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At least 343 records · Page 19

Optical and Probe Diagnostics Applied to Reacting Flows

We plan to explore three major threads during the fellowship period. The first interrogates the flame synthesis of carbon nanotubes using aerosol catalysts. Laser light scattering will reveal changes in particle size at various heights above the burner. Analysis of the flame gas by mass spectroscopy will reveal the chemical composition of the mixture. Finally, absorption measurements will map the nanotube concentration within the flow. The second thread explores soot oxidation kinetics. Cavity ring-down absorption measurements of the carbonaceous aerosol can provide a measure of the mass concentration with time and, hence, an oxidation rate. Spectroscopic and direct probe measurements will provide the temperature of the system needed for subsequent modeling. The third thread will explore the details of turbulent flame dynamics. Laser induced incandescence will be applied to measurements of soot volume fraction in a 2-d configuration. Analysis of seed tracer particles by planar laser light MIE scattering will reveal the elemental fuel mixture fraction in the flames. Cavity ring-down spectroscopy, a pulsed transient absorption method, will determine the instantaneous mass loading and its fluctuation. Finally, fluorescence measurements will investigate the formation of PAH's in these flames.

Ticich, Thomas M.↗

An X-ray, optical and radio study of PKS 0745-191 - A massive cooling flow

The X-ray source 3A 0745-191 is identified with intracluster gas surrounding the giant galaxy containing the radio source, PKS 0745-191, which lies at z = 0.1. The gas is cooling at the unprecedented rate of 1000 solar mass/yr. Optical line-emitting gas extends more than 10 kpc from the centre of the galaxy and corroborates the high mass-flow rate. The optical spectrum is similar to that of distant 3CR radio galaxies reported by others. It is concluded that formation of a giant galaxy was observed.

Fabian, A. C.↗

Combined visualisation of cavitation and vortical structures in a real-size optical diesel injector

A high-speed flow visualisation set-up comprising of combined diffuse backlight illumination (DBI) and schlieren imaging has been developed to illustrate the highly transient, two-phase flow arising in a real-size optical fuel injector. The different illumination nature of the two techniques, diffuse and parallel light respectively, allows for the capturing of refractive-index gradients due to the presence of both interfaces and density gradients within the orifice. Hence, the onset of cavitation and secondary-flow motion within the sac and injector hole can be concurrently visualised. Experiments were conducted utilising a diesel injector fitted with a single-hole transparent tip (ECN spray D) at injection pressures of 700–900 bar and ambient pressures in the range of 1–20 bar. High-speed DBI images obtained at 100,000 fps revealed that the orifice, due to its tapered layout, is mildly cavitating with relatively constant cavity sheets arising mainly in regions of manufacturing imperfections. Nevertheless, schlieren images obtained at the same frame rate demonstrated that a multitude of vortices with short lifetimes arise at different scales in the sac and nozzle regions during the entire duration of the injection cycle but the vortices do not necessarily result in phase change. The magnitude and exact location of coherent vortical structures have a measurable influence on the dynamics of the spray emerging downstream the injector outlet, leading to distinct differences in the variation of its cone angle depending on the injection and ambient pressures examined.

42 ENGINEERING↗

Correlation of optical phase distortion with turbulent structure in a homogeneous shear flow

The relative importance of small-scale and large-scale turbulent structure to phase distortion in propagation through the homogeneous shear flow is the focus of this study. The importance of large-scale vortical structure and the associated scalar distribution to optical distortion induced by propagation through a turbulent shear flow has been established (Truman and Lee 1989). Phase errors induced in a coherent optical beam by these turbulent fluctuations are computed. This scalar field shows elongated regions of intense fluctuations which have an inclination with respect to the mean flow similar to that of the characteristic hairpin eddies. Long-term plans include an examination of the effects of inhomogeneity through consideration of direct numerical simulations of the channel flow, boundary layer or mixing layer.

