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At least 343 records · Page 19
All sourcesNASA NTRSDOE OSTI
NASA NTRS2024

DDFRG3: Double-Differential FRaGmentation model for Neutron production

A Double-Differential FRaGmentation (DDFRG) model for neutron production from nucleus - nucleus collisions is developed for space radiation applications. DDFRG1 was a previous model developed for production of protons and light ions, and DDFRG2 was a model developed for pion production. A new model (DDFRG3) for neutron production is developed in the present work, and is based upon thermal production of neutrons from the projectile, the target and central fireball sources. The Lorentz-invariant double-differential cross sections are calculated in the various source frames, and are Lorentz transformed to the laboratory frame, resulting in a closed-form analytic formula involving no numerical integration, and which can be run very efficiently in radiation transport codes. The Lorentz-invariant double-differential cross section is then integrated over angle to give the single-differential energy spectral distribution. The DDFRG3 neutron model compares very well to an extensive experimental data set.

neutrons↗
DOE OSTI2020

Methods for separating non-fibrous solids from liquids using a double-roller

A method for separating solids from liquids is disclosed. A double-roller system is provided. A process fluid is provided to the double-roller system. The process fluid comprises a suspended solid and a process liquid. The suspended solid comprises non-fibrous solid particles. A portion of the process fluid is compressed through the double-roller system to produce a compressed portion of the suspended solid. A product stream and a dilute fluid stream are separated. The product stream comprises a compressed portion of the suspended solid and a first portion of the process liquid. The dilute fluid stream comprises a second portion of the suspended solid and a second portion of the process liquid.

42 ENGINEERING↗
DOE OSTI2022

Alloyed halide double perovskites as solar-cell absorbers

An alloyed halide double perovskite material, an alloyed halide double perovskite solar-cell absorber and solar cells constructed with such absorbers, the alloyed halide double perovskite material having the formula A2B1-aB′1-bDxX6, where A is an inorganic cation, an organic cation, a mixture of inorganic cations, a mixture of organic cations, or a mixture of one or more inorganic cations and one or more organic cations, where B is a metal, a mixture of metals, a metalloid, a mixture of metalloids, any mixture thereof, or is a vacancy, where B′ is a metal, a mixture of metals, a metalloid, a mixture of metalloids, any mixture thereof, or is a vacancy, where D is a dopant, and where X is a halide, a pseudohalide, a mixture of halides, a mixture of pseudohalides, or a mixture of halides and pseudohalides, and where x=a+b.

Karunadasa, Hemamala Indivari↗
DOE OSTI2026

First CLAS12 Double-Pion (Npp) Electroproduction Analysis

The N* program aims to explore strong interaction dynamics of the three-valence quark distance-dependent structure. The electroproduction and photoproduction studies provide insight into the nucleon resonance structure. One of the primary objectives of N* is to extract the electroexcitation amplitudes, which are crucial in determining the inner structure of various nucleon excitation states and their underlying degrees of freedom. Studying them on the nucleon length scale reveals also parts of the complex nature of the universe and its origin at their most fundamental level. The extraction of these amplitudes is mostly based on the single-pion, and particularly at higher invariant masses W, on the double-pion electroproduction channels, because nucleon resonance dominantly couple to them. CLAS has produced mostly all of the world data on charged double-pion electroproduction in the nucleon resonance region for photon virtualities Q2 up to 5 GeV2. The kinematic range can be extended with CLAS12, which can explore these amplitudes in the still almost unexplored range of Q2 > 5.0 GeV2. This will offer opportunities to understand the resonance structure at distances where the three-bound quark degree of freedom dominates and pave the way towards perturbative Quantum Chromodynamics (pQCD). This dissertation presents new double-pion electroproduction cross sections in the W range [1.4, 2.10] GeV and the Q2 range [2.0, 8.0] GeV2, using the Run Group A Fall-2018 dataset. This data was taken with the CLAS12 detector in Hall B at Thomas Jefferson National Laboratory (JLab) at an electron beam energy of 10.6 GeV. These cross sections are the basis for the extraction of resonance electroexcitation amplitudes using the phenomenological JLab- Moscow State University (JM) model.

