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Comparison of Satellite and Aircraft Measurements of Cloud Microphysical Properties in Icing Conditions During ATREC/AIRS-II

Satellites are ideal for continuous monitoring of aircraft icing conditions in many situations over extensive areas. The satellite imager data are used to diagnose a number of cloud properties that can be used to develop icing intensity indices. Developing and validating these indices requires comparison with objective "cloud truth" data in addition to conventional pilot reports (PIREPS) of icing conditions. Minnis et al. examined the relationships between PIREPS icing and satellite-derived cloud properties. The Atlantic-THORPEX Regional Campaign (ATReC) and the second Alliance Icing Research Study (AIRS-II) field programs were conducted over the northeastern USA and southeastern Canada during late 2003 and early 2004. The aircraft and surface measurements are concerned primarily with the icing characteristics of clouds and, thus, are ideal for providing some validation information for the satellite remote sensing product. This paper starts the process of comparing cloud properties and icing indices derived from the Geostationary Operational Environmental Satellite (GOES) with the aircraft in situ measurements of several cloud properties during campaigns and some of the The comparisons include cloud phase, particle size, icing intensity, base and top altitudes, temperatures, and liquid water path. The results of this study are crucial for developing a more reliable and objective icing product from satellite data. This icing product, currently being derived from GOES data over the USA, is an important complement to more conventional products based on forecasts, and PIREPS.

Nguyen, Louis↗

A Mission to Observe Ice in Clouds from Space

To date there have been multiple satellite missions to observe and retrieve cloud top properties and the liquid in, and precipitation from, clouds. There are currently a few missions that attempt to measure cloud ice properties as a byproduct of other observations. However, we do not yet quantitatively understand the processes that control the water budget of the upper troposphere where ice is the predominant phase, and how these processes are linked to precipitation processes and the radiative energy budget. The ice in clouds either melts into rain or is detrained, and persists, as cirrus clouds affecting the hydrological and energy cycle, respectively. Fully modeling the Earth's climate and improving weather and climate forecasts requires accurate satellite measurements of various cloud properties at the temporal and spatial scales of cloud processes. The uncertainty in knowledge of these ice characteristics is reflected in the large discrepancies in model simulations of the upper tropospheric water budget. Model simulations are sensitive to the partition of ice between precipitation and outflow processes, i.e., to the parameterization of ice clouds and ice processes. This presentation will describe the Submillimeter-wave InfraRed Ice Cloud Experiment (SIRICE) concept, a satellite mission designed to acquire global Earth radiance measurements in the infrared and submillimeter-wave region (183-874 GHz). If successful, this mission will bridge the measurement gap between microwave sounders and shorter-wavelength infrared and visible sensors. The brightness temperatures at submillimeter-wave frequencies are especially sensitive to cirrus ice particle sizes (because they are comparable to the wavelength). This allows for more accurate ice water path estimates when multiple channels are used to probe into the cloud layers. Further, submillimeter wavelengths offer simplicity in the retrieval algorithms because they do not probe into the liquid and near surface portions of clouds, thus requiring only one term of the radiative transfer equation (ice scattering) to relate brightness temperatures to ice. Scientific justification and the SIRICE approach to measuring ice water path and particle size that span a range encompassing both the hydrologically active and radiatively active components of cloud systems will be presented.

Ackerman, S.↗

Calculations of the variability of ice cloud radiative properties at selected solar wavelengths

This study shows that there is surprising little difference in values of reflectance, absorptance, and transmittance for many of the intermediate-size particle spectra. Particle size distributions with mode radii ranging from approximately 50 to 300 microns, irrespective of particle shape and nearly independent of the choice of size distribution representation, give relatively similar flux values. The very small particle sizes, however, have significantly larger values of reflectance and transmittance with corresponding smaller values of absorptance than do the larger particle sizes. The very large particle modes produce very small values of reflectance and transmittance along with very large values of absorptance. Such variations are particularly noticeable when plotted as a function of wavelength.

