Infrared optical characteristics of ice spheres
Normalized extinction cross section, asymmetry factor, and single-scattering albedo for spherical homogeneous ice particles in infrared region
LIGHT SCATTERING↗
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Geometrical control of topological charge transfer in Shakti-Cairo colloidal ice
Lattice transformations that preserve the system topology, but not its geometry, are common in condensed matter systems. However, how geometric constrains influence the topological properties of the lattices is still unclear. Here we show that a geometric transformation between two mixed coordination lattices, from Shakti to Cairo in an artificial colloidal ice, leads to a breakdown of the ice rule in all but one specific geometry. We observe a transfer of topological charge among sublattices which can be controlled in sign and intensity, vanishing at the ice-rule point. These unusual topological effects are absent in magnetic spin ices and they are due to collective, non-local geometric frustration in the particle ice. By merging numerical simulations, theory and experiments, we demonstrate how the charge transfer occurs in the Cairo geometry. The broader implication of our results is that we demonstrate how geometric constraints can control the topological properties of a mesoscopic colloidal system.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
KAZR Hydrometeor and Insect Masks
The Ka-band ARM zenith pointing radar (aka, KAZR) is so sensitive that it detects cloud particles and individual insects. While detecting insects with Ka-band radar is beneficial and desirable to advance radar entomology, this sensitivity can be detrimental to radar meteorology because insects could be interpreted as clouds or precipitation. For example, misclassifying insects as clouds has been a problem for the ARM Active Remote Sensing of Clouds (ARSCL) Value Added Product since its inception (Clothiaux et al. 2000). Based on cloud particle and insect radar scattering properties, an algorithm was developed that identifies clouds, raindrops, ice particles, and insects in KAZR co- and cross-polarimeteric Doppler velocity spectra. The algorithm produces affirmative masks in the KAZR native time and height resolution indicating time-height locations of hydrometeors and insects. The hydrometeor mask contains binary information (e.g., yes/no hydrometeor presence), and the insect mask includes a proxy for insect activity that increases when more insects are detected in the Doppler velocity spectra. The algorithm was developed using KAZR medium sensitivity mode (MD) observations and was applied to two summer seasons of KAZR observations at the Southern Great Plains (SGP) Central Facility: May-October 2018 and 2019. In the future, this data set will be expanded to include other KAZR operating modes and observations from other ARM field sites. Details of the algorithm and data set can be found in: Williams, C.R., K.L. Johnson, S.E. Giangrande, J. C. Hardin, R. Oktem, and D. M. Romps, 2021: Identifying Insects, Clouds, and Precipitation using Vertically Pointing Polarimetric Radar Doppler Velocity Spectra. Atmospheric Measurement Techniques, submitted 6-Feb-2021. https://amt.copernicus.org/preprints/amt-2021-27/#discussion.For more information on the ARSCL VAP, see Clothiaux, E. E., T. P. Ackerman, G. G. Mace, K. P. Moran, R. T. Marchand, M. A. Miller, and B. E. Martner, 2000; J. Appl. Meteor., 39, 645-665.
54 ENVIRONMENTAL SCIENCES↗
Parameterizations of Depositional Growth of Cloud Ice in a Bulk Microphysical Scheme
Two aspects of the cloud ice parameterization in the Goddard Cumulus Ensemble Model cloud physics parameterization are examined: the conversion of cloud ice to snow by depositional growth, designated PSFI, and the saturation adjustment scheme. The original formulation of PSFI is shown to produce excessive conversion of cloud ice to snow because of an implicit assumption that the relative humidity is 100% with respect to water even though the air may actually be quite less humid. Two possible corrections to this problem are proposed, the first involving application of a relative humidity dependent correction factor to the original formulation of PSFI, and the second involving a new formulation of PSFI based on the equation for depositional growth of cloud ice. The sensitivity of these formulations of PSFI to the assumed masses of the ice particles is examined. Possible problems associated with using a saturation adjustment scheme for cloud ice are discussed and simulations of a squall line with and without application of the adjustment scheme for ice are compared.
