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Climate-driven Chemistry and Aerosol Feedbacks in CMIP6 Earth System Models

Feedbacks play a fundamental role in determining the magnitude of the response of the climate system to external forcing, such as from anthropogenic emissions. The latest generation of Earth system models includes aerosol and chemistry components that interact with each other and with the biosphere. These interactions introduce a complex web of feedbacks that is important to understand and quantify. This paper addresses multiple pathways for aerosol and chemical feedbacks in Earth system models. These focus on changes in natural emissions (dust, sea salt, dimethyl sulfide, biogenic volatile organic compounds (BVOCs) and lightning) and changes in reaction rates for methane and ozone chemistry. The feedback terms are then given by the sensitivity of a pathway to climate change multiplied by the radiative effect of the change. We find that the overall climate feedback through chemistry and aerosols is negative in the sixth Coupled Model Intercomparison Project (CMIP6) Earth system models due to increased negative forcing from aerosols in a climate with warmer surface temperatures following a quadrupling of CO2 concentrations. This is principally due to increased emissions of sea salt and BVOCs which are sensitive to climate change and cause strong negative radiative forcings. Increased chemical loss of ozone and methane also contributes to a negative feedback. However, overall methane lifetime is expected to increase in a warmer climate due to increased BVOCs. Increased emissions of methane from wetlands would also offset some of the negative feedbacks. The CMIP6 experimental design did not allow the methane lifetime or methane emission changes to affect climate, so we found a robust negative contribution from interactive aerosols and chemistry to climate sensitivity in CMIP6 Earth system models.

Aerosol feedbacks↗

ISMIP6: Ice Sheet Model Intercomparison Project for CMIP6

ISMIP6 (Ice Sheet Model Intercomparison Project for CMIP6) targets the Cryosphere in a Changing Climate and the Future Sea Level Grand Challenges of the WCRP (World Climate Research Program). Primary goal is to provide future sea level contribution from the Greenland and Antarctic ice sheets, along with associated uncertainty. Secondary goal is to investigate feedback due to dynamic ice sheet models. Experiment design uses and augment the existing CMIP6 (Coupled Model Intercomparison Project Phase 6) DECK (Diagnosis, Evaluation, and Characterization of Klima) experiments. Additonal MIP (Model Intercomparison Project)- specific experiments will be designed for ISM (Ice Sheet Model). Effort builds on the Ice2sea, SeaRISE (Sea-level Response to Ice Sheet Evolution) and COMBINE (Comprehensive Modelling of the Earth System for Better Climate Prediction and Projection) efforts.

CMIP6↗

Evaluation of Clouds, Radiation, and Precipitation in CMIP6 Models Using Global Weather States Derived from ISCCP-H Cloud Property Data

A clustering methodology is applied to cloud optical depth cloud top pressure (TAU-PC) histograms from the new, 1-degree resolution, ISCCP-H dataset, to derive an updated global Weather State (WS) dataset. Then, PC-TAU histograms from current-climate CMIP6 model simulations are assigned to the ISCCP-H WSs along with their concurrent radiation and precipitation properties, to evaluate model cloud, radiation, and precipitation properties in the context of the Weather States. The new ISCCP-H analysis produces WSs that are very similar to those previously found in the lower resolution ISCCP-D dataset. The main difference lies in the splitting of the ISCCP-D thin stratocumulus WS between the ISCCP-H shallow cumulus and stratocumulus WSs, which results in the reduction by one of the total WS number. The evaluation of the CMIP6 models against the ISCCP-H Weather States, shows that, in the ensemble mean, the models are producing an adequate representation of the frequency and geographical distribution of the WSs, with measurable improvements compared to the WSs derived for the CMIP5 ensemble. However, the frequency of shallow cumulus clouds continues to be underestimated, and, in some WSs the good agreement of the ensemble mean with observations comes from averaging models that significantly overpredict and underpredict the ISCCP-H WS frequency. In addition, significant biases exist in the internal cloud properties of the model WSs, such as the model underestimation of cloud fraction in middle-top clouds and secondarily in midlatitude storm and stratocumulus clouds, that result in an underestimation of cloud SW cooling in those regimes.

