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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 343 records · Page 19
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Probing circular polarization and magnetic field structure in active galactic nuclei

The composition and magnetic field morphology of relativistic jets can be studied using circular polarization (CP) measurement. Recent three-dimensional relativistic magnetohydrodynamic (3D RMHD) simulations coupled with radiative transfer (RT) calculations make strong predictions about the level (and morphology) of the jet’s CP emission. These simulations show that the sign of CP and the electric vector position angle (EVPA) are both sensitive to the jet’s magnetic field morphology within the radio core. We probe this theory by exploring whether the jet’s radio core EVPA orientation is consistent with the observed sign of the core CP in deep full-track polarimetric observations. Based on a selection of sources from earlier MOJAVE observations, we aim to probe the nature of linear polarization (LP) and CP in the innermost regions of jets from a small sample of nine blazars. This sample includes sources that have exhibited: (i) positive CP; (ii) negative CP; or (iii) positive and negative CP simultaneously in the radio core region. By coupling deep polarimetric observations of a carefully selected sample of blazars with state-of-the-art RMHD and RT calculations, we hope to gain a deeper understanding of the physics of blazar jets.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1995

Plasma properties and magnetic field structure of the solar corona, based on coordinated Max 1991 observations from SERTS, the VLA, and magnetographs

The purposes of this investigation are to determine the plasma properties and magnetic field structure of the solar corona using coordinated observations obtained with NASA/GSFC's Solar EUV rocket Telescope and Spectrograph (SERTS), the Very Large Array (VLA), and magnetographs. The observations were obtained under the auspices of NASA's Max '91 program. The methods of achieving the stated purposes of this investigation are: (1) to use SERTS spectra and spectroheliograms to determine coronal plasma properties such as temperature, density, and emission measure; (2) to use the coronal plasma properties to calculate the intensity of the thermal bremsstrahlung microwave emission from the coronal plasma (the minimum microwave intensity expected from the emitting plasma); (3) to establish which emission mechanism(s) contribute to the observed microwave emission by comparing the calculated thermal bremsstrahlung intensity with the observed microwave intensity; (4) to derive the coronal magnetic field for regions in which gyroemission contributes to the microwave emission by determining the appropriate harmonic of the local electron gyrofrequency; (5) to derive the coronal magnetic field for regions in which thermal bremsstrahlung emission alone is responsible for the observed microwave emission by calculating the magnetic field which yields the observed microwave polarization; (6) to derive three-dimensional models of the coronal plasma and magnetic field which are consistent with all of the EUV spectra and spectroheliograms, as well as with the intensity and polarization maps at all of the microwave observing frequencies; and (7) to compare the coronal magnetic field derived from the coordinated multiwaveband observations with extrapolations from photospheric magnetograms.

Brosius, Jeffrey W.↗
NASA NTRS1996

Plasma Properties and Magnetic Field Structure of the Solar Corona, Based on Coordinated Max 1991 Observations from SERTS, the VLA, and Magnetographs

The purposes of this investigation are to determine the plasma properties and magnetic field structure of the solar corona using coordinated observations obtained with NASA/GSFC's Solar EUV Rocket Telescope and Spectrograph (SERTS), the Very Large Array (VLA), and magnetographs. The observations were obtained under the auspices of NASA's Max '91 program. The methods of achieving the stated purposes are to use SERTS spectra and spectroheliograms to determine coronal plasma properties such as temperature, density, and emission measure. These properties are subsequently used to calculate the intensity of the thermal bremsstrahlung microwave emission from the coronal plasma (the minimum microwave intensity expected from the emitting plasma). This, in turn, can be used to establish which emission mechanism(s) contribute to the observed microwave emission. Because both mechanisms that may contribute to quiescent active region microwave emission (thermal bremsstrahlung and thermal gyroemission) depend upon the coronal magnetic field in known ways, this information can ultimately be used to derive the coronal magnetic field. Ideally, three-dimensional models of the coronal plasma and magnetic field which are consistent with all of the EUV spectra and spectroheliograms, as well as with the intensity and polarization maps at all of the microwave observing frequencies, can be derived. For completeness, the coronal magnetic field derived from the coordinated multiwaveband observations must be compared with extrapolations from photospheric magnetograms.

