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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 343 records · Page 19

Structural characterization and gas reactions of small metal particles by high-resolution TEM and TED

The interaction of 100 and 200 keV electron beams with amorphous alumina, titania, and aluminum nitride substrates and nanometer-size palladium particulate deposits was investigated for the two extreme cases of (1) large-area electron-beam flash-heating and (2) small-area high-intensity electron-beam irradiation. The former simulates a short-term heating effect with minimum electron irradiation exposure, the latter simulates high-dosage irradiation with minimum heating effect. All alumina and titania samples responded to the flash-heating treatment with significant recrystallization. However, the size, crystal structure, shape, and orientation of the grains depended on the type and thickness of the films and the thickness of the Pd deposit. High-dosage electron irradiation also readily crystallized the alumina substrate films but did not affect the titania films. The alumina recrystallization products were usually either all in the alpha phase, or they were a mixture of small grains in a number of low-temperature phases including gamma, delta, kappa, beta, theta-alumina. Palladium deposits reacted heavily with the alumina substrates during either treatment, but they were very little effected when supported on titania. Both treatments had the same, less prominent localized crystallization effect on aluminum nitride films.

Heinemann, K.↗

Measurement of gamma-induced reactions between 10 and 19 MeV on natural zinc with potential application to 67 Cu production

As part of a broader campaign to understand gamma-induced charged particle emission with multiple materials, the cross sections of the (γ, p), and (γ, α) reactions on a natural zinc target were measured. Here, these cross sections were measured experimentally using a kinematically-complete, event-by-event methodology, using monoenergetic gamma ray beams from the High Intensity Gamma Source (HIγS) facility, ranging from 10 to 19 MeV, to bombard a natural metallic zinc target in vacuum. The measured cross sections are compared with theoretical predictions using the statistical model approach, which is important for the use of such models in real-world applications such as the production of the 67 Cu theranostic via the 68 Zn(γ, p) reaction.

Gamma-induced reactions↗

Neutrinos and Dark Matter Across Energies and Epochs (Final Technical Report)

The opportunities afforded by upcoming next-generation neutrino experiments offer new physics potential that is complementary to high-energy collider searches. Although much lower in energy, the combination of large detectors and high intensity proton beams yields novel sensitivity to new physics. The types of new physics signals include both those which are terrestrially sourced as well as astrophysically produced. Within this project specific focuses include: (1) BSM searches at neutrino and dark matter experiments to look for axion-like particles, heavy neutrinos, and new force carriers; and (2) BSM signals from astrophysics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Feasibility study: Monodisperse polymer particles containing laser-excitable dyes

The optical properties associated with small particles, which include aerosols, hydrosols and solid microspheres have an impact on several areas of science and engineering. Since the advent of high-speed computers and lasers, the interaction of light with matter in the form of small particles with a discontinuous optical boundary relative to the surroundings has been much better understood. Various nonlinear optical effects have been observed involving interaction of a laser beam with both solid microspheres and liquid microdroplets. These include observation of second and third harmonic generation, four wave mixing, optical visibility, two photon absorption, observation of stimulated emission and lasing, and Stimulated Raman Scattering. Many of these effects are observed with laser intensities which are orders of magnitude less than that required by threshold condition for interactions in macroscopic bulk medium. The primary reason for this is twofold. The front surface of the microsphere acts as a thick lens to enhance the internal intensity of the input laser radiation, and the spherical shape of the droplet acts as an optical cavity to provide feedback at specific wavelengths corresponding to the whispering gallery modes or the morphology dependent resonances (MDR's). The most interesting and significant recent finding in this field is undoubtedly the existence of resonance peaks in linear and nonlinear optical spectra. Such resonance peaks are only dependent on the particle morphology, which means the size, shape and refractive index of the particle. Because of the simultaneous presence of these resonances, they have been referred to by many names, including structural resonances, whispering modes or whispering gallery modes, creeping waves, circumferential waves, surfaces modes, and virtual modes. All of these names refer to the same phenomena, i.e. morphology dependent resonances (MDR's) which has already been described and predicted precisely by electromagnetic theory and Loentz-Mie theory since 1908. MDR's can become important when the particle size (radius a) approaches and exceeds the wavelength of the electromagnetic wave (lambda) and the refractive index of the particle is greater than that of the surrounding medium. Such resonances are easiest to observe from a single particle with high symmetry, such as a sphere, spheroid, or cylinder. MDR's correspond to solutions of the characteristic equations of the electromagnetic fields in the presence of a sphere.

