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At least 343 records · Page 19

Investigation of the fine structure of antihydrogen

At the historic Shelter Island Conference on the Foundations of Quantum Mechanics in 1947, Willis Lamb reported an unexpected feature in the fine structure of atomic hydrogen: a separation of the 2S 1/2 and 2P 1/2 states. The observation of this separation, now known as the Lamb shift, marked an important event in the evolution of modern physics, inspiring others to develop the theory of quantum electrodynamics. Quantum electrodynamics also describes antimatter, but it has only recently become possible to synthesize and trap atomic antimatter to probe its structure. Mirroring the historical development of quantum atomic physics in the twentieth century, modern measurements on anti-atoms represent a unique approach for testing quantum electrodynamics and the foundational symmetries of the standard model. Here we report measurements of the fine structure in the n = 2 states of antihydrogen, the antimatter counterpart of the hydrogen atom. Using optical excitation of the 1S–2P Lyman-α transitions in antihydrogen, we determine their frequencies in a magnetic field of 1 tesla to a precision of 16 parts per billion. Assuming the standard Zeeman and hyperfine interactions, we infer the zero-field fine-structure splitting (2P 1/2 –2P 3/2 ) in antihydrogen. The resulting value is consistent with the predictions of quantum electrodynamics to a precision of 2 per cent. Using our previously measured value of the 1S–2S transition frequency, we find that the classic Lamb shift in antihydrogen (2S 1/2 –2P 1/2 splitting at zero field) is consistent with theory at a level of 11 per cent. Our observations represent an important step towards precision measurements of the fine structure and the Lamb shift in the antihydrogen spectrum as tests of the charge–parity–time symmetry8 and towards the determination of other fundamental quantities, such as the antiproton charge radius, in this antimatter system.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Spin–orbit interaction mediated molecular dissociation

The effect of the spin–orbit interaction to photofragmentation is investigated in the mercury(II) bromide (HgBr{sub 2}) molecule. Changes in the fragmentation between the two spin–orbit components of Hg 5d photoionization, as well as within the molecular-field-splitted levels of these components are observed. Dissociation subsequent to photoionization is studied with synchrotron radiation and photoelectron-photoion coincidence spectroscopy. The experimental results are accompanied by relativistic ab initio analysis of the photoelectron spectrum.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Infrared spectral studies of pre- and post-irradiated Li{sub 0.5(1+x)}Ti{sub x}Al{sub 0.1}Fe{sub 2.4-1.5x}O{sub 4} system

The consequences of 50 MeV Li{sup 3+} ions irradiation on the structural behaviour of polycrystalline samples of spinel ferrite system Li{sub 0.5(1+x)}Ti{sub x}Al{sub 0.1}Fe{sub 2.4-1.5x}O{sub 4} are investigated by using infrared absorption spectroscopy. The IR spectrum showed two main absorption bands ν{sub 1} and ν{sub 2} in the range 400-700 cm{sup −1} arising from tetrahedral and octahedral interstitial sites in the spinel lattice. The shifting and splitting observed in IR frequency bands ν{sub 1} and ν{sub 2} for tetrahedral and octahedral sites under irradiation effect are ascribed to redistribution of cations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Reentrant Correlated Insulators in Twisted Bilayer Graphene at 25 T ( 2 π Flux)

Twisted bilayer graphene (TBG) is remarkable for its topological flat bands, which drive strongly interacting physics at integer fillings, and its simple theoretical description facilitated by the Bistritzer-MacDonald Hamiltonian, a continuum model coupling two Dirac fermions. Because of the large moiré unit cell, TBG offers the unprecedented opportunity to observe reentrant Hofstadter phases in laboratory-strength magnetic fields near 25 T. This Letter is devoted to magic angle TBG at 2π flux where the magnetic translation group commutes. Here we use a newly developed gauge-invariant formalism to determine the exact single-particle band structure and topology. We find that the characteristic TBG flat bands reemerge at 2π flux, but, due to the magnetic field breaking C 2z T, they split and acquire Chern number ±1. We show that reentrant correlated insulating states appear at 2π flux driven by the Coulomb interaction at integer fillings, and we predict the characteristic Landau fans from their excitation spectrum.

