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NASA NTRS1986

Analysis and interpretation of the shocklike electrostatic noise observed during the AMPTE solar wind lithium releases

During the AMPTE (Active Magnetospheric Particle Tracer Explorers) solar wind lithium release on September 11, and again on September 20, 1984, an intense burst of electrostatic noise was observed near the upstream edge of the ion cloud. Comparisons with measurements by the IMP-6 and ISEE-1 spacecraft show that the spectrum and overall features of this noise are very similar to electrostatic noise observed at the Earth's bow shock. A stability analysis using realistic parameters shows that the electrostatic noise can be accounted for by an ion beam-plasma instability caused by the solar wind proton beam streaming through the nearly stationary lithium cloud. The growth rate of this instability is largest when the ion density and solar wind proton density are similar, which explains why the noise only occurs near the outer edge of the ion cloud. The similarity to the noise in the Earth's bow shock suggest that a shock may exist in the solar wind plasma flow upstream of the ion cloud. If the noise is associated with a shock, then it must be an electrostatic shock, since the ion cyclotron radii are too small for the existence of a MHD shock. Since the electrostatic instability occurs at phase velocities near the lithium thermal velocity, the electrostatic turbulence may play a role in heating the lithium ions and transferring momentum from the solar wind to the ion cloud.

Gurnett, D. A.↗

NASA NTRS2006

Electrostatic Screen for Transport of Martian and Lunar Regolith

The Martian and Lunar Regolith contain fine particulate including those in the size range from 0.5 to 200 micron [1-2]. Martian dust can be transported and deposited by Aeolian processes, including "Dust Devils". Due to the ultra high vacuum (10e-12 Torr), transport of dust on the Moon is solely a result of collision/ballistic motion. Dust obscuration of solar cells is one of the primary factors limiting the duration of Martian missions, including the Mars Exploration Rovers. Dust contamination in vacuum seals is one of the primarily factors that limited lunar excursions during the Apollo missions. Controlled transportation of dust on Mars and the Moon is important for many reasons, including both contamination mitigation and in situ resource utilization (ISRU). Since both the monopole and dipole electrostatic moments result in non-trivial forces on particles in an electrostatic field, dust particles, whether charged or not, can be transported by electrostatic fields. In the electrostatic screen, alternating waveforms of voltage applied to patterned grids of electrodes will transport dust. The authors will show that the canonical methods for transporting dust via electrostatic screen can be readily applied to transport of Martian and Lunar regolith. Experiments have been performed in ambient, low humidity, Martian, and Lunar conditions. Screen parameters have been examined for application to each regolith, such as grid spacing, trace width, grid voltage, pulse pattern, pulse frequency, and coating type. The authors have also developed an electrostatic screen based on optically transparent conductors that can be placed over solar arrays, windows, visors, lenses, etc.

Immer, C.↗

DOE OSTI2020

Electrostatic Barriers to Nanoparticle Accessibility of a Porous Matrix

Translocation from one cavity to another through a narrow constriction (i.e., a “hole”) represents the fundamental elementary process underlying hindered mass transport of nanoparticles and macromolecules within many natural and synthetic porous materials, including intracellular environments. This process is complex and may be influenced by long-range (e.g., electrostatic) particle–wall interactions, transient adsorption/desorption, surface diffusion, and hydrodynamic effects. In this study, we used a three-dimensional (3D) tracking method to explicitly visualize the process of nanoparticle diffusion within periodic porous nanostructures, where electrostatic interactions were mediated via ionic strength. The effects of electrostatic interactions on nanoparticle transport were surprisingly large. For example, an increase in the Debye length of only a few nanometers (in a material with a hole diameter of ~100 nm) increased the mean cavity escape time 3-fold. A combination of computational and experimental analyses indicated that this hindered cavity escape was due to an electrostatic energy barrier in the region of the hole, which was quantitatively explained using DLVO theory. These findings explicitly demonstrate that the cavity escape process was barrier-limited and dominated by electrostatic effects.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