Neupane, Krishna↗
DOE OSTI2025

PHOTOPRODUCTION OF np^0 BY DOUBLE-REGGE EXCHANGE

The GlueX experiment is a photoproduction experiment based at Jeferson Lab in Newport News, Virginia. A major aim of GlueX is to look for hybrid mesons, which are a quark and an anti-quark bound by an excited gluonic field that contributes to the quantum numbers. The reaction ¿p ¿ ¿e0p is of particular interest since ¿e is a potential decay mode of states with exotic quantum numbers JPC =1¿+, which are forbidden in the constituent quark model. Finding such a resonance would be a clear sign of non-quark model physics. In concert with the Joint Physics Analysis Center we have developed a model for double-Regge interactions in this channel. These non-resonant processes generate asymmetries in the distributions of decay angles, which could be falsely attributed to the interference between exotic odd partial waves and even partial waves. In previous searches for light exotics we have seen evidence for the necessity of accounting for the presence of these non-resonant productions. We present a double-Regge model for photoproduction of ¿e0 and the application of it by measuring the asymmetry of ¿e0 production in the double Regge limit, as well as a comparison of the measured results to current theoretical predictions.

Barsotti, Rebecca [Indiana Univ. Southeast, New Al↗
DOE OSTI2021

Search for double-β decay of 76 Ge to excited states of 76 Se with the Majorana Demonstrator

The M AJORANA DEMONSTRATOR is a neutrinoless double-β decay search consisting of a low-background modular array of high-purity germanium detectors, ~2/3 of which are enriched to 88% in 76 Ge. The experiment is also searching for double-beta decay of 76 Ge to excited states (e.s.) in 76 Se. 76 Ge can decay into three daughter states of 76 Se, with clear event signatures consisting of a ββ-decay followed by the prompt emission of one or two γ rays. This results with high probability in multi-detector coincidences. In this work, the granularity of the DEMONSTRATOR detector array enables powerful discrimination of this event signature from backgrounds. Using 41.9 kg yr of isotopic exposure, the DEMONSTRATOR has set world leading limits for each e.s. decay of 76 Ge, with 90% CL lower half-life limits in the range of (0.75–4.0) × 10 24 yr. In particular, for the 2ν transition to the first 0 + e.s. of 76 Se, a lower half-life limit of 7.5 × 10 23 yr at 90% CL was achieved.

59 ≤ A ≤ 89↗
DOE OSTI2021

Projected sensitivity of the LUX-ZEPLIN experiment to the two-neutrino and neutrinoless double $\beta$ decays of $^{134}$Xe

The projected sensitivity of the LUX-ZEPLIN (LZ) experiment to two-neutrino and neutrinoless double beta decay of 134 Xe is presented. LZ is a 10-tonne xenon time projection chamber optimized for the detection of dark matter particles, that is expected to start operating in 2021 at Sanford Underground Research Facility, USA. Its large mass of natural xenon provides an exceptional opportunity to search for the double beta decay of 134 Xe, for which xenon detectors enriched in 136 Xe are less effective. For the two-neutrino decay mode, LZ is predicted to exclude values of the half-life up to 1.7 x 10 24 years at 90% confidence level (CL), and has a three-sigma observation potential of 8.7 x 10 23 years, approaching the predictions of nuclear models. For the neutrinoless decay mode LZ, is projected to exclude values of the half-life up to 7.3 x 10 24 years at 90% CL.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Coupled-Cluster Calculations of Neutrinoless Double- β Decay in Ca 48

We use coupled-cluster theory and nuclear interactions from chiral effective field theory to compute the nuclear matrix element for the neutrinoless double-$\beta$ decay of $^{48}$Ca. Benchmarks with the no-core shell model in several light nuclei inform us about the accuracy of our approach. For $^{48}$Ca we find a relatively small matrix element. We also compute the nuclear matrix element for the two-neutrino double-$\beta$ decay of $^{48}$Ca with a quenching factor deduced from two-body currents in recent ab initio calculation of the Ikeda sum rule in $^{48}$Ca [Gysbers et al., Nat. Phys. 15, 428 (2019)].

