2 ps FWHM at optimal power operation and 133 ± 2 ps and 121 ± 3 ps CTR at 5 mW. BGO crystals 3 × 3 × 20 mm 3 in size show 271 ± 5 ps FWHM CTR (1174 ± 14 ps full-width-at-tenth-maximum (FWTM)) at optimal power dissipation and 289 ± 8 ps (1296 ± 33 ps FWTM) at 5 mW. The compact and low power readout topology that achieves this performance thereby offers a platform to greatly advance PET system CTR and also opportunities to provide high performance TOF-PET at reduced material cost.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Computed Tomography of Dry Cask Storage for Used Fuel

The demand for dry cask storage for used nuclear fuel is on the rise due to the continuous operation of currently existing nuclear plants which are reaching or have reached the capacity of their used fuel pools. Dry cask storage allows used fuel that has already been cooled in the used fuel pool for at least five years to be surrounded by an inert gas inside a specially designed and licensed cask. Currently, 75 of the 78 U.S.A reactor sites either have or are pursuing an independent spent fuel storage installation (ISFSI) for dry cask fuel storage with over 2,000 casks already loaded. Cask loading will only continue to increase until a final repository solution is operational or the U.S. begins to recycle fuel. The challenge of monitoring the condition of the used fuel inside the cask without exposing the used fuel has been apparent since the 1980's. The objective of the University of Florida (UF) project is ultimately to investigate the feasibility of imaging the used fuel assemblies' location and evaluating the inner structural condition using emission source computed tomography (CT). A combination of radiation transport models will be used to simulate gamma-rays and neutrons traversing through the used fuel, structure, and cask body materials. In the simulations, multiple linear detector arrays will record the radiation outside the cask wall and will be placed at various angles in order to model rotating a linear detector array around the entire cask. The combination of data from all the detectors will give the planar radiation projection onto the detectors, more commonly called the Radon transform, of the structure of used fuel assemblies. This project can be processed with filtered back projection or other more advanced reconstructive imaging algorithms to recreate the fuel structures. A majority of the historical work done for used fuel has been on verification, diversion detection, and burnup credit validation in order to meet regulatory guidelines. One of the more commonly used systems for single assembly verification is the Fork Detector developed at Los Alamos National Laboratory in 1988. A group at the Idaho National Laboratory developed a Compton Dry-Cask Imaging Scanner that has the ability to detect empty vs full storage positions but it suffered a setback when transported to the Doel Nuclear Power Plant near Antwerp, Belgium; the system was unable to detect full energy peaks because of the additional scattering caused by a thick ballistic steel shield. As detectors, computational power, and modeling improves, a few groups have leveraged these advancements and started to investigate CT hoping, that despite the difficulties, the technique can give information on fuel condition. So far the groups have mostly limited the tomographic work to a per assembly basis , rather than the full dry cask as the University of Florida plans to investigate. The downsides of CT versus simpler verification and validation are the amount of data required and the time it takes to acquire that data. Given that dry casks are intended to sit undistributed for up to 60 years, a scanning time of several weeks to several months is not unreasonable if such systems do not require human operators beyond the initial setup. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Development of an advanced combined iodine dispenser/detector

Injection of iodine into water is widely used to control microbial growth. An entirely automated device for I2 injection has been developed for spacecraft application. Transfer of I2 into the water from a concentrated form is controlled electrochemically via feedback from an integrated photometric I2 level detector. All components are contained within a package weighing only 1.23 kg (2.7 lb) dry, which occupies only 1213 cu cm (74 cu in) of space, and which has the capacity to iodinate 10,900 kg (24,000 lb) of water of 5 ppm. These features exceed design specifications. The device performed satisfactorily during extended testing at variable water flow rates and temperatures. Designed to meet specifications of the Shuttle Orbiter, the device will find application in the regenerative water systems of advanced spacecraft.

