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At least 343 records · Page 19

Electron densities and the excitation of CN in molecular clouds

In molecular clouds of modest density and relatively high fractional ionization, the rotational excitation of CN is controlled by a competition among electron impact, neutral impact and the interaction with the cosmic background radiation. The degree of excitation can be measured through optical absorption lines and millimeter-wave emission lines. The available, accurate data on CN in diffuse and translucent molecular clouds are assembled and used to determine electron densities. The derived values, n(e) = roughly 0.02 - 0.5/cu cm, imply modest neutral densities, which generally agree well with determinations by other techniques. The absorption- and emission-line measurements of CN both exclude densities higher than n(H2) = roughly 10 exp 3.5/cu cm on scales varying from 0.001 to 60 arcsec in these clouds.

Black, John H.↗

The effect of the solar cycle on the maintenance of the nightside ionosphere of Venus

The behavior of the Venus nightside ionosphere at solar maximum and solar minimum is discussed based on Pioneer Venus radio occultation measurements. Although some solar maximum measurements are similar to those observed at minimum, which have an average peak density of about 7000/cu cm, others show much higher peak densities, reaching values of about 40,000/cu cm. These elevated peak densities also occur at higher altitudes. The integrated electron column densities for these measurements indicate the presence of substantial ionization above the main peak. The magnitudes of both the peak density and the integrated content above the peak are anticorrelated with the solar wind dynamic pressure, indicating that these enhancements during solar maximum are due to transterminator transport of O(+) ions from the dayside. The resulting ionization peak can be many times the concentration produced by energetic electron fluxes impacting the neutral atmosphere on the nightside.

Kliore, Arvydas J.↗

Impact of ionization peak location on measured opaqueness in DIII-D H-mode plasmas

This study investigates the relationship between electron pedestal density and the location of the ionization peak on neutral penetration in DIII-D H-mode plasmas, utilizing a database of Lyman-α emission measurements. The high electron density leads to neutrals being ‘screened’ and the ionization front being pushed out into the Scrape-Off Layer (SOL). This is also referred to as the neutral opaqueness, which is heuristically expected to scale with edge plasma density and machine size. However, at lower electron pedestal density, the penetration depth of the neutrals varies, and measured opaqueness deviates from the heuristic scaling. The database reveals that at low density, when the ionization peak is located in SOL region, the linear relationship between the electron density and neutral penetration holds. However, when the peak is located inside the separatrix, the penetration of the neutrals (λ n 0 ) is much wider ~3.0–3.5 cm, breaking the heuristic opaqueness approximation. These findings provide valuable insights into fueling efficiency and plasma behavior, with implications for Fusion Pilot Plants where high pedestal densities are anticipated and where the neutral opaqueness behaves like its heuristic approximation. This analysis offers a framework to refine neutral opaqueness approximations, enhancing the predictive capability for advanced tokamak operations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Control of electron recollision and molecular nonsequential double ionization

Abstract Intense laser pulses lasting a few optical cycles, are able to ionize molecules via different mechanisms. One such mechanism involves a process whereby within one optical period an electron tunnels away from the molecule, and is then accelerated and driven back as the laser field reverses its direction, colliding with the parent molecule and causing correlated non-sequential double ionization (NSDI). Here we report control over NSDI via spectral-phase pulse shaping of femtosecond laser pulses. The measurements are carried out on ethane molecules using shaped pulses. We find that the shaped pulses can enhance or suppress the yield of dications resulting from electron recollision by factors of 3 to 6. This type of shaped pulses is likely to impact all phenomena stemming from electron recollision processes induced by strong laser fields such as above threshold ionization, high harmonic generation, attosecond pulse generation, and laser-induced electron diffraction.