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Double Doping of Semiconducting Polymers Using Ion-Exchange with a Dianion

The interactions between counterions and electronic carriers in electrically doped semiconducting polymers are important for delocalization of charge carriers, electronic conductivity, and thermal stability. The introduction of a dianions in semiconducting polymers leads to double doping where there is one counterion for two charge carriers. Double doping minimizes structural distortions, but changes the electrostatic interactions between the carriers and counterions. Polymeric ionic liquids (PIL) with croconate dianions are helpful to investigate the role of the counterion in p-type semiconducting polymers. PILs prevent diffusion of the cation into the semiconducting polymers during ion exchange. The redox-active croconate dianions undergo ion exchange with doped semiconducting polymers depending on their ionization energy. Croconate dianions are found to reduce doped films of poly(3-hexyl thiophene), but undergo ion exchange with a polythiophene with tetraethylene glycol side chains, P(g 4 2T-T), that has a lower ionization energy. The croconate dianion maintains crystalline order in P(g 4 2T-T) and leads to a lower activation energy for the electrical conductivity than PF 6 – counterions. The control of the doping level with croconate allows optimization of the thermoelectric performance of the semiconducting polymer. Finally, the thermal stability of the doped films of P(g 4 2T-T) is found to depend strongly on the nature of the counterion.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Reconstructing neutrinoless double beta decay event kinematics in a xenon gas detector with vertex tagging

If neutrinoless double beta decay is discovered, the next natural step would be understanding the lepton number violating physics responsible for it. Several alternatives exist beyond the exchange of light neutrinos. Some of these mechanisms can be distinguished by measuring phase-space observables, namely the opening angle cos θ among the two decay electrons, and the electron energy spectra, T 1 and T 2 . In this work, we study the statistical accuracy and precision in measuring these kinematic observables in a future xenon gas detector with the added capability to precisely locate the decay vertex. For realistic detector conditions (a gas pressure of 10 bar and spatial resolution of 4 mm), we find that the average $\overline{cos θ}$ and $\overline{T_1}$ values can be reconstructed with a precision of 0.19 and 110 keV, respectively, assuming that only 10 neutrinoless double beta decay events are detected.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

CUPID: The Next-Generation Neutrinoless Double Beta Decay Experiment

We report CUPID is a next-generation tonne-scale bolometric neutrinoless double beta decay experiment that will probe the Majorana nature of neutrinos and discover lepton number violation in case of observation of this singular process. CUPID will be built on experience, expertise and lessons learned in CUORE and will be installed in the current CUORE infra-structure in the Gran Sasso underground laboratory. The CUPID detector technology, successfully tested in the CUPID-Mo experiment, is based on scintillating bolometers of Li 2 MoO 4 enriched in the isotope of interest 100 Mo. In order to achieve its ambitious science goals, the CUPID collaboration aims to reduce the backgrounds in the region of interest by a factor 100 with respect to CUORE. This performance will be achieved by introducing the high efficient α/β discrimination demonstrated by the CUPID-0 and CUPID-Mo experiments, and using a high transition energy double beta decay nucleus such as 100 Mo to minimize the impact of the gamma background. CUPID will consist of about 1500 hybrid heat-light detectors for a total isotope mass of 250 kg. The CUPID scientific reach is supported by a detailed and safe background model based on CUORE, CUPID-Mo and CUPID-0 results. The required performances have already been demonstrated and will be presented.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Direct Fabrication of Vertically Stacked Double Barrier Tunnel Junctions Based on Graphene and h-BN

