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At least 343 records · Page 19

FAST-1.1: A Computer Code for Thermal-Mechanical Nuclear Fuel Analysis under Steady-state and Transients (Developed under NQA-1-2017)

Fuel Analysis under Steady-state and Transients (FAST) is the U.S. Nuclear Regulatory Commission (NRC)’s computer code that calculates the steady-state and transient response of nuclear reactor fuel rods during long-term in-reactor burnup, anticipated operational occurrences (AOOs), design basis accidents (DBAs), and dry storage conditions. The code calculates the temperature, pressure, and deformation of a fuel rod as functions of time-dependent fuel rod power and coolant boundary conditions. The phenomena modeled by the code include: * heat conduction through the fuel and other materials * heat transfer from the cladding-to-coolant * cladding elastic and plastic deformation, including creep * fuel-cladding mechanical interaction * fission gas release from the fuel * rod internal pressure and void volume * cladding oxidation The code contains necessary material and coolant properties, as well as clad-to-coolant heat transfer correlations, for normal operation through postulated accidents and AOOs for today’s U.S.-based light water reactor (LWR) fuel designs. FAST-1.1 also contains preliminary materials and models for new LWR fuel concepts, such as accident tolerant fuel (ATF), and non-LWR fuel concepts such as metallic fuels for sodium fast reactors (SFRs). FAST has been developed for use on Windows and Linux operating systems. This document describes FAST-1.1 and is one of a series of documents on the code; the other documents detail the material properties used by FAST as well as its integral assessment to experiments and commercial data.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

FAST-1.2.2: A Computer Code for Thermal-Mechanical Nuclear Fuel Analysis under Steady-state and Transients

Fuel Analysis under Steady-state and Transients (FAST) is the U.S. Nuclear Regulatory Commission (NRC)’s computer code that calculates the steady-state and transient response of nuclear reactor fuel rods during long-term in-reactor burnup, anticipated operational occurrences (AOOs), design basis accidents (DBAs), and dry storage conditions. The code calculates the temperature, pressure, and deformation of a fuel rod as functions of time-dependent fuel rod power and coolant boundary conditions. The phenomena modeled by the code include heat conduction through the fuel and other materials, heat transfer from the cladding-to-coolant, cladding elastic and plastic deformation (including creep), fuel-cladding mechanical interaction, fission gas release from the fuel, rod internal pressure, void volume, and cladding oxidation. The code contains necessary material and coolant properties, as well as clad-to-coolant heat transfer correlations, for normal operation through postulated accidents and AOOs for today’s U.S.-based light water reactor (LWR) fuel designs. FAST-1.2.2 also contains preliminary materials and models for new LWR fuel concepts, such as accident tolerant fuel (ATF), and non-LWR fuel concepts such as metallic fuels for sodium fast reactors (SFRs). FAST has been developed for use on Windows and Linux operating systems. This document describes FAST-1.2.2 and is one of a series of documents on the code; the other documents detail the material properties used by FAST as well as its integral assessment to experiments and commercial data.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of Cone Wedge Ring Expansion Test to Evaluate Mechanical Properties of Clad Tubing Structure

To determine the hoop tensile properties of irradiated fuel cladding in a hot cell, a cone wedge ring expansion test method was developed. A four-piece wedge insert was designed with tapered angles matched to the cone shape of a loading piston. The ring specimen was expanded in the radial direction by the lateral expansion of the wedges under the downward movement of the piston. The advantages of the proposed method are that implementation of the test setup in a hot cell is simple and easy, and that it enables a direct strain measurement of the test specimen from the piston’s vertical displacement soon after the wedge-clad contact resistance is initiated.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

FAST-1.2: A Computer Code for Thermal-Mechanical Nuclear Fuel Analysis under Steady-state and Transients