Clouds↗

Harmonization of global land use change and management for the period 850–2100 (LUH2) for CMIP6

Human land use activities have resulted in large changes to the biogeochemical and biophysical properties of the Earth's surface, with consequences for climate and other ecosystem services. In the future, land use activities are likely to expand and/or intensify further to meet growing demands for food, fiber, and energy. As part of the World Climate Research Program Coupled Model Intercomparison Project (CMIP6), the international community has developed the next generation of advanced Earth system models (ESMs) to estimate the combined effects of human activities (e.g., land use and fossil fuel emissions) on the carbon–climate system. A new set of historical data based on the History of the Global Environment database (HYDE), and multiple alternative scenarios of the future (2015–2100) from Integrated Assessment Model (IAM) teams, is required as input for these models. With most ESM simulations for CMIP6 now completed, it is important to document the land use patterns used by those simulations. Here we present results from the Land-Use Harmonization 2 (LUH2) project, which smoothly connects updated historical reconstructions of land use with eight new future projections in the format required for ESMs. The harmonization strategy estimates the fractional land use patterns, underlying land use transitions, key agricultural management information, and resulting secondary lands annually, while minimizing the differences between the end of the historical reconstruction and IAM initial conditions and preserving changes depicted by the IAMs in the future. The new approach builds on a similar effort from CMIP5 and is now provided at higher resolution (0.25°×0.25°) over a longer time domain (850–2100, with extensions to 2300) with more detail (including multiple crop and pasture types and associated management practices) using more input datasets (including Landsat remote sensing data) and updated algorithms (wood harvest and shifting cultivation); it is assessed via a new diagnostic package. The new LUH2 products contain > 50 times the information content of the datasets used in CMIP5 and are designed to enable new and improved estimates of the combined effects of land use on the global carbon–climate system.

land use land cover change↗

Climate model projections from the Scenario Model Intercomparison Project (ScenarioMIP) of CMIP6

The Scenario Model Intercomparison Project (ScenarioMIP) defines and coordinates the main set of future climate projections, based on concentration-driven simulations, within the Coupled Model Intercomparison Project phase 6 (CMIP6). This paper presents a range of its outcomes by synthesizing results from the participating global coupled Earth system models. We limit our scope to the analysis of strictly geophysical outcomes: mainly global averages and spatial patterns of change for surface air temperature and precipitation. We also compare CMIP6 projections to CMIP5 results, especially for those scenarios that were designed to provide continuity across the CMIP phases, at the same time highlighting important differences in forcing composition, as well as in results. The range of future temperature and precipitation changes by the end of the century (2081–2100) encompassing the Tier 1 experiments based on the Shared Socioeconomic Pathway (SSP) scenarios (SSP1-2.6, SSP2-4.5, SSP3-7.0 and SSP5-8.5) and SSP1-1.9 spans a larger range of outcomes compared to CMIP5, due to higher warming (by close to 1.5 °C) reached at the upper end of the 5 %–95 % envelope of the highest scenario (SSP5-8.5). This is due to both the wider range of radiative forcing that the new scenarios cover and the higher climate sensitivities in some of the new models compared to their CMIP5 predecessors. Spatial patterns of change for temperature and precipitation averaged over models and scenarios have familiar features, and an analysis of their variations confirms model structural differences to be the dominant source of uncertainty. Models also differ with respect to the size and evolution of internal variability as measured by individual models' initial condition ensemble spreads, according to a set of initial condition ensemble simulations available under SSP3-7.0. These experiments suggest a tendency for internal variability to decrease along the course of the century in this scenario, a result that will benefit from further analysis over a larger set of models. Benefits of mitigation, all else being equal in terms of societal drivers, appear clearly when comparing scenarios developed under the same SSP but to which different degrees of mitigation have been applied. It is also found that a mild overshoot in temperature of a few decades around mid-century, as represented in SSP5-3.4OS, does not affect the end outcome of temperature and precipitation changes by 2100, which return to the same levels as those reached by the gradually increasing SSP4-3.4 (not erasing the possibility, however, that other aspects of the system may not be as easily reversible). Central estimates of the time at which the ensemble means of the different scenarios reach a given warming level might be biased by the inclusion of models that have shown faster warming in the historical period than the observed. Those estimates show all scenarios reaching 1.5 °C of warming compared to the 1850–1900 baseline in the second half of the current decade, with the time span between slow and fast warming covering between 20 and 27 years from present. The warming level of 2 °C of warming is reached as early as 2039 by the ensemble mean under SSP5-8.5 but as late as the mid-2060s under SSP1-2.6. The highest warming level considered (5 °C) is reached by the ensemble mean only under SSP5-8.5 and not until the mid-2090s.d-2090s.

