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DOE OSTI2025

Optically Addressing Circularly Polarized Vibrations in Molecules

Circularly polarized (CP) vibrations are the nuclear-motion analog of CP light, emerging in molecules with non-Abelian point-group symmetry that support orthogonal and degenerate vibrational normal modes. Here, in this work, we theoretically explore the optical addressability of CP vibrations, motivated by their potential as nanoscale angular momentum states suitable for information storage and manipulation. We investigate how symmetry-breaking chemical modifications affect a molecule’s capacity to support CP vibrations. Notably, we find cases where modes retain their orthogonality and degeneracy in spite of such modifications, broadening the opportunities afforded by CP vibrations beyond non-Abelian point-group molecules. Prospects for experimental implementations using CP pump–probe techniques are briefly discussed.

group theory↗

NASA NTRS1982

High-accuracy linear and circular polarization measurements at 21 cm

New high-accuracy linear and circular polarization measurements have been obtained for 27 small-diameter radio sources, using the Westerbork Synthesis Radio Telescope at 21 cm (1415 MHz). From these and other observed properties of the sources, estimates of the average internal magnetic field strengths in the sources are made by applying the uniform synchrotron emission model to the measured circular polarization and by using equipartition arguments. These two values are compared and found to be in agreement to within an order of magnitude, as was previously found by Weiler and de Pater (1980). Also, the magnetic fields estimated from circular polarization measurements at two different wavelengths (49 and 21 cm) are compared and found to be in rough agreement, but with indications of differences between variable and nonvariable sources. A comparison of the magnitudes of linear and circular polarization in sources shows no correlations.

De Pater, I.↗

DOE OSTI2023

First M87 Event Horizon Telescope Results. IX. Detection of Near-horizon Circular Polarization

Event Horizon Telescope (EHT) observations have revealed a bright ring of emission around the supermassive black hole at the center of the M87 galaxy. EHT images in linear polarization have further identified a coherent spiral pattern around the black hole, produced from ordered magnetic fields threading the emitting plasma. Here we present the first analysis of circular polarization using EHT data, acquired in 2017, which can potentially provide additional insights into the magnetic fields and plasma composition near the black hole. Interferometric closure quantities provide convincing evidence for the presence of circularly polarized emission on event-horizon scales. We produce images of the circular polarization using both traditional and newly developed methods. All methods find a moderate level of resolved circular polarization across the image ( $\langle$| v |$\rangle$ < 3.7%), consistent with the low image-integrated circular polarization fraction measured by the Atacama Large Millimeter/submillimeter Array (| v int |< 1%). Despite this broad agreement, the methods show substantial variation in the morphology of the circularly polarized emission, indicating that our conclusions are strongly dependent on the imaging assumptions because of the limited baseline coverage, uncertain telescope gain calibration, and weakly polarized signal. We include this upper limit in an updated comparison to general relativistic magnetohydrodynamic simulation models. This analysis reinforces the previously reported preference for magnetically arrested accretion flow models. We find that most simulations naturally produce a low level of circular polarization consistent with our upper limit and that Faraday conversion is likely the dominant production mechanism for circular polarization at 230 GHz in M87*.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1981

Antenna feed system for receiving circular polarization and transmitting linear polarization

An object is to provide for receiving a circularly polarized signal from an antenna feed (10) connected to orthogonally spaced antenna elements (11, 12, 13, 14) and for transmitting a linearly polarized signal through the same feed without switches, and without suffering a 3 dB polarization mismatch loss, using an arrangement of hybrid junctions. The arrangement is comprised of two dividing hybrid junctions (15, 16), each connected to a different pair of antenna elements and a summing hybrid junction (17). In one embodiment, a receiver (18) is connected to the summing hybrid junction directly. A diplexer (19a or 19b) is used to connect a transmitter (20a or 20b) to only one pair of antenna elements. In an alternative embodiment, designated left and right circularly polarized (LCP and RCP) transmitters (21, 22) are connected to the summing hybrid junction by separate diplexers (23, 24), and separate LCP and RCP sensitive receivers (25, 26) are connected to the diplexers in order to transmit linearly polarized signals using all four antenna elements while receiving circularly polarized signals as before. An orthomode junction (30) and horn antenna (32) may replace the two dividing hybrid junctions (15, 16) and antenna feed (10).