Fuel Analysis under Steady-state and Transients (FAST) is the U.S. Nuclear Regulatory Commission (NRC)’s computer code that calculates the steady-state and transient response of nuclear reactor fuel rods during long-term in-reactor burnup, anticipated operational occurrences (AOOs), design basis accidents (DBAs), and dry storage conditions. The code calculates the temperature, pressure, and deformation of a fuel rod as functions of time-dependent fuel rod power and coolant boundary conditions. The phenomena modeled by the code include: • heat conduction through the fuel and other materials • heat transfer from the cladding-to-coolant • cladding elastic and plastic deformation, including creep • fuel-cladding mechanical interaction • fission gas release from the fuel • rod internal pressure and void volume • cladding oxidation The code contains necessary material and coolant properties, as well as clad-to-coolant heat-transfer correlations, for normal operation through postulated accidents and AOOs for today’s U.S.-based light water reactor (LWR) fuel designs. FAST-1.2 also contains preliminary materials and models for new LWR fuel concepts, such as accident tolerant fuel (ATF), and non-LWR fuel concepts such as metallic fuels for sodium fast reactors (SFRs). FAST has been developed for use on Windows and Linux operating systems. This document describes FAST-1.2 and is one of a series of documents on the code; the other documents detail the material properties used by FAST as well as its integral assessment to experiments and commercial data.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

ADVANCED TEST REACTOR (ATR) CONVERSION TO LOW ENRICHED URANIUM (LEU) FUEL

The United States Department of Energy (DOE), National Nuclear Security Administration (NNSA), Office of Material Management and Minimization (MMM) is working to convert research reactors globally from highly enriched uranium (HEU) fuel to low-enriched uranium (LEU) fuel. MMM and its predecessor programs have converted or verified the shutdown of 88 HEU research reactors and isotope production facilities, using LEU fuel developed in the 1980s. However, there is a small set of high performance research reactors which require a new high density LEU fuel for conversion, including six U.S. high performance research reactors (USHPRRs), which include the Advanced Test Reactor (ATR) and the ATR Critical (ATRC) Facility at the Idaho National Laboratory (INL) near Idaho Falls, ID; University of Missouri Research Reactor (MURR) at Columbia, MO; Massachusetts Institute of Technology Reactor (MITR) at MIT in Cambridge, MA; High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory (ORNL) near Oak Ridge, TN; and National Bureau of Standards Reactor (NBSR) at the National Institute of Standards and Technology (NIST) Center for Neutron Research (NCNR) in Gaithersburg, MA. These reactors will share the same uranium-molybdenum (U-Mo) fuel plate design. The U-Mo fuel meat foil will have a zirconium (Zr) diffusion barrier with aluminum cladding. Three different application methods for the Zr diffusion barrier layer are being pursued – co-rolled, electroplating and plasma spraying. Fabrication of the higher density LEU U-Mo fuel has presented several challenges. Because the U-Mo fuel fabrication process uses the existing stockpile of 93% highly enriched uranium (HEU) to be blended with molybdenum and depleted uranium (DU) to form 19.75% LEU, cost benefits of enriching to 19.75% will not be realized. Homogeneity of the U-235 and molybdenum in the metal foil is a challenge due to U-Mo casting process results in variations between adjacent cast U-Mo plates. LEU will not require less U-235 as previously believed due to self-shielding properties of U-238 requiring additional U-235 to be loaded in each fuel element. Although the overall dimensions of the ATR fuel element remain unchanged, the weight of the LEU ATR fuel element is 72% greater than a HEU ATR fuel element. During waste recovery and recycling efforts, separation of aluminum cladding from the HEU fuel meat is a relatively simple chemical dissolution, however, separation of the Zr diffusion barrier from the U-Mo fuel meat is significantly more challenging.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Reactivity-initiated accidents in two pressurized water reactor high burnup core designs

