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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 325 records · Page 18
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

To Substitute Rather Than Intercalate: Chimie douce Approach to Induce Ferromagnetism in Metastable Pt 0.8 M 0.2 Se 2 ( M = Cr, Co, Ni)

Two-dimensional (2D) magnetic materials with exotic magnetic properties have garnered significant interest due to their potential applications in spintronics and data storage technologies. However, the limited availability of intrinsic 2D magnetic materials has driven efforts to induce and manipulate magnetism in otherwise nonmagnetic 2D systems through approaches such as chemical intercalation, defect engineering, and substitutional doping. Herein, we present a facile, chimie douce method for incorporating 3d transition metals (Cr, Co, and Ni) into the nonmagnetic PtSe 2 sublattice. This synthetic approach enables control over layer thickness of Pt 1–x M x Se 2 (M = Cr, Co, Ni) nanosheets by varying the M identity and annealing conditions. Comprehensive scattering and spectroscopic characterizations confirm the successful and homogeneous substitution of M atoms at the Pt site, rather than intercalation, and reveal a strong correlation between nanosheet thickness and the identity of the substituting metal. High-temperature annealing of the nanosheets promotes an irreversible transformation toward the bulk phase, allowing for detailed characterization of structural and magnetic properties. A case study of Pt 0.8 Cr 0.2 Se 2 reveals that nanosheet thickness plays a critical role in modulating local magnetic interactions. While Cr atoms in the as-synthesized few-layers-thick nanosheets exhibit predominantly short-range antiferromagnetic interactions, the emergence of short-range ferromagnetic exchange is revealed in the bulk material. Detailed ac susceptibility and remanent magnetization measurements further demonstrate that bulk Pt 0.8 Cr 0.2 Se 2 adopts a frustrated magnetic ground state with clear signatures of ferromagnetic cluster-glass behavior. The systematic investigation presented herein establishes a clear and robust protocol for the synthesis and in-depth characterization of 2D transition-metal-substituted PtSe2 materials with varying layer thickness and paves a path toward their realization in spintronic and magnetic device applications.

crystallinity↗
DOE OSTI2025

Superstructure magnetic anisotropy in Fe 3 O 4 nanoparticle chains

Magnetic anisotropy is essential for many applications of ferromagnetic/ferrimagnetic materials, including permanent magnets and magnetic recording media. Attempts have been made recently to build up 3-D nanoparticle and quantum dot assemblies, however, it is not understood yet if a nanoparticle assembly can possess high magnetic anisotropy with low anisotropic materials. In this article, we report our discovery of high magnetic anisotropy resulted from Fe 3 O 4 nanoparticle chains. We started with closely-packed nanoparticle assemblies of spherical Fe 3 O 4 nanoparticles that exhibit low magnetocrystalline anisotropy and shape anisotropy, and corresponding negligible coercivity. When the nanoparticle assemblies are compressed under pressure, they form bundles or arrays that consist of Fe 3 O 4 chains with a length scale of several hundred nanometers. Magnetic measurements show that these Fe 3 O 4 chain arrays possess a high uniaxial magnetic anisotropy (K eff ~ 2.9×10 5 J/m 3 ) and significant magnetic coercivity. Our simulations reveal that interparticle magnetic dipolar interactions contribute to this type of superstructure magnetic anisotropy. This study demonstrates the feasibility and approaches to create “patterned” high magnetic anisotropy in nanoparticle superstructures/assemblies.

Mohapatra, Jeotikanta (ORCID:0000000151968626)↗
DOE OSTI2026

Determining the nature of magnetism in altermagnetic candidate RuO 2

The terminology “altermagnetism” has recently been adopted to describe collinear magnetic order with no net magnetization and nonrelativisitic, momentum-dependent spin splitting. The archetypal material used to theoretically explore altermagnetism is RuO 2 , but there has been significant debate as to whether RuO 2 possesses magnetic, let alone altermagnetic, order. To address questions surrounding the nature of magnetism in RuO 2 , we combine symmetry-sensitive torque magnetometry and magnetization measurements in single crystals up to 31 T. The data are inconsistent with collinear magnetic order possessing a Néel vector along the 𝑐 axis. Torque magnetometry further demonstrates an isotropic, field-independent magnetic susceptibility within the 𝑎⁢𝑏 plane, indicative of neither a Néel vector within the 𝑎⁢𝑏 plane nor a field-induced Néel vector reorientation. Magnetic quantum oscillations from both techniques reveal a nearly spherical Fermi surface pocket at the Brillouin zone center, in agreement with paramagnetic electronic structure calculations. Taken together, these data indicate that high-quality RuO 2 single crystals are itinerant paramagnets with no detectable long-range magnetic order and, by extension, no altermagnetism.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1993

