Results for “Measurement Campaign” — Page 2

DOE OSTI2021

A Statistical Evaluation of WRF-LES Trace Gas Dispersion Using Project Prairie Grass Measurements

In recent years, new measurement systems have been deployed to monitor and quantify methane emissions from the natural gas sector. Large-eddy simulation (LES) has complemented measurement campaigns by serving as a controlled environment in which to study plume dynamics and sampling strategies. However, with few comparisons with controlled-release experiments, the accuracy of LES for modeling natural gas emissions is poorly characterized. In this paper, we evaluate LES from the Weather Research and Forecasting (WRF) Model against Project Prairie Grass campaign measurements and surface layer similarity theory. Using WRF-LES, we simulate continuous emissions from 30 near-surface trace gas sources in two stability regimes: strong convection and weak convection. We examine the impact of grid resolutions ranging from 6.25 to 52 m in the horizontal dimension on model results. We evaluate performance in a statistical framework, calculating fractional bias and conducting Welch’s t tests. WRF-LES accurately simulates observed surface concentrations at 100 m and beyond under strong convection; simulated concentrations pass t tests in this region irrespective of grid resolution. However, in weakly convective conditions with strong winds, WRF-LES substantially overpredicts concentrations—the magnitude of fractional bias often exceeds 30%, and all but one t test fails. The good performance of WRF-LES under strong convection correlates with agreement with local free convection theory and a minimal amount of parameterized turbulent kinetic energy. The poor performance under weak convection corresponds to misalignment with Monin–Obukhov similarity theory and a significant amount of parameterized turbulent kinetic energy.

17 WIND ENERGY↗

DOE OSTI2021

Gamma spectrometry uranium isotopic analysis rodeo: Summary of GADRAS results

This report summarizes GADRAS methods and gamma spectrometry rodeo uranium isotopic analysis results for high energy resolution H3D M400 cadmium zinc telluride (CZT) and ORTEC Micro Detective high-purity germanium (HPGe) spectra of uranium isotopic standards collected at Oak Ridge National Laboratory (ORNL) and Lawrence Livermore National Laboratory (LLNL) over a two-year measurement campaign. During the campaign, measurements were performed with the detectors unshielded, side shielded, and collimated. In addition, measurements of the uranium isotopic standards were performed unshielded and shielded.

07 ISOTOPE AND RADIATION SOURCES↗

DOE OSTI2023

Limited Role of Absolute Humidity in Intraurban Heat Variability

Abstract Monitoring and understanding the variability of heat within cities is important for urban planning and public health, and the number of studies measuring intraurban temperature variability is growing. Recognizing that the physiological effects of heat depend on humidity as well as temperature, measurement campaigns have included measurements of relative humidity alongside temperature. However, the role the spatial structure in humidity, independent from temperature, plays in intraurban heat variability is unknown. Here we use summer temperature and humidity from networks of stationary sensors in multiple cities in the United States to show spatial variations in the absolute humidity within these cities are weak. This variability in absolute humidity plays an insignificant role in the spatial variability of the heat index and humidity index (humidex), and the spatial variability of the heat metrics is dominated by temperature variability. Thus, results from previous studies that considered only intraurban variability in temperature will carry over to intraurban heat variability. Also, this suggests increases in humidity from green infrastructure interventions designed to reduce temperature will be minimal. In addition, a network of sensors that only measures temperature is sufficient to quantify the spatial variability of heat across these cities when combined with humidity measured at a single location, allowing for lower-cost heat monitoring networks. Significance Statement Monitoring the variability of heat within cities is important for urban planning and public health. While the physiological effects of heat depend on temperature and humidity, it is shown that there are only weak spatial variations in the absolute humidity within nine U.S. cities, and the spatial variability of heat metrics is dominated by temperature variability. This suggests increases in humidity will be minimal resulting from green infrastructure interventions designed to reduce temperature. It also means a network of sensors that only measure temperature is sufficient to quantify the spatial variability of heat across these cities when combined with humidity measured at a single location.