Here, this paper presents a safety analysis of two proposed core loadings for 24-month Pressurized Water Reactor (PWR) fuel cycles. This analysis focuses on reactivity-initiated accidents (RIAs) and evaluates core safety performance impacts of rod-averaged burnup limits up to 75 GWD/MTU and less than 7 % enriched UO 2 . The capabilities of Polaris, PARCS, and RELAP5-3D are leveraged to evaluate the core neutronic and thermal–hydraulic behavior for normal-operation, uncontrolled control rod withdrawal (CRW) transients, and control rod ejection (CRE) accidents. The two core designs are compared to identify features of realistic high burnup/extended enrichment core design approaches which have significant safety impact, identify experimental data needs for high-fidelity predictive modeling, and provide recommendations for future high burnup core designs. The first core design evaluated in this study was developed by Southern Nuclear Company and used an ZrB 2 Integral Fuel Burnable Absorber (IFBA) and B 4 C Wet-Annular Burnable Absorber (WABA)-based burnable poison strategy. The second core design assessed in this work used a Gd 2 O 3 -doped UO 2 burnable poison, similar to that used in boiling water reactors or French PWRs. Results indicate that fuel thermal limits are maintained for limiting CRW and hot full power (HFP) CRE transients. Cladding failure is predicted for the highest energy deposition rods in each core during limiting hot zero power (HZP) CRE accidents (where maximum radially averaged enthalpy exceeds 120 cal/g), though licensing may be permissible with a limited number of failed rods. While concerns exist regarding high critical boron concentration during steady state for the IFBA core and large plenum pressures for the gadolinia core design, the analysis demonstrates adequate safety performance during limiting RIA accident scenarios for two representative high burnup core designs. Design changes limiting plenum pressures and implementation of accident tolerant fuel (ATF) cladding features which minimize hydriding and susceptibility to pellet-cladding mechanical interaction (PCMI) are recommended for future high burnup fuel concepts. To support the technical basis for burnup limit increases, high-fidelity fuel performance models are needed to address physical effects not considered in this analysis, and high burnup irradiated fuel tests are required to extend applicability of the fuel failure limits and validate existing and future models.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Plastic flow and microstructural instabilities during high-pressure torsion of Cu/ZnO composites

Highlights: • Hybrid bulk metal - ceramic nanoparticle material was processed by HPT. • ZnO nanoparticles exhibited significant plasticity of up to 86%. • Hydrodynamic instability determined the flow mode of ZnO particle clusters. • Microstructural stability of Cu decreased due to the co-deformation with ZnO. - Abstract: We conducted high-pressure torsion (HPT) of hybrid materials composed of two copper disks with a layer of ZnO ceramic nanoparticles sandwiched in-between. A detailed microstructural analysis of the processed samples revealed a surprisingly high level of plastic deformation introduced in individual ZnO particles, even though they possess a much high hardness than the surrounding Cu. Moreover, we demonstrated that by tailoring the initial geometry of the system (i.e. introducing holes in the cladding Cu disks), we can effectively change the flow mode of ZnO particle clusters from laminar to turbulent one and facilitate their deagglomeration process. Finally, the presence of ZnO particles decreased the microstructural stability of the Cu matrix. We discussed the obtained results in terms of hydrodynamic and microstructural instabilities during plastic deformation. This work expands our understandings of the cooperative severe plastic deformation of two dissimilar materials and sheds new light on the design of hybrid materials.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Design and analysis of oxidation tests to inform FeCrAl ATF severe accident models

Iron-chromium-aluminum (FeCrAl) alloys are being considered as advanced fuel cladding concepts with enhan ced accident tolerance. At high temperatures, FeCrAl alloys have slower oxidation kinetics and higher strength compared with zirconium-based alloys. FeCrAl could be used for fuel cladding and spacer or mixing vane grids in light water reactors and/or as ch annel box material in boiling water reactors (BWRs). There is a need to assess the potential gains afforded by the FeCrAl accident-tolerant-fuel (ATF) concept over the existing zirconium-based materials employed today. To accurately assess the response of FeCrAl aloys under severe accident conditions, a number of FeCrAl properties and characteristics are required. These include thermophysical properties as well as burst characteristics, oxidation kinetics, possible eutectic interactions, and failure temperatures. These properties can vary among different FeCrAl alloys.