36 MATERIALS SCIENCE↗

L = 1 rotational splitting detected from a 69 day run using the magneto-optical filter installed at JPL

The preliminary analysis of a 69 day observation run taken at the JPL using the magneto-optical filter is presented. The aim is to estimate the rotational splitting of l = 1 modes. A value of Delta nu = 0.44 +/- 0.09 micro-Hz is found. In a second, more accurate analysis, it is planned to investigate the low frequency part of the power spectrum. The observational statistics are presented.

Cacciani, A.↗

Micromagnetic simulations of spin-wave normal modes and the spin-transfer-torque driven magnetization dynamics of a ferromagnetic cross

We studied spin-transfer-torque (STT) switching of a cross-shaped magnetic tunnel junction in a recent report [Roy et al., J. Appl. Phys. 113, 223904 (2013)]. In that structure, the free layer is designed to have four stable energy states using the shape anisotropy of a cross. STT switching showed different regions with increasing current density. Here, we employ the micromagnetic spectral mapping technique in an attempt to understand how the asymmetry of cross dimensions and spin polarization direction of the injected current affect the magnetization dynamics. We compute spatially averaged frequency-domain spectrum of the time-domain magnetization dynamics in the presence of the current-induced STT term. At low currents, the asymmetry of polarization direction and that of the arms are observed to cause a splitting of the excited frequency modes. Higher harmonics are also observed, presumably due to spin-wave wells caused by the regions of spatially non-uniform effective magnetic field. The results could be used towards designing a multi-bit-per-cell STT-based random access memory with an improved storage density.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A SEYFERT-2-LIKE SPECTRUM IN THE HIGH-MASS X-RAY BINARY MICROQUASAR V4641 SGR

We present an analysis of three archival Chandra observations of the black hole V4641 Sgr, performed during a decline into quiescence. The last two observations in the sequence can be modeled with a simple power law. The first spectrum, however, is remarkably similar to spectra observed in Seyfert-2 active galactic nuclei, which arise through a combination of obscuration and reflection from distant material. This spectrum of V4641 Sgr can be fit extremely well with a model including partial-covering absorption and distant reflection. This model recovers a Γ ≅ 2.0 power-law incident spectrum, typical of black holes at low Eddington fractions. The implied geometry is plausible in a high-mass X-ray binary like V4641 Sgr, and may be as compelling as explanations invoking Doppler-split line pairs in a jet, and/or unusual Comptonization. We discuss potential implications and means of testing these models.

79 ASTRONOMY AND ASTROPHYSICS↗

The 12 micron band of ethane: A spectral catalog from 765 cm(-1) to 900 cm(-1)

The high resolution laboratory absorption spectrum of the 12 micro band of ethane gas is studied. The data were obtained using the McMath Solar Telescope 1 meter Fourier Transform interferometer at Kitt Peak National Observatory and tunable diode laser spectrometers at the University of Tennessee and NASA/Goddard Space Flight Center. Over 200 individual vibration rotation transitions were analyzed taking into account many higher order effects including torsional splitting. Line positions were reproduced to better than 0.001/cm. Both ground and upper state molecular constants were determined in the analysis. The experimental details, the analysis procedures and the results are addressed. A list of ethane transitions occurring near (14)CO2 laser lines needed for heterodyne searches for C2H6 in extraterrestrial sources is also included. A spectral catalog of the ethane nu sub g fundamental from 765/cm to 900/cm is provided. A high dispersion (1/cm 12 in.) plot of both the Kitt Peak interferometric data and a simulated spectrum with Doppler limited resolution, a table of over 8500 calculated transitions listed quantum number assignments, frequencies and intensities are provided.

