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At least 343 records · Page 19

Space radiation studies for the reporting period, June 1983 - July 1984

Two Active Radiation Dosimeters (ARD's) flown on Spacelab 1, performed without fault and were returned to Space Science Laboratory, MSFC for recalibration. During the flight in December 1983, performance was monitored at the Huntsville Operations Center (HOSC). Despite some problems with the Shuttle data system handling the VFI, it could be established that the ARD's were operating normally. Postflight calibrations of both units determined that sensitivities were essentially unchanged from preflight values. Flight tapes were received for approximately 60% of the flight and it appears that this is the total available. The next phase of effort will involve close collaboration with Space Science Laboratory, MSFC, in the analysis of this data. The Nuclear Radiation Monitor (NRM) was under assembly and testing at MSFC. Support was rendered in the areas of materials control and parts were supplied for the supplementary heaters, dome gas-venting device and photomultiplier tube housing. Performance characteristics of some flight-space photomultipliers were measured.

Source record↗

Chemical Pre-Treatment of used Fuel for Long–Term Storage

Repository programs throughout the world have been slowed by the need for increased local public involvement in the siting and licensing process. The result has been an increase in the dry storage of used fuel at reactor sites and the potential that such storage may be extended for many decades, even centuries. While there are sound technical reasons to believe that dry storage can be conducted safely, there are increasing concerns that the ultimate transfer to either a future repository or a centralized separations plant may result in fractured cladding and serious handling issues, including criticality concerns. These concerns would be increased for higher burn-up fuels. Currently, various chemical pre-treatment processes under R&D for application to commercial used oxide fuel have been investigated at the laboratory scale as methods to simplify and increase the safety of the remaining stages of conventional solvent extraction processing. This includes advanced decladding methods and various oxidation/reduction processes designed to release volatile and semi-volatile fission products, produce finely divided uranium oxide powder, and ameliorate the subsequent nitric acid dissolution step. The paper examines the potential for combining several chemical and physical pre-treatment steps to minimize long-term concerns about safe transport of used fuel, possibly providing another option for future nuclear waste management. Laboratory data from both cold and hot testing will provide the basis for the evaluation. An example of a potential pre-treatment process includes shearing, advanced voloxidation and off-gas treatment, the possible mixing of the resulting uranium oxide with a secondary oxide, and densification and recanning in nitric acid-soluble storage containers for extended time periods. Chemical decladding may be feasible to replace shearing. Zirconium recycle may also be feasible, significantly reducing high level waste quantities. Both analytic and experimental data will be applied to the examination of this potential fuel cycle option.

Bresee, James↗

System Thermal-Hydraulic Modeling of the Phénix Dissymmetric Test Benchmark

Phénix is a French pool-type sodium-cooled prototype reactor; before the definitive shutdown, occurred in 2009, a final set of experimental tests are carried out in order to increase the knowledge on the operation and the safety aspect of the pool-type liquid metal-cooled reactors. One of the experiments was the Dissymmetric End-of-Life Test which was selected for the validation benchmark activity in the frame of SESAME project. The computer code validation plays a key role in the safety assessment of the innovative nuclear reactors and the Phénix dissymmetric test provides useful experimental data to verify the computer codes capability in the asymmetric thermal-hydraulic behaviour into a pool-type liquid metal-cooled reactor. This paper shows the comparison of the outcomes obtained with six different System Thermal-Hydraulic (STH) codes: RELAP5-3D©, SPECTRA, ATHLET, SAS4A/SASSYS-1, ASTEC-Na and CATHARE. The nodalization scheme of the reactor was individually achieved by the participants; during the development of the thermal-hydraulic model, the pool nodalization methodology had a special attention in order to investigate the capability of the STH codes to reproduce the dissymmetric effects which occurs in each loop and into pools, caused by the azimuthal asymmetry of the boundary conditions. The modelling methodology of the participants is discussed and the main results are compared in this paper to obtain useful guide lines for the future modelling of innovative liquid metal pool-type reactors.