Welch, R. M.↗

Comparison of the CALIPSO Level 3 Ice Cloud Product with the DARDAR and 2C-ICE products

Understanding the vertical distribution of ice clouds is crucial for climate modeling and weather forecasting. Since its launch to space in 2006, the Cloud-Aerosol Lidar with Orthogonal Polarization instrument (CALIOP) onboard the CALIPSO spacecraft has been providing unprecedented high-quality profiles of ice clouds, especially optically thin cirrus clouds, during both day and night, on a global scale. Recently the lidar science working group at the NASA Langley Research Center delivered a level 3 (L3) ice cloud product which reports monthly statistics of ice cloud extinction coefficient and ice water content on a uniform 3-dimensional spatial grid. This presentation compares the ice cloud climatology derived from this product with two other ice cloud products, namely the raDAR/liDAR(DARDAR) ice cloud product and the CloudSat-CALIPSO Ice Cloud Property Product (2C-ICE). Using processing similar to the CALIPSO L3 product, granules of DARDAR and 2C-ICE data have been processed into monthly statistics for a better comparison. Similarities and differences will be presented and discussed. The findings illustrate the strengths of the different products and help to identify which product might be most appropriate for a given research topic.

Xia Cai↗

Dependence of Mass–Dimensional Relationships on Median Mass Diameter

Retrievals of ice cloud properties require accurate estimates of ice particle mass. Empirical mass–dimensional ( m – D ) relationships in the form m = a D b are widely used and usually universally applied across the complete range of particle sizes. For the first time, the dependence of a and b coefficients in m–D relationships on median mass diameter ( D mm ) is studied. Using combined cloud microphysical data collected during the Olympic Mountains Experiment and coincident observations from Airborne Precipitation Radar Third Generation, D mm -dependent ( a , b ) coefficients are derived and represented as surfaces of equally plausible solutions determined by some tolerance in the chi-squared difference χ 2 that minimizes the difference between observed and retrieved radar reflectivity. Robust dependences of a and b on D mm are shown with both parameters significantly decreasing with D mm , leading to smaller effective densities for larger D mm ranges. A universally applied constant m–D relationship overestimates the mass of large aggregates when D mm is between 3–6 mm and temperatures are between −15–0 °C. Multiple m–D relations should be applied for different D mm ranges in retrievals and simulations to account for the variability of particle sizes that are responsible for the mass and thus for the variability of particle shapes and densities.

54 ENVIRONMENTAL SCIENCES↗

A Sample of What We Have Learned from A-Train Cloud Measurements

The A-train active sensors CloudSat and CALIPSO provide detailed information about cloud vertical structure. Coarse vertical information can also be obtained from a combination of passive sensors (e.g. cloud liquid water content from AMSR-E, cloud ice properties from MLS and HIRDLS, cloud-top pressure from MODIS and AIRS, and UVNISINear IR absorption and scattering from OMI, MODIS, and POLDER). In addition, the wide swaths of instruments such as MODIS, AIRS, OMI, POLDER, and AMSR-E can be exploited to create estimates of the three-dimensional cloud extent. We will show how data fusion from A-train sensors can be used, e.g., to detect and map the presence of multiple layer/phase clouds. Ultimately, combined cloud information from Atrain instruments will allow for estimates of heating and radiative flux at the surface as well as UV/VIS/Near IR trace-gas absorption at the overpass time on a near-global daily basis. CloudSat has also dramatically improved our interpretation of visible and UV passive measurements in complex cloudy situations such as deep convection and multiple cloud layers. This has led to new approaches for unique and accurate constituent retrievals from A-train instruments. For example, ozone mixing ratios inside tropical deep convective clouds have recently been estimated using the Aura Ozone Monitoring Instrument (OMI). Field campaign data from TC4 provide additional information about the spatial variability and origin of trace-gases inside convective clouds. We will highlight some of the new applications of remote sensing in cloudy conditions that have been enabled by the synergy between the A-train active and passive sensors.

Joiner, Joanna↗

A Machine Learning Framework for Predicting Microphysical Properties of Ice Crystals From Cloud Particle Imagery

The microphysical properties of ice crystals are important because they significantly alter the radiative properties and spatiotemporal distributions of clouds, which in turn strongly affect Earth's climate. However, it is challenging to measure key properties of ice crystals, such as mass or morphological features. Here, we present a proof-of-concept framework for predicting three-dimensional (3D) microphysical properties of ice crystals from in situ two-dimensional (2D) imagery. First, we computationally generated synthetic ice crystals using 3D modeling software along with geometric parameters estimated from the 2021 Ice Cryo-Encapsulation Balloon (ICEBall) field campaign. Then, we used synthetic crystals to train machine learning (ML) models to predict effective density ($ρ_e$), effective surface area ($A_e$), and number of bullets ($N_b$) from synthetic rosette imagery. On unseen synthetic images, our ML models accurately predicted ice crystal properties. ResNet-18 performed best, achieving $R^2$ values of 0.99 and 0.98 for $ρ_e$ and $A_e$, respectively, and MAE of 0.10 for mathematical equation in single view tasks. Stereo view ResNet-18 further reduced RMSE by 40% for $ρ_e$ and $A_e$ and reduced MAE by 0.08 for $N_b$. This work provides a novel ML-driven framework for estimating ice microphysical properties from in situ imagery, which will allow for downstream constraints on microphysical parameterizations, such as the mass-size relationship.

