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NASA NTRS2001

Airborne Sunphotometry of Aerosol Optical Depth and Columnar Water Vapor During ACE-Asia

During the Intensive Field Campaign (IFC) of the Aerosol Characterization Experiment - Asia (ACE-Asia), March-May 2001, the 6-channel NASA Ames Airborne Tracking Sunphotometer (AATS-6) operated during 15 of the 19 research flights aboard the NCAR C- 130, while its 14-channel counterpart (AATS- 14) was flown successfully on all 18 research flights of a Twin Otter aircraft operated by the Center for Interdisciplinary Remotely Piloted Aircraft Studies (CIRPAS), Monterey, CA. ACE-Asia was the fourth in a series of aerosol characterization experiments and focused on aerosol outflow from the Asian continent to the Pacific basin. Each ACE was designed to integrate suborbital and satellite measurements and models so as to reduce the uncertainty in calculations of the climate forcing due to aerosols. The Ames Airborne Tracking Sunphotometers measured solar beam transmission at 6 (380-1021 nm, AATS-6) and 14 wavelengths (353-1558 nm, AATS-14) respectively, yielding aerosol optical depth (AOD) spectra and column water vapor (CWV). Vertical differentiation in profiles yielded aerosol extinction and water vapor concentration. The wavelength dependence of AOD and extinction indicates that supermicron dust was often a major component of the aerosol. Frequently this dust-containing aerosol extended to high altitudes. For example, in data flights analyzed to date 34 +/- 13% of full-column AOD(525 nm) was above 3 km. In contrast, only 10 +/- 4% of CWV was above 3 km. In this paper, we will show first sunphotometer-derived results regarding the spatial variation of AOD and CWV, as well as the vertical distribution of aerosol extinction and water vapor concentration. Preliminary comparison studies between our AOD/aerosol extinction data and results from: (1) extinction products derived using in situ measurements and (2) AOD retrievals using the Multi-angle Imaging Spectro-Radiometer (MISR) aboard the TERRA satellite will also be presented.

Redemann, Jens↗

NASA NTRS2002

The Measurement of Aerosol Optical Properties using Continuous Wave Cavity Ring-Down Techniques

Large uncertainties in the effects that aerosols have on climate require improved in situ measurements of extinction coefficient and single-scattering albedo. This paper describes the use of continuous wave cavity ring-down (CW-CRD) technology to address this problem. The innovations in this instrument are the use of CW-CRD to measure aerosol extinction coefficient, the simultaneous measurement of scattering coefficient, and small size suitable for a wide range of aircraft applications. Our prototype instrument measures extinction and scattering coefficient at 690 nm and extinction coefficient at 1550 nm. The instrument itself is small (60 x 48 x 15 cm) and relatively insensitive to vibrations. The prototype instrument has been tested in our lab and used in the field. While improvements in performance are needed, the prototype has been shown to make accurate and sensitive measurements of extinction and scattering coefficients. Combining these two parameters, one can obtain the single-scattering albedo and absorption coefficient, both important aerosol properties. The use of two wavelengths also allows us to obtain a quantitative idea of the size of the aerosol through the Angstrom exponent. Minimum sensitivity of the prototype instrument is 1.5 x 10(exp -6)/m (1.5 M/m). Validation of the measurement of extinction coefficient has been accomplished by comparing the measurement of calibration spheres with Mie calculations. This instrument and its successors have potential to help reduce uncertainty currently associated with aerosol optical properties and their spatial and temporal variation. Possible applications include studies of visibility, climate forcing by aerosol, and the validation of aerosol retrieval schemes from satellite data.