Meteorology & Atmospheric Sciences↗

DOE OSTI2023

Analysis of the MUSIC 3 He Multiplicity Data

A measurement campaign called the Measurement of Uranium Subcritical and Critical (MUSiC) was performed on a range of configurations of highly-enriched uranium (HEU) from December 2020 through April of 2021. While part of the focus was to measure reactor kinetics parameters on delayed supercritical systems, an additional focus was performing neutron noise measurements on subcritical configurations from deeply subcritical to nearly delayed critical. Multiple detector systems were used to perform these measurements, such as a 3 He multiplicity detector called the Neutron Multiplicity Array Detector (NoMAD) and a liquid scintillator system called the Rossi-α Measurement Rapid Organic Discriminating Detector (RAM-RODD). Also included were a scintillator system from the University of Michigan and a set of small 3He tubes that have previously been used to measure Rossi-α values on near-critical systems. The focus of this paper will be a comparison of prospective analysis methods for the NoMAD measurements. Previous subcritical measurements at the National Criticality Experiments Research Center (NCERC) submitted to the International Criticality Safety Benchmark Evaluation Project (ICSBEP) used the Hage-Cifarelli formalism of the Feynman Variance-to-Mean method. This relies on the time correlations of neutron detections to infer the spontaneous fission rate and neutron multiplication of a system through binning the time tagged detections and analyzing resulting histograms of the numbers of counts. However, there are other neutron noise methods that rely on similar processes, such as the Hansen-Dowdy formalism which uses a slightly different methodology to extract multiplication from the neutron multiplicity counting moments. Comparisons can be made between these experimental results and those obtained through simulations to validate or identify deficiencies in analysis, detection methods, or the underlying nuclear data. Different time gating strategies and their effects on count rate uncertainties are also investigated.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2023

Wind Loading on Parabolic Trough Collectors: Wind and Structural Loads Measurements at an Operational Powerplant

Concentrated Solar Power (CSP) is a promising method for using solar power for electricity generation with thermal energy storage for industrial applications. Solar collectors constitute almost 1/3 of the total cost of the power plant. One of the primary drivers of unrealiability of these collectors is wind-driven loading of mirrors, support structures, and drives. To date, the design of the solar collector structures has relied on data from wind tunnels that do not adequately capture the dynamic effects observed at scale. NREL initiated a field measurement campaign at the operational Nevada Solar One (NSO) parabolic trough powerplant. At this plant, parabolic trough solar collectors track the sun from east to west in the course of a day and face varying wind loads depending on the wind properties and the angle of the troughs. The aim of the project is a detailed characterization of prevailing wind and turbulence conditions and resulting operational loads on parabolic troughs, providing insights into structural dynamic response, and generating a comprehensive wind-loading dataset for validating simulations of wind loading on collector structures. The measurements at NSO consist of sonic anemometers on masts at different heights to characterize the incoming flow and conditions at four trough rows at the edge of the trough field. In addition, a Doppler Lidar scans the horizontal plane above the troughs. The wind measurements at NSO have been continuously collecting data since October 2021 and are combined with structural load measurements that started in November 2022. The load measurements were installed on the same four outermost trough rows and include support structure bending moments, drive torque moments, dynamic accelerations of the spaceframe, mirror displacement, and tilt angles. Measurements are planned to continue until May 2023, providing a first-of-a-kind, high-resolution multi-month dataset of combined wind and load measurements. In this presentation, we show first results of the measurement campaign. Based on the measurements, we identified three main factors altering the flow over the parabolic troughs: Wind speed, wind direction, and the angle of the parabolic troughs. Most interactions between incoming wind and the trough field are observed when the wind blows perpendicular to the trough rows. In this case, the first rows experience the highest wind speed and block the downwind rows, creating conditions with decreased wind speed and enhanced turbulence within the trough field. Also, turbulent length scales are smaller after the first row. This leads to the highest static loads (bending and torque moments) at the first row but potentially increased dynamic loads within the field. We illustrate our findings with case studies focused on different wind conditions and will present fatigue analysis to highlight the impact of wind-driven loads on collector structures.

