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NASA NTRS2017

PM2.5 Variation Related to AOD and Meteorological Conditions on Diurnal Scale in Beijing, China

PM2.5 (particulate matter with diameter less than 2.5um) is one of the major air pollutants in many regions around the globe. Column integrated aerosol optical depth (AOD) measurement provides a potential way to estimate surface PM2.5 concentration from the remote sensing technics. In this analysis, we compiled hourly measurements of surface PM2.5 and AOD made in Beijing, China and meteorological conditions provided by NASA Global Modeling and Assimilation Office's Modern-Era Retrospective Analysis for Research and Applications (MERRA) product in recent years. On daily basis, hourly PM2.5 and AOD show positive correlation, i.e. correlation coefficient (R) is higher than 0.5 on about 50% of days. We apply multi-variant analysis to this dataset and estimate the magnitude of AOD variance that can be explained by or related to PM2.5 and relevant meteorological conditions changes.

PM2.5↗

NASA NTRS2019

Near Real-Time Global Composition Forecasts at 25km Horizontal Resolution

We present a new high-resolution global composition forecast system produced by NASA's Global Modeling and Assimilation Office. The NASA Goddard Earth Observing System (GEOS) model has been expanded to provide global near-real-time 5-day forecasts of atmospheric composition at unprecedented horizontal resolution of 0.25 degrees (~25 km). This composition forecast system (GEOS-CF) system combines the operational GEOS weather forecasting model with the state-of-the-science GEOS-Chem chemistry module (version 12) to provide detailed analysis of a wide range of air pollutants such as ozone, carbon monoxide, nitrogen oxides, and fine particulate matter (PM2.5). Satellite observations are assimilated into the system for improved representation of weather and smoke.

Knowland, K. Emma↗

NASA NTRS2019

Near Real-Time Air Quality Forecasts Using the NASA GEOS Model

Knowland, K. Emma↗

NASA NTRS2019

Near Real-Time Air Quality Forecasts Using the NASA GEOS Model

Knowland, K. Emma↗

NASA NTRS2019

Further Characterization of Aerosols Sampled on the International Space Station

Spacecraft cabin air quality is of fundamental importance to crew health, with concerns encompassing both gaseous contaminants and airborne particles. Quantification of spacecraft indoor aerosols will increase our understanding of crew exposure and cabin cleanliness. Aerosols on the International Space Station (ISS) have been sampled and brought back to Earth for analysis to characterize the airborne particulate matter in the cabin. Microscopic analyses have been performed to determine morphology and particle size information, and Energy Dispersive X-ray Spectroscopy (EDS) provides information on the chemical elements present in the particles. With the use of IntelliSEM software for computer-controlled scanning electron microscopy (CCSEM), this data provides particle size distribution information and statistics on particle materials. Many of the particles collected were made up of multiple elements and had uncommon morphologies compared to typical indoor aerosols on Earth. These characteristics are thought to be from unique formation mechanisms in the microgravity environment. Several notable particle types are examined further in this work. Bromine-containing particles and cadmium-containing particles are discussed as they constitute a health hazard to crew members. Humans in indoor living and working spaces are typically the single largest particle emission source, and this was observed in the sampled aerosols in ISS as well.

Sampling↗

NASA NTRS2019

Air Pollution Forecasts Using the NASA GEOS Model: A Unified Tool from Local to Global Scales

Knowland, K. Emma↗

NASA NTRS2017

The MERRA-2 Aerosol Reanalysis, 1980 Onward. Part II: Evaluation and Case Studies

The Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2) is NASA’s latest reanalysis for the satellite era (1980-present) using the Goddard Earth Observing System version 5 (GEOS-5) Earth system model. MERRA-2 provides several improvements over its predecessor (MERRA), including the inclusion of interactive aerosols for the entire period. In addition to assimilating bias-corrected Aerosol Optical Depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) on the Terra and Aqua satellites, it also includes the assimilation of bias-corrected AOD from Advanced Very High Resolution Spectroradiometer (AVHRR) instruments, Multi-angle Imaging SpectroRadiometer (MISR) AOD over bright surfaces, and ground-based Aerosol Robotic Network (AERONET) AOD. This paper is the second of a pair that summarizes our efforts to assess the quality of the MERRA-2 aerosol assimilation. In this study, we first follow previous work performed with version 1 of the MERRA Aerosol Reanalysis (MERRAero) using independent observations. The evaluation of MERRA-2 Absorption Aerosol Optical Depth (AAOD) and ultra-violet Aerosol Index (UV-AI) against the Ozone Monitoring Instrument (OMI) observations show good agreement, particularly over dusty regions where our previous efforts improved model aerosol optical properties. Next, we find that aerosol assimilation system improves the aerosol vertical structure when compared to estimates from the same version of the model without AOD assimilation. A similar conclusion is found for MERRA-2 aerosol surface fine particulate matter (PM (sub 2.5)). However, deficiencies in the forward model such as missing emissions noted during the MERRAero study still explain the MERRA-2 PM(sub 2.5) bias relative to observations over the United States. Finally, to illustrate successes and weaknesses of the AOD assimilation, we focus on the performance of the MERRA-2 aerosol system during several major aerosol events: the Mount Pinatubo eruption in 1991, a Saharan dust event and transportation over the Atlantic Ocean during April 2010, the Rim Fire of summer 2013 in California, and an extreme pollution event over China in January 2013. We conclude with a summary that points to best practices for utilizing the MERRA-2 aerosol reanalysis in future studies.

V Buchard↗

NASA NTRS2019

File Specification for GEOS-CF Products

The NASA Global Earth Observing System (GEOS) model has been expanded to provide global near-real-time forecasts of atmospheric composition at a horizontal resolution of 0.25 degrees (about 25 km). This GEOS Composition Forecast (GEOS-CF) system combines the GEOS weather analysis and forecasting system with the state-of-the-science GEOS-Chem chemistry module (Bey et al., 2001; Keller et al., 2014; Long et al., 2015) to provide detailed chemical analysis of a wide range of air pollutants including ozone, carbon monoxide, nitrogen oxides, and fine particulate matter (PM2.5).

Knowland, Katherine E.↗

NASA NTRS2019

Developing an Air Quality Index for Microgravity Indoor Environments/Space Missions

Indoor pollution sources (on Earth) that release gases or particles into the air are the primary cause of air quality problems in indoor environments. The development of an adequate tool to understand pollution levels in a certain location is of high importance. This tool must be able to inform about the levels of pollution in a simple and understandable way but also, used to take a series of predetermined measures to protect the health of the exposed population. One of the most useful and up to date approaches for characterizing air pollution is the Air Quality Index (AQI). It is an easily-calculated powerful data-driven tool, that summarizes a complex phenomenon, such as air pollution, in straightforward indicators. The AQI system has been developed in different countries around the world, mainly for outdoor environments, based on the results of risk assessments, epidemiology studies, and current local air pollution regulations and standards.Air quality in microgravity indoor environments is of fundamental importance to crew health, with concerns encompassing both gaseous contaminants and particulate matter. Although the concentration of gases in the microgravity indoor environment is well studied, aerosols remain one of the major pollutants that affect air quality and has reported adverse health effects and hasn't been reported under these unique conditions. Earth-based AQIs can't be extrapolated to microgravity indoor environments due to different aerosol characteristics and altered lung deposition in low gravity.Concurrent with the aerosol-focused AQI effort, we assess and document how the process would apply for combining particles & gases into a composite index, with the ability to query each AQI independently. All this information can be combined in a spacecraft-specific AQI for future space missions and habitats. The objective of this work are to determine what areas of expertise will contribute, what research and data will be required, and explore the scope of effort needed to formulate a spacecraft AQI in addition to analyzing ISS aerosol sampling data and incorporate results from both aerosol Sampling experiments (the only relevant data available from space).

