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At least 37 records · Page 2

Longwave Radiative Forcing of Saharan Dust Aerosols Estimated from MODIS, MISR and CERES Observations on Terra

Using observations from the Multi-angle Imaging Spectroradiometer (MISR), the Moderate Resolution Imaging Spectroradiometer (MODIS), and the Clouds and the Earth's Radiant Energy System (CERES) instruments onboard the Terra satellite; we present a new technique for studying longwave (LW) radiative forcing of dust aerosols over the Saharan desert for cloud-free conditions. The monthly-mean LW forcing for September 2000 is 7 W/sq m and the LW forcing efficiency' (LW(sub eff)) is 15 W/sq m. Using radiative transfer calculations, we also show that the vertical distribution of aerosols and water vapor are critical to the understanding of dust aerosol forcing. Using well calibrated, spatially and temporally collocated data sets, we have combined the strengths of three sensors from the same satellite to quantify the LW radiative forcing, and show that dust aerosols have a "warming" effect over the Saharan desert that will counteract the shortwave "cooling effect" of aerosols.

Zhang, Jiang-Long↗

Intensification of North American Megadroughts through Surface and Dust Aerosol Forcing

Tree-ring-based reconstructions of the Palmer drought severity index (PDSI) indicate that, during the Medieval Climate Anomaly (MCA), the central plains of North America experienced recurrent periods of drought spanning decades or longer. These megadroughts had exceptional persistence compared to more recent events, but the causes remain uncertain. The authors conducted a suite of general circulation model experiments to test the impact of sea surface temperature (SST) and land surface forcing on the MCA megadroughts over the central plains. The land surface forcing is represented as a set of dune mobilization boundary conditions, derived from available geomorphological evidence and modeled as increased bare soil area and a dust aerosol source (32deg-44degN, 105deg-95degW). In the experiments, cold tropical Pacific SST forcing suppresses precipitation over the central plains but cannot reproduce the overall drying or persistence seen in the PDSI reconstruction. Droughts in the scenario with dust aerosols, however, are amplified and have significantly longer persistence than in other model experiments, more closely matching the reconstructed PDSI. This additional drying occurs because the dust increases the shortwave planetary albedo, reducing energy inputs to the surface and boundary layer. The energy deficit increases atmospheric stability, inhibiting convection and reducing cloud cover and precipitation over the central plains. Results from this study provide the first model-based evidence that dust aerosol forcing and land surface changes could have contributed to the intensity and persistence of the central plains megadroughts, although uncertainties remain in the formulation of the boundary conditions and the future importance of these feedbacks.

Earth surface↗

Satellite-Based Assessment of Possible Dust Aerosols Semi-Direct Effect on Cloud Water Path over East Asia

The semi-direct effects of dust aerosols are analyzed over eastern Asia using 2 years (June 2002 to June 2004) of data from the Clouds and the Earth s Radiant Energy System (CERES) scanning radiometer and MODerate Resolution Imaging Spectroradiometer (MODIS) on the Aqua satellite, and 18 years (1984 to 2001) of International Satellite Cloud Climatology Project (ISCCP) data. The results show that the water path of dust-contaminated clouds is considerably smaller than that of dust-free clouds. The mean ice water path (IWP) and liquid water path (LWP) of dusty clouds are less than their dust-free counterparts by 23.7% and 49.8%, respectively. The long-term statistical relationship derived from ISCCP also confirms that there is significant negative correlation between dust storm index and ISCCP cloud water path. These results suggest that dust aerosols warm clouds, increase the evaporation of cloud droplets and further reduce cloud water path, the so-called semi-direct effect. The semi-direct effect may play a role in cloud development over arid and semi-arid areas of East Asia and contribute to the reduction of precipitation.

Huang, Jianping↗

African Dust Aerosols as Atmospheric Ice Nuclei

Measurements of the ice nucleating ability of aerosol particles in air masses over Florida having sources from North Africa support the potential importance of dust aerosols for indirectly affecting cloud properties and climate. The concentrations of ice nuclei within dust layers at particle sizes below 1 pn exceeded 1/cu cm; the highest ever reported with our device at temperatures warmer than homogeneous freezing conditions. These measurements add to previous direct and indirect evidence of the ice nucleation efficiency of desert dust aerosols, but also confirm their contribution to ice nuclei populations at great distances from source regions.

