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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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A colinear Second-Harmonic Orthogonal Polarized (SHOP) interferometer diagnostic capable of making electron areal density measurements of plasmas formed in Magnetically Insulated Transmission Lines (MITLs) has been developed.
The magnetic dipole strength 𝐵(𝑀1 ↑) of 40 Ar was measured in the excitation energy range between 9.3 and 10.3 MeV. The nuclear resonance fluorescence technique was used with monoenergetic, linearly polarized incident photon beams. The new data increase the known 𝐵(𝑀1 ↑) strength in this important excitation energy range by a factor of 2, resulting in an equivalent increase of the calculated neutral current neutrino cross section of 40 Ar . This observation is of special interest for liquid-argon (LAr)-based neutrino detectors. 𝐵(𝑀1 ↑) strength has not been found between 10.3 and 11.7 MeV excitation energy. In conclusion, with the new data, a more reliable detection capability of the large Deep Underground Neutrino Experiment LAr detectors can be derived for potential core-collapse supernova neutrinos via the neutral current interaction.
In this paper, we study the electrodeposited Ni—Pt magnetic wires, exploring the mechanisms by which changes in geometry and composition influence the local magnetic structure. The samples were prepared by electrodeposition, their elemental composition was analyzed by energy dispersive X-ray spectroscopy, and phase analysis was carried out by an X-ray diffraction measurement. Magnetic force microscopy measurements, and magnetic force microscopy measurements in magnetic field were carried out to study the domain morphology of the prepared samples. Magnetization characteristics were measured via vibrating sample magnetometry mode of a superconducting quantum interference device. Here, the results were analyzed and compared with micromagnetic simulations. It is shown that a strong perpendicular magnetic anisotropy is responsible for the characteristic checkerboard-like surface magnetization patterns, which can be tuned by geometrical constriction and Ni content. Understanding these relationships provides insights into the design of magnetic materials with tailored properties for advanced applications, like magnetic sensors.
Atomically precise ligated nanoclusters (NC) are promising cluster-based materials with novel molecular architectures and tunable magnetic properties. Herein, the synthesis and characterization of a nickel sulfide NC Ni 3 S 3 H(PEt 3 ) 5 (PEt 3 = triethylphosphine) with distinct magnetic properties are reported. Magnetization measurements reveal its magnetic moment of 1.5 µ B in the solid phase, consistent with the existence of one unpaired electron predicted by density functional theory (DFT) calculations. Additionally, experimental measurements indicate the presence of ferromagnetic ordering within each Ni 3 S 3 H(PEt 3 ) 5 NC and strong coercivity at temperatures below 20 K. Ion mobility-mass spectrometry is employed in conjunction with DFT calculations and collision cross-section simulations to investigate the structure of the isolated Ni 3 S 3 H(PEt 3 ) 5 . Theoretical studies show that [Ni 3 S 3 H(PEt 3 ) 5 ] + has a planar Ni 3 S 3 core where three Ni atoms are arranged in a triangle with three bridging S atoms residing in the same plane. This structure is preserved in both solution and solid phases, which is confirmed by spectroscopic studies of Ni 3 S 3 H(PEt 3 ) 5 . Additionally, DFT calculations indicate that all spins at the Ni sites are aligned parallel, confirming the presence of ferromagnetic coupling. Overall, this study provides key insights into the structure and magnetic properties of Ni 3 S 3 H(PEt 3 ) 5 , which will facilitate the design of new NC-based magnetic materials.
The goal of this Exploratory Express project was to explore the possibility of tunable ferromagnetism in Mn or Cr incorporated epitaxial Ga 2 O 3 films. Tunability of magnetic properties can enable novel applications in spintronics, quantum computing, and magnetism-based logics by allowing control of magnetism down to the nanoscale. Carriers (electrons or holes) mediated ferromagnetic ordering in semiconductor can lead to tunable ferromagnetism by leveraging the tunability of carrier density with doping level, gate electric field, or optical pumping of the carriers. The magnetic ions (Cr or Mn) in Ga 2 O 3 act as localized spin centers which can potentially be magnetically coupled through conduction electrons to enable ferromagnetic ordering. Here we investigated tunable ferromagnetism in beta Ga 2 O 3 semiconductor host with various n-doping levels by incorporating 2.4 atomic percent Mn or Cr. The R&D approach involved growth of epitaxial Ga 2 O 3 film on sapphire or Ga 2 O 3 substrate, implantation of Mn or Cr ions, annealing of the samples post implantation, and magnetic measurements. We studied magnetic behavior of Mn:Ga 2 O 3 as a function of different n-doping levels and various annealing temperatures. The vibrating sample magnetometry (VSM) measurement exhibited strong ferromagnetic signals from the annealed Mn:Ga 2 O 3 sample with n-doping level of 5E19 cm -3 . This ferromagnetic behavior disappears from Mn:Ga 2 O 3 when the n-doping level is reduced to 5E16 cm -3 . Although these results are to be further verified by other measurement schemes due to the observation of background ferromagnetism from the growth substrate, these results indicate the possibility of tunable ferromagnetism in Mn:Ga 2 O 3 mediated by conduction electrons.
