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At least 325 records · Page 18

Excitation functions of proton-induced nuclear reactions on $$^{86}$$Sr, with particular emphasis on the formation of isomeric states in $$^{86}$$Y and $$^{85}$$Y

Abstract Cross sections of proton-induced nuclear reactions on enriched $$^{\mathrm {86}}$$ 86 Sr target were measured by the activation technique up to proton energies of 44 MeV. The isomeric cross-section ratios for $$^{\mathrm {86m,g}}$$ 86 m , g Y and $$^{\mathrm {85m,g}}$$ 85 m , g Y as a function of projectile energy were deduced from their measured data. The present experimental data for the nuclear reaction products, namely $$^{\mathrm {86m}}$$ 86 m Y, $$^{\mathrm {86g+xm}}$$ 86 g + xm Y, $$^{\mathrm {85m}}$$ 85 m Y, $$^{\mathrm {85g}}$$ 85 g Y, $$^{\mathrm {84}}$$ 84 Rb and $$^{\mathrm {83}}$$ 83 Rb were compared with the results of nuclear model calculations using the code TALYS, which combines the statistical, precompound, and direct interactions. In general, the experimental cross-section data as well as the isomeric cross-section ratios are reproduced well by the model calculations, provided the input model parameters are properly chosen and the level structure of the product nucleus is thoughtfully considered. The quality of the agreement between experimental data and model calculations was numerically quantified. For products formed via emission of a light complex particle as well as multi-nucleons (e.g., $$\alpha $$ α and 2p2n), the contribution of the latter process starts increasing when its energy threshold is crossed.

Uddin, M. S.↗

First study of neutrino angle reconstruction using quasielasticlike interactions in MicroBooNE

We investigate the expected precision of the reconstructed neutrino direction using a 𝜈 𝜇 -argon quasielasticlike event topology with one muon and one proton in the final state and the reconstruction capabilities of the MicroBooNE liquid argon time projection chamber. This direction is of importance in the context of DUNE sub-GeV atmospheric oscillation studies. MicroBooNE allows for a data-driven quantification of this resolution by investigating the deviation of the reconstructed muon-proton system orientation with respect to the well-known direction of neutrinos originating from the Booster Neutrino Beam with an exposure of 1.3 ×10 21 protons on target. Using simulation studies, we derive the expected sub-GeV DUNE atmospheric-neutrino reconstructed simulated spectrum by developing a reweighting scheme as a function of the true neutrino energy. We further report flux-integrated single- and double-differential cross section measurements of charged-current 𝜈 𝜇 quasielasticlike scattering on argon as a function of the muon-proton system angle using the full MicroBooNE data sets. We also demonstrate the sensitivity of these results to nuclear effects and final state hadronic reinteraction modeling.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Measurement of proton electromagnetic form factors in the time-like region using initial state radiation at BESIII

The electromagnetic process e + e - → $p\bar{p}$ is studied with the initial-state-radiation technique using 7.5 fb -1 of data collected by the BESIII experiment at seven energy points from 3.773 to 4.600 GeV. The Born cross section and the effective form factor of the proton are measured from the production threshold to 3.0 GeV/c 2 using the $p\bar{p}$ invariant-mass spectrum. The ratio of electric and magnetic form factors of the proton is determined from the analysis of the proton-helicity angular distribution.

79 ASTRONOMY AND ASTROPHYSICS↗

Nuclear structure and elastic scattering observables obtained consistently with different N N interactions

Nucleon-nucleon ($NN$) interactions based on chiral effective theories are commonly used in ab initio calculations of light nuclei. Here we present a study based on three different $NN$ interactions (up to next-to-next-to-leading order) for which structure and elastic proton scattering observables are consistently calculated for $^4$He, $^{12}$C, and $^{16}$O. The interactions are compared at the two-body level in terms of Wolfenstein amplitudes, and their predictions for ground state energies, point-proton radii, and charge form factors, as well as proton elastic scattering observables in the leading-order spectator expansion in the energy range between 65 and 160 MeV projectile energy are presented. Finally, to gain further insight into differences visible in elastic scattering observables, we investigate the behavior of the calculated effective nucleon-nucleus interactions for the $^{12}$C nucleus based on the different $NN$ interactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A New Family of Proton‐Conducting Electrolytes for Reversible Solid Oxide Cells: BaHf x Ce 0.8− x Y 0.1 Yb 0.1 O 3− δ