Brosius, Jeffrey W.↗
NASA NTRS2011

Interplanetary Magnetic Field Guiding Relativistic Particles

The origin and the propagation of relativistic solar particles (0.5 to few Ge V) in the interplanetary medium remains a debated topic. These relativistic particles, detected at the Earth by neutron monitors have been previously accelerated close to the Sun and are guided by the interplanetary magnetic field (IMF) lines, connecting the acceleration site and the Earth. Usually, the nominal Parker spiral is considered for ensuring the magnetic connection to the Earth. However, in most GLEs the IMF is highly disturbed, and the active regions associated to the GLEs are not always located close to the solar footprint of the nominal Parker spiral. A possible explanation is that relativistic particles are propagating in transient magnetic structures, such as Interplanetary Coronal Mass Ejections (ICMEs). In order to check this interpretation, we studied in detail the interplanetary medium where the particles propagate for 10 GLEs of the last solar cycle. Using the magnetic field and the plasma parameter measurements (ACE/MAG and ACE/SWEPAM), we found widely different IMF configurations. In an independent approach we develop and apply an improved method of the velocity dispersion analysis to energetic protons measured by SoHO/ERNE. We determined the effective path length and the solar release time of protons from these data and also combined them with the neutron monitor data. We found that in most of the GLEs, protons propagate in transient magnetic structures. Moreover, the comparison between the interplanetary magnetic structure and the interplanetary length suggest that the timing of particle arrival at Earth is dominantly determined by the type of IMF in which high energetic particles are propagating. Finally we find that these energetic protons are not significantly scattered during their transport to Earth.

Masson, S.↗
DOE OSTI2025

Role of magnetic and structural symmetry breaking in forming the Mott insulating gap in Nb 3 ⁢Cl 8

The α-phase of the gapped insulator Nb 3 Cl 8 has recently emerged as the long-sought critical testing bed for examining the importance of strong interelectronic correlation vs symmetry breaking in understanding insulation of such Mott compounds. Structural symmetry breaking detected by density functional theory (DFT) energy lowering (such as dimer formation, disproportionation, or Jahn-Teller distortions) explains insulation in both d-electron Mott-like systems and in non-d-electron cases without recourse to strong correlation. Yet, in Nb 3 Cl 8 , structural symmetry breaking alone (viz. formation of Nb trimers) fails to explain insulation, leading instead to a partially occupied metallic flat band, in contrast with experimental observations. We examine the role of magnetic symmetry breaking, noting that Nb 3 Cl 8 is an observed paramagnet (not an antiferromagnet), thus potentially carrying also short-range ordered magnetic moments. Describing the latter as a polymorphous distribution of nonzero local moments with total zero net magnetization is demonstrated to lower the DFT total energy, while gapping the system without recourse to strong correlation or long-range magnetic order. This suggests that degeneracy removal by symmetry breaking in mean-field-like approaches—either structural, or magnetic, or both—can reduce or eliminate the need for strong correlation, allowing the use of DFT for such Mott systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Structure and magnetic properties of Ba 9 ⁢V 3 ⁢Te 15 with ferromagnetic spin chains

Here we report a ferromagnetic compound Ba9⁢V3⁢Te15 with quasi-one-dimensional (1D) spin chains. It was synthesized at high-temperature and high-pressure conditions and systematically investigated via structural, transport, magnetic and heat capacity measurements. Ba9⁢V3⁢Te15 mainly consists of trimerized face-sharing V⁢Te6 octahedral chains running along the 𝑐 axis, which are separated by a distance of 10.184⁢(8)⁢Å, thus demonstrating a strong 1D structural character. Ba9⁢V3⁢Te15 is a semiconductor with a band gap ∼128meV and undergoes a ferromagnetic transition with 𝑇C∼3.6K. Far above 𝑇C, the short-range spin orders due to the intrachain spin coupling have developed, which leads to a negative magnetoresistance effect, the deviation of magnetic susceptibility from the Curie-Weiss law and 𝑇1/2 dependence of magnetic heat capacity. Our results reveal that Ba9⁢V3⁢Te15 provides a good opportunity to study the intrinsic properties of a system with quasi-1D ferromagnetic spin chains.