Narcisi, V.↗

Thermal Evolution near Heat-Generating Nuclear Waste Canisters Disposed in Horizontal Drillholes

We consider the disposal of spent nuclear fuel and high-level radioactive waste in horizontal holes drilled into deep, low-permeable geologic formations using directional drilling technology. Residual decay heat emanating from these waste forms leads to temperature increases within the drillhole and the surrounding host rock. The spacing of waste canisters and the configuration of the various barrier components within the horizontal drillhole can be designed such that the maximum temperatures remain below limits that are set for each element of the engineered and natural repository system. We present design calculations that examine the thermal evolution around heat-generating waste for a wide range of material properties and disposal configurations. Moreover, we evaluate alternative layouts of a monitoring system to be part of an in situ heater test that helps determine the thermal properties of the as-built repository system. A data-worth analysis is performed to ensure that sufficient information will be collected during the heater test so that subsequent model predictions of the thermal evolution around horizontal deposition holes will reliably estimate the maximum temperatures in the drillhole. The simulations demonstrate that the proposed drillhole disposal strategy can be flexibly designed to ensure dissipation of the heat generated by decaying nuclear waste. Moreover, an in situ heater test can provide the relevant data needed to develop a reliable prediction model of repository performance under as-built conditions.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Measurement of Charged-Pion Production in Deep-Inelastic Scattering off Nuclei with the CLAS Detector

Background: Energetic quarks in nuclear deep-inelastic scattering propagate through the nuclear medium. Processes that are believed to occur inside nuclei include quark energy loss through medium-stimulated gluon bremsstrahlung and intranuclear interactions of forming hadrons. More data are required to gain a more complete understanding of these effects. Purpose: To test the theoretical models of parton transport and hadron formation, we compared their predictions for the nuclear and kinematic dependence of pion production in nuclei. Methods: We have measured charged-pion production in semi-inclusive deep-inelastic scattering off D, C, Fe, and Pb using the CLAS detector and the CEBAF 5.014-GeV electron beam. We report results on the nuclear-to-deuterium multiplicity ratio for π + and π - as a function of energy transfer, four-momentum transfer, and pion energy fraction or transverse momentum—the first three-dimensional study of its kind. Results: The π + multiplicity ratio is found to depend strongly on the pion fractional energy z and reaches minimum values of 0.67 ± 0.03, 0.43 ± 0.02, and 0.27 ± 0.01 for the C, Fe, and Pb targets, respectively. The z dependencies of the multiplicity ratios for π + and π - are equal within uncertainties for C and Fe targets but show differences at the level of 10% for the Pb-target data. The results are qualitatively described by the GIBUU transport model, as well as with a model based on hadron absorption, but are in tension with calculations based on nuclear fragmentation functions. Conclusions: These precise results will strongly constrain the kinematic and flavor dependence of nuclear effects in hadron production, probing an unexplored kinematic region. They will help to reveal how the nucleus reacts to a fast quark, thereby shedding light on its color structure and transport properties and on the mechanisms of the hadronization process.

Moran, S.↗

Post-Irradiation Examination of Zircaloy-4 Samples in Target Capsules and Initiation of Bending Fatigue Testing for Used Nuclear Fuel Vibration Integrity Investigations (FY 2013 Summary Report)

This report documents ongoing work performed at Oak Ridge National Laboratory (ORNL) for the Department of Energy, Office of Fuel Cycle Technology Used Fuel Disposition Campaign (UFDC), and satisfies the deliverable for milestone M2FT-13OR0805041, “Data Report on Hydrogen Doping and Irradiation in HFIR.” This work is conducted under WBS 1.02.08.05, Work Package FT-13OR080504 ST “Storage and Transportation-Experiments – ORNL.” The objectives of work packages that make up the S&T Experiments Control Account are to conduct the separate effects tests (SET) and small-scale tests that have been identified in the Used Nuclear Fuel Storage and Transportation Data Gap Prioritization (FCRD-USED-2012-000109). In FY 2013, the R&D focused on cladding and container issues and small-scale tests as identified in Sections A-2.9 and A-2.12 of the prioritization report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

OSIRIS Validation and Verification Report

The On-Site Inspection RadioIsotopic Spectroscopy (OSIRIS) system is a gamma-ray spectroscopy instrument for on-site inspections conducted under the Comprehensive Nuclear-Test-Ban Treaty (CTBT). The OSIRIS software filters spectral analysis data, revealing information to users on only 17 CTBT-relevant fission-product isotopes. In this report, we review the CTBT requirements for on-site inspection radionuclide identifiers, plus additional requirements imposed by the design team. Then a series of validation tests conducted during OSIRIS development are described. The validation tests were designed to gauge if the nascent OSIRIS system met those requirements. We conclude with a set of recommended verification tests to ensure that newly-manufactured OSIRIS systems also will meet the requirements.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

An Overview in the Development of a Multi-Sensor Data Science System for Monitoring a Solvent Extraction Process