CSP collectors↗

DOE OSTI2023

Methane Emissions Produced by Pneumatic Devices and Produced Water Tanks on Natural Gas Wellsites

In recent years, more scrutiny has been placed on the release of greenhouse gasses (GHGs) by the oil and gas industry in North America as climate concerns increase. In the coming years, stricter regulations proposed by the Environmental Protection Agency (EPA) concerning the release of GHGs will further direct attention to GHG emissions quantification, modeling, and overall reduction. Active natural gas wellsites employ production equipment that routinely emits methane during normal operation. Production equipment often includes, but is not limited to, gas production units (GPUs), pneumatic controllers (PCs) and actuators powered by produced natural gas, and produced water storage tanks. This work details direct methane emission measurements taken at active natural gas wellsites originating from intermittent pneumatic controllers and produced water storage tanks. Efforts to model methane flows originating from these sources are also detailed, and those results are compared to direct measurement. The direct methane emissions measurement campaign collected flow data from two active dry wellsites in the Marcellus shale region. These measurement campaigns captured, in total, several weeks of continuous data from these sites. Data included multiple pneumatic device vent flowrate channels, a single channel monitoring total emissions vented from the produced water storage tanks, and corresponding site weather data. Periodic composition measurements were taken from flows vented from produced water tanks. Computational modeling efforts attempted to mimic a given site’s methane emissions behavior given limited input parameters. Direct measurement data and simulation data yielded, through reduction and analysis, apparent methane emissions factors, statistics on pneumatic device actuation events, important relationships between GPU parameters and pneumatic device actuation events, produced water storage tank vent flows and flow compositions, and parameters most contributing to the magnitude and frequency of these fugitive methane emissions. Measurements, considering data from a 72hr period, produced PC emissions factors from 0.008 to 0.03 SCFH per device with an average device emitting 0.026 SCFH at the first site. The second site produced PC emissions factors spanning from 0.05 to 25.47 SCFH with an average device emitting 1.93 SCFH not including the 25.47 SCFH device, which was assumed to be malfunctioning. Two unique water tank emission measurements were made, 618 g CH4 per hour and 32.6 g CH4 per hour. On a water basis, the water tank emissions factors were 0.66 and 0.042 kg CH4 per bbl of water, respectively.

03 NATURAL GAS↗

DOE OSTI2023

NCERC Provides Unique Opportunities for University Student Researchers

Five students and one faculty member - sponsored by the Defense Nuclear Nonproliferation (DNN, NA 22) university consortia - visited the National Criticality Experiments Research Center (NCERC) in July of 2023 to measure radiation signatures from Category I Special Nuclear Material (SNM) in a week-long measurement campaign organized by staff at Los Alamos National Laboratory. Participants included University of Florida, University of Michigan, and University of Illinois-Champaign Urbana. The measurement campaign was organized on behalf of the Consortium for Monitoring, Testing, and Verification (MTV), the Nuclear Science and Security Consortium (NSSC), and the Consortium for Enabling Technologies and Innovation (ETI).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2024

An Experimental Setup for Mechanical Vibration Analysis Using VLC

This study explores the potential applications across various domains, including earthquake detection and warning systems, where the system’s sensitivity to ground vibrations can contribute to early seismic event detection. Additionally, the study paves the way of developing applications of VLC/T in mechanical vibration and stability analysis of engines and platforms, offering insights into structural integrity and performance optimization. These multifaceted applications underscore the adaptability and potential of VLC/T systems in diverse fields, heralding advancements in sensing, communication, and security technologies. To achieve this, in this study, Peak to Average Power Ratio (PAPR) is proposed to represent the impact of mechanical shocks and vibrations generated by several weights dropped onto the platform with which the receiver is fixed. Even though non-contact measurement methodology is preferred for various reasons, the proposed measurement campaign obtains the data in contact form; however, the system and signal model proposed in this study could easily be extended into non-contact form. Considering the fact that the proposed measurement campaign employs off-the-shelf products, it is cost-effective and very scalable.

Yilmaz, Ahmet Mucahit↗

DOE OSTI2021

UNH TDP - Concurrent Measurements of Inflow, Power Performance, and Loads for a Grid-Synchronized Vertical Axis Cross-Flow Turbine Operating in a Tidal Estuary

