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At least 37 records · Page 2

Multiphase computational fluid dynamics modeling of reacting flows in absorption columns for carbon capture

First-principles derived computational fluid dynamics (CFD) simulations have been proposed as a fundamental tool for investigating solvent-based CO 2 absorption in packed columns due to their ability to accurately represent the underlying nonlinear, multiscale dynamics. Numerous studies have previously utilized such CFD simulations to investigate hydrodynamics of columns with structured and random packings by assessing the key hydrodynamic metrics such as the interfacial and wetted areas. While mapping such metrics for different conditions is essential to the optimization of absorption columns, it is not sufficient, as the CO 2 capture rate depends also on the coupled, nonlinear dynamics from the underlying chemical reaction kinetics, thermodynamics, and heat-transfer rates. In this work, we present detailed CFD simulation results augmented by incorporating the effects of interfacial physical mass transfer of CO 2 , heat release from chemical reaction kinetics, and thermophysical property variations from resulting temperature gradients. We demonstrate the applicability of the proposed approach in numerically assessing the performance of packed columns by evaluating key hydrodynamic quantities, CO 2 absorption rates, and temperature rise in a reference column with packings that are structurally similar to the Sulzer Mellapak™ 250.Y packing, for different solvent inflow velocities and temperatures. Predictions from simulation results are found to be consistent with the trends in experimental observations from the literature, suggesting that the predictive capabilities of the simulation framework can be leveraged to guide the future development of absorber-column designs and optimized process flowsheets.

Absorption columns↗

An Engineering Prototype of a Late Stage Ionization Cooling Cell for a Muon Collider

Achieving the low emittances required for a muon collider requires ionization cooling. Much of that cooling occurs in compact cooling cells where superconducting coils and conventional RF cavities are closely interleaved. The real challenges for these cooling cells reside in their engineering challenges: high field solenoids, RF cavities, and absorbers, often designed near technological limits, placed in close proximity to each other. We thus propose to build a prototype ionization cooling cell to demonstrate the capability of constructing an ionization cooling channel reaching the lowest emittances and to provide engineering input for the design of such beamlines.

43 PARTICLE ACCELERATORS↗

MODELING AND METHOD FOR OPTICAL PERFORMANCE OF A RECEIVER COATING AND ITS DEGRADATION DUE TO OPERATION

The optical properties of the coating used on a concentrated solar power (CSP)’s receiver directly impact the performance of the power plant. Receiver coatings are designed to absorb as much heat as possible and transfer it to the circulating fluid. Over time, the absorptivity of the receiver coating degrades due to environmental and operational conditions. This project aims to (1) create a test apparatus that allows coatings to undergo accelerated lifetime testing under conditions that mimic what the coating will experience on-tower; and (2) develop a mathematical model that based on the test data predicts absorptivity over time. To create the mathematical model, samples of BrightSource Energy’s Gen1 and Gen2 coatings were tested first looking at individual failure modes (such as high temperature cycling) and then for combined failure modes in the newly developed apparatus. In addition to taking optical measurements, the samples were destroyed to allow for metalogical evaluation to understand what was happening on a microscopic level. Pre-existing models from the literature that describe accelerated testing as well as individual phenomena observed in the coating were then combined to create the model. Additionally, the Gen2 and Gen3 coatings are being testing at the Plataforma Solar de Almería (PSA) facility in Almeria, Spain to confirm that the apparatus test results are similar to those received on-sun. (PSA’s facility closely mimics on-tower conditions). The goal is to enable industry players to test coatings using the new apparatus, gather absorptivity measurements (without needing to destroy samples), and input the information into the model to determine how the coating will perform over time, thus allowing the optical performance of coatings to be compared even before they are used on-tower. The model will be publicly available by the end of the project (currently projected as December 2024).

