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DOE OSTI2022

Observation and diagnostic application of Kr K-shell emission in magnetized liner inertial fusion experiments at Z

In a series of Magnetized Liner Inertial Fusion (MagLIF) experiments performed at the Z pulsed power accelerator of Sandia National Laboratories, beryllium liners filled with deuterium gas pressures in the 4–8 atm range and a tracer amount of krypton were imploded. At the collapse of the cylindrical implosion, temperatures in the 1–3 keV range and atom number densities of ∼1023 cm−3 were expected. The plasma was magnetized with a 10 T axial magnetic field. Krypton was added to the fuel for diagnosing implosion plasma conditions. Krypton K-shell line emission was recorded with the CRITR time-integrated transmission crystal x-ray spectrometer. The observation shows n = 2 to n = 1 line emissions in B-, Be-, Li-, and He-like Kr ions and is characteristic of the highest electron temperatures achieved in the thermonuclear plasma. Detailed modeling of the krypton atomic kinetics and radiation physics permits us to interpret the composite spectral feature, and it demonstrates that the spectrum is temperature sensitive. We discuss temperatures extracted from the krypton data analysis for experiments performed with several filling pressures.

Clapp, J. T. (ORCID:0000000219928146)↗

DOE OSTI2024

Combined search for electroweak production of winos, binos, higgsinos, and sleptons in proton-proton collisions at s = 13 TeV

A combination of the results of several searches for the electroweak production of the supersymmetric partners of standard model bosons, and of charged leptons, is presented. All searches use proton-proton collision data at s = 13 TeV recorded with the CMS detector at the LHC in 2016–2018. The analyzed data correspond to an integrated luminosity of up to 137 fb − 1 . The results are interpreted in terms of simplified models of supersymmetry. Two new interpretations are added with this combination: a model spectrum with the bino as the lightest supersymmetric particle together with mass-degenerate Higgsinos decaying to the bino and a standard model boson, and the compressed-spectrum region of a previously studied model of slepton pair production. Improved analysis techniques are employed to optimize sensitivity for the compressed spectra in the wino and slepton pair production models. The results are consistent with expectations from the standard model. The combination provides a more comprehensive coverage of the model parameter space than the individual searches, extending the exclusion by up to 125 GeV, and also targets some of the intermediate gaps in the mass coverage. © 2024 CERN, for the CMS Collaboration 2024 CERN

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2025

Antiprotons and Elementary Particles over a Solar Cycle: Results from the Alpha Magnetic Spectrometer

We present results over an 11-year Solar cycle of cosmic antiprotons based on 1.1 × 10 6 events in the rigidity range from 1.00 to 41.9 GV. The $\bar{𝑝}$ fluxes exhibit distinct properties. The magnitude of the $\bar{𝑝}$ flux temporal variation is significantly smaller than those of 𝑝, 𝑒 − , and 𝑒 + . A hysteresis between the $\bar{𝑝}$ fluxes and the 𝑝 fluxes is observed, whereas the $\bar{𝑝}$ and 𝑒 − fluxes show a linear correlation. With a model-independent analysis, we found a universal relation between the shape of the rigidity spectrum and the magnitude of flux temporal variation over an 11-year Solar cycle for both positively and negatively charged particles. The simultaneous results on $\bar{𝑝}$ and 𝑝, 𝑒 − , and 𝑒 + provide unique information for understanding particle transport in the Solar System as a function of mass, charge, and spectral shape.

cosmic ray composition & spectra↗

DOE OSTI2023

Laboratory Constraints on the Neutron-Spin Coupling of feV-Scale Axions

Ultralight axionlike particles can contribute to the dark matter near the Sun, leading to a distinct, stochastic signature in terrestrial experiments. We search for such particles through their neutron-spin coupling by reanalyzing approximately 40 days of data from a K- 3 He comagnetometer with a new frequency-domain likelihood-based formalism that properly accounts for stochastic effects over all axion coherence times relative to the experimental time span. Assuming that axions make up all of the dark matter in the Sun’s vicinity, we find a median 95% upper limit on the neutron-spin coupling of 2.4 × 10 −10 GeV −1 for most axion masses from 0.4 to 4 feV, which is about 5 orders of magnitude more stringent than previous laboratory bounds in that mass range. Although several peaks in the experiment’s magnetic power spectrum suggest the rejection of a white-noise null hypothesis, further analysis of their line shapes yields no positive evidence for a dark-matter axion.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2021

Missing-Data Nonparametric Coherency Estimation

Chave recently proposed an estimator for multitaper spectral density where the time series contains missing values. In this article we generalize this technique to a multitaper estimator of coherence and phase and show that one can also obtain bootstrapped confidence intervals. Additionally, we give two examples. The first is a toy example in which the true coherence is known. In the second example we show that the multitaper missing-data coherence estimator computed on real data with a single gap comprising 11% of the data outperforms the Daniell-smoothed coherence estimator where there are no gaps. The case where the two time series have different missing indices is also discussed.