Colloidal Stability of PFSA-Ionomer Dispersions. Part I. Single-Ion Electrostatic Interaction Potential Energies

Charged colloidal particles neutralized by a single counterion are increasingly important for many emerging technologies. Attention here is paid specifically to hydrogen fuel cells and water electrolyzers whose catalyst layers are manufactured from a perfluorinated sulfonic acid polymer (PFSA) suspended in aqueous/alcohol solutions. Partially dissolved PFSA aggregates, known collectively as ionomers, are stabilized by the electrostatic repulsion of overlapping diffuse double layers consisting of only protons dissociated from the suspended polymer. We denote such double layers containing no added electrolyte as "single ion". Size-distribution predictions build upon interparticle interaction potential energies from the Derjaguin-Landau-Verwey-Overbeek (DLVO) formalism. However, when only a single counterion is present in solution, classical DLVO electrostatic potential energies no longer apply. Accordingly, here a new formulation is proposed to describe how single-counterion diffuse double layers interact in colloidal suspensions. Part II (Srivastav, H.; Weber, A. Z.; Radke, C. J. Langmuir 2024 DOI: 10.1021/acs.langmuir.3c03904) of this contribution uses the new single-ion interaction energies to predict aggregated size distributions and the resulting solution pH of PFSA in mixtures of n-propanol and water. A single-counterion diffuse layer cannot reach an electrically neutral concentration far from a charged particle. Consequently, nowhere in the dispersion is the solvent neutral, and the diffuse layer emanating from one particle always experiences the presence of other particles (or walls). Thus, in addition to an intervening interparticle repulsive force, a backside osmotic force is always present. With this new construction, we establish that single-ion repulsive pair interaction energies are much larger than those of classical DLVO electrostatic potentials. The proposed single-ion electrostatic pair potential governs dramatic new dispersion behavior, including dispersions that are stable at a low volume fraction but unstable at a high volume fraction and finite volume-fraction dispersions that are unstable with fine particles but stable with coarse particles. Finally, the proposed single-counterion electrostatic pair potential provides a general expression for predicting colloidal behavior for any charged particle dispersion in ionizing solvents with no added electrolyte.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

Colloidal Dispersions of Sterically and Electrostatically Stabilized PbS Quantum Dots: Structure Factors, Second Virial Coefficients, and Film-Forming Properties

Electrostatically stabilized nanocrystals (NCs) and, in particular, quantum dots (QDs) hold promise for forming strongly coupled superlattices due to their compact and electronically conductive surface ligands. However, studies of the colloidal dispersion and interparticle interactions of electrostatically stabilized sub-10 nm NCs have been limited, hindering the optimization of their colloidal stability and self-assembly. In this study, we employed small-angle X-ray scattering (SAXS) experiments to investigate the interparticle interactions and arrangement of PbS QDs with thiostannate ligands (PbS-Sn2S64-) in polar solvents. The study reveals significant deviations from the ideal solution behavior in electrostatically stabilized QD dispersions. Our results demonstrate that PbS-Sn2S64- QDs exhibit long-range interactions within the solvent, in contrast to the short-range steric repulsion characteristic of PbS QDs with oleate ligands (PbS-OA). Introducing highly charged multivalent electrolytes screens electrostatic interactions between charged QDs, reducing the length scale of the repulsive interactions. Furthermore, we calculated the second virial (B2) coefficients from SAXS data, providing insights into how surface chemistry, solvent, and size influence pair potentials. Finally, we explore the influence of long-range interparticle interactions of PbS-Sn2S64- QDs on the morphology of films produced by drying or spin-coating colloidal solutions. The long-range repulsive term of PbS-Sn2S64- QDs promotes the formation of amorphous films, and screening the electrostatic repulsion by the addition of an electrolyte enables the formation of crystalline domains. These findings highlight the critical role of NC-NC interactions in tailoring the properties of functional materials made of colloidal NCs.