Strawa, Anthony W.↗

NASA NTRS2002

Airborne Sunphotometer Measurements of Aerosol Optical Depth and Water Vapor in ACE-Asia and Their Comparisons to Correlative Measurements

In the Spring 2001 phase of the Asian Pacific Regional Aerosol Characterization Experiment (ACE-Asia), the 6-channel NASA Ames Airborne Tracking Sunphotometer (AATS-6) operated on 15 of the 19 research flights of the NCAR C-130, while its 14-channel counterpart (AATS-14) flew successfully on all 19 research flights of the CIRPAS Twin Otter. ACE-Asia studied aerosol outflow from the Asian continent to the Pacific basin. It was designed to integrate suborbital and satellite measurements and models to reduce the uncertainty in calculations of the climate forcing due to aerosols. AATS-6 and AATS-14 measured solar beam transmission at six and 14 wavelengths (380-1021 and 354-1558 nm, respectively), yielding aerosol optical depth (AOD) spectra and columnar water vapor (CWV). Vertical differentiation in profiles yielded aerosol extinction spectra and water vapor concentration. In this paper, we plan to present examples of the following, preliminary findings that are based in part on our airborne sunphotometer measurements: (1) The wavelength dependence of sunphotometer-derived AOD and extinction indicates that supermicron dust was often a major component of the aerosol, frequently extending to high altitudes. The percentage of full-column AOD (525 nm) that Jay above 3 km was typically 34+/-13%. In contrast, the analogous percentage of columnar water vapor was only 10+/-4%; (2) Initial comparison studies between AOD data obtained by AATS-6 and AATS-14 during coordinated low-level flight legs show agreement well within the instruments' error bars; (3) Aerosol extinction has been derived from airborne in situ measurements of scattering (nephelometers) and absorption (particle soot/ absorption photometer, PSAP) or calculated from particle size distribution measurements (mobility analyzers and aerodynamic particle sizers). Comparison with corresponding extinction values derived from the Ames airborne sunphotometer measurements shows good agreement for the vertical distribution of aerosol layers. However, the level of agreement in absolute magnitude of the derived aerosol extinction/optical depth varied among the aerosol layers sampled; (4) Initial comparisons of sunphotometer and satellite-derived AOD using SeaWiFS, MISR and AVHRR show promising results. We also plan to include comparisons with MODIS and TOMS: (5) Initial comparisons of sunphotometer-derived AOD and aerosol extinction profiles with lidars in Tokyo and on a ship show reasonable agreement.

Schmid, B.↗

NASA NTRS2002

The Measurement of Aerosol Optical Properties Using Continuous Wave Cavity Ring-Down Techniques

Large uncertainties in the effects that aerosols have on climate require improved in-situ measurements of extinction coefficient and single-scattering albedo. This abstract describes the use of continuous wave cavity ring-down (CW-CRD) technology to address this problem. The innovations in this instrument are the use of CW-CRD to measure aerosol extinction coefficient, the simultaneous measurement of scattering coefficient, and small size suitable for a wide range of aircraft applications. Our prototype instrument measures extinction and scattering coefficient at 690 nm and extinction coefficient at 1550 nm. The instrument itself is small (60 x 48 x 15 cm) and relatively insensitive to vibrations. The prototype instrument has been tested in our lab and used in the field. While improvements in performance are needed, the prototype has been shown to make accurate and sensitive measurements of extinction and scattering coefficients. Combining these two parameters, one can obtain the single-scattering albedo and absorption coefficient, both important aerosol properties. The use of two wavelengths also allows us to obtain a quantitative idea of the size of the aerosol through the Angstrom exponent. Minimum sensitivity of the prototype instrument is 1.5 x 10(exp -6)/m (1.5/Mm). Validation of the measurement of extinction coefficient has been accomplished by comparing the measurement of calibration spheres with Mie calculations. This instrument and its successors have potential to help reduce uncertainty currently associated with aerosol optical properties and their spatial and temporal variation. Possible applications include studies of visibility, climate forcing by aerosol, and the validation of aerosol retrieval schemes from satellite data.

Strawa, A. W.↗

NASA NTRS2003

Effect of Smoke on Cloud Formation during the Biomass Burning Season over the Amazon Basin

Aerosol absorption of sunlight reduces surface irradiation and heats the aerosol layer. The consequent changes in the temperature and humidity profiles can affect cloud formation extent and life time, which is called the semi-direct effect. We evaluate this aerosol semi-direct effect using data collected during the 2002 biomass burning season over the Amazon basin from the MODIS instrument on the Aqua satellite. MODIS measures the cloud coverage and the aerosol optical thickness among the clouds. We found that the radiative heating of the atmosphere and cooling of the surface due to the presence of the smoke decreases the cloud coverage. A very clear negative correlation emerges between the cloud fraction and the smoke optical depth. The results are compared to calculations using 1-D radiation model (M.D. Chou), and used to calculate this regional semi direct effect on climate forcing.