DeMott, Paul J.↗

A Comparison of Seasonal and Interannual Variability of Soil Dust Aerosols Over the Atlantic Ocean as Inferred by the Toms AI and AVHRR AOT Retrievals

The seasonal cycle and interannual variability of two estimates of soil (or 'mineral') dust aerosols are compared: Advanced Very High Resolution Radiometer (AVHRR) aerosol optical thickness (AOT) and Total Ozone Mapping Spectrometer (TOMS) aerosol index (AI), Both data sets, comprising more than a decade of global, daily images, are commonly used to evaluate aerosol transport models. The present comparison is based upon monthly averages, constructed from daily images of each data set for the period between 1984 and 1990, a period that excludes contamination from volcanic eruptions. The comparison focuses upon the Northern Hemisphere subtropical Atlantic Ocean, where soil dust aerosols make the largest contribution to the aerosol load, and are assumed to dominate the variability of each data set. While each retrieval is sensitive to a different aerosol radiative property - absorption for the TOMS AI versus reflectance for the AVHRR AOT - the seasonal cycles of dust loading implied by each retrieval are consistent, if seasonal variations in the height of the aerosol layer are taken into account when interpreting the TOMS AI. On interannual time scales, the correlation is low at most locations. It is suggested that the poor interannual correlation is at least partly a consequence of data availability. When the monthly averages are constructed using only days common to both data sets, the correlation is substantially increased: this consistency suggests that both TOMS and AVHRR accurately measure the aerosol load in any given scene. However, the two retrievals have only a few days in common per month so that these restricted monthly averages have a large uncertainty. Calculations suggest that at least 7 to 10 daily images are needed to estimate reliably the average dust load during any particular month, a threshold that is rarely satisfied by the AVHRR AOT due to the presence of clouds in the domain. By rebinning each data set onto a coarser grid, the availability of the AVHRR AOT is increased during any particular month, along with its interannual correlation with the TOMS AI The latter easily exceeds the sampling threshold due to its greater ability to infer the aerosol load in the presence of clouds. Whether the TOMS AI should be regarded as a more reliable indicator of interannual variability depends upon the extent of contamination by sub-pixel clouds.

Cakmur, R. V.↗

Dust Aerosol Retrieval Over the Oceans With the MODIS/VIIRS Dark‐Target Algorithm: 1. Dust Detection

To prepare for implementation of a new aerosol retrieval specifically designed for dust aerosol over ocean in the operational Dark-Target (DT) algorithms for the Moderate-resolution Imaging Spectrometer (MODIS) and Visible Infrared Imaging Radiometer Suite (VIIRS) satellite sensors, we focus on the challenge of detecting dust. We first survey the literature on existing dust detection algorithms and then develop an innovative algorithm that combines near-UV (deep blue), visible, and thermal infrared (TIR) wavelength spectral tests. The new detection algorithm is applied to Terra and Aqua MODIS granules and compared with other dust detection possibilities from existing MODIS products. Quantitative evaluation of the new dust detection algorithm is conducted using both a collocated AERONET-MODIS data set and collocated Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO)-MODIS data set. From comparison with both AERONET and CALIOP measurements, we estimate the new dust detection algorithm detects about 30% of weakly dusty pixels and more than 80% of heavily dusty pixels, with false detections in the range of 1–2%. The very low false detection rate is particularly noteworthy in comparison with existing literature. Compared with the dust flag currently available as part of the MODIS cloud mask product (MOD35/MYD35), and dust classification based on commonly used thresholds with aerosol optical depth (AOD) and Angstrom exponent (AE), the new dust detection algorithm finds more dusty pixels and fewer false detections.