This data was collected between October 12 and December 15 of 2021 at the University of New Hampshire (UNH) and Atlantic Marine Energy Center (AMEC) turbine deployment platform (TDP). This data set includes over 29 days of grid connected turbine operation during this 65 day time frame. The priority for this measurement campaign was to collect data while the turbine was electrically connected to the grid by means of a rectifier and inverter. The Fall_2021_UNH_Measurement_Timeline.png highlights when each instrument was functioning and the Fall_2021_UNH_Test_Log.jpg indicates the four main regions for analysis available from this measurement campaign. The TDP is a floating structure moored on the Portsmouth facing side of Memorial Bridge pier #2, which spans the Piscataqua River between Portsmouth, NH and Kittery, ME. The Piscataqua River connects the Great Bay Estuary to the Gulf of Maine and the river currents are dominated by tidal forcing with water velocities exceeding 2.5 m/s during spring ebb tides at this site which were previously characterized by Kaelin Chancey (Assessment Of The Localized Flow And Tidal Energy Conversion System At An Estuarine Bridge - UNH MS Thesis 2019). The turbine under test was a modified New Energy Corporation (Calgary, CA) model EVG-025 4-blade H-Darrius type vertical axis cross flow turbine that rotates in the clockwise direction with a rotor diameter of 3.2m and blade length of 1.7m. The hydro-foil profile was a NACA 0021 with a 10 inch chord length and a blade preset pitch angle of +4deg with a positive angle corresponding with the toe in direction. The standard EVG-025 has a rotor diameter of 3.4m and its rated power output is 25kW at 3 m/s. The rotor diameter was reduced to accommodate the size of the existing TDP moon-pool. This project was pursued to quantify device performance for cross flow turbines operating in a marine environment. Accurate physical models, to characterize cross flow turbine performance, require real operational data sets due to the complexity of blade fluid interactions. This data can help support model development which will help predict turbine performance when analyzing perspective project locations in the future. Instrumentation was deployed to measure; water speed/direction, electrical power output, turbine shaft speed, turbine thrust force, and platform motion. Concurrent measurements of these parameters allow for correlations (cause and affect) to be inferred, allowing for characterization of device performance over a range of operating conditions. Water currents were measured using Acoustic Doppler Current Profilers (ADCP's) and Acoustic Doppler Velocimeters (ADV's) directly upstream and downstream of the turbine for inflow, wake and turbulence measurements. Electrical power output was measured using the Voltsys rectifier and the Shark power meter. Shaft speed was calculated based on the Voltsys measurements of the permanent magnet three phase generator AC generation frequency, coupled directly to the cross flow turbine under test (i.e., no gear box). Platform motions were captured using a Yost IMU (inertial measurement unit). Turbine thrust loading was measured using a reaction arm about the turbine deployment platform spanning beam, where two bi-directional load cells were connected to the system via a pinned connection. This submission includes zipped folders for each instrument containing quality controlled (QC'd) data in daily .csv files for the relevant duration specific to each instrument, along with separate .csv file that contains the units for each variable. Some instrument daily files are quite large and can pose a challenge for a visual spreadsheet editor to open. A processing software like MATLAB or Python is recommended. Note the degree of QC varied between each instrument due to time constraints. Particular time and attention was given to perform quality control tests on the acoustic based instruments that are particularly suscep...

16 TIDAL AND WAVE POWER↗

DOE OSTI2023

In Situ Wind and Turbulence Measurements in a Field of Full-Size Parabolic Trough Solar Collectors

Concentrated Solar Power (CSP) is a promising method for using Solar power for electricity generation with thermal energy storage. One of the primary drivers of structural design costs of CSP collector structures is wind loading. To date, the design of these structures has relied on data from wind tunnels that do not adequately capture the dynamic effects observed at scale. NREL initiated a field measurement campaign at the operational Nevada Solar One (NSO) powerplant that uses parabolic troughs as solar collectors. The aim of the project is a detailed characterization of prevailing wind and turbulence conditions and resulting operational loads on parabolic troughs, providing insights on structural dynamic response, and generating a first-of-a-kind, comprehensive, high-resolution wind-loading dataset available for validating simulations of wind loading on collector structures. The measurements at NSO consist of Sonic anemometers on masts at different heights to characterize the incoming flow and conditions within and above the trough field, in combination with a Doppler Lidar scanning the horizontal plane above the troughs. The wind measurements at NSO have been continuously operating since October 2021 and provide a year-long dataset characterizing wind and turbulence conditions. The structural load measurements start in November 2022 and will complement the wind measurements. In this poster, we present first results of the wind measurement campaign by highlighting days with different atmospheric flow conditions. We identified three main factors altering the flow over the parabolic troughs: Wind speed, wind direction, and the angle of the parabolic troughs. The highest loads are expected when the wind blows perpendicular to the trough rows. In this case, the first rows experience the highest loads and block the subsequent rows, creating conditions with decreased wind speed and enhanced turbulence within the trough field. Also, turbulent length scales change. These affected conditions produce unique load cases on the structures that will be captured by the load measurements. If the wind blows along the trough rows, wind and turbulence conditions are less influenced by the troughs.

