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DOE OSTI2021

Exploring the elevated water vapor signal associated with the free tropospheric biomass burning plume over the southeast Atlantic Ocean

In southern Africa, widespread agricultural fires produce substantial biomass burning (BB) emissions over the region. The seasonal smoke plumes associated with these emissions are then advected westward over the persistent stratocumulus cloud deck in the southeast Atlantic (SEA) Ocean, resulting in aerosol effects which vary with time and location. Much work has focused on the effects of these aerosol plumes, but previous studies have also described an elevated free tropospheric water vapor signal over the SEA. Water vapor influences climate in its own right, and it is especially important to consider atmospheric water vapor when quantifying aerosol-cloud interactions and aerosol radiative effects. Here we present airborne observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) campaign over the SEA Ocean. In observations collected from multiple independent instruments on the NASA P-3 aircraft (from near-surface to 6-7 km), we observe a strongly linear correlation between pollution indicators (carbon monoxide (CO) and aerosol loading) and atmospheric water vapor content, seen at all altitudes above the boundary layer. The focus of the current study is on the especially strong correlation observed during the ORACLES-2016 deployment (out of Walvis Bay, Namibia), but a similar relationship is also observed in the August 2017 and October 2018 ORACLES deployments. Using reanalyses from the European Centre for Medium-Range Weather Forecasts (ECMWF) and Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2), and specialized WRF-Chem simulations, we trace the plume-vapor relationship to an initial humid, smoky continental source region, where it mixes with clean, dry upper tropospheric air and then is subjected to conditions of strong westward advection, namely the southern African easterly jet (AEJ-S). Our analysis indicates that air masses likely left the continent with the same relationship between water vapor and carbon monoxide as was observed by aircraft. This linear relationship developed over the continent due to daytime convection within a deep continental boundary layer (up to ~5-6 km) and mixing with higher-altitude air, which resulted in fairly consistent vertical gradients in CO and water vapor, decreasing with altitude and varying in time, but this water vapor does not originate as a product of the BB combustion itself. Due to a combination of conditions and mixing between the smoky, moist continental boundary layer and the dry and fairly clean upper-troposphere air above (~6 km), the smoky, humid air is transported by strong zonal winds and then advected over the SEA (to the ORACLES flight region) following largely isentropic trajectories. Hybrid Single-Particle Lagrangian Integrated Trajectory model (HYSPLIT) back trajectories support this interpretation. This work thus gives insights into the conditions and processes which cause water vapor to covary with plume strength. Better understanding of this relationship, including how it varies spatially and temporally, is important to accurately quantify direct, semi-direct, and indirect aerosol effects over this region.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1994

Contrasting conditions of surface water balance in wet years and dry years as a possible land surface-atmosphere feedback mechanism in the West African Sahel

The climate of West Africa, in particular the Sahel, is characterized by multiyear persistence of anomalously wet or dry conditions. Its Southern Hemisphere counterpart, the Kalahari, lacks the persistence that is evident in the Sahel even though both regions are subject to similar large-scale forcing. It has been suggested that land surface-atmosphere feedback contributes to this persistence and to the severity of drought. In this study, surface energy and water balance are quantified for nine stations along a latitudinal transect that extends from the Sahara to the Guinea coast. In the wetter regions of West Africa, the difference between wet and dry years is primarily reflected in the magnitude of runoff. For the Sahel and drier locations, evapotranspiration and soil moisture are more sensitive to rainfall anomalies. The increase in evapotranspiration, and hence latent heating, over the Sahel in wet years alters the thermal structure and gradients of the overlying atmosphere and thus the strength of the African easterly jet (AEJ) at 700 mb. The difference between dry and wet Augusts corresponds to a decrease in magnitude of the AEJ at 15 deg N on the order of 2.6 m/s, which is consistent with previous studies of observed winds. Spatial patterns were also developed for surface water balance parameters for both West Africa and southern Africa. Over southern Africa, the patterns are not as spatially homogeneous as those over West Africa and are lower in magnitude, thus supporting the suggestion that the persistence of rainfall anomalies in the Sahel might be due, at least in part, to land-atmosphere feedback, and that the absence of such persistence in the Kalahari is a consequence of less significant changes in surface water and energy balance.

