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DOE OSTI2024

Spatially Resolved Near Field Spectroscopy of Vibrational Polaritons at the Small N Limit

Vibrational polaritons, which have been primarily studied in Fabry–Pérot cavities with a large number of molecules (N ~ 10 6 –10 10 ) coupled to the resonator mode, exhibit various experimentally observed effects on chemical reactions. However, the exact mechanism is elusively understood from the theoretical side, as the large number of molecules involved in an experimental strong coupling condition cannot be represented completely in simulations. This discrepancy between theory and experiment arises from computational descriptions of polariton systems typically being limited to only a few molecules, thus failing to represent the experimental conditions adequately. To address this mismatch, we used surface phonon polariton (SPhP) resonators as an alternative platform for vibrational strong coupling. SPhPs exhibit strong electromagnetic confinement on the surface and thus allow for coupling to a small number of molecules. As a result, this platform can enhance nonlinearity and slow down relaxation to the dark modes. In this study, we fabricated a pillar-shaped quartz resonator and then coated it with a thin layer of cobalt phthalocyanine (CoPc). By employing scattering-type scanning near-field optical microscopy (s-SNOM), we spatially investigated the dependency of vibrational strong coupling on the spatially varying electromagnetic field strength and demonstrated strong coupling with 38,000 molecules only–reaching to the small N limit. Through s-SNOM analysis, we found that strong coupling was observed primarily on the edge of the quartz pillar and the apex of the s-SNOM tip, where the maximum field enhancement occurs. In contrast, a weak resonance signal and lack of coupling were observed closer to the center of the pillar. This work demonstrates the importance of spatially resolved polariton systems in nanophotonic platforms and lays a foundation to explore polariton chemistry and chemical dynamics at the small N limit–one step closer to reconcile with high-level quantum calculations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2025

Dataset for: Rooftop solar and energy storage programs can remediate energy-limiting behaviors of energy insecure households

Energy insecurity affects most low-income households in the United States. Energy insecurity, which is characterized by a household’s inability to afford their energy needs, often leads to risky choices, causing other forms of insecurity including food and health. Although there are government programs designed to provide relief to low-income households that face energy insecurity, eligibility for these programs is usually determined by household income, and those with incomes close to the threshold face uncertainty or may be left out. In many cases, these households turn to energy-limiting behaviors as a strategy to lower their electric utility bills. This paper explores the relationship between energy insecurity and energy-limiting behaviors to investigate alternative solutions that target the households that may fall out of available energy assistance programs. We explore the role of battery energy storage systems and rooftop solar photovoltaics in improving energy affordability. The results show that residential rooftop solar and behind-the-meter energy storage can offset two-thirds of the bill savings that households attain through energy-limiting behavior. Household renewable energy systems could complement existing energy assistance programs to provide long-term bill relief, enabling occupants to live in their homes with comfort and dignity. This dataset is intended to allow readers to reproduce and customize the analysis performed in this work to their benefit.

Kerby, Jessica [Pacific Northwest National Laborat↗

DOE OSTI2025

Assessing the limitations of commercial sensors and models for supporting marine carbon dioxide removal monitoring: a case study

