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All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Proton decay spectroscopy of S 28 and Cl 30

States in 28 S and 30 Cl have been studied using one- and two-proton decay spectroscopy. In the first spectrometer setting, states in 28 S were populated following one-neutron knockout from a fast 29 S beam. Three new states are observed in 28 S from one- and two-proton decay. For the two-proton case the nature of the decay was investigated and found to proceed via sequential two-proton emission. For the second setting, states in 30 Cl were populated via one-proton knockout from a fast 31 Ar beam. The decay energy of the ground and first excited state were measured, with the ground-state decay energy found to be in disagreement with a previous measurement. Here, the spin and parity of these two 30 Cl states were inferred from shell-model calculations.

20 ≤ A ≤ 38↗
NASA NTRS1985

Instrumental background in balloon-borne gamma-ray spectrometers and techniques for its reduction

Instrumental background in balloon-borne gamma-ray spectrometers is presented. The calculations are based on newly available interaction cross sections and new analytic techniques, and are the most detailed and accurate published to date. Results compare well with measurements made in the 20 keV to 10 MeV energy range by the Goddard Low Energy Gamma-ray Spectrometer (LEGS). The principal components of the continuum background in spectrometers with GE detectors and thick active shields are: (1) elastic neutron scattering of atmospheric neutrons on the Ge nuclei; (2) aperture flux of atmospheric and cosmic gamma rays; (3) beta decays of unstable nuclides produced by nuclear interactions of atmospheric protons and neutrons with Ge nuclei; and (4) shield leakage of atmospheric gamma rays. The improved understanding of these components leads to several recommended techniques for reducing the background.

Gehrels, N.↗
NASA NTRS1987

Gamma-ray/neutron spectroscopy from the Mars observer

The Gamma-Ray Spectrometer (GRS) experiment on Mars Observer will measure gamma rays and neutrons that escape from Mars. The intensities of gamma-ray lines and of the thermal and epithermal neutrons can be used to study many problems related to Martian volcanism and volatiles. The results of theoretical calculations for the production and transport of gamma rays and neutrons indicate that the GRS should be able to determine the abundances of many elements and the amounts and stratigraphy of H2O and CO2 on and in the top meter of the Martian surface. Design considerations of the GRS are discussed.

Englert, P.↗
NASA NTRS2005

Lunar and Planetary Science XXXVI, Part 13

Contents include the following: A Fast, Non-Destructive Method for Classifying Ordinary Chondrite Falls Using Density and Magnetic Susceptibility. An Update on Results from the Magnetic Properties Experiments on the Mars Exploration Rovers, Spirit and Opportunity. Measurement Protocols for In Situ Analysis of Organic Compounds at Mars and Comets. Piping Structures on Earth and Possibly Mars: Astrobiological Implications. Uranium and Lead in the Early Planetary Core Formation: New Insights Given by High Pressure and Temperature Experiments. The Mast Cameras and Mars Descent Imager (MARDI) for the 2009 Mars Science Laboratory. MGS MOC: First Views of Mars at Sub-Meter Resolution from Orbit. Analysis of Candor Chasma Interior Layered Deposits from OMEGA/MEX Spectra. Analysis of Valley Networks on Valles Marineris Plateau Using HRSC/MEX Data. Solar Abundance of Elements from Neutron-Capture Cross Sections. Preliminary Evaluation of the Secondary Ion/Accelerator Mass Spectrometer, MegaSIMS. Equilibrium Landforms in the Dry Valleys of Antarctica: Implications for Landscape Evolution and Climate Change on Mars. Continued Study of Ba Isotopic Compositions of Presolar Silicon Carbide Grains from Supernovae. Paleoenviromental Evolution of the Holden-Uzboi Area. Stability of Magnesium Sulfate Minerals in Martian Environments. Tungsten Isotopic Constraints on the Formation and Evolution of Iron Meteorite Parent Bodies. Migration of Dust Particles and Volatiles Delivery to the Inner Planets. On the Sitting of Trapped Noble Gases in Insoluble Organic Matter of Primitive Meteorites. Trapping of Xenon Upon Evaporation-Condensation of Organic Matter Under UV Irradiation: Isotopic Fractionation and Electron Paramagnetic Resonance Analysis. Stability of Water on Mars. A Didactic Activity. Analysis of Coronae in the Parga Chasma Region, Venus. Photometric and Compositional Surface Properties of the Gusev Crater Region, Mars, as Derived from Multi-Angle, Multi-Spectral Investigation of Mars Express HRSC Data. Mapping Compositional Diversity on Mars: Spatial Distribution and Geological Implications. A New Simulation Chamber for Studying Planetary Environments. Folded Structure in Terra Sirenum. Mars. Nitrogen-Noble Gas Static Mass Spectrometry of Genesis Collector Materials. Neon Isotope Heterogeneity in the Terrestrial Mantle: Implication for the Acquisition of Volatile Elements in Terrestrial Planets. The Cosmic Clock, the Cycle of Terrestrial Mass Extinctions.

