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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 343 records · Page 19
All sourcesNASA NTRSDOE OSTI
NASA NTRS2004

Spatial and Temporal Distribution of Tropospheric Clouds and Aerosols Observed by MODIS Onboard the Terra and Aqua Satellites

Remote sensing of cloud and aerosol optical properties is routinely obtained using the Moderate Resolution Imaging Spectroradiometer (MODIS) onboard the Terra and Aqua satellites. Techniques that are being used to enhance our ability to characterize the global distribution of cloud and aerosol properties include well-calibrated multispectral radiometers that rely on visible, near-infrared, and thermal infrared channels. The availability of thermal channels to aid in cloud screening for aerosol properties is an important additional piece of information that has not always been incorporated into sensor designs. In this paper, we describe the radiative properties of clouds as currently determined from satellites (cloud fraction, optical thickness, cloud top pressure, and cloud effective radius), and highlight the global and regional cloud microphysical properties currently available for assessing climate variability and forcing. These include the latitudinal distribution of cloud optical and radiative properties of both liquid water and ice clouds, as well as joint histograms of cloud optical thickness and effective radius for selected geographical locations around the world. In addition, we will illustrate the radiative and microphysical properties of aerosol particles that are currently available from space-based observations, and show selected cases in which aerosol particles are observed to modify the cloud optical properties.

King, Michael D.↗
DOE OSTI2026

Spatial Heterogeneity in Cloud Condensation Nuclei (SHINE) Field Campaign Report

Multiple land-atmosphere coupling processes influence the spatial distribution of boundary-layer energy, moisture, aerosol, or cloud condensation nuclei (CCN) properties. Accurately quantifying the spatial and temporal distributions of CCN concentrations is essential for investigating aerosol-cloud interactions and reducing uncertainties in aerosol radiative forcing estimates of Earth's system.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Interfacial Dark Aging Is an Overlooked Source of Aqueous Secondary Organic Aerosol

In this work, the relative yields of aqueous secondary organic aerosols (aqSOAs) at the air–liquid (a–l) interface are investigated between photochemical and dark aging using in situ time-of-flight secondary ion mass spectrometry (ToF-SIMS). Our results show that dark aging is an important source of aqSOAs despite a lack of photochemical drivers. Photochemical reactions of glyoxal and hydroxyl radicals (•OH) produce oligomers and cluster ions at the aqueous surface. Interestingly, different oligomers and cluster ions form intensely in the dark at the a–l interface, contrary to the notion that oligomer formation mainly depends on light irradiation. Furthermore, cluster ions form readily during dark aging and have a higher water molecule adsorption ability. This finding is supported by the observation of more frequent organic water cluster ion formation. The relative yields of water clusters in the form of protonated and hydroxide ions are presented using van Krevelen diagrams to explore the underlying formation mechanisms of aqSOAs. Large protonated and hydroxide water clusters (e.g., (H2O)nH+, 17 < n ≤ 44) have reasonable yields during UV aging. In contrast, small protonated and hydroxide water clusters (e.g., (H2O)nH+, 1 ≤ n ≤ 17) form after several hours of dark aging. Moreover, cluster ions have higher yields in dark aging, indicating the overlooked influence of dark aging interfacial products on aerosol optical properties. Molecular dynamic simulation shows that cluster ions form stably in UV and dark aging. AqSOAs molecules produced from dark and photochemical aging can enhance UV absorption of the aqueous surface, promote cloud condensation nuclei (CCN) activities, and affect radiative forcing.

