MUlti-SpEctra, MUlti-SpEcies, Multi-SEnsors (MUSEs) retrievals of Ozone and Carbon Monoxide during 2019 FIREX-AQ
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The Fire Influence on Regional to Global Environments and Air Quality (FIREX AQ) field campaign was conducted during August 2019 to investigate the impact of wildfire and biomass smoke on air quality and weather in the continental United States. Ultra-spectral resolved infrared measurements contain information about tropospheric carbon monoxide (CO) and ozone (O3), as well as other trace species. A methodology of retrieving these tropospheric trace species from such remotely sensed spectral data has been developed and validated for the National Airborne Sounder Testbed-Interferometer (NAST I). NAST I CO and O3 measurements from the recent FIREX AQ field campaign are presented herein and used to estimate wildfire plume age. Results show enhanced CO plume evolution and transport away from fire ground site, and its plume age associated with the plume distance in both vertical and horizontal directions from the wildfire location, as enabled by the moderate-vertical and high-horizontal resolution obtained from the NAST I remotely sensed IR spectrometer onboard NASA ER 2 aircraft. This study advances our knowledge of fire-induced plume with its evolution and age in 3-dimensional space.
Ultra-spectral resolved infrared measurements from aircraft and space-based observations contain information about tropospheric carbon monoxide (CO) and ozone (O3), as well as other trace species. A methodology of retrieving these tropospheric trace species from such remotely sensed spectral data has been developed and validated for the National Airborne Sounder Testbed-Interferometer (NAST-I). The Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) field campaign was conducted during August 2019 to investigate the impact of wildfire and biomass smoke on air quality and weather in the continental United States. NAST-I CO and O3 measurements from the recent FIREX-AQ field campaign are presented herein and used to estimate wildfire plume age. Results show enhanced CO plume evolution and transport away from fire ground site, and its plume age associated with the plume distance in both vertical and horizontal directions from the wildfire location, as enabled by the moderate-vertical and high-horizontal resolution obtained from the NAST-I remotely sensed IR spectrometer onboard NASA ER-2 aircraft. This study advances our knowledge of fire-induced plume with its evolution and age in 3-dimensional space.
Emissions of trace gases and particles from fires have a major impact on climate, visibility, air quality, and public health. Biomass burning emissions include reactive nitrogen gases, among which ammonia (NH3) plays a prominent role. NH3 is a short-lived gas that acts as precursor for secondary inorganic aerosols. This process is still poorly constrained in downwind fire plumes. In summer 2019, NASA and NOAA carried out the joint airborne FIREX-AQ (Fire Influence on Regional to global Environments and Air Quality) mission over the continental US to sample plumes from wildfires and agricultural fires. On board the NASA DC-8, we used a modified PTR-ToF-MS instrument for measuring NH3 in situ and at high time resolution. Over the course of the mission, we collected a large set of NH3 data in plumes emitted from fires differing in fuel type and burning stage. Herein, we will present the measured NH3 emissions ratios and factors, compare them with the literature, and investigate the dependence of NH3 emissions on fuel type and burning conditions.