SAXS↗

DOE OSTI2024

Diffusioosmotic flow reversals due to ion–ion electrostatic correlations

Existing theories of diffusioosmosis have neglected ion–ion electrostatic correlations, which are important in concentrated electrolytes. Here, we develop a mathematical model to numerically compute the diffusioosmotic mobilities of binary symmetric electrolytes across low to high concentrations in a charged parallel-plate channel. We use the modified Poisson equation to model the ion–ion electrostatic correlations and the Bikerman model to account for the finite size of ions. We report two key findings. First, ion–ion electrostatic correlations can cause a unique reversal in the direction of diffusioosmosis. Such a reversal is not captured by existing theories, occurs at ≈ 0.4 M for a monovalent electrolyte, and at a much lower concentration of ≈ 0.003 M for a divalent electrolyte in a channel with the same surface charge. This highlights that diffusioosmosis of a concentrated electrolyte can be qualitatively different from that of a dilute electrolyte, not just in its magnitude but also its direction. Second, we predict a separate diffusioosmotic flow reversal, which is not due to electrostatic correlations but the competition between the underlying chemiosmosis and electroosmosis. This reversal can be achieved by varying the magnitude of the channel surface charge without changing its sign. However, electrostatic correlations can radically change how this flow reversal depends on the channel surface charge and ion diffusivity between a concentrated and a dilute electrolyte. Furthermore, the mathematical model developed here can be used to design diffusioosmosis of dilute and concentrated electrolytes, which is central to applications such as species mixing and separation, enhanced oil recovery, and reverse electrodialysis.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1979

Coherent anomalous resistivity in the region of electrostatic shocks

Anomalous resistivity in a phase-coherent electrostatic ion cyclotron wave in the region of the auroral electrostatic shocks observed by the S3-3 satellite is considered. It is shown that current-driven shocks and anomalous resistivity will be most important above 5,000 km, where the electron drift velocity is maximized and parallel electric fields are possible. A model for the parallel field based on the dissipation of an Alfven wave pulse by current-driven electrostatic ion cyclotron turbulence is presented. In the model, coherent electrostatic ion cyclotron waves lead to anomalous resistivity by electron trapping, producing parallel electric fields greater than 1 mV/m, and may set up the parallel populations necessary to support oblique electrostatic shocks.

Lysak, R. L.↗

NASA NTRS1981

Electrostatic disruption of a charged conducting spheroid

Electrostatic disruption of elongated parent grains following sudden charging to high electrostatic potentials is proposed as a specific mechanism for the appearance of striae or pseudosynchronic bands which have been observed in several comets. The polar and equatorial electrostatic tension for axis ratios between 0.01 and 1000 are calculated, and the polar pressure is found to be larger than the equatorial pressure for prolate spheroids. The electrostatic polar pressure profile along the polar axis for prolate spheroids is calculated, and the pressure is found to increase monotonically from a minimum at the center to a maxima at the ends. This indicates that as a prolate spheroid of uniform tensile strength is charged up, it will continue to chip off at the ends when the electrostatic pressure there exceeds the uniform tensile strength of the grain. The result can be a prolate grain or a grain which continues chipping until it explodes.

Hill, J. R.↗

NASA NTRS1987

The electrostatic effect for the collisionless tearing mode

Electron dynamics has not been self-consistently considered in collisionless tearing mode theories to date because of the mathematical complexity of the Vlasov-Maxwell equations. It has been found, using computer simulations, that electrostatic fields play an important role in the tearing mode. Vlasov theory, including the electrostatic field, is investigated for topologies with both antiparallel and nonantiparallel magnetic field lines. The electrostatic field influences the resonant current in the neutral sheet which is a non-MHD effect, and modifies the linear growth rate. At the magnetopause, where the field lines are not antiparallel, the electrostatic effect acts to raise the linear growth rate of the tearing mode. On the other hand, in the magnetotail, where magnetic field lines are antiparallel, the electrostatic effect reduces the tearing mode growth rate.

