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At least 37 records · Page 2

Aerosol Sources, Absorption, and Intercontinental Transport: Synergies Among Models, Remote Sensing, and Atmospheric Measurements

Aerosol climate forcing is one of the largest uncertainties in assessing the anthropogenic impact on the global climate system. This uncertainty arises from the poorly quantified aerosol sources, especially black carbon emissions, our limited knowledge of aerosol mixing state and optical properties, and the consequences of intercontinental transport of aerosols and their precursors. Here we use a global model GOCART to simulate atmospheric aerosols, including sulfate, black carbon, organic carbon, dust, and sea salt, from anthropogenic, .biomass burning, and natural sources. We compare the model calculated aerosol extinction and absorption with those quantities from the ground-based sun photometer measurements from AERON" at several different wavelengths and the field observations from ACE-Asia, and model calculated total aerosol optical depth and fine mode fractions with the MODIS satellite retrieval. We will also estimate the intercontinental transport of pollution and dust aerosols from their source regions to other areas in different seasons.

Chin, Mian↗

The interactive global fire module pyrE (v1.0)

Fires affect the composition of the atmosphere and Earth’s radiation balance by emitting a suite of reactive gases and particles. An interactive fire module in an Earth system model (ESM) allows us to study the natural and anthropogenic drivers, feedbacks, and interactions of open fires. To do so, we have developed pyrE, the NASA GISS (Goddard Institute for Space Studies) interactive fire emissions *module. The pyrE module is driven by environmental variables like flammability and cloud-to-ground lightning, calculated by the GISS ModelE ESM, and parameterized by anthropogenic impacts based on population density data. Fire emissions are generated from the flaming phase in pyrE (active fires). Using pyrE, we examine fire occurrence, regional fire suppression, burned area, fire emissions, and how it all affects atmospheric composition. To do so, we evaluate pyrE by comparing it to satellite-based datasets of fire count, burned area, fire emissions, and aerosol optical depth (AOD). We demonstrate pyrE’s ability to simulate the daily and seasonal cycles of open fires and resulting emissions. Our results indicate that interactive fire emissions are biased low by 32 %–42 %, depending on emitted species, compared to the GFED4s (Global Fire Emissions Database) inventory. The bias in emissions drives underestimation in column densities, which is diluted by natural and anthropogenic emissions sources and production and loss mechanisms. Regionally, the resulting AOD of a simulation with interactive fire emissions is underestimated mostly over Indonesia compared to a simulation with GFED4s emissions and to MODIS AOD. In other parts of the world pyrE’s performance in terms of AOD is marginal to a simulation with prescribed fire emissions.

Fires↗

Interpretation of Lidar and Satellite Data Sets Using a Global Photochemical Model

A primary goal of the NASA Tropospheric Chemistry Program (TCP) is to "contribute substantially to scientific understanding of human impacts on the global troposphere". In order to analyze global or regional trends and factors of the troposphere chemistry, for example, its oxidation capacity or composition, a continuous global/regional data coverage as well as model simulations are needed. The Global Tropospheric Experiment (GTE), a major component of the TCP, provides data vital to these questions via aircraft measurement of key trace chemical species in various remote regions of the world. Another component in NASA's effort are satellite projects for exploration of tropospheric chemistry and dynamics. A unique data product is the Tropospheric Ozone Residual (TOR) utilizing global tropospheric ozone data. Another key research tool are simulation studies of atmospheric chemistry and dynamics for the theoretical understanding of the atmosphere, the extrapolation of observed trends, and for sensitivity studies assessing a changing anthropogenic impact to air chemistry and climate. In the context with model simulations, field data derived from satellites or (airborne) field missions are needed for two purposes: 1. To initialize and validate model simulations, and 2., to interpret field data by comparison to model simulation results in order to analyze global or regional trends and deviations from standard tropospheric chemistry and transport conditions as defined by the simulations. Currently, there is neither a sufficient global data coverage available nor are existing well established global circulation models. The NASA LARC CTM model is currently not yet in a state to accomplish a sufficient tropospheric chemistry simulation, so that the current research under this cooperative agreement focuses on utilizing field data products for direct interpretation. They will be also available for model testing and a later interpretation with a finally utilized model.

