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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 343 records · Page 19
All sourcesNASA NTRSDOE OSTI
NASA NTRS1992

Auroral X-ray imaging from high- and low-earth orbit

Observations of bremsstrahlung X-rays emitted by energetic electrons impacting the earth's atmosphere can be used for remotely sensing the morphology, intensity, and energy spectra of electron precipitation from the magnetosphere. Two auroral X-ray imagers, developed for future spaceflight, will be discussed. Polar Ionospheric X-ray Imaging Experiment is scheduled for launch on the NASA International Solar-Terrestrial Physics/Global Geospace Science program POLAR satellite in May, 1994. The POLAR orbit, with an apogee and perigee of 9 and 1.8 R(E) (earth radii), respectively, affords the opportunity to image the aurora from high altitude above the north pole continuously for several hours. The Magnetospheric Atmospheric X-ray Imaging Experiment is scheduled for launch aboard the NOAA-I satellite in late 1992. The 800-km polar orbit passes over both the northern and southern auroral zones every 101 minutes. The presentation emphasizes the experimental approaches used to exploit these very different orbits for remote sensing of the earth's auroral zones.

Mckenzie, D. L.↗
NASA NTRS1975

Differential spectra and phase space densities of trapped electrons at Jupiter

Using Pioneer 10 data, differential spectra and phase-space densities have been constructed for trapped electrons at Jupiter. These quantities should assist in calculating synchrotron radiation from these particles and in evaluating the diffusion mechanisms that accelerate the particles. Absorption by the moons Io and Europa is evident, and injection by Io is demonstrated by a density peak in phase space, which demands a local source. There is also a rapid decrease in density between the moons, which could call for either a local loss mechanism or nonlocal losses fed by diffusion.

Mcilwain, C. E.↗
NASA NTRS1985

Reestimation of the production spectra of cosmic ray secondary positrons and electrons in the ISM

A detailed calculation of the production spectra of charged hadrons produced by interactions of cosmic rays in the interstellar medium is presented along with a thorough treatment of pion and muon decays. Newly parameterized inclusive cross sections of hadrons were used and exact kinematic limitations were taken into account. Single parametrized expressions for the production spectra of both secondary positrons and electrons in the energy range .1 to 100 GeV are presented. The results are compared with other authors' predictions. Equilibrium spectra using various models are also presented.

Wong, C. M.↗
NASA NTRS1971

Rotational temperature determination in flowing nitrogen using an electron beam

The measurement of rotational temperature by the electron-beam fluorescence technique is investigated for temperatures between 78 K and 300 K by using the 0-0 band of the nitrogen first negative system. Existing methods for calculating the rotational temperature from electron-beam spectra result in values which are higher than the true temperature and the error increases with density and electron-beam current. The errors are believed to arise through neglect of the effects of secondary electrons. Excitation by low-energy secondary electrons can increase the population of the sparsely populated rotational ground states at the expense of the abundantly populated states. This secondary excitation is proposed as the cause of the error in the calculated rotational temperature and a theoretical study determines that the density and beam current govern the excitation rate. Rotational-temperature measurements are made in a flowing stream of nitrogen at a known temperature for a range of densities and beam currents.

Lillicrap, D. C.↗
DOE OSTI2025

Comparing Machine Learning and Physics-Based Nanoparticle Geometry Determinations Using Far-Field Spectral Properties

Anisotropic metal nanostructures exhibit polarization-dependent light scattering, a property which has been widely studied and exploited to determine orientations of subwavelength structures using far-field microscopy. Here we explore the use of variational autoencoders (VAEs) to determine the geometries of gold nanorods (NRs) such as in-plane orientation and aspect ratio under linearly polarized dark-field illumination in an optical microscope. We enforce a shared latent space to connect two VAEs trained separately with polarized dark-field scattering spectra and electron microscopy images and achieve image prediction (shape, orientation, and size) of Au NRs using only polarized dark-field scattering spectra. We determine the geometrical parameters of orientational angle and aspect ratio quantitatively via both our dual-VAE and physics-based analysis on the input scattering spectra. We show that orientational angle prediction by dual-VAE performs well with only a small (~300 particle) training set, yielding a mean absolute error (MAE) of 14.4° and a concordance correlation coefficient (CCC) of 0.95. This performance is only marginally worse than the physics-based cos(2?) fitting approach between the scattering intensity and the polarizing angle, which achieves MAE of 8.78° and CCC of 0.99. Aspect ratio determination is also comparable for the dual-VAE and physics-based fitting comparison (MAE of 0.21 vs. 0.23 and CCC of 0.53 vs. 0.68). Here, this dual encoder-decoder architecture effectively exploits the structure-property relationships of plasmonic nanostructures to construct a cross-modal machine learning (ML) approach, providing a pathway to employ ML approaches to address other structure-property relationships in materials science.