Atakan, A. K.↗

Magnetic field-, strain-, and disorder-induced responses in an energy spectrum of graphene

We study numerically a role of the uniaxial tensile strains and disordered defects in their impact on electronic density of states (DOS) in graphene exposed to an external magnetic field. The DOS curves are calculated using the tight-binding Hamiltonian, where the perpendicular magnetic field and uniaxial tension are included via the relevant modifications of the hopping parameters. Observed non-equidistant Landau levels (LLs) in the energy spectrum of a defectless graphene undergo the displacement towards the non-shiftable zero-energy Landau level (LL), thus they get contraction as the uniaxial tension is applied independently on the stretching direction. The presence of both point and extended defects reduces LLs peaks, broadens, smears, and can even suppress the LLs depending on a degree of disorders, their strength, and largely effective ranges. Splitting of the zero-energy LL is observable in case of a short-range disorder. Alteration of the localized electronic states in graphene is sensitive to the axis of strain: the uniaxial tensile strains along armchair- and zigzag-edge directions can result to competing phenomena associated with enhancement and reduction of the DOS, respectively. Mutual action of the perpendicular magnetic field and uniaxial stress along the zigzag-edge direction in graphene contributes to the band gap observed in its energy spectrum: the gap becomes more pronounced and even wider as compared with that emerges in case of a zigzag strain effect only, i.e. beyond magnetic field effect.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Lepton number violation as a key to low-scale leptogenesis

We explore the possibility of having a successful leptogenesis through oscillations between new sterile fermion states added to the Standard Model field content in a well motivated framework, naturally giving rise to the required mass splitting between the sterile states through a small total lepton number violation. We propose a framework with only two sterile states forming a pseudo-Dirac state, in which their mass difference as well as the smallness of the neutrino masses are due to two sources of lepton number violation with ΔL=2, corresponding to an Inverse Seesaw framework extended by a Linear Seesaw mass term. We also explore the pure Inverse Seesaw mechanism in its minimal version, requiring at least four new sterile states in order to comply with neutrino data. Our analytical and numerical studies reveal that one can have a successful leptogenesis at the temperature of the electroweak scale through oscillations between the two sterile states with a “natural” origin of the strong degeneracy in their mass spectrum. We also revisit the analytical expression of the baryon asymmetry of the Universe in the weak washout regime of this framework.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Energy flow along the medium-induced parton cascade

We discuss the dynamics of parton cascades that develop in dense QCD matter, and contrast their properties with those of similar cascades of gluon radiation in vacuum. We argue that such cascades belong to two distinct classes that are characterized respectively by an increasing or a constant (or decreasing) branching rate along the cascade. In the former class, of which the BDMPS, medium-induced, cascade constitutes a typical example, it takes a finite time to transport a finite amount of energy to very soft quanta, while this time is essentially infinite in the latter case, to which the DGLAP cascade belongs. The medium induced cascade is accompanied by a constant flow of energy towards arbitrary soft modes, leading eventually to the accumulation of the initial energy of the leading particle at zero energy. It also exhibits scaling properties akin to wave turbulence. These properties do not show up in the cascade that develops in vacuum. There, the energy accumulates in the spectrum at smaller and smaller energy as the cascade develops, but the energy never flows all the way down to zero energy. Our analysis suggests that the way the energy is shared among the offsprings of a splitting gluon has little impact on the qualitative properties of the cascades, provided the kernel that governs the splittings is not too singular.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Ultra-fast computation of electronic spectra for large systems by tight-binding based simplified Tamm-Dancoff approximation (sTDA-xTB)