Abstract Reversible solid oxide cells based on ceramic proton conductors have potential to be the most efficient system for large‐scale energy storage. The performance and long‐term durability of these systems, however, are often limited by the ionic conductivity or stability of the proton‐conducting electrolyte. Here new family of solid oxide electrolytes, BaHf x Ce 0.8− x Y 0.1 Yb 0.1 O 3− δ (BHCYYb), which demonstrate a superior ionic conductivity to stability trade‐off than the state‐of‐the‐art proton conductors, BaZr x Ce 0.8− x Y 0.1 Yb 0.1 O 3− δ (BZCYYb), at similar Zr/Hf concentrations, as confirmed by thermogravimetric analysis, Raman, and X‐ray diffraction analysis of samples over 500 h of testing are reported. The increase in performance is revealed through thermodynamic arguments and first‐principle calculations. In addition, lab scale full cells are fabricated, demonstrating high peak power densities of 1.1, 1.4, and 1.6 W cm −2 at 600, 650, and 700 °C, respectively. Round‐trip efficiencies for steam electrolysis at 1 A cm −2 are 78%, 72%, and 62% at 700, 650, and 600 °C, respectively. Finally, CO 2 H 2 O electrolysis is carried out for over 700 h with no degradation.

Murphy, Ryan↗

Search for a resonance decaying into a scalar particle and a Higgs boson in the final state with two bottom quarks and two photons in proton–proton collisions at $\sqrt{s}$ = 13 TeV with the ATLAS detector

A search for the resonant production of a heavy scalar X decaying into a Higgs boson and a new lighter scalar S, through the process X → S(→ $b\overline{b}$)H(→γγ), where the two photons are consistent with the Higgs boson decay, is performed. The search is conducted using an integrated luminosity of 140 fb -1 of proton-proton collision data at a centre-of-mass energy of 13 TeV recorded with the ATLAS detector at the Large Hadron Collider. The search is performed over the mass range 170 ≤ m X ≤ 1000 GeV and 15 ≤ m S ≤ 500 GeV. Parameterised neural networks are used to enhance the signal purity and to achieve continuous sensitivity in a domain of the (m X , m S ) plane. No significant excess above the expected background is found and 95% CL upper limits are set on the cross section times branching ratio, ranging from 39 fb to 0.09 fb. The largest deviation from the background-only expectation occurs for (m X , m S ) = (575, 200) GeV with a local (global) significance of 3.5 (2.0) standard deviations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for flavor changing neutral current interactions of the top quark in final states with a photon and additional jets in proton-proton collisions at s = 13 TeV

A search for the production of a top quark in association with a photon and additional jets via flavor changing neutral current interactions is presented. The analysis uses proton-proton collision data recorded by the CMS detector at a center-of-mass energy of 13 TeV, corresponding to an integrated luminosity of 138 fb - 1 . The search is performed by looking for processes where a single top quark is produced in association with a photon, or a pair of top quarks where one of the top quarks decays into a photon and an up or charm quark. Events with an electron or a muon, a photon, one or more jets, and missing transverse momentum are selected. Multivariate analysis techniques are used to discriminate signal and standard model background processes. No significant deviation is observed over the predicted background. Observed (expected) upper limits are set on the branching fractions of top quark decays: B ( t → u γ ) < 0.95 × 10 - 5 ( 1.20 × 10 - 5 ) and B ( t → c γ ) < 1.51 × 10 - 5 ( 1.54 × 10 - 5 ) at 95% confidence level, assuming a single nonzero coupling at a time. The obtained limit for B ( t → u γ ) is similar to the current best limit, while the limit for B ( t → c γ ) is significantly tighter than previous results.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for production of four top quarks in final states with same-sign or multiple leptons in proton–proton collisions at $\sqrt{s}=13$ ${TeV}$