Venkateswarlu, Putcha↗

Towards the optimization of direct laser acceleration

Experimental measurements using the OMEGA EP laser facility demonstrated direct laser acceleration (DLA) of electron beams to (505 ± 75) MeV with (140 ± 30) nC of charge from a low-density plasma target using a 400 J, picosecond duration pulse. Similar trends of electron energy with target density are also observed in self-consistent two-dimensional particle-in-cell simulations. The intensity of the laser pulse is sufficiently large that the electrons are rapidly expelled from along the laser pulse propagation axis to form a channel. The dominant acceleration mechanism is confirmed to be DLA and the effect of quasi-static channel fields on energetic electron dynamics is examined. A strong channel magnetic field, self-generated by the accelerated electrons, is found to play a comparable role to the transverse electric channel field in defining the boundary of electron motion.

43 PARTICLE ACCELERATORS↗

Cross-Beam Energy Transfer Saturation by Ion Heating

Cross-beam energy transfer (CBET) saturation by ion heating was measured in a gas-jet plasma characterized using Thomson scattering. Here, a wavelength-tunable ultraviolet (UV) probe laser beam was interacted with four intense UV pump beams to drive large-amplitude ion-acoustic waves. For the highest-intensity interactions, the power transferred to the probe laser dropped, demonstrating ion-acoustic wave saturation. Over this time, the ion temperature was measured to increase by a factor of 7 during the 500-ps interaction. Particle-in-cell simulations show ion trapping and a subsequent ion heating consistent with measurements. Linear kinetic CBET models were found to agree well with the observed energy transfer when the measured plasma conditions were used.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Artificial auroras in the upper atmosphere. II - Imaging results

On the ATLAS 1 mission (STS-45, launched March 24, 1992) two experiments, AEPI (Atmospheric Emissions Photometric Imaging) and SEPAC (Space Experiments with Particle Accelerators) performed the first of a series of active experiments intended to probe the atmosphere, ionosphere and magnetosphere with electron beams. The luminous artificial aurora generated by the electron beam interaction was detected and measured by AEPI both in white light and in a narrow wavelength band at 427.8 nm (peak intensity 5 kR). Modelling calculation showed that there was a significant contribution from emissions originating near the spacecraft. The spatial intensity distribution of the observed auroral patch is consistent with emission contribution from both high and low altitude regions. An extended tail in the direction of the shuttle wake was observed in the 427.8 nm channel, consistent with a decay time associated with the dissipation of the hot electron plasma.

Mende, S. B.↗

Synchrotron X-Ray Diffraction Studies of Olivine from Comet Wild 2

We have analyzed a collection of the Comet Wild 2 coma grains returned by the NASA Stardust Mission, using micro-area Laue diffraction equipment. The purpose of the diffraction experiment is to permit the structure refinement of olivine including site occupancies. In addition to the intrinsic importance of the olivine structures for revealing the thermal history of Wild 2 materials, we wish to test reports that olivine recovered after hypervelocity capture in silica aerogel has undergone a basic structural change due to capture heating [1]. The diffraction equipment placed at beam line BL- 4B1 of PF, KEK was developed with a micropinhole and an imaging plate (Fuji Co. Ltd.) using the Laue method combined with polychromatic X-ray of synchrotron radiation operated at energy of 2.5 GeV. The incident beam is limited to 1.6 m in diameter by a micropinhole set just upstream of the sample [2, 3]. It is essential to apply a microbeam to obtain diffracted intensities with high signal to noise ratios. This equipment has been successfully applied to various extraterrestrial materials, including meteorites and interplanetary dust particles [4]. The Laue pattern of the sample C2067,1,111,4 (Fig. 1) was successfully taken on an imaging plate after a 120 minute exposure (Fig. 2).