36 MATERIALS SCIENCE↗

Postirradiation characterization of palladium as an additive for fuel cladding chemical interaction mitigation in metallic fuel

This work describes the microstructural and elemental characterization of irradiated metallic fuels containing palladium as an additive. The use of additives has been proposed to control Fuel-Cladding Chemical Interaction (FCCI) and thus to promote higher fuel utilization (i.e., higher burnup). In this work, Pd has been investigated as a potential additive to metallic fuel to bind lanthanides, impeding their migration and attack on the cladding. The influence of Pd on the microstructure, chemistry and performance of metallic fuel has been characterized via scanning electron microscopy for two metallic fuel designs—namely, annular and solid fuel. Pd was observed to play an important role in the chemistry of the fuel. Indeed, the addition of Pd leads to the formation of new phases. Pd was detected to combine not only with the lanthanides, as intended, but also with Zr, a main element of the fuel matrix. While Pd proved to be effective in preventing lanthanide migration and their attack on the cladding, the Pd-Zr compound may potentially lead to other unexpected fuel-performance issues, such as the formation of low-melting point phases and increased unalloyed U available for FCCI interaction with Fe in the cladding. Even the increase of Zr to 13wt%. did not completely mitigate this adverse phenomenon generated by the Pd-Zr interaction. Furthermore, the efficacy of using this additive needs further investigation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Implementation of an Orificing Optimization Algorithm in the DASSH Subchannel Analysis Code

The Ducted Assembly Steady-State Heat transfer code (DASSH) performs full-core subchannel thermal hydraulics calculations in liquid metal fast reactors. One of the applications of subchannel codes is to optimize coolant flow orificing. As a design activity, the primary task is to determine the best way to divide assemblies into groups and distribute coolant flow rates among them. This report documents an algorithm implemented in DASSH to automatically optimize coolant orificing. Over the course of multiple iterations, DASSH determines the orifice grouping and flow distribution that minimizes peak coolant, clad, or fuel temperatures across all timesteps for a user-specified number of assembly groups. The total coolant flow rate in the reactor is constrained to achieve the specified core-average outlet temperature. The flow rate to each orifice group may also be constrained by the allowable pressure drop. The distribution of coolant flow among groups is accelerated using a predictor-corrector algorithm based on interpolated results from single-assembly parametric calculations. The assembly orificing grouping is initially predicted based on assembly power but can be refined if results demonstrate that an assembly would fit better in another group. The algorithm is demonstrated with two case studies. The first is a simple model for a reactor core consisting of just fuel assemblies; the pin power distributions are specified to create a situation where the initial assembly grouping prediction is suboptimal. This example is used to describe the initial grouping, demonstrate convergence over multiple iterations, and highlight the impact of regrouping. Then, the algorithm is applied to minimize peak clad and fuel temperatures in an example sodium-cooled fast reactor, the Versatile Test Reactor. The multicycle optimization confirms prior calculations for the reference core design. The example highlights how optimizing for different peak temperatures affects the results and demonstrates the use of the pressure drop constraint to limit the maximum flow rate.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Update on the Thermal Hydraulic Investigations of a Horizontal Dry Cask Simulator

The thermal performance of commercial spent nuclear fuel dry storage casks is evaluated through detailed numerical analysis. These modeling efforts are completed by the vendor to demonstrate performance and regulatory compliance. The calculations are then independently verified by the Nuclear Regulatory Commission (NRC). Canistered dry storage cask systems rely on ventilation between the inner canister and the overpack to convect heat away from the canister to the surrounding environment for both horizontal and vertical configurations. Recent advances in dry storage cask designs have significantly increased the maximum thermal load allowed in a canister in part by increasing the efficiency of internal conduction pathways and by increasing the internal convection through greater canister helium pressure. Carefully measured data sets generated from testing of full-sized casks or smaller cask analogs are widely recognized as vital for validating these models. While several testing programs have been previously conducted, these earlier validation studies did not integrate all the physics or components important in a modern, horizontal dry cask system. The purpose of the present investigation is to produce data sets that can be used to benchmark the codes and best practices presently used to determine cladding temperatures and induced cooling air flows in modern horizontal dry storage systems. The horizontal dry cask simulator (HDCS) has been designed to generate this benchmark data and add to the existing knowledge base. The objective of the HDCS investigation is to capture the dominant physics of a commercial dry storage system in a well-characterized test apparatus for any given set of operational parameters. The close coupling between the thermal response of the canister system and the resulting induced cooling air flow rate is of particular importance.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Stress rupture of SiC/SiC composite tubes under high-temperature steam