Magnetic fields and nonuniform structures of the Moon

Direct magnetic measurements performed by space probes demonstrated the existence of small-scale, stationary surface magnetic fields on the Moon. The magnetic field averaged over a region of approximately 600 km was found to be no larger than approximately 10(exp -5) G, that of the regions approximately 100-200 km is approximately 10(exp -5) to 10(exp -4) G, and that of approximately 10-100 km reaches approximately 10(exp -3) G. Investigations of certain lunar rocks reveal stable residual magnetization, which could have been acquired during the crystallization of the rocks in the presence of the outer magnetic field, provided such a field existed at the initial stage of lunar evolution. Estimates show that 4 x 10(exp 9) yr ago the field was small, then it rose to approximately 1.3 G at the beginning of 3.9 x 10(exp 9) yr with a subsequent exponential decrease during the period of 3.9 x 10(exp 9) yr to 3.2 x 10(exp 9) yr ago. Small-scale fields have been explained by some authors as due to mechanical impacts produced by meteors. The theory of this effect is not elaborated in detail. This can in no way explain the paleomagnetic data. These data are commonly explained as a result of the dynamo action in the liquid lunar core.

Dolginov, A. Z.↗
NASA NTRS2016

Extended Magnetohydrodynamics with Embedded Particle-in-Cell Simulation of Ganymede's Magnetosphere

We have recently developed a new modeling capability to embed the implicit particle-in-cell (PIC) model iPIC3D into the Block-Adaptive-Tree-Solarwind-Roe-Upwind-Scheme magnetohydrodynamic (MHD) model. The MHD with embedded PIC domains (MHO-EPIC) algorithm Is a two-way coupled kinetic-fluid model. As one of the very first applications of the MHD-EPIC algorithm, we simulate the Interaction between Jupiter's magnetospherlc plasma and Ganymede's magnetosphere. We compare the MHO-EPIC simulations with pure Hall MHD simulations and compare both model results with Galileo observations to assess the Importance of kinetic effects In controlling the configuration and dynamics of Ganymede's magnetosphere. We find that the Hall MHD and MHO-EPIC solutions are qualitatively similar, but there are significant quantitative differences. In particular. the density and pressure inside the magnetosphere show different distributions. For our baseline grid resolution the PIC solution is more dynamic than the Hall MHD simulation and it compares significantly better with the Galileo magnetic measurements than the Hall MHD solution. The power spectra of the observed and simulated magnetic field fluctuations agree extremely well for the MHD-EPIC model. The MHO-EPIC simulation also produced a few flux transfer events (FTEs) that have magnetic signatures very similar to an observed event. The simulation shows that the FTEs often exhibit complex 3-0 structures with their orientations changing substantially between the equatorial plane and the Galileo trajectory, which explains the magnetic signatures observed during the magnetopause crossings. The computational cost of the MHO-EPIC simulation was only about 4 times more than that of the Hall MHD simulation.