Direct manufacturing of two-dimensional material-based double barrier (DB) tunnel junctions, based on a lithography-free approach was developed. Graphene/h-BN/Graphene/h-BN/Graphene devices were deposited on Si/SiO2 substrates by employing a plasma enhanced chemical vapor deposition technique in a sequential manner. DB tunneling junctions with varying barrier widths (by varying the thickness of the second graphene layer) were studied. Samples were characterized using Raman, Atomic Force Microscopy and X-ray photoemission spectroscopy. The I–V characteristics of tunneling current showed resonant tunneling behavior at room temperature with a negative differential conductance. The behavior could be explained with quantum mechanical double barrier tunneling model in which analytic solutions to Schrödinger’s equation were obtained in each region of the system. Resonances in transmission probability coefficient for varying barrier widths were evaluated and compared with the experimental results.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Analysis of the electrical double layer using electrochemical X-ray photoelectron spectroscopy

The element-sensitivity of X-ray spectroscopies offers the potential to disentangle the individual chemistries of water, ions, and adsorbates at the electrode-electrolyte interface in an element-by-element manner. However, targeted experimental design is needed to establish interface-sensitive in situ X-ray spectroscopy in a realistic electrochemical environment. Here, we demonstrate how electrochemical X-ray photoelectron spectroscopy (EC-XPS) in the dip-and-pull geometry can be used to specifically probe the behavior of ions in the electrical double layer. Taking the case study of a polycrystalline Au foil in 50 mM KClO 4 electrolyte, we tracked the electrochemical response of interfacial K + cations across a broad potential range. We show how, in combination with modeling, key parameters such as the potential of zero charge (PZC), ion packing behavior, dielectric saturation, and the electrostatic potential decay in the double layer can be extracted from the data. Importantly, we also analyze how the experimental conditions and non-idealities can influence the results and put forward criteria for reliable experimentation and data analysis.

Dip-and-pull↗
DOE OSTI2023

Human DNA polymerase η promotes RNA-templated error-free repair of DNA double-strand breaks

A growing body of evidence indicates that RNA plays a critical role in orchestrating DNA double-strand break repair (DSBR). Recently, we showed that homologous nascent RNA can be used as a template for error-free repair of double-strand breaks (DSBs) in the transcribed genome and to restore the missing sequence at the break site via the transcription-coupled classical nonhomologous end-joining (TC-NHEJ) pathway. TC-NHEJ is a complex multistep process in which a reverse transcriptase (RT) is essential for synthesizing the DNA strand from template RNA. However, the identity of the RT involved in the TC-NHEJ pathway remained unknown. Here, we report that DNA polymerase eta (Pol η), known to possess RT activity, plays a critical role in TC-NHEJ. We found that Pol η forms a multiprotein complex with RNAP II and other TC-NHEJ factors, while also associating with nascent RNA. Moreover, purified Pol η, along with DSBR proteins PNKP, XRCC4, and Ligase IV can fully repair RNA templated 3'-phosphate-containing gapped DNA substrate. In addition, we demonstrate here that Pol η deficiency leads to accumulation of R-loops and persistent strand breaks in the transcribed genes. Finally, we determined that, in Pol η depleted but not in control cells, TC-NHEJ-mediated repair was severely abrogated when a reporter plasmid containing a DSB with several nucleotide deletion within the E. coli lacZ gene was introduced for repair in lacZ-expressing mammalian cells. Thus, our data strongly suggest that RT activity of Pol η is required in error-free DSBR.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2020

Metamagnetism and kinetic arrest in a long-range ferromagnetically ordered multicaloric double perovskite Y 2 CoMnO 6

A systematic magnetic study of the double perovskite oxide Y 2 CoMnO 6 (YCMO) has been performed. A monoclinic P21/n phase of YCMO was synthesized using a sol-gel method. Neutron diffraction (ND) measurements evidence the onset of long-range ferromagnetic (FM) ordering at TC ~ 76 K, which persists down to 5 K. The presence of 25% antisite disorder, estimated from the ND data, leads to the appearance of short-range antiferromagnetic (AFM) interactions. The existence of thermal hysteresis due to competing interactions between FM and AFM phases is observed in the M vs. T measurements. The pinning of magnetic domain walls at the Co/Mn antiphase boundaries results in a metamagnetic-like behavior. The field dependence of thermomagnetic irreversibility and the nature of virgin curves indicate the occurrence of a kinetic arrest phenomenon, which is further verified via cooling and heating of the system in an unequal fields (CHUF) protocol. In full agreement with the ND data, a detailed analysis of critical exponents near the paramagnetic (PM)-FM phase transition also establishes YCMO as a long-range interacting mean-field system. A close examination of the temperature- and field-dependent magnetic entropy change yields an in-depth understanding of coexisting magnetically ordered and disordered phases in YCMO, leading to a comprehensive magnetic phase diagram of this multifunctional double perovskite system.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Decoupling mass transport and electron transfer by a double-cathode structure of a Li-O 2 battery with high cyclic stability