Dark-field scattering↗
DOE OSTI2022

Surface analysis insight note: Differentiation methods applicable to noisy data for determination of sp2‐ versus sp3‐hybridization of carbon allotropes and AES signal strengths

The derivatives of the spectra are commonly used for quantification in Auger Electron Spectroscopy (AES) spectra, while the derivative of the KLL C Auger line has proven to be valuable in obtaining a measure of the relative proportions of sp 2 ‐ and sp 3 ‐hybridization using the D‐parameter in both AES and X‐ray Photoelectron Spectroscopy (XPS). Differentiation of X‐ray Photoelectron Spectroscopy (XPS) and Auger Electron Spectroscopy (AES) spectra by numerical means is presented and illustrated for polymeric, such as PEEK and Nylon, as well as for graphitic materials including highly ordered pyrolytic graphite and graphene oxide. The most commonly available Savitzky–Golay method is explained mathematically and developed through the case of constructing a 5‐point quadratic polynomial convolution kernel suitable for differentiating spectra of adequate signal to noise. The concept of differentiation of spectra where signal to noise is less than adequate is also developed. Two alternative strategies to Savitzky–Golay differentiation are presented, which fit curves to data that allow derivatives to be obtained where Savitzky–Golay would otherwise fail. These alternative methods involve constructing a parametric curve that fits data over the entire energy interval of interest. Derivatives of spectra are then obtained by differentiating these parametric curves directly. A comparison of results for different materials for which specific sp 2 ‐ vs sp 3 ‐hybridized carbon proportions are of interest is used to emphasize the importance of characterizing methods used to differentiate spectra and understanding the characteristics of instrumentation used to measure spectra. The case for using Principal Component Analysis noise reduction with C KLL spectra is made for spectra collected from a heterogeneous graphene oxide sample.

Fairley, Neal↗
DOE OSTI2022

Resonant double-core excitations with ultrafast, intense X-ray pulses

Intense few-to-sub-femtosecond soft X-ray pulses can produce neutral, two-site excited double-core-hole states by promoting two core electrons to the same unoccupied molecular orbital. We theoretically investigate double nitrogen K-edge excitations of nitrous oxide (N$_2$O) with multiconfigurational electronic structure calculations. We show that the second core-excitation energy is reduced with respect to its ground state value. A site-selective double core-excitation mechanism using intense few-femtosecond x-rays is investigated using time-dependent Schrodinger equation (TDSE) simulations. The subsequent two-step Auger-Meitner and two-electrons-one-electron decay spectra of the double core-excited states are analysed using a Mulliken population analysis of the multiconfirational wavefunctions. The change in the electron emission lineshape between the absorption of 1 or 2 photons in the resonant core-excitation is predicted by combining this approach with the TDSE simulations. Furthermore, we examine the possibility of resolving the double core-excited states with X-ray pump-probe techniques by calculating the chemical shifts of the core-electron binding energy of the core-excited states and decay products.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1993

PET - A proton/electron telescope for studies of magnetospheric, solar, and galactic particles

The Proton/Electron Telescope (PET) on SAMPEX is designed to provide measurements of energetic electrons and light nuclei from solar, galactic, and magnetospheric sources. PET is an all solid-state system that will measure the differential energy spectra of electrons from about 1 to about 30 MeV and H and He nuclei from about 20 to about 300 MeV/nuc, with isotope resolution of H and He extending from about 20 to about 80 MeV/nuc. As SAMPEX scans all local times and geomagnetic cutoffs over the course of its near-polar orbit, PET will characterize precipitating relativistic electron events during periods of declining solar activity, and it will examine whether the production rate of odd nitrogen and hydrogen molecules in the middle atmosphere by precipitating electrons is sufficient to affect O3 depletion. In addition, PET will complement studies of the elemental and isotopic composition of energetic heavy (Z greater than 2) nuclei on SAMPEX by providing measurements of H, He, and electrons. Finally, PET has limited capability to identify energetic positrons from potential natural and man-made sources.

Cook, Walter R.↗
NASA NTRS1986

Density fluctuations in the interstellar medium: Evidence for anisotropic magnetogasdynamic turbulence. II - Stationary structures

A model of anisotropic, plasma-fluid variations was used to investigate the unknown origin of the power spectra of interstellar electron fluctuations inferred by Armstrong, Cordes, and Rickett (1981). The modeled electron variations are interpreted as density components of an anisotropic stationary mode of nonlinear magnetogasdynamics-tangential pressure balances. It is suggested that the wavenumber spectra of electron variations are identical to the spectra of the convecting velocity fields over a wide range of wavenumbers.