Several unknowns remain surrounding marine Carbon Dioxide Removal (mCDR) monitoring, reporting, and verification (MRV) practices and capabilities. Current in-situ sensor technology is limited (primarily pH and pCO 2 ), requiring calculations and assumptions to estimate changes in carbonate chemistry parameters, including total alkalinity (TA). Considering that cost, energy consumption, and accuracy of commercial sensors can vary by orders of magnitude, understanding how well existing sensors perform in an mCDR context is important for this emerging community. Likewise, documenting sensor limitations and how relatively simple models can optimize sensor deployments will improve MRV efforts and support protocol development. Here we (1) compare performance a variety of commercially available sensors in a blind mesocosm experiment simulating ocean alkalinity enhancement (OAE), and how sensor performance impacted carbonate chemistry estimates; (2) evaluate if sensors can distinguish the OAE signal from natural variability during a small scale OAE field test in Sequim Bay, WA, USA, and (3) use an idealized ocean biogeochemistry model to explore optimal sensor network design based on (1) and (2). Our mesocosm results indicate that correctly constraining pH uncertainty will be critical for accurate TA estimates with current sensor technology compared to the less impactful variation caused by uncertainty in pCO 2 (pH data that are presented throughout are reported on the total scale (pH T ) unless otherwise noted). Our pilot field test demonstrated that sensors were capable of distinguishing mCDR signatures from natural variability under optimal real-world conditions. Idealized modeling simulations of the field test showed that a range of sparse and dense (3 to 100) sensors sampling areas of detectable increases will underestimate the net change in surface pH by at least 35–55%, at both realistic and highly elevated alkalinity input levels. We also highlight the limitations of current sensing technology for MRV, and the importance of ocean biogeochemistry models as critical tools for predicting when and where mCDR signals will be detectable using available sensors. Overall, our findings suggest that commercially available pCO 2 sensors and some pH sensors will form an important backbone for mCDR MRV tasks, though complete MRV characterization will require these data to be used in combination with other tools.

OAE↗

DOE OSTI2026

Voltage Service Limits Smart Contract Using Distributed Ledger Technology for Electrical Utility Grid with Customer-Owned Generator

Modern electrical grids face growing stability risks from customer-owned generators, especially at points of common couplings (PCCs). Disruptive behavior from power-electronic sources can cause protective relays to isolate problematic generators, making measurement integrity critical. This article presents a distributed ledger technology (DLT) approach that uses smart contracts to evaluate PCC voltage measurements and trigger backup breaker operations. The approach is framed as a verifiable, multi-organization attestation and audit layer, not as a real-time control security mechanism. In the proposed architecture, voltage measurements from a hardware protective relay are anchored on a DLT through the Cyber Grid Guard (CGG) system for attestation by both the grid utility and customer-owned generator. A Voltage Service Limits (VSLs) smart contract evaluates the on-chain measurements against allowable phase-voltage limits derived from the ANSI C84.1 standard. The framework is validated in a hardware-relay-in-the-loop test bed under sustained-undervoltage, sustained-overvoltage, and transient line-to-line fault scenarios. The results show that the VSL smart contract can process these measurements and issue backup breaker actions consistent with the defined service-limit criteria, demonstrating the DLT potential as a verifiable audit layer at the PCC that complements primary protection.

cyber security↗

DOE OSTI2024

A Model for Pair Production Limit Cycles in Pulsar Magnetospheres

Abstract It was recently proposed that the electric field oscillation as a result of self-consistent e ± pair production may be the source of coherent radio emission from pulsars. Direct particle-in-cell simulations of this process have shown that the screening of the parallel electric field by this pair cascade manifests as a limit cycle, as the parallel electric field is recurrently induced when pairs produced in the cascade escape from the gap region. In this work, we develop a simplified time-dependent kinetic model of e ± pair cascades in pulsar magnetospheres that can reproduce the limit-cycle behavior of pair production and electric field screening. This model includes the effects of a magnetospheric current, the escape of e ± , as well as the dynamic dependence of pair production rate on the plasma density and energy. Using this simple theoretical model, we show that the power spectrum of electric field oscillations averaged over many limit cycles is compatible with the observed pulsar radio spectrum.

Astronomy & Astrophysics↗

NASA NTRS1968

Computer program determines exact two-sided tolerance limits for normal distributions

Computer program determines by numerical integration the exact statistical two-sided tolerance limits, when the proportion between the limits is at least a specified number. The program is limited to situations in which the underlying probability distribution for the population sampled is the normal distribution with unknown mean and variance.

Friedman, H. A.↗

NASA NTRS1969

Millivolt signal limiter

Low-voltage limiter circuit suppresses the output of platinum probes at temperatures beyond their operating range. The limiter circuit comprises an operational amplifier with a dual feedback loop. The signal limiter is useful in low-voltage instrumentation circuits normally operable or set for cryogenic temperatures.

Hansen, I. G.↗

NASA NTRS1970

Transistor current and voltage limiting switch

Limiting circuit protects the main power supply of electronic modules and limits the current drawn by each module should a short circuit occur. It limits current within one mA when used with direct current of either polarity, or with pulse or ac power sources from direct current to 100 kHz.