Source record↗

Design of a broadband, high-power, off-axis spiral polarization reflector

Spirally polarized beams are known to produce a strong longitudinal field under high numerical aperture focusing. Here, we report on the design of a reflective optical element with an off-axis geometry that is capable of transforming a uniformly polarized beam into a predominantly spirally polarized beam. By utilizing the retardance present in Fresnel reflection, our device can operate over a broad range of wavelengths. The output polarization and intensity structure of a beam passing through the reflector are calculated using polarization and scalar ray tracing. Vector diffraction is used to calculate the polarization and intensity structure under $f/0.656$ focusing. The off-axis reflective design is well-suited for high-power laser applications and could enable current and future laser-based particle accelerators to achieve strong longitudinal fields at focus.

Black, A. Nicholas [Univ. of Rochester, NY (United↗

Ionization-Based Optical Structures for the Control of Short-Pulse Lasers (Full LDRD Report)

High-power lasers require enormous beam sizes to avoid optics damage; without plasma control of light, future higher-power systems will have prohibitive costs. The laser-induced formation of ionization patterns in gases provides an opportunity to manipulate the spatial and temporal properties of femtosecond to picosecond beams with precise control at high intensity, providing a path towards compact multi-petawatt lasers. In this project, we proposed new concepts of diffractive optics elements relying on ionization-based structures, including a holographic lens and a compression grating. The theoretical characterization of these optical elements was supported by particle-in-cell simulations. Experiments have been carried out to achieve reflective elements (i.e., plasma-based gratings) that demonstrated high robustness and efficiencies on the order of 50%, which validates the feasibility of our new concepts and paves the way for future plasma-based high-power laser systems.

47 OTHER INSTRUMENTATION↗

Retrieving images from tarnished daguerreotypes using X-ray fluorescence imaging with an X-ray micro beam with tunable energy

We report recent observations using a synchrotron X-ray micro-beam to retrieve images from tarnished 19th century daguerreotypes. We confirm that high quality image can always be retrieved from tarnished plates using Hg L α XRF as long as the bulk of the image particles and their distribution remains intact. We also report results from using tunable tender X-rays (2 - 7 keV) to conduct imaging in high vacuum at energy above the Ag L-edge and the Hg M-edge, extracting images using Ag L α and Hg M α , respectively among others (e.g., S to track corrosion). Images obtained with the surface sensitive total electron yield (TEY) and the bulk sensitive fluorescence yield (FLY) as well as corresponding micro-XANES are reported. Flux tolerance to high intensity X-beam is also explored. These results and their implications for cultural heritage research are discussed.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Magnetosheath bursts of predominantly medium nuclei observed with Imp 8 on February 16, 1974

This paper presents observations made with detectors aboard Imp 8 of a unique series of charged particle bursts that occurred on February 16, 1974, while the spacecraft was traversing the dawn magnetosheath region. This event was unlike any other observation of Imp 7 and 8 in 5.5 years of operation in orbit. The measurements are most directly interpreted as an intense (6000/(sq cm s sr MeV/nucleon)), highly collimated beam flowing in the antisolar direction composed of medium (carbon, nitrogen, or oxygen) nuclei. Both the degree of collimation in arrival direction and the composition are unique to this event. The event is possibly an important signature of terrestrial O(+) ions escaping from the magnetosphere.