Braun, Scott A.↗
Panel Discussion: Life in the Cosmos
Water appears to be essential to all life on Earth. For this reason, "Follow the Water" has been adopted as a mantra for the search for Life in the Cosmos. Expeditions have helped to establish the limits and biodiversity of life in the most extreme environments on Earth. Microbial extremophiles inhabit acidic streams; hypersaline and hyperalkaline lakes and pools; the cold deep sea floor, permafrost, rocks, glaciers, and perennially ice-covered lakes of the polar environments; geysers, volcanic fumaroles, hydrothermal vents and hot rocks deep within the Earth's crust. The ESA Venus Express Spacecraft entered Venusian Orbit in 2006 and continues to produce exciting results. The Visible and Infrared Thermal Imaging Spectrometer (VIRTIS) instrument made the first detection of hydroxyl in the atmosphere of Venus, indicating it is much more similar to Earth and Mars than previously thought. Huge hurricane-like vortices have been found above the poles of the planet and as yet unidentified UV absorbers that form mysterious dark bands in the upper atmosphere. At 70 km and below, water vapor and sulfur dioxide combine to form sulfuric acid droplets that create a haze above the cloud tops. Thermophilic acidophiles, such as have recently been discovered on Earth, could possibly survive in the hot sulfuric acid droplets that exist in the upper atmosphere of Venus. In order to understand how to search for life elsewhere in the Solar System, over 40 VIRTIS images of Earth from Venus have been obtained to search for evidence of life on Earth. The signatures of water and molecular Oxygen were detected in the Earth s atmosphere, but the atmosphere of Venus also exhibits these signatures. The water and water ice are far more abundant on comet, the polar caps and permafrost of Mars and the icy moons of Jupiter and Saturn. These "frozen worlds" of our Solar System, are much more promising regimes where extant or extinct microbial life may exist. The ESA Mars Advanced Radar for Subsurface and Ionospheric Sounding (MARSIS) probe has found that both the North and South Polar Caps of Mars are approximately 3.5 km thick and are composed almost entirely of water ice. In winter, a thin dry ice layer covers the caps, but it sublimates directly to CO2 in the spring. The ESA Mars Express Orbiter images reveal Rupes Tenuis to be a vast snow-laden region on the southern edge of the Martian North Polar Cap. The Mars Exploration Rover Spirit found alkaline volcanic rocks in the Gusev Crater and the Phoenix Mars Lander has shown that the soil of Mars is much more alkaline than previously expected. The Phoenix Mars Lander has also made direct observations of frozen and liquid water on Mars. It is known that microorganisms from Alaska, Siberia and Antarctica can remain alive frozen in permafrost or ice for long periods of time. These discoveries increase the possibility that the Labeled Release Experiment may have discovered life on Mars during the Viking Mission and provide strong impetus for the return of life detection experiments to Mars. Changes in the spin rate of Saturn's moon Titan indicate that it may also harbor a 300 km thick liquid water ocean beneath its icy crust. The NASA/ESA/Italian Space Agency Cassini Spacecraft has imaged geysers containing water vapor, methane, carbon dioxide and organics erupting from the "tiger stripe" regions near the South Pole of Saturn's moon Enceladus. The high temperatures observed, the water vapor and large number of ice particles expelled suggest that a liquid water lake may exist beneath the "tiger stripe" ice cracks of Enceladus. The NASA Deep Impact probe found the surface temperature of comet 9P/Temple 1 at 1.5 AY was slightly above the ice/water phase change temperature (273 K). This suggests melting of water ice near the comet surface. A spectrometer the spacecraft detected a mixture of clay and carbonate minerals (that form in the presence of liquid water) streaming off the comet after the collision with the pactor. The study of chemical and mineral biomarkers, chiral amino acids and possible indigenous microfossils in SNC and carbonaceous meteorites continues. These results suggest that comets should be considered prime targets in the search for Life in the Cosmos. The ESA Rosetta mission is on track to rendezvous with comet 67P/Churyumov-Gerasimenko. The recent space observations combined with new information about the ability of microbial extremophiles to thrive in polar environments suggest that life may be far more widely distributed in the Cosmos than previously thought possible. The Panelists will review recent discoveries and provide their own insights about Life in the Cosmos -- followed by a question and answer session with the audience.