Scenario Model Intercomparison Project (ScenarioMI↗

The Brewer–Dobson Circulation in CMIP6

The Brewer–Dobson circulation (BDC) is a key feature of the stratosphere that models need to accurately represent in order to simulate surface climate variability and change adequately. For the first time, the Climate Model Intercomparison Project includes in its phase 6 (CMIP6) a set of diagnostics that allow for careful evaluation of the BDC. Here, the BDC is evaluated against observations and reanalyses using historical simulations. CMIP6 results confirm the well-known inconsistency in the sign of BDC trends between observations and models in the middle and upper stratosphere. Nevertheless, the large uncertainty in the observational trend estimates opens the door to compatibility. In particular, when accounting for the limited sampling of the observations, model and observational trend error bars overlap in 40 % of the simulations with available output. The increasing CO2 simulations feature an acceleration of the BDC but reveal a large spread in the middle-to-upper stratospheric trends, possibly related to the parameterized gravity wave forcing. The very close connection between the shallow branch of the residual circulation and surface temperature is highlighted, which is absent in the deep branch. The trends in mean age of air are shown to be more robust throughout the stratosphere than those in the residual circulation.

Brewer–Dobson circulation↗

Comment on “Advanced Testing of Low, Medium, and High ECS CMIP6 GCM Simulations Versus ERA5-T2m” by N. Scafetta (2022)

Scafetta (2022, https://doi.org/10.1029/2022gl097716) purports to test Coupled Model Intercomparison Project Phase 6 (CMIP6) climate models through a comparison of temperature changes over three decades. Unfortunately, the paper contains numerous conceptual and statistical errors that undermine all of the conclusions. First, no uncertainty is given for the observational temperature difference, making it impossible to assess compatibility with any model result. Second, the CMIP6 data are the ensemble means for each model, but the metric being tested is sensitive to the internal variability and so the full ensemble for each model must be used. When this is corrected, the conclusion that “all models with ECS > 3.0°C overestimate the observed global surface warming” is not sustained. Third, the statistical test in Section 2 would reject all models even in a perfect model setup given sufficient ensemble members, thus the second conclusion “that spatial t-statistics rejects the data-model agreement” is also not sustainable.

CMIP6↗

Evaluation of CMIP6 Model Simulations of PM 2.5 and its Components Over China

Earth system models (ESMs) participating in the latest Coupled Model Intercomparison Project Phase 6 (CMIP6) simulate various components of fine particulate matter (PM 2.5 ) as major climate forcers. Yet the model performance for PM 2.5 components remains little evaluated due in part to a lack of observational data. Here, we evaluate near-surface concentrations of PM 2.5 and its five main components over China as simulated by 14 CMIP6 models, including organic carbon (OC; available in 14 models), black carbon (BC; 14 models), sulfate (14 models), nitrate (4 models), and ammonium (5 models). For this purpose, we collect observational data between 2000 and 2014 from a satellite-based dataset for total PM2.5 and from 2469 measurement records in the literature for PM 2.5 components. Seven models output total PM 2.5 concentrations, and they all underestimate the observed total PM 2.5 over eastern China, with GFDL-ESM4 (−1.5 %) and MPI-ESM-1-2-HAM (−1.1 %) exhibiting the smallest biases averaged over the whole country. The other seven models, for which we recalculate total PM 2.5 from the available component output, underestimate the total PM 2.5 concentrations partly because of the missing model representations of nitrate and ammonium. Concentrations of the five individual components are underestimated in almost all models, except that sulfate is overestimated in MPI-ESM-1-2-HAM by 12.6 % and in MRI-ESM2-0 by 24.5 %. The underestimation is the largest for OC (by −71.2 % to −37.8 % across the 14 models) and the smallest for BC (−47.9 % to −12.1 %). The multi-model mean (MMM) reproduces the observed spatial pattern for OC (R = 0.51), sulfate (R = 0.57), nitrate (R = 0.70) and ammonium (R = 0.74) fairly well, yet the agreement is poorer for BC (R = 0.39). The varying performances of ESMs on total PM 2.5 and its components have important implications for the modeled magnitude and spatial pattern of aerosol radiative forcing.