The computational bottleneck of the extremely fast simplified Tamm-Dancoff approximated (sTDA) time-dependent density functional theory procedure [S. Grimme, J. Chem. Phys. 138, 244104 (2013)] for the computation of electronic spectra for large systems is the determination of the ground state Kohn-Sham orbitals and eigenvalues. This limits such treatments to single structures with a few hundred atoms and hence, e.g., sampling along molecular dynamics trajectories for flexible systems or the calculation of chromophore aggregates is often not possible. The aim of this work is to solve this problem by a specifically designed semi-empirical tight binding (TB) procedure similar to the well established self-consistent-charge density functional TB scheme. The new special purpose method provides orbitals and orbital energies of hybrid density functional character for a subsequent and basically unmodified sTDA procedure. Compared to many previous semi-empirical excited state methods, an advantage of the ansatz is that a general eigenvalue problem in a non-orthogonal, extended atomic orbital basis is solved and therefore correct occupied/virtual orbital energy splittings as well as Rydberg levels are obtained. A key idea for the success of the new model is that the determination of atomic charges (describing an effective electron-electron interaction) and the one-particle spectrum is decoupled and treated by two differently parametrized Hamiltonians/basis sets. The three-diagonalization-step composite procedure can routinely compute broad range electronic spectra (0-8 eV) within minutes of computation time for systems composed of 500-1000 atoms with an accuracy typical of standard time-dependent density functional theory (0.3-0.5 eV average error). An easily extendable parametrization based on coupled-cluster and density functional computed reference data for the elements H–Zn including transition metals is described. The accuracy of the method termed sTDA-xTB is first benchmarked for vertical excitation energies of open- and closed-shell systems in comparison to other semi-empirical methods and applied to exemplary problems in electronic spectroscopy. As side products of the development, a robust and efficient valence electron TB method for the accurate determination of atomic charges as well as a more accurate calculation scheme of dipole rotatory strengths within the Tamm-Dancoff approximation is proposed.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

On-Chip Cavity Electroacoustics Using Lithium Niobate Phononic Crystal Resonators

Mechanical systems are pivotal in quantum technologies because of their long coherent time and versatile coupling to qubit systems. So far, the coherent and dynamic control of gigahertz-frequency mechanical modes mostly relies on optomechanical coupling and piezoelectric coupling to superconducting qubits. Here, we demonstrate on-chip cavity electroacoustic dynamics using our microwave-frequency electrically modulated phononic crystal resonators on lithium niobate. Leveraging the high dispersion of phononic crystal, our acoustic modes space unevenly in the frequency spectrum, emulating atomic energy levels. Atomiclike transitions between different acoustic modes are selectively achieved by applying electrical fields to modulate acoustic modes via the nonlinear piezoelectricity of lithium niobate. Among two modes, we demonstrate Autler-Townes splitting, ac Stark shift, and Rabi oscillation with a maximum cooperativity of 4.18. Extending to three modes, we achieve nonreciprocal frequency conversions with an isolation up to 20 dB. Nonreciprocity can be tuned by the time delay between the two modulating pulses. Finally, our cavity electroacoustic platform could find broad applications in sensing, microwave signal processing, acoustic computing, and quantum acoustics.

Rabi model↗

Measurement of Muon Neutrino Disappearance with the NOvA Experiment

The NOvA experiment consists of two functionally identical tracking calorimeter detectors which measure the neutrino energy and flavour composition of the NuMI beam at baselines of 1~km and 810~km. Measurements of neutrino oscillation parameters are extracted by comparing the neutrino energy spectrum in the far detector with predictions of the oscillated neutrino energy spectra that are made using information extracted from the near detector. Observation of muon neutrino disappearance allows NOvA to make measurements of the mass squared splitting $\Delta m^2_{32}$ and the mixing angle $\theta_{23}$. The measurement of $\theta_{23}$ will provide insight into the make-up of the third mass eigenstate and probe the muon-tau symmetry hypothesis that requires $\theta_{23} = \pi/4$. This thesis introduces three methods to improve the sensitivity of NOvA's muon neutrino disappearance analysis. First, neutrino events are separated according to an estimate of their energy resolution to distinguish well resolved events from events that are not so well resolved. Second, an optimised neutrino energy binning is implemented that uses finer binning in the region of maximum muon neutrino disappearance. Third, a hybrid selection is introduced that selects muon neutrino events with greater efficiency and purity. The combination of these improvements produces an increase in the sensitivity of the analysis equivalent to collecting 40-100\% more data across the range of possible values of $\Delta m^2_{32}$ and $\sin^2\theta_{23}$. This thesis presents new results using a 14~ktonne detector equivalent exposure of $6.05\times 10^{20}$~protons~on~target. A fit to the far detector data, assuming normal hierarchy, produces $\Delta m^2_{32}=2.45^{+0.087}_{-0.079}\times10^{-3}~\text{eV}^2$ and $\sin^2\theta_{23}$ in the range 0.429~-~0.593 with two statistically degenerate best fit points at 0.481 and 0.547. This measurement is consistent with maximal mixing where $\theta_{ 23} = \pi/4$. The data used for this thesis is 1/6 of the to! tal data that NOvA expects to collect.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