Ko, J. [Columbia Univ., New York, NY (United State↗

The Influence of Sea ice on Arctic Cloud Properties: What Can We Learn by Applying a In Situ Observational Strategy to Satellite Data?

Sea ice is declining because of anthropogenic climate change. This change alters many aspects of the Arctic climate system, including the way that the surface and atmosphere interact. Atmosphere-surface coupling processes represent an important cloud feedback mechanism that can alter the Arctic surface energy budget. For the Arctic, it has been hypothesized that a reduction in sea ice cover could lead to an increase in clouds. If this process were to occur as originally hypothesized, sea ice loss in all seasons would lead to an increase in clouds. Recent observational studies find a cloud response to sea ice loss in non-summer months and no cloud response in summer months. However, previous studies rely on inter-annual variability and reanalysis to control for the influence of meteorology, reducing the confidence in the resulting conclusions. We adopt a phenomenological, event-based approach that does not need to use meteorological reanalysis. The approach analyzes cloud properties derived from CALIPSO-CloudSat over sea ice and adjacent ice-free footprints by compositing individual satellite ground tracks that cross the Arctic sea ice edge. The underlying assumption, which we verify, is that footprints that are close to each other in space and time experience similar large-scale meteorological conditions. Our results show larger cloud fraction and more cloud liquid water over ice-free than over sea ice footprints and provide additional evidence for a seasonal dependence of cloud-sea ice coupling that is in line with previous work. We find a different result where the maximum cloud property differences between sea ice and ice-free ocean occurs in spring, not fall as earlier studies suggest. We argue that these cloud differences between sea ice and ice-free ocean are primarily caused by the influence of the surface type on the thermodynamic stability of the lower troposphere and not principally from an increase in surface evaporation. In addition, we explore the sensitivity of these results to marginal ice zone width, season, Atlantic vs. Pacific sector, and the cloud property dependence on the distance from the sea ice edge. Overall, our results provide further evidence that cloud-sea ice coupling processes are not offsetting the observed surface energy budget perturbation due to sea ice loss in summer; thus, the cloud response to declining sea ice appears to contribute to amplified Arctic warming.

Patrick C Taylor↗

Overview and Statistical Analysis of Boundary Layer Clouds and Precipitation Over the Western North Atlantic Ocean

Due to their fast evolution and large natural variability in macro- and microphysical properties, the accurate representation of boundary layer clouds in current climate models remains a challenge. One of the regions with large intermodel spread in the Coupled Model Intercomparison Project Phase 6 ensemble is the western North Atlantic Ocean. Here, statistically representative in situ measurements can help to develop and constrain the parameterization of clouds in global models. To this end, we performed comprehensive measurements of boundary layer clouds, aerosol, trace gases, and radiation in the western North Atlantic Ocean during the NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) mission. In total, 174 research flights with 574 flight hours for cloud and precipitation measurements were performed with the HU-25 Falcon during three winter (February–March 2020, January–April 2021, and November 2021–March 2022) and three summer seasons (August–September 2020, May–June 2021, and May–June 2022). Here we present a statistical evaluation of 16 140 individual cloud events probed by the fast cloud droplet probe and the two-dimensional stereo cloud probe during 155 research flights in a representative and repetitive flight strategy allowing for robust statistical data analyses. We show that the vertical profiles of distributions of the liquid water content and the cloud droplet effective diameter (ED) increase with altitude in the marine boundary layer. Due to higher updraft speeds, higher cloud droplet number concentrations (N liquid ) were measured in winter compared to summer despite lower cloud condensation nucleus abundance. Flight cloud cover derived from statistical analysis of in situ data is reduced in summer and shows large variability. This seasonal contrast in cloud coverage is consistent with a dominance of a synoptic pattern in winter that favors conditions for the formation of stratiform clouds at the western edge of cyclones (post-cyclonic). In contrast, a dominant summer anticyclone is concomitant with the occurrence of shallow cumulus clouds and lower cloud coverage. The evaluation of boundary layer clouds and precipitation in the N liquid ED phase space sheds light on liquid, mixed-phase, and ice cloud properties and helps to categorize the cloud data. Ice and liquid precipitation, often masked in cloud statistics by a high abundance of liquid clouds, is often observed throughout the cloud. The ACTIVATE in situ cloud measurements provide a wealth of cloud information useful for assessing airborne and satellite remote-sensing products, for global climate and weather model evaluations, and for dedicated process studies that address precipitation and aerosol–cloud interactions.

