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At least 325 records · Page 18

Response of an interactive two-dimensional model to ozone changes - An estimate of the radiative dynamical feedback effect

The response of the interactive two-dimensional stratospheric model described by Schneider et al. (1989) to an increased chemical removal of ozone and the sensitivity of the calculated assessments to the choice of eddy diffusion coefficients are investigated using a simplified ozone chemistry model. It was found that the radiative dynamical feedback in the model leads to ozone losses at high altitudes to be about one third smaller than predicted by a model with fixed temperature and circulation. The radiative feedback has a smaller effect on ozone (losses decrease by about one sixth) in the lower stratosphere. Predicted ozone losses increase with decreasing dissipation and eddy diffusion in the lower stratosphere.

Schneider, Hans R.↗

A new reeling technique for very long extension scanning in the stratosphere

A balloon-borne winching system has been developed for extending a very long tether with payload down into the stratosphere and recovering it, this has been flight proven by being carrried to an altitude of 40 km, lowering a 62-kg stratospheric photochemistry experiment 12 km at a descent velocity of about 6-8 m/sec and recovering it at comparable velocities. During the first flight, the data gave no evidence of dynamic instabilities due to the system or the stratospheric interactions. The future utility of this payload is discussed with attention to the design factors that bound the range of performance of this type of system.

Hazen, N. L.↗

Variability in the Speed of the Brewer-Dobson Circulation as Observed by Aura/MLS

We use Aura/MLS stratospheric water vapour (H2O) measurements as tracer for dynamics and infer interannual variations in the speed of the Brewer-Dobson circulation (BDC) from 2004 to 2011. We correlate one-year time series of H2O in the lower stratosphere at two subsequent pressure levels (68 hPa, approx.18.8 km and 56 hPa, approx 19.9 km at the Equator) and determine the time lag for best correlation. The same calculation is made on the horizontal on the 100 hPa (approx 16.6 km) level by correlating the H2O time series at the Equator with the ones at 40 N and 40 S. From these lag coefficients we derive the vertical and horizontal speeds of the BDC in the tropics and extra-tropics, respectively. We observe a clear interannual variability of the vertical and horizontal branch. The variability reflects signatures of the Quasi Biennial Oscillation (QBO). Our measurements confirm the QBO meridional circulation anomalies and show that the speed variations in the two branches of the BDC are out of phase and fairly well anti-correlated. Maximum ascent rates are found during the QBO easterly phase. We also find that transport of H2O towards the Northern Hemisphere (NH) is on the average two times faster than to the Southern Hemisphere (SH) with a mean speed of 1.15m/s at 100 hPa. Furthermore, the speed towards the NH shows much more interannual variability with an amplitude of about 21% whilst the speed towards the SH varies by only 10 %. An amplitude of 21% is also observed in the variability of the ascent rate at the Equator which is on the average 0.2mm/s.

Brewer-Dobson circulation↗

Natural and anthropogenic perturbations of the stratospheric ozone layer

The paper reviews potential causes for reduction in the ozone abundance. The response of stratospheric ozone to solar activity is discussed. Ozone changes are simulated in relation with the potential development of a fleet of high-speed stratospheric aircraft and the release in the atmosphere of chlorofluorocarbons. The calculations are performed by a two-dimensional chemical-radiative-dynamical model. The importance of heterogeneous chemistry in polar stratospheric clouds and in the Junge layer (sulfate aerosol) is emphasized. The recently reported ozone trend over the last decade is shown to have been largely caused by the simultaneous effects of increasing concentrations of chlorofluorocarbons and heterogeneous chemistry. The possibility for a reduction in stratospheric ozone following a large volcanic eruption such as that of Mount Pinatubo in 1991 is discussed.

Brasseur, Guy P.↗

Transient medium-scale wave activity in the summer stratosphere

Observations of medium-scale transient wave activity in the middle-latitude Southern Hemisphere summer stratosphere are interpreted using isentropic potential vorticity (IPV) distributions inferred from temperature data from the Nimbus-7 Limb Infrared Monitor of the Stratosphere (LIMS) instrument. Despite problems with errors in reference-level synoptic height information, the derived IPV distributions clearly exhibit dynamically coherent signatures of eddy mixing due to medium-scale disturbances in the lower-middle stratosphere during early January 1979. The IPV distributions are shown to be strongly correlated with those of a contemporaneous set of isentropic maps of quasi-conservative tracers such as ozone and nitric acid. The results suggest that IPV maps inferred from satellite temperature data provide a useful diagnostic for studies of large-scale dynamics and/or transport in the extratropical stratosphere. Furthermore, the comparatively high vertical resolution of the LIMS data has enabled the vertical attenuation of Southern Hemisphere wave activity to be diagnosed in greater detail than could be achieved from nadir-viewing satellite information.