Wildfire smoke is one of the most significant concerns of human and environmental health, associated with its substantial impacts on air quality, weather, and climate. However, biomass burning emissions and smoke remain among the largest sources of uncertainties in air quality forecasts. In this study, we evaluate the smoke emissions and plume forecasts from 12 state-of-the-art air quality forecasting systems during the Williams Flats fire in Washington State, US, August 2019, which was intensively observed during the Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) field campaign. Model forecasts with lead times within 1 d are intercompared under the same framework based on observations from multiple platforms to reveal their performance regarding fire emissions, aerosol optical depth (AOD), surface PM2.5, plume injection, and surface PM2.5 to AOD ratio. The comparison of smoke organic carbon (OC) emissions suggests a large range of daily totals among the models, with a factor of 20 to 50. Limited representations of the diurnal patterns and day-to-day variations of emissions highlight the need to incorporate new methodologies to predict the temporal evolution and reduce uncertainty of smoke emission estimates. The evaluation of smoke AOD (sAOD) forecasts suggests overall underpredictions in both the magnitude and smoke plume area for nearly all models, although the high-resolution models have a better representation of the fine-scale structures of smoke plumes. The models driven by fire radiative power (FRP)-based fire emissions or assimilating satellite AOD data generally outperform the others. Additionally, limitations of the persistence assumption used when predicting smoke emissions are revealed by substantial underpredictions of sAOD on 8 August 2019, mainly over the transported smoke plumes, owing to the underestimated emissions on 7 August. In contrast, the surface smoke PM2.5 (sPM2.5) forecasts show both positive and negative overall biases for these models, with most members presenting more considerable diurnal variations of sPM2.5. Overpredictions of sPM2.5 are found for the models driven by FRP-based emissions during nighttime, suggesting the necessity to improve vertical emission allocation within and above the planetary boundary layer (PBL). Smoke injection heights are further evaluated using the NASA Langley Research Center's Differential Absorption High Spectral Resolution Lidar (DIAL-HSRL) data collected during the flight observations. As the fire became stronger over 3–8 August, the plume height became deeper, with a day-to-day range of about 2–9 km a.g.l. However, narrower ranges are found for all models, with a tendency of overpredicting the plume heights for the shallower injection transects and underpredicting for the days showing deeper injections. The misrepresented plume injection heights lead to inaccurate vertical plume allocations along the transects corresponding to transported smoke that is 1 d old. Discrepancies in model performance for surface PM2.5 and AOD are further suggested by the evaluation of their ratio, which cannot be compensated for by solely adjusting the smoke emissions but are more attributable to model representations of plume injections, besides other possible factors including the evolution of PBL depths and aerosol optical property assumptions. By consolidating multiple forecast systems, these results provide strategic insight on pathways to improve smoke forecasts.
Biomass burning has been identified as a primary emission source for a host of gas and aerosol phase compounds which can damage environmental and human health. During FIREX-AQ collaborators from UNH, NASA Langley Aerosol Research Group Experiment (LARGE), and Brown University conducted measurements out of NASA Langley’s mobile laboratory during July and August of 2019. Nitrous acid (HONO) and nitric acid (HNO3) concentrations were measured at nominal 5-minute resolution using a dual mist chamber-ion chromatograph system resulting in approximately 1,200 total samples from five separate fires in the western US. Enhancement ratios between PM2.5 and carbon monoxide were used to discriminate between young and aged smoke plumes. Average HONO concentrations were significantly higher (P << 0.01) in young daytime compared to nighttime smoke while no statistical differences (P > 0.05) were observed between young and aged smoke during day or night. In daytime smoke from the Williams Flats fire (75 km SE of Spokane, WA on the Columbia River) UV-A irradiation was highly correlated with HONO to nitrogen dioxide (NO2) ratios; indicating that heterogenous NO2 to HONO conversion more than compensated for rapid photolytic loss of HONO. Black carbon (BC) may serve as a stable proxy for total available aerosol surface area in biomass burning plumes when total aerosol size distributions are unavailable. During the day HONO/NO2 is weakly correlated to BC when BC abundance exceeds 1 ug/m3 but at lower BC concentrations the relationship breaks down. At night this relationship was stronger, partly due to consistently high BC concentrations. These observations suggest that heterogenous conversion of NO2 to HONO on aerosol is a significant source of HONO in dense smoke plumes. In more diffuse smoke conversion on other surfaces (soil, foliage) becomes more important.