Sorek-Hamer, Meytar↗

NASA NTRS2019

Satellite Mapping of PM2.5 Episodes in the Wintertime San Joaquin Valley: A "Static" Model Using Column Water Vapor

The use of satellite Aerosol Optical Thickness (AOT) from imaging spectrometers has been successful in quantifying and mapping high PM2.5 (particulate matter mass <2.5Âµm diameter) episodes for pollution abatement and health studies. However, some regions have high PM2.5 but poor estimation success. The challenges in using Aerosol Optical Thickness (AOT) from imaging spectrometers to characterize PM2.5 worldwide was especially evident in the wintertime San Joaquin Valley (SJV). The SJV's attendant difficulties of high-albedo surfaces and very shallow, variable vertical mixing also occur in other significantly polluted regions around the world. We report on more accurate PM2.5 maps for the whole-winter period in the SJV, Nov 14, 2012?Dec 11, 2013. Intensive measurements by including NASA aircraft were made for several weeks in that winter, the DISCOVER-AQ California mission.We found success with a relatively simple method based on calibration and checking with surface monitors and a characterization of vertical mixing, and incorporating specific understandings of the region's climatology. We estimate PM2.5 to within ~7Âµgm?3 RMSE and with R values of ~0.9, based on remotely sensed MAIAC (Multi-Angle Implementation of Atmospheric Correction) observations, and that certain further work will improve that accuracy. Mapping is at 1km resolution. This allows a time sequence of mapped aerosols at 1km for cloud-free days. We describe our technique as a "static estimation". Estimation procedures like this one, not dependent on well-mapped source strengths or on transport error, should help full source-driven simulations by deconstructing processes. They also provide a rapid method to create a long-term climatology.Essential features of the technique are (a) daily calibration of the AOT to PM2.5 using available surface monitors, and (b) characterization of mixed-layer dilution using column water vapor (CWV, otherwise "precipitable water"). We noted that on multi-day timescales both water vapor and particles share near-surface sources and both fall to very low values with altitude; indeed, both are largely removed by precipitation. The existence of layers of H2O or aerosol not within the mixed layer adds complexity, but mixed-effects statistical regression captures essential proportionality of PM2.5 and the ratio variable (AOT/CWV). Accuracy is much higher than previous statistical models, and can be extended to the whole Aqua-satellite data record. The maps and time-series we show suggest a repeated pattern for large valleys like the SJV ? progressive stabilization of the mixing height after frontal passages: PM2.5 is somewhat more determined by day-by-day changes in mixing than it is by the progressive accumulation of pollutants (revealed as increasing AOT).

Chatfield, Robert B.↗

NASA NTRS2019

Near Real-Time Sub/Seasonal Prediction of Aerosol and Air Quality at the NASA Global Modeling and Assimilation Office

Version 2 of the coupled modeling and analysis system used to produce near real time subseasonal to seasonal forecasts was released almost two years ago by the NASA/Goddard Global Modeling and Assimilation Office. The model runs at approximately 1/2 degree globally in the atmosphere and ocean, contains a realistic description of the cryosphere, and includes an interactive aerosol model. The data assimilation used to produce initial conditions is weakly coupled, in which the atmosphere-only assimilated state is coupled to an ocean data assimilation system using a Local Ensemble Transform Kalman Filter. Results of aerosol-derived air quality (Particulate Matter) from an extensive series of retrospective forecasts will be shown, with particular focus on the continental United States and eastern Asia. In addition, under some circumstances, the interactive aerosol is shown to improve seasonal time scale prediction skill. Plans for a future version of the system with predicted biomass burning from fires will also be discussed.

Molod, Andrea↗

NASA NTRS2020

Emission Characteristics of an Axially Staged Sector Combustor for a Small Core High OPR Subsonic Aircraft Engine

Gaseous (NOx, CO) and non-volatile particulate matter (nvPM) emissions from a small-core high-pressure Axially Controlled Stoichiometry (ACS) combustor are reported. NOx and CO emissions characteristics are similar to a previous version of ACS combustor. Emissions of nvPM at low-power (fuel-rich front end) was found to procude significantly higher nvPM emissions compared to a high-power configuration (fuel-lean front end). NOx emissions for the ACS combustor were 82-89% below the ICAO CAEP/6 standard for aggressive NASA N+3 high-pressure cycles based on NOx correlations developed from experimental measurements.