74 ATOMIC AND MOLECULAR PHYSICS↗

Ionisation cross sections of rare-gas atoms by electron impact

A pulsed electron beam and ion extraction method is used to measure normalized values of partial ionization cross sections for rare gases from threshold to 1000 eV. Cross sections obtained for singly ionized species are used to calibrate the mass transmission efficiency of the ion extraction/analyzer/detection system by the relative flow technique, and this mass transmission curve is then used to determine the absolute cross sections of the multiply ionized species. Total ion cross sections are found by summation of the individual partial cross sections with proper weighting for charge.

Krishnakumar, E.↗

High-energy ballistic electrons in low-pressure radio-frequency plasmas

This study demonstrates the presence of a small number of high-energy ballistic electrons (HEBEs) that originate from secondary electrons in low-pressure radio-frequency (rf) plasmas. The kinetic behaviors of the HEBEs are illustrated through electron energy probability functions from the fully kinetic particle-in-cell simulations, showing two wavy high-energy tails and two bifurcations during one rf cycle. Test-particle simulations and a semi-analytical method associated with nonlocal electron kinetics are performed to characterize the HEBE trajectories, which reveal the ballistic nature of the HEBEs and their typical bouncing features between the rf sheaths. Parameter dependence of the HEBEs on the discharge conditions (e.g., gas pressure, gap distance, and rf frequency) are identified, which is relevant to the plasma collisionality. With a pronounced presence of HEBEs, the overall impacts of the secondary electron emission on discharge parameters, such as electron power absorption and ionization rate, are also illustrated.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Titan's atomic nitrogen torus - Inferred properties and consequences for the Saturnian aurora

A population of warm, approximately keV N(-) ions furnishing the greater part of the mass and energy input to the Titan magnetosphere, at a power level of 2 x 10 to the 11th W, is generated by ionization of Titan's nitrogen torus by both solar EUV photons and magnetospheric electron impact. Magnetospheric electrons also accelerate pickup ions to keV energies by means of lower hybrid emissions, on a time scale comparable to the plasma residence time. It is presently suggested that the aurora is excited by ion and electron precipitation from the outer magnetosphere; the energetics in question can be accounted for entirely on the basis of the titanogenic plasma supply proper to a corotation-dominated magnetosphere.

Barbosa, D. D.↗

Ion formation by electron impact

Dissociative attachment and polar dissociation cross sections were measured for the following molecules: HC1, NO, N2O, C6H6, SiH4, Si2H6, and LiH. Direct ionization and dissociative ionization cross sections were determined for the following molecules: H2, D2, N2, O2, He, Ne, Ar, Kr, Xe, H2O, Co, CO2, CH4, SiH4, Sih4, Si2H6, N2*, and NH3. An experimental apparatus for a pulsed extraction technique was fabricated and successfully tested.

Srivastava, Santosh K.↗

Tunneling-assisted impact ionization for a superlattice

Tunneling-assisted impact ionization across the conduction-band-edge discontinuity of quantum-well heterostructures is investigated and applied to a new superlattice structure. Multiquantum-well structures where the quantum-well regions are heavily doped and the undoped barrier regions are essentially insulating were considered. Incident hot electrons due to the applied electric field perpendicular to the heterointerface interact with the two-dimensional electrons confined to the quantum wells through Coulomb force. The resultant electrons can either have enough energy to get out of the wells or to tunnel through the triangular barriers. A new analytical approximation for the impact ionization rate is given which compares favorably with numerical results. The tunneling-assisted impact ionization rates and the ionization coefficients are calculated. It is shown that the tunneling effect reduces the ionization threshold and enhances the ionization rate significantly.

Chuang, S. L.↗

Electron impact excitation coefficients for laboratory and astrophysical plasmas

Electron impact excitation rate coefficients have been obtained for a number of transitions in highly ionized ions of interest to astrophysical and laboratory plasmas. The calculations were done using the method of distorted waves. Results are presented for various transitions in highly ionized Ne, Na, Al, Si, A, Ca, Ni and Fe.