Hoshino, Masahiro↗

NASA NTRS1991

Electrostatic fields in a dusty Martian environment

While there have been several studies suggesting the possibility of electrical activity on Mars, to date there have been no measurements to search for evidence of such activity. In the absence of widespread water clouds and convective storm systems similar to those on the Earth and Jupiter, the most likely candidate for the creation of electrostatic charges and fields is triboelectric charging of dust, i.e., the friction between blown dust and the ground, and of dust particles with each other. Terrestrial experience demonstrates that electric fields 5 to 15 kV-m(exp -1) are not uncommon in dust storms and dust devils in desert regions, where the polarity varies according to the chemical composition and grain size. Simple laboratory experiments have demonstrated that modest electrostatic fields of roughly 5,000 V-m(exp -1) may be produced, along with electrical spark discharges and glow discharges, in a simulation of a dusty, turbulent Martian surface environment. While the Viking landers operated for several years with no apparent deleterious effects from electrostatic charging, this may have been at least partly due to good engineering design utilizing pre-1976 electronic circuitry to minimize the possibility of differential charging among the various system components. However, free roaming rovers, astronauts, and airborne probes may conceivably encounter an environment where electrostatic charging is a frequent occurrence, either by way of induction from a static electric field or friction with the dusty surface and atmosphere. This raises the possibility of spark discharges or current surges when subsequent contact is made with other pieces of electrical equipment, and the possibility of damage to modern microelectronic circuitry. Measurements of electrostatic fields on the surface of Mars could therefore be valuable for assessing this danger. Electric field measurements could also be useful for detecting natural discharges that originate in dust storms. This detection could be performed at distances ranging from 10s of km in the case of J-charge-like discharge signatures, to planetary distances if there exists a global electrical circuit or Schumann resonance spectrum.

Sentman, D. D.↗

NASA NTRS1996

Numerical Investigation of Two-Phase Flows With Charged Droplets in Electrostatic Field

A numerical method to solve two-phase turbulent flows with charged droplets in an electrostatic field is presented. The ensemble-averaged Navier-Stokes equations and the electrostatic potential equation are solved using a finite volume method. The transitional turbulence field is described using multiple-time-scale turbulence equations. The equations of motion of droplets are solved using a Lagrangian particle tracking scheme, and the inter-phase momentum exchange is described by the Particle-In-Cell scheme. The electrostatic force caused by an applied electrical potential is calculated using the electrostatic field obtained by solving a Laplacian equation and the force exerted by charged droplets is calculated using the Coulombic force equation. The method is applied to solve electro-hydrodynamic sprays. The calculated droplet velocity distributions for droplet dispersions occurring in a stagnant surrounding are in good agreement with the measured data. For droplet dispersions occurring in a two-phase flow, the droplet trajectories are influenced by aerodynamic forces, the Coulombic force, and the applied electrostatic potential field.

Kim, Sang-Wook↗

DOE OSTI2023

Electrostatic dust remediation for future exploration of the Moon

Dust accumulation is one of the critical issues that must be mitigated on in-situ lunar explorations because an in-situ probe is exposed to small dust particles, which are easily attached to it, during its operations. The Lunar Dust Science Definition Team is organized by the Jet Propulsion Lab/California Institute of Technology through NASA’s Biological and Physical Sciences Division to define key science questions and assess dust remediation techniques. Here, we assess three electrostatic remediation technology concepts: electrostatic dust shield; surface electrostatically collecting dust, later called attractive surface; and electron beam — plasma jet inducing electrostatic dust lofting from a surface. We qualitatively investigate their maturity by defining six operational factors: Time and location; Amount of dust removal; Contamination of target surfaces; Operation duration; Installation; and Safety. In addition to these techniques, we discuss a supporting system that loads dust particles onto a test article to examine dust removal efficiency. Here, the results show that further development increases the maturity of all the technologies. While laboratory and theoretical demonstrations reported whether each technology robustly work on the Moon, which hosts a complex, heterogeneous dust environment, we find that it is still uncertain if this is the case because none has been tested in the lunar environment. Particularly, operation duration and safety are critical to be addressed further on both laboratory and spaceflight scales.