Higdon, J. C.↗
NASA NTRS2006

Laboratory Spectroscopy of Large Carbon Molecules and Ions in Support of Space Missions. A New Generation of Laboratory & Space Studies

Polycyclic Aromatic Hydrocarbons (PAHs) are an important and ubiquitous component of carbon-bearing materials in space. A long-standing and major challenge for laboratory astrophysics has been to measure the spectra of large carbon molecules in laboratory environments that mimic (in a realistic way) the physical conditions that are associated with the interstellar emission and absorption regions [1]. This objective has been identified as one of the critical Laboratory Astrophysics objectives to optimize the data return from space missions [2]. An extensive laboratory program has been developed to assess the properties of PAHs in such environments and to describe how they influence the radiation and energy balance in space. We present and discuss the gas-phase electronic absorption spectra of neutral and ionized PAHs measured in the UV-Visible-NIR range in astrophysically relevant environments and discuss the implications for astrophysics [1]. The harsh physical conditions of the interstellar medium characterized by a low temperature, an absence of collisions and strong VUV radiation fields - have been simulated in the laboratory by associating a pulsed cavity ringdown spectrometer (CRDS) with a supersonic slit jet seeded with PAHs and an ionizing, penning-type, electronic discharge. We have measured for the {\it first time} the spectra of a series of neutral [3,4] and ionized [5,6] interstellar PAHs analogs in the laboratory. An effort has also been attempted to quantify the mechanisms of ion and carbon nanoparticles production in the free jet expansion and to model our simulation of the diffuse interstellar medium in the laboratory [7]. These experiments provide {\it unique} information on the spectra of free, large carbon-containing molecules and ions in the gas phase. We are now, for the first time, in the position to directly compare laboratory spectral data on free, cold, PAH ions and carbon nano-sized carbon particles with astronomical observations in the UV-NIR range (interstellar UV extinction, DIBs in the NUV-NIR range). This new phase offers tremendous opportunities for the data analysis of current and upcoming space missions geared toward the detection of large aromatic systems Le., the "new frontier space missions" (Spitzer, HST, COS, JWST, SOFIA,...).

Salama, Farid↗
NASA NTRS1968

On auroral electrons.

Rocket studies of energy spectra of primary auroral electrons, giving model for auroral display

Evans, D. S.↗
NASA NTRS1972

Electron impact excitation cross sections and energy degradation in CO.

We determine a comprehensive set of electron impact cross sections for carbon monoxide mainly on the basis of recently accumulated data on electron impact spectra, the Born approximation at high energies, and simple rules developed earlier to take into account low-energy effects. The calculation of the complete energy degradation of electrons incident on CO is carried out with these input cross sections, and the efficiencies associated with possible loss channels are presented.

Sawada, T.↗
NASA NTRS2002

On the Consistency of Gamma-Ray Burst Spectral Indices with the Synchrotron Shock Model

The current scenario for gamma-ray bursts (GRBs) involves internal shocks for the prompt GRB emission phase and external shocks for the afterglow phase. Assuming optically thin synchrotron emission from isotropically distributed energetic shocked electrons, GRB spectra observed with a low-energy power-law spectral index greater than -2/3 (for positive photon number indices E(exp alpha) indicate a problem with this model. For spectra that do not violate this condition, additional tests of the shock model can be made by comparing the low- and high-energy spectral indices, on the basis of the model's assertion that synchrotron emission from a single power-law distribution of electrons is responsible for both the low-energy and the high-energy power-law portions of the spectra. We find in most cases that the inferred relationship between the two spectral indices of observed GRB spectra is inconsistent with the constraints from the simple optically thin synchrotron shock emission model. In this sense, the prompt burst phase is different from the afterglow phase, and this difference may be related to anisotropic distributions of particles or to their continual acceleration in shocks during the prompt phase.

Preece, R. D.↗
NASA NTRS1975

Observations of Jovian accelerated particles both inside and outside the Jovian magnetosphere - Results from the Goddard-U. of New Hampshire experiment on Pioneer 10

This paper discusses measurements of the energetic-particle population inside Jupiter's magnetosphere as well as observations of energetic particles in interplanetary space that have escaped from that magnetosphere. The discussion is based on Pioneer 10 data obtained when the spacecraft was outside the bow shock but within about 1 AU of the planet and on electron data obtained near earth by various IMP spacecraft. Pioneer 10 particle measurements in the Jovian magnetosphere are reviewed, the differential proton and electron energy spectra are described, and it is suggested that very little particle acceleration occurs in the outer magnetosphere. Additional data are examined in regard to Jovian alpha particles, proton and electron angular distributions, protons in the inner magnetosphere, effects of Io on the proton flux, electron acceleration outside the bow shock, and observations of Jovian electrons near earth. All these data are shown to support the conclusion that most, if not all, quiet-time increases in low-energy electron fluxes near earth are of Jovian origin.

Trainor, J. H.↗