To enhance nuclear nonproliferation stewardship, Idaho National Laboratory is building the Beartooth nuclear fuel cycle processing test bed. The Beartooth test bed will allow researchers the opportunity to study nuclear fuel processing operations including the use of centrifugal contactors in solvent extraction processes. The test bed is designed to support data collection and machine learning to monitor process operations. As part of this project, researchers will study data collected from a host of sensors that have not been typically used to monitor solvent extraction processes such as vibration, acoustic, colormetric, and thermal measurement data. The goal of this research is to employ machine learning and data analytics to study the confluence of signals collected from both traditionally and non-traditionally used sensors to provide operator process awareness and discover process anomalies. An overview of planned sensors and experiments that will focus on signal discovery will be presented.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

An Overview in the Development of a Multi-Sensor Data Science System for Monitoring a Solvent Extraction Process

To enhance nuclear nonproliferation stewardship, Idaho National Laboratory is building the Beartooth nuclear fuel cycle processing test bed. The Beartooth test bed will allow researchers the opportunity to study nuclear fuel processing operations including the use of centrifugal contactors in solvent extraction processes. The test bed is designed to support data collection and machine learning to monitor process operations. As part of this project, researchers will study data collected from a host of sensors that have not been typically used to monitor solvent extraction processes such as vibration, acoustic, colormetric, and thermal measurement data. The goal of this research is to employ machine learning and data analytics to study the confluence of signals collected from both traditionally and non-traditionally used sensors to provide operator process awareness and discover process anomalies. An overview of planned sensors and experiments that will focus on signal discovery will be presented.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

BAYESIAN CALIBRATION OF SAFETY CODES USING DATA FROM SEPARATE-AND INTEGRAL EFFECTS TESTS

Large-scale system codes for simulation of safety performance of nuclear plants may contain parameters whose values are not known very accurately. In order to be able to use the results of these simulation codes with confidence, it is important to learn how the uncertainty on the values of these parameters affects the output of the codes. New information from tests or operating experience is incorporated into safety codes by a process known as calibration, which reduces uncertainty in the output of the safety code, and thereby improves its support for decision-making. Modern analysis capabilities afford very significant improvements on classical ways of doing calibration, and the work reported here implements some of those improvements. The key innovation has come from development of safety code surrogate model (code emulator) construction and prediction algorithms. A surrogate is needed for calibration of plant-scale simulation codes because the multivariate nature of the problem (i.e., the need to adjust multiple uncertain parameters at once to fit multiple pieces of new information) calls for multiple evaluations of performance, which, for a computation-intensive model, makes calibration very computation-intensive. Use of a fast surrogate makes the calibration processes used here with Markov Chain Monte Carlo (MCMC) sampling feasible. Moreover, most traditional surrogates do not provide uncertainty information along with their predictions, but the Gaussian Process (GP) based code surrogates used here do. This improves the soundness of the code calibration process. Results are demonstrated on a simplified scenario with data from Separate and Integral Effect Tests.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Measurements of Neutron Importance Distribution in {sup 235}U Fast Critical Reactor

The reactor physics related integral experiments are significant to criticality safety analysis and the design of the next generation nuclear system. Measurements of parameters such as prompt neutron decay constant α, prompt neutron generation time Λ, effective delayed neutron fraction β{sub eff}, neutron importance distribution, etc., can provide data for the verification of calculation methods, computer codes and cross-section data in criticality safety analysis and test the design of new reactors. Among these parameters, neutron importance distribution has its unique value. Beside verification and validation of nuclear data, computer codes, and simulation methods, the experimental results of neutron importance distribution are also useful to the correcting of the spatial effects in Rossi-α measurement, which is based on point-reactor neutron kinetics. The relative neutron importance distribution experiments were performed on the {sup 235}U fast critical reactor of China Academy of Engineering Physics (CAEP). The key experimental objective was to obtain the importance distribution data for nuclear data validation and criticality safety analysis. We demonstrate in this paper the experiment and the data analysis. {sup 252}Cf neutron importance spatial distributions in the diametral hole of a depleted uranium reflected {sup 235}U fast critical reactor were measured. The evaluated uncertainties of the experiment data were varying with the source location but within 1.5% ranges in all. The experiment results can provide useful data for applications like nuclear data validation and the determination of rectification factor R of Rossi-a measurements. However, the experimental uncertainties are not satisfying and can be further reduced by using a {sup 252}Cf source with much higher intensity, recording more precisely the absolute position of the neutron source, and carrying out the experiment in more shallow subcritical states in which the system multiplication is larger. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Systematic muon capture rates in PQRPA

