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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 325 records · Page 18

A proposed high-intensity radiometer calibration method using concentrated solar radiation

Accurate calibration of irradiance measurement devices, or radiometers, is essential for ensuring the reliability of measurements in high heat applications such as concentrating solar power (CSP), aerospace, defense, and pulsed power systems. Despite the critical need, existing calibration standards and service providers are limited to irradiance levels below 100 kW/m 2 and specific radiation sources, which is insufficient for many applications. For instance, CSP technologies, particularly those under the Department of Energy’s Solar Energy Technologies Office (SETO) Gen 3 program, require accurate measurements of broadband irradiance at levels exceeding 2000 kW/m 2 . In even more extreme scenarios, such as re-entry vehicles, heat levels can surpass 10000 kW/m 2 . Current ISO standards, specifically ISO 14934–2 and ISO 14934–3, are constrained to lower irradiance levels and dependent on black body heat sources, limiting their applicability for high-intensity broadband irradiance measurements, particularly in concentrated solar applications. Here, to address this shortfall, the National Solar Thermal Test Facility (NSTTF) at Sandia National Laboratories (SNL) proposes a calibration method and facility capable of characterizing radiometers up to 2750 kW/m 2 using concentrated solar irradiance. Calibrating with concentrated sunlight is important for solar applications as it aligns the calibration process with the solar spectrum. This alignment is crucial for minimizing systematic errors and avoiding the need for additional corrections that may arise when radiometers designed for solar applications are calibrated using black-body or electrical sources. This paper presents the present day NSTTF characterization facility and procedure, detailing the proposed calibration method and uncertainty quantification. The presented method builds upon 1980′s NSTTF methodology and involves both theoretical and empirical methods to establish a robust relationship between gauge voltage output and irradiance intensity, quantifying both measurement and fitting errors. By addressing the limitations of existing standards and extending the characterization range, this work provides an advancement in the field of high-intensity irradiance measurement and instrumentation characterization.

Gardon gauge↗

Enhancements to the New TREAT Automatic Reactor Control System (ARCS)

The Transient Reactor Test (TREAT) facility recently replaced the automatic reactor control system (ARCS). Here, this paper discusses some of the enhancements that were made during the ARCS replacement such as calculations to take into account the nonadiabatic effects and increasing the dynamic range for power and period indication. This paper also discusses upgrades that had been planned but were unable to implemented and potential upgrades for the future.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Accelerated radiation tolerance testing of Ti-based MAX phases

MAX phases have recently attracted significant attention for potential nuclear applications due to their novel properties such as unique hexagonal-compact nanolayered crystal structure, high-machinability due to lower hardness levels compared to conventional ceramics, and high-chemical inertness. In order for MAX phases to be used in nuclear reactors, two aspects deserve detailed investigations: (i) their phase stability at high-temperatures and (ii) microstructural defect formation and recovery induced by energetic particle irradiation. To date, degradation mechanisms of MAX phases at high-temperatures and following irradiation are largely unexplored fields of research. This work focuses on the evaluation of two Ti-based MAX phases – Ti 2 AlC and Ti 3 SiC 2 – within the context of extreme environments. To accomplish this, a one-of-a-kind comparison between neutron irradiations, performed over a decade of research at the High Flux Isotope Reactor (HFIR), and heavy-ion irradiations, carried out in situ in a Transmission Electron Microscope (TEM) at the MIAMI-2 facility, has been conducted. The results show Ti-based MAX phases are prone to accelerated decomposition under the conditions investigated. This questions the hypothesis that MAX phases exhibit high phase stability, especially when used in future nuclear energy systems where energetic particle irradiation is a dominating degradation mechanism.