Lare, A. R.↗

NASA NTRS2003

Summer Synoptic-Scale Waves over Tropical West Africa Observed by TRMM

A 5-year daily rainfall dataset (3B42) from TRMM (Tropical Rainfall Measuring Mission) is used to investigate the activity and properties of westward-propagating synoptic-scale waves over tropical West Africa. Evident wave signals appearing in wavenumber-frequency space show their modulations on the surface rainfall pattern during the boreal summer. Interannual variability exists in both their intensity and spectral properties, i. e., dominant frequency and wavenumber ranges. These variabilities can be partly ascribed to year-to-year variations of their embedded large-scale environment, especially the status of mid-tropospheric African easterly jet (AEJ). Generally, a stronger (weaker) AEJ indicates more (less) instability energy yielding a stronger (weaker) wave activity season. Seasonal mean rainfall has shown an impact on these waves in some years. However, the impact is not as clear and consistent as AEJ, implying the complexity of their relationship with large-scale environment. To fully understand interannual variability of synoptic-scale waves over tropical West Africa, including the variability in their preferred frequencies and wavenumbers, it is therefore necessary to examine possible intra-seasonal variations existing in both wave activity and large-scale fields, in addition to their structure, propagation, and associated convection.

Starr, David O.↗

NASA NTRS2004

African Equatorial and Subtropical Ozone Plumes: Recurrences Timescales of the Brown Cloud Trans-African Plumes and Other Plumes

We have found repeated illustrations in the maps of Total Tropospheric Ozone (TTO) of apparent transport of ozone from the Indian Ocean to the Equatorial Atlantic Ocean. Most interesting are examples that coincide with the INDOEX observations of late northern winter, 1999. Three soundings associated with the SHADOZ (Southern Hemisphere Additional Ozonesondes) network help confirm and quantify degree of influence of pollution, lightning, and stratospheric sources, suggesting that perhaps 40% of increased Atlantic ozone could be Asian pollution during periods of maximum identified in the TTO maps. We outline recurrent periods of apparent ozone transport from Indian to Atlantic Ocean regions both during and outside the late-winter period. These are placed in the context of some general observations about factors controlling recurrence timescales for the expression of both equatorial and subtropical plumes. Low-level subtropical plumes are often controlled by frontal systems approaching the Namib coast; these direct mid-level air into either easterly equatorial plumes or westerly mid- troposphere plumes. Equatorial plumes of ozone cross Africa on an easterly path due to the occasional coincidence of two phenomena: (1) lofting of ozone to mid and upper levels, often in the Western Indian Ocean, and (2) the eastward extension of an Equatorial African easterly jet.

Chatfield, Robert B.↗

NASA NTRS2009

Improving Our Understanding of Atlantic Hurricanes Through Knowledge of the Saharan Air Layer: Hope Or Hype?

The existence of the Saharan air layer (SAL), a layer of warm, dry, dusty air frequently present over the tropical Atlantic Ocean, has long been appreciated. The nature of its impact on hurricanes remains unclear, with some researchers arguing that the SAL amplifies hurricane development and with others arguing that it inhibits it. The potential negative impacts of the SAL include 1) low-level vertical wind shear associated with the African easterly jet; 2) warm air aloft, which increases thermodynamic stability; and 3) dry air, which produces cold downdrafts. Some investigators have assumed the validity of these proposed negative influences and have frequently used them to explain the failure of individual storms to intensify or to explain the relative inactivity of recent hurricane seasons. Multiple NASA satellite data sets and National Centers for Environmental Prediction global analyses are used to characterize the SAL's properties and evolution in relation to developing hurricanes. The results will shows that neither jet--induced vertical wind shear nor warm SAL air (high stability) produce significant negative impacts on Atlantic storms. Dry air appears to be a key mechanism for SAL influence, but the presence of dry SAL air is not always a good indicator of whether a storm will weaken since many examples of intensifying storms surrounded by such dry air can be found. Idealized simulations will be used to evaluate the role of dry air. Finally, two case studies of supposedly "prime examples" of SAL influence will show that the negative influences of the SAL are perhaps too readily ascribed to individual storms that fail to reach their maximum potential intensity.