42 ENGINEERING↗

DOE OSTI2021

Neat, Simple, and Wrong: Debunking Electrostatic Fallacies Regarding Noncovalent Interactions

Multipole moments such as charge, dipole, and quadrupole are often invoked to rationalize intermolecular phenomena, but a low-order multipole expansion is rarely a valid description of electrostatics at the length scales that characterize nonbonded interactions. This is illustrated by examining several common misunderstandings rooted in erroneous electrostatic arguments. First, the notion that steric repulsion originates in Coulomb interactions is easily disproved by dissecting the interaction potential for Ar2. Second, the Hunter-Sanders model of π–π interactions, which is based on quadrupolar electrostatics, is shown to have no basis in accurate calculations. Third, curved “buckybowls” exhibit unusually large dipole moments, but these are ancillary to the forces that control their intermolecular interactions, as illustrated by two examples involving corannulene. Finally, the assumption that interactions between water and small anions are dictated by the dipole moment of H 2 O is shown to be false in the case of binary halide–water complexes. Furthermore, these examples present a compelling case that electrostatic explanations based on low-order multipole moments are very often counterfactual for nonbonded interactions at close range and should not be taken seriously in the absence of additional justification.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2024

Charging, aggregation, and electrostatic dispersion of radioactive and nonradioactive particles in the atmosphere

Electrostatic dispersion can significantly impact the microphysical behavior of charged particles and ions until reaching zero space charge. However, although radioactive particles can be strongly charged in air, the influence of electrostatic dispersion has been neglected in understanding their behavior. This study is aimed at investigating the time evolution of the charge and size distributions of radioactive and nonradioactive particles in air and developing simple approaches for applications. With processes involving charging, aggregation, and electrostatic dispersion, a comprehensive population balance model (PBM) has been developed to examine particle charge/size distribution dynamics. It is shown that compared to nonradioactive particles, the charge and size distributions of radioactive particles may evolve differently with time because radioactivity and electrostatic dispersion can significantly affect the charging and aggregation kinetics of the particles. It is found that, after the Fukushima accident, background aerosols in the pathway of radioactive plumes might be highly charged due to ionizing radiation, suggesting that radiation fields may strongly influence in situ measurements of charged atmospheric particles. The comprehensive PBM is simplified, and then the verification and application of the simplified PBMs are discussed. This study provides useful insight into how radioactivity can affect the dynamic behavior of particles in atmospheric systems including radiation sources.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRSDate not supplied

Electrostatic Regolith Interaction Experiment (ERIE) Electrometer Instrument Development

The Electrostatic Regolith Interaction Experiment (ERIE) is a joint venture between the University of Central Florida (UCF) Center for Microgravity Research (CMR) and the NASA Kennedy Space Center (KSC) Electrostatics and Surface Physics Laboratory (ESPL) seeking to examine charged dust grain behavior in a microgravity environment. Two separate systems have been combined for this suborbital flight experiment: the COLLisions Into Dust Experiment (COLLIDE) developed by the UCF CMR and the Wheel Electrostatic Spectrometer (WES) developed by the NASA KSC ESPL. This combination will advance the understanding of the natural and induced charged grain behavior on the Moon, asteroids, and other low gravity bodies comprised of charged dust particles. COLLIDE retains granular material under vacuum in a shallow tray behind a metal door, which then opens and releases the particles into a larger open volume when microgravity is achieved. The experiment is observed with a high-speed camera, such that the motions of these particles can then be tracked so the kinematics of each grain may be analyzed. The original application for this apparatus was to study cratering events into granular beds, but electrostatic repulsion was detected in the early frames of the video data returned from completed experiments, so a re-flight with a focus on these events was proposed. Agitation of the grains during launch combined with the frictional charge transfer between the grains and the door as it slides open provides an opportunity to use this setup to observe material tribocharging and charged particle behaviors in microgravity. In this updated version, the charged particles released into the chamber will traverse through an electric field produced by high voltage parallel plates and their resulting trajectories will be determined by their net charges. WES was originally developed to characterize the triboelectric properties of the Martian regolith through the contact of a rover wheel with the surface as it rotates. Improvements were made upon this legacy system to develop a sensor suite that will be installed within the COLLIDE door to measure charge transferred between the granular material and insulating disks protruding through the door. These insulator disks span the triboelectric series so, as they slide across the particulate matter when the door opens, each will accumulate a charge consistent with its relative position to the grains within the series. This charge on each insulator is distributed between two capacitances in series with an electrometer amplifier returning an analog voltage proportional to the charge accumulated. Calibration of this system has been performed using applications of known charge to the inputs and characterization of the frictional charge transfer between various regolith simulants and the sensor insulators is currently being examined in the lab.