Van Krevelen diagram↗
NASA NTRSDate not supplied

Uncertainties in an Observation-Based Estimate of the Global Aerosol Direct Radiative Effect

Aerosols impact Earth’s radiation budget directly through interactions with radiation and indirectly via interactions with clouds. Aerosols have significant radiative impacts on Earth’s energy budget and represent the largest uncertainty in the radiative forcing of the current climate. Although the magnitude of the aerosol direct radiative effect (DRE) is estimated to be less than that of the indirect effect, uncertainties are large. While model-based estimates of aerosol radiative forcing are subject to uncertainties in modeled aerosol properties and uncertainties in simulated cloud cover and albedo, most observation-based studies of global aerosol DRE have their own difficulties with aerosol optical properties and have been limited to cloud-free skies in most cases. Estimates of the uncertainty of the aerosol DRE are themselves uncertain and have varied widely among different published studies. In this study we use the CERES-CALIPSO-CloudSat-MODIS (C3M) product to estimate the global clear-sky and all-sky aerosol DRE. C3M merges collocated data from CERES, CALIPSO, CloudSat, and MODIS with information from reanalysis and an aerosol transport model. With CALIOP observations of aerosol below optically thin clouds and above clouds, co-located with cloud albedo from MODIS, the C3M dataset allows a detailed exploration of observational uncertainties. By perturbing the aerosol properties used and comparing radiative effects in perturbed cases with the base case we characterize uncertainties in estimated aerosol DRE due to uncertainties in the aerosol properties involved. The results also provide a basis for determining measurement requirements to improve the accuracy of DRE estimates. We will describe the approach and present results.

Dave Winker↗
NASA NTRS2022

Vertical structure of biomass burning aerosol transported over the southeast Atlantic Ocean

Biomass burning in southwestern Africa produces smoke plumes that are transported over the Atlantic Ocean and overlie vast regions of stratocumulus clouds. This aerosol layer contributes to direct and indirect radiative forcing of the atmosphere in this region particularly during the months of August, September, and October. There was a multi-year international campaign to study this aerosol and its interactions with clouds. Here, we report on the evolution of aerosol distributions and properties as measured by the airborne high spectral resolution lidar (HSRL-2) during the ORACLES (Observations of Aerosols above Clouds and their intEractionS) campaign in September 2016. The NASA Langley HSRL-2 instrument was flown on the NASA ER-2 aircraft for several days in September 2016. Data were aggregated at two pairs of 2° × 2° grid boxes to examine the evolution of the vertical profile of aerosol properties during transport over the ocean. Results showed that the structure of the profile of aerosol extinction and microphysical properties is maintained over a 1 to 2 d timescale. In the 3–5 km altitude range, 95 % of the aerosol extinction was contributed by particles in the 0.05–0.50 µm radius size range with the aerosol in this size range having an average effective radius of 0.16 µm. This indicates that there is essentially no scavenging or dry deposition at these altitudes. Moreover, there is very little day-to-day variation in these properties, such that time sampling as happens in such campaigns may be representative of longer periods such as monthly means. Below 3 km, there is considerable mixing with larger aerosol, most likely continental source near land. Furthermore, these measurements indicated that there was often a distinct gap between the bottom of the aerosol layer and cloud tops at the selected locations as evidenced by a layer of several hundred meters that contained relatively low aerosol extinction values above the clouds.

lidar↗
NASA NTRS2003

The MODIS Aerosol Algorithm, Products, Validation and Applications

The MODerate resolution Imaging Spectroradiometer (MODIS) currently aboard both the Terra and Aqua satellites produces a suite of products designed to characterize global aerosol distribution, optical thickness and particle size. Never before has a space-borne instrument been able to provide such detailed information, complementing field and modeling efforts to produce a comprehensive picture of aerosol characteristics. The three years of Terra-MODIS data have been validated by comparing with co-located AERONET observations of aerosol optical thickness and derivations of aerosol size parameters. Some 8000 comparison points located at 133 AERONET sites around the globe show that the MODIS aerosol optical thickness retrievals are accurate to within the pre-launch expectations. MODIS-derived size parameters are also compared with AERONET retrievals and found to agree well for fine-mode dominated aerosol regimes. Aerosol regimes dominated by dust aerosol are less accurate, attributed to what is thought to be nonsphericity. Errors due to nonsphericity will be reduced by introducing a new set of empirical phase functions, derived without any assumptions of particle shape. The major innovation that MODIS bring to the field of remote sensing of aerosol is the measure of particle size and the separation of finemode and coarsemode dominated aerosol regimes. Particle size can separate finemode man-made aerosols created during combustion, from larger natural aerosols originating from salt spray or wind erosion. This separation allows for the calculation of aerosol radiative effect and the estimation of the man-made aerosol radiative forcing. MODIS can also be used in regional studies of aerosol-cloud interaction that affect the global radiative and hydrological cycles.