Biomass Burning (BB) fires are expected to occur more frequently in the future due to climate change, the build‐up of fuels due to fire suppression, and the expansion of the wildland‐urban interface [Schoennagel et al., 2017; Shivdenko & Schepaschenko, 2013; Stevens et al., 2014; Turner et al., 2019; Yue et al., 2015; Tilman et al., 2001]. Accurate knowledge of the abundance, distribution, and optical properties of absorbing aerosols such as BB smoke is essential to understanding regional and global aerosol radiative effects [Boucher et al., 2013]. It is recognized that differing fuel types (e.g., rice straw, ponderosa pine), combustion modes (i.e., flaming, smoldering or both) and temperature/ moisture content produce smoke with differing optical characteristics (e.g., aerosol light scattering and absorption) and component mixing ratios [e.g., BC, OC and inorganic species such as sulfate, potassium, chloride; Streets et al. 2003; Reid et al., 2005a, b; Janhäll et al., 2010; Sayer et al., 2014]. However, climate models often ascribe a fixed set of emission factors [i.e., amount of particulate for a given species released in the atmosphere per unit dry fuel burned; Darmenov and Dasilva, 2013] and optical properties [Hess et al., 1998] to all BB aerosol plumes, inherently limiting accurate representation of the global and regional heterogeneity of BB. The overarching goal of the proposed work is to improve the microphysical and optical representation of different types of Biomass Burning in Chemistry Transport Models. Our strategy is to capitalize on multiple airborne campaigns (e.g., ARCTAS, SEAC4RS, ORACLES, FIREX-AQ), which sampled different types of BB plumes at different aging stages. Models, when improved and combined with satellite, airborne, and ground observations will help address many aerosol science objectives from the NASA Decadal survey [National Academies of Sciences, Engineering, and Medicine. 2018].
The relatively simple dark-target (DT) aerosol retrieval algorithm provides products of spectral aerosol optical depth (AOD) from measurements of multi-spectral reflectance in visible, near-infrared and shortwave infrared wavelength bands. Originally developed for Moderate-resolution Imaging Spectroradiometer (MODIS aboard Terra and Aqua) in Low-Earth Orbit (LEO), DT has been ported to Visible Infrared Imaging Suite (VIIRS aboard Suomi-NPP and NOAA-20, also in LEO), to enhanced-MODIS Airborne Simulator (eMAS, on an airborne platform), and now to sensors in GEOstationary orbit (Advanced Himawari Imager - AHI aboard Himawari-8 and Advanced Baseline Imagers – ABI aboard GOES-16 and 17). Together, these new datasets not only extend upon the 20+ year MODIS aerosol record, but also expand the temporal sampling and/or spatial resolution. Between July and October of 2019, NASA participated in two field experiments on opposite sides of the globe. These included FIREX-AQ which focused on fire and smoke in the Western U.S., and then CAMP2EX which targeted aerosol/cloud interactions around the Philippines. We have performed DT aerosol retrievals on all images from all sensors during these three months, validated against ground observations from stationary and mobile sunphotometer sites, and have begun to develop a synergy that represents semi-global observations every half hour. The resulting aerosol products are being used as context and for model assimilation, thus providing the framework for more complete characterization of global aerosol transport and lifecycle. Here, we report on progress, as well as remaining challenges such as data management, computer processing, and accounting for differences between GEO and LEO observation geometry and surface reflectance parameterization.
A series of flights were performed by the NASA DC-8 for the FIREX-AQ missions to observe the effects of wildfires and agricultural fires on air quality and climate in selected locations of the United States. Borescope evaluations after these flights indicated accelerated damage had occurred over this flight series to the blades in the high pressure compressor section of all four CFM56-2C1 turbine engines. This erosion and impact damage appeared to vary in severity, and appeared most severe for engines 3 and 4 located on the right wing of the DC-8.Engine 3 had the most flight hours and cycles since last overhaul of 7,152 h and 2,502 cycles. Engine 4 had the lowest flight hours and cycles since last overhaul of 1,354 h and 369 cycles. For these reasons, three noticeably damaged blades were selected from the high pressure compressor for each of these two engines, and then evaluated at NASA GRC using optical and scanning electron microscopy. Engine 3 compressor blades had both erosion and impact damage that were observed and characterized. The erosion damage was associated with embedded particles 13 μm to 42 μm in sectioned width, composed of varied compositions ranging from SiO2 to SiO2 also containing Ca, Mg, and Al (CMAS). The impact damage was associated with the impacts of larger objects at least 650 μm to 850 μm in width, but only small fragments 5 μm to 15 μm in sectioned width were embedded in the impact surface, also composed of SiO2 to SiO2 containing Ca, Mg, and Al (CMAS). On the other hand, engine 4 blades had only impact damage that was observed and characterized. This impact damage was associated with impacts of objects at least 1,480 μm to 2,080μm in width. Small fragments 5 μm to 15 μm in sectioned width were embedded in the impact surface. For one impact, the fragments were again composed of SiO2 to SiO2 containing Ca, Mg, and Al (CMAS). For two other impacts, the fragments were often composed of Fe, and less frequently Cu.
