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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 325 records · Page 18
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Studies of optical and chemical properties of aged and fresh biomass burning absorbing aerosols for climate models

Particulate emissions from burning fuels from sub-Saharan Africa is currently poorly characterized. With increasing population and industrialization, emissions are expected to grow. Optical methods for measuring light absorption in the ultraviolet (UV) and visible (vis) regions of the spectrum are crucial for understanding the optical properties of BB aerosols (Bond and Bergstrom, 2006; Lack and Cappa, 2010; Moschos et al., 2021). One such instrument is the dual-spot AE33 model aethalometer is a common filter-based instrument that can be used to measure aerosol absorption properties (Hansen et al., 1984). This instrument has many figures of merit; however, the method's limitations include potential biases from scattering within the filter material, multiple scattering effects of the particles, filter loading (i.e. particle shadowing), and the need for wavelength-specific correction factors (Cλ), which depend on accurate intercomparison with other in situ techniques (Bond et al., 1999; Collaud Coen et al., 2010). This work aims to: 1. Optically characterize BB aerosol generated from African fuel 2. Correct the aethalometer at multiple wavelengths 3. Parametrize these correction factors. 4. Combusting the same fuels with two difference tube furnace systems assess the general applicability of this flexible means of producing BB aerosol. This was accomplished by conducting laboratory studies at Los Alamos National Laboratory (LANL) and North Carolina A&T State University (NCA&T), where aethalometer measurements were compared to in situ optical measurements. Mass cross sections of BB aerosol from these under-studied fuels will be determined along with their wavelength dependence.

09 BIOMASS FUELS↗
DOE OSTI2025

Advancing the Understanding of Cloud Microphysical Processes and Aerosol Indirect Effects in High-Latitude Mixed-Phase Clouds by Linking ARM Measurements with Climate Model Simulations (Final Report)

The key objectives of this project were to advance our understanding of cloud microphysical characteristics and aerosol indirect effects on mixed-phase clouds in high latitudes. To improve the representation of ice and mixed-phase clouds in Earth System Models (ESMs), we propose an integrated observation and modeling study of cloud macro- and microphysical properties, including spatial heterogeneities, mass partitioning between ice crystals and supercooled liquid water, effects of ice nucleating particles (INPs), and efficiency of secondary ice production (SIP), etc. Specifically, we took four main approaches in this project: (1) examining macro- and microphysical properties of ice and mixed-phase clouds based on in-situ and ground-based observations from multiple field campaigns funded by the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program, including the Mixed-Phase Arctic Cloud Experiment (M-PACE), Indirect and Semi-Direct Aerosol Campaign (ISDAC), Ice Nucleating Particle Sources at Oliktok Point (INPOP), ARM West Antarctic Radiation Experiment (AWARE), Measurements of Aerosols, Radiation, and Clouds over the Southern Ocean (MARCUS), and Macquarie Island Cloud and Radiation Experiment (MICRE); (2) evaluating the DOE Energy Exascale Earth System Model (E3SM) simulations based on observations, particularly for ice and mixed-phase cloud microphysical properties; (3) examining the impacts of INPs on ice and mixed-phase clouds. Specifically, a series of comparisons were conducted using observations over the Arctic, Southern Ocean, and Antarctica, including comparisons between the lower and higher southern latitudes as well as comparisons between the northern and southern hemispheres. In addition, aerosol indirect effects from distinct sources of dust particles were examined; and (4) investigating the impacts of SIP. Ultimately, these results helped to improve cloud microphysics and aerosol-cloud interaction parameterizations in the E3SM model. Overall, the project provided improved understanding regarding various factors, including thermodynamic, dynamic, and aerosol conditions, on the micro- and macrophysical properties of ice and mixed-phase clouds in the high latitudes. Resulting analysis helped to provide an improved physical basis for refining the current cloud microphysics parameterizations related to ice and mixed-phase clouds in E3SM.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2017

A radiative transfer module for calculating photolysis rates and solar heating in climate models: Solar-J v7.5