Remer, L. A.↗
NASA NTRS2018

Radiative Heating Profiles over Ascension Island during the 2016 and 2017 Biomass Burning Seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between cloud morphology and the environmental conditions in which marine boundary layer clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean, where it is likely that the absorbing and heating properties of these aerosols modify the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to observe thermodynamic, cloud and aerosol properties during two consecutive biomass burning seasons from July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). These observations in conjunction with radiation transfer modeling were used to assess the impact of biomass burning carbonaceous aerosol plumes as they passed over the site.Thermodynamic profiles were generated using a combination of radiosonde data and thermodynamic profilers to provide high temporal resolution profiles of quantities that are important for cloud development, such as CAPE and CIN. Coincident Ka-band radar and lidar profiles were used to characterize the cloud and sub-cloud structure. The resulting thermodynamic and cloud profiles are used as input forcing for the Rapid Radiative Transfer Model (RRTM) to compute radiative heating profiles over the observation site. Idealized experiments using RRTM, with and without aerosols present, are used to assess the impacts of the absorbing aerosol on the heating rate profiles.

Cumulus↗
NASA NTRS2017

Radiation, Smoke and Clouds Observed in the Southeastern Atlantic With the Research Scanning Polarimeter During ORACLES

The ObseRvations of Aerosols above Clouds and their interactions (ORACLES) project is making a series of field deployments to the southeastern Atlantic with NASA ER-2 and P3 aircraft to acquire both detailed remote sensing observations and in situ measurements of the aerosols and clouds in that region. This area is home to one of the largest low-level cloud decks on Earth that is seasonally affected by vast plumes of smoke from biomass burning, which in effect provides a natural experiment testing the radiative and microphysical interactions between the smoke and the clouds. The downward solar radiation at the surface, or cloud top, is always reduced by the presence of smoke. However, whether the amount of sunlight reflected back out to space is increased, or decreased by the presence of smoke is sensitively dependent on the brightness of the clouds and the fraction of light that the smoke absorbs each time light hits a smoke particle. In this study we use data from the Research Scanning Polarimeter, an along track scanning instrument, that provides measurements of the Stokes parameters I, Q and U at 410, 470, 555, 670, 865, 960, 1590, 1880 and 2260 nm at 150 viewing angles over a range of +/- 60° from nadir for each contiguous sub-aircraft pixel (~ 300 m in size). A retrieval algorithm is applied to the data acquired with a table look up technique, similar to that of the operational POLDER algorithm, to provide a first guess of the complex refractive index, optical depth and size distribution of the smoke particles together with cloud droplet size and optical depth. A subsequent iterative fitting procedure, where the fact that the doubling/adding method allows the construction of the Green's function for the radiative transfer equation, is used to obtain an efficient and statistically optimal estimate of the aerosol and cloud retrieval parameters. These retrieval parameters are evaluated against in situ observations, when available, and the optical depth and intensive lidar variables that are measured by the High Spectral Resolution Lidar 2. Finally, the aerosol and cloud retrievals are used to evaluate the variations in top of the atmosphere, surface/cloud top shortwave radiative forcing and atmospheric absorption that are caused by variations in the smoke and clouds.