The standard model (SM) production of four top quarks ($\text {t} {}{\overline{\text {t}}} \text {t} {}{\overline{\text {t}}} $) in proton–proton collisions is studied by the CMS Collaboration. The data sample, collected during the 2016–2018 data taking of the LHC, corresponds to an integrated luminosity of 137$\,\text {fb}^{-1}$ at a center-of-mass energy of 13$\,\text {TeV}$. The events are required to contain two same-sign charged leptons (electrons or muons) or at least three leptons, and jets. The observed and expected significances for the $\text {t} {}{\overline{\text {t}}} \text {t} {}{\overline{\text {t}}} $ signal are respectively 2.6 and 2.7 standard deviations, and the $\text {t} {}{\overline{\text {t}}} \text {t} {}{\overline{\text {t}}} $ cross section is measured to be $12.6^{+5.8}_{-5.2}\,\text {fb} $. The results are used to constrain the Yukawa coupling of the top quark to the Higgs boson, $y_{\text {t}}$, yielding a limit of $|y_{\text {t}}/y_{\text {t}}^{\mathrm {SM}} | < 1.7$ at $95\%$ confidence level, where $y_{\text {t}}^{\mathrm {SM}}$ is the SM value of $y_{\text {t}}$. They are also used to constrain the oblique parameter of the Higgs boson in an effective field theory framework, $\hat{H}<0.12$. Limits are set on the production of a heavy scalar or pseudoscalar boson in Type-II two-Higgs-doublet and simplified dark matter models, with exclusion limits reaching 350–470$\,\text {GeV}$ and 350–550$\,\text {GeV}$ for scalar and pseudoscalar bosons, respectively. Upper bounds are also set on couplings of the top quark to new light particles.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Level Structure of {sup 31}S Via {sup 32}S({ital p,d}) {sup 31}S

Background: Properties of proton-unbound S-31 states determine the P-30(p, gamma) S-31 reaction rate, which has a significant impact on explosive hydrogen burning in classical novae and type-I x-ray bursts. Despite several previous studies, uncertainties still remain with respect to the nuclear structure of S-31 near the proton threshold. Purpose: The level structure of S-31 has been presently investigated via a charged-particle spectroscopy experiment using the S-32(p, d) S-31 reaction. Method: Deuterons corresponding to S-31 excited states with 3.285 <= E-x <= 10.8 MeV were momentum analyzed via an Enge split-pole spectrograph at six laboratory angles between 10 degrees and 62 degrees. Differential cross sections of the S-32(p, d)S-31 reaction were measured at E-p = 34.5 MeV. Distorted-wave Born approximation calculations were performed to constrain the spin-parity assignments of several of the observed levels. Results: We have detected 72 excited states of S-31, out of which 17 are within the astrophysical region of interest corresponding to the temperature range of 0.1-1.5 GK. We have resolved the discrepancy in the spin and parity of an excited state with E-x = 6542 keV, showing that is it not J(pi) = 3/2(-), and therefore the contribution of this state to the P-30(p, gamma) reaction rate is likely much less significant than previously thought owing to the larger angular-momentum transfer required to populate this excited state. Moreover, our measurement results help consolidate the spin-parity assignments for the 6377 and 6636 keV states in S-31. Conclusions: This work presents the most comprehensive spin-parity assignments to date from a single-neutron transfer reaction on S-32 to S-31 excited states in the region between 6 to 7 MeV excitation energy. This region is significant for the determination of the P-30(p, gamma)S-30 reaction rate over the temperatures characteristic of explosive hydrogen burning in novae.

Setoodehnia, K.↗

Measurement of the Ground State Spin and Parity of 22 Al Disfavors Halo Formation

We report the decisive resolution of the ground state spin and parity of the proton–drip line nucleus 22 Al, a prime candidate for a proton halo. The resolution stems from the first 𝛽-delayed charged particle emission experiment in the gas stopping area at the Facility for Rare Isotope Beams (FRIB), leveraging high-intensity, low-energy beams extracted from the Advanced Cryogenic Gas Stopper (ACGS). The pristine beam quality from FRIB and the ACGS enabled a sensitive particle identification technique using thin silicon detectors, allowing for the suppression of the dominant proton background and the first observation of the weak 𝛽-delayed 𝛼 transition from the isobaric analog state in 22 Mg to the 18 Ne ground state. This observation uniquely fixes the 22 Al ground state as 4 + . The valence proton is confined by a dominant 𝑑-wave centrifugal barrier which, combined with the Coulomb repulsion, hinders the tunneling required for halo formation despite the exceptionally low proton separation energy of 22 Al.