36 MATERIALS SCIENCE↗

FRIB Beam Power Ramp-up: Status and Plans

After project completion on scope, on cost, and ahead of schedule, the Facility for Rare Isotope Beams began operations for scientific users in May of 2022. The ramp-up to a beam power of 400 kW is planned over a six-year period; 1 kW was delivered for initial user runs from in 2022, and 5 kW was delivered as of February 2023. Test runs with 10 kW 36Ar and 48Ca beams were conducted in July 2023. Upgrade plans include doubling the primary-beam energy to 400 MeV/nucleon for enhanced discovery potential (¿FRIB 400¿). This talk reports on the strategic plans towards high power operations emphasizing challenges and resolutions in beam-interception devices and targetry systems, radiation protection and controls, and legacy system renovation and integration.

43 PARTICLE ACCELERATORS↗

Fast Neutron Irradiation of a Multichannel JFET-Based Optical Encoder

Modern electrical components are susceptible to damage from high levels of radiation and extreme temperatures found near reactors in terrestrial nuclear power plants and in aerospace applications. Radiation-hardened electronics are being developed, largely for the aerospace industry, but they sometimes rely on application-specific, small-batch semiconductor fabrication processes. These processes tend to be prohibitively expensive to develop and maintain outside major industrial facilities or governmental agencies. Recently, commercially available, nonradiation-rated junction-gate field-effect transistors (JFETs) were shown to maintain their functionality at gamma doses exceeding 1 MGy, suggesting that nonrated, commercially available electrical components could be used to develop systems that are tolerant to ionizing radiation. However, gamma ray survival is not indicative of neutron dose survival, and few studies characterize JFETs under neutron irradiation. To address this knowledge gap, a JFET-based analog multiplexer and optical pulsewidth modulation (PWM) encoder was developed and irradiated using a 252 Cf source to 1.6×10 13 n/cm 2 . The multiplexed optical encoder (MOE) system maintained functionality throughout testing and showed little evidence of radiation effects. These results indicate that circuitry tolerant to fast neutron damage can be developed using low-cost, nonradiation-rated, commercially available JFETs, which could provide a lower production cost alternative to specialized semiconductor processes when designing and building electronics better able to survive neutron irradiation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

RaDIATE Collaboration for Material Studies

In the recent past, major accelerator facilities have been limited in beam power not by their accelerators, but by the beam intercepting device survivability. As next-generation accelerator target facilities (High Energy Physics, Spallation Sources, …) become increasingly more powerful and intense, high power target systems face key technical challenges. Beam-intercepting devices such as beam windows and secondary particle-production targets are continuously bombarded by high-energy high-intensity pulsed proton beams to produce secondary particles. Energy deposition from the primary beam induces near instantaneous heating (thermal shock) and microstructural changes (radiation damage) in the beam-intercepting materials. Both thermal shock and radiation damage ultimately degrade the performance and lifetime of targets and have been identified as the leading cross-cutting challenges of high-power target facilities. In order to operate reliable beam-intercepting devices in the framework of energy and intensity increase for next generation accelerators, the RaDIATE collaboration (Radiation Damage In Accelerator Target Environment) managed by Fermilab, brings together existing expertise in nuclear material and accelerator targets from 20 international institutions to execute a coordinated strategy for high power targetry R&D. This collaboration is generating new and useful materials data for application within the accelerator and the fission/fusion communities. I will give an overview of the RaDIATE R&D program and the achievement in the last few years on material studies in support of High Power Targetry development, including results obtained from irradiation test, development of novel materials and the prospective towards future irradiation campaign. A highlight will be given to the results in collaboration with our colleagues from J-PARC.

Pellemoine, Frederique↗

Analysis of Air-Purifying Respirator (APR) and Powered Air-Purifying Respirator (PAPR) Cartridge Performance Testing on Hanford Tanks BY-108 and BY-110 Volume 2: Raw Analytical Data