42 ENGINEERING↗

DOE OSTI2024

Time series methods for the analysis of soundscapes and other cyclical ecological data

Biodiversity monitoring has entered an era of ‘big data’, exemplified by a near-continuous collection of sounds, images, chemical and other signals from organisms in diverse ecosystems. Such data streams have the potential to help identify new threats, assess the effectiveness of conservation interventions, as well as generate new ecological insights. However, appropriate analytical methods are often still missing, particularly with respect to characterizing cyclical temporal patterns. Here, we present a framework for characterizing and analysing ecological responses that represent nonstationary, complex temporal patterns and demonstrate the value of using Fourier transforms to decorrelate continuous data points. In our example, we use a framework based on three approaches (spectral analysis, magnitude squared coherence, and principal component analysis) to characterize differences in tropical forest soundscapes within and across sites and seasons in Gabon. By reconstructing the underlying, cyclic behaviour of the soundscape for each site, we show how one can identify circadian patterns in acoustic activity. Soundscapes in the dry season had a complex diel cycle, requiring multiple harmonics to represent daily variation, while in the wet season there was less variance attributable to the daily cyclic patterns. Our framework can be applied to most continuous, or near-continuous ecological data collected at a fine temporal resolution, allowing ecologists to explore patterns of temporal autocorrelation at multiple levels for biologically meaningful trends. Such methods will become indispensable as biological big data are used to understand the impact of anthropogenic pressures on biodiversity and to inform efforts to mitigate them.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

IRMA

IRMA (In)elastic Representation of Materials As S(α,β) evaluations IRMA turns one phonon model into three outputs that usually require three separate tool chains: an evaluated nuclear-data file, predicted neutron-scattering spectra, and scattering kernels for Monte Carlo transport. The three outputs draw on a single, consistent description of the material, so the evaluation, the spectroscopy that can validate it, and the transport that uses it always agree about the physics. Nuclear data. IRMA writes ENDF-6 File 7 thermal scattering evaluations on automatically constructed (α, β) grids. This part reimplements and generalizes NJOY's LEAPR: the classic kernels reproduce freshly generated NJOY2016 tapes digit for digit and published reference tapes to about 1e-4, and the generalized paths add the exact coherent one-phonon term, anisotropic Debye-Waller tensors, coherent elastic for arbitrary crystals, and a per-species partition for polyatomic materials. The tapes feed NJOY, AMPX, FUDGE, and every transport code downstream of them. Neutron spectroscopy. The irma.spectra forward model projects the same physics onto an instrument's kinematics and resolution: INS spectra for VISION and generic indirect geometries, and 2-D S(Q,E) powder maps for direct-geometry spectrometers, from a phonopy model or straight from a phonon DOS. It can be used to predict a proposed measurement before beam time; in analysis, it supplies the calculated single-scattering counterpart of a measured spectrum, from the same material description the evaluation was built from. Monte Carlo transport. The irma.ncrystal exporter writes per-temperature scattering kernels for the companion NCrystal plugin, so McStas, OpenMC, and other NCrystal-aware codes sample the same physics. The exported kernels carry the per-site anisotropic Debye-Waller tensors, keeping directional coherent-elastic physics that NCrystal's standard scalar treatment does not represent. With the same physics inside a transport code, an entire beamline becomes a virtual experiment: IRMA's end-to-end validation ran a custom McStas implementation of the ARCS spectrometer, assembled from the existing McVine and McStas models, against measured data. From a bare crystal structure. The irma mlip front end builds the phonon model itself: a structure file and a choice of potential are enough. Nine pretrained machine-learned interatomic potentials are supported, on a laptop CPU, with no first-principles calculation; an approximate phonon model for a new material costs minutes, not a DFT campaign, and the build emits prefilled inputs for all three outputs. The result is a good starting point rather than a finished evaluation: survey-quality physics with every parameter exposed for review. A converged atomistic calculation enters the same way, as a phonopy model, when higher fidelity is needed.