Hoover, Richard B.↗
Ice Cloud Backscatter Study and Comparison with CALIPSO and MODIS Satellite Data
An invariant imbedding T-matrix (II-TM) method is used to calculate the single-scattering properties of 8-column aggregate ice crystals. The II-TM based backscatter values are compared with those calculated by the improved geometric-optics method (IGOM) to refine the backscattering properties of the ice cloud radiative model used in the MODIS Collection 6 cloud optical property product. The integrated attenuated backscatter-to-cloud optical depth (IAB-ICOD) relation is derived from simulations using a CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite) lidar simulator based on a Monte Carlo radiative transfer model. By comparing the simulation results and co-located CALIPSO and MODIS (Moderate Resolution Imaging Spectroradiometer) observations, the non-uniform zonal distribution of ice clouds over ocean is characterized in terms of a mixture of smooth and rough ice particles. The percentage of the smooth particles is approximately 6 percent and 9 percent for tropical and mid-latitude ice clouds, respectively.
MODIS↗
An overview of shed ice impact in the NASA Lewis Icing Research Tunnel
One of the areas of active research in commercial and military rotorcraft is directed toward developing the capability of sustained flight in icing conditions. The emphasis to date has been on the accretion and subsequent shedding of ice in an icing environment, where the shedding may be natural or induced. Historically, shed-ice particles have been a problem for aircraft, particularly rotorcraft. Because of the high particle velocities involved, damage to a fuselage or other airframe component from a shed-ice impact can be significant. Design rules for damage tolerance from shed-ice impact are not well developed because of a lack of experimental data. Thus, NASA Lewis (LeRC) has begun an effort to develop a database of impact force and energy resulting from shed ice. This effort consisted of a test of NASA LeRC's Model Rotor Test Rig (MRTR) in the Icing Research Tunnel (IRT). Both natural shedding and forced shedding were investigated. Forced shedding was achieved by fitting the rotor blades with Small Tube Pneumatic (STP) deicer boots manufactured by BF Goodrich. A detailed description of the test is given as well as the design of a new impact sensor which measures the force-time history of an impacting ice fragment. A brief discussion of the procedure to infer impact energy from a force-time trace are required for the impact-energy calculations. Recommendations and future plans for this research area are also provided.
Bond, Thomas H.↗
An overview of shed ice impact studies in the NASA Lewis Icing Research Tunnel
One of the areas of active research in commercial and military rotorcraft is directed toward developing the capability of sustained flight in icing conditions. The emphasis to date has been on the accretion and subsequent shedding of ice in an icing environment, where the shedding may be natural or induced. Historically, shed-ice particles have been a problem for aircraft, particularly rotorcraft. Because of the high particle velocities involved, damage to a fuselage or other airframe component from a shed-ice impact can be significant. Design rules for damage tolerance from shed-ice impact are not well developed because of a lack of experimental data. Thus, NASA Lewis (LeRC) has begun an effort to develop a database of impact force and energy resulting from shed ice. This effort consisted of a test of NASA LeRC's Model Rotor Test Rig (MRTR) in the Icing Research Tunnel (IRT). Both natural shedding and forced shedding were investigated. Forced shedding was achieved by fitting the rotor blades with Small Tube Pneumatic (STP) deicer boots manufactured by BF Goodrich. A detailed description of the test is given as well as the design of a new impact sensor which measures the force-time history of an impacting ice fragment. A brief discussion of the procedure to infer impact energy from a force-time trace are required for the impact-energy calculations. Recommendations and future plans for this research area are also provided.