Cairns, Brian↗
NASA NTRS1991

Atlas of the Earth's radiation budget as measured by Nimbus-7: May 1979 to May 1980

This atlas describes the seasonal changes in the Earth's radiation budget for the 13-month period, May 1979 to May 1980. It helps to illustrate the strong feedback mechanisms by which the Earth's climate interacts with the top-of-the-atmosphere insolation to modify the energy that various regions absorb from the Sun. Cloud type and cloud amount, which are linked to the surface temperature and the regional climate, are key elements in this interaction. Annual, seasonal, and monthly maps of the albedo, outgoing longwave and net radiation, noontime cloud cover, and mean diurnal surface temperatures are presented. Annual and seasonal net cloud forcing maps are also given. All of the quantities were derived from Nimbus-7 satellite measurements except for the temperatures, which were used in the cloud detection algorithm and came originally from the Air Force 3-dimensional nephanalysis dataset. The seasonal changes are described. The interaction of clouds and the radiation budget is briefly discussed.

Kyle, H. Lee↗
DOE OSTI2025

Features of mid- and high-latitude low-level clouds and their relation to strong aerosol effects in the Energy Exascale Earth System Model version 2 (E3SMv2)

The E3SMv2 model, like various other global models that include representations of aerosol–cloud interactions, uses an empirically chosen lower bound on the simulated in-cloud cloud droplet number concentration (CDNC) to help constrain the effective radiative forcing of anthropogenic aerosols, ERFaer. This study identifies where ultra-low CDNCs (i.e., concentrations lower than 10 cm−3) occur in the stratiform and shallow convective clouds simulated by E3SMv2 and which of the occurrences have the strongest impact on ERF aer . Process-level analyses are presented to reveal characteristics of the cloud droplet formation and removal processes associated with impactful ultra-low CDNCs. Simulations performed with present-day emissions show that ultra-low CDNCs are most frequently found over the mid- and high-latitude oceans in both hemispheres, while the occurrences are also frequent in polluted continental regions despite the high aerosol concentrations. Ultra-low CDNCs with the largest impacts on the simulated regional and global mean ERF aer are found in the lower troposphere in the Northern Hemisphere middle and high latitudes. These cases are typically associated with large cloud fractions, strong water vapor condensation, weak turbulence, and lack of cloud droplet nucleation from aerosol activation. Under such atmospheric conditions, boosting aerosol activation and enhancing turbulent mixing of cloud droplet number can increase the simulated CDNCs, although the magnitude of the global mean ERF aer increases undesirably. The reason for this model behavior is discussed. Overall, our study suggests that mid- and high-latitude low-level stratus occurring under weak turbulence is a cloud regime worth further investigating for the purpose of identifying and addressing the root causes of ultra-low CDNCs and strong ERF aer in E3SM.

Aerosol-Cloud Interaction↗
NASA NTRS1985

Cirrus clouds. I - A cirrus cloud model. II - Numerical experiments on the formation and maintenance of cirrus

A simplified cirrus cloud model is presented which may be used to investigate the role of various physical processes in the life cycle of a cirrus cloud. The model is a two-dimensional, time-dependent, Eulerian numerical model where the focus is on cloud-scale processes. Parametrizations are developed to account for phase changes of water, radiative processes, and the effects of microphysical structure on the vertical flux of ice water. The results of a simulation of a thin cirrostratus cloud are given. The results of numerical experiments performed with the model are described in order to demonstrate the important role of cloud-scale processes in determining the cloud properties maintained in response to larger scale forcing. The effects of microphysical composition and radiative processes are considered, as well as their interaction with thermodynamic and dynamic processes within the cloud. It is shown that cirrus clouds operate in an entirely different manner than liquid phase stratiform clouds.