Source record↗
NASA NTRS1984

Method and apparatus for mapping the distribution of chemical elements in an extended medium

Contaminants in an extended medium such as the wall of a building are mapped by locating neutron excitation source on one side of the wall and a gamma ray spectrometer, including a gamma ray detector on the opposite side of the wall facing the excitation source. The source and detector are moved in unison in discrete steps over opposing wall surfaces so as to determine the chemical composition of the elements in a hemispheric region of the wall adjacent the detector with the radius of the region being substantially that of the mean free path distance of gamma rays emitted from elements interacting with neutrons on the detector side of the wall. The source and detector are reversed for relatively thick walls for mapping the distribution of elements on the other side of the wall thickness. The output of the detector is fed to a multichannel pulse height analyzer where the intensity of the various gamma ray spectral lines are indicated relative to a dominant constituent element such as silicon. Resolution of anomalies such as the presence of voids and/or determining the bulk density of the medium is achieved by substituting a gamma ray source technique is also applied to metal alloys, such as iron alloys, in either the solid or molten state.

Evans, L. G.↗
DOE OSTI2026

Spectral Flux Measurements on SNS Direct Geometry Spectrometers at IRP-2 End-of-Life

The Inner Reflector Plug (IRP) of the Spallation Neutron Source (SNS) was replaced during the SNS shutdown period beginning 25 November 2025. This IRP, IRP-2, was first placed in service in May 2018, and was in use for 42.5 GW-hrs of operation, somewhat longer than its original design life of 30 GW-hrs, or even a refined estimate of 33 GW-hrs for the water moderator poison plate and 39 GW-hrs on the decoupled-poisoned hydrogen moderator decoupler (Gallmeier, Lu, and Iverson 2018). The time-integrated power history for IRP-2 is tracked in Figure 1.

43 PARTICLE ACCELERATORS↗
NASA NTRS1999

Martian Radiation Environment Experiment (MARIE)

Space radiation presents a very serious hazard to crews of interplanetary human missions. The two sources of this radiation are the galactic cosmic rays (GCR) and solar energetic particle (SEP) events. The GCR provides a steady source of low dose rate radiation that is primarily responsible for stochastic effects, such as cancer, and can effect the response of the central nervous system. Nuclear interactions of these components with the Martian atmosphere produces substantial flux of neutrons with high Radio Biological Effectiveness. The uncertainty in the knowledge of many fragmentation cross sections and their energy dependence required by radiation transport codes, uncertainties in the ambient radiation environment, and knowledge of the Martian atmosphere, lead to large enough uncertainties in the knowledge of calculated radiation dose in both free space (cruise phase), in Martian orbit, and on Martian surface. Direct measurements of radiation levels, the relative contributions of protons, neutrons, and heavy ions, and Martian atmospheric characteristics is thus a prerequisite for any human mission. An integrated suite of two spectrometers to provide these data will be described. The Orbiter spectrometer will measure the energy spectrum of SEP events from 15 to 500 MeV/n, and when combined with data from other space based instruments, such as the Advanced Composition Explorer (ACE), would provide accurate GCR spectra also. The Lander spectrometer would measure the absorbed dose rate, dose equivalent dose rate, and the linear energy transfer (LET) spectra and is capable of separating the relative contribution of these quantities from protons, neutrons, and high Z particles. There are two separate flight instruments, one for the Orbiter and one for the Lander, based on a common design of the backplane, the central processing unit (CPU), power supply, and onboard data storage. The Orbiter instrument consists of an energetic particle spectrometer that can measure the elemental energy spectra of charged particles over energy range of 15-500 MeV/n. The spectrometer will be mounted on the science deck and has an angular acceptance of 50 degrees. As the spacecraft orbits Mars, the axis of this field of view sweeps a cone of directions on the sky. During each orbit, the angle between the axis of the spectrometer's field of view and the mean interplanetary field direction varies from 90 degrees to 180 degrees. The Lander instrument is designed: (1) to measure the accumulated absorbed dose and dose rate in tissue as a function of time, (2) to determine the radiation quality factor, (3) to determine the energy deposition spectrum from 0.1 keV/micron to 1500 keV/micron, and (4) to separate the contribution of protons, neutrons, and HZE particles to these quantities.