14 SOLAR ENERGY↗

Biconjugate Impedance Matching Control of the HERO WEC: Preprint

Effective control strategies are essential for maximizing the power output of wave energy converters (WECs). In this study, we explore the methodology of port-based modelling which can be used for bi-conjugate impedance matching, a type of reactive control that involves maximizing power transfer by setting the load (PTO) impedance to be the complex conjugate of the source impedance (WEC). Despite its foundational role in electrical engineering, this method has seen limited application in wave energy and has not yet been demonstrated in wave-powered desalination systems. We represent our complex multidisciplinary system as an equivalent circuit to explore frequency-based relations. The HERO WEC, a small-scale, modular point absorber (PA) designed for reverse osmosis desalination is used as a case study to demonstrate port-based modelling for control applications. Improving the performance of wave-powered water desalination systems could play a critical role in addressing freshwater scarcity for coastal communities, especially those in remote or disaster-prone regions.

16 TIDAL AND WAVE POWER↗

Fiber-optic silicon Fabry–Perot interferometric bolometer with improved detection limit for magnetic confinement fusion

Fiber-optic bolometers (FOBs) intended for plasma radiation measurement in magnetically confined fusion have been previously developed using a silicon pillar that functions as both a Fabry–Perot interferometer (FPI) for temperature measurement and an absorber for the radiation. We report an FOB design that can significantly improve the detection sensitivity over earlier designs by engineering the absorber of the FOB. Our design uses the fact that, compared with a silicon pillar, a gold film with the same x-ray absorption thickness will show a much higher temperature rise from a given power density of the radiation. Therefore, the responsivity of an FOB can be improved by attaching a large gold disk to the silicon FPI as the absorber. We have developed a fabrication method for FOBs of such design and obtained an FOB with a 4-µm-thick, 0.6-mm-diameter gold disk attached to a 200-µm-diameter, 100-µm-thick silicon FPI. We have characterized the noise, responsivity, response time, and noise-equivalent power density (NEPD) and compared these with the earlier design where the absorber is mainly the silicon FPI itself. The experimental result suggests that the FOB with the gold disk achieves a responsivity of ∼2.8 mK/(W/m2) and a noise-equivalent-power-density of 0.13 W/m2, which are, respectively, more than nine times larger and six times smaller compared to the FOB using a previous design. Improved NEPD and good absorption over a broad frequency range will make the FOB more attractive for applications in magnetic-confinement fusion devices.

Uddin, Nezam↗

Cooperative Education

Los Alamos National Laboratory (LANL) is a multidisciplinary national laboratory that conducts research and development in national security, engineering, materials science, computational modeling, and advanced manufacturing. The laboratory develops innovative technologies to address complex scientific and engineering challenges. This project focuses on the development and evaluation of high-performance absorbing structures through computational design, simulation, and engineering analysis. Absorbing structures are used in applications where damage mitigation, structural protection, and material efficiency are critical performance requirements. The increasing demand for lightweight, high-strength, and highly efficient structural systems has created a need for improved design methodologies capable of maximizing absorption while minimizing weight and material usage. The project utilizes advanced engineering software, including 3D CAD software and FEA, to generate and optimize structural concepts. Computational simulations are performed to evaluate structural behavior under loading conditions, while mathematical analyses are conducted using Python-based tools as well as established analytical equations from material and structural mechanics. The project benefits LANL by supporting the development of advanced design methodologies and improving the understanding of material and structural performance. During the internship term, a significant portion of the design development, simulation, and data analysis activities will be completed. Success of the project depends on collaboration among engineering mentors and technical staff members. Work will be conducted at Los Alamos National Laboratory using laboratory computing resources and engineering software.

42 ENGINEERING↗

IER-519 CED-2: Final Design for Thermal/Epithermal eXperiments (TEX) with Absorbers to Provide Validation Benchmarks for Hanford Tank Farms

The Hanford tank farms contain 56 million gallons of waste across 177 tanks. The primary criticality safety concern for the waste is the plutonium inventory in waste solids – approximately 670 kg in total. Criticality safety analysis credits the absorption and dilution properties of the large quantities of other elements (aluminum, chromium, iron, manganese, nickel, silicon, sodium, and zirconium) present in the waste. Of these, iron and manganese are by far the most significant neutron absorbers, particularly for the waste compositions of highest criticality safety concern. The criticality safety analyses at the Hanford Waste Treatment and Vitrification Plant (WTP) and the Savannah River tank farms also credit iron and manganese as the primary neutron absorbers to demonstrate subcriticality.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Final Design for Thermal/Epithermal eXperiments (TEX) with Absorbers to Provide Validation Benchmarks for Y-12 Electrorefining Facility

One of the main goals of the Thermal/Epithermal eXperiments (TEX) project is to use existing Nuclear Criticality Safety Program (NCSP) assets to create critical experiment plutonium and uranium test beds for materials important to criticality safety that have insufficient benchmark evaluations. The plutonium test bed experiments were completed in 2018 and are published in the 2020 edition of the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook. The uranium test bed assemblies were measured in 2020, with benchmark preparation underway.