atmospheric turbulence↗

DOE OSTI2023

In Situ Wind and Turbulence Measurements in a Field of Full-Size Parabolic Trough Collectors

Concentrated Solar Power (CSP) is a promising method for using Solar power for electricity generation with thermal energy storage. One of the primary drivers of structural design costs of CSP collector structures is wind loading. To date, the design of these structures has relied on data from wind tunnels that do not adequately capture the dynamic effects observed at scale. NREL initiated a field measurement campaign at the operational Nevada Solar One (NSO) powerplant that uses parabolic troughs as solar collectors. The aim of the project is a detailed characterization of prevailing wind and turbulence conditions and resulting operational loads on parabolic troughs, providing insights on structural dynamic response, and generating a first-of-a-kind, comprehensive, high-resolution wind-loading dataset available for validating simulations of wind loading on collector structures. The measurements at NSO consist of Sonic anemometers on masts at different heights to characterize the incoming flow and conditions within and above the trough field, in combination with a Doppler Lidar scanning the horizontal plane above the troughs. The wind measurements at NSO have been continuously operating since October 2021 and provide a year-long dataset characterizing wind and turbulence conditions. The structural load measurements start in November 2022 and will complement the wind measurements. In this poster, we present first results of the wind measurement campaign by highlighting days with different atmospheric flow conditions. We identified three main factors altering the flow over the parabolic troughs: Wind speed, wind direction, and the angle of the parabolic troughs. The highest loads are expected when the wind blows perpendicular to the trough rows. In this case, the first rows experience the highest loads and block the subsequent rows, creating conditions with decreased wind speed and enhanced turbulence within the trough field. Also, turbulent length scales change. These affected conditions produce unique load cases on the structures that will be captured by the load measurements. If the wind blows along the trough rows, wind and turbulence conditions are less influenced by the troughs.

concentrated solar power↗

DOE OSTI2025

Tidal energy resource characterization measurements at Cook Inlet’s East Foreland: Velocity and turbulence

To characterize tidal current and turbulence at a top tidal energy site off the East Foreland in Cook Inlet, Alaska, United States, three moorings were deployed for two months between July and August 2021, and a transect survey was conducted over the course of two tidal cycles at the end of the deployment period. Measurements of velocity and turbulence were then analyzed to better understand the site's hydrodynamics and power potential. Analysis reveals that swift, north-flowing flood currents peak at 4~m/s, while south-flowing ebb currents reach just over 3~m/s. Turbulence intensity ranges from 23\% at the seafloor to 8\% near the surface, and the presence of the foreland creates more intense turbulence near-shore during ebb tide than flood. Power availability at the site could be as high as 720~MW, or 13~kW/m$^2$, though the energy available to a marine energy device will be smaller than this estimate because of water-to-wire efficiency and wake losses. The results from this measurement campaign will inform the validation of a high-resolution tidal hydrodynamic model, as well as early tidal energy projects that are beginning to move beyond the prototyping and demonstration stages to full-scale deployments.

McVey, James R.↗

DOE OSTI2023

Simulation Study of Monoenergetic Photon Source LiDAR System Performance for Emergency Response Applications

The following report summarizes the results of a Monte Carlo simulation and modeling study of the Lawrence Berkeley National Laboratory’s (LBL) Monoenergetic Photon Source (MPS) as part of a high-energy LiDAR system for use in emergency response applications. A set of image quality indicators (IQI) and nonsensitive phantoms or generalized surrogates for search targets have been identified for use in the planned measurement campaign at the Berkeley Lab Laser Accelerator (BELLA) Center toward the end FY2023. These items were modeled and the time-of-flight (TOF) spectral responses following irradiation were calculated for a set of varying operating conditions. The goal of this study was to both predict the LiDAR system performance as well as determine if minor modifications to the IQI and phantom designs were required before fabrication. It was found that the IQI and target designs both overlap and extend towards the limit of performance of the system and are thus suitable for the final project measurement campaign.