Electrostatics↗

NASA NTRSDate not supplied

Electrostatic Regolith Interaction Experiment (ERIE) Electrometer Initial Flight Results

The Electrostatic Regolith Interaction Experiment (ERIE) is a suborbital flight payload studying electrostatically charged dust particle dynamics under microgravity, jointly developed by University of Central Florida (UCF) and NASA Kennedy Space Center (KSC). ERIE combines components from two systems, the COLLisions Into Dust Experiment (COLLIDE) from UCF and the Wheel Electrostatic Spectrometer (WES) from NASA KSC, to advance understanding of charged grain behavior on low gravity bodies such as the Moon and asteroids. ERIE slides a door containing an electrometer system monitoring various insulating disks across the surface of a regolith simulant bed. The experiment is activated when the payload enters the microgravity potion of the flight. The grains in the simulant bed tribocharge via agitation during launch as well as through frictional interactions with the door and its protruding insulators. As the retention door retracts, particles are allowed to loft into an open volume, achieving motion due to electrostatic repulsion. The electrometer system measures the charge transfer between the granular material and the insulators. As the charged grains exit the bed, they travel through an applied electric field and a camera observes the kinematics of the individual grains whose trajectories are determined by their net charges. The design of the ERIE electrometer instrument and initial results from the first flight was presented at the 2021 AGU Fall Meeting under P55E-2002. Shortly after microgravity was achieved and the retaining door began to open, the rate of charge acquisition measured by the electrometer increased, indicating the insulators were accumulating triboelectric charge. Charged grains were observed in the video data to traverse across the external electric field and become deflected from a linear path due to their charges. Pairs of grains were also observed to orbit one another as expected from two oppositely charged bodies in proximity to one another. Improvements to the design of the instrument and preliminary results obtained from the second flight scheduled for Q3 2022 will be presented at this meeting.

Electrostatics↗

NASA NTRSDate not supplied

Electrostatic Regolith Interaction Experiment (ERIE) Electrometer Initial Flight Results

Electrostatics↗

DOE OSTI2020

Electrostatic control of photoisomerization pathways in proteins

Rotation around a specific bond after photoexcitation is central to vision and emerging opportunities in optogenetics, super-resolution microscopy, and photoactive molecular devices. Competing roles for steric and electrostatic effects that govern bond-specific photoisomerization have been widely discussed, the latter originating from chromophore charge transfer upon excitation. We systematically altered the electrostatic properties of the green fluorescent protein chromophore in a photoswitchable variant, Dronpa2, using amber suppression to introduce electron-donating and electron-withdrawing groups to the phenolate ring. Through analysis of the absorption (color), fluorescence quantum yield, and energy barriers to ground- and excited-state isomerization, we evaluate the contributions of sterics and electrostatics quantitatively and demonstrate how electrostatic effects bias the pathway of chromophore photoisomerization, leading to a generalized framework to guide protein design.

59 BASIC BIOLOGICAL SCIENCES↗