Aprotic lithium-oxygen (Li-O 2 ) batteries have attracted extensive attention due to their ultrahigh theoretical energy density. However, slow and undesired electron transfer during cathodic reactions causes low cyclic stability in these batteries. Here, in this paper, we demonstrate that O 2 mass transport and electron transfer for cathodic reactions in Li-O 2 batteries could be decoupled by a double-cathode structure that efficiently enables stable electron transfer between the cathode and Li 2 O 2 /O 2 . This resolves various side reactions and slow Li 2 O 2 reaction kinetics issues in conventional Li-O 2 batteries, leading to stable operation of the cell for nearly 2 months at a capacity of 0.2 and 5 mAh cm -2 , with more than 4- and 10-fold increases in cycle life when compared with single-cathode batteries. These remarkable improvements in the cyclic stability of Li-O 2 batteries with double cathodes provide an interesting concept for improving the operational stability of other metal-rechargeable batteries with conversion-type chemistry.

25 ENERGY STORAGE↗
DOE OSTI2023

The infinite level normal forms for non-resonant double Hopf singularities

Here, in this paper, we explore hypernormal forms of vector fields that have non-resonant double Hopf singularities with a non-zero radial cubic part. Our primary focus is on investigating the infinite-level normal form classification of this type of singularities. We provide a normal form decomposition in terms of planar-rotating and planar-radial vector fields, which greatly facilitate the pattern recognition and analysis of the corresponding generalized homological maps. Notably, our paper represents the first instance of the normal form classification for general non-resonant double Hopf singularities without structural symmetry.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2023

Detailed investigation of electrical and optical properties of textured n-type and roughened p-type tunnel oxide passivated contacts for screen-printed double-side passivated contact silicon solar cell application

Here, this paper presents detailed characterization and analyses of the optical, electrical, and contact properties of a 35 nm phosphorus-doped (n-type) polysilicon (poly-Si) and a 250 nm boron-doped (p-type) poly-Si deposited respectively on textured and roughed surface. These layers could be applied respectively to the front and rear sides of an n-type Si to produce back junction bifacial screen-printed double-side tunnel oxide passivated contacts (DS-TOPCon) solar cells. Optical and device modeling revealed a short circuit current density loss of 1.5 mA/cm 2 and 0.5 mA/cm 2 due to absorption in the front n-TOPCon and rear side p-TOPCon layers, respectively. The passivation and contact properties including metalized and unmetallized recombination current density (J 0 ), as well as contact resistivity, were determined as a function of contact firing temperature in the range of 700~800°C. The passivation quality of the front thin n-TOPCon was found to deteriorate with increased firing temperature while the rear thick p-TOPCon improved. The study showed that the simulated contact firing at 730°C resulted in the best unmetallized double-side TOPCon precursor, with an excellent implied open-circuit voltage of 730 mV and implied fill factor of ~86 %. However, the metalized J0 increased and contact resistivity decreased monotonically with the increase in the firing temperature. The 2D device simulations revealed that these layers can produce screen-printed DS-TOPCon cells with an efficiency of ~22.5 %. Solar cell modeling also showed that the DS-TOPCon solar cell efficiency can reach 24.1 % by decreasing the n-TOPCon thickness to 20 nm and lowering the full area metalized J 0 to ~100 mA/cm 2 .

14 SOLAR ENERGY↗