43 - PARTICLE ACCELERATORS↗

DOE OSTI2025

Validation and demonstration of the AEFC as a practical safeguards tool for inventory verification

The Advanced Experimental Fuel Counter (AEFC) is a nondestructive assay (NDA) instrument designed to determine the residual fissile mass in irradiated fuel assemblies for safeguards verification purposes. This is done by actively interrogating an assembly with a neutron source and measuring the total (Singles) and correlated (Doubles) neutron count rates resulting from induced fissions in the irradiated nuclear fuel and relating those rates to the residual fissile mass using calibration curves. Comprehensive NDA measurements of the irradiated fuel inventory at Israeli Research Reactor 1 (IRR-1) were taken with the AEFC to validate a set of previously developed calibration curves. During the campaign, measurements were acquired of 32 standard fuel assemblies and three control assemblies in just nine days. This is a significant majority of the research reactor's irradiated fuel inventory and the largest data set gathered by the AEFC to date. Many of the fuel assemblies measured during the campaign had much shorter cooling times than those assemblies previously measured with the instrument. Calibration curves developed from previous AEFC deployments were used to determine the residual 235 U mass in the measured standard fuel assemblies. The results of the campaign demonstrated that the AEFC can be used to estimate the 235 U mass remaining in a large number of irradiated fuel assemblies with 1%–5% uncertainty in a reasonable amount of time despite operating in a high dose environment.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

DOE OSTI2020

Development of Gamma Background Radiation Digital Twin with Machine Learning Algorithms: Application of Unsupervised Machine Learning to Detection of Anomalies and Nuisances in Gamma Background Radiation Environmental Screening Data

Environmental screening of gamma radiation consists of detecting weak nuisance and anomaly signal in the presence of strong and highly varying background. In a typical scenario, a mobile detector-spectrometer continuously measures gamma radiation spectra in short, e.g., one-second, signal acquisition intervals. The measurement data is a 2D matrix, where one dimension is gamma ray energy, and the other dimension is the number of measurements or total time. In principle, gamma radiation sources can be detected and identified from the measured data by their unique spectral lines. Detecting sources from data measured in a search scenario is difficult due to the highly varying background because of naturally occurring radioactive material (NORM), and low signal-to-noise ratio (S/N) of spectral signal measured during one-second acquisition intervals. The objective of this work is to explore unsupervised machine learning (ML) algorithms for development of a digital twin of gamma radiation background, and for detection and identification of weak nuisances and anomalies events in the presence of highly fluctuating background. In one segment of work, we developed a gamma background estimation model using a Longshort term memory (LSTM) network for one-step CPS time series prediction. The LSTM model was validated with two data sets of measurements from two independent NaI detectors positioned on a mobile platform. The data sets contained background radiation only and no orphan isotope sources. The LSTM model was constructed and tested using data from one of the detectors. Performance of the LSTM model was validate through one-step prediction of CPS time series of another NaI detector without re-training. This approach allows to create a digital twin for nuclear background estimation. Using LSTM, it could be possible to detect a source through subtraction of the estimated counts from the measured background. In another segment of work, we investigated detection of gamma emitting sources in the presence of complex background using unsupervised machine learning. Spectral lines of isotopes are difficult to observe in one-second measurements. Averaging over the entire measurement campaign data set reveals spectral lines of most common background isotopes. Spectral lines of orphan sources, which might appear only in a few measurements during the campaign, will be washed out if averaging is performed over the entire measurement data set. The approach we have explored consists of extracting one-second measurements containing weak spectral features through data clustering. Averaging one-second spectra in a cluster should reveal the presence of anomaly sources. We created two ML models using K-means clustering and Neural Network Self-organizing Map (SOM). Performance of these ML models was benchmarked using search data. One data set contained 137 Cs source, and another dataset contained 131 I source.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Detection of Anomalies in Gamma Background Radiation Data with K-Means and Self-Organizing Map Clustering Algorithms (Consortium on Nuclear Security Technologies (CONNECT) Q1 Report)

