DOE OSTI2016
In this paper, the possibility of using an accelerator-driven subcritical reactor to produce helium-3 is explored. Current supply of helium-3 in the United States is running low. Helium-3 has many applications in neutron detection, high-energy physics, and national security, and has a growing demand in the scientific community for its properties. The main source of helium-3 in the United States is from dismantling nuclear arms, where tritium is allowed to decay into helium-3. There are no current, significant future plans for increasing helium-3 production. However, the projected demand of this isotope is expected to increase dramatically, with greater research into aneutronic fusion, and allotments of helium for the Spallation Neutron Source, and ITER expected in years to come. Tritium, with a half-life of 12.3 years, will take time to decay to helium-3, which means production needs to start now to counter the future deficit. This helium-3 production system sets out to be an economical, and safe solution for this future deficit. A zirconium-lithium mixture is utilized as a target for breeding helium-3. Specifically, the target rods will consist of lithium aluminate pellets with diameters ranging from 100 to 500 microns, dispersed within a zirconium matrix. Lithium targets in pellet form were chosen over a solid rod, or annulus, in order to reduce self-shielding effects within the lithium, and to further facilitate tritium loading and containment within the zirconium. Additionally, a stainless steel 316 cladding surrounds the target rods, to further reduce outgassing of helium. The core is made up of 6480 fuel pins, enriched to 4.75% wt% U-235/U, and 3660 lithium pins in mixed assemblies arranged in hexagonal lattices, with the lithium enriched to 75% lithium-6, and a total lithium loading of approximately 70 kg. An accelerator is used as a neutron source, firing 800 MeV protons at a liquid lead target loop. Neutronics analysis and burnup calculation were performed with the aid of MCNP6. (authors)
07 ISOTOPE AND RADIATION SOURCES↗