42 ENGINEERING↗

Neutron Absorber Plate Characterization Plan for Criticality Experiments Design [Slides]

The goal of this presentation is to show the feasibility of performing a critical experiment with a B 4 C/Aluminum alloy neutron absorber plate. The motivation of this experiment is to provide integral data on modern neutron absorber product “Boralcan” by Rio Tinto. In 2020, used in about 20% of spent fuel pools in the US, and in casks for storage and transportation in the US and in Europe. The added value of this experiment: Neutron absorber plate modeling method verification: homogeneous or not, a lot of potential savings by relaxing boron loading credit limits. No available critical benchmark involving Boralcan, other boron-related experiments are relatively old. Nuclear data validation for B, C, and Al in the form of B 4 C in Al matrix.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Final Design for Thermal/Epithermal eXperiments (TEX) with Chloride Absorbers to Provide Validation Benchmarks for Y-12 Electrorefining Facility

Uranium electrorefining operations at Y-12 require validation for chlorine absorption and reflection. Plutonium chloride solution operations at Los Alamos National Laboratory require chlorine absorption validation. The growing need for chlorine validation is evident to the wider criticality safety community, with multiple attendees at the recent TEX 2.0 meeting at Lawrence Livermore National Laboratory (May 2023) requesting validation for chlorine (Idaho National Laboratory (INL), Institute de radioprotection et de surete nucleaire (IRSN), Savannah River Nuclear Site (SRNS), LANL, and Y-12). Los Alamos National Laboratory has recently performed, and benchmarked, an experiment titled Chlorine Worth Study (CWS) for the internal operations at the lab, but due to the difficulties in precisely characterizing the material compositions of the chlorine absorbers it is advantageous to perform a complimentary study with a different chlorine-based absorber material. Furthermore, having a uranium-based vs plutonium-based experiment provides a separate and important validation basis for criticality safety and nuclear data evaluation. The original final design report for the study of chlorine absorption using the TEX-HEU experimental base was presented in 2022, but used the same chlorine-bearing materials that were found to be difficult to characterize in the LANL benchmark. A complete redesign of the experiment has been performed looking at alternative absorber materials in various forms to produce an experiment that is fully characterizable. This report presents five novel chlorine experiments using the TEX-HEU test bed which provides direct comparison to the Y-12 and INL/Terrapower application needs, utilizing sodium chloride (NaCl) absorber plates. The absorber plates will consist of granulated NaCl (≥99.5% pure), which will be fully encapsulated in aluminum tins, providing a simple but effective chlorine-based absorber material that can be completely characterized. Of the five configurations presented in this report, it is expected that two or three configurations will be down selected for the actual experiment, with the other configurations being alternates. Three of the configurations are in the standard configuration, where the absorber is placed directly on the HEU fuel plates, and two in the sandwich configuration, where the absorber is surrounded by polyethylene moderators to force additional neutron thermalization prior to reaching the absorber. There are two thicknesses of NaCl absorber plates: 3/16” and 1/4” active thicknesses (i.e. not including the encapsulation). Both variations of the absorbers have an active absorber radius of 6” and a total radius of 7.5” to match the diameter of the HEU plates, with the outer 1.5” being aluminum encapsulation. The high-density polyethylene (HDPE) moderators are of the thicknesses: 27/16”, 7/4”, 1/8”, 11/16”, and 3/4”. The final configurations have six (one sandwich and one standard configuration), eight (one sandwich and one standard configuration), and 18 total fuel layers (standard configuration). The standard and sandwich configurations were designed such that the differences in moderator thicknesses are 1” HDPE, which were already procured for the original CED-2. The proposed configurations were precisely tuned to closely match the sensitivity profiles and neutron spectra of the Y-12 upset cases and were also compared to the INL/Terrapower upset cases. The assessment of experimental uncertainties of the non-absorber components was predicted to be 0.00114 Δk eff . The assessment of uncertainties resulting from the absorbers was predicted to be 0.00029 Δk eff . This results in a total uncertainty of 0.00118 Δk eff . Many of the largest uncertainties, namely the moderator densities, may be reduced with precision dimensional inspection of the components. The 1” HDPE moderators as well as the HDPE reflectors from the original CED-2 were incorporated in the final designs presented here. Additional HDPE moderator plates must be fabricated to complete the configurations. NaCl absorber plates will by fabricated at LLNL. The total additional cost is expected to be $\$$54,250 for the remaining components. Precise inspection, including dimensional, mass, density, and impurity, is recommended for all components. LLNL estimates that these costs are around $\$$12,000. It is expected, based on previous TEX-HEU experiments, that three weeks of experimental facility time is needed to complete the experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Preliminary Design of a New Pulsed-Neutron Die--Away Experiments with Absorbers (IER-552 CED-1)