20 ≤ A ≤ 38↗

Improved Solid-State Reaction Method for Scaled-Up Synthesis of Ceramic Proton-Conducting Electrolyte Materials

Protonic ceramic electrochemical cells (PCECs) represent promising technologies in the production of clean electricity, decarbonized hydrogen, chemicals, and fuels at intermediate temperatures. One of the challenges in commercializing PCECs is to produce the electrolyte materials on a large scale. The conventional solid-state reaction (SSR) method suffers from tedious synthesis procedures and low phase purity of the products due to the formation of unwanted secondary phases. Herein, we report an improved SSR (i-SSR) method for kilogram-scale production of high phase-purity electrolyte material BaZr 0.4 Ce 0.4 Y 0.1 Yb 0.1 O 3–δ (BZCYYb4411). In this method, the ball-milled precursor powders are pelletized prior to calcination, which effectively reduces the length of the diffusion paths between the components during perovskite phase formation. In this study, the synthesis procedure and calcination temperature are carefully optimized for efficient and repeatable production based on the powder crystallization behavior. A combined technoeconomic analysis and life cycle assessment modeling suggest that the i-SSR method could reduce the total production cost and greenhouse gas emissions by up to 19% and 39%, respectively, compared to the conventional SSR method. The high quality of the synthesized electrolyte material is corroborated by the excellent electrical conductivity and electrochemical performance of the fabricated PCEC cells.

36 MATERIALS SCIENCE↗

Search for R-parity-violating supersymmetry in a final state containing leptons and many jets with the ATLAS experiment using $\sqrt{s}=13\hbox{TeV}$ proton–proton collision data

A search for R-parity-violating supersymmetry in final states characterized by high jet multiplicity, at least one isolated light lepton and either zero or at least three b-tagged jets is presented. The search uses 139fb –1 of $\sqrt{s}=13\hbox{TeV}$ proton–proton collision data collected by the ATLAS experiment during Run 2 of the Large Hadron Collider. The results are interpreted in the context of R-parity-violating supersymmetry models that feature gluino production, top-squark production, or electroweakino production. The dominant sources of background are estimated using a data-driven model, based on observables at medium jet multiplicity, to predict the b-tagged jet multiplicity distribution at the higher jet multiplicities used in the search. Machine-learning techniques are used to reach sensitivity to electroweakino production, extending the data-driven background estimation to the shape of the machine-learning discriminant. No significant excess over the Standard Model expectation is observed and exclusion limits at the 95% confidence level are extracted, reaching as high as 2.4 TeV in gluino mass, 1.35 TeV in top-squark mass, and 320 (365) GeV in higgsino (wino) mass.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Demonstration of cooling by the Muon Ionization Cooling Experiment

The use of accelerated beams of electrons, protons or ions has furthered the development of nearly every scientific discipline. However, high-energy muon beams of equivalent quality have not yet been delivered. Muon beams can be created through the decay of pions produced by the interaction of a proton beam with a target. Such ‘tertiary’ beams have much lower brightness than those created by accelerating electrons, protons or ions. High-brightness muon beams comparable to those produced by state-of-the-art electron, proton and ion accelerators could facilitate the study of lepton–antilepton collisions at extremely high energies and provide well characterized neutrino beams. Such muon beams could be realized using ionization cooling, which has been proposed to increase muon-beam brightness. Here we report the realization of ionization cooling, which was confirmed by the observation of an increased number of low-amplitude muons after passage of the muon beam through an absorber, as well as an increase in the corresponding phase-space density. The simulated performance of the ionization cooling system is consistent with the measured data, validating designs of the ionization cooling channel in which the cooling process is repeated to produce a substantial cooling effect. The results presented here are an important step towards achieving the muon-beam quality required to search for phenomena at energy scales beyond the reach of the Large Hadron Collider at a facility of equivalent or reduced footprint.