Davis, J.↗

Periodic variations in Io's sodium and potassium clouds

Spectra of Io's sodium cloud taken 7.5 to 45 sec north and south of Io at a variety of magnetic latitudes of Io obtained during 17 nights of the 1975 apparition of Jupiter confirm the weakening of the cloud in the neighborhood of Jupiter's magnetic equator. The time scale for these changes is 1.5 hours or less. For impact ionization to cause these changes, a minimum flux of 100 billion/sq cm/sec 15 eV electrons or 40 billion/sq cm/sec 8 keV protons is required. Sodium velocities near 10 km/sec are required to explain the replenishment of ionized regions of the cloud. We also obtained spectra of Io's potassium cloud on eight nights during the 1975 apparition. This cloud appears to behave like the sodium cloud as Io's magnetic latitude varies. The potassium, however, may become much weaker as Io passes through the magnetic equator. The brightest intensity measured for the 7665 A resonance line was about 1 kR at a point 7.5 sec east of Io.

Trafton, L.↗

The EUV Emission in Comet-Solar Corona Interactions

The Atmospheric Imaging Assembly (AlA) on the Solar Dynamics Observatory (SDO) viewed a comet as it passed through the solar corona on 2011 July 5. This was the first sighting of a comet by a EUV telescope. For 20 minutes, enhanced emission in several of the AlA wavelength bands marked the path of the comet. We explain this EUV emission by considering the evolution of the cometary atmosphere as it interacts with the ambient solar atmosphere. Water ice in the comet rapidly sublimates as it approaches the Sun. This water vapor is then photodissociated, primarily by Ly-alpha, by the solar radiation field to create atomic Hand O. Other molecules present in the comet also evaporate and dissociate to give atomic Fe and other metals. Subsequent ionization of these atoms can be achieved by a number of means, including photoionization, electron impact, and charge exchange with coronal protons and other highly-charged species. Finally, particles from the cometary atmosphere are thermalized to the background temperature of the corona. Each step could cause emission in the AlA bandpasses. We will report here on their relative contribution to the emission seen in the AlA telescopes.

Bryans, Paul↗

Probing transport energies and defect states in organic semiconductors using energy resolved electrochemical impedance spectroscopy

Abstract Determining the relative energies of transport states in organic semiconductors is critical to understanding the properties of electronic devices and in designing device stacks. Futhermore, defect states are also highly important and can greatly impact material properties and device performance. Recently, energy‐resolved electrochemical impedance spectroscopy (ER‐EIS) is developed to probe both the ionization energy (IE) and electron affinity (EA) as well as sub‐bandgap defect states in organic semiconductors. Herein, ER‐EIS is compared to cyclic voltammetry (CV) and photoemission spectroscopies for extracting IE and EA values, and to photothermal deflection spectroscopy (PDS) for probing defect states in both polymer and molecular organic semiconductors. The results show that ER‐EIS determined IE and EA are in better agreement with photoemission spectroscopy measurements as compared to CV for both polymer and molecular materials. Furthermore, the defect states detected by ER‐EIS agree with sub‐bandgap features detected by PDS. Surprisingly, ER‐EIS measurements of regiorandom and regioregular poly(3‐hexylthiophene) (P3HT) show clear defect bands that occur at significantly different energies. In regioregular P3HT the defect band is near the edge of the occupied states while it is near the edge of the unoccupied states in regiorandom P3HT.

14 SOLAR ENERGY↗

The 825-1110 angstroms EUV spectrum of Venus

On 15 August 1994 we launched the EUVS sounding rocket payload to observe the 825-1110 angstrom region of Venus's far ultraviolet airglow spectrum. The EUVS telescope/spectrograph obtained good data at five times higher spectral resolution than was previously available in the far ultraviolet. We present these data and compare our results to those obtained by the Galileo UVS and Venera 11/12 UV spectrophotometers. We identify several new spectral emission features, including both singly ionized nitrogen and molecular nitrogen in Venus's spectrum. We also see evidence for electron-impact-induced emission from CO. Finally, the EUVS data indicate that the "Ar" emissions detected in Venus's far ultraviolet spectrum by Venera 11/12 spectrophotometers are in fact not due to argon, thus eliminating the discrepancy between in situ and remote sensing measurements.