CMIP6↗

Biogeochemical Protocols and Diagnostics for the CMIP6 Ocean Model Intercomparison Project (OMIP)

The Ocean Model Intercomparison Project (OMIP) focuses on the physics and biogeochemistry of the ocean component of Earth system models participating in the sixth phase of the Coupled Model Intercomparison Project (CMIP6). OMIP aims to provide standard protocols and diagnostics for ocean models, while offering a forum to promote their common assessment and improvement. It also offers to compare solutions of the same ocean models when forced with reanalysis data (OMIP simulations) vs. when integrated within fully coupled Earth system models (CMIP6). Here we detail simulation protocols and diagnostics for OMIP's biogeochemical and inert chemical tracers. These passive-tracer simulations will be coupled to ocean circulation models, initialized with observational data or output from a model spin-up, and forced by repeating the 1948-2009 surface fluxes of heat, fresh water, and momentum. These so-called OMIP-BGC simulations include three inert chemical tracers (CFC-11, CFC-12, SF [subscript] 6) and biogeochemical tracers (e.g., dissolved inorganic carbon, carbon isotopes, alkalinity, nutrients, and oxygen). Modelers will use their preferred prognostic BGC model but should follow common guidelines for gas exchange and carbonate chemistry. Simulations include both natural and total carbon tracers. The required forced simulation (omip1) will be initialized with gridded observational climatologies. An optional forced simulation (omip1-spunup) will be initialized instead with BGC fields from a long model spin-up, preferably for 2000 years or more, and forced by repeating the same 62-year meteorological forcing. That optional run will also include abiotic tracers of total dissolved inorganic carbon and radiocarbon, CTabio and 14CTabio, to assess deep-ocean ventilation and distinguish the role of physics vs. biology. These simulations will be forced by observed atmospheric histories of the three inert gases and CO2 as well as carbon isotope ratios of CO2. OMIP-BGC simulation protocols are founded on those from previous phases of the Ocean Carbon-Cycle Model Intercomparison Project. They have been merged and updated to reflect improvements concerning gas exchange, carbonate chemistry, and new data for initial conditions and atmospheric gas histories. Code is provided to facilitate their implementation.

Carbon↗

The Surface Albedo of Sea Ice in CMIP6 and the Implications for the Surface Albedo Feedback

The Arctic has experienced rapid sea ice loss and a substantial decline in surface albedo, significantly impacting its radiation budget. Climate models from the Coupled Model Intercomparison Project (CMIP6) reproduce these changes. However, inconsistencies remain among models regarding the magnitude, spatial distribution, and seasonal patterns of Arctic surface albedo evolution. This study investigates these discrepancies by comparing model outputs with observation from the Clouds and the Earth's Radiant Energy System (CERES). We develop a decomposition method to assess the contributions of sea ice albedo, sea ice concentration, and sea ice extent to Arctic surface albedo. Over land, differences in snow cover account for the substantial inter-model spread in surface albedo, while over the ocean, sea ice albedo, concentration, and extent all contribute. Comparisons between CMIP6 and the Atmospheric Model Intercomparison Project (AMIP) simulations, which use identically prescribed sea ice concentrations, reveals considerable inter-model spread in Arctic Ocean surface albedo due to differences in sea ice albedo. Applying the decomposition method to projections shows that models predicting larger decreases in sea ice concentration and extent, especially in the Central Arctic, exhibit lower surface albedo and stronger sea ice albedo feedback. Beyond 2050, Arctic Ocean surface albedo decline is mainly influenced by sea ice extent indicating that the retreat of the ice edge is the most important process to constrain the surface albedo feedback. This study provides insights into factors contributing to the spread and changes in Arctic surface albedo and the associated sea ice albedo feedback.