Vicarious calibration approaches using in-situ measurements are key techniques applied to on-orbit remote sensors. The in-situ measurements have advantages in terms of traceability and quantifiable accuracy that make them ideal for inter-consistency studies of on-orbit sensors. The Committee on Earth Observation Satellites Working Group on Calibration and Validation Infrared Visible Optical Sensors initiated the Radiometric Calibration Network (RadCalNet) to provide automated surface and top-of-atmosphere (TOA) reflectance data from multiple participating ground sites to the worldwide user community. RadCalNet standardizes protocols for collecting data, processes TOA reflectance, and provides International System of Units traceable uncertainty budgets for the five currently operating sites. RadCalNet data from the Railroad Valley Playa, Nevada, site was used to provide an SI-traceable, absolute radiometric calibration of the Enhanced MODIS Airborne Simulator as part of an overflight of opportunity during the FIREX-AQ campaign. The results shown here demonstrate the utility of RadCalNet data for absolute radiometric calibration of airborne imagers making flights of opportunity without the need for coordination with a field validation team.
Burning of small fires in the Arctic is important to climate change related processes and in the past the importance has been overlooked. Similarly, small fire burning in the Southeast United states has been underestimated and overlooked, but has just as much burned area as wildfires in the Western United States. Using FIREX-AQ campaign data, we are looking at the ability of satellites to detected the fires. Possible similarities in small fires between the Central and Southeastern US and the Arctic give ideas for collaboration and quantification of burned area.
The number of variables measured during airborne field campaigns has increased more than tenfold over the last thirty years. With this increase in measurements, the complexity for distributed active archive centers (DAACs) to distribute the data and for data users to search for and find measurements of interest has also increased. Part of this complexity arises from the unique variable names in suborbital atmospheric composition field studies. With limited guidelines related to variable naming, variable names and structures can vary significantly, even for the same type of variable. It is common for instrument scientists to use their intended measurable quantity as the data variable name. This can make it difficult for users to locate and interact with a particular variable across multiple data sets. One effective solution to this problem, identified by the Earth Science Data System (ESDS) ICARTT Refresh Working Group [1], was to introduce variable standard names that can be used as tags for each data variable. This allows similar measurements (e.g., dew point) to be categorized and located across field campaigns, regardless of what variable name the instrument scientist has used. From this the atmospheric composition variable standard names were developed with the goal to use Findable, Accessible, Interoperable, and Reusable (FAIR) principles [2] and provide context for all users, while remaining connected to those in the subject area. These standard names have been successfully implemented in FIREX-AQ, CAMP 2EX, ACTIVATE, and DCOTSS field campaigns.
During the 2019 Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) study, the NASA DC-8 carried out in situ chemical measurements in smoke plumes emitted from wildfires and agricultural fires in the contiguous United States. The DC-8 payload included a modified proton-transfer-reaction time-of-flight mass spectrometer (PTR-ToF-MS) for the fast measurement of gaseous ammonia (NH 3 ) and a high-resolution time-of-flight aerosol mass spectrometer (AMS) for the fast measurement of submicron particulate ammonium (NH 4 + ). We herein report data collected in smoke plumes emitted from 6 wildfires in the Western United States, 2 prescribed grassland fires in the Central United States, 1 prescribed forest fire in the Southern United States, and 66 small agricultural fires in the Southeastern United States. Smoke plumes contained double to triple digit ppb levels of NH 3 . In the wildfire plumes, a significant fraction of NH 3 had already been converted to NH 4 + at the time of sampling (≥2 h after emission). Substantial amounts of NH 4 + were also detected in freshly emitted smoke from corn and rice field fires. We herein present a comprehensive set of emission factors of NH 3 and NH x , with NH x = NH 3 + NH 4 + . Average NH 3 and NH x emission factors for wildfires in the Western United States were 1.86±0.75 g kg −1 and 2.47±0.80 g kg −1 of fuel burned, respectively. Average NH 3 and NH x emission factors for agricultural fires in the Southeastern United States were 0.89±0.58 and 1.74±0.92 g kg −1 , respectively. Our data show no clear inverse correlation between modified combustion efficiency (MCE) and NH 3 emissions. The observed NH 3 emissions were significantly higher than measured in previous laboratory experiments in the FIREX FireLab 2016 study.