1-dimensional spin chains↗
DOE OSTI2021

Structural and magnetic transitions of CoFeMnNiAl high-entropy alloys caused by composition and annealing

Tailoring magnetic behavior by composition and annealing is an effective way. The phase transition from the face-centered-cubic (FCC) to B2 structure influenced by the Al content on the CoFeMnNiAl x alloys leads to the enhanced magnetization. However, the excessive Al addition in the B2-structured alloys impairs the magnetization. The phase transformation caused by annealing also indicates that the saturation magnetization of the alloy depends on the volume fraction of the B2 phase, and a higher content of the B2 phase is beneficial to the large saturation magnetization. Ab initio calculations are used to explain the magnetic behavior of the present HEAs and the effects of phase structures on magnetic characteristics. The phase stability of the CoFeMnNiAl x alloy is thoroughly studied by both the existing phase-formation empirical criteria and annealing. Here, the existing empirical criteria used to predict the phase formation are not universal. However, combining the ΔH mix -δ relation and the φ value, whether the single disordered solid-solution phase is formed can be preliminarily predicted.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Effects of Co substitution on the structural and magnetic properties of Sr ( Ni 1 - x Co x ) 2 P 2

Although SrNi 2 P 2 adopts the common ThCr 2 Si 2 structure for T ≥ 325 K, being in an uncollapsed tetragonal state rather than a collapsed tetragonal version, it is a special case for the ThCr 2 Si 2 class: on cooling below 325 K it adopts a one-third collapsed orthorhombic phase where one out of every three P rows bonds across the Sr layers. On the other hand, SrCo 2 P 2 only exhibits the uncollapsed ThCr 2 Si 2 structure from room temperature down to 1.8 K. Regardless of their low-temperature structures, neither SrNi 2 P 2 nor SrCo 2 P 2 manifests magnetic transitions down to 50 mK and 2 K, respectively. In this work we report the effects of Co substitution in Sr(Ni 1 - x Co x ) 2 P 2 , which allows for tuning the transition between the one-third collapsed and the uncollapsed structure. We find a rapid decrease of the one-third collapsed structural transition temperature with increasing Co fraction, until reaching full suppression for x ≥ 0.1. Substitution levels in the range 0.11 ≤ x ≤ 0.58 show no signs of any transition down to 1.8 K in the magnetization or resistance measurements in the range 1.8 ≤ T ≤ 300 K. However, different magnetically ordered states emerge for x ≥ 0.65, and disappear for x ≥ 0.99, recovering the known paramagnetic properties of the parent compound SrCo 2 P 2 . Further, these results are summarized in a phase diagram, built upon the characterization by energy dispersive x-ray spectroscopy, x-ray diffraction, temperature-dependent resistance, and field- and temperature-dependent magnetization measurements done on single crystals with different Co fraction. Both the magnetic and structural properties are compared to other systems with ThCr 2 Si 2 structure that exhibit magnetic ordering and collapsed tetragonal transitions. The magnetic ordering and moment formation are well described by Takahashi's spin fluctuation theory of itinerant electron magnetism.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Optical and photoemission investigation of structural and magnetic transitions in the iron-based superconductor Sr 0.67 Na 0.33 Fe 2 As 2