Koren, I.↗

NASA NTRS2003

TRMM Fire Algorithm, Product and Applications

Land fires are frequent menaces to human lives and property. They also change the state of the vegetation and contribute to the climate forcing by releasing large amount of aerosols and greenhouse gases into the atmosphere. This paper summarizes methodologies of detecting global land fires from the Tropical Rainfall Measuring Mission (TRMM) Visible Infrared Scanner FIRS) measurements. The TRMM Science Data and Information System (TSDIS) fire products include global images of daily hot spots and monthly fire counts at 0.5 deg. x 0.5 deg. resolution, as well as text fiies that details necessary information of all fire pixels. The information includes date, orbit number, pixel number, local time, solar zenith angle, latitude, longitude, reflectance of visible/near infrared channels, brightness temperatures of infrared channels, as well as background brightness temperatures of infrared channels. These products have been archived since January 1998. The TSDIS fire products are compared with the coincidental European Commission (EC) Joint Research Center (JRC) 1 km AVHRR fire products. Analyses of the TSDIS monthly fire products during the period from 1998 to 2003 manifested seasonal cycles of biomass fires over Southeast Asia, Africa, North America and South America. The data also showed interannual variations associated with the 98/99 ENS0 cycle in Central America and the Indonesian region. In order to understand the variability of global land fires and their effects on the distribution of atmospheric aerosols, statistical methods were applied to the TSDIS fire products as well as to the Total Ozone Mapping Spectrometer (TOMS) aerosol index products for a period of five years from January 1998 to December 2002. The variability of global atmospheric aerosol is consistent with the fire variations over these regions during this period. The correlation between fire count and TOMS aerosol index is about 0.55 for fire pixels in Southeast Asia, Indonesia, and Africa. Parallel statistical analyses such as Empirical Orthogonal Function (EOF) analysis and Singular Spectrum Analysis (SSA) methods were applied to pentad TRMM fire data and TOMS aerosol data. The EOF analyses showed contrast between North and South hemispheres and also inter- continental transitions in Africa and America. EOF and SSA analyses also identified 25-60 day intra-seasonal oscillations that were superimposed on the annual cycles of both fire and aerosol data. The intra-seasonal variability of fires showed similarity of tropical rainfall oscillation modes. The TRMM fire products were also compared to the coincident TRMh4 rainfall and other rainfall products to investigate the interaction between rainfall and fire. The results indicate that the annual, interannual and intraseasonal variability of fire are dominated by global rainfall variations. However, the feedback of fire to the rainfall occurrence at regional scale for certain regions is also evident.

Ji, Yi-Min↗

NASA NTRS2003

Advanced Global Atmospheric Gases Experiment (AGAGE): MIT Contribution

We describe in detail the instrumentation and calibrations used in the ALE, GAGE and AGAGE experiments and present a history of the majority of the anthropogenic ozone- depleting and climate-forcing gases in air based on these experiments. Beginning in 1978, these three successive automated high frequency in-situ experiments have documented the long-term behavior of the measured concentrations of these gases over the past twenty years, and show both the evolution of latitudinal gradients and the high frequency variability due to sources and circulation. We provide estimates of the long-term trends in total chlorine contained in long- lived halocarbons involved in ozone depletion. We summarize interpretations of these measurements using inverse methods to determine trace gas lifetimes and emissions. Finally, we provide a combined observational and modeled reconstruction of the evolution of chlorocarbons by latitude in the atmosphere over the past sixty years which can be used as boundary conditions for interpreting trapped air in glaciers and oceanic measurements of chlorocarbon tracers of the deep oceanic circulation. Some specific conclusions are: (a) International compliance with the Montreal Protocol is so far resulting in chlorofluorocarbon and chlorocarbon mole fractions comparable to target levels, (b) Mole fractions of total chlorine contained in long-lived halocarbons (CCl2F2, CCl3F, CH3CCl3, CCl4, CHClF2, CCl2FCClF2, CH3Cl, CH2Cl2, CHCl3, CCl2=CCl2) in the lower troposphere reached maximum values of about 3.6 ppb in 1993 and are beginning to slowly decrease in the global lower atmosphere, (c) The chlorofluorocarbons have atmospheric lifetimes consistent with destruction in the stratosphere being their principal removal mechanism, (d) Multi-annual variations in chlorofluorocarbon and chlorocarbon emissions deduced from ALUGAGWAGAGE data are consistent approximately with variations estimated independently from industrial production and sales data where available (CCl2F2 (CFC-12) and CCl2FCClF2 (CFC-113) show the greatest discrepancies), (e) The mole fractions of the hydrochlorofluorocarbons and hydrofluorocarbons, which are replacing the regulated halocarbons, are rising very rapidly in the atmosphere but, with the exception of the much longer manufactured CHClF2 (HCFC-22), they are not yet at levels sufficient to contribute significantly to atmospheric chlorine loading. These replacement species could in the future provide independent estimates of the global weighted-average OH concentration provided their industrial emissions are accurately documented, (f) In the future, analysis of pollution events measured using high frequency in-situ measurements of chlorofluorocarbons and their replacements may enable emission estimates at the regional level which, together with industrial end-use data, are of sufficient accuracy to be capable of identifying regional non-compliance with the Montreal Protocol.