Miles, T.↗

Planetary wave-mean flow interaction in the stratosphere: A comparison between the Northern and Southern Hemispheres

Based on satellite-derived data supplied by the National Meteorological Center (NMC), the dynamical interaction between planetary waves and mean zonal winds in the stratosphere is investigated. Special attention is paid to the differences between the Northern Hemisphere (NH) and the Southern Hemisphere (SH). An analysis is made using Eliassen-Palm (E-P) flux diagnostics for the period from June 1981 to May 1982. In a climatological sense, different seasonal evolutions of large-scale motions between the NH and the SH in the stratosphere are demonstrated. Vertical cross-section analysis is presented to show the day-to-day variation in the mean zonal wind and wave activity, in particular, the following phenomena: (1) the poleward shifting of the westerly jet, and (2) episodes after the shifting of the westerly jet.

Shiotani, M.↗

Evolution of microwave limb sounder ozone and the polar vortex during winter

The evolution of polar ozone observed by the Upper Atmosphere Research Satellite (UARS) Microwave Limb Sounder (MLS) is described for the northern hemisphere (NH) winters of 1991/1992, 1992/1993, and 1993/1994 and the southern hemisphere (SH) winters of 1992 and 1993. Imterannual and interhemispheric variability in polar ozone evolution are closely related to differences in the polar vortex and to the frequency, duration and strength of stratospheric sudden warmings. Ozone in the midstratospheric vortices increases during the winter, with largest increases associated with stratospheric warmings and a much larger increase in the NH than in the SH. A smaller NH increase was observed in 1993/1994, when the middle stratospheric vortex was stronger. During strong stratospheric warmings in the NH, the upper stratospheric vortex may be so much eroded that it presents little barrier to poleward transport; in contrast, the SH vortex remains strong throughout the stratosphere during wintertime warmings, and ozone increases only below the mixing ratio peak, due to enhanced diabatic descent. Ozone mixing ratios decrease rapidly in the lower stratosphere in both SH late winters, as expected from chemical destruction due to enhanced reactive chlorine. The interplay between dynamics and chemistry is more complex in the NH lower stratosphere and interannual variability is greater. Evidence has previously been shown for chemical ozone destruction in the 1991/1992 and 1992/1993 winters. We show here evidence suggesting some chemical destruction in late February and early March 1994. In the NH late winter lower stratosphere the pattern of high-ozone values (typical of the vortex) seen in mid-latitudes is related to the strength of the lower-stratospheric vortex, with the largest areal extent of high ozone outside the vortex in 1994, when the lower stratospheric vortex is relatively weak, and the least extent in 1993 when the lower stratospheric vortex is strongest.

Manney, G. L.↗

Analysis of the effects of zonal averaging on reaction rate calculations in two-dimensional atmospheric models

The usual assumption by which chemical reaction rates are calculated in two-dimensional atmospheric models is by using a product of zonal means of rate coefficients and constituent concentrations rather than the rigorous zonal mean of the corresponding products. This assumption has been tested for the reactions O + NO2 yields NO + O2 and NO + O3 yields NO2 + O2 using mapped limb infrared monitor of the stratosphere data from the Nimbus 7 satellite and found to be quite satisfactory for winter 1979 at 60 deg N in the upper stratosphere. Relative differences between the two-dimensional averaged rate and the more rigorous rate, calculated from the full, longitudinally varying temperatures and mixing ratios, were small (usually below 5 percent) and exceeded 15 percent only during times of strong dynamical activity. At those times or locations where stratospheric circulation is primarily zonal, the two averages agreed to within a few percent.