As the Tank Operations Contractor for U.S. Department of Energy operations at the Hanford site in Washington State, Washington River Protection Solutions (WRPS) is responsible for managing highly radioactive wastes stored in tanks at Hanford. WRPS tests air-purifying respirator (APR) and powered air-purifying respirator (PAPR) chemical cartridges commonly used by workers at Hanford Tank Farms to determine the period of time that the cartridges would provide adequate performance for APRs and PAPRs used to protect workers when exposed to a mixture of Chemicals of Potential Concern (COPC) from any vapors exiting headspaces in the storage tanks. The Occupational Safety and Health Administration (OSHA) Standard promulgated in Title 29 of the Code of the Federal Regulations (CFR) 1910.134(d)(3)(iii)(b)(2) specifies that for protection against gases and vapors, employers shall implement a schedule for cartridges to ensure that change-outs occur before the end of service life. The change schedule can be based on objective information or data that ensures cartridge change-outs occur before the end of their service life. The primary function of the WRPS Cartridge Test Program is to obtain objective data to determine service lives for the APR and PAPR cartridges used at Hanford Tank Farms. WRPS contracted with Pacific Northwest National Laboratory to analyze the test data and offer an independent analysis and any recommendations. This report summarizes data analysis of APR and PAPR cartridge testing on BY-110 and BY-108 headspace vapors, respectively. Two different APR cartridges from SCOTT Safety (Monroe, North Carolina) were assessed for the BY-110 headspace vapors, and two different PAPR cartridges—one from MSA Safety Inc. (Pittsburgh, Pennsylvania) and another from 3M (Maplewood, Minnesota)—were assessed for the BY-108 headspace vapors. Volume 1 of this report documents the testing, data analysis, results, conclusions, and recommendations resulting from the cartridge testing of vapors from the BY-110 and BY-108 headspaces. Volume 2 provides an introduction to the raw data, including analytical laboratory analysis results that supported the analysis and conclusions documented in Volume 1.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Modernizing the Legacy Fission Wire Measurement System for the Advanced Test Reactor-Critical Facility

Operational lifetime extensions of existing research reactors have emphasized the need for refurbishment, replacements, and upgrades to supporting equipment and instrumentation. The Advanced Test Reactor (ATR) at Idaho National Laboratory (INL), which entered service in 1967, has recently completed the sixth core internals change-out and has scheduled operations until at least 2040. Reactor maintenance and operational risk management is critically important in the research reactor community, however supporting measurement systems sometimes get overlooked when maintenance is planned. The Fission Wire Measurement System (FWMS) is a custom measurement system designed in the 1960s to measure the beta-particle activity of irradiated uranium-aluminum fission wires. This measurement is conducted to determine the fission rate profile of the Advanced Reactor Test Critical (ATR-C) facility. The ATR-C is an open-pool, low-power test reactor that was purpose driven to resemble ATR and is used to qualify experiment configurations and verify core models prior to full-power experiment irradiations in ATR. A power distribution measurement in ATR-C uses uranium-aluminum wires that are distributed throughout the ATR-C core to validate simulation and modeling results. These measurements require 340 to 1500 wires to be irradiated and measured within a 12-hour window. The activity of the wires is measured in the required time with the FWMS, which was put into service in 1965 at the Radiation Measurements Laboratory (RML). The system consists of 4 measurement channels and one reference channel, each with a 2-pi proportional gas flow detector and the measurement channels each have an automated sample changer. This legacy system is crucial to the continued operations of ATR and has undergone some minor hardware upgrades since 1965, however the system presently relies on custom control boards, custom gas ion chambers, analog amplifiers/discriminators, and a user interface (UI) for the system written in outdated code. Much of the equipment and software is custom with no commercial replacements or support and limited documentation. The existing control software requires an operating system that is no longer supported, creating more vulnerabilities to continued operations. A project is underway with a third-party vendor to design, build, and document a new control and data acquisition system (CDAS) for the FWMS. The new upgrade will replace the control system, computer, UI, sample changer motors, and main power supply while maintaining the interface with existing detector hardware. The upgraded system will be operated in parallel with the current hardware and software to conduct validation testing. This equipment upgrade demonstrates the commitment at ATR to ensuring successful operations and potential future research reactors at INL.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