Environmental screening of gamma radiation consists of detecting weak nuisance and anomaly signal in the presence of strong and highly varying background. In a typical scenario, a mobile detector-spectrometer continuously measures gamma radiation spectra in short, e.g., one-second, signal acquisition intervals. The measurement data is a 2D matrix, where one dimension is gamma ray energy, and the other dimension is the number of measurements or total time. In principle, gamma radiation sources can be detected and identified from the measured data by their unique spectral lines. Detecting sources from data measured in a search scenario is difficult due to the highly varying background because of naturally occurring radioactive material (NORM), and low signal-to-noise ratio (S/N) of spectral signal measured during one-second acquisition intervals. The objective of this work is to explore unsupervised machine learning (ML) algorithms for detection and identification of weak nuisances and anomalies events in the presence of highly fluctuating background. The challenge is that spectral lines of isotopes are difficult to observe in one-second measurements. Averaging over the entire measurement campaign data set reveals spectral lines of most common background isotopes. Spectral lines of orphan sources, which might appear only in a few measurements during the campaign, will be washed out if averaging is performed over the entire measurement data set. The approach we have explored consists of extracting one-second measurements containing weak spectral features through data clustering. Averaging one-second spectra in a cluster should reveal the presence of anomaly sources. We created two ML models using K-means clustering and Neural Network Self-organizing Map (SOM). Performance of these ML models was benchmarked using search data. One data set contained 137 Cs source, and another dataset contained 131 I source.

61 RADIATION PROTECTION AND DOSIMETRY↗

DOE OSTI2023

Empirical Bounding Analysis and User Recommendations for a Neutron Multiplicity Detector

Neutron multiplicity detectors are useful for a variety of applications including nuclear emergency response, nuclear nonproliferation, safeguards, and criticality safety. When measuring black-box problems (i.e., when the system being measured is completely unknown) with systems that have relatively low detection efficiency, expert analysis is frequently required to determine appropriate bounds for system parameters such as neutron multiplication and neutron leakage. This is because the detection efficiency can vary wildly, which also means that the resulting system parameters can have large variations. This work applies an empirical approach to provide bounds on system parameters (such as system multiplication, neutron leakage, and detector efficiency). The results of this bounding analysis are then used as inputs to provide recommendations to users regarding criticality safety. In addition to describing the method used, this work provides sample results from a measurement campaign performed at the National Criticality Experiments Research Center (NCERC).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2024

Uranium measurements in the field using high-resolution cadmium zinc telluride detectors

A new generation of cadmium zinc telluride (CZT) detectors has become available and is being evaluated by the International Atomic Energy Agency (IAEA) for safeguards verifications in the field. The new CZT detector, model M400, is a room temperature spectrometer manufactured by H3D, Inc. The M400 demonstrates superior energy resolution, effective isotope identification capabilities, and convenient usability features when tested in a controlled laboratory environment. These characteristics define the M400 as a potential platform for IAEA field detection applications, which could become suitable for nuclear material characterization (e.g., enrichment verification) and nuclear safeguards missions. The capabilities of gamma spectrometry codes including Fixed energy, Response function Analysis with Multiple efficiencies (FRAM) from Los Alamos National Laboratory, CZT for Uranium (CZTU) from Lawrence Livermore National Laboratory, and Gamma Detector Response and Analysis Software (GADRAS) from Sandia National Laboratories were adapted for M400 spectra, and the performance of the codes has been validated. This was reported in a prior work. To further validate the performance of the high-energy resolution CZT detector and the isotopic analysis codes, a field measurement campaign consisting of uranium hexafluoride (UF 6 ) cylinder measurements was conducted at a fuel fabrication facility. A total of 34 Type 30B cylinders containing UF6 were measured using three different M400 CZT detectors. Each detector was outfitted with a custom rectangular collimator and shield made out T-Flex®, a tungsten-impregnated polymer. Measurements were performed at three different locations of the cylinder, ensuring that the measurement geometry satisfied the infinite thickness criterion. The spectra from the M400 CZT were analyzed using the code General Enrichment Meter (GEM). For analyzing the gamma-ray spectra from UF 6 cylinder, the GEM code is the appropriate tool since it relies only on the gamma-ray emissions from 235 U and not from other isotopes. Results from the spectral analysis were compared with the known abundance of 235 U in the cylinders, as well as with the International Target Values 2020 (ITV2020). The suitability of the different underlying techniques used by the various codes for UF 6 analysis is discussed. The challenges of measuring UF 6 contained in cylinders and mitigation strategies are highlighted.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