Zenker, Thomas↗

Chemistry and transport in a multi-dimensional model

The focus of our research program is the achievement of a quantitative understanding of the spatial distribution and temporal variation of chemical species in the terrestrial middle atmosphere, with emphasis on ozone. Although not directed at assessments of anthropogenic impacts, our activities contribute to a refinement of model descriptions of chemical and dynamical processes that are needed for assessment tasks. A unique feature of our research effort is a close interaction with the chemical kinetics group at JPL and the field measurement groups at JPL. The principal tools used in our investigations are l-D and 2-D photochemical models. The advective component of the meridional transport in these models is approximated by the diabatic circulation, which is derived diagnostically from the net radiative heating rates. We are developing accurate radiative transfer algorithms to find the net heating rates and the diabatic circulation for use in the 2-D model.

Yung, Yuk L.↗

Establishing the Global Fresh Water Sensor Web

This paper presents an approach to measuring the major components of the water cycle from space using the concept of a sensor-web of satellites that are linked to a data assimilation system. This topic is of increasing importance, due to the need for fresh water to support the growing human population, coupled with climate variability and change. The net effect is that water is an increasingly valuable commodity. The distribution of fresh water is highly uneven over the Earth, with both strong latitudinal distributions due to the atmospheric general circulation, and even larger variability due to landforms and the interaction of land with global weather systems. The annual global fresh water budget is largely a balance between evaporation, atmospheric transport, precipitation and runoff. Although the available volume of fresh water on land is small, the short residence time of water in these fresh water reservoirs causes the flux of fresh water - through evaporation, atmospheric transport, precipitation and runoff - to be large. With a total atmospheric water store of approx. 13 x 10(exp 12)cu m, and an annual flux of approx. 460 x 10(exp 12)cu m/y, the mean atmospheric residence time of water is approx. 10 days. River residence times are similar, biological are approx. 1 week, soil moisture is approx. 2 months, and lakes and aquifers are highly variable, extending from weeks to years. The hypothesized potential for redistribution and acceleration of the global hydrological cycle is therefore of concern. This hypothesized speed-up - thought to be associated with global warming - adds to the pressure placed upon water resources by the burgeoning human population, the variability of weather and climate, and concerns about anthropogenic impacts on global fresh water availability.

Hildebrand, Peter H.↗

Advances in Landslide Hazard Forecasting: Evaluation of Global and Regional Modeling Approach

A prototype global satellite-based landslide hazard algorithm has been developed to identify areas that exhibit a high potential for landslide activity by combining a calculation of landslide susceptibility with satellite-derived rainfall estimates. A recent evaluation of this algorithm framework found that while this tool represents an important first step in larger-scale landslide forecasting efforts, it requires several modifications before it can be fully realized as an operational tool. The evaluation finds that the landslide forecasting may be more feasible at a regional scale. This study draws upon a prior work's recommendations to develop a new approach for considering landslide susceptibility and forecasting at the regional scale. This case study uses a database of landslides triggered by Hurricane Mitch in 1998 over four countries in Central America: Guatemala, Honduras, EI Salvador and Nicaragua. A regional susceptibility map is calculated from satellite and surface datasets using a statistical methodology. The susceptibility map is tested with a regional rainfall intensity-duration triggering relationship and results are compared to global algorithm framework for the Hurricane Mitch event. The statistical results suggest that this regional investigation provides one plausible way to approach some of the data and resolution issues identified in the global assessment, providing more realistic landslide forecasts for this case study. Evaluation of landslide hazards for this extreme event helps to identify several potential improvements of the algorithm framework, but also highlights several remaining challenges for the algorithm assessment, transferability and performance accuracy. Evaluation challenges include representation errors from comparing susceptibility maps of different spatial resolutions, biases in event-based landslide inventory data, and limited nonlandslide event data for more comprehensive evaluation. Additional factors that may improve algorithm performance accuracy include incorporating additional triggering factors such as tectonic activity, anthropogenic impacts and soil moisture into the algorithm calculation. Despite these limitations, the methodology presented in this regional evaluation is both straightforward to calculate and easy to interpret, making results transferable between regions and allowing findings to be placed within an inter-comparison framework. The regional algorithm scenario represents an important step in advancing regional and global-scale landslide hazard assessment and forecasting.