The x-ray diffraction, Raman, and infrared spectroscopies and magnetic measurements were used to explore the correlated changes of the structure, lattice dynamics, and magnetic properties of the LuFeO3 nanoparticles, which appear in dependence on their sintering temperature. We revealed a gradual substitution of the hexagonal phase by the orthorhombic phase in the nanoparticles, with sintering temperature increasing from 700 to 1100 °C. The origin and stability of the hexagonal phase in the LuFeO3 nanoparticles are of the special interest, because the nanoparticles in the phase can be a room-temperature multiferroic with a weak ferromagnetic and pronounced structural and ferroelectric long-range ordering. The antiferromagnetic and nonpolar orthorhombic phase is more stable in the bulk LuFeO3. To define the ranges of the hexagonal phase stability, we determine the bulk and interface energy densities of different phases from the comparison of the Gibbs model with experimental results. Using effective parameters of the Gibbs model, we predict the influence of size effects and temperature on the structural and polar properties of the LuFeO3 nanoparticles. Analysis of the obtained results shows that the combination of the x-ray diffraction, Raman and infrared spectroscopies, magnetic measurements, and theoretical modeling of structural and polar properties allows us to establish the interplay between the phase composition, lattice dynamics, and multiferroic properties of the LuFeO3 nanoparticles prepared under different conditions.
Quantum two-dimensional materials, including ultrathin superconducting films, are of great current research interest. These films are typically fabricated under ultra-high vacuum (UHV) conditions and are sensitive to the environment—prone to oxidation and contamination when exposed to the atmosphere. This hampers the study of their intrinsic properties by standard ex situ techniques. Here, we present a variable-temperature mutual inductance probe system integrated under UHV with molecular beam epitaxy (MBE) synthesis and low-energy electron microscopy, enabling nondestructive in situ characterization of superconducting thin films. The system employs a reflection-type configuration and reaches a low temperature (∼4 K) using a high-cooling-power, vibration-isolated cryocooler. In conclusion, we demonstrate the system performance by measuring the superconducting critical temperature in a copper-oxide thin film.
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Sawtooth crashes on tokamak plasmas exhibit relaxation much faster than resistive time scales via a mechanism not fully understood. Using core magnetic measurements from the Radial Interferometer-Polarimeter (RIP) diagnostic on the DIII-D tokamak, Grad–Shafranov equilibria constrained by internal magnetic measurements that have high time resolution (<1μs) can be computed, allowing analysis of how equilibrium parameters such as safety factor q, current density J, and parallel electric field E ∥ , particularly on-axis, evolve. At the sawtooth crash, on-axis safety factor q 0 is observed to rise by 5% but remain below 1 throughout the cycle, and on-axis current density J 0 is observed to drop by 5%. On-axis parallel electric field E ∥ (0) is found to be balanced by ηJ 0 (resistivity times on-axis current density) except during the 200 µs crash period, where E ∥ (0) reaches 22 V m –1 , exceeding ηJ 0 by a factor of more than 2000. These first measurements in tokamak plasmas verify that generalized Ohm's law is not balanced during the crash by resistive effects alone; this is a finding expected due to the relaxation being much faster than resistive timescales. As a result, measurement of the electric field during the tokamak sawtooth serves to illuminate the physical mechanisms at work.