L-shell Auger and Coster-Kronig spectra from relativistic theory

The intensities of L-shell Auger and Coster-Kronig transitions in heavy atoms have been calculated relativistically. A detailed comparison is made with measured Auger spectra of Pt and U. The pertinent transition energies were computed from relativistic wave functions with inclusion of the Breit interaction, self-energy, a vacuum-polarization correction, and complete atomic relaxation. Multiplet splitting is found to distribute Auger electrons from certain transitions among several lines. The analysis leads to reassignment of a number of lines in the measured spectra. Lines originally identified as L2-L3Ni in the U spectrum are shown to arise from M4,5 Auger transitions instead.

Chen, M. H.↗

Chemical sensing of copper phthalocyanine sol-gel glass through organic vapors

The sensitivities of metallophthalocyanine to vapor phase electron donors has gained significance in many areas and disciplines due to their sensing properties and ease of operation. In the present study the interaction mechanism of organic vapors in Copper Phthalocyanine (CuPc) sol-gel glass has been studied. The interaction mechanism is affected by many factors like morphology, electrical or optical properties of film. CuPc sol-gel glass has been synthesized using chemical route sol-gel method. Its structural characterization was conducted using XRD and the amorphous nature of the silicate glass was observed with characteristic α polymorph phase of CuPc at around 6.64° with 13.30Å interplanar spacing. The size of the particle as determined using Debbye Scherre’s formula comes out around 15.5 nm. The presence of α phase of CuPc was confirmed using FTIR with the appearance of crystal parameter marker band at 787 cm-1. Apart from this A2u and Eu symmetry bands of CuPc have also been observed. The UV absorption spectrum of CuPc exhibits absorption peaks owing to π→ π* and n→ π* transitions. A blue shift in the prepared CuPc glass has been observed as compared to the dopant CuPc salt indicating increase of band gap. A split in B (Soret) band and Q band appears as observed with the help of Lorentzian fitting. CuPc sol gel glass has been exposed with chemical vapors of Methanol, Benzene and Bromine individually and the electrical measurements have been carried out. These measurements show the variation in conductivity and the interaction mechanism has been analyzed.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Spectroscopy of triply charmed baryons from lattice QCD

The spectrum of excitations of triply-charmed baryons is computed using lattice QCD including dynamical light quark fields. The spectrum obtained has baryonic states with well-defined total spin up to 7/2 and the low-lying states closely resemble the expectation from models with an SU(6) x O(3) symmetry. As a result, energy splittings between extracted states, including those due to spin-orbit coupling in the heavy quark limit are computed and compared against data at other quark masses.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

IceCube can constrain the intrinsic charm of the proton [IC at IC: IceCube can constrain the intrinsic charm of the proton]

Here, the discovery of extraterrestrial neutrinos in the ~30 TeV–PeV energy range by IceCube provides new constraints on high energy astrophysics. An important background to the signal are the prompt neutrinos which originate from the decay of charm hadrons produced by high energy cosmic-ray particles interacting in the Earth’s atmosphere. It is conventional to use the calculations of charm hadroproduction using gluon splitting g → c¯c alone. However, QCD predicts an additional “intrinsic" component of the heavy quark distribution which arises from diagrams where heavy quarks are multiply connected to the proton’s valence quarks. We estimate the prompt neutrino spectrum due to intrinsic charm. We find that the atmospheric prompt neutrino flux from intrinsic charm is comparable to those calculated using QCD computations not including intrinsic charm, once we normalize the intrinsic charm differential cross sections to the ISR and the LEBC-MPS collaboration data. In the future, IceCube will constrain the intrinsic charm content of the proton and will contribute to one of the major questions in high energy physics phenomenology.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