Kirschbaum, Dalia B.↗

Perfluorinated Alkyl Acids in Plasma of American Alligators (Alligator Mississippiensis) from Florida and South Carolina

This study aimed to quantitate fourteen perfluoroalkyl acids (PFAAs) in 125 adult American alligators at twelve sites across the southeastern US. Of those fourteen PFAAs, nine were detected in 65% - 100% of the samples: PFOA, PFNA, PFDA, PFUnA, PFDoA, PFTriA, PFTA, PFHxS, and PFOS. Males (across all sites) showed significantly higher concentrations of four PFAAs: PFOS (p = 0.01), PFDA (p = 0.0003), PFUnA (p = 0.021), and PFTriA (p = 0.021). Concentrations of PFOS, PFHxS, and PFDA in plasma were significantly different among the sites in each sex. Alligators at Merritt Island National Wildlife Refuge and Kiawah Nature Conservancy both exhibited some of the highest PFOS concentrations (medians 99.5 ng/g and 55.8 ng/g respectively) in plasma measured to date in a crocodilian species. A number of positive correlations between PFAAs and snout-vent length (SVL) were observed in both sexes suggesting PFAA body burdens increase with increasing size. In addition, several significant correlations among PFAAs in alligator plasma may suggest conserved sources of PFAAs at each site throughout the greater study area. This study is the first to report PFAAs in American alligators, reveals potential PFAA hot spots in Florida and South Carolina, and provides and additional contaminant of concern when assessing anthropogenic impacts on ecosystem health.

crocodilians↗

Radar Altimetry as a Proxy for Determining Terrestrial Water Storage Variability in Tropical Basins

The Gravity Recovery and Climate Experiment (GRACE) mission has provided us with unforeseen information on terrestrial water-storage (TWS) variability, contributing to our understanding of global hydrological processes, including hydrological extreme events and anthropogenic impacts on water storage. Attempts to decompose GRACE-based TWS signals into its different water storage layers, i.e., surface water storage (SWS), soil moisture, groundwater and snow, have shown that SWS is a principal component, particularly in the tropics, where major rivers flow over arid regions at high latitudes. Here, we demonstrate that water levels, measured with radar altimeters at a limited number of locations, can be used to reconstruct gridded GRACE-based TWS signals in the Amazon basin, at spatial resolutions ranging from 0.5 to 3°, with mean absolute errors (MAE) as low as 2.5 cm and correlations as high as 0.98. We show that, at 3° spatial resolution, spatially-distributed TWS time series can be precisely reconstructed with as few as 41 water-level time series located within the basin. The proposed approach is competitive when compared to existing TWS estimates derived from physically based and computationally expensive methods. Also, a validation experiment indicates that TWS estimates can be extrapolated to periods beyond that of the model regression with low errors. The approach is robust, based on regression models and interpolation techniques, and offers a new possibility to reproduce spatially and temporally distributed TWS that could be used to fill inter-mission gaps and to extend GRACE-based TWS time series beyond its timespan.

Terrestrial water storage↗

Late Glacial and Holocene Environmental Variability, Lago Trasimeno, Italy

Lago Trasimeno (central Italy), 10 km wide and < 6m deep, fills a basin of tectonic origin, and is one of Europe's few endorheic lakes. We report on a multidisciplinary stratigraphic study based on seismic reflection profiles and two sediment cores, aimed at providing information on the vegetational, lithological, and climate history of this area. Trace elements, palynology, macrofossils, organic carbon, and C isotopes, coupled with AMS C-14 dating, describe environmental changes from Late-Glacial to present. The base of the cores records a Late-Glacial steppic vegetation (Poaceae, Artemisia, Amaranthaceae), with dry and cold conditions and a high charcoal/pollen ratio. An ensuing shift to a warmer and moister climate is shown by the rise of Pinus and Quercus, and shallow water aquatics such as Nitella. Early Holocene warming, indicated by Quercus, Oleaceae, Corylus, and Betula, is followed by a hiatus suggesting one or more severe drought events between 9000 and 3000 yr BP. Late Holocene presence of Alnus and Fagus indicates increased moisture, probably in winter, which would have increased lake level. Heavy metal pollution indicators (Pb, Cu, Zn) in the upper portion of the cores imply industrialization. Due to its location, to intensive and uninterrupted anthropogenic impacts since proto historical times, and to its shallow depths, Lago Trasimeno provides an important observation point for climate and environmental changes in the central Mediterranean region during and before Holocene times.