Armstrong, T. P.↗

Broadband hard X-ray attosecond pulses from extremely chirped electron beams

Attosecond pulses from free-electron lasers have opened the doors to atomic site-specific studies of bound electronic dynamics on their natural, sub-femtosecond timescales. Key to their success has been electron beam shaping techniques enabling the generation of sub-femtosecond current spikes with peak currents on the order of 10 kA. We demonstrate in an RF linac the generation of current spikes with extreme chirps on the order of 350 MeV/micron, directly competitive with the chirps expected from beam-driven plasma wakefield accelerators. Leveraging chirp-taper compensation, we use these highly chirped beams to generate hard X-ray attosecond pulses with bandwidths exceeding 30 eV, a factor of two beyond previous demonstrations. We simultaneously present the first explicit experimental evidence of chirp-taper compensation in an attosecond XFEL, finding that optimal tapering improves the bandwidth and pulse energy by factors of two and five, respectively, for our conditions. In addition to the immediate utility of such broadband hard X-ray pulses, electron beams with such extreme chirps can be utilized for unique new experimental modalities by performing further compression after the undulators. Such post-lasing compression can enable subsequent superradiant light emission at longer wavelengths, or direct excitation of quantum systems with the beam's intense space-charge field for unique attosecond pump-probe possibilities.

43 PARTICLE ACCELERATORS↗

The Search for μ+ → e+γ with 10–14 Sensitivity: The Upgrade of the MEG Experiment

The MEG experiment took data at the Paul Scherrer Institute in the years 2009–2013 to test the violation of the lepton flavor conservation law, which originates from an accidental symmetry that the Standard Model of elementary particle physics has, and published the most stringent limit on the charged lepton flavor violating decay μ+→e+γ: BR(μ+→e+γ) <4.2×10−13 at 90% confidence level. The MEG detector has been upgraded in order to reach a sensitivity of 6×10−14. The basic principle of MEG II is to achieve the highest possible sensitivity using the full muon beam intensity at the Paul Scherrer Institute (7×107 muons/s) with an upgraded detector. The main improvements are better rate capability of all sub-detectors and improved resolutions while keeping the same detector concept. In this paper, we present the current status of the preparation, integration and commissioning of the MEG II detector in the recent engineering runs.

physics beyond the Standard Model↗

Electron cloud simulations in the Fermilab booster

As part of Fermilab's Proton Improvement Plan-II (PIP-II),the Fermilab Booster synchrotron will operate at a higherintensity, increasing from 4.5 x 10^12 to 6.7 x 10^12 protons per pulse (ppp). A potential challenge for achievinghigh intensity performance arises from rapid transverse instabilities induced by electron cloud (EC). This researchpresents EC simulations using PyECLOUD, which is anadvanced computational tool that incorporates measurements of the secondary electron yield (SEY) from theBooster's combined function magnet material. By systematically varying beam parameters in PyECLOUD, such asbunch structure, SEY, bunch length, and intensity, it becomes possible to forecast the impact of EC effects on thebeam stability of the PIP-II era Booster.

43 PARTICLE ACCELERATORS↗

Proposal for a Proton-Bunch Compression Experiment at IOTA in the Strong Space-Charge Regime

The longitudinal compression of intense proton bunches with strong space-charge force is an essential component of a proton-based muon source for a muon collider. This paper discusses a proton-bunch compression experiment at the Integrable Optics Test Accelerator (IOTA) storage ring at Fermilab to explore optimal radio frequency (RF) cavity and lattice configurations. IOTA is a compact fixed-energy storage ring that can circulate a 2.5-MeV proton beam with varying beam parameters and lattice configurations. The study will aim to demonstrate a bunch-compression factor of at least 2 in the IOTA ring while examining the impact of intense space-charge effects on the compression process.

43 PARTICLE ACCELERATORS↗

Status of the Mu2e experiment at Fermilab

The Mu2e experiment at Fermilab aims to measure the charged-lepton flavour violating (CLFV) neutrino-less conversion of a negative muon into an electron in the field of a nucleus with an unprecedented single event sensitivity of 3x10^{-17}. This document illustrates the physics motivation and design of the experiment.In the current schedule Mu2e is expected to start taking data in 2025 with a reduced average beam intensity for about two years (Run 1). After a shut down for the upgrade of Fermilab accelerator complex, data taking will restart at full beam intensity (Run 2). A detailed update of the expected experiment sensitivity for Mu2e Run 1 is presented, together with an estimate of the final Mu2e sensitivity.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