Hilbert, E. E.↗

NASA NTRS1972

Ground and flight test methods for determining limit cycle and structural resonance characteristics of aircraft stability augmentation systems

Performance criteria and test techniques are applied to stability augmentation systems (SAS) during ground testing to predict objectionable limit cycles and preclude structural resonance during flight. Factors that give rise to these problems, means of suppressing their effects, trade-offs to be considered, and ground test methods that have been developed are discussed. SAS performance predicted on the basis of these tests is compared with flight data obtained from three lifting body vehicles and the X-15 research airplane. Limit cycle and structural resonance test criteria, based upon ground and flight experience and data, were successfully applied to these vehicles. The criteria used were: The limit cycle amplitude (SAS gain multiplied by peak-to-peak angular rate) shall not exceed 0.5 deg for the highest product of control power and SAS gain that will be used in flight; the maximum in-flight SAS gain should never exceed 50 percent of the value at which a structural resonance can be sustained during ground test.

Painter, W. D.↗

NASA NTRS1972

Stably trapped proton limits for Jupiter

A general introduction to pitch-angle diffusion for Earth and Jupiter magnetospheres is given. The instabilities which might limit the trapped fluxes in the earth magnetosphere are identified as the interchange or ballooning mode, electrostatic loss cone modes, and electromagnetic ion cyclotron wave. The instability theory of the ion cyclotron wave is discussed. This wave can be unstable only if protons can be in cyclotron resonance with the wave. The instability growth rate is proportional to the cyclotron frequency, the fractional number density of fast particles, and the anisotropy of the fast particle distribution. The critical proton energy is the lowest energy for which the stably trapped limit applies, and is calculated to be 150 MeV at L = 2 and for 10 ion pairs/cu cm. Particles above the critical threshold energy are considered and their stability limit is approximately 3 x 10 to the 10th power/sq cm/sec divided by L to the 4th power.

Kennel, C.↗

NASA NTRS1972

Compression of transmission bandwidth requirements for a certain class of band-limited functions.

A study of source-encoding techniques that afford a reduction of data-transmission rates is made with particular emphasis on the compression of transmission bandwidth requirements of band-limited functions. The feasibility of bandwidth compression through analog signal rooting is investigated. It is found that the N-th roots of elements of a certain class of entire functions of exponential type possess contour integrals resembling Fourier transforms, the Cauchy principal values of which are compactly supported on an interval one N-th the size of that of the original function. Exploring this theoretical result, it is found that synthetic roots can be generated, which closely approximate the N-th roots of a certain class of band-limited signals and possess spectra that are essentially confined to a bandwidth one N-th that of the signal subjected to the rooting operation. A source-encoding algorithm based on this principle is developed that allows the compression of data-transmission requirements for a certain class of band-limited signals.

Smith, I. R.↗

NASA NTRS1972

Rocket ascent G-limited moment-balanced optimization program (RAGMOP)

This document describes the RAGMOP (Rocket Ascent G-limited Momentbalanced Optimization Program) computer program for parametric ascent trajectory optimization. RAGMOP computes optimum polynomial-form attitude control histories, launch azimuth, engine burn-time, and gross liftoff weight for space shuttle type vehicles using a search-accelerated, gradient projection parameter optimization technique. The trajectory model available in RAGMOP includes a rotating oblate earth model, the option of input wind tables, discrete and/or continuous throttling for the purposes of limiting the thrust acceleration and/or the maximum dynamic pressure, limitation of the structural load indicators (the product of dynamic pressure with angle-of-attack and sideslip angle), and a wide selection of intermediate and terminal equality constraints.

Lyons, J. T.↗

NASA NTRS1973

Mariner 9 ultraviolet spectrometer experiment - Upper limits on the Lyman-alpha flux from clusters of galaxies.

Data from the ultraviolet spectrometer on the Mariner 9 Mars orbiter have been used to set upper limits on the redshifted Lyman-alpha flux from the Perseus and Pegasus I (NGC 7619) clusters of galaxies. The limit for the Perseus cluster implies that the temperature of the intergalactic gas required for gravitational binding must be greater than 100,000 K, if it exists. A less severe limit is set for the Pegasus I cluster.