Lago trasimeno↗

A model investigation of the impact of increases in anthropogenic NOx emissions between 1967 and 1980 on tropospheric ozone

The impact of anthropogenic NOx emission on tropospheric ozone has been investigated. Two statistical models were used for estimating annual global emissions of NOx and for driving the trend in the emission for the years 1966-1980. Both models show a steady increase in the NOx emission, except for two brief periods of leveling off: after 1973 and after 1978. The impact was estimated by calculating the rates of emissions as functions of latitude, longitude, and year, with a one-dimensional (latitudinal) model, which included coupled tropospheric photochemistry and diffusive meridional transport. Steady-state photochemical calculations with prescribed NOx emissions appropriate for 1966 and 1980 indicate an ozone increase of 8-11 percent in the Northern Hemisphere, a result compatible with the rise in ozone suggested by the observations.

Dignon, J.↗

Assessment of Anthropogenic and Climatic Impacts on the Global Carbon Cycle Using a 3-D Model Constrained by Isotopic Carbon Measurements and Remote Sensing of Vegetation

Our original proposal called for improved modeling of the terrestrial biospheric carbon cycle, specifically using biome-specific process models to account for both the energy and water budgets of plant growth, to facilitate investigations into recent changes in global atmospheric CO2 abundance and regional distribution. The carbon fluxes predicted by these models were to be incorporated into a global model of CO2 transport to establish large-scale regional fluxes of CO2 to and from the terrestrial biosphere subject to constraints imposed by direct measurements of atmospheric CO2 and its 13C/12C isotopic ratio. Our work was coordinated with a NASA project (NASA NAGW-3151) at the University of Montana under the direction of Steven Running, and was partially funded by the Electric Power Research Institute. The primary objective of this project was to develop and test the Biome-BGC model, a global biological process model with a daily time step which simulates the water, energy and carbon budgets of plant growth. The primary product, the unique global gridded daily land temperature, and the precipitation data set which was used to drive the process model is described. The Biome-BGC model was tested by comparison with a simpler biological model driven by satellite-derived (NDVI) Normalized Difference Vegetation Index and (PAR) Photosynthetically Active Radiation data and by comparison with atmospheric CO2 observations. The simple NDVI model is also described. To facilitate the comparison with atmospheric CO2 observations, a three-dimensional atmospheric transport model was used to produce predictions of atmospheric CO2 variations given CO2 fluxes owing to (NPP) Net Primary Productivity and heterotrophic respiration that were produced by the Biome-BGC model and by the NDVI model. The transport model that we used in this project, and errors associated with transport simulations, were characterized by a comparison of 12 transport models.

Keeling, Charles D.↗

Impact of Nonabsorbing Anthropogenic Aerosols on Clear-Sky Atmospheric Absorption

Absorption of solar radiation by atmospheric aerosol has become recognized as important in regional and global climate. Nonabsorbing, hydrophilic aerosols, such as sulfate, potentially affect atmospheric absorption in opposing ways: first, decreasing absorption through aging initially hydrophobic black carbon (BC) to a hydrophilic state, enhancing its removal by wet scavenging, and consequently decreasing BC lifetime and abundance, and second, increasing absorption through enhancement of the BC absorption efficiency by internal mixing as well as through increasing the amount of diffuse solar radiation in the atmosphere. On the basis of General Circulation Model studies with an embedded microphysical aerosol module we systematically demonstrate the significance of these mechanisms both on the global and regional scales. In remote transport regions, the first mechanism prevails, reducing atmospheric absorption, whereas in the vicinity of source regions, despite enhanced wet scavenging, absorption is enhanced owing to the prevalence of the second mechanisms. Our findings imply that the sulfur to BC emission ratio plays a key role in aerosol absorption.