We report the temperature-dependent optical conductivity and angle-resolved photoemission spectroscopy (ARPES) studies of the multiband iron-based superconductor Sr 0.67 Na 0.33 Fe 2 As 2 . Measurements were made in the high-temperature tetragonal paramagnetic phase, below the structural and magnetic transitions at $T_N$ $≃$ 125 K in the orthorhombic spin-density-wave (SDW)-like phase and $T_r$ $≃$42 K in the reentrant tetragonal double-Q magnetic phase where both charge and SDWorder exist, and below the superconducting transition at $T_c$ $≃$ 10 K. The free-carrier component in the optical conductivity is described by two Drude contributions: one strong and broad and the other weak and narrow. The broad Drude component decreases dramatically below TN and Tr , with much of its strength being transferred to a bound excitation in the midinfrared, while the narrow Drude component shows no anomalies at either of the transitions, actually increasing in strength at low temperature while narrowing dramatically. The behavior of an infrared-active mode suggests zone folding below Tr. Below Tc the dramatic decrease in the low-frequency optical conductivity signals the formation of a superconducting energy gap. ARPES reveals holelike bands at the center of the Brillouin zone (BZ), with both electron- and holelike bands at the corners. Below $T_N$, the hole pockets at the center of the BZ decrease in size, consistent with the behavior of the broad Drude component; however, below $T_r$ the electronlike bands shift and split, giving rise to a low-energy excitation in the optical conductivity at $≃$20 meV. The $C_2$ and $C_4$ magnetic states, with resulting spin-density-wave and charge-SDW order, respectively, lead to a significant reconstruction of the Fermi surface that has profound implications for the transport originating from the electron and hole pockets but appears to have relatively little impact on the superconductivity in this material.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS2002

Relation Between Polar Plumes and Fine Structure in the Solar Wind from Ulysses High-Latitude Observations

Ulysses observations showed that pressure balance structures (PBSs) are a common feature in the high-latitude and high-speed solar winds near the solar minimum. On the other hand, coronal plumes are common in polar coronal holes. PBSs are believed to be remnants of coronal plumes and to be related to network activity such as magnetic reconnection in the photosphere from previous studies. This suggests that information on the magnetic structure of PBSs would help to confirm the relation between PBSs and polar plumes We have investigated the magnetic structures of the PBSs by applying a minimum variance analysis to Ulysses/Magnetometer data and by examining the pitch-angle distribution of energetic electrons measured with Ulysses/SWOOPS. We have found that PBSs have relatively more tangential discontinuities rather than rotational from the minimum variance analysis. Further, most PBSs also show bi-directional electron flux or isotropic pitch-angle distribution or the distribution expected in association with current-sheet structures from the analysis of high-energy electron data. In this, we find further evidence that PBSs are generated due by network activity at the base of polar plumes and their magnetic structures are like current sheets or plasmoids.

Yamauchi, Yohei↗
DOE OSTI2023

Sublattice-Dependent Antiferromagnetic Transitions in Rare Earth Nickelates

Perovskite rare earth nickelates exhibit remarkably rich physics in their metal-insulator and antiferromagnetic transitions, and there has been a long-standing debate on whether their magnetic structures are collinear or noncollinear. Through symmetry consideration based on the Landau theory, we discover that the antiferromagnetic transitions on the two nonequivalent Ni sublattices occur separately at different Néel temperatures induced by the O breathing mode. It is manifested by two kinks on the temperature-dependent magnetic susceptibilities with the secondary kink being continuous in the collinear magnetic structure but discontinuous in the noncollinear one. Here, the prediction on the secondary discontinuous kink is corroborated by an existing magnetic susceptibility measurement on bulk single-crystalline nickelates, thus strongly supporting the noncollinear nature of the magnetic structure in bulk nickelates, thereby shedding new light on the long-standing debate.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Electronic, magnetic and structural properties of CoFeVAl and CoFeV 0.5 Mn 0.5 Al

Abstract In this study, we present results of a comprehensive computational and experimental study of CoFeVAl and CoFeV 0.5 Mn 0.5 Al Heusler alloys. It is shown that while CoFeVAl exhibits a fairly large degree of spin polarization, this material is not half-metallic due to the presence of the vanadium spin-down states at the Fermi level. However, replacing 50% of vanadium with manganese results in a nearly half-metallic transition, largely due to the shift of the Fermi level towards occupied states. Moreover, the half-metallicity of CoFeV 0.5 Mn 0.5 Al is rather robust in a wide range of considered mechanical strain and under experimentally observed B2-type atomic disorder, thus making this alloy potentially suitable for practical spintronic applications. Both considered alloys exhibit ferromagnetic alignment at larger lattice constants, aside from a relatively small magnetic moment of vanadium which is anti-aligned with the magnetic moments of Co, Fe and Mn. We have synthesized both CoFeVAl and CoFeV 0.5 Mn 0.5 Al alloys in cubic structure with some structural disorder using arc melting and annealing. The structural and magnetic properties of the synthesized CoFeV 0.5 Mn 0.5 Al alloy are in good agreement with the theoretical calculations but vary slightly from the parent compound.