Truman, C. Randall↗

Control of liquid crystals combining surface acoustic waves, nematic flows, and microfluidic confinement

The optical properties of liquid crystals serve as the basis for display, diagnostic, and sensing technologies. Such properties are generally controlled by relying on electric fields. In this work, we investigate the effects of microfluidic flows and acoustic fields on the molecular orientation and the corresponding optical response of nematic liquid crystals. Several previously unknown structures are identified, which are rationalized in terms of a state diagram as a function of the strengths of the flow and the acoustic field. The new structures are interpreted by relying on calculations with a free energy functional expressed in terms of the tensorial order parameter, using continuum theory simulations in the Landau-de Gennes framework. Taken together, the findings presented here offer promise for the development of new systems based on combinations of sound, flow, and confinement.

74 ATOMIC AND MOLECULAR PHYSICS↗

Observations of liquid jets injected into a highly accelerated supersonic boundary layer

Experiments were conducted to observe the cross-sectional structure and streamwise growth of round transverse liquid jets injected into a highly accelerated boundary layer in supersonic flow. The accompanying shock structure was also visualized. In one case, a round jet of acetone was injected into a fully turbulent Mach 2.5 boundary layer that was subsequently accelerated and partially laminarized through a sharp Prandtl-Meyer expansion corner. In the second case, a jet was injected into the laminarized Mach 3.2 boundary layer downstream of the expansion corner at the same jet-to-freestream momentum ratio. The jet and shock structure in both cases were visualized using schlieren optics. Wall-flow patterns were visualized using paints. It was found that the lateral spreading of jets injected downstream of the expansion fan was augmented close to the wall and had a cross-sectional structure significantly different from that of the jet injected upstream: the upstream jet spreads rapidly at the expansion corner in both the lateral and vertical directions.

Johnson, Arthur W.↗

Continuous Counter‐Current Microfluidic Liquid–Liquid Extraction Achieved Using a Pair of Wettable Screen Meshes

Continuous counter‐current microfluidic liquid–liquid extraction performs separations by flowing immiscible liquids in opposing directions within a single flow channel. In principle, this flow arrangement enables a large number of theoretical separation units in a small footprint, without using interstage valving, pumping, and phase separation. Despite its potential for excellent separation performance, this microfluidic scheme rarely appears in literature due to the requirement for capillary forces to be greater than hydrodynamic forces for stable flow. We present a novel microfluidic device and flow approaches that overcome this force‐balance challenge, enabling stable, long‐duration continuous counter‐current flow. Additionally, we cover a suite of methodologies for quantifying the performance of the microfluidic device, revealing the number of theoretical equilibrium stages achieved. The enabling technologies include a woven mesh screen‐based microfluidic device architecture that is easily fabricated outside of a clean room, surface functionalization strategies to promote conjugate (organic/aqueous) wettability, flow approaches to eliminate bubbles and carryover, and computer‐aided flow automation with optical measurement of extraction performance. The reported experiments lasted for over 36 h, terminated only at experiment conclusion, where the device still exhibited good performance. Automated Raman spectroscopy was used for solute quantitation of the ternary system tert‐butanol in a toluene/water matrix, a ternary system that was specifically chosen to analyze the device's performance with a small solute partition ratio and to enable in‐line Raman measurements of solute concentrations in both phases. The microfluidic device possessed a 55 mm contact length and a 38.5 µL internal volume. During counter‐current flow, we observed approximately 37 equilibrium stages (37 ± 13) based on a best‐fit of the solute fraction remaining in the aqueous phase using a Kremser Group Method analysis.

36 MATERIALS SCIENCE↗

Integrated positron emission particle tracking (PEPT) and X-ray computed tomography (CT) imaging of flow phenomena in twisted tape swirl flow

Abstract A combined positron emission particle tracking (PEPT) and X-ray computed tomography (CT) technique is presented, and its utility is demonstrated through investigation of flow in a pipe with twisted tape swirl insert with varying flow conditions (diameter-based Reynolds numbers 16,300–63,300). A description of this technique is given, as well as data handling practices used to relate geometric information captured by CT to fluid flow data gathered via PEPT. It is found that the CT component is readily capable of capturing the stainless steel insert geometry in this present system, but the use of combined plastic and metal materials leads to artifacts in imaging of the plastic surface. Nonetheless, CT data are related to PEPT flow measurements, and average velocity fields are calculated via a pseudo-framing and interpolation scheme and used to visualize and interrogate key flow phenomena within the system. Radial velocity profiles of the mean flow characteristics are seen to collapse to a nearly common form across all flow conditions considered. Helical vortices are seen propagating through the flow field, generated by bypass flow around the gap between the insert and pipe wall, with additional coherent secondary flow structures seen in the higher Reynolds number cases. These findings enhance the understanding of the mixing mechanisms in these swirl flows and encourage the continued development of PEPT-CT methodologies for 3D flow measurements in optically inaccessible systems.