Aerosol↗

Simulations of Infrared Radiances Over a Deep Convective Cloud System Observed During TC4- Potential for Enhancing Nocturnal Ice Cloud Retrievals

Retrievals of ice cloud properties using infrared measurements at 3.7, 6.7, 7.3, 8.5, 10.8, and 12.0 microns can provide consistent results regardless of solar illumination, but are limited to cloud optical thicknesses tau < approx.6. This paper investigates the variations in radiances at these wavelengths over a deep convective cloud system for their potential to extend retrievals of tau and ice particle size D(sub e) to optically thick clouds. Measurements from the Moderate Resolution Imaging Spectroradiometer Airborne Simulator--ASTER, the Scanning High-resolution Interferometer Sounder, the Cloud Physics Lidar (CPL), and the Cloud Radar System (CRS) aboard the NASA ER-2 aircraft during the NASA TC4 (Tropical Composition, Cloud and Climate Coupling) experiment flight during 5 August 2007, are used to examine the retrieval capabilities of infrared radiances over optically thick ice clouds. Simulations based on coincident in-situ measurements and combined cloud tau from CRS and CPL measurements are comparable to the observations. They reveal that brightness temperatures at these bands and their differences (BTD) are sensitive to tau up to approx.20 and that for ice clouds having tau > 20, the 3.7 - 10.8 microns and 3.7 - 6.7 microns BTDs are the most sensitive to D(sub e). Satellite imagery appears consistent with these results. Keywords: clouds; optical depth; particle size; satellite; TC4; multispectral thermal infrared

CRS and CPL↗

Radiative Properties of Cirrus Clouds in the Infrared (8-13 microns) Spectral Region

Atmospheric radiation in the infrared (IR) 8-13 microns spectral region contains a wealth of information that is very useful for the retrieval of ice cloud properties from aircraft or space-borne measurements. To provide the scattering and absorption properties of nonspherical ice crystals that are fundamental to the IR retrieval implementation, we use the finite-difference time domain (FDTD) method to solve for the extinction efficiency, single-scattering albedo, and the asymmetry parameter of the phase function for ice crystals smaller than 40 microns. For particles larger than this size, the improved geometric optics method (IGOM) can be employed to calculate the asymmetry parameter with an acceptable accuracy, provided that we properly account for the inhomogeneity of the refracted wave due to strong absorption inside the ice particle. A combination of the results computed from the two methods provides the asymmetry parameter for the entire practical range of particle sizes between 1 micron and 10000 microns over wavelengths ranging from 8 microns to 13 microns. For the extinction and absorption efficiency calculations, several methods including the IGOM, Mie solution for equivalent spheres (MSFES), and the anomalous diffraction theory (ADT) can lead to a substantial discontinuity in comparison with the FDTD solutions for particle sizes on the order of 40 microns. To overcome this difficulty, we have developed a novel approach called the stretched scattering potential method (SSPM). For the IR 8-13 microns spectral region, we show that SSPM is a more accurate approximation than ADT, MSFES, and IGOM. The SSPM solution can be further refined numerically. Through a combination of the FDTD and SSPM, we have computed the extinction and absorption efficiency for hexagonal ice crystals with sizes ranging from 1 to 10000 microns at 12 wavelengths between 8 and 13 microns Calculations of the cirrus bulk scattering and absorption properties are performed for 30 size distributions obtained from various field campaigns for midlatitude and tropical cirrus cloud systems. Parameterization of these bulk scattering properties is carried out by using second-order polynomial functions for the extinction efficiency and the single-scattering albedo and the power law expression for the asymmetry parameter. We note that the volume-normalized extinction coefficient can be separated into two parts: one is inversely proportional to effective size and is independent of wavelength, and the other is the wavelength-dependent effective extinction efficiency. Unlike conventional parameterization efforts, the present parameterization scheme is more accurate because only the latter part of the volume-normalized extinction coefficient is approximated in terms of an analytical expression. After averaging over size distribution, the single-scattering albedo is shown to decrease with an increase in effective size for wavelengths shorter than 10.0 microns whereas the opposite behavior is observed for longer wavelengths. The variation of the asymmetry parameter as a function of effective size is substantial when the effective size is smaller than 50 microns. For effective sizes larger than 100 microns, the asymmetry parameter approaches its asymptotic value. The results derived in this study can be useful to remote sensing applications involving IR window bands under cirrus cloud conditions.