Toth, Gabor↗
DOE OSTI2025

Pseudogap and Fermi arc induced by Fermi surface nesting in a centrosymmetric skyrmion magnet

Skyrmions in noncentrosymmetric materials are believed to occur due to the Dzyaloshinskii-Moriya interaction. By contrast, the skyrmion formation mechanism in centrosymmetric materials remains elusive. Here, in this work, we reveal the intrinsic electronic structure of the centrosymmetric GdRu 2 Si 2 by selectively measuring magnetic domains using angle-resolved photoemission spectroscopy (ARPES). We found robust Fermi surface (FS) nesting, consistent with the magnetic modulation q -vector detected by the previous resonant x-ray scattering measurements. The pseudogap opens at the nested FS portions, which vary for different magnetic domains. The anomalous pseudogap disconnects the FS to generate Fermi arcs with twofold symmetry. These results indicate that the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction plays a decisive role in generating the screw spin modulation responsible for the skyrmion formation in GdRu 2 Si 2 . Furthermore, we demonstrate the flexible nature of magnetism in GdRu 2 Si 2 by manipulating magnetic domains with magnetic field and temperature cyclings, providing potential future applications for data storage and processing devices.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS2020

Hall2De Simulations of a Magnetic Nozzle

The two-dimensional, fluid-based Hall thruster code Hall2De is adapted to simulate a low temperature propulsive magnetic nozzle. Electron cyclotron resonance (ECR) thrusters developed at the Office National d’Etudes et de Recherches Aérospatiales (ONERA) in France and the University of Michigan are investigated. For each device, the simulated domain is defined from the nozzle throat to a location 10 thruster radii downstream. A numerical mesh is defined based on the measured magnetic field, and the governing fluid equations for singlycharge ions, electrons, and neutrals are solved. The boundary conditions for the throat of the magnetic nozzle are based on measured values of electron temperature and ion velocity. Multiple boundary conditions for the electron temperature in the downstream regions of the domain are considered. The simulated ion velocity and potential agrees well with experiment, while the simulated divergence efficiencies and thrusts are 25% lower and 45-55% higher than experiment. When a Neumann boundary condition for electron temperature is applied to the far-plume boundaries, the nozzle was seen to be purely isothermal. This suggests that the thermal conductivity along field lines in real devices is much lower than classical simulations predict, and anomalous resistivity may be needed to reproduce the temperature distribution observed in experiment. The larger beam divergence observed in our simulation may also be related to the lack of anomalous resistivity.

Jorns, Benjamin A.↗
NASA NTRS1987

A model of ocean basin crustal magnetization appropriate for satellite elevation anomalies

A model of ocean basin crustal magnetization measured at satellite altitudes is developed which will serve both as background to which anomalous magnetizations can be contrasted and as a beginning point for studies of tectonic modification of normal ocean crust. The model is based on published data concerned with the petrology and magnetization of the ocean crust and consists of viscous magnetization and induced magnetization estimated for individual crustal layers. Thermal remanent magnetization and chemical remanent magnetization are excluded from the model because seafloor spreading anomalies are too short in wavelength to be resolved at satellite altitudes. The exception to this generalization is found at the oceanic magnetic quiet zones where thermal remanent magnetization and chemical remanent magnetization must be considered along with viscous magnetization and induced magnetization.

Thomas, Herman H.↗
NASA NTRS1995

Tape casting and partial melting of Bi-2212 thick films

To produce Bi-2212 thick films with high critical current densities tape casting and partial melting is a promising fabrication method. Bi-2212 powder and organic additives were mixed into a slurry and tape casted onto glass by the doctor blade tape casting process. The films were cut from the green tape and partially molten on Ag foils during heat treatment. We obtained almost single-phase and well-textured films over the whole thickness of 20 microns. The orientation of the (a,b)-plane of the grains was parallel to the substrate with a misalignment of less than 6 deg. At 77 K/0T a critical current density of 15, 000 A/sq cm was reached in films of the dimension 1 cm x 2 cm x 20 microns (1 micron V/cm criterion, resistively measured). At 4 K/0T the highest value was 350,000 A/sq cm (1 nV/cm criterion, magnetically measured).