Braun, Scott↗

NASA NTRS2010

Re-Evaluating the Role of the Saharan Air Layer in Atlantic Tropical Cyclogenesis and Evolution

Braun, Scott A.↗

NASA NTRS2011

An Investigation of Interaction of Saharan Dust and Atlantic ITCZ Using Cloudsat-Calipso and A-Train Data

In this study, we investigate the radiative forcing of Saharan dust, its interactions with the Atlantic Intertropical Convergence Zone (ITCZ), through African easterly waves (AEW), African easterly jets (AEJ), and its impacts in short term numerical forecasts of tropical cyclogenesis using the GOCART-GEOS5 forecast system. Our approach is to develop and use an A-Train satellite simulator (ATSS) to constrain the observed aerosol index of refraction and particle size distribution by finding the values that simultaneously minimize the difference between observed CALIOP, CloudSat, OMI, and MODIS radiances and simulated radiances inverted from atmospheric model output using procedures and physical principles consistent with those used in corresponding retrieval algorithms. We use observations from the A-train and TRMM to determine relationships among the Saharan dust layer, transport by the AEW, and possible responses to dust radiative forcing in developing tropical cyclones in the A-ITCZ. Preliminary model results showing physical processes associated with the generation and transport of the Saharan dust layer, their interactions with the incipient moisture, clouds and rainfall in developing tropical cyclones will be presented. Also presented will be results of a case study of possible radiative impacts on AEW and AEJ during the NAMMA field campaign.

Lau, W.↗

NASA NTRS2010

A Northward Shift of the North Atlantic Ocean Intertropical Convergence Zone in Response to Summertime Saharan Dust Outbreaks

The influence on the summertime North Atlantic Ocean inter-tropical convergence zone (ITCZ) of Saharan dust outbreaks is explored using nine years of continuous satellite observations and atmospheric reanalysis products. During dust outbreak events rainfall along the ITCZ shifts northward by 1 to 4 degrees latitude. Dust outbreaks coincide with warmer lower-tropospheric temperatures compared to low dust conditions, which is attributable to advection of the warm Saharan Air Layer, enhanced subtropical subsidence, and radiative heating of dust. The enhanced positive meridional temperature gradient coincident with dust outbreaks is accompanied by an acceleration of the easterly winds on the n011h side of the African Easterly Jet (AEJ). The center of the positive vorticity region south of the AEJ moves north drawing the center of low-level convergence and ITCZ rainfall northward with it. The enhanced precipitation on the north side of the ITCZ occurs in spite of widespread sea surface temperature cooling north of the ITCZ owing to reduced surface solar insolation by dust scattering.

Wilcox, Eric M.↗

NASA NTRS2010

African Easterly Waves in 30-day High-Resolution Global Simulations: A Case Study During the 2006 NAMMA Period

In this study, extended -range (30 -day) high-resolution simulations with the NASA global mesoscale model are conducted to simulate the initiation and propagation of six consecutive African easterly waves (AEWs) from late August to September 2006 and their association with hurricane formation. It is shown that the statistical characteristics of individual AEWs are realistically simulated with larger errors in the 5th and 6th AEWs. Remarkable simulations of a mean African easterly jet (AEJ) are also obtained. Nine additional 30 -day experiments suggest that although land surface processes might contribute to the predictability of the AEJ and AEWs, the initiation and detailed evolution of AEWs still depend on the accurate representation of dynamic and land surface initial conditions and their time -varying nonlinear interactions. Of interest is the potential to extend the lead time for predicting hurricane formation (e.g., a lead time of up to 22 days) as the 4th AEW is realistically simulated.