Seidel, Boris L.↗

NASA NTRS2022

Circular Polarization in Atmospheric Aerosols

Recent technological advances have demonstrated the feasibility of deploying spaceborne optical detectors with full polarimetric capabilities. The measurement of all four Stokes coefficients opens significant new opportunities for atmospheric aerosol studies and applications. While considerable amounts of attention have been dedicated to sensors with sensitivity to the total intensity and linear polarization (represented by Stokes coefficients I, U, Q), there has been less attention to the additional information brought by measuring circular polarization (coefficient V). This report fills this gap in knowledge by providing an overview of aerosol sources of circular polarization in the atmosphere and discusses possible remote sensing signatures. In this manuscript, circularly polarized radiation that results from the interaction of incident unpolarized radiation are considered in three physical settings: optical activity originating in biogenic aerosols, alignment of non-spherical particles in the presence of electrical fields (such as dust, smoke, and volcanic ash) and aerosol multiple scattering effects. Observational and theoretical evidence of, and the settings and conditions for non-zero aerosol circular polarization generated from incident unpolarized radiation are here gathered and discussed. In addition, novel radiative transfer simulations are shown to illustrate notable spectral and other features where circular polarization may provide additional information that is possibly independent from total intensity and linear polarization only observations. Current techniques for detection of aerosol composition (also referred as aerosol type) from space provide limited information. Remote identification of aerosols such as smoke, volcanic ash, and dust particles can only be accomplished with some degree of confidence for moderate to high concentrations. When the same aerosols are found at lower concentrations (but still high enough to be of importance for air quality and cloud formation), these methods often produce ambiguous results. The circular polarization of aerosols is rarely utilized, and we explore its value for improved determination aerosol composition. This study is presented as an overview with a goal to provide a new perspective on an overlooked optical property and to trigger interest in further exploration of this subject.

Aerosol type↗

NASA NTRS1978

Circular polarization of sunlight reflected by planetary atmospheres

Multiple scattering calculations are performed in order to investigate the nature of the circular polarization of sunlight reflected by planetary atmospheres. Contour diagrams as a function of size parameter and phase angle are made for the integrated light from a spherical but locally plane-parallel atmosphere of spherical particles. To investigate the origin of the circular polarization, results are also computed for second-order scattering and for a simpler semiquantitative model of scattering by two particles. Observations of the circular polarization of the planets are presently too meager for accurate deduction of cloud particle properties. However, certain very broad constraints can be placed on the properties of the dominant cloud particles on Jupiter and Saturn. The cloud particle size and refractive index deduced for the Jupiter clouds by Loskutov, Morozhenko, and Yanovitskii from analyses of the linear polarization are not consistent with the circular polarization. The few available circular polarization observations of Venus are also examined.

Kawata, Y.↗

DOE OSTI2024

Direct Observation of Circularly Polarized Nonlinear Optical Activities in Chiral Hybrid Lead Halides

Circularly polarized light emission is a crucial application in imaging, sensing, and photonics. However, utilizing low-energy photons to excite materials, as opposed to high-energy light excitation, can facilitate deep-tissue imaging and sensing applications. The challenge lies in finding materials capable of directly generating circularly polarized nonlinear optical effects. In this study, we introduce a chiral hybrid lead halide (CHLH) material system, R/S-DPEDPb 3 Br 8 ·H 2 O (DPED = 1,2-diphenylethylenediammonium), which can directly produce circularly polarized second harmonic generation (CP-SHG) through linearly polarized infrared light excitation, exhibiting a polarization efficiency as high as 37% at room temperature. To understand the spin relaxation mechanisms behind the high polarization efficiency, we utilized two models, so-called D’yakonov–Perel’ (DP) and Bir–Aronov–Pikus (BAP) mechanisms. The unique zigzag inorganic frameworks within the hybrid structure are believed to reduce the dielectric confinement and exciton binding energy, thus enhancing spin polarization, especially in regions with a high excitation pump fluence based on the DP mechanism. In the case of low excitation pump fluence, the BAP mechanism dominates, as evidenced by the observed decrease in the polarization ratio from CP-SHG measurement. Using density functional theory analysis, we elucidate how the distinctive 8-coordination environment of lead bromide building blocks effectively suppresses spin–orbit coupling at the conduction band minimum. This suppression significantly diminishes spin-splitting, thereby slowing the spin relaxation rate.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1972

Search for optical circular polarization in quasars and Seyfert nuclei.