Kurylo, Michael↗

NASA NTRS2005

Entrainment, Drizzle, and the Indirect Effect in Stratiform Clouds

Activation of some fraction of increased concentrations of sub-micron soluble aerosol particles lead to enhanced cloud droplet concentrations and hence smaller droplets, increasing their total cross sectional area and thus reflecting solar radiation more efficiently (the Twomey, or first indirect, effect). However, because of competition during condensational growth, droplet distributions tend to broaden as numbers increase, reducing the sensitivity of cloud albedo to droplet concentration on the order of 10%. Also, smaller droplets less effectively produce drizzle through collisions and coalescence, and it is widely expected (and found in large-scale models) that decreased precipitation leads to clouds with more cloud water on average (the so-called cloud lifetime, or second indirect, effect). Much of the uncertainty regarding the overall indirect aerosol effect stems from inadequate understanding of such changes in cloud water. Detailed simulations based on FIRE-I, ASTEX, and DYCOMS-II conditions show that suppression of precipitation from increased droplet concentrations leads to increased cloud water only when sufficient precipitation reaches the surface, a condition favored when the overlying air is-humid or droplet concentrations are very low. Otherwise, aerosol induced suppression of precipitation enhances entrainment of overlying dry air, thereby reducing cloud water and diminishing the indirect climate forcing.

Ackerman, Andrew↗

NASA NTRS2005

Global Retrieval of Aerosol Properties over Desert and Semi-Desert Regions from SeaWiFS and MODIS

Mineral aerosols (dust) play an important role in both climate forcing and oceanic productivity throughout the entire year. Due to the relatively short lifetime (a few hours to about a week), the distributions of these airborne dust particles vary extensively in both space and time. Consequently, satellite observations are needed over both source and sink regions for continuous temporal and spatial sampling of dust properties. However, despite their importance, the high spatial resolution satellite measurements of dust near its source have been lacking. In this paper, we will demonstrate the capability of a new satellite algorithm to retrieve aerosol optical thickness and single scattering albedo over bright-reflecting surfaces such as urban areas and deserts. Such retrievals have been difficult to perform using previously available algorithms that use wavelengths from the mid-visible to the near IR because they have trouble separating the aerosol signal from the contribution due to the bright surface reflectance. The new algorithm, called Deep Blue, utilizes blue-wavelength measurements from instruments such as SeaWiFS and MODIS to infer the properties of aerosols, sinre the stirfare reflectance nver land in the blue part of the spectrum is much lower than for longer wavelength channels. We have validated the satellite retrieved aerosol optical thickness with data from AERONET sunphotometers over desert and semi-desert regions. The comparisons show reasonable agreements between these two. These new satellite products will allow scientists to determine quantitatively the aerosol properties near sources using high spatial resolution measurements from SeaWiFS and MODIS-like instruments.