Shen, Bo-Wen↗

NASA NTRS2013

Impact of Radiatively Interactive Dust Aerosols in the NASA GEOS-5 Climate Model: Sensitivity to Dust Particle Shape and Refractive Index

We investigate the radiative effects of dust aerosols in the NASA GEOS-5 atmospheric general circulation model. GEOS-5 is improved with the inclusion of a sectional aerosol and cloud microphysics module, the Community Aerosol and Radiation Model for Atmospheres (CARMA). Into CARMA we introduce treatment of the dust and sea salt aerosol lifecycle, including sources, transport evolution, and sinks. The aerosols are radiatively coupled to GEOS-5, and we perform a series of multi-decade AMIP-style simulations in which dust optical properties (spectral refractive index and particle shape distribution) are varied. Optical properties assuming spherical dust particles are from Mie theory, while those for non-spherical shape distributions are drawn from a recently available database for tri-axial ellipsoids. The climatologies of the various simulations generally compare well to data from the MODIS, MISR, and CALIOP space-based sensors, the ground-based AERONET, and surface measurements of dust deposition and concentration. Focusing on the summertime Saharan dust cycle we show significant variability in our simulations resulting from different choices of dust optical properties. Atmospheric heating due to dust enhances surface winds over important Saharan dust sources, and we find a positive feedback where increased dust absorption leads to increased dust emissions. We further find that increased dust absorption leads to a strengthening of the summertime Hadley cell circulation, increasing dust lofting to higher altitudes and strengthening the African Easterly Jet. This leads to a longer atmospheric residence time, higher altitude, and generally more northward transport of dust in simulations with the most absorbing dust optical properties. We find that particle shape, although important for radiance simulations, is a minor effect compared to choices of refractive index, although total atmospheric forcing is enhanced by greater than 10 percent for simulations incorporating a spheroidal shape distribution versus ellipsoidal or spherical shapes.

radiative forcing↗

NASA NTRS2018

Microphysics and Radiation Effect of Dust on Saharan Air Layer: An HS3 Case Study

A Saharan air layer (SAL) event associated with a nondeveloping African easterly wave (AEW) over the main development region of the eastern Atlantic was sampled by the NASA Global Hawk aircraft on 24-25 August 2013 during the NASA Hurricane and Severe Storm Sentinel (HS3) campaign and was simulated with the NASA Unified Weather Research and Forecasting (NU-WRF) Model. Airborne, ground-based, and spaceborne measurements were used to evaluate the model performance. The microphysical and radiative effects of dust and other aerosols on the SAL structure and environment were investigated with the factor-separation method. The results indicate that relative to a simulation without dust-radiative and microphysical impacts, Saharan dust and other aerosols heated the SAL air mainly through shortwave heating by the direct aerosol-radiation (AR) effect, resulting in a warmer (up to 0.6 K) and drier (up to 5% RH reduction) SAL and maintaining the strong temperature inversion at the base of the SAL in the presence of predominant longwave cooling. Radiative heating of the dust accentuated a vertical circulation within the dust layer, in which air rose (sank) in the northern (southern) portions of the dust layer. Furthermore, above and to the south of the dust layer, both the microphysical and radiative impacts of dust tended to counter the vertical motions associated with the Hadley circulation, causing a small weakening and southward shift of convection in the intertropical convergence zone (ITCZ) and reduced anvil cloud to the north. Changes in moisture and cloud/precipitation hydrometeors were largely driven by the dust induced changes in vertical motion. Dust strengthened the African easterly jet by up to ~1ms(exp -1) at the southern edge of the jet, primarily through the AR effect, and produced modest increases in vertical wind shear within and in the vicinity of the dust layer. These modulations of the SAL and AEW environment clearly contributed to the nondevelopment of this AEW.

Tao, Zhining↗

NASA NTRS2018

Recent Rainfall Decline in West Africa Due to Enhanced Biomass Burning and Dust Emission

Rainfall in West Africa during boreal summer is primarily controlled by the low-level southerly monsoon flow that transports moisture from the Gulf of Guinea to the region and the African Easterly Jet that modulates the convective systems. However, the role of aerosols in rainfall variability of this region, despite the large emissions of dust and black carbon in Africa, is not well-understood. Our study reveals a decline in precipitation over Southern West Africa (SWA) in the past two decades that its trend and interannual variability present an indirect relationship with the aerosols loadings. Examining the local and remote sources of aerosols, we found that the latter have a larger contribution. We have used MERRA-2 large scale atmospheric dynamics and physics data to determine the mechanisms responsible for aerosol-rainfall interactions in the region. Our results have important implications for the people and ecosystem as the increasing rates of land use change, deforestation and urbanization in the continent are expected to enhance the aerosols. This will result in an increase in the frequency and intensity of the extreme events including droughts.