SiC-fiber–reinforced SiC matrix composite cladding for light water reactor fuel elements must withstand high-temperature steam oxidation in a loss-of-coolant accident scenario (LOCA). Current composite designs include an outer monolithic SiC layer, in part, to increase steam oxidation resistance. However, it is not clear how such a structure would behave under high-temperature steam in the case when the monolithic layer cracks and carbon interphases and SiC fibers are exposed to the environment. To fill this knowledge gap, stress-rupture tests of prototypic SiC composite cladding at 1000°C under steam and inert environments were conducted. The applied stress was ~120 MPa, which was beyond the initial cracking stress. The failure lifetime under steam was 400–1300 s, while 75% of the composite specimens did not fail after 3 h of total exposure under inert gases. Microstructural observations suggest that steam oxidation activated slow crack growth in the fibers, which led to failure of the composite. The results from this study suggest that stress rupture in steam environments could be a limiting factor of the cladding under reactor LOCA conditions.

36 MATERIALS SCIENCE↗

Cladding and Butt-Joining Dissimilar Aluminum Alloys Simultaneously via Shear Assisted Processing and Extrusion

Shear assisted processing and extrusion has been used to fabricate multi-metallic tubing that incorporates regions with clad and butt-joined structures. In this work, aluminum alloys 6061, 7075, and 1100 are combined to create a monolithic extruded tubing with weldable ends (6061), a high strength center (7075), and a corrosion-resistant cladding (1100). Optical microscopy shows a gradual, defect-free, transition between alloys at the butt-joint interfaces and a sharp transition between alloys at the clad interface. Tensile testing proved the mechanical coherency of the joint, with failure occurring outside the tri-metallic structure. In conclusion, smoothed particle hydrodynamic simulations identified a spiral pattern of the cladding alloy that leads to inconsistent cladding thickness, and identified a simplified 2-alloy combination of aluminum alloys 6082 and 2014 that accomplished the design objectives of the tri-metallic structure.

Coatings↗

Novel intercore-cladding lithium niobate thin film coated MOEMS fiber sensor/modulator

A MOEMS fiber modulator/sensor is fabricated by depositing a lithium niobate sol-gel thin film between the core and cladding of a fiber preform. The preform is then drawn into 125-micron fibers. Such a MOEMS modulator design is expected to enhance existing lithium niobate undersea acousto-optic sound wave detectors. In our proposed version, the lithium niobate thin film alters the ordinary silica core/cladding boundary conditions such that, when a stress or strain is applied to the fiber, the core light confinement factor changes, leading to modulation of fiber light transmission. Test results of the lithium niobate embedded fiber with a 1550-nm, 4-mW laser source revealed a reduction in light transmission with applied tension. As a comparison, using the same laser source, an ordinary silica core/cladding fiber did not exhibit any reduction in transmitted light when the same strain was applied. Further experimental work and theoretical analysis is ongoing.

Jamlson, Tracee L.↗

Integral Heat Transfer Test Method for Determining Thermal Resistance of Silicon Carbide Cladding and Liquid Tin System at Elevated Temperatures - Master's Thesis Presentation University of Idaho

Presentation for master's work at University of Idaho discussing Integral Heat Transfer Test Method for Determining Thermal Resistance of Silicon Carbide Cladding and Liquid Tin System at Elevated Temperatures. Presentation covers slight literature review results/previous work, discussions on system design and approach for thermal property measurement of SiC composite and Tin system, modeling efforts, and results.