Yang, Ping↗

CloudSat-Constrained Cloud Ice Water Path and Cloud Top Height Retrievals from MHS 157 and 183.3 GHz Radiances

Ice water path (IWP) and cloud top height (ht) are two of the key variables in determining cloud radiative and thermodynamical properties in climate models. Large uncertainty remains among IWP measurements from satellite sensors, in large part due to the assumptions made for cloud microphysics in these retrievals. In this study, we develop a fast algorithm to retrieve IWP from the 157, 183.3+/-3 and 190.3 GHz radiances of the Microwave Humidity Sounder (MHS) such that the MHS cloud ice retrieval is consistent with CloudSat IWP measurements. This retrieval is obtained by constraining the empirical forward models between collocated and coincident measurements of CloudSat IWP and MHS cloud-induced radiance depression (Tcir) at these channels. The empirical forward model is represented by a lookup table (LUT) of Tcir-IWP relationships as a function of ht and the frequency channel.With ht simultaneously retrieved, the IWP is found to be more accurate. The useful range of the MHS IWP retrieval is between 0.5 and 10 kg/sq m, and agrees well with CloudSat in terms of the normalized probability density function (PDF). Compared to the empirical model, current operational radiative transfer models (RTMs) still have significant uncertainties in characterizing the observed Tcir-IWP relationships. Therefore, the empirical LUT method developed here remains an effective approach to retrieving ice cloud properties from the MHS-like microwave channels.

cloud top height↗

Millimeter- and Submillimeter-Wave Remote Sensing Using Small Satellites

Cloud ice properties and processes play fundamental roles in atmospheric radiation and precipitation. Limited knowledge and poor representation of clouds in global climate models have led to large uncertainties about cloud feedback processes under climate change. Ice clouds have been used as a tuning parameter in the models to force agreement with observations of the radiation budget at the top of the atmosphere, and precipitation at the bottom. The lack of ice cloud measurements has left the cloud processes at intermediate altitudes unconstrained. Millimeter (mm) and submillimeter (submm)-wave radiometry is widely recognized for its potential to fill the cloud measurement gap in the middle and upper troposphere. Analyses have shown that channels from 183900 GHz offer good sensitivity to ice cloud scattering and can provide ice water path (IWP) products to an accuracy of 25 by simultaneously retrieving ice particle size (Dme) and IWP. Therefore, it is highly desirable to develop a cost-effective, compact mm/submm-wave instrument for cloud observations that can be deployed on future small satellites.This paper presents a conceptual study for a mm/submm-wave instrument for multispectral measurements of ice clouds. It discusses previous work at these frequencies by NASA Goddard Space Flight Center (GSFC) and the current instrument study, as well as receiver architectures and their anticipated performance. And finally, it describes a microsatellite prototype intended for use with this mm/submm-wave instrument.

small satellites↗

Effective radiative forcing of anthropogenic aerosols in E3SM version 1: historical changes, causality, decomposition, and parameterization sensitivities