Flight Experiment↗

Ionization Yield in Silicon for eV-Scale Electron-Recoil Processes

The development of single charge resolving, macroscopic silicon detectors has opened a window into rare processes at the O(eV) scale. In order to reconstruct the energy of a given event, or model the charge signal obtained for a given amount of energy absorbed by the electrons in a detector, an accurate charge yield model is needed. In this paper we review existing measurements of charge yield in Silicon, focusing in particular on the region below 1 keV. We highlight a calibration gap between 12-50 eV (referred to as the "UV-gap") and employ a phenomenological model of impact ionization to explore the likely charge yield in this energy regime. Finally, we explore the impact of variations in this model on a test case, that of dark matter scattering off electrons, to illustrate the scientific impact of uncertainties in charge yield.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Photonuclear Physics in SCALE

Radiation shielding modeling involves a wide range of applications, such as power reactors, critical experiments, portable sources, linear accelerators, and fusion systems. Particle energy ranges vary from thermal energies to fast energy spectra. MAVRIC, as the radiation shielding sequence of the SCALE code system [1] developed and maintained by Oak Ridge National Laboratory, is capable of modeling both neutron and photon interactions in matter and is widely used by the US Nuclear Regulatory Commission, Department of Energy, the National Nuclear Security Administration, and radiation shielding practitioners all around the world. Although most applications don’t involve highly energetic photons that can cause photonuclear reactions and create coupled chains of high energy, ionized electrons and bremsstrahlung radiation within a material medium, when present, these reactions can have a significant impact upon the downstream particle fluxes from incident photons above 20 MeV. For example, linear accelerators used for medical isotope production are examples of applications in which high-energetic photons are generated and used for driving or controlling other components of a complex facility. Radiation shielding analyses of such a facility would require accounting for any and all significant sources of radiation. Unfortunately, MAVRIC included no data and methods to model either photonuclear reactions or the bremsstrahlung photons until this work, which enabled accounting for both. Photonuclear reaction cross sections were imported from the Evaluated Nuclear Data File libraries, and corresponding methods were implemented in the SCALE code system; see Section 2 for how the nuclear data are imported and used. Bremsstrahlung photons were modeled by assuming thick-target approximation whereby all generated electrons and positrons due to photon interactions are assumed to be absorbed within the same material in which they were born, yielding a quick particle transport simulation method by using fast lookup tables for generating subsequent gammas; see Section 4 for details. A suite of verification models was used to test implemented methods and associated data. Tests yielded satisfactory results for the new features. Enhancements will be released as part of the next major SCALE release (v7.0), which is anticipated to be deployed in 2025, with beta releases available in the interim.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Theory of the intercluster medium

A set of computer models for the evolution of intercluster matter (ICM) in expanding cosmologies which includes processes of electron impact ionization/excitation, radiative and dielectronic recombination, thermal bremsstrahlung, Compton scattering, and photoionization is presented. The thermal, ionization, and excitation histories of major constituents were found as functions of time, and predictions of emission spectra, the possible distortions of the cosmic 3 K microwave background, and optical depths of absorption troughs in QSO continua at various redshifts were obtained. It is concluded that the present Friedmann cosmology can be dominated by hot intercluster matter which would contain H and He in their cosmic ratio and traces of heavier elements. For a narrow range of parameters it is possible to generate cosmologies with a closure density of ICM which do not exceed the diffuse X-ray measurements. In open cosmologies distortion of the 3 K microwave background occurs, while closed cases show negligible change from the unperturbed spectrum.

Sherman, R. D.↗