42 ENGINEERING↗

Cascade Dielectrophoretic Separation for Selective Enrichment of Polyhydroxybutyrate (PHB)-Producing Cyanobacterium Synechocystis sp. PCC 6803

Maintaining favorable biological productivities in photosynthetic biomanufacturing systems, especially when the risk of contamination with competing microbes is high, remains a challenge to achieve while maintaining economic feasibility. This study presents a dielectrophoresis (DEP)-based microfluidic approach for isolating a desired strain within a co-culture. The cyanobacterium Synechocystis sp. PCC 6803 (a strain capable of producing the bioplastic precursor polyhydroxybutyrate, or PHB) was enriched from mixed cultures containing the competing cyanobacterium Synechococcus elongatus PCC 7942 (which does not naturally produce PHB). A DEP cascade electrode system was established to increase purification efficiency through sequential enrichment, which leveraged inherent differences in cell morphology and dielectric properties, to achieve the selective separation of these strains under physiological conditions. A substantial increase in the relative abundance of PHB-producing cells was assessed by optical microscopy and flow cytometry characterization, confirming more than five-fold reduction of the Synechococcus fraction in the refined cell mix. The presented electrokinetic platform offers a scalable and effective approach for selectively enhancing desired microbial components within microbial biomanufacturing systems, leading towards improved product yields.

60 APPLIED LIFE SCIENCES↗

Laboratory studies of lean combustion

The fundamental processes controlling lean combustion were observed for better understanding, with particular emphasis on the formation and measurement of gas-phase pollutants, the stability of the combustion process (blowout limits), methods of improving stability, and the application of probe and optical diagnostics for flow field characterization, temperature mapping, and composition measurements. The following areas of investigation are described in detail: (1) axisymmetric, opposed-reacting-jet-stabilized combustor studies; (2) stabilization through heat recirculation; (3) two dimensional combustor studies; and (4) spectroscopic methods. A departure from conventional combustor design to a premixed/prevaporized, lean combustion configuration is attractive for the control of oxides of nitrogen and smoke emissions, the promotion of uniform turbine inlet temperatures, and, possibly, the reduction of carbon monoxide and hydrocarbons at idle.

Sawyer, R. F.↗

Optical measurement methods in thermogasdynamics

A review is presented of a number of optical methods of flow measurements. Consideration is given to such spectroscopic methods as emission and absorption techniques, electron beam-stimulated fluorescence, and light scattering - Rayleigh, Raman and Mie - methods. The following visualization methods are also discussed: shadow photography, schlieren photography, interferometry, holographic interferometry, laser anemometry, particle holography, and electron-excitation imaging. A large bibliography is presented and the work is copiously illustrated with figures and photographs.

Stursberg, K.↗

Spectral line shapes in spherically symmetric radially moving clouds

We present a method for the analysis of spectral line shapes arising in homogeneous, moving gas clouds in which velocity and molecular line excitation have power-law dependences on radial distance from the center. Analytical expressions are obtained for radial flows, for both optically thick and optically thin lines. The additional case of an optically thick line from a differentially rotating cloud is considered qualitatively. The method is applied to the interpretation of the C(12)O line observed in the direction of the Kleinmann-Low infrared nebula in Orion. While gravitational collapse and accelerated outflows would produce lines qualitatively similar to the observed profile, it does not appear to be possible to fit either model to the observations in detail.

Kuiper, T. B. H.↗

Laser anemometer optimization

The design, construction, and testing of laser anemometer configurations for hot section velocity measurements is discussed. The optimization of the laser anemometer systems include the data processing algorithms used. Some relevant hot section properties considered are high temperature with a large background radiation, difficulty of optical access, large flow velocity variations, the presence of solid surfaces that generate reflections and low seed particle density.