Ramic, Kemal [Oak Ridge National Laboratory (ORNL)↗

DOE OSTI2021

Improving Fission Products at CARIBU: Near Field Detection (Q1/FY21 Quarterly Progress Report)

After receiving funds at the beginning of FY21 we were able to resume work on the project. We continued data analysis of 156 Eu decay. The project has also gone through an Independent Review in November. Following the previously reported steps in the analysis of 156 Eu, specifically removing random coincidences from the gamma ray spectrum, we look not only at the peak of interest (811 keV) but all other gamma rays that are visible. Determining the area of all gamma ray peaks in this random coincidence free spectrum is not only necessary to calculate the gamma ray branching ratios but combined with the peak areas of the gamma ray singles spectrum we are able to determine experimentally the efficiency of the beta detector.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2020

Place polarized neutron reflectivity data in bins of constant wavevector transfer

Code to place polarized neutron reflectivity into bins of constant Qz with regard for Zeeman energy change to the spin-flip channel. The code is written as a Jupyter notebook. Example data are included as separate files (spin_down.txt and spin_up.txt). As a first step, run all cells in the notebook. Opportunities are identified for users to make their own choices for analysis of the data. The code is written to be a stand-alone operation on data collected from a pulse neutron source that have been previously normalized to the wavelength dependence of the incident beam spectrum, background subtracted, etc. The constant Qz binning (this code) is the last step to perform in the analysis (reduction) workflow. This step yields the the reflectivities for the four neutron spin cross-sections. A future intention is to create a version of this code that will be one module of many in the data analysis workflow.

Fitzsimmons, Michael [Oak Ridge National Lab. (ORN↗

DOE OSTI2024

Short-Wave Infrared Upconverting Nanoparticles

Optical technologies enable real-time, noninvasive analysis of complex systems but are limited to discrete regions of the optical spectrum. While wavelengths in the short-wave infrared (SWIR) window (typically, 1700-3000 nm) should enable deep subsurface penetration and reduced photodamage, there are few luminescent probes that can be excited in this region. Here, we report the discovery of lanthanide-based upconverting nanoparticles (UCNPs) that efficiently convert 1740 or 1950 nm excitation to wavelengths compatible with conventional silicon detectors. Screening of Ln3+ ion combinations by differential rate equation modeling identifies Ho3+/Tm3+ or Tm3+ dopants with strong visible or NIR-I emission following SWIR excitation. Experimental upconverted photoluminescence excitation (U-PLE) spectra find that 10% Tm3+-doped NaYF4 core/shell UCNPs have the strongest 800 nm emission from SWIR wavelengths, while UCNPs with an added 2% or 10% Ho3+ show the strongest red emission when excited at 1740 or 1950 nm. Mechanistic modeling shows that addition of a low percentage of Ho3+ to Tm3+-doped UCNPs shifts their emission from 800 to 652 nm by acting as a hub of efficient SWIR energy acceptance and redistribution up to visible emission manifolds. Parallel experimental and computational analysis shows rate equation models are able to predict compositions for specific wavelengths of both excitation and emission. These SWIR-responsive probes open a new IR bioimaging window, and are responsive at wavelengths important for vision technologies.

Qi, Xiao↗

DOE OSTI2022

Stability analysis of a one-dimensional multiphysics model of a molten salt fast reactor

Reactor designs with a fast neutron spectrum have recently moved into the research focus for possible Generation IV reactor concepts - a representative of which is the molten salt fast reactor (MSFR). In order to assess the safety and reliability of this reactor concept, it is necessary to obtain knowledge of the system behaviour. An important part of this research concerns the dynamical stability of the MSFR. Research regarding the MSFR stability so far has either been using linearized models for stability criteria or only been examining certain transients at fixed parameter values. This work delivers a comprehensive stability analysis for a non-linearized MSFR model, and a wide range of values for all relevant parameters. For this purpose, a one-dimensional MSFR model was set up, taking neutron kinetics and thermal hydraulics in the form of a system of differential equations into account. The stability of this model was investigated by means of the numerical tool MATCONT, which was used to monitor the evolution of a so-called fixed-point solution, here referring to the steady state at operating conditions of the system, while system parameters got varied. The MATCONT analyses showed no loss of stability for any of the considered parameter variations and no solutions that might co-exist in parallel with the steady-state fixed-point solution. Therefore these results indicate a stable fixed point to which all solution transients converge, making the considered MSFR model insusceptible to deviations from the equilibrium. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