Kaye, Jack A.↗

Faster Tropical Upper Stratospheric Upwelling is Driving Changes in Ozone Chemistry

Trends in N2O and the chlorofluorocarbons (CFCs) cause trends in O3 through changes in their reactive product gases, NOx and ClOx, but transport plays an important role because it controls the distribution of the long‐lived source gases that produce ozone‐destroying radicals. In this study we show that increased tropical upwelling 10‐5 hPa from 2013‐2021 has changed upper stratospheric (UpS) composition and shifted the balance of O3 loss processes. We use N2O, HNO3, NOx, temperature and O3 data from the Aura Microwave Limb Sounder (MLS) and the SCI‐Sat Atmospheric Chemistry Experiment Fourier Transport Spectrometer (ACE‐FTS) over a 16‐year period to show how changes in reactive nitrogen species affected gas phase ozone chemistry above 30 hPa between June 2013‐May 2021 compared to the previous 8 years, June 2005‐May 2013. We use 2 simulations of the Global Modeling Initiative (GMI) chemistry transport model (CTM), with and without time varying MERRA2 meteorology, to understand how dynamical changes during this 16‐yr period affected O3 through changes in loss via the NOx and ClOx cycles. We also identify the role that the quasi‐biennial oscillation (QBO) in tropical zonal winds plays in the UpS composition changes. We find large increases in tropical upwelling and poleward transport in the northern branch of the UpS transport circulation since 2013 that dramatically increased the abundance of the N2O and its odd nitrogen product gases, NOx and HNO3. O3 loss by NOx in the Arctic UpS increased due to dynamically driven composition change, explaining the observed weak O3 recovery in that region since 2005. The increased upwelling also drove decreases in tropical NOx, leading to increased tropical O3 from 12‐6 hPa.

middle atmosphere chemistry and composition↗

First results from the Nimbus 7 total ozone mapping spectrometer

The Total Ozone Mapping Spectrometer (TOMS) instrument was launched on the Nimbus 7 satellite in October 1978. This instrument is designed to measure spatial variations in the total ozone field. The employed technique is an extension of the Backscattered Ultraviolet (BUV) total ozone method. The TOMS instrument has an improved capability for detailed monitoring of total ozone. The obtained data appear to contain information about dynamical processes in the upper troposphere and the lower stratosphere. Investigations are being conducted to determine qualitatively the conditions, if any, where total ozone fails as a predictor for tropopause height. Quantitative relations between the dynamic parameters and total ozone are also being studied.

Krueger, A. J.↗

Stratosphere chemistry in a 2-D model with residual circulation

The objective of this research was to examine the effects of chemical perturbations on the stratosphere using models which can incorporate fully interactive radiative, chemical, and dynamical responses, in the context of a zonally averaged model. Model runs for the unperturbed, chlorine-perturbed and simultaneously chlorine-and CO2-perturbed cases were completed using the JPL-87 chemical kinetics data. The base case was analyzed and submitted for publication. The perturbed cases show substantial sensitivity of the predicted column ozone depletion to the perturbations affecting lower stratosphere temperature, but less to far dynamical perturbations. The column ozone distribution changed substantially when the kinetics data was changed. This implies a greater-than-expected uncertainty in predicted latitude distributions of ozone depletion, due to uncertainty about the accuracy and completeness of the chemical kinetics data set.

Guthrie, Paul D.↗

Quantifying Chemical Ozone Loss in the Arctic Stratosphere with GEOS-STRATCHEM Data Assimilation System

A faithful representation of polar stratospheric chemistry in models and its connection with dynamical variability is essential for our understanding of the evolution of the ozone layer in a changing climate and during the projected continuing decline of ozone depleting substances in the atmosphere. We use a new configuration of the Goddard Earth Observing System Data Assimilation System with a stratospheric chemistry model to study ozone depletion in the Arctic polar stratosphere during the exceptionally cold (in the stratosphere) winters 2015/2016 and 2010/2011.

Arctic↗

An observational study of the final warming in the Southern Hemisphere stratosphere

The final warming in the Southern Hemisphere stratosphere during the period September 1-November 30 for the years 1978-1983 is studied. The change in zonally averaged temperatures during that period is almost the same for each year. However, there is substantial interannual variability in the time evolution of the warming as events of enhanced wave, mean-flow interaction associated with bursts of upward propagating planetary waves develop at different times in different years. Polar temperatures in the middle stratosphere can increase as much as about 20 K in 4 days during these events. Such dynamical processes can play a significant role in the interannual variability of stratospheric ozone and other constituents.