In this work we performed a systematic study of the inclusive muon capture rates for several nuclei with A < 60 using the Projected Random Quasi-particle Phase Approximation (PQRPA) as nuclear model, because it is the only RPA model that treats the Pauli Principle correctly. We reckon that the comparison between theory and data for the inclusive muon capture is not a fully satisfactory test on the nuclear model that is used. The exclusive muon transitions are more robust for such a purpose.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

TREAT neutronics analysis and design support, Part I: Multi-SERTTA

Experiment vehicle design is necessary in preparation for Transient Reactor Test (TREAT) facility restart and the resumption of transient testing to support Accident Tolerant Fuel (ATF) characterization and other future fuels testing requirements. Currently the most mature vehicle design is the Multi-SERTTA (Static Environments Rodlet Transient Test Apparatuses), which can accommodate up to four concurrent rodlet-sized specimens under separate environmental conditions. Robust test vehicle design requires neutronics analyses to support design development, optimization of the power coupling factor (PCF) to efficiently maximize energy generation in the test fuel rodlets, and experiment safety analyses. Calculations were performed to support analysis of a near-final design of the Multi-SERTTA vehicle, the design process for future TREAT test vehicles, and establish analytical practices for upcoming transient test experiments. Models of the Multi-SERTTA vehicle containing typical PWR-fuel rodlets were prepared and neutronics calculations were performed using MCNP6.1 with ENDF/B-VII.1 nuclear data libraries. Calculation of the PCF for reference conditions of a PWR fuel rodlet in clean water at operational temperature and pressure provided results between 1.10 and 1.73 W/g-MW depending on the location of the four Multi-SERTTA units with the stack. Basic changes to the Multi-SERTTA secondary vessel containment and support have minimal impact on PCF; using materials with less neutron absorption can improve expected PCF values, especially in the primary containment. An optimized balance is needed between structural integrity, experiment safety, and energy deposition in the experiment. Type of medium and environmental conditions within the primary vessel surrounding the fuel rodlet can also have a significant impact on resultant PCF values. The estimated reactivity insertion worth into the TREAT core is impacted more by the primary and secondary Multi-SERTTA vehicle structure with the experiment content and contained environment having a near negligible impact on overall system reactivity. Additional calculations were performed to evaluate the peak-to-average assembly powers throughout the TREAT core, as well as the nuclear heat generation for the various structural components of the Multi-SERTTA assembly. Future efforts include the evaluation of flux collars to shape the PCF for individual Multi-SERTTA units during an experiment such as to achieve uniformity in test unit environmental conditions impacted by the non-uniform axial flux/power profile of TREAT. Upon resumption of transient testing, experimental results from both the Multi-SERTTA and Multi-SERTTA-CAL will be compared against calculational results and methods for further optimization and design strategies. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGR-1 Thermocouple Data Analysis

This report documents an effort to analyze measured and simulated data obtained in the Advanced Gas Reactor (AGR) fuel irradiation test program conducted in the INL's Advanced Test Reactor (ATR) to support the Next Generation Nuclear Plant (NGNP) R&D program. The work follows up on a previous study (Pham and Einerson, 2010), in which statistical analysis methods were applied for AGR-1 thermocouple data qualification. The present work exercises the idea that, while recognizing uncertainties inherent in physics and thermal simulations of the AGR-1 test, results of the numerical simulations can be used in combination with the statistical analysis methods to further improve qualification of measured data. Additionally, the combined analysis of measured and simulation data can generate insights about simulation model uncertainty that can be useful for model improvement. This report also describes an experimental control procedure to maintain fuel target temperature in the future AGR tests using regression relationships that include simulation results. The report is organized into four chapters. Chapter 1 introduces the AGR Fuel Development and Qualification program, AGR-1 test configuration and test procedure, overview of AGR-1 measured data, and overview of physics and thermal simulation, including modeling assumptions and uncertainties. A brief summary of statistical analysis methods developed in (Pham and Einerson 2010) for AGR-1 measured data qualification within NGNP Data Management and Analysis System (NDMAS) is also included for completeness. Chapters 2-3 describe and discuss cases, in which the combined use of experimental and simulation data is realized. A set of issues associated with measurement and modeling uncertainties resulted from the combined analysis are identified. This includes demonstration that such a combined analysis led to important insights for reducing uncertainty in presentation of AGR-1 measured data (Chapter 2) and interpretation of simulation results (Chapter 3). The statistics-based simulation-aided experimental control procedure described for the future AGR tests is developed and demonstrated in Chapter 4. The procedure for controlling the target fuel temperature (capsule peak or average) is based on regression functions of thermocouple readings and other relevant parameters and accounting for possible changes in both physical and thermal conditions and in instrument performance.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