He, Zhuohui J.↗

NASA NTRS2020

High Resolution Global Coupled Chemistry-Meteorology Simulations Using the NASA GEOS Composition Forecast System, GEOS-CF

We will give an overview of the NASA Global Earth Observing System Composition Forecast system (GEOS-CF), a high-resolution (0.25 degree) global composition model developed by the NASA Global Modeling and Assimilation Office (GMAO). This system combines the GEOS weather and aerosol model with the GEOS-Chem chemistry module (version 12) to provide a holistic view of atmospheric composition that captures a wide range of air pollutants such as ozone, nitrogen oxides, volatile organic compounds, and fine particulate matter. The spatial resolution of 0.25 degrees (approx. 25 km) is fine enough to resolve local features such as nighttime ozone titration previously resolved only by urban or regional models. Furthermore, since there are no boundary conditions for a global model, the GEOS-CF captures large-scale processes such as long-range transport of air pollutants from forest fires. Comparisons against surface observations highlight the model’s overall capability to reproduce the diurnal variability of air pollutants under a variety of meteorological conditions. In addition, we show how machine learning techniques can be used to correct for sub-grid variability, which further improves model estimates at a given surface observation site. The GEOS-CF system offers a new tool for scientists and the public health community alike and is being developed jointly with several government and non-profit partners. As an example, we will show the use of GEOS-CF during the Satellite Coastal and Oceanic Atmospheric Pollution Experiment (SCOAPE). The campaign, conducted in collaboration between NASA and the Bureau of Ocean Energy Management (BOEM), aims to investigate the response of onshore air quality to Outer Continental Shelf (OCS) oil and gas exploration, development and production. Detailed gas-phase chemistry, as provided by GEOS-CF, is critical to understand the formation of air pollution related to hydrocarbon emissions from offshore oil and gas activities. The accuracy of GEOS-CF can be further improved by incorporating detailed offshore emissions compiled by BOEM.

Knowland, K. Emma↗

NASA NTRS2019

Connecting Crop Productivity, Residue Fires, and Air Quality over Northern India

Northwestern India is known as the “breadbasket” of the country producing two-thirds of food grains, with wheat and rice as the principal crops grown under the crop rotation system. Agricultural data from India indicates a 25% increase in the post-monsoon rice crop production in Punjab during 2002–2016. NASA’s A-train satellite sensors detect a consistent increase in the vegetation index (net 21%) and post-harvest agricultural fire activity (net ~60%) leading to nearly 43% increase in aerosol loading over the populous Indo-Gangetic Plain in northern India. The ground-level particulate matter (PM2.5) downwind over New Delhi shows a concurrent uptrend of net 60%. The effectiveness of a robust satellite-based relationship between vegetation index—a proxy for crop amounts, and post-harvest fires—a precursor of extreme air pollution events, has been further demonstrated in predicting the seasonal agricultural burning. An efficient crop residue management system is critically needed towards eliminating open field burning to mitigate episodic hazardous air quality over northern India.

Hiren Jethva↗

NASA NTRS2019

Anthropogenic Control over Wintertime Oxidation of Atmospheric Pollutants

Anthropogenic air pollutants such as nitrogen oxides (NO(x) = NO + NO(2)), sulfur dioxide (SO(2)), and volatile organic compounds (VOC), among others, are emitted to the atmosphere throughout the year from energy production and use, transportation, and agriculture. These primary pollutants lead to the formation of secondary pollutants such as fine particulate matter (PM(2.5)) and ozone (O(3)) and perturbations to the abundance and lifetimes of short-lived greenhouse gases. Free radical oxidation reactions driven by solar radiation govern the atmospheric lifetimes and transformations of most primary pollutants and thus their spatial distributions. During winter in the mid and high latitudes, where a large fraction of atmospheric pollutants are emitted globally, such photochemical oxidation is significantly slower. Using observations from a highly instrumented aircraft, we show that multi-phase reactions between gas-phase NO(x) reservoirs and aerosol particles, as well as VOC emissions from anthropogenic activities, lead to a suite of atypical radical precursors dominating the oxidizing capacity in polluted winter air, and thus, the distribution and fate of primary pollutants on a regional to global scale.