DOE OSTI2024

Godiva IV Simulated Radiation Field Characterization and Variance Reduction

Godiva IV is a system comprised of highly enriched uranium alloyed with molybdenum in the form of fuel plate rings. The reactor, along with its predecessors, was designed with the unique ability to satisfy interests in the super-prompt-critical reactor operation space. Originally, the reactor was part of the Los Alamos Critical Experiments Facility (LACEF) at Technical Area-18 (TA-18). The radiation field around Godiva at this facility was well characterized and understood. As a fast neutron system, the neutron spectrum in and around Godiva was close to a Watt Fission spectrum. The Kiva where Godiva IV was located at LACEF was made of thin, sheet metal walls which did not contribute significantly to the neutron spectrum. Following the transition of LACEF to the National Critical Experiments and Research Center (NCERC) in Nevada, Godiva-IV was moved from TA-18 to the Device Assembly Facility (DAF) at the Nevada National Security Site (NNSS). Part of this move brought renewed interest in radiation field characterization. The new facility introduced significant changes to the environment surrounding Godiva, and preliminary foil irradiation results suggested that the room contribution to the neutron spectrum was significant. Unlike at TA-18, a large thermal neutron signature was added to the fast spectrum from Godiva due to significant room return. A primary goal due to the additional complexity that the room return adds to the Godiva IV radiation emission spectrum was the development of an efficient Monte Carlo N-Particle (MCNP) calculation capable of characterizing the neutron spectrum anywhere in the room around Godiva. A campaign of activation foil irradiations and analysis were completed to support the validation of the MCNP model. The modeling of these foils in MCNP can be easily done with a standard volumetric neutron flux tally. However, given the multitude of locations and reaction rates to be modeled, further steps must be taken to increase the efficiency of these calculations in MCNP. During this study, a benchmark model currently under development for Godiva IV was used. A qualitative assessment of the thermal neutron contributors was performed using spatial neutron distribution plots. Additional detail was added to the model based on the qualitative results showing the thermal spectrum’s large sensitivity to hydrogenous material. Neutron energy spectra was evaluated at discrete locations in the room around Godiva to quantify the relative contribution of various components. It was discovered that the concrete walls are the largest contributor to the thermal signature, with minor contributions from plastic components surrounding Godiva. Following these results, two different variance reduction techniques were implemented to improve the problem efficiency in these calculations. In the first approach, an F5 point detector tally was implemented in the standard Godiva IV criticality problem. The second approach involved a weight-window generator implementation with an F5 point detector tally in a fixed source problem. The weight window implementation reduced the runtime from 42739.55 minutes to 1803.34 minutes (computer time), compared to the F5 KCODE implementation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2022

A multiwavelength study of the flat-spectrum radio quasar NVSS J141922−083830 covering four flaring episodes

We present multiwavelength observations and a model for flat-spectrum radio quasar (FSRQ) NVSS J141922−083830, originally classified as a blazar candidate of unknown type (BCU II object) in the Third Fermi-LAT AGN Catalog. Relatively bright flares (>3 magnitudes) were observed on 2015 February 21 (MJD 57074) and 2018 September 8 (MJD 58369) in the optical band with the MASTER Global Robotic Net telescopes. Optical spectra obtained with the Southern African Large Telescope on 2015 March 1 (MJD 57082), during outburst, and on 2017 May 30 (MJD 57903), during quiescence, showed emission lines at 5325 Å and at ≈3630 Å that we identified as the Mg II III] 1909 Å lines, respectively, and hence derived a redshift z = 0.903. Analysis of Fermi-Large Area Telescope (LAT) data was performed in the quiescent regime (5 yr of data) and during four prominent flaring states in 2014 February–April, 2014 October–November, 2015 February–March, and 2018 September. We present spectral and timing analysis with Fermi-LAT . We report a hardening of the gamma-ray spectrum during the last three flaring periods, with a power-law spectral index Γ = 2.0–2.1. The maximum gamma-ray flux level was observed on 2014 October 24 (MJD 56954) at (7.57 ± 1.83) × 10 −7 ph cm −2 s −1 . The multiwavelength spectral energy distribution (SED) during the 2015 February–March flare supports the earlier evidence of this blazar to belong to the FSRQ class. The SED can be well represented with a single-zone leptonic model with parameters typical of FSRQs, but also a hadronic origin of the high-energy emission cannot be ruled out.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

Isomeric yield ratios of fission products: A missing piece in reactor antineutrino summation calculations