Lantz, J. B.↗

Computed Tomography of Dry Cask Storage for Used Fuel

The demand for dry cask storage for used nuclear fuel is on the rise due to the continuous operation of currently existing nuclear plants which are reaching or have reached the capacity of their used fuel pools. Dry cask storage allows used fuel that has already been cooled in the used fuel pool for at least five years to be surrounded by an inert gas inside a specially designed and licensed cask. Currently, 75 of the 78 U.S.A reactor sites either have or are pursuing an independent spent fuel storage installation (ISFSI) for dry cask fuel storage [1] with over 2,000 casks already loaded [2]. Cask loading will only continue to increase until a final repository solution is operational or the U.S. begins to recycle fuel. The challenge of monitoring the condition of the used fuel inside the cask without exposing the used fuel has been apparent since the 1980s. The objective of the University of Florida (UF) project is ultimately to investigate the feasibility of imaging the used fuel assemblies’ location and evaluating the inner structural condition using emission source computed tomography (CT). A combination of radiation transport models will be used to simulate gamma-rays and neutrons traversing through the used fuel, structure, and cask body materials. In the simulations, multiple linear detector arrays will record the radiation outside the cask wall and will be placed at various angles in order to model rotating a linear detector array around the entire cask. The combination of data from all the detectors will give the planar radiation projection onto the detectors, more commonly called the Radon transform, of the structure of used fuel assemblies. This project can be processed with filtered back projection or other more advanced reconstructive imaging algorithms to recreate the fuel structures. A majority of the historical work done for used fuel has been on verification, diversion detection, and burnup credit validation in order to meet regulatory guidelines. One of the more commonly used systems for single assembly verification is the Fork Detector developed at Los Alamos National Laboratory in 1988 [3]. A group at the Idaho National Laboratory developed a Compton Dry-Cask Imaging Scanner that has the ability to detect empty vs full storage positions but it suffered a setback when transported to the Doel Nuclear Power Plant near Antwerp, Belgium; the system was unable to detect full energy peaks because of the additional scattering caused by a thick ballistic steel shield [4]. As detectors, computational power, and modeling improves, a few groups have leveraged these advancements and started to investigate CT hoping, that despite the difficulties, the technique can give information on fuel condition. So far the groups have mostly limited the tomographic work to a per assembly basis [5] [6] [7], rather than the full dry cask as the University of Florida plans to investigate. The downsides of CT versus simpler verification and validation are the amount of data required and the time it takes to acquire that data. Given that dry casks are intended to sit undistributed for up to 60 years, a scanning time of several weeks to several months is not unreasonable if such systems do not require human operators beyond the initial setup.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Advancing Artificial Intelligence with Liquid Argon Neutrino Experiments (Technical Report)

The grant allowed two main contributions: 1) The development of a first successful demonstration of the employment of Optimal Transport in liquid argon time projection chamber neutrino detectors. Optimal Transport, used in other contexts and specifically with LHC calorimetric data, was adapted to address a key particle identification challenge in LArTPCs: the separation of pi0 backgrounds from single-electrons produced in charged-current electron neutrino interactions. The work, leveraging ML methods such as k-nearest-neighbor (kNN) and support-vector-machine (SVM), showed an increase in background rejection of a factor of two or more. Work is now ongoing to incorporate this development in physics analyses for LArTPC experiments and more broadly expand the use of OT in LArTPC detectors including DUNE. This work was done in collaboration with the phenomenology group led by Nathaniel Craig at UCSB. 2) The deployment of NuGraph2, a graph neural network developed for LArTPC reconstruction, in the MicroBooNE experiment. NuGraph2 uses novel graph-neural-network methods on the rather simple LArTPC inputs of reconstructed hits, greatly simplifying the workflow compared to the use of waveform or signal-deconvolved wire ROIs. The network performed particle classification and was shown to address many challenging problems in LArTPC imaging including track-shower separation and the identification of protons and charged pions from primary muons. Our group collaborated with Giuseppe Cerati (FNAL scientist) who is one of the core developers of NuGraph2 to integrate this tool in MicroBooNE’s analysis framework. This consisted in tow key contributions: a) Studying performance on real data, which came with several months of iterations because the MC-trained version of the network was found to show significant bias that our group investigated and addressed. b) Integrating the output hit labeling of NuGraph2 into the existing particle tracking and shower reconstruction code. As a result of this work led by our team NuGraph2 is now enabling a suite of new analyses which benefit from enhanced capabilities and thus broader physics reach. The grant supported primarily the salary of UCSB graduate student Chuyue “Michaelia” Fang as well as partial summer salary support for PI Caratelli. Some funds were used for travel by Michaelia to ML related schools and conferences.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