Pegasus-III is an ultralow aspect ratio spherical tokamak providing a dedicated US experiment for comparative solenoid-free startup studies. A new magnetic diagnostic suite for equilibrium and low frequency (<200 kHz) magnetohydrodynamic mode analysis has been installed. These new diagnostics address the significant challenges of measuring magnetic field in a high noise environment with the majority constrained to fit in an 8 mm diagnostic gap on the high field side. Electrostatic switching noise generated by the 16 independent current feedback-controlled power supplies produces dV cm /dt ~ 1 kV/μs and volt level common mode noise on the magnetics. Immunity to this switching noise is accomplished through differential signal runs and signal processing, along with end-to-end electromagnetic interference shielding. The magnetic measurements are simultaneously digitized at 1 MHz and conditioned by precision 8 pole Butterworth filters with a corner frequency of 200 kHz to prevent aliasing down to the 16-bit level over the full passband. Ex-vessel calibrations of the B p coils were completed with a typical uncertainty of <0.5%. Stray toroidal field pickup from coil misalignment or positioning errors is corrected using a physics-based model. Comparisons of the corrected measurements to modeling agree to within 1.3% on average. This is within the 1.5% measurement uncertainty that a sensitivity analysis determined is needed for accurate fast boundary and equilibrium reconstruction.
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Magnets are integral components of particle accelerators, with different multipoles used to perform various beam conditioning functions, like steering and focusing. Testing accelerator magnets to ensure compliance with specification is a crucial step of fabrication. One of the most popular techniques for verifying magnetic field strength and integrity is the harmonic coil probe. Harmonic coil probes are comprised of passive loops that are rotated around the aperture of a magnet and are used to measure magnetic flux. Oftentimes the measurements of the harmonic coil probe are affected by transverse vibrations along the axis of rotation and torsional vibrations of the position closure sensor, both causing spurious harmonics. To make matters challenging, it is difficult to distinguish between the real harmonics of the magnet and the spurious harmonics during analysis. This research explores the use of a novel configuration of harmonic coil probe, Multi-Vertex Probe (MVP), to address multiple factors that affect the accuracy and repeatability of harmonic coil probe measurement. Most of the results are based on simulation data, in which artificial torsional distortions are introduced and removed with the proposed processing method. In addition to implementing torsional vibration removal in simulation, laboratory analysis regarding the source of vibrations was performed using a pre-fabricated MVP. More specifically, various mechanical conditions were used to explore the standard deviation of main harmonic’s flux amplitude. The conditions included: coupling type (rigid or soft), rotation speed, probe starting position within magnetic field, and cabling location inside the magnetic field. Along with this, the MVP’s measured noise floor in and outside a magnetic field was quantified.
This work introduces a new current model into the EFIT code for plasma current profile reconstruction. Using this model, edge-localized current density profiles are reconstructed solely from external magnetic measurements. Quantitative comparisons show that edge current profiles obtained with the new current model align closely with those from kinetic equilibrium reconstruction. The new model enables current density reconstruction with fewer diagnostics than kinetic equilibrium reconstruction (Lao et al 1990 Nucl. Fusion 30 1035–49), demonstrating that edge-localized current density information can be obtained from external magnetic measurements only, without the help of kinetic profiles and internal diagnostics, and without using the bootstrap current model. Furthermore, with the constraints of external magnetic and MSE measurements, current profiles in full radius obtained from the new model are in good agreement with the results of kinetic equilibrium reconstruction, which not only improves the efficiency of current reconstruction but also helps avoid possible errors caused by different kinds of diagnoses. Possible applications are also discussed, and a brief analysis of the evolution of the full-radius current density is performed. Noticeable decreases in both the magnitude and gradient of the edge current around the time of ELM bursts are observed. Moreover, analysis of the full radius current density profiles ( ρ N = 0 − 1.0, ρN denotes to square root of the normalized toroidal flux) reveals that as the edge current changes, the inner current also changes following a sinusoidal-like pattern at almost all time slices during four type-I ELMs in discharge 161493. The current evolution in the inner region ( ρ N = 0.2 − 0.6) is synchronized with the boundary region ( ρ N = 0.89 − 1.0), while the intermediate region ( ρ N = 0.6 − 0.89) shows opposite behavior. This sinusoidal-like variations in full-radius current density profile indicates strong core-pedestal coupling, suggesting ELMs significantly affect core plasmas, though current changes manifest differently across radial regions.