Starr, D. OC.↗
NASA NTRS2014

Millimeter- and Submillimeter-Wave Remote Sensing Using Small Satellites

Cloud ice properties and processes play fundamental roles in atmospheric radiation and precipitation. Limited knowledge and poor representation of clouds in global climate models have led to large uncertainties about cloud feedback processes under climate change. Ice clouds have been used as a tuning parameter in the models to force agreement with observations of the radiation budget at the top of the atmosphere, and precipitation at the bottom. The lack of ice cloud measurements has left the cloud processes at intermediate altitudes unconstrained. Millimeter (mm) and submillimeter (submm)-wave radiometry is widely recognized for its potential to fill the cloud measurement gap in the middle and upper troposphere. Analyses have shown that channels from 183900 GHz offer good sensitivity to ice cloud scattering and can provide ice water path (IWP) products to an accuracy of 25 by simultaneously retrieving ice particle size (Dme) and IWP. Therefore, it is highly desirable to develop a cost-effective, compact mm/submm-wave instrument for cloud observations that can be deployed on future small satellites.This paper presents a conceptual study for a mm/submm-wave instrument for multispectral measurements of ice clouds. It discusses previous work at these frequencies by NASA Goddard Space Flight Center (GSFC) and the current instrument study, as well as receiver architectures and their anticipated performance. And finally, it describes a microsatellite prototype intended for use with this mm/submm-wave instrument.

small satellites↗
DOE OSTI2023

On the differences in the vertical distribution of modeled aerosol optical depth over the southeastern Atlantic

Abstract. The southeastern Atlantic is home to an expansive smoke aerosol plume overlying a large cloud deck for approximately a third of the year. The aerosol plume is mainly attributed to the extensive biomass burning activities that occur in southern Africa. Current Earth system models (ESMs) reveal significant differences in their estimates of regional aerosol radiative effects over this region. Such large differences partially stem from uncertainties in the vertical distribution of aerosols in the troposphere. These uncertainties translate into different aerosol optical depths (AODs) in the planetary boundary layer (PBL) and the free troposphere (FT). This study examines differences of AOD fraction in the FT and AOD differences among ESMs (WRF-CAM5, WRF-FINN, GEOS-Chem, EAM-E3SM, ALADIN, GEOS-FP, and MERRA-2) and aircraft-based measurements from the NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign. Models frequently define the PBL as the well-mixed surface-based layer, but this definition misses the upper parts of decoupled PBLs, in which most low-level clouds occur. To account for the presence of decoupled boundary layers in the models, the height of maximum vertical gradient of specific humidity profiles from each model is used to define PBL heights. Results indicate that the monthly mean contribution of AOD in the FT to the total-column AOD ranges from 44 % to 74 % in September 2016 and from 54 % to 71 % in August 2017 within the region bounded by 25∘ S–0∘ N–S and 15∘ W–15∘ E (excluding land) among the ESMs. ALADIN and GEOS-Chem show similar aerosol plume patterns to a derived above-cloud aerosol product from the Moderate Resolution Imaging Spectroradiometer (MODIS) during September 2016, but none of the models show a similar above-cloud plume pattern to MODIS in August 2017. Using the second-generation High Spectral Resolution Lidar (HSRL-2) to derive an aircraft-based constraint on the AOD and the fractional AOD, we found that WRF-CAM5 produces 40 % less AOD than those from the HSRL-2 measurements, but it performs well at separating AOD fraction between the FT and the PBL. AOD fractions in the FT for GEOS-Chem and EAM-E3SM are, respectively, 10 % and 15 % lower than the AOD fractions from the HSRL-2. Their similar mean AODs reflect a cancellation of high and low AOD biases. Compared with aircraft-based observations, GEOS-FP, MERRA-2, and ALADIN produce 24 %–36 % less AOD and tend to misplace more aerosols in the PBL. The models generally underestimate AODs for measured AODs that are above 0.8, indicating their limitations at reproducing high AODs. The differences in the absolute AOD, FT AOD, and the vertical apportioning of AOD in different models highlight the need to continue improving the accuracy of modeled AOD distributions. These differences affect the sign and magnitude of the net aerosol radiative forcing, especially when aerosols are in contact with clouds.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Aerosol characteristics at the Southern Great Plains site during the HI-SCALE campaign