The calculation of the spectrum of antineutrinos ($\bar{v}_e$) from a reactor is a complicated problem requiring several nuclear data and physics inputs. Many of these have been investigated thoroughly to improve calculations and properly account for uncertainties. One input which has heretofore escaped consideration is the fission-yield distribution between ground and isomeric states. Here, in this work, we explore the effect of incorporating newly evaluated isomeric yield ratios (IYR) for 43 fission products into summation calculations and identify the disproportionate importance of certain isotopes, particularly at higher energies. Our analysis indicates that updated IYRs contribute to a significant increase in the $\bar{v}_e$ spectrum around and above 7 MeV, with increases of more than 50% at higher energies. Through a detailed sensitivity study, we highlight a number of isotopes for which the IYR has a substantial effect on the $\bar{v}_e$ spectrum. This work stresses the critical role of isomeric yields in calculations of reactor $\bar{v}_e$ spectra and points to the necessity for their accurate experimental determination, especially for key fission products, in order to refine our understanding and address the observed anomalies between measured and calculated $\bar{v}_e$ spectra.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2020

A Wide and Deep Exploration of Radio Galaxies with Subaru HSC (WERGS). III. Discovery of a z = 4.72 Radio Galaxy with the Lyman Break Technique

We report a discovery of a z = 4.72 radio galaxy, HSC J083913.17+011308.1, using the Lyman break technique with the Hyper Suprime-Cam Subaru Strategic Survey (HSC-SSP) catalog for Very Large Array Faint Images of the Radio Sky at Twenty centimeter radio sources. The number of known high-z radio galaxies (HzRGs) at z > 3 is quite small to constrain the evolution of HzRGs so far. The deep and wide-area optical survey by HSC-SSP enables us to apply the Lyman break technique to a large search for HzRGs. For an HzRG candidate among pre-selected r-band dropouts with a radio detection, a follow-up optical spectroscopy with the Gemini Multi-Object Spectrographs (GMOS)/Gemini has been performed. The obtained spectrum presents a clear Lyα emission line redshifted to z = 4.72. The spectral energy distribution fitting analysis with the rest-frame UV and optical photometries suggests the massive nature of this HzRG with logM{sub ∗}/M{sub ⊙}=11.4. The small equivalent width of Lyα and the moderately red UV colors indicate its dusty host galaxy, implying a chemically evolved and dusty system. The radio spectral index does not meet a criterion for an ultra-steep spectrum, α{sub 1400}{sup 325} of −1.1 and α{sub 1400}{sup 150} of −0.9, demonstrating that the HSC-SSP survey compensates for a subpopulation of HzRGs that are missed in surveys focusing on an ultra-steep spectral index.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

Isomeric Yield Ratios of fission products: a missing piece in reactor antineutrino summation calculations

The calculation of the spectrum of antineutrinos ( $\overline{V}$ e ) from a reactor is a complicated problem requiring several nuclear data and physics inputs. Many of these have been investigated thoroughly to improve calculations and properly account for uncertainties. One input which has heretofore escaped consideration is the fission yield distribution between ground and isomeric states. In this work, we explore the effect of incorporating newly evaluated isomeric yield ratios (IYR) for 43 fission products into summation calculations and identify the disproportionate importance of certain isotopes, particularly at higher energies. Our analysis indicates that updated IYRs contribute to a significant increase in the $\overline{V}$ e spectrum around and above 7 MeV, with increases of more than 50% at higher energies. Through a detailed sensitivity study, we highlight a number of isotopes for which the IYR has a substantial effect on the $\overline{V}$ e spectrum. This work stresses the critical role of isomeric yields in calculations of reactor $\overline{V}$ e spectra and points to the necessity for their accurate experimental determination, especially for key fission products, in order to refine our understanding and address the observed anomalies between measured and calculated $\overline{V}$ e spectra.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2022

Uncertainty Quantification of Bifacial Performance Modeling

Analysis on uncertainty in the annual energy of PV systems that can be attributed to parameters of particular importance to bifacial PV modules is presented. Monte Carlo simulations are used to evaluate the effect of uncertain module bifaciality factors, module transmission fractions, albedo values, and ground clearance. The analyses cover a wide spectrum of potential PV array archetypes through variation of installation parameters. The results of the Monte Carlo analysis reveal that the uncertainty is largely dependent on albedo uncertainty, but more simulations are needed to identify trends across system archetypes. The simulations are aimed at attributing an annual energy uncertainty factor for bifacial considerations that can be applied in post-processing of project probability of exceedance analysis.

energy modeling↗

DOE OSTI2022

Uncertainty Quantification of Bifacial Performance Modeling

bifacial↗