This report presents the preliminary design (CED-1) of IER-552, pulsed-neutron die-away (PNDA) experiments with absorbers, to be conducted by Lawrence Livermore National Laboratory (LLNL). The goal of the PNDA experiments with absorbing materials is to produce high-quality, low-cost integral benchmarks that can be used to validate cross sections that are high priority nuclear data for the Department of Energy’s Nuclear Criticality Safety Program (NCSP). PNDA experiments can be used to generate nuclear data validation benchmarks quickly and cheaply, as they do not require fissile material or a nuclear facility to conduct them. The original PNDA experiments were set up at LLNL under IER-501. Extending the PNDA experiments to include absorbing materials leverages existing facilities and resources at LLNL to validate cross sections, with a basic experiment design that uses a neutron generator to impinge a short, mono-energetic neutron pulse on a poisoned, moderating target sample. The neutron pulse lasts 100 µs, after which the neutron population in the sample reaches thermal equilibrium and later spatial equilibrium. In this fully equilibrized state, the neutron population has a characteristic decay-time eigenvalue. The eigenvalue can be used as an integral parameter to validate nuclear data involved with neutron scattering and absorption. Two observables can be measured: the neutron population and the population of secondary γ-rays produced by inelastic and capture reactions. This report explores the feasibility of both approaches. For γ-ray measurements, this allows for direct measurement of reactions of interest for validation. During the neutron burst time, inelastic (prompt) γ-rays dominate, and these data can be isolated for validation of neutron inelastic scattering data. After the pulse ends, neutron capture (delayed) γ-rays dominate and are produced by many reaction channels as neutrons slow down to thermal energies. Two sets of γ-ray spectra (inelastic, capture) can be produced for validation. Additionally, the time-dependent decay of the capture γ-ray population when the neutron population is thermalized and in its fundamental mode can be used for validation. Two experiments can be imagined where pulsed neutrons are used to validate the nuclear data of absorbing materials. The first integrates well into the existing PNDA testbed at LLNL. The absorber material would be introduced into a moderating target and the same neutron generator, neutron detectors, electronics, and shielding box used for IER-501 would be employed. From the same experimental setup, many absorbing materials can be validated by simply changing the neutron poison in the moderator. The only significant modification would be the introduction of a γ-ray detector. Such an experiment would primarily serve to validate nuclear data in the thermal energy range. The second kind of experiment would validate the fast and epithermal energy range. It would involve pulsing neutron into a bare assembly of the absorber material and measuring the die-away of neutrons. The fast leakage of such an assembly requires nanosecond neutron-generator pulse widths and fast detectors/electronics that could measure ~200 ns die-away curves. This kind of experiment would ideally be performed at a cyclotron, like that available at Lawrence Berkeley National Laboratory.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

High-power test results for a cylindrical-shell silicon carbide higher-order-mode damper