Abstract. Large uncertainties exist in global climate model predictions of radiative forcing due to insufficient understanding and simplified numerical representation of cloud formation and cloud–aerosol interactions. The Holistic Interactions of Shallow Clouds, Aerosols and Land Ecosystems (HI-SCALE) campaign was conducted near the DOE's Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) site in north-central Oklahoma to provide a better understanding of land–atmosphere interactions, aerosol and cloud properties, and the influence of aerosol and land–atmosphere interactions on cloud formation. The HI-SCALE campaign consisted of two intensive observational periods (IOPs) (April–May and August–September, 2016), during which coincident measurements were conducted both on the G-1 aircraft platform and at the SGP ground site. In this study we focus on the observations at the SGP ground site. An Aerodyne high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS) and an Ionicon proton-transfer-reaction mass spectrometer (PTR-MS) were deployed, characterizing chemistry of non-refractory aerosol and trace gases, respectively. Contributions from various aerosol sources, including biogenic and biomass burning emissions, were retrieved using factor analysis of the AMS data. In general, the organic aerosols at the SGP site was highly oxidized, with oxygenated organic aerosol (OOA) identified as the dominant factor for both the spring and summer IOP though more aged in spring. Cases of isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) and biomass burning events were further investigated to understand additional sources of organic aerosol. Unlike other regions largely impacted by IEPOX chemistry, the IEPOX SOA at SGP was more highly oxygenated, likely due to the relatively weak local emissions of isoprene. Biogenic emissions appear to largely control the formation of organic aerosol (OA) during the HI-SCALE campaign. Potential HOM (highly oxygenated molecule) chemistry likely contributes to the highly oxygenated feature of aerosols at the SGP site, with impacts on new particle formation and global climate.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

Surface Observations From Atmospheric Radiation Measurement Sites Constrain the Anthropogenic Contribution to Cloud Droplet Number

Uncertainty in anthropogenic forcing driven by aerosol-cloud interactions (aci) limits our ability to infer the sensitivity of the Earth system to forcing from historical records. The driver of aci is the change in cloud droplet number concentration (N d ) due to changes in aerosol serving as cloud condensation nuclei (CCN). Here, we combine a perturbed parameter ensemble run in a global Earth system model with observations of CCN and single-layer-cloud N d at surface sites in the Azores, the Southern Great Plains, and Ascension Island to provide a constraint on the anthropogenic contribution to present-day N d . These observational lines of evidence constrain the preindustrial to present-day change in N d to be between 11 and 43 cm −3 . This is consistent with the upper end of some previous estimates but has a higher minimum perturbation, pointing to a stronger historical aerosol cooling.

ARM↗
DOE OSTI2024

Aerosol-induced closure of marine cloud cells: enhanced effects in the presence of precipitation

Abstract. The Weather Research Forecasting (WRF) version 4.3 model is configured within a Lagrangian framework to quantify the impact of aerosols on evolving cloud fields. Kilometer-scale simulations utilizing meteorological boundary conditions are based on 10 case study days offering diverse meteorology during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA). Measurements from aircraft, the ground-based Atmosphere Radiation Measurement (ARM) site at Graciosa Island in the Azores, and A-Train and geostationary satellites are utilized for validation, demonstrating good agreement with the WRF-simulated cloud and aerosol properties. Higher aerosol concentration leads to suppressed drizzle and increased cloud water content in all case study days. These changes lead to larger radiative cooling rates at cloud top, enhanced vertical velocity variance, and increased vertical and horizontal wind speed near the base of the lower-tropospheric inversion. As a result, marine cloud cell area expands, narrowing the gap between shallow clouds and increasing cloud optical thickness, liquid water content, and the top-of-atmosphere outgoing shortwave flux. While similar aerosol effects are observed in lightly to non-raining clouds, they tend to be smaller by comparison. These simulations show a relationship between cloud cell area expansion and the radiative adjustments caused by liquid water path and cloud fraction changes. The adjustments are positive and scale as 74 % and 51 %, respectively, relative to the Twomey effect. While higher-resolution large-eddy simulations may provide improved representation of cloud-top mixing processes, these results emphasize the importance of addressing mesoscale cloud-state transitions in the quantification of aerosol radiative forcing that cannot be attained from traditional climate models.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2022