Stier, Philip↗

Anthropogenic Sulfate, Clouds, and Climate Forcing

This research work is a joint effort between research groups at the Battelle Pacific Northwest Laboratory, Virginia Tech University, Georgia Institute of Technology, Brookhaven National Laboratory, and Texas A&M University. It has been jointly sponsored by the National Aeronautics and Space Administration, the U.S. Department of Energy, and the U.S. Environmental Protection Agency. In this research, a detailed tropospheric aerosol-chemistry model that predicts oxidant concentrations as well as concentrations of sulfur dioxide and sulfate aerosols has been coupled to a general circulation model that distinguishes between cloud water mass and cloud droplet number. The coupled model system has been first validated and then used to estimate the radiative impact of anthropogenic sulfur emissions. Both the direct radiative impact of the aerosols and their indirect impact through their influence on cloud droplet number are represented by distinguishing between sulfuric acid vapor and fresh and aged sulfate aerosols, and by parameterizing cloud droplet nucleation in terms of vertical velocity and the number concentration of aged sulfur aerosols. Natural sulfate aerosols, dust, and carbonaceous and nitrate aerosols and their influence on the radiative impact of anthropogenic sulfate aerosols, through competition as cloud condensation nuclei, will also be simulated. Parallel simulations with and without anthropogenic sulfur emissions are performed for a global domain. The objectives of the research are: To couple a state-of-the-art tropospheric aerosol-chemistry model with a global climate model. To use field and satellite measurements to evaluate the treatment of tropospheric chemistry and aerosol physics in the coupled model. To use the coupled model to simulate the radiative (and ultimately climatic) impacts of anthropogenic sulfur emissions.

Ghan, Steven J.↗

Anthropogenic Nitrogen Inputs and Impacts on Oceanic N2O Fluxes in the Northern Indian Ocean: the Need for an Integrated Observation and Modelling Approach

Anthropogenically-derived nitrogen input to the northern Indian Ocean has increased significantly in recent decades, based on both observational and model derived estimates This external nutrient source is supplied by atmospheric deposition and riverine fluxes, and has the potential to affect the vulnerable biogeochemical systems of the Arabian Sea and Bay of Bengal, influencing productivity and oceanic production of the greenhouse-gas nitrous-oxide (N2O). We summarize current estimates of this external nitrogen source to the northern Indian Ocean from observations and models, highlight implications for regional marine N2O emissions using model-based analyses, and make recommendations for measurement and model needs to improve current estimates and future predictions of this impact. Current observationally-derived estimates of deposition and riverine nitrogen inputs are limited by sparse measurements and uncertainties on accurate characterization of nitrogen species composition. Ocean model assessments of the impact of external nitrogen sources on regional marine N2O production in the northern Indian Ocean estimate potentially significant changes but also have large associated uncertainties. We recommend an integrated program of basin-wide measurements combined with high-resolution modeling and more detailed characterization of nitrogen-cycle process to address these uncertainties and improve current estimates and predictions.

Parvadha Suntharalingam↗

Impacts of Intercontinental Transport of Anthropogenic Fine Particulate Matter on Human Mortality