Edwards, R. V.↗

Observations of the 63 micron forbidden O I line in Herbig-Haro objects

The paper presents observations of the 63 micron forbidden O I line from Herbig-Haro objects and their exciting stars. Forbidden O I 63 micron emission is detected toward the HH-exciting stars T Tau, DG Tau, L1551 IRS 5, and toward the HH objects HH 7-11, HH 42A, and HH 43 which are displaced from their exciting stars. The forbidden O I emission is associated with these flows on the basis of its spatial coincidence and its negative radial velocities. If the exciting stars drive bipolar flows in which the 63 micron emission follows that at 6300 A, the absence of redshifted 63 micron lines from the three exciting stars might indicate that the disks hypothesized to overlie the receding lobes of these flows are still optically thick in the far-infrared.

Cohen, Martin↗

The use of holographic interferometry for measurements of temperature in a rectangular heat pipe

Holographic interferometry is a nonintrusive method and as such possesses considerable advantages such as not disturbing the velocity and temperature field by creating obstacles which would alter the flow field. These optical methods have disadvantages as well. Holography, as one of the interferometry methods, retains the accuracy of older methods, and at the same time eliminates the system error of participating components. The holographic interferometry consists of comparing the objective beam with the reference beam and observing the difference in lengths of optical paths, which can be observed during the propagation of the light through a medium with locally varying refractive index. Thus, change in refractive index can be observed as a family of nonintersecting surfaces in space (wave fronts). The object of the investigation was a rectangular heat pipe. The goal was to measure temperatures in the heat pipe, which yields data for computer code or model assessment. The results were obtained by calculating the temperatures by means of finite fringes.

Marn, Jure↗

The Cosmic Battery Revisited

We reinvestigate the generation and accumulation of magnetic flux in optically thin accretion flows around active gravitating objects. The source of the magnetic field is the azimuthal electric current associated with the Poynting-Robertson drag on the electrons of the accreting plasma. This current generates magnetic field loops which open up because of the differential rotation of the flow. We show through simple numerical simulations that what regulates the generation and accumulation of magnetic flux near the center is the value of the plasma conductivity. Although the conductivity is usually considered to be effectively infinite for the fully ionized plasmas expected near the inner edge of accretion disks, the turbulence of those plasmas may actually render them much less conducting due to the presence of anomalous resistivity. We have discovered that if the resistivity is sufficiently high throughout the turbulent disk while it is suppressed interior to its inner edge, an interesting steady-state process is established: accretion carries and accumulates magnetic flux of one polarity inside the inner edge of the disk, whereas magnetic diffusion releases magnetic flux of the opposite polarity to large distances. In this scenario, magnetic flux of one polarity grows and accumulates at a steady rate in the region inside the inner edge and up to the point of equipartition when it becomes dynamically important. We argue that this inward growth and outward expulsion of oppositely-directed magnetic fields that we propose may account for the approx. 30 min cyclic variability observed in the galactic microquasar GRS1915+105.

Contopoulos, Ioannis↗

Influence of Reduced Mass Flow Rate and Chamber Backpressure on Swirl Injector Fluid Mechanics

Industry interest in variable-thrust liquid rocket engines places a demand on engine injector technology to operate over a wide range of liquid mass flow rates and chamber backpressures. One injection technology of current interest for variable thrust applications is an injector design with swirled fluids. Current swirl injector design methodologies do not take into account how swirl injector design parameters respond to elevated chamber backpressures at less than design mass flow rates. The current work was created to improve state-of-the-art swirl injector design methods in this area. The specific objective was to study the effects of elevated chamber backpressure and off-design mass flow rates on swirl injector fluid mechanics. Using a backpressure chamber with optical access, water was flowed through a swirl injector at various combinations of chamber backpressure and mass flow rates. The film thickness profile down the swirl injector nozzle section was measured through a transparent nozzle section of the injector. High speed video showed measurable increases in the film thickness profile with application of chamber backpressure and mass flow rates less than design. At prescribed combinations of chamber backpressure and injected mass flow rate, a discrete change in the film thickness profile was observed. Measured injector discharge coefficient values showed different trends with increasing chamber backpressure at low mass flow rates as opposed to near-design mass flow rates. Downstream spray angles showed classic changes in morphology as the mass flow rate was decreased below the design value. Increasing chamber backpressure decreased the spray angle at any injection mass flow rate. Experimental measurements and discussion of these results are reported in this paper.

Kenny, R Jeremy↗