A search for optical circular polarization has been made in six quasars, the nuclei of three Seyfert galaxies, BL Lac, and OJ 287. No positive effect was found in any of these objects, several of which have been reported to show circular polarization at radio wavelengths. It thus appears that optical circular polarization in quasars, if there is any, is not as strong as at radio wavelengths, and in the best-measured objects it is definitely less than 0.2%.

Landstreet, J. D.↗

NASA NTRS1979

Antenna feed system for receiving circular polarization and transmitting linear polarization

An invention is described which provides for receiving a circularly polarized signal from an antenna feed connected to orthogonally spaced antenna elements. It also provides for transmitting a linearly polarized signal through the same feed without switches, and without suffering a 3 dB polarization mismatch loss, using an arrangement of hybrid junctions. The arrangement is comprised of two dividing hybrid junctions, each connected to a different pair of antenna elements and a summing hybrid junction. In one version, a receiver is connected to the summing hybrid junction directly. A diplexer is used to connect a transmitter to only one pair of antenna elements. In another version, designated left and right circularly polarized (LCP and RCP) transmitters are connected to the summing hybrid junction by separate diplexers, and separate LCP and RCP sensitive receivers are connected to the diplexers in order to transmit linearly polarized signals using all four antenna elements while receiving circularly polarized signals as before. An orthomode junction and horn antenna may replace the two dividing hybrid junctions and antenna feed.

Seidel, B. L.↗

NASA NTRS1972

Circular polarization of twilight.

Review of observations of circular polarization of twilight performed with a polarimeter which uses an electronically switched Pockels cell operated as a reversible quarter-wave plate to convert circular into linear polarization. The latter was then analyzed by a Wollaston prism followed by two gallium-arsenide photomultipliers. The discovery of a definite natural circular polarization at twilight does suggest that, with increased observation precision, measurements of the small daylight component are possible. These could give useful information about particles in the atmosphere and be valuable in studies of meteorology and air pollution.

Angel, J. R. P.↗

NASA NTRS2000

Beam scanning reflectarray antenna with circular polarization

A novel means of scanning a circularly polarized reflectarray antenna. The reflectarray is an array of metallic elements arranged on a surface designed to compensate for the various path lengths of the optical rays from an illuminating feed to the reflecting surface and then to the antenna aperture. With appropriate design, the phase in the aperture can be made to vary linearly in any desired direction and also to produce a radiated beam normal to the constant phase surface. In the case of circular polarization, this path length compensation can be accomplished by rotation of the individual elements.

Huang, John↗

NASA NTRS1980

Circular polarization from scattering by circumstellar grains

It is suggested that observations of circular polarization can be a valuable tool for the study of circumstellar nebulae. A simple model is presented to predict the percentage of circular polarization produced by scattering from the dust contained within such nebulae; it was found that a significant component of circular polarization can be produced in nebulae which have a net linear polarization. Possible observations of the red supergiants mu Cep and alpha Ori are given as examples.

Shafter, A.↗

NASA NTRS1971

Circular polarization of sunlight reflected by clouds.

Measurements of circular polarization of visible light from planets have recently been reported. It is pointed out that the values measured for the circular polarization for Jupiter and Venus are of the magnitude expected for sunlight reflected by a cloudy planetary atmosphere. The variations of the sense of the polarization with phase angle and with location on the planetary disk are also consistent with expectations for reflection by clouds.

Hansen, J. E.↗

DOE OSTI2023

Increased range and contrast in fog with circularly polarized imaging

Fogs, low lying clouds, and other highly scattering environments pose a challenge for many commercial and national security sensing systems. Current autonomous systems rely on optical sensors for navigation whose performance is degraded by highly scattering environments. In our previous simulation work, we have shown that polarized light can penetrate through a scattering environment such as fog. We have demonstrated that circularly polarized light maintains its initial polarization state better than linearly polarized light, even through large numbers of scattering events and thus ranges. This has recently been experimentally verified by other researchers. In this work, we present the design, construction, and testing of active polarization imagers at short-wave infrared and visible wavelengths. We explore multiple polarimetric configurations for the imagers, focusing on linear and circular polarization states. The polarized imagers were tested at the Sandia National Laboratories Fog Chamber under realistic fog conditions. Here, we show that active circular polarization imagers can increase range and contrast in fog better than linear polarization imagers. We show that when imaging typical road sign and safety retro-reflective films, circularly polarized imaging has enhanced contrast throughout most fog densities/ranges compared to linearly polarized imaging and can penetrate over 15 to 25 m into the fog beyond the range limit of linearly polarized imaging, with a strong dependence on the interaction of the polarization state with the target materials.