Haskins, J. D.↗

NASA NTRSDate not supplied

TPSAS-NF1676L-35847-DND

Aerosols, especially particulate matter with aerodynamic diameters smaller than 2.5 ?m (PM2.5), contribute to air pollution and negatively impact human health. Past studies have estimated PM2.5 concentrations through the use of aerosol optical thickness (AOT) datasets from passive satellite sensors like MODIS and MISR. However, a major limitation of using passive AOTs for PM2.5 applications is that they are column-integrated, while PM2.5 is a surface measurement. In this study, we employ a bulk-mass-modeling-based method to directly derive PM2.5 concentrations over the contiguous United States (CONUS) using two years (2008-2009) of daytime and nighttime near-surface aerosol extinction retrievals from the NASA Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument, bulk mass extinction efficiencies, and model-based hygroscopicity. Results reveal that CALIOP-derived PM2.5 agrees reasonably well with ground-based PM2.5 observations from the U.S. Environmental Protection Agency (EPA), implying this method exhibits some merit in monitoring PM2.5 concentrations from CALIOP data. The newly developed method is then applied to CALIOP aerosol extinction retrievals using nearly the entire CALIOP data record (2007-2018), and an initial trend analysis is conducted. Results from various sensitivity studies are also shown, including those of surface layer height and assumed aerosol type.

Travis D Toth↗

NASA NTRSDate not supplied

TPSAS-NF1676L-11435-DND

Acoustical studies of atmospheric events like convective storms, shear-induced turbulence, acoustic gravity waves, microbursts, hurricanes, and clear air turbulence (CAT) over the past thirty years have established that these events are strong emitters of infrasound. Several mechanisms for the production of infrasound have been proposed, for example by the acceleration of vorticity or by space-time correlations of the turbulent Reynolds stresses (Lighthill theory). Electromagnetic (EM) sensors suffer two severe disadvantages in the detection of clear air turbulence and severe storms. The first is the inability to receive returns in clear air, where reflective targets (precipitation, particulate matter) are absent. The second disadvantage is that EM systems, being active, require scanning to locate an event, as opposed to a passive infrasonic array, which receives infrasonic radiation independently of event location. Further, EM systems, even weather radar ("NEXRAD"), do not have the extensive range (hundreds of miles) characteristic of infrasound. The leading laboratory for studies on atmospheric infrasound over the past thirty years has been the Environmental Technology Laboratory of the National Oceanic and Atmospheric Administration. This laboratory conducted measurements of infrasound from many sources, among which clear air turbulence was but a small part of the overall program. The summary of the results of this program suggests for development of a practical detection system. In other words, despite the progress made in this area, there does not exist today a National network of stations to monitor infrasound from turbulence. Under Innovative Partnership Program, Researchers at NASA Langley Research Center have been working to achieve that goal. As a first step, NASA Langley has designed and developed a portable infrasonic detection system which can be used to make useful infrasound measurements at a location where it was not possible previously. The design and results of the compact system, based upon laboratory and field experiments, will be presented.

Qamar Shams↗

NASA NTRS2020

Application of Low-Cost Fine Particulate Mass Monitors to Convert Satellite Aerosol Optical Depth Measurements to Surface Concentrations in North America and Africa

Low-cost particulate mass sensors provide opportunities to assess air quality at unprecedented spatial and temporal resolutions. Established traditional monitoring networks have limited spatial resolution and are simply absent in many major cities across sub-Saharan Africa (SSA). Satellites provide snapshots of regional air pollution but require ground-truthing. Low-cost monitors can supplement and extend data coverage from these sources worldwide, providing a better overall air quality picture. We investigate the utility of such a multi-source data integration approach using two case studies. First, in Pittsburgh, Pennsylvania, both traditional monitoring and dense low-cost sensor networks are compared with satellite aerosol optical depth (AOD) data from NASA's MODIS system, and a linear conversion factor is developed to convert AOD to surface fine particulate matter mass concentration (as PM2.5). With 10 or more ground monitors in Pittsburgh, there is a 2-fold reduction in surface PM2.5 estimation mean absolute error compared to using only a single ground monitor. Second, we assess the ability of combined regional-scale satellite retrievals and local-scale low-cost sensor measurements to improve surface PM2.5 estimation at several urban sites in SSA. In Rwanda, we find that combining local ground monitoring information with satellite data provides a 40 % improvement in surface PM2.5 estimation accuracy with respect to using low-cost ground monitoring data alone. A linear AOD-to-surface-PM2.5 conversion factor developed in Kigali, Rwanda, did not generalize well to other parts of SSA and varied seasonally for the same location, emphasizing the need for ongoing and localized ground-based monitoring, which can be facilitated by low-cost sensors. Overall, we find that combining ground-based low-cost sensor and satellite data, even without including additional meteorological or land use information, can improve and expand spatiotemporal air quality data coverage, especially in data-sparse regions.

AOD↗