43 PARTICLE ACCELERATORS↗

Structural insights into functional properties of the oxidized form of cytochrome c oxidase

Abstract Cytochrome c oxidase (C c O) is an essential enzyme in mitochondrial and bacterial respiration. It catalyzes the four-electron reduction of molecular oxygen to water and harnesses the chemical energy to translocate four protons across biological membranes. The turnover of the C c O reaction involves an oxidative phase, in which the reduced enzyme (R) is oxidized to the metastable O H state, and a reductive phase, in which O H is reduced back to the R state. During each phase, two protons are translocated across the membrane. However, if O H is allowed to relax to the resting oxidized state (O), a redox equivalent to O H , its subsequent reduction to R is incapable of driving proton translocation. Here, with resonance Raman spectroscopy and serial femtosecond X-ray crystallography (SFX), we show that the heme a 3 iron and Cu B in the active site of the O state, like those in the O H state, are coordinated by a hydroxide ion and a water molecule, respectively. However, Y244, critical for the oxygen reduction chemistry, is in the neutral protonated form, which distinguishes O from O H , where Y244 is in the deprotonated tyrosinate form. These structural characteristics of O provide insights into the proton translocation mechanism of C c O.

36 MATERIALS SCIENCE↗

Measurement of cross sections for mesonless charged-current muon neutrino interactions on argon with and without protons at MicroBooNE

urrent and upcoming neutrino experiments at Fermilab will rely on liquid argon time projection chambers (LArTPCs) as the primary detector technology. To reach the ambitious precision required for their physics goals, a detailed understanding of neutrino-argon scattering must be achieved. For the present Short-Baseline Neutrino program, the dominant reaction channel is charged-current muon neutrino interactions leading to mesonless final states with and without protons. Using a large data set of neutrino interactions recorded by the MicroBooNE LArTPC detector at Fermilab, we report progress towards new measurements of differential cross sections in this channel. The analysis leverages multiple event reconstruction paradigms and observables specifically chosen to maximize sensitivity to nuclear effects of interest for improving neutrino scattering models. Related previous cross-section results from MicroBooNE and a preview of what to expect from the new analysis will both be featured in this presentation.

Liu, Liang [Fermilab]↗

The impact of second coordination sphere functional group extension on product selectivity for manganese bipyridyl CO 2 reduction electrocatalysts

Utilizing the well established manganese bipyridyl class of homogeneous electrocatalyst, four new ligands are studied to probe the influence of distal, outer coordination sphere, H-bonding and steric effects on product selectivity for proton-coupled electrocatalytic CO 2 reduction. The presence of a simple acetate functional group in the second coordination sphere provides a high selectivy for CO 2 -to-CO conversion irrespective of proton source (H 2 O vs. PhOH) or applied potential. The o-(methoxybenzoate)phenyl second/outer coordination sphere at the bipyridyl 6,6′-positions imparts poor product selectivity. In contrast, upon conjugation of the acetate functional group with the N-Boc-alanine moiety, a CO : HCO 2 − product selectivity of ∼1 : 1 is observed at the high overpotential catalytic wave (for both H 2 O and PhOH acids). Computed enthalpy and free energy of activation parameters suggest that selective CO 2 insertion at the manganese hydride transition state is favored, over protonation, consistent with negligible hydrogen production during controlled potential electrolysis studies.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Charmonium production in $p$Ne collisions at $\sqrt{s_{\scriptscriptstyle \text {NN}}} =68.5$ GeV

The measurement of charmonium states produced in proton-neon (pNe) collisions by the LHCb experiment in its fixed-target configuration is presented. The pro duction of J/ψ and ψ(2S) mesons is studied with a beam of 2.5 TeV protons colliding on gaseous neon targets at rest, corresponding to a nucleon-nucleon centre-of-mass energy $\sqrt{s_{NN}}$ = 68.5 GeV. The data sample corresponds to an integrated luminosity of 21.7 ± 1.4 nb -1 . The J/ψ and ψ(2S) hadrons are reconstructed in μ + μ - final states. The J/ψ production cross-section per target nucleon in the centre-of mass rapidity range y* ϵ [-2.29, 0] is found to be 506 ± 8 ± 46 nb/nucleon. The ratio of J/ψ and D 0 cross-sections is evaluated to (1.06 ± 0.02 ± 0.09)%. The ψ(2S) to J/ψ relative production rate is found to be (1.67 ± 0.27 ± 0.10)% in good agreement with other measurements involving beam and target nuclei of similar sizes.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