spectral dust detection↗

Evaluation of the MODIS Retrievals of Dust Aerosol over the Ocean during PRIDE

The Puerto Rico Dust Experiment (PRIDE) took place in Roosevelt Roads, Puerto Rico from June 26 to July 24,2000 to study the radiative and physical properties of African dust aerosol transported into the region. PRIDE had the unique distinction of being the first major field experiment to allow direct comparison of aerosol retrievals from the MODerate Imaging Spectro-radiometer (MODIS) with sunphotometer and in-situ aerosol measurements. Over the ocean, the MODIS algorithm retrieves aerosol optical depth (AOD) as well as information about the aerosols size distribution. During PRIDE, MODIS derived AODs in the red wavelengths (0.66 micrometers) compare closely with AODs measured from sunphotometers, but, are too large at blue and green wavelengths (0.47 and 0.55 micrometers) and too small in the infrared (0.87 micrometers). This discrepancy of spectral slope results in particle size distributions retrieved by MODIS that are small compared to in-situ measurements, and smaller still when compared to sunphotometer sky radiance inversions. The differences in size distributions are, at least in part, associated with MODIS simplification of dust as spherical particles. Analysis of this PRIDE data set is a first step towards derivation of realistic non-spherical models for future MODIS retrievals.

Levy, Robert C.↗

Dust Aerosol Retrieval Over the Oceans With the MODIS/VIIRS Dark Target Algorithm: 2. Nonspherical Dust Model

The Dark‐target (DT) aerosol algorithm retrieves spectral Aerosol Optical Depth (AOD) and other aerosol properties from Moderate‐resolution Imaging Spectrometer (MODIS) reflectance observations. Over the ocean, the DT algorithm is known to contain scattering‐angle‐dependent biases in its retrievals of AOD, Angstrom Exponent (AE), and Fine Mode Fraction (FMF) for dust aerosols. Following a two‐step strategy to improve the DT retrieval of dust over ocean, for which the first step is to identify dusty pixels (reported in “Part 1”), in this “Part 2,” we report on construction of a new dust model lookup table (LUT) and the strategy for applying it within the existing DT algorithm. In particular, we evaluate different characterizations of dust optical properties from a variety of frameworks and databases, and compare them with the current DT retrieval assumptions. Substituting the standard operational LUT with a spheroid dust model with identified dusty pixels shows significant improvement when compared with collocated AERONET‐identified dusty pixels. Specifically, the application of the new dust model to dusty pixels reduces their AOD bias from 0.06 to 0.02 while improving the fraction of retrievals within expected error from 64% to 82%. At the same time, the overall bias in AE is reduced from 0.13 to 0.06, and the scattering‐angle‐dependent AE bias is largely eliminated. In testing on two full months of data (April and July), the new retrieval will reduce the monthly mean AOD by up to 0.1 and 0.2 in the north Atlantic and Arabian seas, respectively. The average AE and FMF are also reduced in these dust heavy regions

dust aerosol retrieval↗

Sources, Sinks, and Transatlantic Transport of North African Dust Aerosol: A Multimodel Analysis and Comparison With Remote Sensing Data

This study evaluates model-simulated dust aerosols over North Africa and the North Atlantic from five global models that participated in the Aerosol Comparison between Observations and Models phase II model experiments. The model results are compared with satellite aerosol optical depth (AOD) data from Moderate Resolution Imaging Spectroradiometer (MODIS), Multiangle Imaging Spectroradiometer (MISR), and Sea-viewing Wide Field-of-view Sensor, dust optical depth (DOD) derived from MODIS and MISR, AOD and coarse-mode AOD (as a proxy of DOD) from ground-based Aerosol Robotic Network Sun photometer measurements, and dust vertical distributions/centroid height from Cloud Aerosol Lidar with Orthogonal Polarization and Atmospheric Infrared Sounder satellite AOD retrievals. We examine the following quantities of AOD and DOD: (1) the magnitudes over land and over ocean in our study domain, (2) the longitudinal gradient from the dust source region over North Africa to the western North Atlantic, (3) seasonal variations at different locations, and (4) the dust vertical profile shape and the AOD centroid height (altitude above or below which half of the AOD is located). The different satellite data show consistent features in most of these aspects; however, the models display large diversity in all of them, with significant differences among the models and between models and observations. By examining dust emission, removal, and mass extinction efficiency in the five models, we also find remarkable differences among the models that all contribute to the discrepancies of model-simulated dust amount and distribution. This study highlights the challenges in simulating the dust physical and optical processes, even in the best known dust environment, and stresses the need for observable quantities to constrain the model processes.