Selection of Components for the Remote, Canister-Monitoring System

This report documents the selection of components as part of the efforts initiated to develop a remote, canister-monitoring system (RCMS) for determining and monitoring environmental conditions within dry fuel storage canisters containing aluminum clad spent nuclear fuel (ASNF) at the Idaho National Laboratory (INL). These efforts are in support of Department of Energy Office of Environmental Management (DOE-EM) investigations into technical issues associated with extended dry storage (50+ years) of ASNF. The capability to establish and monitor the performance of ASNF in situ provides the opportunity to (1) evaluate the appropriate technologies for monitoring, (2) collect canister environment conditions as soon as possible, (3) verify and validate current laboratory-based study results and analytic modeling approaches, and (4) potentially identify additional dry storage options for ASNF at the INL site. The improved understanding of ASNF behavior gained by performing this work would also contribute to the safety basis for extended dry storage in current and future configurations as well as to provide information for future transportation, conditioning, and disposal of ASNF. The parameters to be monitored by the RCMS include temperature, relative humidity, hydrogen gas concentration and radiation environment (dose). Components are selected based on the expected environmental conditions within the canister and fuel storage area, and the desired performance of the RCMS. Several of these components have been purchased and received. Future activities include component testing and calibration, software development for operation of the integrated sensor module and fabrication of a representative test volume. The results of these tests and changes to desired performance characteristics will inform subsequent activities.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Mercury Modeling of TREAT Big-BUSTER Free Field Characterization Experiments

This report summarizes modeling of Big-BUSTER free field characterization (FFC) experiments at the Idaho National Laboratory (INL) Transient Reactor Test Facility (TREAT) reactor performed from December 20th, 2023, to February 22nd, 2024. TREAT is an air-cooled graphite moderated research reactor that can be used to study material response to neutron irradiation. The BUSTER (Broad Use Specimen Transient Experiment Rig) refers to a containment module for placing experiments in the reactor core. The Big-BUSTER is an analogous platform for a modified core configuration with a larger experimental cavity.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Towards a Unified Setup to Simulate Mid‐Latitude and Tropical Mesoscale Convective Systems at Kilometer‐Scales

Abstract Mesoscale convective systems (MCSs) are the main source of precipitation in the tropics and parts of the mid‐latitudes and are responsible for high‐impact weather worldwide. Studies showed that deficiencies in simulating mid‐latitude MCSs in state‐of‐the‐art climate models can be alleviated by kilometer‐scale models. However, whether these models can also improve tropical MCSs and whether we can find model settings that perform well in both regions is understudied. We take advantage of high‐quality MCS observations collected over the Atmospheric Radiation Measurement (ARM) facilities in the US Southern Great Plains (SGP) and the Amazon basin near Manaus (MAO) to evaluate a perturbed physics ensemble of simulated MCSs with 4 km horizontal grid spacing. A new model evaluation method is developed that enables to distinguish biases stemming from spatiotemporal displacements of MCSs from biases in their reflectivity and cloud shield. Amazon MCSs are similarly well simulated across these evaluation metrics than SGP MCSs despite the challenges anticipated from weaker large‐scale forcing in the tropics. Generally, SGP MCSs are more sensitive to the choice of model microphysics, while Amazon cases are more sensitive to the planetary boundary layer (PBL) scheme. Although our tested model physics combinations had strengths and weaknesses, combinations that performed well for SGP simulations result in worse results in the Amazon basin and vice versa. However, we identified model settings that perform well at both locations, which include the Thompson and Morrison microphysics coupled with the Yonsei University (YSU) PBL scheme and the Thompson scheme coupled with the Mellor‐Yamada‐Janjic PBL scheme.