Antiperovskite nitrides with the general formula M 3 AN have attracted significant attention due to their tunable electronic and magnetic properties. Among them are many cobalt-based compounds predicted to exhibit high thermodynamic stability and intriguing magnetic behavior. Here, we report the synthesis and magnetic characterization of epitaxial Co3ZnN thin films grown by radio frequency sputtering on SrTiO 3 (STO) and MgO substrates. X-ray diffraction confirms phase-pure (00l)-oriented films with cube-on-cube epitaxy on STO, with a c-lattice parameter of 3.752 Å. Magnetic measurements reveal clear hysteresis at 2 K with a coercive field of ∼0.11 T and a small net moment of 0.108 μ B /f.u., suggesting either a canted antiferromagnetic (AFM) or ferrimagnetic (FiM) configuration. Temperature-dependent magnetization measurements show a transition near 25 K, with strong AFM interactions with Curie–Weiss temperature (Θ) = −80.13 K. Complementary density functional theory and Monte Carlo simulations indicate a ferromagnetic (FM) ground state, with the FM–AFM energy difference decreasing systematically with increasing supercell size, consistent with competition between FM and AFM/FiM interactions. These results highlight Co3ZnN as a magnetically complex antiperovskite nitride with competing exchange interactions.
Magnetotransport measurements of Pr4Ni3O10 single crystals performed under externally applied pressures up to 73 GPa in diamond anvil cells with either KBr or Nujol oil as pressure media yield signatures of superconductivity with a maximum onset temperature of approximately 31 K. True zero resistance was not observed, consistent with a nonpercolating superconducting volume fraction. Magnetization measurements provided corroborating evidence of superconductivity, with a pressure-dependent diamagnetic signal occurring below the onset temperature, and an estimate from the absolute value of the susceptibility suggests a superconducting volume fraction on the order of 10%. We observe sample to sample variations in the magnitude and pressure dependence of 𝑇𝑐 as well as a dependence on the configuration of electrical contacts on a given sample. Possible causes of this behavior may be significant inhomogeneities in the pressure and/or damage to the samples induced by the pressure media as well as inhomogeneities in the crystals themselves. The results imply that our as-grown Pr4Ni3O10 single crystals are not bulk superconductors but that there is a minority structure present within the crystals that is indeed superconductin
A one-year experimental program was performed using the Multi-TeraWatt (MTW) laser at the Laboratory for Laser Energetics (LLE) to investigate the efficiency and physical process of laser-driven—wire THz generation. This process was evaluated as a potential high-repetition-rate source of powerful THz pulses for use in THz pulsed polarimetry of a moderate-density magnetic-confinement fusion concept developed by TAE. The goal was to develop a source for short pulses in the THz regime (150 μm wavelength) containing 10’s of mJ. The campaign tested the impact of Cu wire diameter (25, 75, 160 μm), length (250 – 750 μm), and laser irradiation orientation on THz production efficiency in comparison to 20-μm thick Cu foils. Of these targets, the 160 µm diameter, 750 µm long wires with sharpened tips and irradiated at the base were found to produce the highest energy and shortest wavelength THz pulses, exceeding 2.5 Joule/sr and meeting the requirements for the polarimetry diagnostic. The brightest THz signal was radiated in the direction of the sharpened wire tip. A combination of two models – a traveling wave antenna combined with coherent transition radiation – describes the emission pattern, pulse energy, and spectrum observed in the experiments.
A series of rare earth magnesium selenosilicates, RE3Mg 0.5 SiSe 7 (RE = Ce, Pr, Nd, Sm, Gd, Tb, Dy) were obtained as single crystal using the flux assisted boron chalcogen mixture (BCM) method. The structures of the crystals were determined by single-crystal X-ray diffraction. The RE3Mg 0.5 SiSe 7 series crystallizes in the hexagonal crystal system in the space group P6 3 . Polycrystalline powders were synthesized to perform physical property measurements. Magnetic measurements over the 2–300 K temperature range reveal that Ce 3 Mg 0.5 SiSe 7 and Gd 3 Mg 0.5 SiSe 7 exhibit paramagnetic behavior with negative Weiss constants (θ W = −14.50, θ W = −6.13 K, respectively). The optical properties of RE 3 Mg 0.5 SiSe 7 (RE = Ce, Pr, Nd, Sm, Gd) were measured by ultraviolet–visible (UV–vis) diffuse reflectance. Density functional theory (DFT) electronic structure calculations were performed. Furthermore, a second harmonic generation measurement was performed on a polycrystalline powder of Ce 3 Mg 0.5 SiSe 7 and was found to be SHG active with an efficiency of 0.11 times the standard potassium dihydrogen phosphate (KDP).
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