Patrick C Taylor↗

Historical (1850‐2014) Aerosol Evolution and Role on Climate Forcing Using the GISS Modele2.1 Contribution to CMIP6

The Earth’s climate is rapidly changing. Over the past centuries, aerosols, via their ability to absorb or scatter solar radiation and alter clouds, played an important role in counterbalancing some of the greenhouse gas (GHG) caused global warming. The multi-century anthropogenic aerosol cooling effect prevented present-day climate from reaching even higher surface air temperatures and subsequent more dramatic climate impacts. Trends in aerosol concentrations and optical depth show that in many polluted regions such as Europe and the United States of America, aerosol precursor emissions decreased back to levels of the 1950s. More recent polluting countries such as China may have reached a turning point in recent years as well, while India still follows an upward trend. Here we study aerosol trends in the CMIP6 simulations of the GISS ModelE2.1 climate model using a fully coupled atmosphere composition onfiguration, including interactive gas-phase chemistry, and either an aerosol microphysical (MATRIX) or a mass-based (OMA) aerosol module. Results show that whether global aerosol radiative forcing is already declining depends on the aerosol scheme used. Using the aerosol microphysical scheme, where the aerosol system reacts more strongly to the trend in sulfur dioxide (SO2) emissions, global peak direct aerosol forcing was reached in the 1980’s, whereas the mass-based scheme simulates peak direct aerosol forcing around 2010.

Aerosol forcing↗

Fast Responses on Pre-Industrial Climate from Present-Day Aerosols in A CMIP6 Multi-Model Study

In this work, we use Coupled Model Intercomparison Project Phase 6 (CMIP6) simulations from 10 Earth system models (ESMs) and general circulation models (GCMs) to study the fast climate responses on pre-industrial climate, due to present-day aerosols. All models carried out two sets of simulations: a control experiment with all forcings set to the year 1850 and a perturbation experiment with all forcings identical to the control, except for aerosols with precursor emissions set to the year 2014. In response to the pattern of all aerosols effective radiative forcing (ERF), the fast temperature responses are characterized by cooling over the continental areas, especially in the Northern Hemisphere, with the largest cooling over East Asia and India, sulfate being the dominant aerosol surface temperature driver for present-day emissions. In the Arctic there is a warming signal for winter in the ensemble mean of fast temperature responses, but the model-to-model variability is large, and it is presumably linked to aerosol-induced circulation changes. The largest fast precipitation responses are seen in the tropical belt regions, generally characterized by a reduction over continental regions and presumably a southward shift of the tropical rain belt. This is a characteristic and robust feature among most models in this study, associated with weakening of the monsoon systems around the globe (Asia, Africa and America) in response to hemispherically asymmetric cooling from a Northern Hemisphere aerosol perturbation, forcing possibly the Intertropical Convergence Zone (ITCZ) and tropical precipitation to shift away from the cooled hemisphere despite that aerosols' effects on temperature and precipitation are only partly realized in these simulations as the sea surface temperatures are kept fixed. An interesting feature in aerosol-induced circulation changes is a characteristic dipole pattern with intensification of the Icelandic Low and an anticyclonic anomaly over southeastern Europe, inducing warm air advection towards the northern polar latitudes in winter.

Pre-industrial climate↗

Tracking Improvement in Simulated Marine Biogeochemistry Between CMIP5 and CMIP6

Purpose of Review The changes or updates in ocean biogeochemistry component have been mapped between CMIP5 and CMIP6 model versions, and an assessment made of how far these have led to improvements in the simulated mean state of marine biogeochemical models within the current generation of Earth system models (ESMs). Recent Findings The representation of marine biogeochemistry has progressed within the current generation of Earth system models. However, it remains difficult to identify which model updates are responsible for a given improvement. In addition, the full potential of marine biogeochemistry in terms of Earth system interactions and climate feedback remains poorly examined in the current generation of Earth system models. Summary Increasing availability of ocean biogeochemical data, as well as an improved understanding of the underlying processes, allows advances in the marine biogeochemical components of the current generation of ESMs. The present study scrutinizes the extent to which marine biogeochemistry components of ESMs have progressed between the 5th and the 6th phases of the Coupled Model Intercomparison Project (CMIP).