Bohlin, R. C.↗

NASA NTRS1974

Limiting performance of ground transportation vehicles subject to transient loading

A computational approach to determining the limiting performance of vehicles subject to transient disturbances based on response variable criteria is set forth. For the purposes of a limiting performance study, the transportation system dynamics are described using second- or first-order equations in which the sought for quantity is a vector of time-varying functions called control or isolator forces that have replaced portions of the physical system. Computations are performed as a linear programming problem. As an example of the limiting performance of vehicles in protecting passengers or cargo under crash conditions, the problem of lading damage of a rail vehicle that is struck by another vehicle is considered.

Pilkey, W. D.↗

NASA NTRS1974

Spontaneous ignition temperature limits of jet A fuel in research-combustor segment

The effects of inlet-air pressure and reference velocity on the spontaneous-ignition temperature limits of Jet A fuel were determined in a combustor segment with a primary-zone length of 0.076 m (3 in.). At a constant reference velocity of 21.4 m/sec (170 ft/sec), increasing the inlet-air pressure from 21 to 207 N/sq cm decreased the spontaneous-ignition temperature limit from approximately 700 to 555 K. At a constant inlet-air pressure of 41 N/sq cm, increasing the reference velocity from 12.2 to 30.5 m/sec increased the spontaneous-ignition temperature limit from approximately 575 to 800 K. Results are compared with other data in the literature.

Ingebo, R. D.↗

NASA NTRS1975

Aerospace technology development of three types of solid state remote power controllers for 120VDC with current ratings of five, and thirty amperes, one type having current limiting

The first generation of remote power controllers (RPC) developed included: a 5-ampere design (Type 1), capable of limiting maximum overload current to 15 amperes for .1 sec; and 5-ampere noncurrent (Type 2) and 30-ampere noncurrent (Type 3) limiting designs, both with selectable instant trip levels for high-current overload. Each design provides overcurrent protection through an inverse I squared T trip-out function with an automatic reset option and demonstrates step-applied fault capability with a 4000-ampere surge, fast-risetime (low-inductance) power source. They also meet MIL - STD - 461A specification for electromagnetic interference. The second generation RPCs traded off specification compliance for reduction in cost and complexity for the Type 1 and 2 designs and give comparable or improved performance in most areas. The noncurrent limiting RPC proved to be a more economical and feasible method of overload protection for certain load types.

Baker, D. E.↗

NASA NTRS1975

Flow field characteristics and performance limitations of quasi-steady magnetoplasmadynamic accelerators

Measurements of terminal voltage, exhaust velocity, current and potential distributions in a quasi-steady MPD arc operating over a range of currents from 3 to 25 kA countervene previous indications of basic limitations on MPD performance. Terminal voltage fluctuations, previously used as an indicator of a unique limiting value of the parameter current squared over mass flow, are shown to be related to cathode surface area rather than to interelectrode plasma phenomena. With improved electrodes and insulators, satisfactory arc operation at specific impulses somewhat beyond previously proposed limits has been demonstrated, and the significant thrust producing mechanisms in such arcs have been identified.

Boyle, M. J.↗

NASA NTRS1975

On the lower mass limit for the carbon detonation scenario

The lower mass limit for carbon detonation (about 4 solar masses) is due to an argument by Paczynski (1970) that stars in the range between 1.4 and 3.5 solar masses will lose their envelopes prior to carbon detonation. This argument is based on two criteria for mass loss: (1) the envelope is unstable to adiabatic oscillations, and (2) the total energy of the envelope is positive. Recent hydrodynamic calculations of red-giant envelopes have shown that the envelopes are highly nonadiabatic and that the second criterion is not a sufficient condition for mass loss. Thus, a calculation which takes into account the nonadiabatic nature of the envelope is required in order to determine the lower mass limit for carbon detonation. This lower mass limit is directly related to the formation mechanisms and statistics of supernovae and pulsars.

Endal, A. S.↗