54 ENVIRONMENTAL SCIENCES↗

Brine Availability Test in Salt, a Heated Borehole Experiment at the Waste Isolation Pilot Plant, New Mexico, USA - 20233

The Brine Availability Tests in Salt is a US Department of Energy Office of Nuclear Energy supported activity as part of the Spent Fuel and Waste Disposition Campaign where we are performing simultaneous heated and control experiments in adjacent horizontal boreholes in the WIPP Salt Disposal Investigation drifts as part of experimental Phase 1. Phase 1a of BATS, a low-cost, small spatial-scale experiment performed in order to design instrumentation and methods for further experimentation in the URL, has been completed (June 2018 - May 2019) and is described elsewhere. In coincidence with multiple physical parameters that will be measured over the duration of the experiment, we will be measuring the liquid and vapor phases of H{sub 2}O as well as its isotopic content (not measured in Phase 1a). Three different forms of water occur in natural salts: as fluid in macro scale (mm size) inclusions, as intergranular free H{sub 2}O and as H{sub 2}O incorporated in hydrous minerals. Each of these forms has potentially different stable isotope signatures and will be influenced differentially by heat induced transport and by interaction with introduced tracers. Continuous measurement of vapor phase H{sub 2}O isotopes during borehole heating will be impacted by several effects: 1) evaporation as liquid brine flows into the borehole and evaporates completely or partially into the dry N{sub 2} stream; 2) steam from dehydration of hydrous minerals, that may enter the borehole; and 3) hydrous minerals that may form in the borehole (preferentially incorporating heavier isotopes). The continuous time series collected over the course of the heating test will be combined with analyses of pre-test and post-test collected samples of test site salt to investigate the contributions of each of the three water types as H{sub 2}O is mobilized due to the effects of heating. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Assessing the Impact of Effective Thermal Conductivity on Gas-cooled Reactor Transients in RELAP5-3D

High-temperature gas-cooled reactors (HTGRs) are a relatively mature advanced reactor concept that are of interest to industry and government for near-term deployment. These systems feature passive safety through low power density, coated particle fuels, and large graphite volumes that lead to slow heatup. In loss of flow transients, cooldown is achieved through conduction and radiation heat transfer. In prismatic block-type reactors, such as the mHTGR-350, the presence of coolant holes and fuel compacts alters the flow of heat through the blocks. To capture this effect in systems codes like RELAP5-3D, relationships for effective thermal conductivity (ETC) must be used to appropriately degrade the thermal conductivity. This work presents an assessment of the impact of ETC on performance of block-type gas-cooled reactors in a pressurized conduction cooldown (PCC) and depressurized conduction cooldown (DCC) transients. Models for PCC and DCC with bulk material thermal conductivity and ETC were run for both the mHTGR-350 and the High-Temperature Test Facility (HTTF) to determine the impact of ETC on transient performance.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Characterization of radiation damage effects in high-energy neutrino target graphite using low-energy ions

Exposure of graphite targets to high intensity proton beams at neutrino production facilities causes changes in the target material that can result in a shortened operation lifetime. The dominant factors in this process are currently thought to be mechanical in nature resulting primarily from microstructural effects that lead to thermal and structural changes in bulk material properties. As currently planned beam facilities with increased proton energy and intensity begin to come online it will be important to thoroughly understand these processes, and ideally to be able to predict the effects of new beam designs on target properties. Direct analysis of targets exposed to existing high-energy proton beams is complicated by several factors, such as very limited access to proton beam facilities, high associated costs, irradiation times on the order of months, and the resulting radioactivity of irradiated samples that requires special facilities for post-irradiation examination. Much of the existing literature concerning irradiation damage in graphite has been focused on the needs of the nuclear engineering community, however high-energy proton targets operate in a much different environment. In comparison to graphite irradiated in a nuclear reactor, graphite used in proton beam targets receives a higher dose rate, have greater gas production, and experience short irradiation pulses as opposed to continuous irradiation. Low-energy ion irradiation offers a method of inducing similar levels of radiation damage to high-energy protons while avoiding many of the difficulties and limitations associated with high-energy proton beams and the corresponding activated specimen testing. My research described in this thesis focused on investigating how low-energy ion irradiation could be used to induce the same or similar types of microstructural alteration and mechanical property degradation as that seen in high-energy neutrino production target graphites by varying damage le vels and irradiation temperatures prior to post-irradiation characterisation.