Aerosols Optical and Radiative Properties in Indonesia Based on AERONET Version 3

Heterogeneity in seasonal aerosol types due to different sources, local characteristics, and meteorology lead to different optical and radiative properties from one place to another. This study analyzes the long-term averages of aerosol optical and radiative properties obtained by the Aerosol Robotic Network (AERONET) version 3 at four sites in Indonesia representing fire prone areas (Palangka Raya, Pontianak, Jambi: 2012–2020), and urban-industrial (Bandung: 2009–2018). We examined the seasonal variation of aerosol optical depth (AOD), Angstrom Exponent (AE), Precipitable Water Vapor (PWV), and Single Scattering Albedo (SSA) combined with meteorological parameters at these Indonesian sites. Multiple clustering techniques from different relationships among various aerosol optical and radiative parameters was employed to further study the aerosol type in respect to different seasonality. The results exhibited a distinct seasonal pattern at all sites except Bandung, whereas AOD increased owing to forest and peat fire outbreaks during the dry season. The trend in AOD annual depicts an increase in Bandung as emission from urban/industrial increases episodically, while it depicts a decrease at the three biomass burning sites. As AOD increased, Palangka Raya, Pontianak, and Jambi exhibited wider ranges of observed AE (1.2–1.8) and high FMF (>0.8) in the dry burning period (June to October). On the other hand, Bandung has more aerosol distribution in the range of FMF values 0.6–1 and AE 1–1.6, compared with other sites, suggesting contribution of complex aerosol emission from different sources and likely due to the formation of secondary aerosol production from trace gases. Palangka Raya, Pontianak, and Jambi exhibited non-absorbing characteristics, as indicated by high SSA (>0.95), high FMF, and high EAE values (1.2–1.7) with no discrepancy in seasonal patterns, implying that biomass burning aerosols in Indonesia tend to cool the atmosphere with strong scattering rather than absorbing. At Bandung, aerosols mixed with slightly absorbing and non-absorbing aerosols owing to urban and industrial emissions. This study lays a foundation for further research on the contribution of aerosol radiative forcing to climate within the complex aerosol and cloud environments in Indonesia.

Aerosol optical depth↗
NASA NTRS2017

Impacts of Solar-Absorbing Aerosol Layers on the Transition of Stratocumulus to Trade Cumulus Clouds

The effects of an initially overlying layer of solar-absorbing aerosol on the transition of stratocumulus to trade cumulus clouds are examined using large-eddy simulations. For lightly drizzling cloud the transition is generally hastened, resulting mainly from increased cloud droplet number concentration (Nc) induced by entrained aerosol. The increased Nc slows sedimentation of cloud droplets and shortens their relaxation time for diffusional growth, both of which accelerate entrainment of overlying air and thereby stratocumulus breakup. However, the decrease in albedo from cloud breakup is more than offset by redistributing cloud water over a greater number of droplets, such that the diurnal-average shortwave forcing at the top of the atmosphere is negative. The negative radiative forcing is enhanced by sizable longwave contributions, which result from the greater cloud breakup and a reduced boundary layer height associated with aerosol heating. A perturbation of moisture instead of aerosol aloft leads to a greater liquid water path and a more gradual transition. Adding absorbing aerosol to that atmosphere results in substantial reductions in liquid water path (LWP) and cloud cover that lead to positive short-wave and negative longwave forcings on average canceling each other. Only for heavily drizzling clouds is the breakup delayed, as inhibition of precipitation overcomes cloud water loss from enhanced entrainment. Considering these simulations as an imperfect proxy for biomass burning plumes influencing Namibian stratocumulus, we expect regional indirect plus semi-direct forcings to be substantially negative to negligible at the top of the atmosphere, with its magnitude sensitive to background and perturbation properties.

Zhou, Xiaoli↗