Solar-J is a comprehensive radiative transfer model for the solar spectrum that addresses the needs of both solar heating and photochemistry in Earth system models. Solar-J is a spectral extension of Cloud-J, a standard in many chemical models that calculates photolysis rates in the 0.18–0.8 µm region. The Cloud-J core consists of an eight-stream scattering, plane-parallel radiative transfer solver with corrections for sphericity. Cloud-J uses cloud quadrature to accurately average over correlated cloud layers. It uses the scattering phase function of aerosols and clouds expanded to eighth order and thus avoids isotropic-equivalent approximations prevalent in most solar heating codes. The spectral extension from 0.8 to 12 µm enables calculation of both scattered and absorbed sunlight and thus aerosol direct radiative effects and heating rates throughout the Earth's atmosphere. The Solar-J extension adopts the correlated-k gas absorption bins, primarily water vapor, from the shortwave Rapid Radiative Transfer Model for general circulation model (GCM) applications (RRTMG-SW). Solar-J successfully matches RRTMG-SW's tropospheric heating profile in a clear-sky, aerosol-free, tropical atmosphere. We compare both codes in cloudy atmospheres with a liquid-water stratus cloud and an ice-crystal cirrus cloud. For the stratus cloud, both models use the same physical properties, and we find a systematic low bias of about 3 % in planetary albedo across all solar zenith angles caused by RRTMG-SW's two-stream scattering. Discrepancies with the cirrus cloud using any of RRTMG-SW's three different parameterizations are as large as about 20–40 % depending on the solar zenith angles and occur throughout the atmosphere. Effectively, Solar-J has combined the best components of RRTMG-SW and Cloud-J to build a high-fidelity module for the scattering and absorption of sunlight in the Earth's atmosphere, for which the three major components – wavelength integration, scattering, and averaging over cloud fields – all have comparably small errors. More accurate solutions with Solar-J come with increased computational costs, about 5 times that of RRTMG-SW for a single atmosphere. There are options for reduced costs or computational acceleration that would bring costs down while maintaining improved fidelity and balanced errors.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

The importance of considering sub-grid cloud variability when using satellite observations to evaluate the cloud and precipitation simulations in climate models

Abstract. Satellite cloud observations have become an indispensable tool for evaluating general circulation models (GCMs). To facilitate the satellite and GCM comparisons, the CFMIP (Cloud Feedback Model Inter-comparison Project) Observation Simulator Package (COSP) has been developed and is now increasingly used in GCM evaluations. Real-world clouds and precipitation can have significant sub-grid variations, which, however, are often ignored or oversimplified in the COSP simulation. In this study, we use COSP cloud simulations from the Super-Parameterized Community Atmosphere Model (SPCAM5) and satellite observations from the Moderate Resolution Imaging Spectroradiometer (MODIS) and CloudSat to demonstrate the importance of considering the sub-grid variability of cloud and precipitation when using the COSP to evaluate GCM simulations. We carry out two sensitivity tests: SPCAM5 COSP and SPCAM5-Homogeneous COSP. In the SPCAM5 COSP run, the sub-grid cloud and precipitation properties from the embedded cloud-resolving model (CRM) of SPCAM5 are used to drive the COSP simulation, while in the SPCAM5-Homogeneous COSP run only grid-mean cloud and precipitation properties (i.e., no sub-grid variations) are given to the COSP. We find that the warm rain signatures in the SPCAM5 COSP run agree with the MODIS and CloudSat observations quite well. In contrast, the SPCAM5-Homogeneous COSP run which ignores the sub-grid cloud variations substantially overestimates the radar reflectivity and probability of precipitation compared to the satellite observations, as well as the results from the SPCAM5 COSP run. The significant differences between the two COSP runs demonstrate that it is important to take into account the sub-grid variations of cloud and precipitation when using COSP to evaluate the GCM to avoid confusing and misleading results.

54 ENVIRONMENTAL SCIENCES↗