QWIPs, SLS, Landsat and the International Space Station

In 1988 DARPA provided funding to NASA’s Goddard Space Flight Center to support the development of GaAs Quantum Well Infrared Photodetectors (QWIP). The goal was to make a single element photodetector that might be expandable to a two-dimensional array format. Ultimately, this led to the development of a 128 x 128 element array in collaboration with AT&T Bell Labs and Rockwell Science Center in 1990. We continued to develop numerous generations of QWIP arrays most recently resulting in the multi-QWIP focal plane for the NASA-US Geological Survey (USGS) Landsat 8 mission launched in 2013 and a similar instrument on the Landsat 9 mission to be launched in 2020. Toward the end of the Landsat 8 QWIP-based Thermal Infrared Sensor (TIRS) instrument the potential of the newly developed Strained Layer Superlattice (SLS) detector array technology became of great interest to NASA for three primary reasons: 1) higher operating temperature; 2) broad spectral response and; 3) higher sensitivity. We have collaborated extensively with QmagiQ, LLC and Northwestern University to further pursue and advance the SLS technology ever since we started back in 2012. In December of 2018 we launched the first SLS-based IR camera system to the International Space Station on board the Robotic Refueling Mission #3 (RRM3). This paper will describe the evolution of QWIP technology leading to the current development of SLS-based imaging systems at the Goddard Space Flight Center over the past 30 years.

Jhabvala, M.↗

Advances in High Resolution Ultrafast Scintillators for Fast timing Applications

Scintillation detectors exhibiting high spatial resolution and fast timing capabilities are of vital importance for synchrotron sources. These detectors may be exposed to a variety of X-ray energies (up to 140 keV) and used in high frame rate applications. Here, we describe the advances in the development of thin-film LuI3:Ce scintillators for higher energy X-ray imaging, with fast timing and high spatial resolution. When grown in a single crystalline form, these scintillators are bright, producing 115 000 photons/MeV. However, to achieve high spatial resolution, these scintillators are grown in thin-film form with a microcolumnar structure, controllable to column diameters of <1-30 mu m. Thus, a much thicker scintillator layer (10 mu m-3 mm or higher) may be grown, providing superior X-ray absorption while achieving high resolutions of 50 mu m or better, at the cost of reduced light yield. To study the timing characteristics of the scintillator, time-resolved X-ray excited optical luminescence (TR-XEOL) was performed on two different sets of three samples of LuI3 at the 1-BM beamline of the Advanced Photon Source at Argonne National Laboratory. Besides, we report timing measurements obtained using a photomultiplier tube (PMT) and oscilloscope at Radiation Monitoring Devices (RMD) Inc. Using the TR-XEOL, we determined the decay constants of LuI3 as a function of Ce doping, recording a fast decay component as low as 3.6 ns (39%), one of the fastest values recorded in inorganic scintillators. This fast decay opens up numerous novel applications, where ultrahigh frame rates are important using synchrotron X-rays. This article will discuss fabrication, characterization, and potential applications for this novel scintillator.

fast timing↗

Elementary Particle Interactions (Final Technical Report)

Neutrinos provide a promising window to probe a wide range of fundamental physics. The past two decades have brought several remarkable neutrino-related discoveries indicating that one may answer the most sought after question of our matter dominated universe from within the neutrino sector. The global neutrino physics program is currently focused on studying neutrino oscillations, and to understand the implications of this phenomena on the evolution of the universe. Addressing all of these open questions and completing the story of neutrino oscillations requires technological advances in neutrino detection. Liquid argon time projection chambers (LArTPCs) are imaging detectors that offer fine-grained tracking, calorimetry and scalability, and are increasingly favored for the next generation of large neutrino detectors. Through leading technical and scientific roles on MicroBooNE, Short-Baseline Near Detector (SBND) and the Deep Underground Neutrino Experiment (DUNE) LArTPC neutrino experiments, the research program supported through this funding has significantly advanced the understanding of neutrino properties along with technical development of LArTPCs for both short- and long-baseline neutrino oscillations physics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