Badhwar, Gautam D.↗
NASA NTRS1992

Gamma-rays and neutrons as a probe of the proton spectrum during the solar flare of 1988 December 16

We have previously reported on high-energy gamma-rays and neutrons from the flare of 1988 December 16 detected by the Gamma-Ray Spectrometer on the SMM satellite. In this paper, we present results on gamma-ray lines seen by the same detector during this flare. Together, these measurements constitute a powerful probe of the proton spectrum that produces the flare neutrals. Analysis of the data suggests a Bessel-function proton spectrum with a shape parameter (alpha T) of 0.054 +/- 0.004 and the number of protons above 30 MeV equal to (9.0 +/- 0.9) x 10 exp 32. The number of neutrons detected from this flare is much smaller than what is predicted from an isotropic distribution of the protons, indicating that the distribution may be nonisotropic.

Dunphy, P. P.↗
DOE OSTI2025

Polarizing 3 He via metastability exchange optical pumping using a 1.2 mbar sealed cell at magnetic fields up to 5 T

Here, we report high nuclear polarization of 1.2 mbar 3 He gas in a sealed cell in magnetic fields up to 5 T using Metastability Exchange Optical Pumping (MEOP). The creation of a highly polarized 3 He gas target for use in the 5 T field of Jefferson Lab’s CLAS12 spectrometer would enable new studies of spin-dependent asymmetries on the neutron. We describe a systematic study which was conducted for the first time up to the full 5 T field required for the final target design to evaluate the effects of discharge intensity, pump laser power, and optical pumping transition schemes on nuclear polarization and pumping rates. Steady-state polarizations up to 86% in magnetic fields between 2 and 5 T were achieved, with a discharge-on relaxation time of 898 s at 5 T. These results underscore the potential of MEOP for high-field applications in nuclear physics experiments.

3He polarization↗
DOE OSTI2026

𝑁 = 8 Shell Breaking in 12 Be from a Single-Particle Perspective

Experimental observations of the low-lying states in 12 Be and their accurate modeling play an essential role in understanding the disappearance of the 𝑁 = 8 magic number. Long-standing experimental ambiguities have been clarified using an one-neutron adding (𝑑, 𝑝) reaction on 11 Be using the ISOLDE Solenoidal Spectrometer at CERN’s HIE-ISOLDE facility. The single-particle energies of 1⁢𝑠 1/2 , 0⁢𝑑 5/2 , and 0⁢𝑝 1/2 orbitals in 12 Be have been determined from the extracted spectroscopic factors. A significant reduction between the separation of 1⁢𝑠 1/2 and 0⁢𝑝 1/2 orbitals is found in comparison with the carbon isotones, highlighting the breakdown of the 𝑁 = 8 shell. These observations serve as an important test of different effects incorporated in theoretical models. It is found that two synergistic mechanisms, core deformation and weak binding, are responsible for the 𝑁 = 8 shell breaking and the exotic near-threshold phenomena observed in 12 Be, including the narrow unnatural-parity resonance $0^{-}_1$ and the possible halolike nature of the $0^+_2$ isomer.