Buhl, D.↗
DOE OSTI2025

Understanding the Electronic Behavior of f-Element Intermetallics

Due to their partially filled f-orbitals, lanthanide and actinide intermetallic materials exhibit intriguing electronic, structural, and magnetic properties. These materials provide a unique platform to explore exotic magnetic and quantum phenomena that arise from their strongly correlated f-electrons, offering insights into f-electron behavior. Incorporating light elements such as boron and carbon can significantly impact the electronic, chemical, and physical properties of these materials, with varying influence between lanthanides and actinides due to the more localized f-electrons in lanthanides. In this work, lanthanide-based intermetallic single crystals containing light atoms were synthesized using the molten metal flux growth method. In this method, one or more low-melting metals such as aluminum, gallium, tin, and bismuth are used in excess as the reaction medium. This solution-state approach allows for lower reaction temperatures compared to solid-state reactions and enables the isolation of kinetic products rather than thermodynamically stable compounds. The synthesized crystals were analyzed using an extensive array of analytical and computational characterization techniques, including single crystal X-ray diffraction, scanning electron microscopy, energy-dispersive spectroscopy, magnetization measurements, and density functional theory calculations. These analyses provided detailed insights into the structural and magnetic properties of the synthesized materials.

37 - INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL C↗
NASA NTRS2019

Highly Structured Slow Solar Wind Emerging From an Equatorial Coronal Hole

At solar minimum, the solar wind is observed at high solar latitudes as a predominantly fast (> 500 km/s), highly Alfvenic, rarefied stream of plasma originating deep within coronal holes, while near the ecliptic plane it is interspersed with a more variable slow (< 500 kms) wind. The precise origins of the slow wind streams are less certain, with theories and observations supporting sources from the tips of helmet streamers, interchange reconnection near coronal hole boundaries, and origins within coronal holes with highly diverging magnetic fields. The heating mechanism required to drive the solar wind is also an open question and candidate mechanisms include Alfven wave turbulence, heating by reconnection in nanoflares, ion cyclotron wave heating and acceleration by thermal gradients1. At 1 au, the wind is mixed and evolved and much of the diagnostic structure of these sources and processes has been lost. Here we present new measurements from Parker Solar Probe at 36 to 54 solar radii that show clear evidence of slow, Alfvenic solar wind emerging from a small equatorial coronal hole. The measured magnetic field exhibits patches of large, intermittent reversals associated with jets of plasma and enhanced Poynting flux and interspersed in a smoother and less turbulent flow with near-radial magnetic field. Furthermore, plasma wave measurements suggest electron and ion velocity-space micro-instabilities that have been identified with plasma heating and thermalization processes. Our measurements suggest an impulsive mechanism associated with solar wind energization and a heating role for micro-instabilities and provide strong evidence for low latitude coronal holes as a significant contribution to the source of the slow solar wind.

Solar physics↗
NASA NTRS1990

Nonlogarithmic magnetization relaxation at the initial time intervals and magnetic field dependence of the flux creep rate in Bi2Sr2Ca(sub I)Cu2Ox single crystals

At the initial time intervals, preceding the thermally activated flux creep regime, fast nonlogarithmic relaxation is found. The fully magnetic moment Pm(t) relaxation curve is shown. The magnetic measurements were made using SQUID-magnetometer. Two different relaxation regimes exist. The nonlogarithmic relaxation for the initial time intervals may be related to the viscous Abrikosov vortices flow with j is greater than j(sub c) for high enough temperature T and magnetic field induction B. This assumption correlates with Pm(t) measurements. The characteristic time t(sub O) separating two different relaxation regimes decreases as temperature and magnetic field are lowered. The logarithmic magnetization relaxation curves Pm(t) for fixed temperature and different external magnetic field inductions B are given. The relaxation rate dependence on magnetic field, R(B) = dPm(B, T sub O)/d(1nt) has a sharp maximum which is similar to that found for R(T) temperature dependences. The maximum shifts to lower fields as temperature goes up. The observed sharp maximum is related to a topological transition in shielding critical current distribution and, consequently, in Abrikosov vortices density. The nonlogarithmic magnetization relaxation for the initial time intervals is found. This fast relaxation has almost an exponentional character. The sharp relaxation rate R(B) maximum is observed. This maximum corresponds to a topological transition in Abrikosov vortices distribution.

Moshchalcov, V. V.↗
NASA NTRS1989

A comparative study of sintered and melt-grown recrystallized YBa2Cu3Ox

This paper compares the properties of yttrium barium cuprate bulk specimens prepared by means of solid-state sintering on one hand and of growth from a largely molten state on the other. The current paper focuses on magnetization measurements at 77 K which show specimens made by the latter method to have high remanence magnetization values.