The next high-current Electron-Ion Collider (EIC) is a new accelerator to be built at Brookhaven National Laboratory in collaboration with Thomas Jefferson National Accelerator Facility. In the EIC Electron Storage Ring (ESR), there will be beam currents of up to 2.5 A, which will excite massive higher-order-mode (HOM) power in the 17 single-cell 591 MHz superconducting radio-frequency (SRF) cavities. Damping the HOM power in the ESR SRF cavities is a challenge. A room temperature cylindrical shell shape silicon carbide (SiC) beamline HOM absorber (BLA) was chosen as the baseline design, due to its broadband and high-power capability, and previous demonstrations at other accelerator facilities, albeit at much lower power. Because the EIC BLA HOM power dissipation is significantly greater than the previous applications, it is imperative to carry out high-power testing to determine the maximum device performance levels achievable for thermal transport, rf breakdown, and mechanical stress, prior to finalizing the design. A SiC HOM absorber with a state-of-the-art geometry size was prototyped to verify the shrink-fit technique, test outgassing rate, and high-power handling capability. This paper presents the HOM damper’s prototyping and test results. Published by the American Physical Society 2024

43 PARTICLE ACCELERATORS↗

High Power Test Results For A Cylindrical-Shell SiC Higher-Order-Mode DAMPER

The next high-current Electron Ion Collider (EIC) is a new accelerator to be built at Brookhaven National Laboratory (BNL) in collaboration with Thomas Jefferson National Accelerator Facility (TJNAF). In the EIC Electron Storage Ring (ESR), there will be beam currents up to 2.5 A, which will excite massive Higher-Order-Modes (HOM) power in the 17 single-cell 591 MHz Superconducting Radio Frequency (SRF) cavities. To damp the HOM power in the ESR SRF cavities is a challenge. A room temperature cylindrical shell shape Silicon Carbide (SiC) Beamline HOM Absorber (BLA) was chosen as the baseline design, due to its broadband and high-power capability, and previous demonstrations at other accelerator facilities, albeit at much lower power. Because the EIC BLA HOM power dissipation is significantly greater than the previous applications, it is imperative to carry out high power testing to determine the maximum device performance levels achievable for thermal transport, RF breakdown, and mechanical stress, prior to finalizing the design. A SiC HOM absorber with state-of-the-art geometry size was prototyped to verify shrink-fit technique, test outgassing rate, and high power handling capability. This paper presents the HOM damper’s prototyping and test results.

43 PARTICLE ACCELERATORS↗

Insights on the Effects of Magnetic Forces on the Efficiency of Vibration Energy Harvesting Absorbers in Controlling Dynamical Systems

This study investigates the effects of magnetic constraints on a piezoelectric energy harvesting absorber while simultaneously controlling a primary structure and harnessing energy. An accurate forcing representation of the magnetic force is investigated and developed. A reduced-order model is derived using the Euler–Lagrange principle, and the impact of the magnetic force is evaluated on the absorber’s static position and coupled natural frequency of the energy harvesting absorber and the coupled primary absorber system. The results show that attractive magnet configurations cannot improve the system substantially before pull-in occurs. A rigorous eigenvalue problem analysis is performed on the absorber’s substrate thickness and tip mass to effectively design an energy harvesting absorber for multiple initial gap sizes for the repulsive configurations. Then, the effects of the forcing amplitude on the primary structure absorber are studied and characterized by determining an effective design of the system for a simultaneous reduction in the primary structure’s motion and improvement in the harvester’s efficiency.

42 ENGINEERING↗

Lattice Design of the Beam Transfer Line (BTL) from PIP-II LINAC to the Booster at Fermilab

PIP-II beam transfer line (BTL) to transport the beam from PIP-II Linac to the Booster ring at Fermilab. The latest design eliminates rolling the dipoles in the beam line to cross over the Tevatron tunnel. Also re-designed is the lattice in the region of the Booster Injection to meet the request of the civil construction needs and accommodate the constrains of the Booster injection request. A beam line to the beam absorber (BAL) is designed based on the request from the results of Mars simulations and ANASYS calculation of the absorber. Simulations with dipole and quadrupole field errors for the Beam Transport Line (BTL) to the Booster, which provides the specifications for all the magnets and Power supplies, will be presented too.