Marine Biogeochemistry↗

CMIP6 Historical Simulations (1850‐2014) with GISS‐E2.1

Simulations of the CMIP6 historical period 1850‐‐2014, characterized by the emergence of anthropogenic climate drivers like greenhouse gases, are presented for different configurations of the NASA Goddard Institute for Space Studies (GISS) Earth System ModelE2.1. The GISS‐E2.1 ensembles are more sensitive to forcing than their CMIP5 predecessors (GISS‐E2), but warm less during recent decades due to reduced total forcing. This forcing reduction is attributed to an increase in longwave opacity in pre‐industrial simulations, resulting in an atmosphere less sensitive to further increases in opacity that result from rising greenhouse gas concentrations. This demonstrates the importance of the base climatology to forcing and forced climate trends. Most model versions match observed temperature trends since 1979 from the ocean to the stratosphere. The choice of ocean model is important to the transient climate response, as found in CMIP5 GISS‐E2: the model that more efficiently exports heat to the deep ocean shows a smaller rise in tropospheric temperature. Model sea level rise over the historical period is traced to excessive drawdown of aquifers to meet irrigation demand with a smaller contribution from thermal expansion. This shows how fully coupled models can provide indirect observational constraints upon forcing, in this case, constraining irrigation rates with observed sea level changes. The overall agreement of GISS‐E2.1 with observed trends is familiar from evaluation of its predecessors, as is the conclusion that these trends are almost entirely anthropogenic in origin.

NASA Goddard Institute for Space Studies (GISS) Ea↗

Drivers of Air-Sea CO2 Flux Seasonality and its Long-Term Changes in the NASA-GISS Model CMIP6 Submission.

Climate change will affect both the mean state and seasonality of marine physical and biogeochemical properties, with important implications for the oceanic sink of atmospheric CO2. Here, we investigate the seasonal cycle of the air-sea exchange of CO2 and pCO2,sw (surface seawater pCO2) and their long term changes using the CMIP6 submission of the NASA-GISS modelE (GISS-E2.1-G). In comparison to the CMIP5 submission (GISS-E2-R), we find that on the global scale, the seasonal cycles of the CO2 flux and NPP have improved, while the seasonal cycles of DIC, alkalinity, and macronutrients have deteriorated. Moreover, for all ocean biogeochemietry fields, changes in skill between E2.1-G and E2-R display large regional variability. For E2.1-G, we find similar modeled and observed CO2 flux seasonal cycles in the subtropical gyres, where seasonal anomalies of pCO2,sw and the flux are temperature-driven, and the Southern Ocean, where anomalies are DIC-driven. Biases in these seasonal cycles are largest in the subpolar and equatorial regions, driven by a combination of biases in temperature, DIC, alkalinity, and wind speed. When comparing the historical simulation to a simulation with an idealized increase in atmospheric pCO2, we find that the seasonal amplitudes of the CO2 flux and pCO2,sw generally increase. These changes are produced by increases in the sensitivity of pCO2,sw to its respective drivers. These findings are consistent with the notion that the sensitivity of pCO2,sw is expected to increase due to the increase of atmospheric pCO2, with changes in the seasonality of temperature, DIC, and alkalinity having secondary influences.