Britton, Randall K.↗
Further Research on the Electrification of Pyrocumulus Clouds
Past research on pyrocumulus electrification has demonstrated that a variety of lightning types can occur, including cloud‐to‐ground (CG) flashes, sometimes of dominant positive polarity, as well as small intra‐cloud (IC) discharges in the upper levels of the pyro‐cloud. In Colorado during summer 2012, the first combined polarimetric radar, multi‐Doppler radar, and three‐dimensional lightning mapping array (LMA) observations of lightning‐producing pyrocumulus were obtained. These observations suggested that the National Lightning Detection Network (NLDN) was not sensitive enough to detect the small IC flashes that appear to be the dominant mode of lightning in these clouds. However, after an upgrade to the network in late 2012, the NLDN began detecting some of this pyrocumulus lightning. Multiple pyrocumulus clouds documented by the University of Wisconsin for various fires in 2013 and 2014 (including over the Rim, West Fork Complex, Yarnell Hill, Hardluck, and several other incidents) are examined and reported on here. This study exploits the increased‐sensitivity NLDN as well as the new nationwide U.S. network of polarimetric Next‐generation Radars (NEXRADs). These observations document the common occurrence of a polarimetric "dirty ice" signature ‐ modest reflectivities (20‐40+ dBZ), near‐zero differential reflectivity, and reduced correlation coefficient (less than 0.9) ‐ prior to the production of lightning. This signature is indicative of a mixture of ash and ice particles in the upper levels of the pyro‐cloud (less than ‐20 C), with the ice interpreted as being necessary for pyro‐cloud electrification. Pseudo‐Geostationary Lightning Mapper (GLM) data will be produced from the 2012 LMA observations, and the ability of GLM to detect small pyrocumulus ICs will be assessed. The utility of lightning and polarimetric radar for documenting rapid wildfire growth, as well as for documenting pyrocumulus impacts on the composition of the upper troposphere/lower stratosphere (UTLS), will be discussed.
Lang, Timothy J.↗
Airborne measurements of cloud forming nuclei and aerosol particles at Kennedy Space Center, Florida
Results of airborne measurements of the sizes and concentrations of aerosol particles, ice nuclei, and cloud condensation nuclei that were taken at Kennedy Space Center, Florida, are presented along with a detailed description of the instrumentation and measuring capabilities of the University of Washington airborne measuring facility (Douglas B-23). Airborne measurements made at Ft. Collins, Colorado, and Little Rock, Arkansas, during the ferry of the B-23 are presented. The particle concentrations differed significantly between the clean air over Ft. Collins and the hazy air over Little Rock and Kennedy Space Center. The concentrations of cloud condensation nuclei over Kennedy Space Center were typical of polluted eastern seaboard air. Three different instruments were used to measure ice nuclei: one used filters to collect the particles, and the others used optical and acoustical methods to detect ice crystals grown in portable cloud chambers. A comparison of the ice nucleus counts, which are in good agreement, is presented.
Radke, L. F.↗
Experimental studies of gas trapping in amorphous ice and thermal modelling of comets: Implications for Rosetta
The trapping of mixtures of CO, CH4, N2 and Ar in amorphous water ice was studied experimentally. It is shown that the ice particles could not have been formed at a higher temperature and, subsequently, cool down. Experiments where ice was deposited at elevated temperatures, then cooled down and gas was flowed into the ice, showed that the amount of trapped gas depends only on the highest temperature at which the ice was formed, or resided, prior to cooling and gas flow into it. Consequently, the cometary ice had to be formed at approx. 48 K and the ice is therefore amorphous. The thermal profile of a comet in Halley's orbit was calculated, including the build-up of an insulating dust layer. It was found that an insulating dust layer a few cm thick is enough to choke most of the water emission from the surface. A similar thermal model was calculated for comet P/Temple-1, a candidate for both CRAF and Rosetta (CNSR) missions. The temperature at a depth of 10 m is approx. 160 K for all models considered and, hence, the ice at this depth is crystalline. A crystalline ice layer 40 to 240 m thick was found to overly the gas-laden amorphous ice. Consequently, it should be difficult for the probes of the two comet missions to sample pristine amorphous ice, unless they are aimed at the bottom of an active crater.