ANS Winter 2024 Summary: Optimizing the ATF-2Ramp Power Profile

When the Halden Boiling Water Reactor closed down in 2018, a need to restore the capability for in-reactor power ramp testing arose. Such testing is valuable for studying pellet-clad interaction phenomena in nuclear fuels. The data from these studies is of great interest to a number of research programs, including the accident-tolerant fuel (ATF) program at Idaho National Laboratory (INL). In 2022, Woolstenhulme et al. proposed several power ramp testing ideas using facilities at INL, including irradiation in the Transient Reactor Test Facility (better known as TREAT) and the Advanced Test Reactor (ATR) [1]. Worrall et al. [2] and Labossiere-Hickman et al. [3] subsequently performed feasibility studies for the ATR testing options in 2023. This summary further investigates the three-pin trefoil design (Fig. 1) for the proposed ATF-2Ramp Experiment discussed in Labossiere-Hickman et al. [3]. ATF-2Ramp is designed to operate in the center flux trap (CFT) of the ATR during a powered axial locator mechanism (PALM) cycle: a short, variable-powered cycle with an asymmetric power distribution. Previously, it was shown that tailoring the thickness of the hafnium (Hf) neutron shields (“mini-shrouds”) surrounding each pin offered a degree of control sufficient to achieve the programmatic linear heat generation rate (LHGR) targets for ATF-2Ramp during the high-power period of a PALM cycle. New work involves shortening the experiment test train for consistency with the fuel pins in ATF-2D [4] and then shaping the axial power profile of the three test pins.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Energy Dependent Fission Product Yields (2nd year Milestone and Deliverables)

Introduction to the project: One of the Laboratory missions is to provide consistent, high-precision fission product; yield data critical for testing fission models and maintaining the safety and security of the nation’s nuclear weapons stockpile. However, high-quality, energy-differential fission product yield data is missing for certain actinides and neutron energies important to constrain the new U.S. Nuclear Data Program evaluation effort; It has been shown that the reactor antineutrino anomaly may be at least partially caused by roughly 20 fission products. The fission product yield data is missing or incomplete for many of these isotopes, thus it is necessary to accurately determine these values to better constrain the anomaly; Aitor Bracho is measuring very short-lived (seconds to minutes) fission product yields of 235 U and 239 Pu using monoenergetic neutron beams at E n = 60 and 560 keV; Aitor Bracho is using a direct approach utilizing a state-of-the-art rabbit transfer system, superior HPGe detector, and digital acquisition systems for fission decay measurements. The goals of this project: lop experimental capabilities and data analysis techniques to carry out the gamma-ray spectra analysis necessary for fission product yield calculation; Provide high-precision and energy-dependent fission product data supporting fission theory, neutrino physics, and applied physics.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Testing nuclear parton distributions with pA collisions at the TeV scale

Global perturbative QCD analyses, based on large data sets from electron-proton and hadron collider experiments, provide tight constraints on the parton distribution function (PDF) in the proton. The extension of these analyses to nuclear parton distribution functions (nPDFs) has attracted much interest in recent years. nPDFs are needed as benchmarks for the characterization of hot QCD matter in nucleus-nucleus collisions, and attract further interest since they may show novel signatures of nonlinear density-dependent QCD evolution. However, it is not known from first principles whether the factorization of long-range phenomena into process-independent parton distribution, which underlies global PDF extractions for the proton, extends to nuclear effects. As a consequence, assessing the reliability of nPDFs for benchmark calculations goes beyond testing the numerical accuracy of their extraction and requires phenomenological tests of the factorization assumption. Here, we argue that a proton-nucleus collision program at the Large Hadron Collider would provide a set of measurements, which allow for unprecedented tests of the factorization assumption, underlying global nPDF fits.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Light Elements $R$-matrix Analyses with the SAMMY code towards the Foundation of Charged-particle Nuclear Data Libraries [Slides]

This presentation covers newly developed SAMMY module for inverse channel transformation. Additionally covered is the R-matrix analysis of 7 Be compound nucleus and the R-­matrix analysis of 17 O compound nucleus. Further touched on is the evaluated Nuclear Data File generation and processing with the AMPX code. The presentation concludes with talks on future evaluation work and tests on light nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