Fine particulate matter with diameter of 2.5 microns or less (PM2.5) is associated with premature mortality and can travel long distances, impacting air quality and health on intercontinental scales. We estimate the mortality impacts of 20 % anthropogenic primary PM2.5 and PM2.5 precursor emission reductions in each of four major industrial regions (North America, Europe, East Asia, and South Asia) using an ensemble of global chemical transport model simulations coordinated by the Task Force on Hemispheric Transport of Air Pollution and epidemiologically-derived concentration-response functions. We estimate that while 93-97 % of avoided deaths from reducing emissions in all four regions occur within the source region, 3-7 % (11,500; 95 % confidence interval, 8,800-14,200) occur outside the source region from concentrations transported between continents. Approximately 17 and 13 % of global deaths avoided by reducing North America and Europe emissions occur extraregionally, owing to large downwind populations, compared with 4 and 2 % for South and East Asia. The coarse resolution global models used here may underestimate intraregional health benefits occurring on local scales, affecting these relative contributions of extraregional versus intraregional health benefits. Compared with a previous study of 20 % ozone precursor emission reductions, we find that despite greater transport efficiency for ozone, absolute mortality impacts of intercontinental PM2.5 transport are comparable or greater for neighboring source-receptor pairs, due to the stronger effect of PM2.5 on mortality. However, uncertainties in modeling and concentration-response relationships are large for both estimates.

human health↗

Intercontinental Transport of Aerosols: Implication for Regional Air Quality

Aerosol particles, also known as PM2.5 (particle diameter less than 2.5 microns) and PM10 (particle diameter less than 10 microns), is one of the key atmospheric components that determine ambient air quality. Current US air quality standards for PM10 (particles with diameter < 10 microns) and PM2.5 (particles with diameter 2.5 microns) are 50 pg/cu m and 15 pg/cu m, respectively. While local and regional emission sources are the main cause of air pollution problems, aerosols can be transported on a hemispheric or global scale. In this study, we use the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model to quantify contributions of long-range transport vs. local/regional pollution sources and from natural vs. anthropogenic sources to PM concentrations different regions. In particular, we estimate the hemispheric impact of anthropogenic sulfate aerosols and dust from major source areas on other regions in the world. The GOCART model results are compared with satellite remote sensing and ground-based network measurements of aerosol optical depth and concentrations.

Chin, Mian↗

Particle Events as a Possible Source of Large Ozone Loss during Magnetic Polarity Transitions

The energy deposition in the mesosphere and stratosphere during large extraterrestrial charged particle precipitation events has been known for some time to contribute to ozone losses due to the formation of potential ozone destroying species like NO(sub x), and HO(sub x). These impacts have been measured and can be reproduced with chemistry models fairly well. In the recent past, however, even the impact of the largest solar proton events on the total amount of ozone has been small compared to the dynamical variability of ozone, and to the anthropogenic induced impacts like the Antarctic 'ozone hole'. This is due to the shielding effect of the magnetic field. However, there is evidence that the earth's magnetic field may approach a reversal. This could lead to a decrease of magnetic field strength to less than 25% of its usual value over a period of several centuries . We show that with realistic estimates of very large solar proton events, scenarios similar to the Antarctic ozone hole of the 1990s may occur during a magnetic polarity transition.

vonKoenig, M.↗

What Does Global Land Climate Look Like at 2°C Warming?

Constraining an increase in global mean temperature below 2°C compared to pre-industrial levels is critical to limiting dangerous and cascading impacts of anthropogenic climate change. Understanding future climatic changes and their spatial heterogeneity at 2°C warming is thus important for policy makers to prepare actionable adaptation and mitigation plans by identifying where and to what extent lives and livelihoods will be impacted. This study uses the recently released NASA Earth eXchange Global Daily Downscaled Projections (NEX-GDDP) CMIP6 data to provide a broad overview of projected changes in six key climate variables and two climate impact indicators at a time when warming exceeds 2°C. Analysis of global mean temperature changes indicates the 2040s as the decade when most CMIP6 models reach 2°C warming with respect to a pre-industrial period (1850–1900). During the 2040s, we find that global mean temperature, precipitation, relative humidity, downwelling shortwave and longwave radiation, and wind speed over land under the high emission scenario are projected to change by +2.8°C, +22.4 mm/year, −0.73%, −2.23 , +15.9 W/m 2 , and −0.04 m/s, respectively. Many of the future changes are expected to exacerbate climate impacts including heat stress and fire danger. Our analysis shows geographic patterns of policy-relevant climatic changes, as parts of the globe will experience significant climate impacts even if the goal to keep warming below 2°C goal is achieved. Our results highlight the urgent need for further studies focused on identifying key hotspots and advancing region-specific actionable adaptation and mitigation plans.

GDDP↗