Hojaji, Hamid↗
NASA NTRS2011

Geomagnetic Variability and Predictability

The Earth's magnetic field varies on time scales from seconds to millions of years. These variations can be measured directly by ground observatories and satellites, and indirectly through laboratories. They are from different electromagnetic processes in magnetosphere and ionosphere (external), ocean and crust (surface), and deep in the Earth's fluid outer core (internal). Of the measured magnetic signals, 95% is from the core, and is called the core field, or internal field. Variation of the core field, often called the geomagnetic secular variation (SV), is the manifestation of the magnetohydrodynamic processes in the core. Therefore, SV provides rich information on the core dynamical state that is then critical for understanding the geophysical mechanisms of the SV, the core-mantle interactions, and contribution of mass transport inside the core on Earth's gravity variation. Traditionally, the core state is probed via two independent methodologies: core flow inversion from the observed SV, and pure numerical dynamo simulation. The former is driven by observations, but does not include necessary interactions among physical variables; the latter is dynamically consistent, but is not constrained by any observation. Therefore, both are very limited in providing appropriate estimates of the core state. To avoid these limitations, a new approach, geomagnetic data assimilation, appears recently. In this approach, simulation results (model forecasts) are constantly corrected with observations, the corrected solutions (analysis), are then used as the initial conditions to make more accurate forecasts of future. Recent studies have demonstrated successfully that assimilation solutions are different from those of free running models. These new solutions are better estimates of the core state, and have been used to provide accurate prediction of SV for the period from 2010 to 2015. This prediction is part of the IGRF field model for international community applications.

Kuang, Weijia↗
DOE OSTI2026

Complex magnetic ground state driving a large rotating magnetocaloric effect in Tb 3 Ni at low temperature

The rotating magnetocaloric effect (RMCE) offers a promising alternative to conventional magnetocaloric configurations by taking advantage of magnetic anisotropy to simplify device architecture and enhance refrigeration efficiency. In this study, the RMCE in a high-quality single crystal of Tb 3 Ni is investigated, a compound previously shown to exhibit significant magnetocaloric behavior along its easy axis of magnetization. By measuring the magnetization and corresponding entropy change along the three principal crystallographic axes using a discontinuous measurement protocol, we verify the anisotropic magnetic properties and derive the RMCE from rotations between hard ( a, b ) and easy ( c ) axes of magnetization. Our results show a maximum value for the rotating entropy change of 19.5 J kg −1 K −1 for µ 0 H = 7 T around 60 K, within the critical temperature window for industrial gas liquefaction applications. Neutron diffraction and magnetic Pair-Distribution Function (mPDF) analysis reveal that the origin of this large anisotropic response lies in a partially ordered incommensurate spin-density wave phase and persistent short-range ferromagnetic (FM) correlations. These complex magnetic states enable the release of a substantial amount of magnetic entropy when the field is applied along the easy c-axis, effectively driving the large RMCE. Comparison with other RMCE materials confirms Tb 3 Ni as one of the most promising candidates in this temperature regime, offering both a large magnetic entropy change and a wide operating window.

Gas liquefaction↗
NASA NTRS1991

Lower critical field measurements in YBa2Cu3O(6+x) single crystals

The temperature dependence of the lower critical field in YBa2Cu3O(6+x) single crystals was determined by magnetization measurements with the applied field parallel and perpendicular to the c-axis. Results are compared with data from the literature and fitted to Ginzberg-Landau equations by assuming a linear dependence of the parameter kappa on temperature. A value of 7 plus or minus 2 kOe was estimated for the thermodynamic critical field at T = O by comparison of calculated H (sub c2) values with experimental data from the literature.

Kaiser, D. L.↗
NASA NTRS1994

A New Approach to Isolating External Magnetic Field Components in Spacecraft Measurements of the Earth's Magnetic Field Using Global Positioning System observables

We review the problem of separating components of the magnetic field arising from sources in the Earth's core and lithosphere, from those contributions arising external to the Earth, namely ionospheric and magnetospheric fields, in spacecraft measurements of the Earth's magnetic field.

magnetic field components ionospheric and magnetos↗