43 PARTICLE ACCELERATORS↗

Final Design for Thermal/Epithermal eXperiments (TEX) with Lithium Absorbers to Provide Validation Benchmarks for Y-12 Electrorefining Facility (IER 575, CED-2 Report)

One of the main goals of the Thermal/Epithermal eXperiments (TEX) project is to use existing Nuclear Criticality Safety Program (NCSP) assets to create critical experiment plutonium and uranium test beds for materials important to criticality safety that have insufficient benchmark evaluations. The plutonium test bed experiments were completed in 2018 and are published in the 2020 edition of the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook. The uranium test bed assemblies were completed in 2023 and accepted in the 2024 edition of the ICSBEP Handbook.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Measurement of correlated charge noise in superconducting qubits at an underground facility

The charge environment of superconducting qubits may be studied through the introduction of controlled, quantified amounts of ionizing radiation. We measure space- and time-correlated charge jumps on a four-qubit device, operating 107 meters below the Earth’s surface in a low-radiation, cryogenic facility designed for the characterization of low-threshold particle detectors. The rock overburden of this facility reduces the cosmic ray muon flux by over 99% compared to laboratories at sea level. Combined with 4π coverage of a movable lead shield, this facility enables quantifiable control over the flux of ionizing radiation on the qubit device. Long-time-series charge tomography measurements on these weakly charge-sensitive qubits capture discontinuous jumps in the induced charge on the qubit islands, corresponding to the interaction of ionizing radiation with the qubit substrate. The rate of these charge jumps scales with the flux of ionizing radiation on the qubit package, as characterized by a series of independent measurements on another energy-resolving detector operating simultaneously in the same cryostat with the qubits. Using lead shielding, we achieve a minimum charge jump rate of $0.19^{+0.04}_{-0.03}$ mHz, almost an order of magnitude lower than that measured in surface tests, but a factor of roughly seven higher than expected based on reduction of ambient gammas alone. We operate four qubits for over 22 consecutive hours with zero correlated charge jumps at length scales above three millimeters.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

OVERVIEW OF RECENT PU-238 PRODUCTION ACTIVITIES AT IDAHO NATIONAL LABORATORY

The Plutonium Fuel Services (PFS) program at Idaho National Laboratory (INL) is active in the qualification of irradiation targets containing Np-237 for irradiation in the Advanced Test Reactor (ATR) to produce Pu-238 for future NASA missions. INL qualified and loaded 7 targets in ATR’s South Flux Trap (SFT) for cycle 169A, which occurred in Spring 2021. This program was reinitiated after two baseline production targets in three positions validated significant production of Pu-238 [ref.1]. The validation model was followed by the PFS-1 experimental test in the ATRC (Critical) facility [ref.2]. This paper outlines the progress and status of the PFS program. The qualification effort, safety analysis, hardware status, and future activities for qualification of an updated target design for use in the ATR will be discussed.

36 MATERIALS SCIENCE↗

DARHT Axis 1 Bremsstrahlung Dose Measurements

he Dual-Axis Radiographic Hydrodynamic Test (DARHT) facility provides flash radiography ca pabilities using two electron Linear Induction Accelerators (LIA’s). Axis-1 of DARHT produces, nominally, a 20-MeV, 1.5-kA, 80-ns-Full Width at Half Max (FWHM) electron beam. The elec tron beam is focused on to a tantalum target to produce a Bremsstrahlung x-ray dose for flash radiography of dynamic systems. This paper will describe and compare a variety of techniques for determining the x-ray dose for two different beam currents produced by a 55mm and 70mm diameter cathode. The data was taken in November of 2022 on DARHT Axis 1. The experimen tal measurement techniques include a platinum calorimeter, a diamond radiation detector (DRD), and a Compton diode (CD). Gafchromic EBT3 self-developing dosimetry film was also used, but no useful results were obtained. Beam charge and energy were recorded and dose was calculated with this information using xtr with Dosecalcx, and simple dose charge-energy scaling. In this pa per, we will discuss the target geometry and experimental layout, the methods of measuring dose, dose diagnostics and measurement of beam charge and energy, and the comparisons of data and calculations.

43 PARTICLE ACCELERATORS↗