Farrara, John D.↗

Some aspects of the interaction between chemical and dynamic processes relating to the Antarctic ozone hole

Observational and modeling studies have been conducted to examine the interaction between the chemical and dynamical processes that occur during springtime in the lower stratosphere of the Southern Hemisphere. The temporal evolution of the ozone distribution and the circulation during 1987 is contrasted with that for 1988 as an illustrative example of how dynamical processes and the resulting meteorological conditions modulate the ozone depletion. Concurrently with the observational analysis, an effort was initiated to simulate the ozone depletion during austral spring using a 3D chemical/transport model. The model includes a parameterized representation of the heterogeneous processes thought to be important in this region. The simulation indicates that the inclusion of this additional chemistry, which results in the release of free chlorine and the redistribution of odd nitrogen into reservoir species, reproduces many aspects of the observations.

Eckman, R. S.↗

Lidar Measurements of Aerosol and Ozone Distributions During the 1992 Airborne Arctic Stratospheric Expedition

The LaRC airborne lidar system was operated from the ARC DC-8 aircraft during the 1992 Airborne Arctic Stratospheric Expedition (ASEE-2) to investigate the distribution of stratospheric aerosols and O3 across the Arctic vortex from Jan. to Mar. 1992. Monthly flights were made across the Arctic vortex from Anchorage, Alaska, to Stavanger, Norway, and then back to Bangor, Maine, and additional round-trip flights north into the vortex were made each month from either Stavanger or Bangor depending on the location of the vortex that month. The airborne lidar system uses the differential absorption lidar (DIAL) technique at laser wavelengths of 301.5 and 310.8 nm to measure O3 profiles above the DC-8 over the 12-25 km altitude range. Lidar measurements of aerosol backscatter and depolarization profiles over the 12-30 km altitude range are made simultaneously with the O3 measurements using infrared (IR) and visible (VIS) laser wavelengths of 603 and 1064 nm, respectively. The measurements of Pinatubo aerosols, polar stratospheric clouds, and O3 made with the airborne DIAL system during the AASE-2 expedition and to chemical and dynamical process that contribute to O3 depletion in the wintertime Arctic stratosphere.

Browell, E. V.↗

Large-scale motion in the Venus stratosphere

To examine a postulate that the horizontal momentum exchanges in the Venusian stratosphere are quasi-nondivergent, the properties of two-dimensional turbulence on a slowly rotating sphere in a high-resolution, one-level numerical model are investigated. It is concluded that the forcing which maintains the stratospheric flow is weak and influences the dynamics far less than the inertial effects. Consequently, the behavior resembles that of vorticity-conserving, two-dimensional flows. On a slowly rotating planet like Venus, such flows are dominated by solid-body rotation and by a planetary wave of unit zonal wavenumber - this wave corresponds to the observed Y-shaped UV feature. Although these largest scales of motion stand out, the dynamic balances of the flow are fundamentally nonlinear, in contrast to the quasi-linear Rossby wave regime on rapidly rotating planets.

Rossow, W. B.↗

Synopsis of the Fifth Conference on the Meteorology of the Stratosphere and Mesosphere

The papers presented at the Fifth Conference on the Meteorology of the Stratosphere and Mesosphere held on April 23-26, 1985, are reviewed. The observational aspects of large-scale circulation, such as summer and winter circulation in the Southern Hemisphere, and analysis schemes, like the multivariate statistical analysis scheme, are discussed. The topics of numerical simulations of the general circulation and sudden-warming are examined. Papers concerning processes of O3, NO2, H2, and HNO3 are described. Research on large-scale mixing processes in the stratosphere is presented. The topic of equatorial dynamics and stability is analyzed. Papers focusing on the effect of gravity waves on the general circulation are studied.

Schoeberl, M. R.↗

Cryogenic Limb Array Etalon Spectrometer (CLAES) - Experiment overview

The Cryogenic Limb Array Etalon Spectrometer (CLAES) is one of a complement of instruments on the NASA Upper Atmosphere Research Satellite which is expected to study atmospheric photochemistry, energy input, and dynamics following a 1991 launch. CLAES measures stratospheric altitude profiles of temperature, pressure, O3, H2O, CH4, N2O, NO, NO2, N2O5, HNO3, ClONO2, HCl, CFC-11, and CFC-12. These data are obtained typically between 10 and 60 km, with 2.5-km vertical resolution and 500-km horizontal grid size. Coverage is obtained between latitudes 80 deg north and south, thereby providing substantial coverage of the Antarctic spring polar ozone-hole region. CLAES derives the listed geophysical parameters from measurement of earth-limb spectral emissions between 3.5 and 13 microns. Brief discussions of the measurement concept, instrument design, and performance are presented, followed by a more detailed discussion of scientific capabilities and measurement modes.

Roche, Aidan E.↗