43 PARTICLE ACCELERATORS↗

Estimating the Contribution of the Nickel to Protium Loading of Full-Length Getters

The full-length getter (FLG) is a critical component of the tritium producing burnable absorber rod (TPBAR), designed to capture tritium produced within the lithium aluminate pellets. However, due to the chemical similarity between protium (¹H) and tritium (³H), the FLG readily absorbs protium, reducing its capacity to absorb tritium and increasing the risk of tritium permeation into the reactor coolant. This study evaluates protium produced from neutron irradiation of nickel plating on the FLG through 5?Ni(n,p) reactions, quantifies its contribution to the total protium observed, and informs models of tritium and hydrogen transport within TPBARs. During irradiation, neutron capture by 58Ni results in the formation of 5?Ni, which undergoes neutron bombardment to produce 4He via 5?Ni(n,a) reactions and protium via 5?Ni(n,p) reactions. The measured helium content post-irradiation provides insight into the neutron capture processes within the getter. The 4He measured within the getter may be useful in determining hydrogen produced by the nickel plating on FLG because 59Ni also produces protium in a 59Ni(n, p) reaction. The contribution of 1H from the nickel in FLG contributed less than 1% of the measured H2 gas in PIE, ranging from 0.005% to 0.614%. These findings refine current knowledge of the protium-tritium interplay in TPBARs and support the development of improved transport models for tritium and hydrogen, ultimately aiding in the optimization of TPBAR design and reactor operations.

Arbova, Dana L.↗

Penetration through Slots in Cylindrical Cavities Operating at Fundamental Cavity Modes in the Presence of Electromagnetic Absorbers

Placing microwave absorbing materials into a high-quality factor resonant cavity may in general reduce the large interior electromagnetic fields excited under external illumination. In this study, we aim to combine two analytical models we previously developed: 1) an unmatched formulation for frequencies below the slot resonance to model shielding effectiveness versus frequency; and 2) a perturbation model approach to estimate the quality factor of cavities in the presence of absorbers. The resulting model realizes a toolkit with which design guidelines of the absorber's properties and location can be optimized over a frequency band. Analytic predictions of shielding effectiveness for three transverse magnetic modes for various locations of the absorber placed on the inside cavity wall show good agreement with both full-wave simulations and experiments, and validate the proposed model. This analysis opens new avenues for specialized ways to mitigate harmful fields within cavities.

36 MATERIALS SCIENCE↗

Constraining the impact of chlorine as a neutron absorber in next-gen fast reactor designs

The role of chlorine as a neutron poison and as a seed for producing radioactive waste in nuclear systems has driven a renewed interest to improve its nuclear data uncertainties. Additionally, basic and applied science programs that use CLYC (Cs 2 LiYCl 6 :Ce) detectors for neutron spectroscopy and monitoring are also very sensitive to any change in chlorine nuclear data for simulations of the detector response. In this work, sensitivities relevant for these different applications are addressed through simulations of the efficiency of CLYC detectors in a fast fission spectrum when applying new chlorine nuclear data as input. These simulations are validated by an experimental measurement using CLYC detectors coupled to an ionization chamber loaded with a 252 Cf spontaneous fission source. The results are then used to obtain the first reliable direct measurement of the 35 Cl(n,p 0 ) and summed Cl(n,p+n,α) fission spectrum average cross sections, found to be 54.7(32) and 105.0(98) mb, respectively. The results are within uncertainty of calculated fission spectrum averaged cross sections based on recently re-evaluated chlorine nuclear data, which confirm recent impact studies performed for the Molten Chloride Reactor Experiment. Meanwhile, there currently exists only one published criticality benchmark experiment that is sufficiently sensitive to chlorine nuclear data. Discrepancies are found with this set of criticality safety benchmarks, which are more sensitive to thermal and epithermal neutron energies than the energies, above 100 keV, tested in this current work. Hence, there is still a need to re-evaluate the chlorine nuclear data at lower energies to assess these discrepancies. Interpretation of the data from future “faster” criticality benchmarks, which are needed for next-gen fast reactor designs, benefit from the improved constraints on the chlorine nuclear data validated in this work.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