Chen, Jie [Southern University of Science and Tech↗
DOE OSTI2022

Thermal expansion and phonon anharmonicity of cuprite studied by inelastic neutron scattering and ab initio calculations

Inelastic neutron scattering measurements were performed with a time-of-flight chopper spectrometer to observe phonons in all parts of the Brillouin zone of a single crystal of cuprite Cu 2 O. We reduced the experimental data to phonon dispersions in the high-symmetry directions, and changes between 10 and 300 K are reported. In this paper, we show ab initio quasiharmonic (QH) and anharmonic (AH) calculations of phonon dispersions. We performed all AH calculations with a temperature-dependent effective potential method. Both QH and AH calculations account for the small negative thermal expansion of cuprite at low temperatures. However, the measured temperature-dependent phonon behavior was predicted more accurately with the AH calculations than the QH ones. Nevertheless, at 300 K, the cubic AH used in this paper did not entirely account for the experimental phonon dispersions in cuprite.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Potential neutron-induced γ-ray background on natural tellurium relevant to 130 Te 0 ν ββ decay searches at the CUORE and SNO+ detectors

Gamma-ray production cross-section data have been obtained for the inelastic neutron scattering reactions 126,128,130 Te(n,n'γ) at five neutron energies between 3.6 and 10 MeV. We report data for the γ-ray energy region relevant to 0ν ββ decay of 130 Te with a Q ββ value of 2527.515 keV, assuming natural-abundance tellurium, as used at CUORE and SNO+. The natural abundance of 130 Te, 128 Te, and 126 Te is 34%, 32%, and 19%, respectively. For CUORE the γ-ray cascades from the excited state in 130 Te at 2527.06 keV and in 126 Te at 2533.85 keV are of concern. For SNO+, accounting for its inferior energy resolution, an additional four levels are important in 130 Te, an additional nine levels in 128 Te, and an additional eight levels in 126 Te. Of these, we report neutron-induced γ-ray production cross sections for the strongest transitions: the 2581.15 keV level in 130 Te, the 2494.20, 2508.06, and 2630.14 keV levels in 128 Te, and the 2496.83 and 2585.46 keV level in 126 Te. Here, the largest cross-section values were found for cascade γ-ray transitions to the ground state, while direct transitions to the ground state are very weak and were not observed in the present work. Both the CUORE and SNO+ detectors, however, may not be able to distinguish between cascade transitions and direct transitions to the ground state, making the neutron-induced excitation of the 2527.06 keV state of 130 Te in particular a potential problem for 0νββ decay searches of 130Te, because it matches its Q ββ value.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Demonstration of sub-micron UCN position resolution using room-temperature CMOS sensor

High spatial resolution of ultracold neutron (UCN) measurement is of growing interest to UCN experiments such as UCN spectrometers, UCN polarimeters, quantum physics of UCNs, and quantum gravity. Here we utilize physics informed deep learning to enhance the experimental position resolution and to demonstrate sub-micron spatial resolutions for UCN position measurements obtained using a room-temperature CMOS sensor, extending our previous work that demonstrated a position uncertainty of 1.5 microns. We explore the use of the open-source software Allpix Squared to generate experiment-like synthetic hit images with ground-truth position labels. We use physics-informed deep learning by training a fully connected neural network (FCNN) to learn a mapping from input hit images to output hit position. The automated analysis for sub-micron position resolution in UCN detection combined with the fast data rates of current and next generation UCN sources will enable improved precision for future UCN research and applications.

10B nanometer thin film↗
DOE OSTI2022

Modulation of intensity emerging from zero effort (MIEZE) with extended Fourier time at large scattering angle

Modulation of Intensity Emerging from Zero Effort (MIEZE) is a neutron resonant spin echo technique that allows one to measure time correlation scattering functions in materials by implementing radio-frequency (RF) intensity modulation at the sample and the detector. The technique avoids neutron spin manipulation between the sample and the detector and, thus, could find applications in cases where the sample depolarizes the neutron beam. However, the finite sample size creates a variance in the path length between the locations where scattering and detection happen, which limits the contrast in intensity modulation that one can detect, in particular, toward long correlation times or large scattering angles. We propose a modification to the MIEZE setup that will enable one to extend those detection limits to longer times and larger angles. Furthermore, we use Monte Carlo simulations of a neutron scattering beamline to show that by tilting the RF flippers in the primary spectrometer with respect to the beam direction, one can shape the wave front of the intensity modulation at the sample to compensate for the path variance from the sample and the detector. The simulation results indicate that this change enables one to operate a MIEZE instrument at much increased RF frequencies, thus improving the effective energy resolution of the technique. For the MIEZE instrument simulated, it shows that for an incident beam with the maximum divergence of 0.33°, the maximum Fourier time can be increased by a factor of 3.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Self-diffusion of liquid deuterium hydride and liquid tritium