Africa↗

Predicting the Mineral Composition of Dust Aerosols: Model Evaluation and Identification of Key Processes with Observations - Part 2

A global compilation of nearly sixty measurement studies is used to evaluate two methods of simulating the mineral composition of dust aerosols in an Earth system model. Both methods are based upon a Mean Mineralogical Table (MMT) that relates the soil mineral fractions to a global atlas of arid soil type. The Soil Mineral Fraction (SMF) method assumes that the aerosol mineral fractions match the fractions of the soil. The MMT is based upon soil measurements after wet sieving, a process that destroys aggregates of soil particles that would have been emitted from the original, undisturbed soil. The second method approximately reconstructs the emitted aggregates. This model is referred to as the Aerosol Mineral Fraction (AMF) method because the mineral fractions of the aerosols differ from those of the wet-sieved parent soil, partly due to reaggregation. The AMF method remedies some of the deficiencies of the SMF method in comparison to observations. Only the AMF method exhibits phyllosilicate mass at silt sizes, where they are abundant according to observations. In addition, the AMF quartz fraction of silt particles is in better agreement with measured values, in contrast to the overestimated SMF fraction. Measurements at distinct clay and silt particle sizes are shown to be more useful for evaluation of the models, in contrast to the sum over all particles sizes that is susceptible to compensating errors, as illustrated by the SMF experiment. Model errors suggest that allocation of the emitted silt fraction of each mineral into the corresponding transported size categories is an important remaining source of uncertainty. Evaluation of both models and the MMT is hindered by the limited number of size-resolved measurements of mineral content that sparsely sample aerosols from the major dust sources. The importance of climate processes dependent upon aerosol mineral composition shows the need for global and routine mineral measurements.

aerosols↗

Dust Aerosols at the Source Region During ACE-ASIA: A Surface/Satellite Perspective

ACE (Aerosol Characterization Experiment)-Asia is designed to study the compelling variability in spatial and temporal scale of both pollution-derived and naturally occurring aerosols, which often exist in high concentrations over eastern Asia and along the rim of the western Pacific. The phase-I of ACE-Asia was conducted from March-May 2001 in the vicinity of the Gobi desert, East Coast of China, Yellow Sea, Korea, and Japan, along the pathway of Kosa (severe events that blanket East Asia with yellow desert dust, peaked in the Spring season). Asian dust typically originates in desert areas far from polluted urban regions. During transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian dust is of special importance in regional-to-global climate issues such as radiative forcing, the hydrological cycle, and primary biological productivity in the mid-Pacific Ocean. During ACE-Asia we have measured continuously aerosol physical/optical/radiative properties, column precipitable water amount, and surface reflectivity over homogeneous areas from surface. The inclusion of flux measurements permits the determination of dust aerosol radiative flux in addition to measurements of loading and optical thickness. At the time of the Terra/MODIS, SeaWiFS, TOMS and other satellite overpasses, these ground-based observations can provide valuable data to compare with satellite retrievals over land. Preliminary results will be presented and discussed their implications in regional climatic effects.

Tsay, Si-Chee↗

Estimation of Asian Dust Aerosol Effect on Cloud Radiation Forcing Using Fu-Liou Radiative Model and CERES Measurements

The impact of Asian dust on cloud radiative forcing during 2003-2006 is studied by using the Earth's Radiant Energy Budget Scanner (CERES) data and the Fu-Liou radiative transfer model. Analysis of satellite data shows that the dust aerosol significantly reduced the cloud cooling effect at TOA. In dust contaminated cloudy regions, the 4-year mean values of the instantaneous shortwave, longwave and net cloud radiative forcing are -138.9, 69.1, and -69.7 Wm(sup -2), which are 57.0, 74.2, and 46.3%, respectively, of the corresponding values in more pristine cloudy regions. The satellite-retrieved cloud properties are significantly different in the dusty regions and can influence the radiative forcing indirectly. The contributions to the cloud radiation forcing by the dust direct, indirect and semi-direct effects are estimated using combined satellite observations and Fu-Liou model simulation. The 4-year mean value of combination of indirect and semi-direct shortwave radiative forcing (SWRF) is 82.2 Wm(sup -2), which is 78.4% of the total dust effect. The direct effect is only 22.7 Wm(sup -2), which is 21.6% of the total effect. Because both first and second indirect effects enhance cloud cooling, the aerosol-induced cloud warming is mainly the result of the semi-direct effect of dust.