Abstract. The effective radiative forcing of anthropogenic aerosols (ERFaer) is an important measure of the anthropogenic aerosol effects simulated by a global climate model. Here we analyze ERFaer simulated by the E3SM version 1 (E3SMv1) atmospheric model using both century-long free-running atmosphere–land simulations and short nudged simulations. We relate the simulated ERFaer to characteristics of the aerosol composition and optical properties, and we evaluate the relationships between key aerosol and cloud properties. In terms of historical changes from the year 1870 to 2014, our results show that the global mean anthropogenic aerosol burden and optical depth increase during the simulation period as expected, but the regional averages show large differences in the temporal evolution. The largest regional differences are found in the emission-induced evolution of the burden and optical depth of the sulfate aerosol: a strong decreasing trend is seen in the Northern Hemisphere high-latitude region after around 1970, while a continued increase is simulated in the tropics. The relationships between key aerosol and cloud properties (relative changes between pre-industrial and present-day conditions) also show evident changes after 1970, diverging from the linear relationships exhibited for the period of 1870–1969. In addition to the regional differences in the simulated relationships, a reduced sensitivity in cloud droplet number and other cloud properties to aerosol perturbations is seen when the aerosol perturbation is large. Consequently, the global annual mean ERFaer magnitude does not increase after around 1970. The ERFaer in E3SMv1 is relatively large compared to the recently published multi-model estimates; the primary reason is the large indirect aerosol effect (i.e., through aerosol–cloud interactions). Compared to other models, E3SMv1 features large relative changes in the cloud droplet effective radius in response to aerosol perturbations. Large sensitivity is also seen in the liquid cloud optical depth, which is determined by changes in both the effective radius and liquid water path. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 are found to have a strong correlation, as the evolution of anthropogenic sulfate aerosols affects both the liquid cloud formation and the homogeneous ice nucleation in cirrus clouds (that causes a large effect on longwave ERFaer). As suggested by a previous study, the large ERFaer appears to be one of the reasons why the model cannot reproduce the observed global mean temperature evolution in the second half of the 20th century. Sensitivity simulations are performed to understand which parameterization and/or parameter changes have a large impact on the simulated ERFaer. The ERFaer estimates in E3SMv1 for the shortwave and longwave components are sensitive to the parameterization changes in both liquid and ice cloud processes. When the parameterization of ice cloud processes is modified, the top-of-model forcing changes in the shortwave and longwave components largely offset each other, so the net effect is negligible. This suggests that, to reduce the magnitude of the net ERFaer, it would be more effective to reduce the anthropogenic aerosol effect through liquid or mixed-phase clouds.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Effective radiative forcing of anthropogenic aerosols in E3SMv1: historical changes, causality, decomposition, and parameterization sensitivities

The effective radiative forcing of anthropogenic aerosols (ERF aer ) is an important measure of the anthropogenic aerosol effects simulated by a global climate model. Here we analyze ERF aer simulated by the E3SMv1 atmosphere model using both century-long free-running atmosphere-land simulations and short nudged simulations. We relate the simulated ERF aer to characteristics of the aerosol composition and optical properties, and evaluate the relationships between key aerosol and cloud properties. In terms of historical changes from the year 1870 to 2014, our results show that the global mean anthropogenic aerosol burden and optical depth increase during the simulation period as expected, but the regional averages show large differences in the temporal evolution. The largest regional differences are found in the emission-induced evolution of the burden and optical depth of the sulfate aerosol: a strong decreasing trend is seen in the Northern Hemisphere high-latitude region after around 1970, while a continued increase is simulated in the tropics. Consequently, although the global mean anthropogenic aerosol burden and optical depth increase from 1870 to 2014, the ERF aer magnitude does not increase after around year 1970. The relationships between key aerosol and cloud properties (relative changes between preindustrial and present-day conditions) also show evident changes after 1970, diverging from the linear relationships exhibited for the period from 1870 to 2014. The ERF aer in E3SMv1 is relatively large compared to the recently published multi-model estimates; the primary reason is the large indirect aerosol effect (i.e., through aerosol-cloud interactions). Compared to other models, E3SMv1 features a stronger sensitivity of the cloud droplet effective radius to changes in the cloud droplet number concentration. Large sensitivity is also seen in the liquid cloud optical depth, which is determined by changes in both the effective radius and liquid water path. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 are found to have a strong correlation, as the evolution of anthropogenic sulfate aerosols affects both the liquid cloud formation and the homogeneous ice nucleation in cirrus clouds. The ERF aer estimates in E3SMv1 for the shortwave and longwave components are sensitive to the parameterization changes in both liquid and ice cloud processes. When the parameterization of ice cloud processes is modified, the top-of-atmosphere forcing changes in the shortwave and longwave components largely offset each other, so the net effect is negligible. This suggests that, to reduce the magnitude of the net ERF aer , it would be more effective to reduce the anthropogenic aerosol effect through liquid or mixed-phase clouds.