Here, we present a quasi-elastic neutron scattering study of liquid deuterium hydride carried out using the Disk Chopper Spectrometer at the National Institute of Standards and Technology. Under saturated vapor pressure, the self-diffusion constant of deuterium hydride obeys an Arrhenius law D = D 0 exp(-E A /k B T), where the prefactor D 0 is given by D 0 = 9.5 ± 1.2 Å 2 /ps and the activation energy is given by E A = 58 ± 2 K. We apply the quantum law of corresponding states to the known diffusion constants of the hydrogen isotopologues. From this application, we estimate that D 0 ≈ 9.1 Å 2 /ps and E A ≈ 75 K in liquid tritium. Young’s theory of quantum-mechanical effects in van der Waals fluids is shown to apply to the diffusion constants of the liquid hydrogens. Our results underscore the importance of nuclear quantum effects in shaping the properties and behavior of the hydrogen isotopologues.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS2013

Mesosiderites on Vesta: A Hyperspectral VIS-NIR Investigation

The discussion about the mesosiderite origin is an open issue since several years. Mesosiderites are mixtures of silicate mineral fragments or clasts, embedded in a FeNi metal matrix. Silicates are very similar in mineralogy and texture to howardites [1]. This led some scientists to conclude that mesosiderites could come from the same parent parent asteroid of the howardite, eucrite and diogenite (HED) meteorites [2, 3]. Other studies found a number of differences between HEDs and mesosiderite silicates that could be explained only by separate parent asteroids [4]. Recently, high precision oxygen isotope measurements of m esosiderites silicate fraction were found to be isotopically identical to the HEDs, requiring common parent body, i.e. 4 Vesta [5]. Another important element in favor of a common origin was given by the identification of a centimeter-sized mesosiderite clast in a howardite (Dar al Gani 779): a metal-rich inclusion with fragments of olivine, anorthite, and orthopyroxene plus minor amounts of chromite, tridymite, and troilite [6]. The Dawn mission with its instruments, the Infrared Mapping Spectrometer (VIR) [7], the Framing Camera [8] and the Gamma-Ray and Neutron Detector (GRaND) [9] confirmed that Vesta has a composition fully compatible with HED meteorites [10]. We investigate here the possibility to discern mesosiderite rich locations on the surface of Vesta by means of hyperspectral IR images.

Palomba, E.↗
NASA NTRS1982

A high-resolution measurement of the 2.223 MeV neutron capture line in a solar flare

An intense solar flare lasting 40 s was observed by the HEAO 3 gamma-ray spectrometer on November 9, 1979, at 3:05 UT. The flare was observed in four high-resolution germanium detectors as well as in five CsI shield detectors over an energy range of 100 keV to above 5 MeV. Of particular interest is a line feature at 2.2248 + or - 0.0010 MeV. The precise energy measurement provides unambiguous evidence that this is the (H-1)(n, gamma)(H-2) line resulting from neutron capture on hydrogen. An upper limit of 5 keV is found for the natural line width. The time dependence of the neutron capture line is discussed as well as the overall characteristics of the November 9 flare.

Prince, T. A.↗
DOE OSTI2021

Mass measurements of neutron-rich indium isotopes for r -process studies

A new series of neutron-rich indium mass measurements is reported from the TITAN multiple-reflection time-of-flight mass spectrometer (MR-TOF-MS). These mass measurements cover 125-134 In (N = 76–85) and include ground states as well as isomeric states. The masses of nuclei in this region are known to be of great importance for accurately modeling r-process nucleosynthesis, and the significance of the reported neutron-rich indium masses is discussed in this context. Results are compared with earlier experimental data where available as well as theoretical mass models. The measurements reported here include the first mass measurements of 133,134 In, as well as the first direct mass measurement of 132 In. The masses of 125-131 In ground states and several isomers were previously measured to higher precision by Penning trap mass spectrometry, which also resolved some low-lying isomers that could not be resolved in this work. The earlier Penning trap measurements serve as excellent cross-checks for the MR-TOF-MS measurements, and in some cases the MR-TOF-MS measurements improve the literature uncertainties of higher-lying isomer masses and excitation energies. Finally, a new isomeric state for 128 In, recently reported for the first time by the JYFLTRAP group, is also confirmed by the TITAN MR-TOF-MS, with a measured excitation energy of 1813(17) keV.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