Bar-Nun, Akiva↗
Computerized reduction of airborne foil impactor data
A new technique for reducing data obtained from a foil impactor carried on the T-28 thunderstorm penetration aircraft is described. The technique employs a video-image processing system that was originally developed for satellite imagery and a computer-reduction program that was originally developed for determining cloud-size distributions to count and size particle impressions on the foil. This eliminates the tedious manual processing that has limited the usefulness of such devices, while at the same time improving objectivity. The technique has been applied to foil data acquired in thunderstorms in the southeastern United States during the Cooperative Huntsville Meteorological Experiment, where most of the particles were at least roughly spherical. Its usefulness for storms in which highly irregular or fragile ice particles predominate has yet to be established.
Peterson, Bret A.↗
Martian North Polar Water-Ice Clouds During the Viking Era
The Viking Orbiters determined that the surface of Mars' northern residual cap consists of water ice. Observed atmospheric water vapor abundances in the equatorial regions have been related to seasonal exchange between reservoirs such as the polar caps, the regolith and between different phases in the atmosphere. Kahn modeled the physical characteristics of ice hazes seen in Viking Orbiter imaging limb data, hypothesizing that ice hazes provide a method for scavenging water vapor from the atmosphere and accumulating it into ice particles. Given that Jakosky found that these particles had sizes such that fallout times were of order one Martian sol, these water-ice hazes provided a method for returning more water to the regolith than that provided by adsorption alone. These hazes could also explain the rapid hemispheric decrease in atmospheric water in late northern summer as well as the increase during the following early spring. A similar comparison of water vapor abundance versus polar cap brightness has been done for the north polar region. They have shown that water vapor decreases steadily between L(sub s) = 100-150 deg while polar cap albedo increases during the same time frame. As a result, they suggested that late summer water-ice deposition onto the ice cap may be the cause of the cap brightening. This deposition could be due to adsorption directly onto the cap surface or to snowfall. Thus, an examination of north polar waterice clouds could lend insight into the fate of the water vapor during this time period. Additional information is contained in the original extended abstract.
Tamppari, L. K.↗
The Polar Summer MLT Plasma Environment as seen by the DROPPS Sounding Rockets
During early July, 1999, the DROPPS (Distribution and Role of Particles in the Polar Summer Mesosphere) campaign launched two rocket payloads whose purpose was to study the polar summer MLT (mesosphere and lower thermosphere), particularly PMSEs (polar mesospheric summer echoes) and PMCs (polar mesospheric clouds). The rockets were launched from the And(\o)ya Rocket Range in Norway the nights of the 5th and 14th of July. Both payloads included a front-mounted PID (Particle Impact Detector) consisting of charge and mass telescopes to measure aerosol and dust mass distributions. Ice particles of nanometer size are believed to be responsible for PMSEs through the process of electron scavenging. Evidence for this process is suggested, for example, by the presence of an electron "biteout" simultaneously measured by several instruments at an altitude of $\sim$82-87 km during the first DROPPS launch. This presentation will characterize similarities and differences between both flights as seen by the charge and mass telescopes, starting at launch until the loss of data on the downleg of each flight. Various stages of the flights will be considered in detail, such as the PMSE layer and the apogee at 117 km, as well as the calibration of the data before launch.