54 ENVIRONMENTAL SCIENCES↗

Advancing Technologies for Climate Observation

Climate research needs Accurate global cloud ice measurements Cloud ice properties are fundamental controlling variables of radiative transfer and precipitation Cost-effective, sensitive instruments for diurnal and wide-swath coverage Mature technology for space remote sensing IceCube objectivesDevelop and validate a flight-qualified 883 GHz receiver for future use in ice cloud radiometer missions Raise TRL (57) of 883 GHz receiver technology Reduce instrument cost and risk by developing path to space for COTS sub-mm-wave receiver systems Enable remote sensing of global cloud ice with advanced technologies and techniques

radiative transfer↗

Simulations of Infrared Radiances Over a Deep Convective Cloud System Observed During TC4: Potential for Enhancing Nocturnal Ice Cloud Retrievals

Retrievals of ice cloud properties using infrared measurements at 3.7, 6.7, 7.3, 8.5, 10.8, and 12.0 microns can provide consistent results regardless of solar illumination, but are limited to cloud optical thicknesses tau < approx.6. This paper investigates the variations in radiances at these wavelengths over a deep convective cloud system for their potential to extend retrievals of tau and ice particle size D(sub e) to optically thick clouds. Measurements from the Moderate Resolution Imaging Spectroradiometer Airborne Simulator--ASTER, the Scanning High-resolution Interferometer Sounder, the Cloud Physics Lidar (CPL), and the Cloud Radar System (CRS) aboard the NASA ER-2 aircraft during the NASA TC4 (Tropical Composition, Cloud and Climate Coupling) experiment flight during 5 August 2007, are used to examine the retrieval capabilities of infrared radiances over optically thick ice clouds. Simulations based on coincident in-situ measurements and combined cloud tau from CRS and CPL measurements are comparable to the observations. They reveal that brightness temperatures at these bands and their differences (BTD) are sensitive to tau up to approx.20 and that for ice clouds having tau > 20, the 3.7 - 10.8 microns and 3.7 - 6.7 microns BTDs are the most sensitive to D(sub e). Satellite imagery appears consistent with these results. Keywords: clouds; optical depth; particle size; satellite; TC4; multispectral thermal infrared

Minnis, Patrick↗

Asymmetries in cloud microphysical properties ascribed to sea ice leads via water vapour transport in the central Arctic

To investigate the influence of sea ice openings like leads on wintertime Arctic clouds, the air mass transport is exploited as a heat and humidity feeding mechanism which can modify Arctic cloud properties. Cloud microphysical properties in the central Arctic are analysed as a function of sea ice conditions during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition in 2019–2020. The Cloudnet classification algorithm is used to characterize the clouds based on remote sensing observations and the atmospheric thermodynamic state from the observatory on board the research vessel (RV) Polarstern. To link the sea ice conditions around the observational site with the cloud observations, the water vapour transport (WVT) being conveyed towards RV Polarstern has been utilized as a mechanism to associate upwind sea ice conditions with the measured cloud properties. This novel methodology is used to classify the observed clouds as coupled or decoupled to the WVT based on the location of the maximum vertical gradient of WVT height relative to the cloud-driven mixing layer. Only a conical sub-sector of sea ice concentration (SIC) and the lead fraction (LF) centred on the RV Polarstern location and extending up to 50 km in radius and with an azimuth angle governed by the time-dependent wind direction measured at the maximum WVT is related to the observed clouds. We found significant asymmetries for cases when the clouds are coupled or decoupled to the WVT and selected by LF regimes. Liquid water path of low-level clouds is found to increase as a function of LF, while the ice water path does so only for deep precipitating systems. Clouds coupled to WVT are found to generally have a lower cloud base and larger thickness than decoupled clouds. Thermodynamically, for coupled cases the cloud-top temperature is warmer and accompanied by a temperature inversion at the cloud top, whereas the decoupled cases are found to be closely compliant with the moist adiabatic temperature lapse rate. The ice water fraction within the cloud layer has been found to present a noticeable asymmetry when comparing coupled versus decoupled cases. This novel approach of coupling sea ice to cloud properties via the WVT mechanism unfolds a new tool to study Arctic surface–atmosphere processes. With this formulation, long-term observations can be analysed to enforce the statistical significance of the asymmetries. Furthermore, our results serve as an opportunity to better understand the dynamic linkage between clouds and sea ice and to evaluate its representation in numerical climate models for the Arctic system.

54 ENVIRONMENTAL SCIENCES↗