Hsu, Nai-Yung↗

NASA NTRS2005

Global Retrieval of Aerosol Properties from Sources to Sinks By MODIS

Mineral dust and smoke aerosols play an important role in both climate forcing and oceanic productivity throughout the entire year. Due to the relatively short lifetime (a few hours to about a week), the distributions of these airborne particles vary extensively in both space and time. Consequently, satellite observations are needed over both source and sink regions for continuous temporal and spatial sampling of dust and smoke properties. However, despite their importance, the high spatial resolution satellite measurements of these aerosols near their sources have been lacking, In this paper, we will demonstrate the capability of a new satellite algorithm to retrieve aerosol optical thickness and single scattering albedo over bright-reflecting surfaces such as urban areas and deserts. Such retrievals have been difficult to perform using previously available algorithms that use wavelengths from the mid-visible to the near IR because they have trouble separating the aerosol signal from the contribution due to the bright surface reflectance. The new algorithm, called Deep Blue, utilizes blue-wavelength measurements from instruments such as MODIS and SeaWiFS to infer the properties of aerosols, since the surface reflectance over land in the blue part of the spectrum is much lower than for longer wavelength channels. We have validated the satellite retrieved aerosol optical thickness with data from AERONET sunphotometers over land, including desert and semi-desert regions. The comparisons show reasonable agreements between these two. Our results show that the dust plumes lifted from the deserts near India/Pakistan border, and over Afghanistan, and the Arabian Peninsula are often observed by MODIS to be transported along the Indo-Gangetic Basin and mixed with the fine mode pollution particles generated by anthropogenic activities in this region, particularly during the pre-monsoon season (April-May). These new satellite products will allow scientists to determine quantitatively the aerosol properties near sources using high spatial resolution measurements from SeaWiFS and MODIS-like instruments.

Hsu, N. Christina↗

NASA NTRS2008

Smoke Invigoration Versus Inhibition of Clouds over the Amazon

The effect of anthropogenic aerosols on clouds is one of the most important and least understood aspects of human-induced climate change. Small changes in the amount of cloud coverage can produce a climate forcing equivalent in magnitude and opposite in sign to that caused by anthropogenic greenhouse gases, and changes in cloud height can shift the effect of clouds from cooling to warming. Focusing on the Amazon, we show a smooth transition between two opposing effects of aerosols on clouds: the microphysical and the radiative. We show how a feedback between the optical properties of aerosols and the cloud fraction can modify the aerosol forcing, changing the total radiative energy and redistributing it over the atmospheric column.

Koren, Ilan↗

NASA NTRS2010

Aerosol Absorption by Black Carbon and Dust: Implications of Climate Change and Air Quality in Asia

Atmospheric aerosol distributions from 2000 to 2007 are simulated with the global model GOCART to attribute light absorption by aerosol to its composition and sources. We show the seasonal and interannual variations of absorbing aerosols in the atmosphere over Asia, mainly black carbon and dust. and their linkage to the changes of anthropogenic and dust emissions in the region. We compare our results with observations from satellite and ground-based networks, and estimate the importance of black carbon and dust on regional climate forcing and air quality.

Chin, Mian↗

NASA NTRS2010

Aircraft Trajectory Optimization and Contrails Avoidance in the Presence of Winds

There are indications that persistent contrails can lead to adverse climate change, although the complete effect on climate forcing is still uncertain. A flight trajectory optimization algorithm with fuel and contrails models, which develops alternative flight paths, provides policy makers the necessary data to make tradeoffs between persistent contrails mitigation and aircraft fuel consumption. This study develops an algorithm that calculates wind-optimal trajectories for cruising aircraft while avoiding the regions of airspace prone to persistent contrails formation. The optimal trajectories are developed by solving a non-linear optimal control problem with path constraints. The regions of airspace favorable to persistent contrails formation are modeled as penalty areas that aircraft should avoid and are adjustable. The tradeoff between persistent contrails formation and additional fuel consumption is investigated, with and without altitude optimization, for 12 city-pairs in the continental United States. Without altitude optimization, the reduction in contrail travel times is gradual with increase in total fuel consumption. When altitude is optimized, a two percent increase in total fuel consumption can reduce the total travel times through contrail regions by more than six times. Allowing further increase in fuel consumption does not seem to result in proportionate decrease in contrail travel times.