The NASA Science Mission Directorate Earth Science Division Airborne Science Program enables access to modified aircraft in support of NASA projects. The Program supports researchers and engineers by enabling testing of new instruments, calibration of on-orbit satellite instruments with airborne sensors, and to support process studies and model development. This talk will provide an overview of the Program capabilities, review past NASA flight projects that have focused on wildfires, and discuss how the Program is poised to support the FireSense project and interagency efforts to incorporate new technologies and observations into the wildfire management community. Past missions including the Western States Fire Mission and FIREX-AQ will be discussed, an overview of relevant NASA sensors will be provided, and an introduction to upcoming flight activity will be presented. Data telemetry, communications, and data standards will also be discussed towards improving timely distribution of data products to land managers.
The National Airborne Sounder Testbed-Interferometer (NAST-I) is an airborne FTS remote sensor that nominally flies on NASA high-altitude aircraft to serve as a spaceborne instrument simulator. NAST-I continues to serve as a pathfinder for future satellite FTS systems and the next generation advanced atmospheric sounders in general. NAST-I provides high resolution spectrally resolved infrared radiances. NAST-I retrieval products characterizing the surface (i.e., skin temperature and spectral emissivity), atmosphere (i.e., profiles of temperature, moisture, ozone, carbon monoxide, and other trace species), and clouds (e.g., optical depth, particle size, temperature, and height) can be used to support fire-related monitoring and research. NAST-I provided 3-d characterizations of wildfire-induced plumes of CO during the FIREX-AQ field campaign (conducted during 2019) which showed the intensity and size evolution of wildfire plumes at high spatial and temporal resolutions. Wildfire-induced CO plumes, in conjunction with their evolution, transport, and age have been identified and recently published in scientific journals. Other research applications, such as surface emissivity changes due to fire burning of ground landscape, have been under investigation. These products could be used in support of wildfire management to better inform decision making and operations for pre-, active, and post-fire environments.
Even though fire can be devastating, wildland fire is a natural and integral force on our landscapes, providing value by decreasing fuels at the Wildland Urban Interface (WUI) to promote safe communities. However, uncontained wildfires can devastate communities, threaten our health, and result in substantial economic losses. There has been greater than a $50B increase in wildfire insurance claims from 2017-2021, which has been exacerbated by climate change. Our partners at Kettle reinsurance are focused on building a smarter reinsurance model for protecting today’s globalized world from the catastrophic effects of climate change. Our objective is to develop a high-confidence grid-based wildfire burn product using multiple sources of satellite data to determine whether a ‘conflagration' (fire larger than 999+ acres) has ‘breached’ a grid cell. This product will substantially decrease the time it takes for homeowners to receive payouts, from over a year to a couple months. Working with our partners at Kettle reinsurance, we use VIIRS (Visible Infrared Imaging Radiometer Suite) 375 m fire detections and Sentinel-2 10 m satellite imagery to create a 20-m gridded fire burn product. Our process is based on the level of confidence in the data source and takes into account vegetation change throughout the life of the fire. For example, Sentinel-2 vegetation-change indices have a higher level of confidence when congruent with VIIRS active-fire detection data, rather than VIIRS detections alone. We have also verified our fire burn product against MODIS/ASTER Airborne Simulator (MASTER) Infrared (IR) data from the Fire Influence on Regional to Global Environments Experiment - Air Quality (FIREX-AQ) 2019 campaign, with 88% overall agreement. The first iteration has been developed for responding to wildfires in California, with the possibility to expand nationwide and globally.
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