36 - MATERIALS SCIENCE↗

RISMC Industry Application no. 1 (ECCS/LOCA) Core characterization automation: Reference PWR designs for IA no. 1

The U.S. NRC is currently proposing rulemaking '10 CFR 50.46c' to revise the loss-of-coolant-accident (LOCA) and emergency core cooling system (ECCS) acceptance criteria to include the effects of higher burn-up on cladding performance. The key implications of this proposition are that both cladding and ECCS performance need to be considered in a coupled manner. This implies that LOCA methodologies will need to be updated for regulatory purposes. The Risk-Informed Safety Margin Characterization (RISMC) Pathway, as part of the DOE Light Water Reactor Sustainability (LWRS) research and development program initialed several programs at the Idaho National Laboratory (INL) to support the industry by offering potential solutions to this new LOCA/ECCS analysis. One of these programs is the Industry Application no. 1 (IA1). It's goal is to develop an integrated evaluation model called LOCA Toolkit for the US (LOTUS) to revisit how risks are evaluated in a LOCA under 10 CFR 50.46c. The focus of LOTUS is to establish the automation interfaces among the physics disciplines involved, namely the core design automation, the fuels/clad performance, the system analysis, the risk assessment and the core design optimization. The risk-informed margins management approach for IA1 will provide a means of quantifying the impact on the key LOCA analysis figures-of-merit like peak cladding temperature (PCT), equivalent cladding reacted (ECR), etc. of a change in LOCA analysis inputs. The information obtained can then be used for decision-making and margin management. The modular approach for LOTUS will enable plant owners/vendors to further customize the LOTUS framework for use within their established codes and methods. One of the LOTUS modules deals with the core design automation (CD-A). The purpose of this module is to supply the LOCA analysis with initial conditions, i.e. assembly/pin power histories, power shapes, etc. to be employed by the Fuels/Clad Performance (EP) and System Analysis (SA) modules. In the CD-A module, the plant owner/operator will characterize his core design with the tools he has. For the current LOTUS demonstration, the tools used are the already coupled codes PHISICS and RELAP5-3D2,3. Cross section generation will be done using the Studsvik lattice code HELIOS-2.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Mechanistic FCCI model for BISON

In this report, multi-scale simulations to develop a mechanistic model of fuel-cladding chemical interaction (FCCI) conducted under the auspices of the Nuclear Energy Advanced Modeling and Simulation (NEAMS) program in FY23 are described. The model assumes that cladding wastage is dominated by the intermetallic phase (Fe,Cr)$_{17}$Nd$_2$, and calculates production and diffusion of Nd in the fuel, diffusion into the cladding, and formation and growth of the intermetallic wastage layer. Atomistic simulations are used to calculate diffusivity of Nd in the (Fe,Cr) system. Mesoscale simulations, informed by previous atomistic calculations, are used to determine the effective diffusivity of Nd through the fuel, accounting for empty and sodium-filled porosity within the fuel. The BISON model incorporates this data and calculates the wastage layer thickness as a function of time, assuming parabolic growth kinetics based on the best available data. The results of the new mechanistic BISON model are compared to existing assessment cases for the X447 experiment in EBR-II, and show good agreement with experimental data and the existing BISON empirical model. To improve predictions of kinetics for future work, a phase-field model that includes fuel, wastage, and cladding phases is developed. Preliminary testing indicates that the kinetics may differ significantly from the assumed parabolic growth law, suggesting direction for future improvement of the model that will allow it to be applied to other fuel designs with greater confidence.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Transient Reactor Test Facility (TREAT) Low Enriched Uranium (LEU) Conversion Progress

The National Nuclear Security Administration Office of Material Management and Minimization (NNSA M3) is working towards converting the Transient Reactor Test Facility (TREAT) located at the Idaho National Laboratory (INL) from its original high-enriched uranium (HEU) core to a low-enriched uranium (LEU) core. TREAT reactor operations were restarted in November of 2017 and data obtained from the initial testing will be used to validate the existing ANL reactor modeling. Fuel block development has progressed with the completion of 2 and 4 inch crack free surrogate fuel blocks. Alternative fabrication methods for the fuel blocks continue to be explored and are showing promising results. Additionally, cladding oxidation studies have been performed and analyzed to initiate the down selection of cladding material to be used for the TREAT LEU fuel elements. This paper describes the current status of the above mentioned activities, and discusses the anticipated path forward for the conversion program as it progresses toward a final fuel design and fuel fabrication process.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