Ng, Hok K.↗

NASA NTRS2011

The NASA Decadal Survey Aerosol, Cloud, Ecosystems Mission

In 2007, the National Academy of Sciences delivered a Decadal Survey (Earth Science and Applications from Space: National Imperatives for the Next Decade and Beyond) for NASA, NOAA, and USGS, which is a prioritization of future satellite Earth observations. The recommendations included 15 missions (13 for NASA, two for NOAA), which were prioritized into three groups or tiers. One of the second tier missions is the Aerosol, Cloud, (ocean) Ecosystems (ACE) mission, which focuses on climate forcing, cloud and aerosol properties and interactions, and ocean ecology, carbon cycle science, and fluxes. The baseline instruments recommended for ACE are a cloud radar, an aerosol/cloud lidar, an aerosol/cloud polarimeter, and an ocean radiometer. The instrumental heritage for these measurements are derived from the Cloudsat, CALIPSO, Glory, SeaWiFS and Aqua (MODIS) missions. In 2008, NASA HQ, lead by Hal Maring and Paula Bontempi, organized an interdisciplinary science working group to help formulate the ACE mission by refining the science objectives and approaches, identifying measurement (satellite and field) and mission (e.g., orbit, data processing) requirements, technology requirements, and mission costs. Originally, the disciplines included the cloud, aerosol, and ocean biogeochemistry communities. Subsequently, an ocean-aerosol interaction science working group was formed to ensure the mission addresses the broadest range of science questions possible given the baseline measurements, The ACE mission is a unique opportunity for ocean scientists to work closely with the aerosol and cloud communities. The science working groups are collaborating on science objectives and are defining joint field studies and modeling activities. The presentation will outline the present status of the ACE mission, the science questions each discipline has defined, the measurement requirements identified to date, the current ACE schedule, and future opportunities for broader community participation.

McClain, Charles R.↗

NASA NTRS2011

Sea-Level Projections from the SeaRISE Initiative

SeaRISE (Sea-level Response to Ice Sheet Evolution) is a community organized modeling effort, whose goal is to inform the fifth IPCC of the potential sea-level contribution from the Greenland and Antarctic ice sheets in the 21st and 22nd century. SeaRISE seeks to determine the most likely ice sheet response to imposed climatic forcing by initializing an ensemble of models with common datasets and applying the same forcing to each model. Sensitivity experiments were designed to quantify the sea-level rise associated with a change in: 1) surface mass balance, 2) basal lubrication, and 3) ocean induced basal melt. The range of responses, resulting from the multi-model approach, is interpreted as a proxy of uncertainty in our sea-level projections. http://websrv.cs .umt.edu/isis/index.php/SeaRISE_Assessment.

Nowicki, Sophie↗

NASA NTRS2012

Recent Progress on Deep Blue Aerosol Algorithm as Applied TO MODIS, SEA WIFS, and VIIRS, and Their Intercomparisons with Ground Based and Other Satellite Measurements

The impact of natural and anthropogenic sources of aerosols has gained increasing attention from scientific communities in recent years. Indeed, tropospheric aerosols not only perturb radiative energy balance by interacting with solar and terrestrial radiation, but also by changing cloud properties and lifetime. Furthermore, these anthropogenic and natural air particles, once generated over the source regions, can be transported out of the boundary layer into the free troposphere and can travel thousands of kilometers across oceans and continents resulting in important biogeochemical impacts on the ecosystem. With the launch of SeaWiFS in 1997, Terra/MODIS in 1999, and Aqua/MODIS in 2002, high quality comprehensive aerosol climatology is becoming feasible for the first time. As a result of these unprecedented data records, studies of the radiative and biogeochemical effects due to tropospheric aerosols are now possible. In this talk, we will demonstrate how this newly available SeaWiFS/MODIS aerosol climatology can provide an important piece of puzzles in reducing the uncertainty of estimated climatic forcing due to aerosols. We will start with the global distribution of aerosol loading and their variabilities over both land and ocean on short- and long-term temporal scales observed over the last decade. The recent progress made in Deep Blue aerosol algorithm on improving accuracy of these Sea WiFS / MODIS aerosol products in particular over land will be discussed. The impacts on quantifying physical and optical processes of aerosols over source regions of adding the Deep Blue products of aerosol properties over bright-reflecting surfaces into Sea WiFS / MODIS as well as VIIRS data suite will also be addressed. We will also show the intercomparison results of SeaWiFS/MODIS retrieved aerosol optical thickness with data from ground based AERONET sunphotometers over land and ocean as well as with other satellite measurements. The trends observed in global aerosol loadings of both natural and anthropogenic sources based upon more than a decade of combined MODIS/SeaWiFS data (1997-2011) will be discussed. We will also address the importance of various key issues such as differences in spatial-temporal sampling rates and observation time between different satellite measurements could potentially impact these intercomparisons results, especially for using the monthly mean data, and thus on estimates of long-term aerosol trends.