Assis, Michael P.↗
The Polar Summer MLT Plasma Environment as Seen by the DROPPS Sounding Rockets
During early July, 1999, the DROPPS (Distribution and Role of Particles in the Polar Summer Mesosphere) campaign launched two rocket payloads whose purpose was to study the polar summer MLT (mesosphere and lower thermosphere), particularly PMSEs (polar mesospheric summer echoes) and PMCs (polar mesospheric clouds). The rockets were launched from the Anderya Rocket Range in Norway the nights of the 5th and 14th of July. Both payloads included a front-mounted PID (Particle Impact Detector) consisting of charge and mass telescopes to measure aerosol and dust mass distributions. Ice particles of nanometer size are believed to be responsible for PMSEs through the process of electron scavenging. Evidence for this process is suggested, for example, by the presence of an electron "biteout" simultaneously measured by several instruments at an altitude of approx. 82 - 87km during the first DROPPS launch. This presentation will characterize similarities and differences between both flights as seen by the charge and mass telescopes, starting at launch until the loss of data on the downleg of each flight. Various stages of the flights will be considered in detail, such as the PMSE layer and the apogee at 117 km, as well as the calibration of the data before launch.
Assis, Michael P.↗
Coagulation of particles in Saturn's rings - Measurements of the cohesive force of water frost
Experimental data are presented on the sticking force of water ice particles which are indicative of the role that the cohesive properties of such particles could play in the dynamics of Saturn ring particles. Sticking forces are dependent on particle impact velocities; a 'Velcro' model is devised to describe the surface structure involved in sticking. The data indicate that below the critical impact velocity of about 0.03 cm/sec, particle cohesion always occurs. Due to the optical depth of micron-sized grains in the Saturn rings, particles are hypothesized to be coated with a layer of frost which will render cohesion an important ring-dynamics process.
Hatzes, A. P.↗
Relationships between Immersion Freezing and Crystal Habit for Arctic Mixed-Phase Clouds—A Numerical Study
Abstract The number concentration of ice particles in Arctic mixed-phase clouds is a major controlling factor of cloud lifetime. The relationships between ice nucleation mode and ice crystal habit development are not yet constrained by observations. This study uses a habit-predicting microphysical scheme within a 3D large-eddy simulation model to evaluate the relationship between immersion freezing and ice habit in a simulated Arctic mixed-phase cloud case. Three immersion freezing parameterizations are considered: a volume-dependent freezing scheme (VF), a parameterization limited to activated droplets (C-AC), and a parameterization limited to coarse aerosol particles (C-CM). Both C-AC and C-CM are based on classical nucleation theory. The freezing rate with VF is found to be greater in downdraft regions than in updraft regions due to the downdraft having a higher number concentration of large droplets. The C-AC cases show active freezing of small droplets near cloud top, whereas in the C-CM cases, mainly the 8–32- μ m-sized droplets freeze in updraft regions near the cloud base. Because the initial crystal size is assumed to affect the axis ratio of hexagonal plates, the VF cases produce crystals with larger axis ratios, resulting in smaller mode radii than the C-AC cases. In all cases, irregular polycrystals dominate near cloud top and a band-like structure develops within the cloud, which qualitatively agrees with previous observations. In the VF and C-CM cases, unactivated large droplets arising from coarse-mode aerosol particles contributed significantly to the freezing rate, producing an important influence on crystal habit.
54 ENVIRONMENTAL SCIENCES↗
The effects of small ice crystals on the infrared radiative properties of cirrus clouds
To be successful in the development of satellite retrieval methodologies for the determination of cirrus cloud properties, we must have fundamental scattering and absorption data on nonspherical ice crystals that are found in cirrus clouds. Recent aircraft observations (Platt et al. 1989) reveal that there is a large amount of small ice particles, on the order of 10 micron, in cirrus clouds. Thus it is important to explore the potential differences in the scattering and absorption properties of ice crystals with respect to their sizes and shapes. In this study the effects of nonspherical small ice crystals on the infrared radiative properties of cirrus clouds are investigated using light scattering properties of spheroidal particles. In Section 2, using the anomalous diffraction theory for spheres and results from the exact spheroid scattering program, efficient parameterization equations are developed for calculations of the scattering and absorption properties for small ice crystals. Parameterization formulas are also developed for large ice crystals using results computed from the geometric ray-tracing technique and the Fraunhofer diffraction theory for spheroids and hexagonal crystals. This is presented in Section 3. Finally, applications to the satellite remote sensing are described in Section 4.
Takano, Y.↗