Physics↗
DOE OSTI2021

Structural and magnetic properties of hard magnetic system Ce(Co 1 -Fe ) 4.4 Cu 0.6 (0 ≤ x ≤ 0.19)

The Ce(Co 1 -Fe ) 4.4 Cu 0.6 (0 ≤ x ≤ 0.19) is a composite, hard magnetic system that is based on the CaCu 5 -type structure (1:5). It shows both, unique magnetic and microstructural features that are essential for permanent magnets, e.g., exceptional squareness of the 2nd. quadrant of the magnetization loops and microstructural features typically needed for pinning. Samples solidified in alumina crucibles are coarse-grained and often clearly faceted and readily align in a magnetic field. X-ray, SEM, and TEM analyses show a 1:5-type single-phase material when quenched from high temperature, which, after heat treatment, transforms into a laminar coherent nanostructure through the formation of a dense array of extended intercalated regions. Furthermore, these extended intercalated regions are comprised of segments of the Ce 2 Ni 7 –type structure (2:7) which segregate into various closely related precipitates forming a nanostructure similar to the SmCo 5 - Sm 2 Co 17 composites seen in Sm-Co permanent magnets. Based on TEM and Lorentz microscopy of well-aligned single grain particles, the magnetic domains’ reversal mechanism is regulated by anisotropy fluctuations occurring along the easy direction of magnetization and strong exchange interactions between the matrix and defects (e.g.: stacking faults). Lorentz microscopy suggests the domain wall is not physically pinned by the defect, but rather is offset/deflected when it interacts with the defect. The Lorentz and magnetization data suggest that defects cause a bending of the moment away from the c axis inside the grains.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Quantum-Accurate Multiscale Modeling of Shock Hugoniots, Ramp Compression Paths, Structural and Magnetic Phase Transitions, and Transport Properties in Highly Compressed Metals

Fully characterizing high energy density (HED) phenomena using pulsed power facilities (Z machine) and coherent light sources is possible only with complementary numerical modeling for design, diagnostic development, and data interpretation. The exercise of creating numerical tests, that match experimental conditions, builds critical insight that is crucial for the development of a strong fundamental understanding of the physics behind HED phenomena and for the design of next generation pulsed power facilities. The persistence of electron correlation in HED materials arising from Coulomb interactions and the Pauli exclusion principle is one of the greatest challenges for accurate numerical modeling and has hitherto impeded our ability to model HED phenomena across multiple length and time scales at sufficient accuracy. An exemplar is a ferromagnetic material like iron, while familiar and widely used, we lack a simulation capability to characterize the interplay of structure and magnetic effects that govern material strength, kinetics of phase transitions and other transport properties. Herein we construct and demonstrate the Molecular-Spin Dynamics (MSD) simulation capability for iron from ambient to earth core conditions, all software advances are open source and presently available for broad usage. These methods are multi-scale in nature, direct comparisons between high fidelity density functional theory (DFT) and linear-scaling MSD simulations is done throughout this work, with advancements made to MSD allowing for electronic structure changes being reflected in classical dynamics. Main takeaways for the project include insight into the role of magnetic spins on mechanical properties and thermal conductivity, development of accurate interatomic potentials paired with spin Hamiltonians, and characterization of the high pressure melt boundary that is of critical importance to planetary modeling efforts.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

High-order harmonics and the reverse of the squaring up process in the triangular-lattice magnet HoPdAl 4 ⁢Ge 2