47 OTHER INSTRUMENTATION↗

NASA NTRS1986

A technique for an array to generate circular polarization with linearly polarized elements

A method is presented for generating circularly polarized radiation from an array composed of linearly polarized elements having unique angular and phase arrangements. With this technique the complexity, weight, and RF loss of the array feed can be significantly reduced, especially in a large array. This uniquely formed array has the capability of generating excellent circular polarization (CP) over a relatively wide frequency bandwidth. In addition, the array is capable of scanning its main beam in the principal planes to relatively wide angles from its broadside direction without serious degradation to its CP quality. Another feature of this uniquely arranged array is a reduction in the occurrence of mutual coupling.

Huang, J.↗

DOE OSTI2024

Self-Powered Circularly Polarized Light Detection Enabled by Chiral Two-Dimensional Perovskites with Mixed Chiral–Achiral Organic Cations

Direct detection of circularly polarized light (CPL) holds great promise for the development of various optical technologies. Chiral 2D organic–inorganic halide perovskites make it possible to fabricate CPL-sensitive photodetectors. However, selectively detecting left-handed circularly polarized (LCP) and right-handed circularly polarized (RCP) light remains a significant challenge. Herein, we demonstrate a greatly enhanced distinguishability of photodiode-type CPL photodetectors based on chiral 2D perovskites with mixed chiral aryl (R)-(+),(S)-(–)-α-methylbenzylammonium (R,S-MBA) and achiral alkyl n-butylammonium (nBA) cations. The (R,S-MBA 0.5 nBA 0.5 ) 2 PbI 4 perovskites exhibit a 10-fold increase in circular dichroism signals compared to (R,S-MBA) 2 PbI 4 perovskites. Here, the CPL photodetectors based on the mixed-cation perovskites exhibit self-powered capabilities with a specific detectivity of 2.45 × 10 12 Jones at a o V bias. Notably, these devices show high distinguishability (gres) factors of –0.58 and +0.54 based on (R,S-MBA 0.5 nBA 0.5 ) 2 PbI 4 perovskites, respectively, surpassing the performance of (R-MBA) 2 PbI 4 -based devices by over 3-fold and setting a record for CPL detectors based on chiral 2D n = 1 perovskites.

36 MATERIALS SCIENCE↗

NASA NTRS2022

All-Metal Dual Band Circular Polarized UHF Patch Antenna

An all-metal circularly polarized UHF antenna element is presented. The patch antenna gives a wideband impedance and axial ratio bandwidth of 24% over the 0.3-0.38 GHz frequency band with 90% efficiency. The main advantage is the use of a single feed point to generate circular polarization (CP). The antenna can be used to set up a dual-band (0.3-0.32 GHz and 0.36-0.38 GHz) communication link, with an axial ratio better than 3 dB and a realized CP gain better than 8 dBiC and 10 dBiC, respectively. The interaction between the cavity walls and the patch element, results in near-field coupling and improves the impedance bandwidth as well as the axial ratio bandwidth of the antenna. Being a high gain, high aperture efficiency, low profile, light weight, and single feed point radiating element, this single patch antenna is an excellent candidate for future antenna array.

Chahat, Nacer↗

NASA NTRS1997

High Performance Circularly Polarized Microstrip Antenna

A microstrip antenna for radiating circularly polarized electromagnetic waves comprising a cluster array of at least four microstrip radiator elements, each of which is provided with dual orthogonal coplanar feeds in phase quadrature relation achieved by connection to an asymmetric T-junction power divider impedance notched at resonance. The dual fed circularly polarized reference element is positioned with its axis at a 45 deg angle with respect to the unit cell axis. The other three dual fed elements in the unit cell are positioned and fed with a coplanar feed structure with sequential rotation and phasing to enhance the axial ratio and impedance matching performance over a wide bandwidth. The centers of the radiator elements are disposed at the corners of a square with each side of a length d in the range of 0.7 to 0.9 times the free space wavelength of the antenna radiation and the radiator elements reside in a square unit cell area of sides equal to 2d and thereby permit the array to be used as a phased array antenna for electronic scanning and is realizable in a high temperature superconducting thin film material for high efficiency.

Bondyopadhyay, Probir K.↗