Su, Jing↗

Dust aerosol retrieval results from MISR (multi-angle imaging spectro-radiometer)

Satellite measurements provide important tools for understanding the effect of mineral dust aerosols on past and present climate and climate predictions. Multi-angle instruments such as Multi-angle Imaging Spectro- Radiometer (MISR) provide independent constraints on aerosol properties based on their sensitivity to the shape of aerosol scattering phase functions. The current MISR operational retrieval algorithm (version 16 and higher) was modified by incorporating new non-spherical dust models that account for naturally occurring dust shapes and compositions. We present selected examples of MISR version 16 retrievals over AERONET sunphotometer land and ocean sites during the passage of dust fronts. Our analysis shows that during such events MISR retrieves Angstrom exponents characteristic of large particles, having little spectral variation in extinction over the MISR wavelength range (442, 550, 672 and 866 nm channels), as expected. The retrieved fraction of non-spherical particles is also very high. This quantity is not retrieved by satellite instruments having only nadir-viewing cameras. Our comparison of current (version 16) MISR-retrieved aerosol optical thickness (AOT) with AERONET instantaneous AOT shows better coverage and stronger correlations than when making identical comparisons with previous AOT retrievals (version 15). The MISR algorithm successful mixtures include a non-spherical dust component with high frequency in retrievals over dark water and slightly lower frequency over land. Selection frequencies of non-spherical dust models also decrease in dusty regions affected by pollution.

Multiangle Imaging Spectroradiometer (MISR)↗

Uptake of Nitrate and Sulfate on Dust Aerosols during TRACE-P

Aerosol data collected near Asia on the DC-8 aircraft platform during TRACE-P has been examined for evidence of uptake of NO3(-) and SO4(-) on dust surfaces. Data is compared between a sector where dust was predominant and a sector where dust was less of an influence. Coincident with dust were higher mixing ratios of anthropogenic pollutants. HNO3, SO2, and CO were higher in the dust sector than the nondust sector by factors of 2.7, 6.2, and 1.5, respectively. The colocation of dust and pollution sources allowed for the uptake of NO3(-) and nss-SO4(-) on the coarse dust aerosols, increasing the mixing ratios of these particulates by factors of 5.7 and 2.6 on average. There was sufficient nss-SO4(-) to take up all of the NH4(+) present, with enough excess nss-SO4(-) to also react with dust CaCO3. This suggests that the enhanced NO3(-) was not in fine mode NH4NO3. Particulate NO3(-) (p-NO3(-)) constituted 54% of the total NO3(-), (t-NO3(-)) on average, reaching a maximum of 72% in the dust sector. In the nondust sector, p-NO3(-) contributed 37% to t-NO3(-), likely due to the abundance of sea salts there. In two other sectors where the influence of dust and sea salt were minimal, p-NO3(-), accounted for < 15% of t-NO3(-).

Jordan, C. E.↗

Lidar Ratios for Dust Aerosols Derived From Retrievals of CALIPSO Visible Extinction Profiles Constrained by Optical Depths from MODIS-Aqua and CALIPSO/CloudSat Ocean Surface Reflectance Measurements

CALIPSO's (Cloud Aerosol Lidar Infrared Pathfinder Satellite Observations) analysis algorithms generally require the use of tabulated values of the lidar ratio in order to retrieve aerosol extinction and optical depth from measured profiles of attenuated backscatter. However, for any given time or location, the lidar ratio for a given aerosol type can differ from the tabulated value. To gain some insight as to the extent of the variability, we here calculate the lidar ratio for dust aerosols using aerosol optical depth constraints from two sources. Daytime measurements are constrained using Level 2, Collection 5, 550-nm aerosol optical depth measurements made over the ocean by the MODIS (Moderate Resolution Imaging Spectroradiometer) on board the Aqua satellite, which flies in formation with CALIPSO. We also retrieve lidar ratios from night-time profiles constrained by aerosol column optical depths obtained by analysis of CALIPSO and CloudSat backscatter signals from the ocean surface.