We uncover high-order harmonics and the reverse of the squaring-up process, in terms of analyzing the evolution of magnetic orders in a centrosymmetric layered triangular-lattice magnet HoPdAl 4 ⁢Ge 2 , based on a detailed study of the crystal structure, magnetic susceptibility, magnetization, heat capacity, and magnetic structure. Temperature dependencies of magnetic susceptibility and heat capacity show two magnetic transitions at T N = 10.5 K and T t = 5.5 K. Below T N , Ho 3+ spins order antiferromagnetically as a transverse spin-density wave with the propagation vector k 1 = (001.5 – δ) with δ ≈ 0.18. Upon further cooling through T t , the high-order harmonics with k n = (001.5 – nδ), n = 3, 5, 7 develop, suggesting a squaring-up process. It is surprising that the squaring-up process does not continue down to 0 K but reverses the trend below 3 K. Magnetic-field-induced metastable transitions were observed in M⁡(H) curves with the fields applied both parallel and perpendicular to the triangular-lattice plane. Neutron-diffraction results suggest that the magnetization process in HoPdAl 4 ⁢Ge 2 involves the conversion of k n = (001.5 – n⁢δ) with n = 1, 3, 5, 7, to a ferromagnetic k F = (000) component. It is worth noting that the already weak seventh harmonic magnetic peak is enhanced by applying a small magnetic field in the ab plane at 1.5 K or warming up to 3 K, accompanied by a slight decrease of δ.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Crystal structure and magnetism of actinide oxides: a review

In actinide systems, the 5f electrons experience a uniquely delicate balance of effects and interactions having similar energy scales, which are often difficult to properly disentangle. This interplay of factors such as the dual nature of 5f-states, strong electronic correlations, and strong spin–orbit coupling results in electronically unusual and intriguing behavior such as multi-k antiferromagnetic ordering, multipolar ordering, Mott-physics, mixed valence configurations, and more. Despite the inherent allure of their exotic properties, the exploratory science of even the more basic, binary systems like the actinide oxides has been limited due to their toxicity, radioactivity, and reactivity. In this article, we provide an overview of the available synthesis techniques for selected binary actinide oxides, including the actinide dioxides, sesquioxides, and a selection of higher oxides. For these oxides, here we also review and evaluate the current state of knowledge of their crystal structures and magnetic properties. In many aspects, substantial knowledge gaps exist in the current body of research on actinide oxides related to understanding their electronic ground states. Bridging these gaps is vital for improving not only a fundamental understanding of these systems but also of future nuclear technologies. To this end, we note the experimental techniques and necessary future investigations which may aid in better elucidating the nature of these fascinating systems.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Transition from an incommensurate spin density wave to a commensurate magnetic order in a triangular lattice compound Ho 2 PdAl 6 Ge 4

Rare-earth (RE) intermetallics on a triangular lattice are promising candidates for generating interesting magnetic phases due to the complex interplay between Ruderman-Kittel-Kasuya-Yoshida (RKKY) interaction and geometrical frustration. Here, in this work, we report the exotic magnetic structure of a layered compound Ho 2 PdAl 6 Ge 4 with triangular lanthanide nets. Magnetization and heat capacity measurements in zero magnetic field reveal two magnetic phase transitions at T N1 = 10.8 K and T N2 = 6.0 K. Neutron powder diffraction demonstrates a commensurate antiferromagnetic phase with k 1 = (0, 0, 1.5) below T N2 . With increasing temperature, another incommensurate vector appears and therefore, the magnetic structure of the intermediate state is identified as an unusual incommensurate spin density wave with two propagation vectors k 1 = (0, 0, 1.5) and k 2 = (0.0492, 0.0492, 1.5). The magnetic moments in the intermediate state rotate continuously and form an unusual S-shaped wave arrangement in the ab plane, sharing similarities with typical cycloid and helix magnetic orders. These results identify Ho 2 PdAl 6 Ge 4 as a candidate for exploring field-induced topological magnetic phases such as skyrmions, opening the way for further investigations on the family of RE 2 PdAl 6 Ge 4 materials.

36 MATERIALS SCIENCE↗