Air-Sea CO2↗

Bias in CMIP6 Models as Compared to Observed Regional Dimming and Brightening

Anthropogenic aerosol emissions have increased considerably over the last century, but climate effects and quantification of the emissions are highly uncertain as one goes back in time. This uncertainty is partly due to a lack of observations in the pre-satellite era, making the observations we do have before 1990 additionally valuable. Aerosols suspended in the atmosphere scatter and absorb incoming solar radiation and thereby alter the Earth's surface energy balance. Previous studies show that Earth system models (ESMs) do not adequately represent surface energy fluxes over the historical era. We investigated global and regional aerosol effects over the time period 1961–2014 by looking at surface downwelling shortwave radiation (SDSR). We used observations from ground stations as well as multiple experiments from eight ESMs participating in the Coupled Model Intercomparison Project Version 6 (CMIP6). Our results show that this subset of models reproduces the observed transient SDSR well in Europe but poorly in China. We suggest that this may be attributed to missing emissions of sulfur dioxide in China, sulfur dioxide being a precursor to sulfate, which is a highly reflective aerosol and responsible for more reflective clouds. The emissions of sulfur dioxide used in the models do not show a temporal pattern that could explain observed SDSR evolution over China. The results from various aerosol emission perturbation experiments from DAMIP, RFMIP and AerChemMIP show that only simulations containing anthropogenic aerosol emissions show dimming, even if the dimming is underestimated. Simulated clear-sky and all-sky SDSR do not differ greatly, suggesting that cloud cover changes are not a dominant cause of the biased SDSR evolution in the simulations. Therefore we suggest that the discrepancy between modeled and observed SDSR evolution is partly caused by erroneous aerosol and aerosol precursor emission inventories. This is an important finding as it may help interpret whether ESMs reproduce the historical climate evolution for the right or wrong reason.

surface downwelling shortwave radiation (SDSR)↗

Climate Change Penalty and Benefit on Surface Ozone: A Global Perspective Based on CMIP6 Earth System Models

This work presents an analysis of the effect of climate change on surface ozone discussing the related penalties and benefits around the globe from the global modelling perspective based on simulations with five CMIP6 (Coupled Model Intercomparison Project Phase 6) Earth System Models. As part of AerChemMIP (Aerosol Chemistry Model Intercomparison Project) all models conducted simulation experiments considering future climate (ssp370SST) and present-day climate (ssp370pdSST) under the same future emissions trajectory (SSP3-7.0). A multi-model global average climate change benefit on surface ozone of −0.96 ± 0.07 ppbv °C−1 is calculated which is mainly linked to the dominating role of enhanced ozone destruction with higher water vapour abundances under a warmer climate. Over regions remote from pollution sources, there is a robust decline in mean surface ozone concentration on an annual basis as well as for boreal winter and summer varying spatially from −0.2 to −2 ppbv °C−1, with strongest decline over tropical oceanic regions. The implication is that over regions remote from pollution sources (except over the Arctic) there is a consistent climate change benefit for baseline ozone due to global warming. However, ozone increases over regions close to anthropogenic pollution sources or close to enhanced natural biogenic volatile organic compounds emission sources with a rate ranging regionally from 0.2 to 2 ppbv C−1, implying a regional surface ozone penalty due to global warming. Overall, the future climate change enhances the efficiency of precursor emissions to generate surface ozone in polluted regions and thus the magnitude of this effect depends on the regional emission changes considered in this study within the SSP3_7.0 scenario. The comparison of the climate change impact effect on surface ozone versus the combined effect of climate and emission changes indicates the dominant role of precursor emission changes in projecting surface ozone concentrations under future climate change scenarios.

surface ozone↗

Upper Arctic Ocean Properties and Relationships with Sea Ice in CMIP6 Historical Simulations

While current-generation CMIP and OMIP models have clear biases in their upper Arctic Ocean hydrography, it is less clear how these biases impact the models' ability to simulate the observed Arctic sea ice mean state and trends. In this study we seek to quantify cross-relationship between sea ice and ocean states in CMIP6 historical simulations and identify common model behaviors. Multi-model mean (MMM) simulations exhibit accelerated changes in the ice and ocean system since the late 20th century. Underlying the MMM is strong inter-model variation in the simulated ice and ocean mean states and their temporal variability including trends. Despite such inter-model differences, all models show a similar ratio between sea ice reduction and upper ocean warming such that models with higher ocean warming also have higher SIE reduction and vice versa. Our results also highlight the urgent needs of reliable Arctic Ocean observations or data products in order to better contextualize modeling results.

Upper Arctic Ocean↗