Young, Stuart A.↗

What we Hope to Learn about Global Mineral Dust Aerosols from EOS Multi-Angle Imaging SpectroRadiometer (MISR)

On global scales, just a few broad atmospheric aerosol compositional groups are commonly observed. Of these, "mineral dust" is the only group which both contains non-spherical particles, and typically has size distributions with enough large particles for particle shape to affect its visible-light-scattering properties. The MISR instrument is scheduled for launch into a 10:30 AM sun-synchronous, polar orbit aboard the EOS Terra satellite in 1999. MISR will measure the upwelling visible radiance from Earth in 4 spectral bands centered at 446, 558, 672, and 866 nm, at each of 9 emission angles spread out in the forward and aft directions along the flight path at +/-70.5 deg, +/-60.0 deg, +/-45.6 deg, +/-26.1deg, and nadir. Over a period of 7 minutes, as the spacecraft flies along, a 360 km wide swath of Earth will successively be viewed by each of the cameras, allowing MISR to sample a very large range of scattering angles; in mid latitudes, the instrument will observe scattering angles between about 60 deg and 160 deg. Global coverage will be acquired about once in 9 days at the equator; the nominal mission lifetime is 6 years. The distinction in single scattering phase function between natural distributions of spherical and randomly oriented, non-spherical particles, with a broad range of aspect ratios, shows up strongly for scattering angles ranging from about 90 deg to near 180 deg. For non-spherical particle distributions, single scattering phase functions tend to be much flatter in this region than for spherical particles. Since MISR samples the relevant range of scattering angles very well, we expect to be able to make critical distinctions between natural distributions of spherical and randomly oriented, non-spherical particles with MISR data. We anticipate that the new multiangle, multispectral data from MISR will also contain other information about particle properties, a major step beyond current spacecraft remote sensing retrievals, which obtain aerosol optical depth based on entirely assumed particle microphysical properties. According to simulations over cloud-free, calm ocean, for pure particles with natural ranges of optical depth, particle size, and indices of refraction, MISR should retrieve column optical depth for all but the darkest particles, to an uncertainty of at most 0.05 or 20%, whichever is larger, even if the particle properties are poorly known. For one common particle type, soot, constraints on the optical depth over dark ocean are very poor. The simulated measurements also should allow us to separate two to four compositional groups based on indices of refraction, and to identify three to four distinct size groups between 0.1 and 2.0 microns characteristic radius at most latitudes. The technique is most sensitive to particle microphysical properties in the "accumulation mode" sizes. where particle scattering undergoes the transition from Rayleigh to large-particle regimes for the MISR wavelengths. Based on these results, we expect to distinguish air masses containing different aerosol types, routinely and globally, with multiangle remote sensing data. Such data complements in situ and field data, which can provide details about aerosol size and composition locally that are needed to assess the radiative effects of aerosols quantitatively. Both field data and correlations in space and time with likely source and sink regions will also be helpful in developing a global picture of mineral dust aerosol budgets. Further work on the expected sensitivity of MISR to natural mixtures of pure particles, including climatologically likely mineral dust components, is currently underway.

Kahn, Ralph↗

Saharan Dust Aerosols Change Deep Convective Cloud Prevalence, Possibly by Inhibiting Marine New Particle Formation

Deep convective clouds (DCCs) are important to global climate, atmospheric chemistry, and precipitation. Dust, a dominant aerosol type over the tropical North Atlantic, has potentially large microphysical impacts on DCCs over this region. However, dust effects are difficult to identify, being confounded by co-varying meteorology and other factors. Here, a method is developed to quantify DCC responses to dust and other aerosols at large spatial and temporal scales despite these uncertainties. Over 7 million tropical North Atlantic cloud, aerosol, and meteorological profiles from CloudSat satellite data and MERRA-2 reanalysis products are used to stratify cloud observations into meteorological regimes, objectively select a priori assumptions, and iteratively test uncertainty sensitivity. Dust is robustly associated with a 54% increase in DCC prevalence. However, marine aerosol proxy concentrations are five times more predictive of dust-associated increases in DCC prevalence than the dust itself, or any other aerosol or meteorological factor. Marine aerosols are also the most predictive factor for the even larger increases in DCC prevalence (61-87%) associated with enhanced dimethyl sulfide and combustion and sulfate aerosols. Dust-associated increases in DCC prevalence are smaller at high dust concentrations than at low concentrations. These observations suggest that not only is dust a comparatively ineffective CCN source, but it may also act as a condensation/coagulation sink for chemical precursors to CCN, reducing total CCN availability over large spatial scales by inhibiting new particle formation from marine emissions. These observations represent the first time this rocess, previously predicted by models, is supported and quantified by measurements.

Aerosol-cloud interactions↗