Dezfuli, Amin↗

NASA NTRSDate not supplied

Exploring the Elevated Water Vapor Signal Associated With the Free Tropospheric Biomass Burning Plume Over the Southeast Atlantic Ocean

In southern Africa, widespread agricultural fires produce substantial biomass burning (BB) emissions over the region. The seasonal smoke plumes associated with these emissions are then advected westward over the persistent stratocumulus cloud deck in the southeast Atlantic (SEA) Ocean, resulting in aerosol effects which vary with time and location. Much work has focused on the effects of these aerosol plumes, but previous studies have also described an elevated free tropospheric water vapor signal over the SEA. Water vapor influences climate in its own right, and it is especially important to consider atmospheric water vapor when quantifying aerosol–cloud interactions and aerosol radiative effects. Here we present airborne observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) campaign over the SEA Ocean. In observations collected from multiple independent instruments on the NASA P-3 aircraft (from near-surface to 6–7 km), we observe a strongly linear correlation between pollution indicators (carbon monoxide (CO) and aerosol loading) and atmospheric water vapor content, seen at all altitudes above the boundary layer. The focus of the current study is on the especially strong correlation observed during the ORACLES-2016 deployment (out of Walvis Bay, Namibia), but a similar relationship is also observed in the August 2017 and October 2018 ORACLES deployments. Using reanalyses from the European Centre for Medium-Range Weather Forecasts (ECMWF) and Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2), and specialized WRF-Chem simulations, we trace the plume–vapor relationship to an initial humid, smoky continental source region, where it mixes with clean, dry upper tropospheric air and then is subjected to conditions of strong westward advection, namely the southern African easterly jet (AEJ-S). Our analysis indicates that air masses likely left the continent with the same relationship between water vapor and carbon monoxide as was observed by aircraft. This linear relationship developed over the continent due to daytime convection within a deep continental boundary layer (up to ∼5–6 km) and mixing with higher-altitude air, which resulted in fairly consistent vertical gradients in CO and water vapor, decreasing with altitude and varying in time, but this water vapor does not originate as a product of the BB combustion itself. Due to a combination of conditions and mixing between the smoky, moist continental boundary layer and the dry and fairly clean upper-troposphere air above (∼6 km), the smoky, humid air is transported by strong zonal winds and then advected over the SEA (to the ORACLES flight region) following largely isentropic trajectories. Hybrid Single-Particle Lagrangian Integrated Trajectory model (HYSPLIT) back trajectories support this interpretation. This work thus gives insights into the conditions and processes which cause water vapor to covary with plume strength. Better understanding of this relationship, including how it varies spatially and temporally, is important to accurately quantify direct, semi-direct, and indirect aerosol effects over this region.

Kristina Pistone↗

NASA NTRSDate not supplied

Biomass Burning Smoke and Coincident Water Vapor Over the Southeast Atlantic Stratocumulus Region: Results from Observations and Models

Kristina Pistone↗

NASA NTRSDate not supplied

Excessive Subsidence of the Southeast Atlantic Biomass Burning Aerosol Plume in the NASA Goddard Earth Observing System (GEOS) Model

Global models struggle to accurately represent the meteorological environment over the Southeast Atlantic Ocean, as evidenced by the poor representation of persistent marine stratocumulus decks off the west coast of southern Africa. This complex regime also experiences significant seasonal biomass burning aerosol plumes that are transported from southern Africa over the Atlantic Ocean, which gradually descend via large scale subsidence and interact radiatively and microphysically with the cloudy environment of the region. In comparisons to space borne lidar and aircraft observations we find that the NASA Goddard Earth Observing System (GEOS) model’s MERRA-2 aerosol and meteorology reanalysis shows that the aerosol plume descends too rapidly due to exaggerated large-scale downward vertical motion. This complicates the evaluation of aerosol properties utilizing aircraft observations collected throughout the ORACLES campaign as well as the model’s representation of the heating rate profiles due to the aerosol itself and its radiative interaction with the semi-permanent cloud deck typically located lower in altitude than the smoke. Two types of modeling experiments using GEOS will be presented to diagnose deficiencies in the model related to the excessive subsidence. Ensembles of free-running model simulations with and without radiatively active biomass burning aerosol will be used to quantify the impact of smoke on the atmospheric circulation. It will be demonstrated that heating within the aerosol layer results in self lofting through a reduction of the subsidence but did not alter the vertical placement or speed of the African Easterly jet. The amount of aerosol absorption required to eliminate the bias in the height of the aerosol plume through self-lofting will then be quantified. Finally, a second type of modeling experiment will be discussed in which the meteorology is constrained to observations. This will allow for biases in the height of the aerosol plume due to the general circulation model to be distinguished from biases that may be induced through the data assimilation process.