Hsu, N. Christina↗

NASA NTRS2012

Constraining Middle Atmospheric Moisture in GEOS-5 Using EOS-MLS Observations

Middle atmospheric water vapor plays an important role in climate and atmospheric chemistry. In the middle atmosphere, water vapor, after ozone and carbon dioxide, is an important radiatively active gas that impacts climate forcing and the energy balance. It is also the source of the hydroxyl radical (OH) whose abundances affect ozone and other constituents. The abundance of water vapor in the middle atmosphere is determined by upward transport of dehydrated air through the tropical tropopause layer, by the middle atmospheric circulation, production by the photolysis of methane (CH4), and other physical and chemical processes in the stratosphere and mesosphere. The Modern-Era Retrospective analysis for Research and Applications (MERRA) reanalysis with GEOS-5 did not assimilate any moisture observations in the middle atmosphere. The plan is to use such observations, available sporadically from research satellites, in future GEOS-5 reanalyses. An overview will be provided of the progress to date with assimilating the EOS-Aura Microwave Limb Sounder (MLS) moisture retrievals, alongside ozone and temperature, into GEOS-5. Initial results demonstrate that the MLS observations can significantly improve the middle atmospheric moisture field in GEOS-5, although this result depends on introducing a physically meaningful representation of background error covariances for middle atmospheric moisture into the system. High-resolution features in the new moisture field will be examined, and their relationships with ozone, in a two-year assimilation experiment with GEOS-5. Discussion will focus on how Aura MLS moisture observations benefit the analyses.

Jin, Jianjun↗

NASA NTRS2012

Impacts of the Convective Transport Algorithm on Atmospheric Composition and Ozone-Climate Feedbacks in GEOS-CCM

Convective transport is one of the dominant factors in determining the composition of the troposphere. It is the main mechanism for lofting constituents from near-surface source regions to the middle and upper troposphere, where they can subsequently be advected over large distances. Gases reaching the upper troposphere can also be injected through the tropopause and play a subsequent role in the lower stratospheric ozone balance. Convection codes in climate models remain a great source of uncertainty for both the energy balance of the general circulation and the transport of constituents. This study uses the Goddard Earth Observing System Chemistry-Climate Model (GEOS CCM) to perform a controlled experiment that isolates the impact of convective transport of constituents from the direct changes on the atmospheric energy balance. Two multi-year simulations are conducted. In the first, the thermodynamic variable, moisture, and all trace gases are transported using the multi-plume Relaxed-Arakawa-Schubert (RAS) convective parameterization. In the second simulation, RAS impacts the thermodynamic energy and moisture in this standard manner, but all other constituents are transported differently. The accumulated convective mass fluxes (including entrainment and detrainment) computed at each time step of the GCM are used with a diffusive (bulk) algorithm for the vertical transport, which above all is less efficient at transporting constituents from the lower to the upper troposphere. Initial results show the expected differences in vertical structure of trace gases such as carbon monoxide, but also show differences in lower stratospheric ozone, in a region where it can potentially impact the climate state of the model. This work will investigate in more detail the impact of convective transport changes by comparing the two simulations over many years (1996-2010), focusing on comparisons with observed constituent distributions and similarities and differences of patterns of inter-annual variability caused by the convective transport algorithm. In particular, the impact on lower stratospheric composition will be isolated and the subsequent feedbacks of ozone on the climate forcing and tropopause structure will be assessed.

Pawson, S.↗