Allison Collow↗

NASA NTRS1993

The influence of land surface properties on Sahel climate. Part 1: Desertification

This is a general circulation model sensitivity study of the physical mechanisms of the effects of desertification on the Sahel drought. The model vegetation types were changed in the prescribed desertification area, which led to changes in the surface characteristics. The model was integrated for three months (June, July, August) with climatological surface conditions (control) and desertification conditions (anomaly) to examine the summer season response to the changed surface conditions. The control and anomaly experiments consisted of five pairs of integrations with different initial conditions and/or sea surface temperature boundary conditions. In the desertification experiment, the moisture flux convergence and rainfall were reduced in the test area and increased to the immediate south of this area. The simulated anomaly dipole pattern was similar to the observed African drought patterns in which the axis of the maximum rainfall shifts to the south. The circulation changes in the desertification experiment were consistent with those observed during sub-Saharan dry years. The tropical easterly jet was weaker and the African easterly jet was stronger than normal. Further, in agreement with the observations, the easterly wave disturbances were reduced in intensity but not in number. Descending motion dominated the desertification area. The surface energy budget and hydrological cycle were also changed substantially in the anomaly experiment.

Xue, Yongkang↗

DOE OSTI2025

More biomass burning aerosol is being advected westward over the southern tropical Atlantic since 2003

Not Available

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2012

The Impact of Dry Saharan Air on Tropical Cyclone Intensification

The controversial role of the dry Saharan Air Layer (SAL) on tropical storm intensification in the Atlantic will be addressed. The SAL has been argued in previous studies to have potential positive influences on storm development, but most recent studies have argued for a strong suppressing influence on storm intensification as a result of dry air, high stability, increased vertical wind shear, and microphysical impacts of dust. Here, we focus on observations of Hurricane Helene (2006), which occurred during the NASA African Monsoon Multidisciplinary Activities (NAMMA) experiment. Satellite and airborne observations, combined with global meteorological analyses depict the initial environment of Helene as being dominated by the SAL, although with minimal evidence that the SAL air actually penetrated to the core of the disturbance. Over the next several days, the SAL air quickly moved westward and was gradually replaced by a very dry, dust-free layer associated with subsidence. Despite the wrapping of this very dry air around the storm, Helene intensified steadily to a Category 3 hurricane suggesting that the dry air was unable to significantly slow storm intensification. Several uncertainties remain about the role of the SAL in Helene (and in tropical cyclones in general). To better address these uncertainties, NASA will be conducting a three year airborne campaign called the Hurricane and Severe Storm Sentinel (HS3). The HS3 objectives are: To obtain critical measurements in the hurricane environment in order to identify the role of key factors such as large-scale wind systems (troughs, jet streams), Saharan air masses, African Easterly Waves and their embedded critical layers (that help to isolate tropical disturbances from hostile environments). To observe and understand the three-dimensional mesoscale and convective-scale internal structures of tropical disturbances and cyclones and their role in intensity change. The mission objectives will be achieved using two Global Hawk (GH) Unmanned Airborne Systems (UASs) with separate comprehensive environmental and over-storm payloads. The GH flight altitudes (>16.8 km) allow overflights of most convection and sampling of upper-tropospheric winds. Deployments from Goddard s Wallops Flight Facility and ~26-hour flight durations will provide coverage of the entire Atlantic Ocean basin, and on-station times up to 5-22 h depending on storm location. Deployments will be in September of 2012 and from late-August to late- September 2013-2014, with up to eleven 26-h flights per deployment.

Braun, Scott A.↗